Optics Commons^™

Vibration Overtone Hyperpolarizability Measured For H2 Using Electric Field Induced Second Harmonic Generation, Rachel Ellis

UNLV Theses, Dissertations, Professional Papers, and Capstones

The vibrational contribution to the second hyperpolarizability (γ) of gas phase H2 was measured using electric field induced second harmonic generation. Measurements were made for the pure vibrational 3-0 Q(J) overtone transitions (v=0,J → v’=3,J for J = 0,1,2,3). Measured intensities were found to be 4-14% larger than ab initio calculations. The first chapter of this thesis provides an introduction to nonlinear optics, second harmonic generation, and the tensor nature of hyperpolarizabilities. The second chapter provides theoretical expressions for γ and relevant static and Raman polarizabilities. The third chapter covers the experimental design and electric field induced second harmonic generation. …

2 × 2 Anisotropic Transfer Matrix Approach For Optical Propagation In Uniaxial Transmission Filter Structures, Hammid Al-Ghezi, Rudra Gnawali, Partha P. Banerjee, Lirong Sun, Jonathan E. Slagle, Dean Evans

Student Publications

Multi-layered metamaterial structures show promise in a wide variety of optical applications such as superlenses, electromagnetic cloaking, tunable filters, sensors, and spatial light modulators. Optical transmission analysis of multilayer metallo-dielectric stacks with overall thickness less than the wavelength of light can be modeled using effective medium theory and the Berreman matrix method. For multilayer anisotropic stacks of arbitrary thickness, a rigorous 4 × 4 transfer matrix embodiment is typically used. In this work, a 2 × 2 anisotropic transfer matrix method is developed to analyze optical propagation through multilayer uniaxial stacks of arbitrary thicknesses. Optical transmission of a multilayer silver–zinc …

Atmospheric Turbulence Study With Deep Machine Learning Of Intensity Scintillation Patterns, Artem V. Vorontsov, Mikhail A. Vorontsov, Grigorii A. Fillimonov, Ernst Polnau

Electro-Optics and Photonics Faculty Publications

A new paradigm for machine learning-inspired atmospheric turbulence sensing is developed and applied to predict the atmospheric turbulence refractive index structure parameter using deep neural network (DNN)-based processing of short-exposure laser beam intensity scintillation patterns obtained with both: experimental measurement trials conducted over a 7 km propagation path, and imitation of these trials using wave-optics numerical simulations. The developed DNN model was optimized and evaluated in a set of machine learning experiments. The results obtained demonstrate both good accuracy and high temporal resolution in sensing. The machine learning approach was also employed to challenge the validity of several eminent atmospheric …

Spontaneous Raman Scattering Enhancement With Microcavities And Multipass Resonators For Trace Gas Detection, Juan Sebastian Gomez Velez

USF Tampa Graduate Theses and Dissertations

The continual increase in production and use of chemicals in an ever-growing field of applications naturally brings forth the necessity to accurately and efficiently measure molecular composition. Spontaneous Raman scattering is a reliable technique which can optically identify molecules based on their intrinsic rotational-vibrational energy structure. The Raman emission from a substance can be spectrally analyzed to detect molecular species simultaneously and with isotopic sensitivity using a single laser source. However, even though the process is non-invasive and effective, the rate at which the emission occurs is notoriously low due to a weak scattering cross-section. Therefore, research into the development …

Enhancing The Visibility Of Vernier Effect In A Tri-Microfiber Coupler Fiber Loop Interferometer For Ultrasensitive Refractive Index And Temperature Sensing, Fangfang Wei, Dejun Liu, Zhe Wang, Zhuochen Wang, Gerald Farrell, Qiang Wu, Gang-Ding Peng, Yuliya Semenova

