Atomic, Molecular and Optical Physics Commons^™

Invisibility: A Mathematical Perspective, Austin G. Gomez

CMC Senior Theses

The concept of rendering an object invisible, once considered unfathomable, can now be deemed achievable using artificial metamaterials. The ability for these advanced structures to refract waves in the negative direction has sparked creativity for future applications. Manipulating electromagnetic waves of all frequencies around an object requires precise and unique parameters, which are calculated from various mathemat- ical laws and equations. We explore the possible interpretations of these parameters and how they are implemented towards the construction of a suitable metamaterial. If carried out correctly, the wave will exit the metamaterial exhibiting the same behavior as when it had entered. …

On The Treatment Of Lumo Energies For Their Use As Descriptors, Paul Burrow, Alberto Modelli

Paul Burrow Publications

Calculated energies of lowest unoccupied molecular orbitals (LUMOs) are frequently employed as descriptors in studies of quantitative structure–activity relationships and linear free energy relationships involving electron transfer. However, the quantum chemical programs with which these are carried out, whether Hartree–Fock or density functional theory, do not treat orbitals of different character, for example, C=C π* and C-Cl σ*, consistently, nor is there consistency among different families of compounds. These problems can be ameliorated with the use of the experimental equivalent of the LUMO energy, the vertical attachment energy (VAE), or by shifting and scaling LUMO energies to a training set …

Domain Wall Roughness And Creep In Nanoscale Crystalline Ferroelectric Polymers, Zhengguo Xiao, Shashi Poddar, Stephen Ducharme, X. Hong

Stephen Ducharme Publications

We report piezo-response force microscopy studies of the static and dynamic properties of domain walls (DWs) in 11 to 36 nm thick films of crystalline ferroelectric poly(vinylidene-fluoride-trifluorethylene). The DW roughness exponent ζ ranges from 0.39 to 0.48 and the DW creep exponent µ varies from 0.20 to 0.28, revealing an unexpected effective dimensionality of ~1.5 that is independent of film thickness. Our results suggest predominantly 2D ferroelectricity in the layered polymer and we attribute the fractal dimensionality to DW deroughening due to the correlations between the in-plane and out-of-plane polarization, an effect that can be exploited to achieve high lateral …

Threshold Alignment Reversal And Circularly Polarized Fluorescence In Rotationally Resolved H2, Jack W. Maseberg, Klaus Bartschat, Timothy J. Gay

Timothy J. Gay Publications

Using H₂ and D₂ targets, we have measured the polarization of Fulcher-band fluorescence resulting from spin-polarized electron-impact excitation of vibrationally and rotationally resolved d ³Π_u→ a ³ ∑_g⁺ transitions for incident electron energies from 14.3 to 28.5 eV. Near threshold, the linear polarization P₁ descends from positive values through zero to negative values, indicating a dynamic production of M_N = 0 states. The circular polarization P₃ is measured to be nonzero, indicating the orientation of rotationally resolved molecular states. For Q-branch transitions, P₃ is consistent with theory based …

Upgrades To Nrlmol Code, Luis Basurto

Open Access Theses & Dissertations

This project consists of performing upgrades to the massively parallel NRLMOL electronic structure code in order to enhance its performance by increasing its flexibility by: a) Utilizing dynamically allocated arrays, b) Executing in a parallel environment sections of the program that were previously executed in a serial mode, c) Exploring simultaneous concurrent executions of the program through the use of an already existing MPI environment; thus enabling the simulation of larger systems than it is currently capable of performing. Also developed was a graphical user interface that will allow less experienced users to start performing electronic structure calculations by aiding …

The Classical Limit Of Quantum Optics: Not What It Seems At First Sight, Yakir Aharonov, Alonso Botero, Shmuel Nussinov, Sandu Popescu, Jeff Tollaksen, Lev Vaidman

Mathematics, Physics, and Computer Science Faculty Articles and Research

What light is and how to describe it has always been a central subject in physics. As our understanding has increased, so have our theories changed: geometrical optics, wave optics and quantum optics are increasingly sophisticated descriptions, each referring to a larger class of phenomena than its predecessor. But how exactly are these theories related? How and when wave optics reduces to geometric optics is a rather simple problem. Similarly, how quantum optics reduces to wave optics has also been considered to be a very simple business. It is not so. As we show here the classical limit of quantum …

Comment On "Density And Physical Current Density Functional Theory", Xiao-Yin Pan, Viraht Sahni

Publications and Research

In this letter to the editor, the authors comment on an earlier article they had published, "Density and Physical Current Density Functional Theory" (Pan, X.-Y. and Sahni, V. (2010), Density and physical current density functional theory. Int. J. Quantum Chem., 110: 2833–2843. doi: 10.1002/qua.22862).

