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2022

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Full-Text Articles in Optics

Photonic Monitoring Of Atmospheric Fauna, Adrien P. Genoud Dec 2022

Photonic Monitoring Of Atmospheric Fauna, Adrien P. Genoud

Dissertations

Insects play a quintessential role in the Earth’s ecosystems and their recent decline in abundance and diversity is alarming. Monitoring their population is paramount to understand the causes of their decline, as well as to guide and evaluate the efficiency of conservation policies. Monitoring populations of flying insects is generally done using physical traps, but this method requires long and expensive laboratory analysis where each insect must be identified by qualified personnel. Lack of reliable data on insect populations is now considered a significant issue in the field of entomology, often referred to as a “data crisis” in the field. …


Atom-Specific Probing Of Electron Dynamics In An Atomic Adsorbate By Time-Resolved X-Ray Spectroscopy, Simon Schreck, Elias Diesen, Martina Dell'angela, Chang Liu, Matthew Weston, Flavio Capotondi, Hirohito Ogasawara, Jerry Larue, Roberto Costantini, Martin Beye, Piter S. Miedema, Joakim Halldin Stenlid, Jörgen Gladh, Boyang Liu, Hsin-Yi Wang, Fivos Perakis, Filippo Cavalca, Sergey Koroidov, Peter Amann, Emanuele Pedersoli, Denys Naumenko, Ivaylo Nikolov, Lorenzo Raimondi, Frank Abild-Pedersen, Tony F. Heinz, Johannes Voss, Alan C. Luntz, Anders Nilsson Dec 2022

Atom-Specific Probing Of Electron Dynamics In An Atomic Adsorbate By Time-Resolved X-Ray Spectroscopy, Simon Schreck, Elias Diesen, Martina Dell'angela, Chang Liu, Matthew Weston, Flavio Capotondi, Hirohito Ogasawara, Jerry Larue, Roberto Costantini, Martin Beye, Piter S. Miedema, Joakim Halldin Stenlid, Jörgen Gladh, Boyang Liu, Hsin-Yi Wang, Fivos Perakis, Filippo Cavalca, Sergey Koroidov, Peter Amann, Emanuele Pedersoli, Denys Naumenko, Ivaylo Nikolov, Lorenzo Raimondi, Frank Abild-Pedersen, Tony F. Heinz, Johannes Voss, Alan C. Luntz, Anders Nilsson

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The electronic excitation occurring on adsorbates at ultrafast timescales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of x-ray absorption spectroscopy (XAS) and x-ray emission spectroscopy (XES) of a simple well-known adsorbate prototype system, namely carbon (C) atoms adsorbed on a nickel [Ni(100)] surface, following intense laser optical pumping at 400 nm. We observe ultrafast (∼100  fs) changes in both XAS and XES showing clear signatures of the formation of a hot electron-hole pair distribution on the adsorbate. This is followed by slower changes on a few picoseconds …


Temperature Influence On The Optical Properties, Attenuation Coefficient, And Total Molecular Cross Section Of Dhunge Dhara Drinking Water, Saddam Husain Dhobi, Bibek Koirala, Kishori Yadav, Jeevan Jyoti Nakarmi, Suresh Prasad Gupta, Santosh Kumar Das, Arun Kumar Shah, Kuldip Paudel, Kushal Dahal, Ram Lal Sah Dec 2022

Temperature Influence On The Optical Properties, Attenuation Coefficient, And Total Molecular Cross Section Of Dhunge Dhara Drinking Water, Saddam Husain Dhobi, Bibek Koirala, Kishori Yadav, Jeevan Jyoti Nakarmi, Suresh Prasad Gupta, Santosh Kumar Das, Arun Kumar Shah, Kuldip Paudel, Kushal Dahal, Ram Lal Sah

Makara Journal of Science

This work aims to measure the different parameters of Dhunge Dhara water (DDW) such as absorbance, transmittance, mass attenuation coefficient (MAC), and molecular cross section (MCS) and experimentally compare the obtained values with those of pure water (PW) at various temperatures (5 °C to 90 °C) using a theremino spectrometer. Observation shows that the parameters vary with temperature and wavelength. The transmittance of DDW ranges from 18% to 85% and absorbance of the same ranges from 0.09 Au to 0.7 Au. Meanwhile, the transmittance of PW ranges from 40% to 98% and the absorbance of the same ranges from 0.09 …