Articles

In this paper a Vernier effect based sensor is analyzed and demonstrated experimentally in a tri-microfiber coupler (Tri-MFC) and polarization-maintaining fiber (PMF) loop interferometer (Tri-MFC-PMF) to provide ultrasensitive refractive index and temperature sensing. The main novelty of this work is an analysis of parameters of the proposed Tri-MFC-PMF with the objective of determining the conditions leading to a strong Vernier effect. It has been identified by simulation that the Vernier effect is a primary factor in the design of Tri-MFC-PMF loop sensing structure for sensitivity enhancement. It is furthermore demonstrated experimentally that enhancing the visibility of the Vernier spectrum in …

A Coded Aperture Microscope For X-Ray Fluorescence Full-Field Imaging, D. P. Siddons, A. J. Kuczewski, A. K. Rumaiz, R. Tappero, M Idir, K. Nakhoda, J. Khanfri, V. Singh, E. R. Farquhar, M. Sullivan, D. Abel, D. J. Brady, X. Yuan

Faculty Publications

The design and construction of an instrument for full-field imaging of the X-ray fluorescence emitted by a fully illuminated sample are presented. The aim is to produce an X-ray microscope with a few micrometers spatial resolution, which does not need to scan the sample. Since the fluorescence from a spatially inhomogeneous sample may contain many fluorescence lines, the optic which will provide the magnification of the emissions must be achromatic, i.e. its optical properties must be energy-independent. The only optics which fulfill this requirement in the X-ray regime are mirrors and pinholes. The throughput of a simple pinhole is very …

Re-Examining The Radial Distributions Of M13 Multiple Populations, Jason P. Smolinski, Willem B. Hoogendam, Alex J. Van Kooten, Peyton Benac

University Faculty Publications and Creative Works

We seek to resolve the tension in the literature regarding the presence of radially segregated multiple populations in the Galactic globular cluster M13. Previous studies of this nearby cluster have presented discordant results about the degree of dynamical mixing in M13's inner region. Using ground-based (UBVI) photometry, we show that cumulative radial distributions of stars on the blue and red sides of the red giant branch are statistically identical. Interestingly, these results are obtained using data from large-aperture, ground-based telescopes as well as a more modestly sized instrument, and both are in agreement with previous work done using Hubble Space …

Generation Of Vector Partially Coherent Optical Sources Using Phase-Only Spatial Light Modulators, Milo W. Hyde Iv, Santasri R. Bose-Pillai

AFIT Patents

A vector partially coherent source (VPCS) generator includes a laser that emits coherent light; an interferometer consisting of polarizing beam splitters (PBSs) to split the laser light into its vertical and horizontal polarization components;] first and second spatial light modulators (SLMs) that respectively control the vertical and horizontal polarization components; and a control system communicatively coupled to the first and second SLMs to adjust beam shape and coherence without physically moving or removing optical elements in the interferometer.

Developing A Portable, Smartphone-Based Schlieren Imaging System, Grace Riermann, Keith R. Stein

Honors Student Works

Schlieren imaging is a technique for visualizing fluid flows that are characterized by spatial variations in density or refractive index. Because schlieren imaging is commonly performed with expensive equipment in a lab setting, we sought cost efficiency, accessibility, and ease of fabrication by designing a portable, smartphone-based system.

Single‐Molecule 3d Orientation Imaging Reveals Nanoscale Compositional Heterogeneity In Lipid Membranes, Jin Lu, Hesam Mazidi, Tianben Ding, Oumeng Zhang, Matthew D. Lew

Electrical & Systems Engineering Publications and Presentations

In soft matter, thermal energy causes molecules to continuously translate and rotate, even in crowded environments, thereby impacting the spatial organization and function of most molecular assemblies, such as lipid membranes. Directly measuring the orientation and spatial organization of large collections (>3000 molecules μm⁻²) of single molecules with nanoscale resolution remains elusive. In this paper, we utilize SMOLM, single‐molecule orientation localization microscopy, to directly measure the orientation spectra (3D orientation plus “wobble”) of lipophilic probes transiently bound to lipid membranes, revealing that Nile red's (NR) orientation spectra are extremely sensitive to membrane chemical composition. SMOLM images resolve …

