Condensed Matter Physics Commons^™

Electronic Transport In Two-Dimensional Systems In The Quantum Hall Regime, Vinicio Tarquini

Wayne State University Dissertations

The integer and the fractional quantum Hall effects are essential to the exploration of quantum matters characterized by topological phases. A quantum Hall system hosts one-dimensional (1D) chiral edge channels that manifest zero magnetoresistance, dissipationless due to the broken time reversal symmetry, and quantized Hall resistance v h e^2 with v being the topological invariant (or Chern number). The 1-1 correspondence between the conducting gapless edge channels to the gapped incompressible bulk states is a defining character of a topological insulator (TI). Understanding this correspondence in real systems, especially the origin of its robustness (in terms of the limit of …

Phase Separation In Lufeo3 Films, Shi Cao, Xiaozhe Zhang, Kishan Sinha, Wenbin Wang, Jian Wang, Peter A. Dowben, Xiaoshan Xu

Peter Dowben Publications

The structural transition at about 1000°C, from the hexagonal to the orthorhombic phase of LuFeO₃, has been investigated in thin films of LuFeO₃. Separation of the two structural phases of LuFeO₃ occurs on a length scale of micrometer, as visualized in real space using X-ray photoemission electron microscopy. The results are consistent with X-ray diffraction and atomic force microscopy obtained from LuFeO₃ thin films undergoing the irreversible structural transition from the hexagonal to the orthorhombic phase of LuFeO₃, at elevated temperatures. The sharp phase boundaries between the structural phases are observed to …

Influence Of Steric Hindrance On The Molecular Packing And The Anchoring Of Quinonoid Zwitterions On Gold Surfaces, Minghui Yuan, Iori Tababe, Jean-Marie Bernard- Schaaf, Qin-Yin Shi, Vicki Schlegel, Rachel Schurhammer, Peter A. Dowben, Bernard Doudin, Lucie Routaboul, Pierre Braunstein

Peter Dowben Publications

Driven by the huge potential of engineering the molecular band offset with highly dipolar molecules for improving charge injection into organic electrics, the anchoring of various N-alkyl substituted quinonoid zwitterions of formula C₆H₂ (···NHR)₂ (···O)₂ (R = iPr, Cy, CH₂CH(Et)CH₂CH₂CH₂CH₃,. . .) on gold surfaces is studied. The N–Au interactions result in an orthogonal arrangement of the zwitterions cores with respect to the surface, and stabilize adsorbed compact rows of molecules. IR spectroscopy is used as a straightforward diagnostic tool to validate the presence of …

Fabrication Of Diisopropylammonium Bromide Aligned Microcrystals With In-Plane Uniaxial Polarization, Shashi Poddar, Haidong Lu, Jingfeng Song, Om Goit, Shah Valloppilly, Alexei Gruverman, Stephen Ducharme

Stephen Ducharme Publications

Textured arrays of ferroelectric microcrystals of diisopropylammonium bromide were grown from solution at room temperature onto silicon substrates and studied by means of x-ray diffraction, atomic force microscopy, electron microscopy, and piezoresponse force microscopy. The needle-shaped crystals had dimensions of approximately 50 μm × 5 μm in the plane and were approximately 200 nm thick, where the dimensions and arrangement were influenced by growth conditions. The observations suggest an Ostwald ripening mechanism of the microcrystal growth. The crystals had the structure of the ferroelectric phase, where the polarization axis was in-plane and parallel to the long axis of …

The Effect Of Impurities On The Superconductivity Of Bscco-2212, John Vastola

Honors Undergraduate Theses

BSCCO-2212 is a high-temperature cuprate superconductor whose microscopic behavior is currently poorly understood. In particular, it is unclear whether its order parameter is consistent with s-wave or d-wave symmetry. It has been suggested that its order parameter might take one of several forms that are consistent with d-wave behavior. We present some calculations using the many-body theory approach to superconductivity that suggest that such order parameters would lead to a suppression of the critical temperature in the presence of impurities. Because some experiments have suggested the critical temperature of BSCCO-2212 is relatively independent of the concentration of impurities, this lends …