Multi-Plane Light Conversion: Devices And Applications, Yuanhang Zhang Dec 2022

Multi-Plane Light Conversion: Devices And Applications, Yuanhang Zhang

Electronic Theses and Dissertations, 2020-2023

Multi-plane light conversion (MPLC) has recently been developed as a versatile tool for manipulating spatial distributions of the optical field through repeated phase modulations. An MPLC Device consists of a series of phase masks separated by free-space propagation. It can convert one orthogonal set of beams into another orthogonal set through unitary transformation, which is useful for a number of applications. In telecommunication, for example, mode-division multiplexing (MDM) is a promising technology that will enable continued scaling of capacity by employing spatial modes of a single fiber. MPLC has shown great potential in MDM devices with ultra-wide bandwidth, low insertion …


Molecular Insights Into The Redox Of Atmospheric Mercury Through Laser Spectroscopy, Rongrong Wu Cohen Dec 2022

Molecular Insights Into The Redox Of Atmospheric Mercury Through Laser Spectroscopy, Rongrong Wu Cohen

Theses and Dissertations

The widespread pollution of mercury motivates research into its atmospheric chemistry and transport. Gaseous elemental mercury (Hg(0)) dominates mercury emission to the atmosphere, but the rate of its oxidation to mercury compound (Hg(II)) plays a significant role in controlling where and when mercury deposits to ecosystems. Atomic bromine is regarded as the main oxidant for Hg(0) oxidation, known to initiate the oxidation via a two-step process in the atmosphere – formation of BrHg (R1) and subsequent reactions of BrHg with abundant free radicals Y, i.e., NO2, HOO, etc. (R2), where the reaction of BrHg +Y could also lead to the …


Six-Dimensional Single-Molecule Imaging With Isotropic Resolution Using A Multi-View Reflector Microscope, Oumeng Zhang, Zijian Guo, Yuanyuan He, Tingting Wu, Michael D. Vahey, Matthew D. Lew Dec 2022

Six-Dimensional Single-Molecule Imaging With Isotropic Resolution Using A Multi-View Reflector Microscope, Oumeng Zhang, Zijian Guo, Yuanyuan He, Tingting Wu, Michael D. Vahey, Matthew D. Lew

Electrical & Systems Engineering Publications and Presentations

Imaging of both the positions and orientations of single fluorophores, termed single-molecule orientation-localization microscopy, is a powerful tool for the study of biochemical processes. However, the limited photon budget associated with single-molecule fluorescence makes high-dimensional imaging with isotropic, nanoscale spatial resolution a formidable challenge. Here we realize a radially and azimuthally polarized multi-view reflector (raMVR) microscope for the imaging of the three-dimensional (3D) positions and 3D orientations of single molecules, with precisions of 10.9 nm and 2.0° over a 1.5-μm depth range. The raMVR microscope achieves 6D super-resolution imaging of Nile red molecules transiently bound to lipid-coated spheres, accurately resolving …


Supercontinuum Light Generation Via Non-Linear Effects In Hollow-Core Fiber, Skyler Gulati Dec 2022

Supercontinuum Light Generation Via Non-Linear Effects In Hollow-Core Fiber, Skyler Gulati

Physics Student Works

The field of non-linear optics has gained traction in the last couple decades due to the variable generation of wavelengths which are less deterministic than within traditional optics. Using non-linear mediums, including hollow-core fibers (HCF), generation of wavelengths spanning into the vacuum ultraviolet (VUV) wavelength range is possible. These short wavelengths can be utilized within electron spectroscopy-based methods of material science like angle-resolved photoemission spectroscopy (ARPES). This technique most often uses specific photoemission lines of atoms in discharge lamps, however, with the frequency dispersion capabilities of HCF, broad band creation can allow for variable wavelength selection through filtering specific wavelengths …


