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Reactive Thin Film Polymers And Thin Film Composite Membranes For The Rapid Screening Of Uranium Isotopes, Abenazer W. Darge 2022 Clemson University

Reactive Thin Film Polymers And Thin Film Composite Membranes For The Rapid Screening Of Uranium Isotopes, Abenazer W. Darge

All Dissertations

Traditional radiochemistry approaches for the detection of trace-level alpha-emitting radioisotopes in water require lengthy offsite sample preparations and do not lend themselves to rapid quantification. Therefore, a novel platform is needed that combines onsite purification, concentration, and isotopic screening with a fieldable detection system. My dissertation research objective was to develop novel reactive thin polymer films and thin film composite membranes for the selective separation of uranium from environmental water followed by direct isotopic analysis by alpha spectroscopy. Chapter 1 reviews progress made on uranium separation from aqueous matrices and discusses methods used for the determination of isotopic composition.

Chapter …


Viability Of Energy And Fuel Sources For Interstellar Travel; Design And Feasibility Of The Construction Of Manned Interstellar Space Shuttles, Lukas Mittelman 2022 University of Nevada, Las Vegas

Viability Of Energy And Fuel Sources For Interstellar Travel; Design And Feasibility Of The Construction Of Manned Interstellar Space Shuttles, Lukas Mittelman

UNLV Theses, Dissertations, Professional Papers, and Capstones

The importance of proving the viability of interstellar transport and addressing its potential hazards and pitfalls is immense. If we do not look toward the future and examine what could be waiting for us, we are doing our children, our children’s children, and so on, a disservice. Here we must attempt to lay the groundwork for our future scientists, engineers, and adventurers. Asking and answering questions like, which propulsion and energy systems must we incorporate to send us through the cosmos? Will we utilize technologies known today, such as fossil fuel rockets, fission or fusion rockets, and antimatter drives (pion …


Electrochemical Impedance Spectroscopy Of Zirconium Oxidation For In-Situ Nuclear Sensing Applications, Michael Andrew Reynolds 2022 Boise State University

Electrochemical Impedance Spectroscopy Of Zirconium Oxidation For In-Situ Nuclear Sensing Applications, Michael Andrew Reynolds

Boise State University Theses and Dissertations

To meet the ever-growing energy demands of the modern world, alternative forms of producing power are necessary, and the field of nuclear engineering holds promise to answer this call. Nuclear fuel cladding in light water reactors (LWRs) currently draws a large amount of attention from scientists and researchers, as it provides many challenges to design around. Since the 1950s, zirconium and its protective oxide layer have been utilized as an effective material for the task, possessing good mechanical strengths, high corrosion resistance, and a low neutron absorption cross section. Despite these beneficial properties, however, fuel cladding remains vulnerable to several …


Towards Improving The Properties And Furthering Acceptance Of Advanced Technology Nuclear Fuels, Jennifer K. Watkins 2022 Boise State University

Towards Improving The Properties And Furthering Acceptance Of Advanced Technology Nuclear Fuels, Jennifer K. Watkins

Boise State University Theses and Dissertations

To avoid detrimental environmental impacts from climate change, the world community needs to push for the use of clean energy technologies. Development of proposed advanced technology nuclear fuels supports efforts to ensure nuclear energy is included as a non-carbon emitting source of electricity generation. Advanced technology nuclear fuels, also referred to as accident tolerant fuels (ATFs), have received renewed interest for use in the current nuclear reactor fleet as well as in advanced reactor technologies due to their high uranium loading, desirable thermophysical properties, and performance under irradiation as compared to the benchmark oxide fuel. A limiting consideration for the …


Wetland Uranium Transport Via Iron-Organic Matter Flocs And Hyporheic Exchange, Connor J. Parker 2022 Clemson University

Wetland Uranium Transport Via Iron-Organic Matter Flocs And Hyporheic Exchange, Connor J. Parker

All Dissertations

Uranium (U) released from the M-Area at the Department of Energy Savannah River Site into Tims Branch, a seasonal wetland and braided stream system, is estimated to be 43,500 kg between 1965 and 1984. The motivation for this work is the uranium’s persistence in the wetland for decades, where it is estimated that 80% of the U currently remains in the Tims Branch wetland. U has begun to incorporate into wetland iron (Fe) and carbon cycles, associating with local Fe mineralogy and deposits of rich wetland organic matter (OM). The objective of this work is to characterize the chemical phases …


Experimental Investigations On Boiling Heat Transfer Characteristics Of Accident-Tolerant-Fuel And Traditional Claddings, Mingfu He Mr. 2022 Department of Nuclear Engineering UNM

Experimental Investigations On Boiling Heat Transfer Characteristics Of Accident-Tolerant-Fuel And Traditional Claddings, Mingfu He Mr.