Multiferroicity In Iron Vanadate, Magnetite And Polyvinylidene Fluoride Nanocomposite Films, Ehab Hamdy Abdelmonaim Abdelhamid

Wayne State University Dissertations

With the increasing demand on cheaper and better performance multifunctional materials for different applications, it is becoming more crucial to have a better understanding of the physics needed to tailor more devices and materials to fit better in every day’s technological needs. Materials which show more than one ferroic order simultaneously –namely, multiferroics– are of particular importance for their potential applications as multiple state memory elements, transducers and electrically tunable microwave devices.

In this work, we studied FeVO4 single crystals as an example on low symmetry multiferroics. We focused on the anisotropy in those crystals in an attempt to nail …

Voltage Ramp-Rate Dependence Of Dc Breakdown In Polymeric Insulators: Physical Models Versus Data, Allen Andersen, Krysta Moser, Jr Dennison

Posters

Purpose/Aim

The standard handbook values for dielectric breakdown strength of necessity come from accelerated test methods. In some applications the breakdown voltage may vary significantly with voltage ramp rates; therefore, a theoretical model for the ramp-rate dependence of breakdown is needed to extrapolate from realistic tests to long-duration material service lifetimes.

Experimental/Modeling methods

Series of step-up to breakdown tests were performed for ramp rates from 0.5 to 500 V/s for biaxially-oriented polypropylene (BOPP), low density polyethylene (LDPE), and polyimide (PI) films. The data were fit with standard empirical methods, as well as two physics-based defect-driven models.

Results/discussion

Table 1 in …

Low-Temperature Fcc To L10 Phase Transformation In Copt(Bi) Nanoparticles, Frank M. Abel, Vasilis Tzitzios, David J. Sellmeyer, George C. Hadjipanayis

Nebraska Center for Materials and Nanoscience: Faculty Publications

This work is focused on the effects of Bi substitution on the synthesis of CoPt nanoparticles with the L1₀ structure using a modified organometallic approach. The structural and magnetic properties of the nanoparticles have been studied and compared directly with those of CoPt nanoparticles synthesized by the same tech- nique but in the absence of Bi substitution. The as-synthesized particles at 330 ◦C have an average size of 11.7 nm and a partially ordered L10 phase with a coercivity of 1 kOe. The coercivity is increased to 9.3 kOe and 12.4 kOe after annealing for 1 hour at 600 …

Electronic Structure And Stability Of Ligated Superatoms And Bimetallic Clusters, William H. Blades

Theses and Dissertations

Quantum confinement in small metal clusters leads to a bunching of states into electronic shells reminiscent of shells in atoms. The addition of ligands can tune the valence electron count and electron distribution in metal clusters. A combined experimental and theoretical study of the reactivity of methanol with Al_nI_m⁻ clusters reveals that ligands can enhance the stability of clusters. In some cases the electronegative ligand may perturb the charge density of the metallic core generating active sites that can lead to the etching of the cluster. Also, an investigation is conducted to understand how the bonding …

Modification Of The G-Phonon Mode Of Graphene By Nitrogen Doping, Pavel V. Lukashev, Liuyan Zhao, Tula R. Paudel, Theanne Schiros, Noah Hurley, Evgeny Y. Tsymbal, Aron Pinczuk, Abhay Pasupathy, Rui He

Nebraska Center for Materials and Nanoscience: Faculty Publications

The effect of nitrogen doping on the phonon spectra of graphene is analyzed. In particular, we employ first-principles calculations and scanning Raman analysis to investigate the dependence of phonon frequencies in graphene on the concentration of nitrogen dopants. We demonstrate that the G phonon frequency shows oscillatory behavior as a function of nitrogen concentration. We analyze different mechanisms which could potentially be responsible for this behavior, such as Friedel charge oscillations around the localized nitrogen impurity atom, the bond length change between nitrogen impurity and its nearest neighbor carbon atoms, and the long-range interactions of the nitrogen point defects. We …