Modulation Of Non-Diffracting Hermite Gaussian Beams And Nonlinear Optical Microscopy For Nanoscale Sulfur Imaging, Gilberto Navarro Dec 2022

Modulation Of Non-Diffracting Hermite Gaussian Beams And Nonlinear Optical Microscopy For Nanoscale Sulfur Imaging, Gilberto Navarro

Open Access Theses & Dissertations

Hermite Gaussian beams are the solutions of the scalar paraxial wave equation in Cartesian coordinates. A method was developed to modulate the intensity profile of non-diffracting Hermite Gaussian (HG) beams. The original HG beamâ??s intensity profile consists of high intense corner lobes and low intense central lobes which is not ideal for structured illumination in light-field microscopy. The modulated HG beams were generated by multiplying the original HGâ??s beam envelope by a super-Gaussian envelope to modify the intensity profile to attain equal intensity lobes. The propagation of the original HG beam and modulated HG beam were compared to determine that …


Fitting Solar Panel Brdf Parameters To Out-Of-Plane Empirical Data, Michael R. Gross Dec 2022

Fitting Solar Panel Brdf Parameters To Out-Of-Plane Empirical Data, Michael R. Gross

Theses and Dissertations

The bidirectional reflectance distribution function (BRDF) describes material reflectance by describing how incident irradiance reflects into all possible scatter angles as a function of incident angle. However, a solar panel has unique features that are not featured in any of these previously known models. A previous project at the Air Force Institute of Technology (AFIT) created a novel microfacet-like BRDF to model a solar panel with a prominent diffractive feature present which had not been previously modeled. This BRDF was coded into MATLAB for modeling purposes and C++ to test its speed with a MEX function call. A previous thesis …


Investigation Of Gaas Double Heterostructures For Photonic Heat Engines, Nathan Giannini-Hutchin Dec 2022

Investigation Of Gaas Double Heterostructures For Photonic Heat Engines, Nathan Giannini-Hutchin

Optical Science and Engineering ETDs

The creation of a laser cooled semiconductor device has been a long sought achievement. GaAs-based devices have emerged as a promising candidate for the realization of this goal. Efforts to improve the efficiency of such devices have enabled the material to exhibit external quantum efficiencies (EQE, a measure of the probability that an excitation leads to the emission of a photon) of 99.5\%. Despite this impressive feat, a laser coolable device remains elusive.

To investigate the obstacles to such a device, the material characteristics of GaAs-based double heterostructures (DHS) are theoretically and experimentally examined. Through this study, a GaAs $\vert$ …


Oil Particle Analysis Using Machine Learning And Holography Imaging, Daniel Cruz Dec 2022

Oil Particle Analysis Using Machine Learning And Holography Imaging, Daniel Cruz

Open Access Theses & Dissertations

Holographic cameras show potential as a sensor to monitor oil spills. Holographic cameras record the light interference from particles in a volume of space, producing an image called a hologram. Processing these holograms is known as hologram reconstruction. It produces a representation of particles located in three-dimensional space. These cameras can record precise shapes and sizes of particles in a volume of water. However, it is very time-consuming and resource-intensive to process the images. Most algorithms that perform particle analysis require the hologram reconstruction step. The well-documented hybrid method is one such algorithm. Machine learning is one possible technique that …


Oam-Based Wavelets In A High Speed Optical Probing System For Measuring The Angular Decomposition Of The Environment, Justin Free Dec 2022

Oam-Based Wavelets In A High Speed Optical Probing System For Measuring The Angular Decomposition Of The Environment, Justin Free

All Theses

This thesis presents the theoretical development of orbital angular momentum (OAM) based wavelets for the analysis of localized OAM information in space. An optical probing system for generating and detecting these wavelets is demonstrated; individual wavelets can scan the environment in 10µs or less. The probing system was applied to a three-dimensional atmospheric turbulence distribution to obtain a continuous wavelet transform of the angular information of the turbulent propagation path about a fixed radius. An entire continuous wavelet transform was measured in 3.8ms; the measurements are much faster than the turbulence and give insight into the short time scale of …


Frequency Domain Diffuse Optics Spectroscopies For Quantitative Measurement Of Tissue Optical Properties, Sadhu Moka Nov 2022

