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Articles 2131 - 2160 of 2426
Full-Text Articles in Atmospheric Sciences
Intercontinental Transport Of Pollution Manifested In The Variability And Seasonal Trend Of Springtime O3 At Northern Middle And High Latitudes, Yuhang Wang, Changsub Shim, Nicola J. Blake, D R. Blake, Yunsoo Choi, Brian Ridley, Jack E. Dibb, Anthony Wimmers, Jennie Moody, F Flocke, Andrew Weinheimer, R. Talbot, Elliot Atlas
Intercontinental Transport Of Pollution Manifested In The Variability And Seasonal Trend Of Springtime O3 At Northern Middle And High Latitudes, Yuhang Wang, Changsub Shim, Nicola J. Blake, D R. Blake, Yunsoo Choi, Brian Ridley, Jack E. Dibb, Anthony Wimmers, Jennie Moody, F Flocke, Andrew Weinheimer, R. Talbot, Elliot Atlas
Earth Sciences
Observations (0–8 km) from the Tropospheric Ozone Production about the Spring Equinox (TOPSE) experiment are analyzed to examine air masses contributing to the observed variability of springtime O3 and its seasonal increase at 40°–85°N over North America. Factor analysis using the positive matrix factorization and principal component analysis methods is applied to the data set with 14 chemical tracers (O3, NOy, PAN, CO, CH4, C2H2, C3H8, CH3Cl, CH3Br, C2Cl4, CFC-11, HCFC-141B, Halon-1211, and 7Be) and one …
Chemical Composition Of Asian Continental Outflow Over The Western Pacific: Results From Transport And Chemical Evolution Over The Pacific (Trace-P), R. S. Russo, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, C. Jordan, H Fuelberg, G W. Sachse, M A. Avery, S Vay, D R. Blake, N J. Blake, E L. Atlas, A Fried, S T. Sandholm, D Tan, H B. Singh, J Snow, B J. Heikes
Chemical Composition Of Asian Continental Outflow Over The Western Pacific: Results From Transport And Chemical Evolution Over The Pacific (Trace-P), R. S. Russo, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, C. Jordan, H Fuelberg, G W. Sachse, M A. Avery, S Vay, D R. Blake, N J. Blake, E L. Atlas, A Fried, S T. Sandholm, D Tan, H B. Singh, J Snow, B J. Heikes
Earth Sciences
We characterize the chemical composition of Asian continental outflow observed during the NASA Transport and Chemical Evolution over the Pacific (TRACE-P) mission during February–April 2001 in the western Pacific using data collected on the NASA DC-8 aircraft. A significant anthropogenic impact was present in the free troposphere and as far east as 150°E longitude reflecting rapid uplift and transport of continental emissions. Five-day backward trajectories were utilized to identify five principal Asian source regions of outflow: central, coastal, north-northwest (NNW), southeast (SE), and west-southwest (WSW). The maximum mixing ratios for several species, such as CO, C2Cl4, …
Large-Scale Ozone And Aerosol Distributions, Air Mass Characteristics, And Ozone Fluxes Over The Western Pacific Ocean In Late Winter/Early Spring, Edward V. Browell, Marta Fenn, Carolyn Butler, William B. Grant, Vincent G. Brackett, Jonathan Hair, Melody A. Avery, Yuanlong Hu, Reginald E. Newell, H Fuelberg, Daniel J. Jacob, Bruce E. Anderson, Elliot Atlas, D R. Blake, William H. Brune, Jack E. Dibb, A Fried, B J. Heikes, G W. Sachse, S T. Sandholm, Hanwant B. Singh, R. Talbot, S Vay, Rodney J. Weber, Karen B. Bartlett
Large-Scale Ozone And Aerosol Distributions, Air Mass Characteristics, And Ozone Fluxes Over The Western Pacific Ocean In Late Winter/Early Spring, Edward V. Browell, Marta Fenn, Carolyn Butler, William B. Grant, Vincent G. Brackett, Jonathan Hair, Melody A. Avery, Yuanlong Hu, Reginald E. Newell, H Fuelberg, Daniel J. Jacob, Bruce E. Anderson, Elliot Atlas, D R. Blake, William H. Brune, Jack E. Dibb, A Fried, B J. Heikes, G W. Sachse, S T. Sandholm, Hanwant B. Singh, R. Talbot, S Vay, Rodney J. Weber, Karen B. Bartlett
Earth Sciences
