Spectroscopic End Point Detection With An Electron Beam Evaporator, 2024 Portland State University
Spectroscopic End Point Detection With An Electron Beam Evaporator, Ryan M. Mcgraw
University Honors Theses
Spectroscopic end point detection is a com- mon tool used for measuring slope changes in
wavelength intensity. Using algorithms able to apply this concept, coatings will be able to be dynamically measured in real time and stopped
at the appropriate level to ensure process uni- formity. It is currently applied to reductive pro- cesses such as etching, where the surface will
start to be eaten away, creating a plasma. When the entire amount of a material on a substrate has been eaten away, the plasma will change
color as it is beginning to etch a different ma- terial. Using a …
6d Single-Fluorogen Orientation-Localization Microscopy For Elucidating The Architecture Of Beta-Sheet Assemblies And Biomolecular Condensates, 2024 Washington University in St. Louis
6d Single-Fluorogen Orientation-Localization Microscopy For Elucidating The Architecture Of Beta-Sheet Assemblies And Biomolecular Condensates, Tingting Wu, Weiyan Zhou, Jai S. Rudra, Rohit V. Pappu, Matthew D. Lew
Electrical & Systems Engineering Publications and Presentations
We develop six-dimensional single-molecule orientation-localization microscopy (SMOLM) to measure the 3D positions and 3D orientations simultaneously of single fluorophores. We show how careful optimization of phase and polarization modulation components can encode phase, polarization, and angular spectrum information from each fluorescence photon into a microscope’s dipole-spread function. We used the transient binding and blinking of Nile red (NR) to characterize the helical structure of fibrils formed by designed amphipathic peptides, KFE8L and KFE8D, and the pathological amyloid-beta peptide Aβ42. We also deployed merocyanine 540 to uncover the interfacial architectures of biomolecular condensates.
Two-Photon Absorption And Fluorescence Of Cadmium Sulfide, 2024 College of Saint Benedict/Saint John's University
Two-Photon Absorption And Fluorescence Of Cadmium Sulfide, Jacob Goranson, Gregory J. Taft
Physics Faculty Publications
The two-photon absorption and fluorescence of bulk cadmium sulfide were studied using 50-fs, 800-nm pulses from an unamplified Ti:sapphire laser. The fluorescence spectrum was measured to have a main peak at 522 nm, and the power of the fluorescence was shown to vary quadratically with the 800-nm beam power. This supports the theory that the fluorescence is excited by two-photon absorption and confirms previous work done with longer duration, higher energy excitation pulses. Pump-probe measurements provided additional confirmation of the two-photon absorption. Measured spectral broadening of the wings of the laser spectrum also was observed, which likely is due to …
Exciton Dynamics, Interaction, And Transport In Monolayers Of Transition Metal Dichalcogenides, 2024 The Graduate Center, City University of New York
Exciton Dynamics, Interaction, And Transport In Monolayers Of Transition Metal Dichalcogenides, Saroj Chand
Dissertations, Theses, and Capstone Projects
Monolayers Transition metal dichalcogenides (TMDs) have attracted much attention in recent years due to their promising optical and electronic properties for applications in optoelectronic devices. The rich multivalley band structure and sizable spin-orbit coupling in monolayer TMDs result in several optically bright and dark excitonic states with different spin and valley configurations. In the proposed works, we have developed experimental techniques and theoretical models to study the dynamics, interactions, and transport of both dark and bright excitons.