Frequency Domain Diffuse Optics Spectroscopies For Quantitative Measurement Of Tissue Optical Properties, Sadhu Moka

USF Tampa Graduate Theses and Dissertations

Tissue oxygen saturation, blood flow and blood volume are physiological bio-markers of tissue health. Diffuse Optical Spectroscopy(DOS) and Diffuse Correlation Spectroscopy (DCS) are two complementary approaches to measure tissue oxygen saturation and blood flow respectively. Quantitative Diffuse Optical Spectroscopy (DOS) uses multi-spectral intensities of near-infrared light that have been modulated at RF frequencies to estimate static tissue optical properties and hence concentrations of oxygenated and de-oxygenated hemoglobin. Diffuse Correlation Spectroscopy estimates tissue dynamics - i.e., blood flow, by measuring temporal intensity auto-correlation function of backscattered light diffusing through the tissue. Conventionally, DCS instruments use coherent light sources with constant intensity. …


Reducing Instrumentation Barriers Of Diffuse Correlation Spectroscopy For Low-Cost Deep Tissue Blood Flow Monitoring, Arindam Biswas Nov 2022

Reducing Instrumentation Barriers Of Diffuse Correlation Spectroscopy For Low-Cost Deep Tissue Blood Flow Monitoring, Arindam Biswas

USF Tampa Graduate Theses and Dissertations

Cerebral blood flow (CBF) is a good indicator of brain health as blood carries necessary nutrients, oxygen, and metabolic byproducts. Quantitative blood flow information can be used in several clinical and therapeutic applications such as stroke detection, measuring autoregulation, evaluating brain injury, or determining neuronal activity. Over the past few decades, light-based deep tissue hemodynamic detection modalities have become popular for non-invasive CBF measurements. In particular, noninvasive Diffuse Correlation Spectroscopy (DCS), has become a tool of choice for research and clinical applications due to its depth sensitivity (>1 cm), portability, validity against other technologies such as Magnetic Resonance Imaging …


A Patient-Specific Algorithm For Lung Segmentation In Chest Radiographs, Manawaduge Supun De Silva, Barath Narayanan Narayanan, Russell C. Hardie Nov 2022

A Patient-Specific Algorithm For Lung Segmentation In Chest Radiographs, Manawaduge Supun De Silva, Barath Narayanan Narayanan, Russell C. Hardie

Electrical and Computer Engineering Faculty Publications

Lung segmentation plays an important role in computer-aided detection and diagnosis using chest radiographs (CRs). Currently, the U-Net and DeepLabv3+ convolutional neural network architectures are widely used to perform CR lung segmentation. To boost performance, ensemble methods are often used, whereby probability map outputs from several networks operating on the same input image are averaged. However, not all networks perform adequately for any specific patient image, even if the average network performance is good. To address this, we present a novel multi-network ensemble method that employs a selector network. The selector network evaluates the segmentation outputs from several networks; on …


Investigation Of Laser And Nonlinear Properties Of Anderson Localizing Optical Fibers, Cody Ryan Bassett Nov 2022

Investigation Of Laser And Nonlinear Properties Of Anderson Localizing Optical Fibers, Cody Ryan Bassett

Optical Science and Engineering ETDs

In this dissertation, I investigate the possibility of lasing and nonlinear phenomena in completely solid-state transverse Anderson localizing optical fibers (TALOFs). I examine three areas within this range of topics. The research in nonlinear phenomena focuses on four-wave mixing (FWM). FWM is of high interest in TALOFs due to the fact that guided localized modes of the fiber each have different propagation constants, and thus unique possible FWM pairs can be generated from the same input pump beam. I demonstrate the generation of FWM in the TALOF by pumping it with 532 nm light into a localized mode and observing …


Submillimeter-Wave Cornea Phantom Sensing Over An Extended Depth Of Field With An Axicon-Generated Bessel Beam, Mariangela Baggio, Aleksi Tamminen, Joel Lamberg, Roman Grigorev, Samu-Ville Pälli, Juha Ala-Laurinaho, Irina Nefedova, Jean-Louis Bourges, Sophie X. Deng, Elliott R. Brown, Vincent P. Wallace, Zachary D. Taylor Nov 2022