Large-scale measurements of ozone (O3) and aerosol distributions were made from the NASA DC-8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) field experiment conducted in February–April 2001. Remote measurements were made with an airborne lidar to provide O3 and multiple-wavelength aerosol backscatter profiles from near the surface to above the tropopause along the flight track. In situ measurements of O3, aerosols, and a wide range of trace gases were made onboard the DC-8. Five-day backward trajectories were used in conjunction with the O3 and aerosol distributions on each flight to …
Reactive Nitrogen In Asian Continental Outflow Over The Western Pacific: Results From The Nasa Transport And Chemical Evolution Over The Pacific (Trace-P) Airborne Mission, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, R. S. Russo, S T. Sandholm, D Tan, H B. Singh, D R. Blake, N J. Blake, Elliot Atlas, G W. Sachse, C. Jordan, Melody A. Avery
Reactive Nitrogen In Asian Continental Outflow Over The Western Pacific: Results From The Nasa Transport And Chemical Evolution Over The Pacific (Trace-P) Airborne Mission, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, R. S. Russo, S T. Sandholm, D Tan, H B. Singh, D R. Blake, N J. Blake, Elliot Atlas, G W. Sachse, C. Jordan, Melody A. Avery
Earth Sciences
We present here results for reactive nitrogen species measured aboard the NASA DC-8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) mission. The large-scale distributions total reactive nitrogen (NOy,sum = NO + NO2 + HNO3 + PAN + C1–C5alkyl nitrates) and O3 and CO were better defined in the boundary layer with significant degradation of the relationships as altitude increased. Typically, NOy,sum was enhanced over background levels of ∼260 pptv by 20-to-30-fold. The ratio C2H2/CO had values of 1–4 at altitudes up to 10 …
Summary Of Measurement Intercomparisons During Trace-P, Fred Eisele, Lee Mauldin, C A. Cantrell, M Zondlo, E C. Apel, A Fried, J Walega, R E. Shetter, Barry Lefer, F Flocke, Andrew Weinheimer, M A. Avery, S Vay, G W. Sachse, J Podolske, G S. Diskin, J D. Barrick, H B. Singh, William H. Brune, H Harder, M Martinez, A R. Bandy, D C. Thornton, B J. Heikes, Y Kondo, D Riemer, S T. Sandholm, R. Talbot, Jack E. Dibb
Summary Of Measurement Intercomparisons During Trace-P, Fred Eisele, Lee Mauldin, C A. Cantrell, M Zondlo, E C. Apel, A Fried, J Walega, R E. Shetter, Barry Lefer, F Flocke, Andrew Weinheimer, M A. Avery, S Vay, G W. Sachse, J Podolske, G S. Diskin, J D. Barrick, H B. Singh, William H. Brune, H Harder, M Martinez, A R. Bandy, D C. Thornton, B J. Heikes, Y Kondo, D Riemer, S T. Sandholm, R. Talbot, Jack E. Dibb
Earth Sciences
The NASA DC-8 and P-3B aircraft flew within about a kilometer or less of each other on three occasions during the Transport and Chemical Evolution Over the Pacific (TRACE-P) campaign in order to intercompare similar measurements on the two aircraft. The first and last intercomparisons were in relatively remote marine environments during transits to and from Asia. The first began with a boundary layer measurement followed by an ascent to 3 km. The second set of intercomparisons was at a fixed altitude of about 5.2 km off the coast of Japan, also in relatively clean air. Finally, the third measurement …
Comparison Between Analytical Probabilistic And Computer Simulation Models, Using Current Design Examples, Barry A. Palynchuk Phd
Comparison Between Analytical Probabilistic And Computer Simulation Models, Using Current Design Examples, Barry A. Palynchuk Phd
Barry A. Palynchuk PhD