Nuclear Engineering ETDs

To make it more clear that how the materials’ thermal-physical properties and wall thickness have influential impacts on boiling heat transfer characteristics of cladding, this dissertation looks into the potential impacts of cladding materials on critical heat flux and heat transfer coefficients by a systematic experimental investigation across a wide range of pool/flow boiling conditions under the steady-state and power-transient heat inputs.

Recent thermal-hydraulics studies have demonstrated that iron-chromium-aluminium (FeCrAl) alloys have the thermal priorities over zircaloys and other commercial alloys including critical heat flux and heat transfer coefficient. However, it is found in our experimental results that FeCrAl-C26M, and …


Utilizing Sensitivity And Correlation Coefficients From Mcnp And Whisper To Guide Microreactor Experiment Design, Alexis Maldonado 2022 The University of New Mexico

Utilizing Sensitivity And Correlation Coefficients From Mcnp And Whisper To Guide Microreactor Experiment Design, Alexis Maldonado

Nuclear Engineering ETDs

When designing experiments for full-scale reactor systems, MCNP and Whisper can be used to create neutronic models and compare the similarity of two nuclear systems via correlation coefficients for 𝑘𝑒𝑓𝑓, effective multiplication factor. This thesis applies this framework to a conceptual heat-pipe, yttrium-hydride moderated microreactor system and experiments. The framework is intended as a supplement to other neutronics/thermal/multiphysics analyses and provides a concrete method to measure the neutronic similarity of two systems. By analyzing the shared nuclear data uncertainty, as well as sensitivity to nuclear data over all neutron energies, highly informative experiments can be designed to aid in the …


Thermal-Hydraulic System Analysis Of A Proposed 1 Mwth Nuclear Gas Cooled Microreactor, Aaron S. Fernandez 2022 University of South Carolina

Thermal-Hydraulic System Analysis Of A Proposed 1 Mwth Nuclear Gas Cooled Microreactor, Aaron S. Fernandez

Theses and Dissertations

Nuclear power plants have historically been large, expensive, and prolonged construction projects. A new generation of reactors categorized as microreactors is currently being designed to address energy needs in remote locations. The University of South Carolina has proposed the MIcro Nuclear In ONe megawatt (MINION-1) design to achieve ten years of operation. The primary loop transfers 1 MW of energy from the reactor core using helium, while the secondary uses air in an open Brayton cycle to produce power and heat. This work focuses on modeling the MINION-1 design using the System Analysis Module (SAM) developed by Argonne National Labs …


Mechanistic Multiphysics Modeling Of Cladding Rupture In Nuclear Fuel Rods During Loss-Of-Coolant Accident Conditions, Kyle Allan Lawrence Gamble 2022 University of South Carolina

Mechanistic Multiphysics Modeling Of Cladding Rupture In Nuclear Fuel Rods During Loss-Of-Coolant Accident Conditions, Kyle Allan Lawrence Gamble

Theses and Dissertations

The Loss of Coolant Accident (LOCA) is a design basis accident that is included as part of the safety analysis of nuclear power plants. As the nuclear industry desires to increase the cycle length and discharge burnup of existing nuclear power plants they must demonstrate safe operation during a LOCA on high burnup fuel. During a LOCA transient on high burnup fuel rods, the rods may undergo a process known as fuel fragmentation, relocation, and dispersal (FFRD). To permit dispersal, the cladding encapsulating the fuel must rupture with an opening size large enough to allow the fragmented fuel particles to …


Aerial Radiation Detection Identification And Measurement System Detector Material Comparison Study, Benjamin C. Troxell, Kacey D. McGee, Christina L. Dugan 2022 20th CBRNE Command

Aerial Radiation Detection Identification And Measurement System Detector Material Comparison Study, Benjamin C. Troxell, Kacey D. Mcgee, Christina L. Dugan