Submillimeter-Wave Cornea Phantom Sensing Over An Extended Depth Of Field With An Axicon-Generated Bessel Beam, Mariangela Baggio, Aleksi Tamminen, Joel Lamberg, Roman Grigorev, Samu-Ville Pälli, Juha Ala-Laurinaho, Irina Nefedova, Jean-Louis Bourges, Sophie X. Deng, Elliott R. Brown, Vincent P. Wallace, Zachary D. Taylor

Physics Faculty Publications

The feasibility of a 220 - 330 GHz zero order axicon generated Bessel beam for corneal water content was explored. Simulation and experimental data from the 25-degree cone angle hyperbolic-axicon lens illuminating metallic spherical targets demonstrate a monotonically decreasing, band integrated, backscatter intensity for increasing radius of curvature from 7 - 11 mm, when lens reflector and optical axis are aligned. Further, for radii >= 9.5 mm, maximum signal was obtained with a 1 mm transverse displacement between lens and reflector optical axes arising from spatial correlation between main lobe and out of phase side lobes. Thickness and permittivity parameter …


Sers Platform For Single Fiber Endoscopic Probes, Debsmita Biswas Nov 2022

Sers Platform For Single Fiber Endoscopic Probes, Debsmita Biswas

LSU Doctoral Dissertations

Molecular detection techniques have huge potential in clinical environments. In addition to many other molecular detection techniques, endoscopic Raman spectroscopy has great ability in terms of minimal invasiveness and real-time spectra acquisition. However, Raman Effect is low in sensitivity, limiting the application. Surface-Enhanced Raman Scattering (SERS), addresses this limitation. SERS brings rough nano-metallic surfaces in contact with specimen molecules which enormously enhances Raman signals. This provides Raman spectroscopy with immense capabilities for diverse fields of applications.

Generally, in clinical probe applications, the spectrometer is brought near the target molecules for detection. Typically, optical fibers are used to couple spectrometers to …


Review Of Structural Color In The Genus Chrysochroa Dejean, 1833 (Coleoptera: Buprestidae), Able Chow Nov 2022

Review Of Structural Color In The Genus Chrysochroa Dejean, 1833 (Coleoptera: Buprestidae), Able Chow

LSU Master's Theses

The jewel beetles, (Coleoptera: Buprestidae Leach, 1815), is the eighth most speciose coleopteran family, with the majority of its members possessing diverse bright, saturated structural coloration of multilayer origin. This study focuses on the genus Chrysochroa Dejean, 1833, which includes some of the most brilliantly and charismatically colored buprestid species. While members of Chrysochroa are prised by entomologists amateurs and professional and are well-represented in museum collections, the evolution and ecology of their structural color remain underexplored. Twenty-eight select taxa including exemplars from all 13 subgenera of Chrysochroa were investigated to provide an overview of the objective optical properties and …


Optimizing Switching Of Non-Linear Properties With Hyperbolic Metamaterials, James A. Ethridge, John G. Jones, Manuel R. Ferdinandus, Michael J. Havrilla, Michael A. Marciniak Nov 2022

Optimizing Switching Of Non-Linear Properties With Hyperbolic Metamaterials, James A. Ethridge, John G. Jones, Manuel R. Ferdinandus, Michael J. Havrilla, Michael A. Marciniak

Faculty Publications

Hyperbolic metamaterials have been demonstrated to have special potential in their linear response, but the extent of their non-linear response has not been extensively modeled or measured. In this work, novel non-linear behavior of an ITO/SiO2 layered hyperbolic metamaterial is modeled and experimentally confirmed, specifically a change in the sign of the non-linear absorption with intensity. This behavior is tunable and can be achieved with a simple one-dimensional layered design. Fabrication was performed with physical vapor deposition, and measurements were conducted using the Z-scan technique. Potential applications include tunable optical switches, optical limiters, and tunable components of laser sources.