In W-based monolayers of TMDs, the momentum dark exciton cannot typically recombine optically, but they represent the lowest excitonic state of the system …
Applications Of Independent And Identically Distributed (Iid) Random Processes In Polarimetry And Climatology, 2024 Michigan Technological University
Applications Of Independent And Identically Distributed (Iid) Random Processes In Polarimetry And Climatology, Dan Kestner
Dissertations, Master's Theses and Master's Reports
The unifying theme of this thesis is the characterization of “perfect randomness,” i.e., independent and identically distributed (IID) stochastic processes as these are applied in physical science. Two specific and mathematically distinct applications are chosen: (i) Radar and optical polarimetry; (ii) Analysis of time series in meteorology. In (i), IID process of a special kind, namely, with a distribution defined by symmetry, is used to link its multivariate Gaussian density to uniformity on the Poincaré sphere. This “statistical ellipsometry” approach is then used to relate polarimetric mismatches or imbalances to ellipsometric variables and suitably chosen cross-correlation measures. In (ii), recently …
Single-Stage Few-Cycle Pulse Amplification, 2024 Manipal Institute of Technology, Manipal University
Single-Stage Few-Cycle Pulse Amplification, Sagnik Ghosh, Nathan G. Drouillard, Tj Hammond
Physics Publications
Kerr instability can be exploited to amplify visible, near-infrared, and midinfrared ultrashort pulses. We use the results of Kerr instability amplification theory to inform our simulations amplifying few-cycle pulses. We show that the amplification angle dependence is simplified to the phase-matching condition of four-wave mixing when the intense pump is considered. Seeding with few-cycle pulses near the pump leads to broadband amplification without spatial chirp, while longer pulses undergo compression through amplification. Pumping in the midinfrared leads to multioctave spanning amplified pulses with single-cycle duration not previously predicted. We discuss limitations of the amplification process and optimizing pump and seed …
Volumetric Imaging Using The Pupil-Matched Remote Focusing Technique In Light-Sheet Microscopy, 2023 University of New Mexico
Volumetric Imaging Using The Pupil-Matched Remote Focusing Technique In Light-Sheet Microscopy, Sayed Hassan Dibaji Foroushani
Optical Science and Engineering ETDs
ABSTRACT
The dissertation explores innovative techniques in light sheet microscopy, a pivotal tool in biomedical imaging, to enhance its speed, resolution, and efficiency in capturing dynamic biological processes. Light sheet microscopy allows for quick 3D imaging of biological specimens ranging from cells to organs with high spatiotemporal resolution, large field-of-view, and minimal damage, making it vital for in vivo imaging.
The first project introduces a novel optical concept designed to optimize Axially Swept Light Sheet Microscopy (ASLM). This technique is crucial for imaging specimens ranging from live cells to chemically cleared organs due to its versatility across different immersion media. …
Development Of An Optical Test Bed For The Fabrication And Characterisation Of An Analog Holographic Wavefront Sensor, 2023 Technological University Dublin
Development Of An Optical Test Bed For The Fabrication And Characterisation Of An Analog Holographic Wavefront Sensor, Emma Branigan, Andreas Zepp, Suzanne Martin, Matthew Sheehan, Szymon Gladysz, Kevin Murphy
Conference Papers
A new holographic recording setup has been developed for the fabrication of single- and multi-mode photopolymer-based analog holographic wavefront sensors. A second setup has been built and used to characterise the sensor at several wavelengths.
Aspects Of Stochastic Geometric Mechanics In Molecular Biophysics, 2023 Clemson University
Aspects Of Stochastic Geometric Mechanics In Molecular Biophysics, David Frost
All Dissertations
In confocal single-molecule FRET experiments, the joint distribution of FRET efficiency and donor lifetime distribution can reveal underlying molecular conformational dynamics via deviation from their theoretical Forster relationship. This shift is referred to as a dynamic shift. In this study, we investigate the influence of the free energy landscape in protein conformational dynamics on the dynamic shift by simulation of the associated continuum reaction coordinate Langevin dynamics, yielding a deeper understanding of the dynamic and structural information in the joint FRET efficiency and donor lifetime distribution. We develop novel Langevin models for the dye linker dynamics, including rotational dynamics, based …
Radiation Exposure Calibration Of The Al2o3:C With Radium-226 And Cesium-137 Using The Osl Method, 2023 Clemson University
Radiation Exposure Calibration Of The Al2o3:C With Radium-226 And Cesium-137 Using The Osl Method, Selma Tepeli Aydin
All Theses