Emulating Condensed Matter Systems In Classical Wave Metamaterials, Matthew Weiner

Dissertations, Theses, and Capstone Projects

One of the best tools we have for the edification of physics is the analogy. When we take our classical set of states and dynamical variables in phase space and treat them as vectors and Hermitian operators respectively in Hilbert space through the canonical quantization, we lose out on a lot of the intuition developed with the previous classical physics. With classical physics, through our own experiences and understanding of how systems should behave, we create easy-to-understand analogies: we compare the Bohr model of the atom to the motion of the planets, we compare electrical circuits to the flow of …

Control Of Molecular Energetics And Transport Via Strong Light-Matter Interaction, Rong Wu

Dissertations, Theses, and Capstone Projects

Strong light-matter coupling in excitonic systems results in the formation of half-light half-matter quasiparticles called exciton polaritons. These hybrid quasiparticles take on the best of both systems, namely, the long-range propagation and coherence arising from the photonic component and the nonlinear interaction from the excitonic component. We develop methods for making high quality factor cavities and investigate the potential applications of these strongly coupled states arising specifically in organic molecular systems.

In the first project we investigate the potential of organic dye molecules to undergo condensation in an optical cavity at room temperature. The second study involves the use of …

Artificial Neural Network Discovery Of A Switchable Metasurface Reflector, J. R. Thompson, J. A. Burrow, P. J. Shah, J. Slagle, E. S. Harper, A. Van Rynbach, I. Agha, M. S. Mills

Electro-Optics and Photonics Faculty Publications

Optical materials engineered to dynamically and selectively manipulate electromag- netic waves are essential to the future of modern optical systems. In this paper, we simulate various metasurface configurations consisting of periodic 1D bars or 2D pillars made of the ternary phase change material Ge2Sb2Te5 (GST). Dynamic switching behavior in reflectance is exploited due to a drastic refractive index change between the crystalline and amorphous states of GST. Selectivity in the reflection and transmission spectra is manipulated by tailoring the geometrical parameters of the metasurface. Due to the immense number of possible metasurface configurations, we train deep neural networks capable of …

Biomedical Applications Of Polarimetry, Nathaniel Owen King

McKelvey School of Engineering Graduate Student Theses & Dissertations

Non- or minimally-invasive data collection is highly desirable for gathering the broad base of information that facilitates moving technology to the point of care. Polarimetry has been making this transition for years. Early forms of polarization-sensitive optics involved custom multiplexing a series of images to generate a single image, but today’s snapshot polarimeters are readily commercially available.

The research presented in this dissertation advances three areas of polarimetric imaging: First, this research develops a reflectance-based measurement for tracking changes in the alignment of dynamically loaded soft tissue, specifically tendon. This work highlights a range of mounting angles across which signal …

Structural Organization And Chemical Activity Revealed By New Developments In Single-Molecule Fluorescence And Orientation Imaging, Tianben Ding

McKelvey School of Engineering Graduate Student Theses & Dissertations

Single-molecule (SM) fluorescence and its localization are important and versatile tools for understanding and quantifying dynamical nanoscale behavior of nanoparticles and biological systems. By actively controlling the concentration of fluorescent molecules and precisely localizing individual single molecules, it is possible to overcome the classical diffraction limit and achieve 'super-resolution' with image resolution on the order of 10 nanometers.

