Condensed Matter Physics Commons^™

Anomalous And Spin Hall Effects In A Magnetic Tunnel Junction With Rashba Spin-Orbit Coupling, A. V. Vedyayev, M. S. Titova, N. V. Ryzhanova, M. Ye. Zhuravlev, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

Anomalous and spin Hall effects are investigated theoretically for a magnetic tunnel junction where the applied voltage produces a Rashba spin-orbit coupling within the tunneling barrier layer. The ferromagnetic electrodes are the source of the spin-polarized current. The tunneling electrons experience a spin-orbit coupling inside the barrier due to the applied electrical field. Charge and spin Hall currents are calculated as functions of the position inside the barrier and the angle between the magnetizations of the electrodes. We find that both charge and spin Hall currents are located inside the barrier near the interfaces. The dependence of the currents on …

The Measurement Of The Dielectric Constant Of Concrete Pipes And Clay Pipes, David Mcgraw

Doctoral Dissertations

To optimize the effectiveness of the rehabilitation of underground utilities, taking in consideration limitation of available resources, there is a need for a cost effective and efficient sensing systems capable of providing effective, in real time and in situ, measurement of infrastructural characteristics. To carry out accurate non-destructive condition assessment of buried and above ground infrastructure such as sewers, bridges, pavements and dams, an advanced ultra-wideband (UWB) based radar was developed at Trenchless Technology Centre (TTC) and Centre for Applied Physics Studies (CAPS) at Louisiana Tech University (LTU). One of the major issues in designing the FCC compliant UWB radar …

Tuning The JEff = 1/2 Insulating State Via Electron Doping And Pressure In The Double-Layered Iridate Sr3Ir2O7, L. Li, P. P. Kong, Tongfei Qi, C. Q. Jin, Shujuan Yuan, Lance E. Delong, P. Schlottmann, Gang Cao

Physics and Astronomy Faculty Publications

Sr₃Ir₂O₇ exhibits a novel J_eff = 1/2 insulating state that features a splitting between J_eff = 1/2 and 3/2 bands due to spin-orbit interaction. We report a metal-insulator transition in Sr3Ir2O7 via either dilute electron doping (La³⁺ for Sr²⁺) or application of high pressure up to 35 GPa. Our study of single-crystal Sr₃Ir₂O₇ and (Sr_1−xLa_x)₃Ir₂O₇ reveals that application of high hydrostatic pressure P leads to a drastic reduction in the electrical resistivity by as much …

Entropy Driven Crystal Formation On Highly Strained Substrates, John R. Savage, Stefan F. Hopp, Rajesh Ganapathy, Sharon J. Gerbode, Andreas Heuer, Itai Cohen

All HMC Faculty Publications and Research

In heteroepitaxy, lattice mismatch between the deposited material and the underlying surface strongly affects nucleation and growth processes. The effect of mismatch is well studied in atoms with growth kinetics typically dominated by bond formation with interaction lengths on the order of one lattice spacing. In contrast, less is understood about how mismatch affects crystallization of larger particles, such as globular proteins and nanoparticles, where interparticle interaction energies are often comparable to thermal fluctuations and are short ranged, extending only a fraction of the particle size. Here, using colloidal experiments and simulations, we find particles with short-range attractive interactions form …

Analysis Of An Unusual Liquid Crystal Phase Transition, Loni Ann Fuller

Physics

Liquid crystals are a unique phase of matter that resemble a state between a solid and liquid. Within these properties, liquid crystal molecules have the ability to align and create layers. From this phenomenon, many electro-optical effects can be investigated, such as measuring the tilt angle between molecules at different temperatures and applied electric fields and also measuring the birefringence, which is a unique property of liquid crystals in which the index of refraction of the sample behaves differently along different axes. In order to better understand these electro- optical effects, we designed a more precise protocol of measuring this …