Faculty Publications

The 20th Chemical Biological Radiological Nuclear and Explosives Command (CBRNE) currently utilizes an airborne sodium iodide gamma and beta detection system to map radiation fields over large areas of interest. The 20th CBRNE explored emergent detector technologies utilizing two detection materials; thallium-activated cesium iodide and high purity germanium (HPGe). These detectors were simulated at various altitudes and compared to background measurements. The sodium iodide detector failed to provide isotopic discrimination at distance. The thallium-activated cesium iodide CsI(Tl) detector provided sufficient absolute efficiency and energy resolution to identify isotopics at distance. The HPGe detector provided the best energy resolution. However, current …


Capability Development For Advanced (N,X) Nuclear Data Measurements, Brian G. Frandsen 2022 Air Force Institute of Technology

Capability Development For Advanced (N,X) Nuclear Data Measurements, Brian G. Frandsen

Theses and Dissertations

Nuclear reaction data are the heart of radiation transport calculations, models, and simulations. Unique approaches are required to improve the measurement capability for many reactions where data are inaccurate or do not exist. First, the newly developed Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) provides the ability to measure neutron inelastic scattering cross sections on different targets. An initial experiment measuring the 16O(n,n’��) reaction calculated the count rate from the second excited state using the full energy and escape peaks. Second, a set of photocurable scintillator resin formulations capable of neutron-gamma discrimination were developed to support light-based …


Verficiation And Validation Of Unstructured Meshing Capabilities In Mcnp6, Micah C. Jeroutek 2022 Air Force Institute of Technology

Verficiation And Validation Of Unstructured Meshing Capabilities In Mcnp6, Micah C. Jeroutek

Theses and Dissertations

Discrepancies were found between the legacy CSGs and the new UMs with the latter's introduction in MCNP6. As such, V&V of UMs in MCNP must be conducted to assist in their further development and increase user confidence in them. Currently, the MCNP test suite is lacking in UM benchmarks, and of the few that are present, their range in problem type is limited. To address these issues, two preliminary test cases covering new applications of UMs were developed for future inclusion in the test suite. The first was for the Athena-I experiment which involved the study of electronic devices' responses …


Modeling Gadolinium Self Powered Neutron Detectors In A Transient Reactor, Alexander L. Q. Spring 2022 Air Force Institute of Technology

Modeling Gadolinium Self Powered Neutron Detectors In A Transient Reactor, Alexander L. Q. Spring

Theses and Dissertations

Contributions to the electron current from the three components of a gadolinium SPND, emitter, insulator, and sheath, are identified, characterized, and quantified to provide information on how the SPND interacts within the transient neutron and photon flux of the TREAT to create a measurable current. These contributions are measured by defining the SPND interactions as a dose response function used within a Monte Carlo simulation of a TREAT experiment. The data obtained from the Monte Carlo simulations are then used to compare against two analytic models, developed by Jaschik and Warren, as well as the experimental results. It was found …


Deep Learning Approach To Multi-Phenomenological Nuclear Fuel Cycle Signals For Nonproliferation Applications, Preston J. Dicks 2022 Air Force Institute of Technology

Deep Learning Approach To Multi-Phenomenological Nuclear Fuel Cycle Signals For Nonproliferation Applications, Preston J. Dicks

Theses and Dissertations

In order to reduce the time required for data analysis and decision-making relevant to nuclear proliferation detection, Artificial Intelligence (AI) techniques are applied to multi-phenomenological signals emitted from nuclear fuel cycle facilities to identify non-human readable characteristic signatures of operations for use in detecting proliferation activities. Seismic and magnetic emanations were collected in the vicinity of the High Flux Isotope Reactor (HFIR) and the McClellan Nuclear Research Center (MNRC). A novel bi-phenomenology DL network is designed to test the viability of transfer learning between nuclear reactor facilities. It is found that the network produces an 84.1% accuracy (99.4% without transient …


Optimization Of A Multi-Layered Target For A Pulsed Power Neutron Source, Zachary D. Bretz 2022 Air Force Institute of Technology

Optimization Of A Multi-Layered Target For A Pulsed Power Neutron Source, Zachary D. Bretz

Theses and Dissertations

The ability to create neutron environments is critical fora wide variety of applications including national security, materials science, and medical research. It is also helpful in medical, material, and other research. The U.S. Naval Research Laboratory (NRL), Washington, DC, is interested in leveraging their pulsed-power facilities to produce an in-house, relatively inexpensive neutron source. NRL’s facilities produce 2 MeV (from Gamble II) and 5 MeV (from Mercury) protons and deuterons. This research explored combinations of target materials to produce the most neutrons in the forward direction. Models of the reactions involved were first validated against literature experiments, then target designs …