Single molecules also can be considered as nanoscale sensors since their fluorescence changes in response to their local nanoenvironment. This dissertation discusses extending this SM approach to resolve heterogeneity and dynamics of nanoscale materials and biophysical structures by using positions and orientations …

Snow-Albedo Feedback In Northern Alaska: How Vegetation Influences Snowmelt, Lucas C. Reckhaus

Theses and Dissertations

This paper investigates how the snow-albedo feedback mechanism of the arctic is changing in response to rising climate temperatures. Specifically, the interplay of vegetation and snowmelt, and how these two variables can be correlated. This has the potential to refine climate modelling of the spring transition season. Research was conducted at the ecoregion scale in northern Alaska from 2000 to 2020. Each ecoregion is defined by distinct topographic and ecological conditions, allowing for meaningful contrast between the patterns of spring albedo transition across surface conditions and vegetation types. The five most northerly ecoregions of Alaska are chosen as they encompass …

Artificial Neural Network Discovery Of A Switchable Metasurface Reflector, J. R. Thompson, J. A. Burrow, P. J. Shah, Jonathan E. Slagle, E. S. Harper, A. Van Rynbach, I. Agha, M. S. Mills

Student Publications

Optical materials engineered to dynamically and selectively manipulate electromagnetic waves are essential to the future of modern optical systems. In this paper, we simulate various metasurface configurations consisting of periodic 1D bars or 2D pillars made of the ternary phase change material Ge2Sb2Te5 (GST). Dynamic switching behavior in reflectance is exploited due to a drastic refractive index change between the crystalline and amorphous states of GST. Selectivity in the reflection and transmission spectra is manipulated by tailoring the geometrical parameters of the metasurface. Due to the immense number of possible metasurface configurations, we train deep neural networks capable of exploring …

A Hybrid Achromatic Metalens, Fatih Balli, Mansoor A. Sultan, Sarah K. Lami, J. Todd Hastings

Electrical and Computer Engineering Faculty Publications

Metalenses, ultra-thin optical elements that focus light using subwavelength structures, have been the subject of a number of recent investigations. Compared to their refractive counterparts, metalenses offer reduced size and weight, and new functionality such as polarization control. However, metalenses that correct chromatic aberration also suffer from markedly reduced focusing efficiency. Here we introduce a Hybrid Achromatic Metalens (HAML) that overcomes this trade-off and offers improved focusing efficiency over a broad wavelength range from 1000-1800 nm. HAMLs can be designed by combining recursive ray-tracing and simulated phase libraries rather than computationally intensive global search algorithms. Moreover, HAMLs can be fabricated …

Designing A Reactor Chamber For Hot Electron Chemistry On Bimetallic Plasmonic Nanoparticles, Bryn Merrill, Bingjie Zhang, Jerry Larue

SURF Posters and Papers

Catalysis provides pathways for efficient and selective chemical reactions by lowering the energy barriers for desired products. Gold nanoparticles (AuNPs) show excellent promise as plasmonic catalysts. Plasmonic materials have localized surface plasmon resonances, oscillations of the electron bath at the surface of a nanoparticle, that generate energetically intense electric fields which rapidly decay into energetically excited electrons. The excited electrons have the potential to destabilize atoms strongly bound to the catalysts through occupation of antibonding orbitals. Tuning the antibonding orbitals to make them accessible for occupancy by electrons is achieved by coating the AuNP in a thin layer of another …

Free Charge Carrier Properties In Two-Dimensional Materials And Monoclinic Oxides Studied By Optical Hall Effect, Sean Knight

Department of Electrical and Computer Engineering: Dissertations, Theses, and Student Research

In this dissertation, optical Hall effect (OHE) measurements are used to determine the free charge carrier properties of important two-dimensional materials and monoclinic oxides. Two-dimensional material systems have proven useful in high-frequency electronic devices due to their unique properties, such as high mobility, which arise from their two-dimensional nature. Monoclinic oxides exhibit many desirable characteristics, for example low-crystal symmetry which could lead to anisotropic carrier properties. Here, single-crystal monoclinic gallium oxide, an AlInN/GaN-based high-electron-mobility transistor (HEMT) structure, and epitaxial graphene are studied as examples. To characterize these material systems, the OHE measurement technique is employed. The OHE is a physical …

