Atomic, Molecular and Optical Physics Commons^™

Noise Characterization And Mitigation In Intermediate-Scale Quantum Systems, Muhammad Qasim Khan

Dartmouth College Ph.D Dissertations

Current quantum processors, at the intermediate scale of tens to hundreds of qubits, remain error-limited. This thesis studies two related sources of error. The first is environmental noise, which may have temporal and spatial correlations and nonclassical components. The second is state-preparation and measurement (SPAM) error, which arises in the operations used to characterize this noise, a prerequisite for boosting operational fidelities. Neither can be characterized alone. Noise spectroscopy techniques use imperfect preparation and readout, while SPAM characterization is affected by qubit decoherence. Our methods vary measurement depth, drive duration, or sequence repetition so each source changes the measured signal …

Libs-Based Detection And Preliminary Classification Of Microplastic Signatures In Soil Samples., Ekhlas Jabir Mahmood

Al-Bahir

Contamination of terrestrial systems by microplastics (MPs) has become a critical environmental hazard, but detection of such contaminants in a complex soil system is a challenge for conventional analytical techniques. This research aims to assess the potential of Laser-Induced Breakdown Spectroscopy (LIBS) for the detection and differentiation of different types of microplastics, including HDPE, LDPE, PP, PS, and PVC, dispersed in the soil of Al Najaf, Iraq. Soil samples were collected from different functional zones, namely, Industrial, Commercial, Agricultural, Residential, and Roadside, at the surface level and 30 cm depth. Detection was done by measuring the intensity of the C/H …

Ultrafast Spectroscopy Of Organic Materials In Strong Light–Matter Interaction And Terahertz Optics, Kamyar Rashidi

Dissertations, Theses, and Capstone Projects

Ultrafast spectroscopy is a powerful tool for investigating phenomena that occur on extremely short timescales and for probing ultrabroadband spectral responses enabled by its ultrashort laser pulses. These capabilities are essential for advancing both the fundamental understanding of light–matter interactions and the development of next-generation optoelectronic technologies. The first part of this thesis investigates the ultrafast dynamics of organic exciton–polaritons and their application to controlling molecular excited-state processes using momentum-resolved pump–probe spectroscopy. A major challenge in these systems is the dark-state problem, where photoexcitation predominantly populates long-lived excitonic reservoir states that obscure the in trinsic dynamics of the hybrid light–matter …

Modeling Kinetics Of 5-Aminolevulinic Acid-Induced Protoporphyrin Ix Accumulation For Optimal Photodynamic Therapy, Priscilla Melebor

Graduate Masters Theses

Photodynamic therapy (PDT) is a minimally invasive treatment that uses light-activated photosensitizers to selectively destroy diseased tissue through the generation of reactive oxygen species. However, conventional in vitro models often fail to accurately reproduce the pharmacokinetics of photosensitizer accumulation and clearance observed in vivo. This study investigated protoporphyrin IX (PpIX) accumulation following 5-aminolevulinic acid (ALA) exposure under physiologically relevant conditions using two-dimensional (2D) monolayers and three-dimensional (3D) spheroids. By comparing continuous ALA exposure with transient exposure followed by ALA washout, this work provides a more biologically relevant framework for studying PpIX kinetics and optimizing photodynamic therapy.

Synthesizing Viscoelasticity: Living Polymers, Micro-Macro Relations, And Paths For Resolution, Adam M. Hasler

Graduate Masters Theses

This thesis investigates the relationship between macroscopic rheological signals and underlying microscopic dynamics in complex fluids, specifically focusing on ”living polymers” within the cetyltrimethylammonium bromide (CTAB) and sodium salicylate (NaSal) surfactant system. The research addresses the inverse parameterization problem, demonstrating how bulk measurements like zero-shear viscosity can mask fundamentally different physical topologies, such as purely cylindrical, reptating micelles versus highly branched networks. Through the successful synthesis of viscoelastically ”degenerate” samples, the study utilizes an array of characterization techniques including frequency sweeps, Large Amplitude Oscillatory Shear (LAOS) to resolve these unique underlying states. Furthermore, the work explores further avenues of study …