Closed form analytical expressions have been developed to solve several basic problems related to the hydrologic design of storm water management facilities. The collection of these analytical expressions is referred to as the Analytical Probabilistic Storm Water Models (APSWM). APSWM can be used as an alternative to the design storm simulation models in the design and analysis of storm water management facilities. In this paper, a comparison is made between APSWM and design storm simulation models as applied to an actual design case. Conventional outputs such as runoff volume, peak discharge, and peak discharge from detention ponds are reviewed and …
Chemical Characterization Of Ambient Aerosol Collected During The Northeast Monsoon Season Over The Arabian Sea: Labile-Fe(Ii) And Other Trace Metals, Anne M. Johansen, Michael R. Hoffmann
Chemical Characterization Of Ambient Aerosol Collected During The Northeast Monsoon Season Over The Arabian Sea: Labile-Fe(Ii) And Other Trace Metals, Anne M. Johansen, Michael R. Hoffmann
All Faculty Scholarship for the College of the Sciences
Ambient aerosol samples were collected over the Arabian Sea during the month of March of 1997, aboard the German R/V Sonne, as part of the German Joint Global Ocean Flux Study (JGOFS) project. This is the third study in a series of analogous measurements taken over the Arabian Sea during different seasons of the monsoon. Dichotomous high‐volume collector samples were analyzed for ferrous iron immediately after collection, while trace metals, anions, and cations were determined upon return to the laboratory. The main crustal component was geochemically well represented by the average crustal composition and amounted to 5.94 ± 3.08 …
Antarctic Oversnow Traverse-Based Southern Hemisphere Climate Reconstruction, Paul Andrew Mayewski
Antarctic Oversnow Traverse-Based Southern Hemisphere Climate Reconstruction, Paul Andrew Mayewski
Earth Science Faculty Scholarship
On 2 January 2003, the U.S. component of the International Trans Antarctic Scientific Expedition (U.S. ITASE) (Figure 1) arrived at the South Pole after completing more than 5000 km of oversnow traverses that included much of west Antarctica and a portion of east Antarctica (Figure 2). During the traverses, which were performed from 1999 through 2003, U.S. ITASE focused on collecting data that will allow the reconstruction of sub-annual scale climate variability and changes in the chemistry of the atmosphere over the last 200+ years.
ITASE is a multi-disciplinary research program supported by 19 nations and endorsed by the Scientific …
Be-10/Be-7 Tracer Of Atmospheric Transport And Stratosphere-Troposphere Exchange, C. Jordan, Jack E. Dibb, R C. Finkel
Be-10/Be-7 Tracer Of Atmospheric Transport And Stratosphere-Troposphere Exchange, C. Jordan, Jack E. Dibb, R C. Finkel
Earth Sciences
The 10Be/7Be ratio is a sensitive tracer of atmospheric transport and stratosphere-troposphere exchange (STE). Data from five NASA aircraft field missions (PEM: West A and B, Tropics A; SONEX; and SUCCESS) have been assembled to produce the largest data set of 10Be,7Be, and their ratio collected to date (>300 samples). Ratios near 0.60 are indicative of tropospheric air with little stratospheric influence, while higher ratios are found in stratospheric air. Samples from the lower stratosphere were all collected within 2.5 km of the tropopause and had ratios >1.27. Of these lower stratosphere samples …
Measurement Of Proton Transfer Reaction Rates In A Microwave Cavity Discharge Flowing Afterglow, George M. Brooke Iv
Measurement Of Proton Transfer Reaction Rates In A Microwave Cavity Discharge Flowing Afterglow, George M. Brooke Iv
Physics Theses & Dissertations
The reaction rate coefficients between the hydronium ion and the molecules ethene (C2H4), propene (C3H6), 1-butene (C4H8) and hydrogen sulfide (H2S) were measured at 296 K. The measured reaction rates were compared to collision rates calculated using average dipole orientation (ADO) theory. Reaction efficiency depends primarily upon the proton affinity of the molecules. All the measurements were obtained using the newly developed microwave cavity discharge flowing afterglow (MCD-FA) apparatus. This device uses an Asmussen-type microwave cavity discharge ion source that is …