Stereographic Visualization Of Bose-Einstein Condensate Clouds To Measure The Gravitational Constant, Ed Wesley Wells

College of Graduate Studies: Theses & Dissertations

This thesis describes a set of tools that can be used for the rapid design of atom interferometer schemes suitable for measuring Newton's Universal Gravitation constant also known as "Big G". This tool set is especially applicable to Bose--Einstein--condensed systems present in NASA's Cold Atom Laboratory experiment to be deployed to the International Space Station in 2017. These tools include a method of approximating the solutions of the nonlinear Schrödinger or Gross--Pitaevskii equation (GPE) using the Lagrangian Variational Method. They also include a set of software tools for translating the approximate solutions of the GPE into images of the optical …

Time-Resolved Photoluminescence Studies Of Point Defects In Gan, Joy Dorene Mcnamara

Theses and Dissertations

Time-resolved photoluminescence (TRPL) measurements paired with steady-state photoluminescence (SSPL) measurements can help to determine the PL lifetime, shape and position of unresolved bands, capture coefficients, and concentrations of free electrons and defects.PL bands that are obscured in the SSPL spectra can be accurately revealed by TRPL measurements. TRPL measurements are able to show if the PL band originates from an internal transition between different states of the same defect. The main defect-related PL bands in high-purity GaN grown by hydride vapor phase epitaxy (HVPE) which have been investigated are the ultraviolet, blue, green, yellow and red luminescence bands (UVL, BL, …

Mimicking Of Pulse Shape-Dependent Learning Rules With A Quantum Dot Memristor, P. Maier, F. Hartmann, Mariama Rebello Sousa Dias, M. Emmerling, C. Schneider, L. K. Castelano, M. Kamp, G. E. Marques, V. Lopez-Richard, S. Höfling

Physics Faculty Publications

We present the realization of four different learning rules with a quantum dot memristor by tuning the shape, the magnitude, the polarity and the timing of voltage pulses. The memristor displays a large maximum to minimum conductance ratio of about 57 000 at zero bias voltage. The high and low conductances correspond to different amounts of electrons localized in quantum dots, which can be successively raised or lowered by the timing and shapes of incoming voltage pulses. Modifications of the pulse shapes allow altering the conductance change in dependence on the time difference. Hence, we are able to mimic different …

Innovations In Thermoelectric Materials Research: Compound Agglomeration, Testing And Preselection, Hugo Lopez

Open Access Theses & Dissertations

Thermoelectric materials have the capacity to convert a temperature differential into electrical power and vice versa. They will represent the next revolution in alternative energies once their efficiencies are enhanced so they can complement other forms of green energies that depend on sources other than a temperature differential.

Progress in materials science depends on the ability to discover new materials to eventually understand them and to finally improve their properties. The work presented here is aimed at dynamizing the screening of materials of thermoelectric interest. The results of this project will enable: theoretical preselection of thermoelectric compounds based on their …

First Results Of Magnetic Field Penetration Measurements Of Multilayer Sis Structures, O. B. Malyshev, L. Gurran, R. Valizadeh, S. Pattalwar, N. Pattalwar, K. D. Dumbell, A. Gurevich

Physics Faculty Publications

The performance of superconducting RF cavities made of bulk Nb is limited by a breakdown field of B_p ≈200 mT, close to the superheating field for Nb. A potentially promising solution to enhance the breakdown field of the SRF cavities beyond the intrinsic limits of Nb is a multilayer coating suggested in [1]. In the simplest case, such a multilayer may be a superconductor-insulator-superconductor (S-I-S) coating, for example, bulk niobium (S) coated with a thin film of insulator (I) followed by a thin layer of another superconductor (S) which could be e.g. dirty niobium [2]. Here we report the …

Non-Conventional Approaches To Syntheses Of Ferromagnetic Nanomaterials, Dustin M. Clifford