Electron Transport In Quantum Dot Chains: Dimensionality Effects And Hopping Conductance, V. P. Kunets, Mariama Rebello Sousa Dias, T. Rembert, M. E. Ware, Y. I. Mazur, V. Lopez-Richard, H. A. Mantooth, G. E. Marques, G. J. Salamo

Physics Faculty Publications

Detailed experimental and theoretical studies of lateral electron transport in a system of quantum dot chains demonstrate the complicated character of the conductance within the chain structure due to the interaction of conduction channels with different dimensionalities. The one-dimensional character of states in the wetting layer results in an anisotropic mobility, while the presence of the zero-dimensional states of the quantum dots leads to enhanced hopping conductance, which affects the low-temperature mobility and demonstrates an anisotropy in the conductance. These phenomena were probed by considering a one-dimensional model of hopping along with band filling effects. Differences between the model and …

Spin Switching And Magnetization Reversal In Single-Crystal Ndfeo3, Shujuan Yuan, W. Ren, F. Hong, Y. B. Wang, J. C. Zhang, L. Bellaiche, Gang Cao

Physics and Astronomy Faculty Publications

We report an experimental and computational study of single-crystal NdFeO₃, which features two inequivalent magnetic sublattices, namely, Fe and Nd sublattices that are coupled in an antiparallel fashion. This paper reveals that a strong interaction between 3d and 4f electrons of the two sublattices along with a spin-lattice coupling drives an extremely interesting magnetic state that is highly sensitive to the orientation and history of weak magnetic field. The following phenomena are particularly remarkable: (1) sharply contrasting magnetization M(T) along the a and c axes; (2) a first-order spin switching along the a …

Multiband S -Wave Topological Superconductors: Role Of Dimensionality And Magnetic Field Response, Shusa Deng, Gerardo Ortiz, Lorenza Viola

Dartmouth Scholarship

We further investigate a class of time-reversal-invariant two-band s-wave topological superconductors introduced earlier [Deng, Viola, and Ortiz, Phys. Rev. Lett. 108, 036803 (2012)]. Provided that a sign reversal between the two superconducting pairing gaps is realized, the topological phase diagram can be determined exactly (within mean field) in one and two dimensions as well as in three dimensions upon restricting to the excitation spectrum of time-reversal-invariant momentum modes. We show how, in the presence of time-reversal symmetry, Z2 invariants that distinguish between trivial and nontrivial quantum phases can be constructed by considering only one of the Kramers’ sectors …

Rapid Diffusion Of Electrons In Gamnas, Christopher P. Weber, Eric A. Kittlaus, Kassandra B. Mattia, Christopher J. Waight, J. Hagmann, X. Liu, M. Dobrowolska, J. K. Furdyna

Physics

We report ultrafast transient‐grating measurements, above and below the Curie temperature, of the dilute ferromagnetic semiconductor (Ga,Mn)As containing 6% Mn. At 80 K (15 K), we observe that photoexcited electrons in the conduction band have a lifetime of 8 ps (5 ps) and diffuse at about 70 cm²/s (60 cm²/s). Such rapid diffusion requires either an electronic mobility exceeding 7700 cm²/V s or a conduction‐band effective mass less than half the GaAs value. Our data suggest that neither the scattering rate nor the effective mass of the (Ga,Mn)As conduction band differs significantly from that …

Magnetic And Crystal Structures Of Sr2Iro4: A Neutron Diffraction Study, Feng Ye, Songxue Chi, Bryan C. Chakoumakos, Jaime A. Fernandez-Baca, Tongfei Qi, Gang Cao

Center for Advanced Materials Faculty Publications

We report a single-crystal neutron diffraction study of the layered Sr₂IrO₄. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the IrO₆ octahedra in Sr₂IrO₄. The long-range antiferromagnetic order has a canted spin configuration with an ordered moment of 0.208(3) μ_B/Ir site within the basal plane; a detailed examination of the spin canting yields 0.202(3) and 0.049(2) μ_B/site for the a axis and the b axis, respectively. It is intriguing that forbidden nuclear reflections …