Symmetry Breaking And Restoration In The Grasshopper Ising Model, Aradh Bisarya

Graduate Masters Theses

Distance-selective interactions in Ising systems give rise to a range of rich and unexpected phenomena. A notable example is the so-called Grasshopper Ising model, a conserved spin Ising model with interactions only between spins at a fixed distance. This model is the discrete version of the following mathematical problem: A grasshopper lands at a random point on a planar lawn of area one. It then makes one jump of fixed distance in a random direction. What lawn shape maximizes the probability that the grasshopper lands on the lawn after the jump? The solution to this problem, corresponding to the ground …

Fabrication Of Objectives For Imaging Ultracold Lithium, Danelle Akanova

Dartmouth College Master’s Theses

This thesis develops a documented, reproducible procedure for building diffraction-limited microscope objectives entirely from catalog singlets, for imaging ultracold 6Li atoms in a ring-trap experiment. The objectives must resolve micron-scale features through a 5 mm fused-silica vacuum window, operate at multiple wavelengths, fit inside a 48 mm magnet bore, and contain no conductive or magnetic material, because the surrounding coils switch 0.1 T fields on microsecond timescales. Commercial long-working-distance objectives are universally housed in metal, which the eddy-current constraint rules out, and custom fabrication of a suitable non-conductive matched pair is estimated at nearly $200k.

The procedure is developed and …

Electronic Structure Discretization And Compression Using Diagonal Basis Sets, Casey Lee Dowdle

Dartmouth College Ph.D Dissertations

Numerically solving the electronic structure problem is a fundamentally difficult problem due to the exponential growth in the dimension of the Hilbert space as the system size increases. In order to solve problems at a chemically relevant accuracy, both the choice of basis set and numerical method are important factors that are intrinsically connected.

In this thesis, we study the discretization and resulting compression of electronic Hamiltonians using diagonal basis sets. A diagonal basis set approximately diagonalizes the matrix and tensor representations of the one- and two-body potentials. This can reduce storage, simplify matrix-vector products, and lower the complexity of …

Development Of Robust Ratio Linear Fitting Method Of Temperature And Emissivity Separation For High-Temperature Data, Mitchell Manzardo, Michael L. Dexter, Shannon R. Young, John Bowlan, Anthony L. Franz

Faculty Publications

Accurate temperature and emissivity separation from thermal infrared radiance is essential for characterizing materials under high-temperature laboratory conditions. Existing temperature and emissivity separation methods have largely been developed for multispectral remote sensing applications, where long atmospheric path lengths require extensive atmospheric compensation. In contrast, the current work considers hyperspectral laboratory measurements acquired over a short optical path, where atmospheric effects are comparatively small but increased measurement uncertainty remains within portions of the measured spectrum. The ABB MR304 FTIR spectrometer used in this study exhibits reduced optical transmission below approximately 2.5 μm, producing increased measurement uncertainty within the spectral region containing …

Bounded Thunderstorm Tracking Of Lightning Events With Muon Detection, Skylar Wardlaw, Ainsley Helgerson, Maria Kaminska, Logan Velvet, Georgii Dubrov, Jackson Stewart, Aaron Jung, Nathaniel O’Hara, Amelia Koth, Nash Mcleod, Emaleth Wyckoff

Discovery Day - Daytona Beach

The muon is a high-energy particle that can be produced by cosmic rays and trigger upper-atmospheric particle cascades and energetic processes. It has been hypothesized that such cascades are at the onset of lightning. As such, muons serve as a valuable probe for investigating the underlying mechanisms of its initiation, whose full governing dynamics remain vastly unknown despite extensive research. Traditional approaches to lightning research involve simulations and observations of the discharge itself, but the role of high-energy particle interactions has yet to be fully constrained. The CosmicWatch Muon Detector design enables the detection of atmospheric muons through scintillation events, …

Enhancing A Mid-Wave Infrared Fourier Transform Hyperspectral Imager For Explosions, James T. Stofel, Kody A. Wilson, Martin Larivière-Bastien, Anthony L. Franz, Michael L. Dexter