Investigation Of Complex Refractive Index Of Grad Phene Oxide Using Polarisation Response Of Graphene Oxide-Coated Planarizeoptical Waveguide, Soon Xin Gan

Student Works (2020-2029)

Since a single atomic layer of carbon, also as known as graphene is being successfully exfoliated from 3D graphite, intense research on graphene and its derivative begins. Among them, graphene oxide (GO) is considered one of the most prominent candidates in the category of graphene derivatives for the application of electronic, optoelectronic and photonics. However, although GO has been applied in many applications like saturable absorbers of Q-switch laser and optical limiters for eye protection, its intrinsic optical properties especially complex refractive index reported so far still has a large deviation. Also, most of the optical characterization research on GO …

Organic Materials As Saturable Absorber For Pulse Generation At Telecommunication Window, Mohammed Hussein Sameer Salam M.H.

Student Works (2020-2029)

This thesis demonstrates several types of fiber lasers based on newly developed organic materials as saturable absorbers (SAs). We used these SAs in all-fiber based erbium-doped fiber laser (EDFL) ring cavity to produce Q-switched and mode-locked pulses at telecommunication window, at ~ 1560 nm. Three different organic materials were used in this thesis: Bis[2-(4,6-difluorophenyl)pyridinato-C2 ,N](picolinato)iridium(III) (FIrpic), bis(8-hydroxyquinoline)zinc (Znq2) and Tris(8-hydroxyquinoline)aluminum (Alq3). Finding new materials is still one of the defining characteristics of nonlinear optics field, as the rapid development of SAs has provided several new opportunities for nonlinear optics. Throughout this work, organic material showed a very interesting performance in …

Development And Demonstration Of A Pico-Watt Calorimeter For Optical Absorption Spectroscopy, Behshad Roshanzadeh

Optical Science and Engineering ETDs

An optical calorimeter for sensitive absorption measurements of non-radiative samples at 4 K was designed, built, and demonstrated. It consists of a cryostat cooled by a commercial pulse tube (PTC) refrigerator, a measurement chamber housing the sample and thermometers, and various fiber-coupled light sources. By employing measures to damp mechanical noise from the environment and active temperature stabilization of critical components of the instrument temperature noise as low as 6 nK/√Hz at 50 mHz was achieved under 15 mW of optical excitation. An optical absorption induced temperature increase of the sample as small as 2.5 nK could be resolved using …

Generation Of Correlated Dual Frequency Combs With Pm Fiber Lasers For High-Precision Metrology, Hanieh Afkhamiardakani

Optical Science and Engineering ETDs

Intracavity Phase Interferometry (IPI) using two correlated, counter-propagating frequency combs (pulse trains) in mode-locked lasers has evolved into a powerful technique for high-precision metrology. In this method a physical parameter to be measured imparts a phase shift onto a pulse circulating in the laser cavity. Inside a laser cavity, that phase shift becomes a frequency shift (phase shift/round-trip time) applied to the whole frequency comb created by this pulse as it exits the cavity at each round-trip. This frequency shift is measured by interfering this comb with a reference comb created by a reference pulse circulating in the same mode-locked …

Improved Antimicrobial Properties Of Silver Nanoparticles With Methylene Blue, Ermek Belekov

Masters Theses & Specialist Projects

Photosensitizing agents are the cornerstone of photodynamic therapy (PDT) that play essential role in deactivation process of multidrug resistant pathogens and tumor treatments. In this work we studied a photosensitizing agent made from mixture of silver nanoparticles (Ag NPs) and methylene blue (MB) which possess improved important characteristics like high photostability and high singlet oxygen yield. Ag NPs were synthesized by pulsed laser ablation technique in different aqueous solutions like Polyvinylpyrrolidone (PVP), citrate and Deionized (DI) water. The synthesized Ag NPs were characterized in depth using with transmission electron microscopy (TEM), UVVisible (UV-Vis), and photoluminescence (PL) spectra. Ag NPs were …