Feasibility Of Fireball Trail Detection Using Ground-Based Gps Receivers, Ian R. Moffett 2022 Air Force Institute of Technology

Feasibility Of Fireball Trail Detection Using Ground-Based Gps Receivers, Ian R. Moffett

Theses and Dissertations

The feasibility of using GPS data to detect fireballs is analyzed by first modeling the fireball’s trail diffusion and plasma chemistry to get a resulting ion density profile of the trail over time. The signal perturbation caused by the fireball trail is simulated for a ground receiver using an analytic solution for diffraction from a Gaussian lens. Five cases were modeled with varying initial peak ion densities and altitudes taken from fireball and reentry vehicle data. This paper shows that it is feasible to detect a fireball trail using GPS if the fireball has a sufficiently high initial ion density, …


Neutron Spectral Effect On Microelectronic Performance Response, Wade Kloppenburg 2022 Air Force Institute of Technology

Neutron Spectral Effect On Microelectronic Performance Response, Wade Kloppenburg

Theses and Dissertations

Response of 2N2222 bipolar junction transistors to neutrons from a pulsed thermonuclear or pulsed fission source are researched. Measurements used for comparing performance included the base-collector junction current-voltage and capacitance-voltage characteristics and device gain degradation. Little change was detected in steady-state operation of the base-collector junction, but evidence in the dynamic and capacitance measurements establish effects based on environment. Experimental results are compared to literature results and parameters are explored using a device model simulation code.


Analysis Of Microscopic Carbon Fiber Fragments, Zachary R. Scott 2022 Air Force Institute of Technology

Analysis Of Microscopic Carbon Fiber Fragments, Zachary R. Scott

Theses and Dissertations

Carbon Fiber (CF) has different tensile strengths and transverse moduli depending on how they are fabricated. Some CF is export controlled as it can be used for weapons, spacecraft, or gas centrifuges for enriching nuclear fuel. This research project explored a new way to prepare micron sized single CF threads to measure their transverse modulus and compare the moduli of non-export controlled CF to that of an export controlled CF. Five total polyacrylonitrile (PAN) fibers were used in this project, one of which was an export controlled fiber.


Addressing Underground, Unmanned Threats: A Case Study Of Gpr Detecting Illegal Objects At Nuclear Facilities And Enhancing Subterranean Physical Protection Systems, Md. Shamsul Huda Sohel, Mohammad Khan, Dr. Debashis Datta 2022 University of Dhaka

Addressing Underground, Unmanned Threats: A Case Study Of Gpr Detecting Illegal Objects At Nuclear Facilities And Enhancing Subterranean Physical Protection Systems, Md. Shamsul Huda Sohel, Mohammad Khan, Dr. Debashis Datta

International Journal of Nuclear Security

In nuclear installations, any unmanned threat is unacceptable. Such threats are a major issue for the nuclear physical protection system (PPS). Although the PPS of a nuclear power plant (NPP) is well prepared to deal with threats above ground level, until now, a special PPS had never been developed for detecting and tackling underground threats. One example of such a threat is a weapon-carrying, unmanned object operated by remote. Using this technology, a terrorist could launch an attack and overcome security barriers. While a normal PPS would not detect the underground activities of a mobile object, a PPS using a …


A Detailed Hydrodynamic Study Of The Split-Plate Airlift Reactor By Using Non-Invasive Gamma-Ray Techniques, Laith S. Sabri, Abbas J. Sultan, Hasan Shakir Majdi, Shadha K. Jebur, Muthanna H. Al-Dahhan 2022 Missouri University of Science and Technology

A Detailed Hydrodynamic Study Of The Split-Plate Airlift Reactor By Using Non-Invasive Gamma-Ray Techniques, Laith S. Sabri, Abbas J. Sultan, Hasan Shakir Majdi, Shadha K. Jebur, Muthanna H. Al-Dahhan

Chemical and Biochemical Engineering Faculty Research & Creative Works

This study focused on detailed investigations of selected local hydrodynamics in split airlift reactor by using an unconventional measurements facility: computed tomography (CT) and radioactive particle tracking (RPT). The local distribution in a cross-sectional manner with its radial's profiles for gas holdup, liquid velocity flow field, shear stresses, and turbulent kinetic energy were studied under various gas velocity 1, 2 and 3 cm/s with various six axial level z = 12, 20, 40, 60, 90 and 112 cm. The distribution in gas-liquid phases in the whole split reactor column, the riser and downcomer sides, including their behavior at the top …


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