Optically stimulated luminescence (OSL) dosimetry was utilized to calibrate Al2O3:C powder dosimeters, available commercially as the nanoDot® from Landauer Inc., and compare the dosimeter response to radium-226 (226Ra) and cesium-137 (137Cs). The signal from the OSL was quantified using a microSTARii® OSL reader also produced by Landauer Inc. Dose-response curves were developed for 226Ra and 137Cs experiments (5 dosimeters each) at thirteen absorbed doses. Individual dosimeter response was tracked by serial number. Linear regression analysis was performed to determine if there were significant differences between the intercepts of the …
Acoustically Levitated Whispering-Gallery Mode Microlasers, 2023 Universidad de Guanajuato
Acoustically Levitated Whispering-Gallery Mode Microlasers, H. M. Reynoso-De La Cruz, E. D. Hernández-Campos, E. Ortiz-Ricardo, A. Martínez-Borquez, I. Rosas-Román, V. Contreras, G. Ramos-Ortiz, B. Mendoza-Santoyo, Cecilia Zurita-Lopez, R. Castro-Beltrán
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Acoustic levitation has become a crucial technique for contactless manipulation in several fields, particularly in biological applications. However, its application in the photonics field remains largely unexplored. In this study, we implement an affordable and innovative phased-array levitator that enables stable trapping in the air of micrometer dye-doped droplets, thereby enabling the creation of microlasers. For the first time, this paper presents a detailed performance of the levitated microlaser cavity, supported by theoretical analysis concerning the hybrid technology based on the combination of whispering-gallery modes and acoustic fields. The pressure field distribution inside the acoustic cavity is numerically solved and …
System-Level Noise Performance Of Coherent Imaging Systems, 2023 University of Arizona
System-Level Noise Performance Of Coherent Imaging Systems, Derek J. Burrell, Joshua H. Follansbee, Mark F. Spencer, Ronald G. Driggers
Faculty Publications
We provide an in-depth analysis of noise considerations in coherent imaging, accounting for speckle and scintillation in addition to “conventional” image noise. Specifically, we formulate closed-form expressions for total effective noise in the presence of speckle only, scintillation only, and speckle combined with scintillation. We find analytically that photon shot noise is uncorrelated with both speckle and weak-to-moderate scintillation, despite their shared dependence on the mean signal. Furthermore, unmitigated speckle and scintillation noise tends to dominate coherent-imaging performance due to a squared mean-signal dependence. Strong coupling occurs between speckle and scintillation when both are present, and we characterize this behavior …
Quantitative, Photocurrent Multidimensional Coherent Spectroscopy, 2023 University of Denver
Quantitative, Photocurrent Multidimensional Coherent Spectroscopy, Adam Halaoui
Electronic Theses and Dissertations
Multidimensional coherent spectroscopy (MDCS) is a quickly growing field that has a lot of advantages over more conventional forms of spectroscopy. These advantages all come from the fact that MDCS allows us to get time resolved correlated emission and absorption spectra using very precisely chosen interactions between the density matrix and the excitation laser. MDCS spectra gives the researcher a lot of information that can be extracted purely through qualitative analysis. This is possible because state couplings are entirely separated on the spectra, and once we know how to read the data, we can see how carriers transport in the …
Active-Illumination Extension To The Priest And Meier Pbrdf, 2023 Air Force Institute of Technology
Active-Illumination Extension To The Priest And Meier Pbrdf, Mark F. Spencer, Milo W. Hyde Iv, Santasri R. Bose-Pillai, Michael A. Marciniak
Faculty Publications
This paper develops a 3D vector solution for the scattering of partially coherent laser-beam illumination from statistically rough surfaces. Such a solution enables a rigorous comparison to the well-known Priest and Meier polarimetric bidirectional reflectance distribution function (pBRDF) [Opt Eng 41(5),988 (2002).]. Overall, the comparison shows excellent agreement for the normalized spectral density and the degree of polarization. Based on this agreement, the 3D vector solution also enables an extension to the Priest and Meier pBRDF that accounts for the effects of active illumination. In particular, the 3D vector solution enables the development of a closed-form expression for the spectral …
Optics Studies For Multipass Energy Recovery At Cebaf: Er@Cebaf, 2023 Old Dominion University
Optics Studies For Multipass Energy Recovery At Cebaf: Er@Cebaf, Isurumali Neththikumara
Physics Theses & Dissertations
Energy recovery linacs (ERLs), focus on recycling the kinetic energy of electron beam for the purpose of accelerating a newly injected beam within the same accelerating structure. The rising developments in the super conducting radio frequency technology, ERL technology has achieved several noteworthy milestones over the past few decades. In year 2003, Jefferson Lab has successfully demonstrated a single pass energy recovery at the CEBAF accelerator. Furthermore, they conducted successful experiments with IR-FEL demo and upgrades, as well as the UV FEL driver. This multi-pass, multi-GeV range energy recovery demonstration proposed to be carried out at CEBAF accelerator at Jefferson …