Radiation-Balanced Fiber Lasers And Amplifiers, Esmaeil Mobini Souchelmaei Mr

Optical Science and Engineering ETDs

Over the past decades, high-power fiber lasers and amplifiers have been extensively under research to achieve higher output powers. However, temperature rise in the core of fiber lasers and amplifiers has been a big issue in power-scaling. Radiation-balancing is a viable technique introduced for effective heat mitigation in lasers and amplifiers by S. Bowman in 1995. Radiation-balancing relies on solid-state laser cooling as a self-cooling mechanism to mitigate the generated heat in lasers and amplifiers. To implement the mentioned idea in fiber lasers and amplifiers, a set of issues should be scrutinized; (i) the amenability of silica glass (as the …

Quantum Two-Photon Laser In Kerr-Like Medium, Ahmed Mathkoor Faisal Hamood

Student Works (2020-2029)

In this thesis, we studied the Kerr nonlinearity effects on nonclassicality and statistics of the laser field besides the effects of detuning, injection rate, and intensity-dependent coupling (IDC). We developed a quantum theory of light generated from a two-photon laser (TPL) with nonlinear Kerr-like medium in a laser dissipative cavity. The full quantum mechanical approach with the density matrix of the particle-field system is used to derive the TPL master equation based on Scully-Lamb’s quantum theory of laser. Various dynamical operators of interest for the cavity field are calculated analytically and computed numerically. The sophisticated computational program was developed to …

Turbulence Profiling Using Pupil Plane Wavefront Data Derived Fried Parameter Values For A Dynamically Ranged Rayleigh Beacon, Steven M. Zuraski, Elizabeth Beecher, Jack E. Mccrae, Steven T. Fiorino

Faculty Publications

Long-range optical imaging applications are typically hindered by atmospheric turbulence. The effect of turbulence on an imaging system can manifest itself as an image blur effect usually quantified by the phase distortions present in the system. The blurring effect can be understood on the basis of the measured strength of atmospheric optical turbulence along the propagation path and its impacts on phase perturbation statistics within the imaging system. One method for obtaining these measurements is by the use of a dynamically ranged Rayleigh beacon system that exploits strategically varied beacon ranges along the propagation path, effectively obtaining estimates of the …

Measurements Of Optical Turbulence Over 149-Km Path, Jack E. Mccrae, Santasri Bose-Pillai, Steven T. Fiorino, Aaron J. Archibald, Joel Meoak, Brannon Elmore, Thomas Kesler, Christopher A. Rice

Faculty Publications

An experiment was conducted to study turbulence along a 149-km path between the Mauna Loa and Haleakala mountain tops using digital cameras and light-emitting diode (LED) beacons. Much of the path is over the ocean, and a large portion of the path is 3 km above sea level. On the Mauna Loa side, six LED beacons were placed in a roughly linear array with pair spacings from 7 to 62 m. From the Haleakala side, a pair of cameras separated by 83.8 cm observed these beacons. Turbulence along the path induces tilts on the wavefronts, which results in displacements of …

Wave-Optics Investigation Of Turbulence Thermal Blooming Interaction: I. Using Steady-State Simulations, Mark F. Spencer

Faculty Publications

Part I of this two-part paper uses wave-optics simulations to look at the Monte Carlo averages associated with turbulence and steady-state thermal blooming (SSTB). The goal is to investigate turbulence thermal blooming interaction (TTBI). At wavelengths near 1 μm, TTBI increases the amount of constructive and destructive interference (i.e., scintillation) that results from high-power laser beam propagation through distributed-volume atmospheric aberrations. As a result, we use the spherical-wave Rytov number and the distortion number to gauge the strength of the simulated turbulence and SSTB. These parameters simplify greatly given propagation paths with constant atmospheric conditions. In addition, we use the …