Density Functional Theory And The Calculation Of Tcmg2O4 Spinel Lattice Parameters, Jon Karlo Macias

Physics

The cohesive energy, lattice constant and bulk modulus of two simple HCP crystal structures of magnesium and technetium were calculated using the vienna ab initio simulation package (VASP) which is based on density functional theory (DFT). The same properties were determined for TcMg₂O₄ spinel. The theoretical results of the lattice constant of the pure crystals were compared to experimental results and found to be in excellent agreement with a difference of less than 2%. The results for the lattice constant of the TcMg₂O₄ spinel were found to be in excellent agreement as well with …

Ab-Initio And Model Studies Of Spin Fluctuation Effects In Transport And Thermodynamics Of Magnetic Metals, James K. Glasbrenner

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Magnetic materials are vital to many devices and the manipulation of spins is central to the operation of novel devices such as spin transistors. It is important to understand the effect of spin fluctuations on such systems. In this dissertation, first-principles calculations and models further the understanding of spin fluctuation effects in the transport and thermodynamics of magnetic metals.

A simple classical spin-fluctuation Hamiltonian with a single itinerancy parameter is studied using the mean-field approximation, Monte Carlo simulations, and a generalized Onsager cavity field method. The results of these different methods are in agreement. It is found that the thermodynamics …

Hydroxyl-Decorated Graphene Systems As Candidates For Organic Metal-Free Ferroelectrics, Multiferroics, And High-Performance Proton Battery Cathode Materials, Menghao Wu, John D. Burton, Evgeny Y. Tsymbal, Xiao Cheng Zeng, Purusottam Jena

Evgeny Tsymbal Publications

Using a first-principles method we show that graphene based materials, functionalized with hydroxyl groups, constitute a class of multifunctional, lightweight, and nontoxic organic materials with functional properties such as ferroelectricity, multiferroicity, and can be used as proton battery cathode materials. For example, the polarizations of semihydroxylized graphane and graphone, as well as fully hydroxylized graphane, are much higher than any organic ferroelectric materials known to date. Further, hydroxylized graphene nanoribbons with proton vacancies at the end can have much larger dipole moments. They may also be applied as high-capacity cathode materials with a specific capacity that is six times larger …

Faraday Cup Designs For High Efficiency Determination Of Energy- And Angular-Resolved Charged Particle Fluxes, Kent D. Hartley

Senior Theses and Projects

Faraday cups provide a simple and efficient apparatus to measure the absolute magnitude of charge particle fluxes, and with the addition of a retarding field analyzer and defining apertures the capability to determine the energy and angular distributions of the fluxes. Through careful design of the electron optics, a Faraday cup can be tailored to meet specific requirements for detector size, minimum detectable flux, collection efficiency, absolute accuracy, energy discrimination, and angular resolution. This project explores optimal design concepts through electric field and charged particle trajectory simulations, theoretical analysis, and evaluation of experimental prototypes to develop compact, high efficiency Faraday …

Strain-Mediated Elastic Coupling In Magnetoelectric Nickel/Barium-Titanate Heterostructures, Robert Streubel, Denny Köhler, Rudolf Schäfer, Lukas M. Eng

Robert Streubel Papers

Multiferroic nanomaterials bear the potential for assembling a manifold of novel and smart devices. For room temperature (RT) applications, however, only the BiFeO3 single-phase perovskites are potential candidates to date. Nevertheless, vertical heterostructures separating magnetic and ferroelectric functionality into different layers are now widely proposed to circumvent this lack in materials' availability. We show here that the second approach is very profitable as illustrated by the strain-mediated coupling between such two layers, i.e., a ferroelectric barium titanate single-crystal (BTO) and a magnetostrictive nickel (Ni) thin film. Applying an electric field across the BTO substrate forces the magnetic easy axis in …