Theses and Dissertations

The work of this dissertation is centered on two non-conventional synthetic approaches to ferromagnetic nanomaterials: high-throughput experimentation (HTE) (polyol process) and continuous flow (CF) synthesis (aqueous reduction and the polyol process). HTE was performed to investigate phase control between Fe_xCo_1-x and Co_3-xFe_xO_y. Exploration of synthesis limitations based on magnetic properties was achieved by reproducing M_s=210 emu/g. Morphological control of Fe_xCo_1-x alloy was achieved by formation of linear chains using an H_ext. The final study of the Fe_xCo_1-x chains used DoE to …

Anisotropy, Phonon Modes, And Free Charge Carrier Parameters In Monoclinic Β-Gallium Oxide Single Crystals, Mathias Schubert, Rafal Korlacki, Sean Knight, Tino Hofmann, Stefan Schöche, Vanya Darakchieva, Erik Janzén, Bo Monemar, Daniela Gogova, Q.-T. Thieu, R. Togashi, H. Murakami, Yoshinao Kumagai, Ken Goto, Akito Kuramata, S. Yamakoshi, Masataka Higashiwaki

Department of Electrical and Computer Engineering: Faculty Publications

We derive a dielectric function tensor model approach to render the optical response of monoclinic and triclinic symmetry materials with multiple uncoupled infrared and far-infrared active modes. We apply our model approach to monoclinic β-Ga₂O₃ single-crystal samples. Surfaces cut under different angles from a bulk crystal, (010) and (2̅01), are investigated by generalized spectroscopic ellipsometry within infrared and far-infrared spectral regions. We determine the frequency dependence of 4 independent β-Ga₂O₃ Cartesian dielectric function tensor elements by matching large sets of experimental data using a point-by-point data inversion approach. From matching our monoclinic …

Theory Of Magnon Motive Force In Chiral Ferromagnets, Utkan Güngördü, Alexey Kovalev

Department of Physics and Astronomy: Faculty Publications

We predict that magnon motive force can lead to temperature dependent, nonlinear chiral damping in both conducting and insulating ferromagnets. We estimate that this damping can significantly influence the motion of skyrmions and domain walls at finite temperatures. We also find that in systems with low Gilbert damping moving chiral magnetic textures and resulting magnon motive forces can induce large spin and energy currents in the transverse direction.

Spin Torque And Nernst Effects In Dzyaloshinskii-Moriya Ferromagnets, Alexey Kovalev, Vladimir Zyuzin

Department of Physics and Astronomy: Faculty Publications

We predict that a temperature gradient can induce a magnon-mediated intrinsic torque in systems with a nontrivial magnon Berry curvature. With the help of a microscopic linear response theory of nonequilibrium magnon-mediated torques and spin currents we identify the interband and intraband components that manifest in ferromagnets with Dzyaloshinskii-Moriya interactions and magnetic textures. To illustrate and assess the importance of such effects, we apply the linear response theory to the magnon-mediated spin Nernst and torque responses in a kagome lattice ferromagnet.

Stability Of Skyrmion Lattices And Symmetries Of Quasi-Two-Dimensional Chiral Magnets, Utkan Güngördü, Rabindra Nepal, Oleg A. Tretiakov, Kirill D. Belashchenko, Alexey Kovalev

Department of Physics and Astronomy: Faculty Publications

Recently there has been substantial interest in realizations of skyrmions, in particular in quasi-two-dimensional (2D) systems due to increased stability resulting from reduced dimensionality. A stable skyrmion, representing the smallest realizable magnetic texture, could be an ideal element for ultradense magnetic memories. Here we use the most general form of the quasi-2D free energy with Dzyaloshinskii-Moriya interactions constructed from general symmetry considerations reflecting the underlying system. We predict that the skyrmion phase is robust and it is present even when the system lacks the in-plane rotational symmetry. In fact, the lowered symmetry leads to increased stability of vortex-antivortex lattices with …