Electro-Optical Sensors For Atmospheric Turbulence Strength Characterization With Embedded Edge Ai Processing Of Scintillation Patterns, Ernst Polnau, Don L. N. Hettiarachchi, Mikhail A. Vorontsov Oct 2022

Electro-Optical Sensors For Atmospheric Turbulence Strength Characterization With Embedded Edge Ai Processing Of Scintillation Patterns, Ernst Polnau, Don L. N. Hettiarachchi, Mikhail A. Vorontsov

Electro-Optics and Photonics Faculty Publications

This study introduces electro-optical (EO) sensors (TurbNet sensors) that utilize a remote laser beacon (either coherent or incoherent) and an optical receiver with CCD camera and embedded edge AI computer (Jetson Xavier Nx) for in situ evaluation of the path-averaged atmospheric turbulence refractive index structure parameter C-n(2) at a high temporal rate. Evaluation of C-n(2) values was performed using deep neural network (DNN)-based real-time processing of short-exposure laser-beacon light intensity scintillation patterns (images) captured by a TurbNet sensor optical receiver. Several pre-trained DNN models were loaded onto the AI computer and used for TurbNet sensor performance evaluation in a set …


Oxygen Vacancies In Lib3O5 Crystals And Their Role In Nonlinear Absorption, Brian C. Holloway, Christopher A. Lenyk, Timothy D. Gustafson, Nancy C. Giles Oct 2022

Oxygen Vacancies In Lib3O5 Crystals And Their Role In Nonlinear Absorption, Brian C. Holloway, Christopher A. Lenyk, Timothy D. Gustafson, Nancy C. Giles

Faculty Publications

LiB3O5 (LBO) crystals are used to generate the second, third, and fourth harmonics of near-infrared solid-state lasers. At high power levels, the material’s performance is adversely affected by nonlinear absorption. We show that as-grown crystals contain oxygen and lithium vacancies. Transient absorption bands are formed when these intrinsic defects serve as traps for “free” electrons and holes created by x rays or by three- and four-photon absorption processes. Trapped electrons introduce a band near 300 nm and trapped holes produce bands in the 500-600 nm region. Electron paramagnetic resonance (EPR) is used to identify and characterize the …


Miniaturized Iii-V/ Si Hybrid Laser With An Integrated Modulator, Praveen Kumar Singaravelu Sep 2022

Miniaturized Iii-V/ Si Hybrid Laser With An Integrated Modulator, Praveen Kumar Singaravelu

Theses

Light interaction with microscopic and nanoscopic structures enable manipulation of its characteristics which can be used to detect objects in 3D sensing, propel satellites to space using photonic propulsion and transmit data through optical communication. For optical communication, the basic components are lasers, modulators and photodetectors. The development of CMOS microfabrication foundries helps to manufacture silicon-based photonic devices with high yield that is directly co-integrated with electronics in a single chip. However, the lack of emission of photons efficiently in silicon propelled the necessity of hybrid photonic devices that inherits the combined advantage of different materials i.e. functionality and volume. …


Pulse-Quality Metric For Nonstationary Partially Coherent Fields, Milo W. Hyde Iv, Olga Korotkova, Mark F. Spencer Sep 2022

Pulse-Quality Metric For Nonstationary Partially Coherent Fields, Milo W. Hyde Iv, Olga Korotkova, Mark F. Spencer

Faculty Publications

This paper generalizes a pulse-quality metric referred to as P2, i.e., the time analogue of Siegman’s beam quality factor M2, to include pulsed (nonstationary) random fields of any state of coherence. The analysis begins with the derivation of a general P2 relation, which we then specialize to the important cases of coherent and Schell-model pulsed beams. As examples, we derive the P2 for two stochastic sources: (1) a cosine Gaussian-correlated Schell-model pulsed beam and (2) a nonuniformly correlated pulsed beam. For both of these sources, we generate (in simulation) random instances of each and …


Deep-Turbulence Phase Compensation Using Tiled Arrays, Mark F. Spencer, Terry J. Brennan Sep 2022

Deep-Turbulence Phase Compensation Using Tiled Arrays, Mark F. Spencer, Terry J. Brennan