A Comparison Of Three Commercially Available Contrast-Detail Phantoms And Evaluation Of The Contrast-Detail Performance Under A Range Of Instrument Settings, Jacinta Browne, Des Hickey, Ashling Mcnabb

Articles

No abstract provided.

Transparent Actuator Made With Few Layer Graphene Electrode And Dielectric Elastomer, For Variable Focus Lens, Taeseon Hwang, Hyeok-Yong Kwon, Joon-Suk Oh, Jung-Pyo Hong, Seung-Chul Hong, Youngkwan Lee, Hyouk Ryeo Choi, Kwang J. Kim, Mainul Hossain Bhuiya, Jae Do Nam

Mechanical Engineering Faculty Research

A transparent dielectric elastomer actuator driven by few-layer-graphene (FLG) electrode was experimentally investigated. The electrodes were made of graphene, which was dispersed inN-methyl-pyrrolidone. The transparent actuator was fabricated from developed FLG electrodes.The FLG electrode with its sheet resistance of 0.45 kΩ/sq (80 nm thick) was implemented to mask silicone elastomer. The developed FLG-driven actuator exhibited an optical transparency of over 57% at a wavenumber of 600 nm and produced bending displacement performance ranging from 29 to 946 μm as functions of frequency and voltage. The focus variation was clearly demonstrated under actuation to study its application-feasibility in …

Measurement Of Transparency Ratios For Protons From Short-Range Correlated Pairs, Clas Collaboration, L. B. Weinstein, K. P. Adhikari, M. J. Amaryan, H. Baghdasaryan, G. E. Dodge, C. E. Hyde, S. E. Kuhn, M. Mayer, H. Seradaryan

Physics Faculty Publications

Nuclear transparency, T_p(A), is a measure of the average probability for a struck proton to escape the nucleus without significant re-interaction. Previously, nuclear transparencies were extracted for quasi-elastic A(e,e′p) knockout of protons with momentum below the Fermi momentum, where the spectral functions are well known. In this Letter we extract a novel observable, the transparency ratio, T_p(A)/T_p(¹²C), for knockout of high-missing-momentum protons from the breakup of short-range correlated pairs (2N-SRC) in Al, Fe and Pb nuclei relative to C. The ratios were measured at momentum transfer Q² ⩾1.5(GeV/c)² and x …

Raman Spectroscopy In Nanomedicine: Current Status And Future Perspectives, Hugh Byrne, Mark Keating

Articles

Raman spectroscopy is a branch of vibration spectroscopy which is capable of probing the chemical composition of materials. Recent advances in Raman microscopy have added significantly to the range of applications which now extend from medical diagnostics to exploring interfaces between biological organisms and nanomaterials. In this review, Raman is introduced in a general context, highlighting some of the areas in which the technique has found success in the past, as well as some of the potential benefits it offers over other analytical modalities. The subset of Raman techniques which specifically probe the nanoscale, namely Surface Enhanced and Tip Enhanced …

Unresolved Question Of The 10he Ground State Resonance, Z. Kohley, J. Snyder, T. Baumann, G. Christian, P.A. Deyoung, J.E. Finck, R.A. Haring-Kaye, M. Jones, E. Lunderberg, B. Luther, S. Mosby, A. Simon, J.K. Smith, A. Spyrou, Sharon L. Stephenson, M. Thoennessen

Physics and Astronomy Faculty Publications

The group state of ¹⁰He was populated using a 2p2n-removal from a 59 MeV/u ¹⁴Be beam. The decay energy of the three body system, 8He + n + n, was measured and a resonance was observed at E = 1.60(25) MeV with a 1.8(4) MeV width. This result is in agreement with previous invariant mass spectroscopy measurements, using the ¹¹Li(-p) reaction, but is consistent with recent transfer reaction results. The proposed explanation that the difference, about 500 keV, is due to the effect of the extended halo nature of ¹¹Li in the one-proton knockout reaction is …

Investigation Of Optical Dipole Traps For Trapping Neutral Atoms For Quantum Computing, Danielle May

Physics

No abstract provided.