Diffusion Of Degenerate Minority Carrier In A P-Type Semiconductor, Christopher P. Weber, Eric A. Kittlaus

Physics

We report ultrafast transient-grating experiments on heavily p-type InP at 15 K. Our measurement reveals the dynamics and diffusion of photoexcited electrons and holes as a function of their density n in the range 2  ×  10¹⁶ to 6  ×  10¹⁷ cm⁻³. After the first few picoseconds, the grating decays primarily due to ambipolar diffusion. While, at low density, we observe a regime in which the ambipolar diffusion is electron-dominated and increases rapidly with n, it appears to saturate at 34 cm²/s at high n. We present a simple calculation that reproduces the main …

Low Energy Positron Interactions With Biological Molecules, Indika Lasantha Wanniarachchi

Wayne State University Dissertations

Calculations of the positron density distribution which can be used for positrons bound to midsize and larger molecules have been tested for smaller molecules and subsequently applied to investigate the most likely e+e- annihilation sites for positrons interacting with biological molecules containing C, H, O, and N. In order to allow consideration of positrons bound to extended molecules with regions of different character and no particular symmetry, atom-centered positron basis sets of Gaussian-type functions were developed for positrons bound to molecules containing O, N, C, H, Li, Na, and Be. Testing shows that there is no need to scale the …

Adherent Cells Avoid Polarization Gradients On Periodically Poled Litao3 Ferroelectrics, Christof Christophis, Elisabetta Ada Cavalcanti-Adam, Maximilian Hanke, Kenji Kitamura, Alexei Gruverman, Michael Grunze, Peter A. Dowben, Axel Rosenhahn

Peter Dowben Publications

The response of fibroblast cells to periodically poled LiTaO₃ ferroelectric crystals has been studied. While fibroblast cells do not show morphological differences on the two polarization directions, they show a tendency to avoid the field gradients that occur between polarization domains of the ferroelectric. The response to the field gradients is fully established after one hour, a time at which fibroblasts form their first focal contacts. If suspension cells, with a lower tendency to establish strong surface contacts are used, no influence of the field gradients is observed.

Proton Transfer In Surface-Stabilized Chiral Motifs Of Croconic Acid, Donna A. Kunkel, James Hooper, Scott Simpson, Geoffrey Rojas, Stephen Ducharme, Timothy Usher, Eva Zurek, Axel Enders

Stephen Ducharme Publications

The structure and cooperative proton ordering of two-dimensional sheets of croconic acid were studied with scanning tunneling microscopy and first-principles calculations. Unlike in the crystalline form, which exhibits a pleated, densely packed polar sheet structure, the confinement of the molecules to the surface results in hydrogenbonded chiral clusters and networks. First-principles calculations suggest that the surface stabilizes networks of configurational isomers, which arise from direct hydrogen transfer between their constituent croconic acid monomers. Some of these configurations have a net polarization. It is demonstrated through constrained molecular dynamics simulations that simultaneous proton transfer between any two molecules can occur spontaneously. …

Infrared Phonon Modes In Multiferroic Single-Crystal Fete2o5br, K. H. Miller, X. S. Xu, H. Berger, V. Cracium, Xiaoxiang Xi, C. Martin, G. L. Carr, D. B. Tanner

Xiaoshan Xu Papers

Reflection and transmission as a function of temperature (7–300 K and 5–300 K respectively) have been measured on single crystals of the multiferroic compound FeTe₂O₅Br utilizing light spanning from the far infrared to the visible. The complex dielectric function and other optical properties were obtained via Kramers-Kronig analysis and by fits to a Drude-Lortentz model. Analysis of the anisotropic excitation spectra via Drude-Lorentz fitting and lattice dynamical calculations have led to the observation of 43 of the 53 modes predicted along the b axis of the monoclinic cell. The phonon response parallel to the a and …