Faculty Publications

Tiled arrays use modulo-2π phase compensation and coherent beam combination to correct for the effects of deep turbulence. As such, this paper uses wave-optics simulations to compare the closed-loop performance of tiled arrays to a branch-point-tolerant phase reconstructor known as LSPV+7 [Appl. Opt. 53, 3821 (2014) [CrossRef] ]. The wave-optics simulations make use of a point-source beacon and are setup with weak-to-strong scintillation conditions. This setup enables a trade-space exploration in support of a power-in-the-bucket comparison with LSPV+7. In turn, the results show that tiled arrays outperform LSPV+7 when transitioning from weak-to-strong scintillation conditions. These results are both …


Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak Sep 2022

Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak

Faculty Publications

Resonant plasmonic–molecular chiral interactions are a promising route to enhanced biosensing. However, biomolecular optical activity primarily exists in the far-ultraviolet regime, posing significant challenges for spectral overlap with current nano-optical platforms. We demonstrate experimentally and computationally the enhanced chiral sensing of a resonant plasmonic–biomolecular system operating in the far-UV. We develop a full-wave model of biomolecular films on Al gammadion arrays using experimentally derived chirality parameters. Our calculations show that detectable enhancements in the chiroptical signals from small amounts of biomolecules are possible only when tight spectral overlap exists between the plasmonic and biomolecular chiral responses. We support this conclusion …


Topological Shadow Of Higher-Order Topological Phases And Non-Hermitian Phases Protected By Generalized Rotational Symmetry, Kai Chen Sep 2022

Topological Shadow Of Higher-Order Topological Phases And Non-Hermitian Phases Protected By Generalized Rotational Symmetry, Kai Chen

Dissertations, Theses, and Capstone Projects

Topological phenomena in condensed matter physics have been investigated intensively in the past decades since the discovery of the integer quantum Hall effect (IQHE). For the IQHE, the energy band can be characterized by its topological invariants (Chern number or TKNN invariant), which relates to the quantized Hall conductance directly. Later, this expression was recognized as the first Chern class of a U(1) principal fiber bundle on a torus, where the fibers and torus correspond respectively to the magnetic Bloch waves and the magnetic Brillouin zone. And then, the discoveries of time-reversal symmetric topological insulators in two and three dimensions …


Degree Of Linear Polarization: An Indicator Of Optical Vortex Beam Entanglement, Ella James Sep 2022

Degree Of Linear Polarization: An Indicator Of Optical Vortex Beam Entanglement, Ella James

Summer Community of Scholars Posters (RCEU and HCR Combined Programs)

No abstract provided.


Control Of Nonlinear Properties Of Van Der Waals Materials, Rezlind Bushati Sep 2022

Control Of Nonlinear Properties Of Van Der Waals Materials, Rezlind Bushati

Dissertations, Theses, and Capstone Projects

Van der Waals materials are a broad class of materials that exhibit unique optoelectronic properties. They provide a rich playground for which they can be integrated into current on-chip devices due to their nanometer-scale size, and be utilized for studying fundamental physics. Strong coupling of emitters to microcavities provides many opportunities for new exotic physics through the formation of hybrid quasi-particles exciton-polaritons. This thesis
focuses on exploring and enhancing nonlinearity of van der Waals materials through strongly coupling to microcavities. By taking advantage of the stacking order of TMDs, we show intense second-harmonic generation from bulk, centrosymmetric TMD systems. In …


Optimizing Optical Switching Of Non-Linear Hyperbolic Metamaterials, James A. Ethridge Sep 2022

Optimizing Optical Switching Of Non-Linear Hyperbolic Metamaterials, James A. Ethridge

Theses and Dissertations

Modern optical materials are engineered to be used as optical devices in specific applications, such as optical computing. For optical computing, efficient forms of a particular device, the optical switch, still have not been successfully demonstrated. This problem is addressed in this research through the use of designed optical metamaterials, specifically, hyperbolic metamaterials, which offer the possibility of large non-linear properties with a low switching intensity. One-dimensional layered hyperbolic metamaterials composed of alternating layers of metal and dielectric were used here, with ITO as the metal and SiO2 as the dielectric. The non-linear behavior of the ITO/SiO2 layered …