Faculty Publications

Capturing reliable hyperspectral imager data at a meaningful frame rate for explosions and other fast-changing scenes is not possible in the mid-wave infrared region under traditional sensor operating configurations and processing techniques, which typically have frame rates on the order of 0.5–2.0 Hz. To combat these shortcomings, the scene acquisition parameters were tailored for explosions and a new method for processing optical signatures of fast transient scenes with Fourier-transform infrared hyperspectral imagers was developed. For this technique, the instrument was first configured to collect asymmetric interferograms while optimizing the number of measurement points on the short side of the interferogram. …

Modeling Formation Of Turbulent Sporadic-E Clouds Using Realistic Wind Data, Aaron M. Schinder, Kenneth S. Obenberger, Jorge L. Chau, Juan M. Urco, Matthias Clahsen, Benjamin F. Akers, Daniel J. Emmons

Faculty Publications

A high resolution two-dimensional multi-fluid model of sporadic-E layers was developed and driven with physically realistic mesosphere, lower thermosphere (MLT) winds measured over Albuquerque, New Mexico. The realistic E-region winds are produced by the HYdrodynamic Point-wise Environment Reconstructor (HYPER) model that ingests meteor derived wind observations from a Spread-spectrum Interferometric Multistatic meteor radar Observing Network (SIMONe) system combined with the Navier-Stokes equations to provide high resolution three-dimensional wind fields over time. Sporadic-E dynamics are simulated using both realistic winds from HYPER as well as idealized hyperbolic tangent windshears to compare and contrast. Overall, the model shows greater inhomogeneity and irregularity …

Algorithmic Sculpting Of Complex Fused Silica Surfaces For Nondestructive, Mode-Matched Cavity Quantum Electrodynamics: Adaptive Co2 Milling And Simulation-Guided Ultrafast Inscription, From Fiber Fabry-Perot Cavities To Monolithic Architectures, Meagan E. Parker

Optical Science and Engineering ETDs

Quantum sensors achieve exceptional measurement sensitivity through coherent, well-isolated quantum systems, but practical deployment is hindered by destructive readouts that require repeated state preparation and create long system dead times. Optical cavities enable continuous, nondestructive measurements with minimal back-action, yet integrating high-finesse cavities into scalable quantum devices remains limited by existing fabrication methods. To overcome these constraints, an adaptive CO₂ laser-milling platform was developed. Guided by glass thermodynamics and melt dynamics, this closed-loop system uses in-situ phase-shifting interferometry to sculpt complex fused-silica surfaces with sub-nanometer root-mean-square roughness. The platform was validated by fabricating extended-length fiber Fabry–Pérot cavities and monolithic micro-cavity …

Coherent Two-Photon Backscattering And Induced Angular Quantum Correlations In Multiple-Scattered Two-Photon States Of The Light, Nooshin M. Estakhri, Theodore B. Norris

Engineering Faculty Articles and Research

We present the emergence of coherent two-photon backscattering, a manifestation of weak localization, in multiple scattering of maximally entangled pure and fully mixed two-photon states and examine the effect of entanglement and classical correlations. Quantum correlations in backscattering are investigated for finite three-dimensional disordered structures in the weak localization regime, as well as systems of a small number of scatterers with specified spatial arrangements. No assumptions are made about the statistical behavior of the scattering matrix elements. Furthermore, we study the interplay between quantum correlations induced by multiple scattering and the correlations that may be present in the illumination fields, …

Lafe0.925ti0.075o3 Perovskite Coated With Ethyl Cellulose: A High-Stability, Low-Hysteresis Platform For Advanced Humidity Sensing, Akhmad Futukhillah Fataba Alaih, Djoko Triyono, Rifqi Almusawi Rafsanjani

Makara Journal of Science

Humidity sensors are pivotal in numerous sectors, such as environmental monitoring, industrial automation, and health-care. This study presents the fabrication and detailed evaluation of an advanced humidity sensor using ethyl cellulose (EC)-coated LaFe_0.925Ti_0.075O₃ (LFTO) perovskite nanoparticles synthesized via the sol-gel method. The LFTO nanopar-ticles exhibited a mesoporous structure with an enhanced surface area, which significantly improved their moisture adsorption capabilities. The innovative application of EC coating addresses critical substrate adhesion issues, enhancing mechanical stability without compromising sensor sensitivity. Comprehensive performance evaluations revealed minimal hysteresis (