Dynamics Of Spin And Charge Of Color Centers In Diamond Under Cryogenic Conditions, 2023 The Graduate Center, City University of New York
Dynamics Of Spin And Charge Of Color Centers In Diamond Under Cryogenic Conditions, Richard G. Monge
Dissertations, Theses, and Capstone Projects
Individual quantum systems in semiconductors are currently the most sought-after platform for applications in quantum science. Most notably, the nitrogen-vacancy (NV) center in diamond features a defect deep within the electronic bandgap, making it amenable for precise manipulation to help pave the way to perform fundamental quantum physics experimentation. The NV center also offers long coherence times and versatile spin-dependent fluorescent properties, making it an ideal candidate for a nanoscale magnetometer. Furthermore, multi-color excitation offers deterministic charge state manipulation. While ambient operation has been key to their appeal, bringing NVs to cryogenic conditions opens new opportunities for alternate forms of …
Nonlinear Processes In Room Temperature Exciton-Polaritons, 2023 The Graduate Center, City University of New York
Nonlinear Processes In Room Temperature Exciton-Polaritons, Prathmesh Deshmukh
Dissertations, Theses, and Capstone Projects
Strong light-matter coupling in solid state systems is an intriguing process that allows one to exploit the advantages of both light and matter. In this context, microcavities have become essential platforms for studying the strong coupling regime, where hybrid light-matter states known as exciton-polaritons form, leading to enhanced light matter interaction, modified material properties, and novel quantum phenomena. In this thesis, we explore the phenomenology of exciton-polaritons in strained TMD microcavities, 2D perovskites, fluorescent proteins and organic dyes encompassing thermalization, polariton lasing, and the observation of nonlinear effects.
Transition metal dichalcogenides (TMDs) have emerged as a remarkable class of two- …
Design And Fabrication Of A Trapped Ion Quantum Computing Testbed, 2023 University of Massachusetts Amherst
Design And Fabrication Of A Trapped Ion Quantum Computing Testbed, Christopher A. Caron
Masters Theses
Here we present the design, assembly and successful ion trapping of a room-temperature ion trap system with a custom designed and fabricated surface electrode ion trap, which allows for rapid prototyping of novel trap designs such that new chips can be installed and reach UHV in under 2 days. The system has demonstrated success at trapping and maintaining both single ions and cold crystals of ions. We achieve this by fabricating our own custom surface Paul traps in the UMass Amherst cleanroom facilities, which are then argon ion milled, diced, mounted and wire bonded to an interposer which is placed …
The Importance Of Contrast Sensitivity, Color Vision, And Electrophysiological Testing In Clinical And Occupational Settings, 2023 University of the Incarnate Word
The Importance Of Contrast Sensitivity, Color Vision, And Electrophysiological Testing In Clinical And Occupational Settings, Frances Silva
Theses & Dissertations
Visual acuity (VA) is universally accepted as the gold standard metric for ocular vision and function. Contrast sensitivity (CS), color vision, and electrophysiological testing for clinical and occupational settings are warranted despite being deemed ancillary and minimally utilized by clinicians. These assessments provide essential information to subjectively and objectively quantify and obtain optimal functional vision. They are useful for baseline data and monitoring hereditary and progressive ocular conditions and cognitive function. The studies in this dissertation highlight the value of contrast sensitivity, color vision, and cone specific electrophysiological testing, as well as the novel metrics obtained with potential practical clinical …
High-Power Laser Cooling And Temperature-Dependent Fluorescence Studies Of Ytterbium Doped Silica, 2023 University of New Mexico
High-Power Laser Cooling And Temperature-Dependent Fluorescence Studies Of Ytterbium Doped Silica, Brian Topper
Optical Science and Engineering ETDs
Experimental observation of optical refrigeration using ytterbium doped silica glass in recent years has created a new solution for heat mitigation in high-power laser systems, nonlinear fiber experiments, integrated photonics, and precision metrology. Current efforts of different groups focus on compositional optimization, fiber fabrication, and investigating how much silica can be cooled with a laser. At the start of this work, the best effort in laser cooling ytterbium doped silica saw cooling by 6 K from room temperature. This dissertation follows the experimental efforts that culminated in the increase of this initial record by one order of magnitude. Comprehensive spectroscopic …