High-Order-Harmonic-Generation Spectroscopy With An Elliptically Polarized Laser Field, M. V. Frolov, N. L. Manakov, T. S. Sarantseva, Anthony F. Starace

Anthony F. Starace Publications

Analytic formulas describing high-order-harmonic generation (HHG) by atoms in an intense laser field with small ellipticity are obtained quantum mechanically in the tunneling limit. The results show that factorization of the HHG yield in terms of an electron wave packet and the photorecombination cross section (PRCS) is valid only for s states of a bound atomic electron, whereas the HHG yield for p states involves two different atomic parameters. For the latter case, elliptic HHG spectroscopy enables one to retrieve both the energy and angular dependence of the PRCS of the target atom, as we illustrate for the case of …

Passive Ranging Using A Dispersive Spectrometer And Optical Filters, Jacob A. Martin

Theses and Dissertations

Monocular passive ranging using atmospheric oxygen absorption has been demonstrated in the past using an FTS. These instruments are very sensitive to vibration making them di cult to use on an airborne platform. This work focuses on whether passive ranging can be done with instruments that are easier to deploy. Two potential instruments are tested and compared: a diffraction grating spectrometer and optical filters. A grating spectrometer was able to estimate range to within 5% for a static solid rocket motor ring at a distance of 910 m using the NIR absorption band of oxygen. Testing at shorter ranges produced …

A Gauge Theoretic Treatment Of Rovibrational Motion In Diatoms, Gregory Colarch

UNLV Theses, Dissertations, Professional Papers, and Capstones

The Born-Oppenheimer approximation has long been the standard approach to solving the Schrödinger equation for diatomic molecules. In it, nuclear and electronic motions are separated into "slow" and "fast" degrees of freedom and couplings between the two are ignored. The neglect of non-adiabatic couplings leads to an incomplete description of diatomic motion, and in a more refined approach, non-adiabatic couplings are uncoupled by transforming the angular momentum of the molecule and electrons into the body-fixed frame.

In this thesis we examine a "modern" form of the Born-Oppenheimer approximation by exploiting a gauge theoretic approach in a description of molecular motion. …

Hybrid Plasmonic Nanoantennas: Fabrication, Characterization, And Application, Shengjie Zhai

UNLV Theses, Dissertations, Professional Papers, and Capstones

As optical counterpart of microwave antennas, plasmonic nanoantennas are important nanoscale devices for converting propagating optical radiation into confined/enhanced electromagnetic fields. Presently, nanoantennas, with a typical size of 200-500 nm, have found their applications in bio-sensing, bio-imaging, energy harvesting, and disease cure and prevention. With the device feature size of next generation IC goes down to 22 nm or smaller, and biological/chemical sensing reaches the Gene’s level, the sizes of the corresponding nanoantennas have to be scaled down to sub-100nm level. In the literature, these sub-100nm nanoantennas are referred as deep subwavelength nanoantennas as size of such miniaturized nanoantennas is …

Threshold Effects In Strong-Field Ionization: Energy Shifts And Rydberg Structures, Katarzyna Krajewska, Ilya I. Fabrikant, Anthony F. Starace

Anthony F. Starace Publications

The behavior of strong-field ionization rates of neutral atoms in the vicinity ofmultiphoton ionization thresholds is analyzed using formal collision theory.Our approach,which accounts nonperturbatively for effects of an intense laser field, shows that the ionization rates have a nearly constant behavior below and above each multiphoton threshold and that between such thresholds there are an apparently finite number of rapid oscillations due to resonances with laser-field-modified Rydberg states. This pattern is typical for any atomic target, as we illustrate specifically for hydrogen and neon atoms. The flat behavior of the ionization yield near multiphoton thresholds gives the appearance of an …

Spectral Engineering Of Optical Fiber Preforms Through Active Nanoparticle Doping, T. Lindstrom, E. Garber, D. Edmonson, T. Hawkins, Y. Chen, G. Turri, M. Bass, J. Ballato

Publications

Europium doped alkaline earth fluoride [Eu:AEF2 (AE = Ca, Sr, Ba)] nanoparticles were synthesized and systematically incorporated into the core of modified chemical vapor deposition (MCVD)-derived silica-based preforms by solution doping. The resulting preforms were examined to determine the impact of the nanoparticles chemistry on the spectroscopic behavior of the glass. The dominant existence of Eu3+ was demonstrated in all preforms, which is in contrast to conventional solution doped preforms employing dissolved europium salts where Eu2+ is primarily observed. Raman spectroscopy and fluorescence lifetime measurements indicated that the nanoparticles composition is effective in controlling, at a local chemical and structural …

Al6h18: A Baby Crystal Of Γ -Alh3, B. Kiran, Anil K. Kandalam, Jing Xu, Y. H. Ding, M. Sierka, K. H. Bowen, H. Schnöckel

Physics & Engineering Faculty Publications

No abstract provided.