Structure Functions For The Inclusive Semileptonic B-Quark Decay At Nnlo: A Semi-Analytic Calculation, A. Broggio, B. Capdevila, A. Ferroglia, P. Gambino

Publications and Research

We present a study of the inclusive charmless semileptonic b decay, b → X_uℓv at next-to-next-to-leading order (NNLO) in perturbative QCD, with the primary aim of extracting the hadronic structure functions Wi at NNLO. The analysis is based on a numerical calculation of the relevant kinematic distributions using a phase-space slicing method to handle infrared-sensitive contributions from real gluon emissions. We use known results from Heavy Quark Effective Theory and Soft-Collinear Effective Theory to extract the singular terms and construct a model for the regular contributions to the structure functions at NNLO, then perform a fit to the …

30 Db On-Chip Ultra-High Inverse Weak Value Amplification, Yuhan Mei, Meiting Song, Andrew N. Jordan, Jaime Cardenas

Mathematics, Physics, and Computer Science Faculty Articles and Research

Weak value amplification (WVA) has emerged as a powerful technique that enhances measurement precision. However, traditional table-top WVA setups and on-chip demonstrations have not achieved an amplification over 20 dB. The practical limit of the amplification is the fidelity of photon post-selection. To address this limit, we design a weak value device with an over 30 dB interferometer extinction ratio, where the stray light in the dark port is minimized with thermally tunable phase shifters. As a result, the device successfully shows 30 dB WVA, termed ultra-high WVA. This WVA optimization strategy by improving interferometer extinction is extensible to a …

Characterizing Stiffness Dynamics Of Normal And Malignant Breast Spheroids Using Brillouin Microscopy, Razanne Rafat Zaghloul, Karlin Hilai, Chenjun Shi, Jitao Zhang

Medical Student Research Symposium

Background: Breast cancer progression and metastasis are closely linked to alterations in the mechanical properties of tumor cells and their microenvironment. Softer, more deformable cells are often associated with higher metastatic potential. While atomic force microscopy (AFM) is the current gold standard for mechanical characterization, it is limited to surface measurements and can damage 3D cultures. It remains unclear how the mechanical properties evolve over time in normal versus malignant spheroids. This study utilizes Brillouin light-scattering microscopy, a non-contact and label-free optical technique, to assess stiffness changes in normal and malignant breast epithelial spheroids over time. Understanding these mechanical signatures …

Optical Nuclear Spin Detection In Diamond And Varifocal Metasurface Optics, Maxwell D. Aiello

Physics & Astronomy ETDs

This dissertation presents two experimental investigations at the intersection of quantum sensing and precision optical instrumentation. The primary project demonstrates optically detected nuclear magnetic resonance (NMR) of ¹³C nuclear spins in diamond, using state-selective Landau-Zener transitions under microwave frequency sweeping to bidirectionally transfer spin polarization between nitrogen-vacancy (NV) electron spins and remote ¹³C nuclear spins. This enables optical polarization and readout of large ensembles of polarized nuclear spins at low magnetic fields and room temperature, with spin dephasing times limited by longitudinal relaxation of nearby NV electron spins. The secondary project reports the design, fabrication, and characterization of …

Constructing A Laser Stabilization System For Frequency Metrology, Stephanie Letourneau

UNLV Theses, Dissertations, Professional Papers, and Capstones

Frequency metrology and quantum control, which uses light as a tool for measurement and manipulation, relies on spectrally narrow, stable lasers. Often thought of as being perfectly monochromatic and coherent, in reality, the free-running instantaneous linewidth of lasers can be on the order of hundreds of kHz in the millisecond time-frame and drift on the order of tens of MHz over hours. To correct for these instabilities in real-time, a variety of laser stabilization methods have been implemented, including the Pound-Drever-Hall (PDH) method, saturation absorption spectroscopy (SAS), and dichroic atomic vapor laser locking (DAVLL). All of these methods rely on …