Data Mining Atmospheric/Oceanic Parameters In The Design Of A Long-Range Nephelometric Forecast Tool, Richard F. Benz
Data Mining Atmospheric/Oceanic Parameters In The Design Of A Long-Range Nephelometric Forecast Tool, Richard F. Benz
Theses and Dissertations
The Department of Defense calls for long-range forecasts to aid in the planning of operations. The goal of this research was to explore the feasibility of predicting, one month in advance, the total monthly cloud cover over the country of Afghanistan. In an attempt to reach this goal, the following objectives were achieved: (1) climatological synoptic study of Afghanistan; (2) survey of Real Time Nephanalysis, outgoing longwave radiation (OLR), and surface observational data; (3) examination of teleconnection indices and sea surface temperatures; (4) standard statistical analysis for prediction; and (5) classification tree analysis (CART), In addition, due to current world …
Stratospheric Influence On The Northern North American Free Troposphere During Topse: 7be As A Stratospheric Tracer, Jack E. Dibb, R. Talbot, Eric Scheuer, Garry Seid, Linsey J. Debell, Barry Lefer, Brian Ridley
Stratospheric Influence On The Northern North American Free Troposphere During Topse: 7be As A Stratospheric Tracer, Jack E. Dibb, R. Talbot, Eric Scheuer, Garry Seid, Linsey J. Debell, Barry Lefer, Brian Ridley
Earth Sciences
We use 7Be, with HNO3 and O3, to identify air masses sampled from the NCAR C-130 during TOPSE that retained clear evidence of stratospheric influence. A total of 43 such air masses, spread fairly evenly across the February to May sampling period, and 40°N–86°N latitude range, were encountered. South of 55°N, nearly all clear stratospheric influence was restricted to altitudes above 6 km. At higher latitudes stratospherically influenced air masses were encountered as low as 2 km. Approximately 12% of all TOPSE sampling time at altitudes above 2 km was spent in stratospherically impacted air, above …
Effect Of Sulfate Aerosol On Tropospheric Nox And Ozone Budgets: Model Simulations And Topse Evidence, Xuexi Tie, L K. Emmons, Larry Horowitz, Guy Brasseur, Brian Ridley, Elliot Atlas, Craig Stround, Peter Hess, Andrzej Klonecki, Sasha Madronich, R. Talbot, Jack E. Dibb
Effect Of Sulfate Aerosol On Tropospheric Nox And Ozone Budgets: Model Simulations And Topse Evidence, Xuexi Tie, L K. Emmons, Larry Horowitz, Guy Brasseur, Brian Ridley, Elliot Atlas, Craig Stround, Peter Hess, Andrzej Klonecki, Sasha Madronich, R. Talbot, Jack E. Dibb
Earth Sciences
The distributions of NOx and O3 are analyzed during TOPSE (Tropospheric Ozone Production about the Spring Equinox). In this study these data are compared with the calculations of a global chemical/transport model (Model for OZone And Related chemical Tracers (MOZART)). Specifically, the effect that hydrolysis of N2O5 on sulfate aerosols has on tropospheric NOx and O3 budgets is studied. The results show that without this heterogeneous reaction, the model significantly overestimates NOx concentrations at high latitudes of the Northern Hemisphere (NH) in winter and spring in comparison to the observations during TOPSE; …
Tunable Diode Laser Measurements Of Formaldehyde During The Topse 2000 Study: Distributions, Trends, And Model Comparisons, A Fried, Yuhang Wang, C A. Cantrell, B Wert, J Walega, Brian Ridley, Elliot Atlas, R E. Shetter, Barry Lefer, Michael T. Coffey, James W. Hannigan, D R. Blake, N J. Blake, Simone Meinardi, R. Talbot, Jack E. Dibb, Eric Scheuer, Oliver Wingenter, J Snow, B J. Heikes, Dieter Ehhalt
Tunable Diode Laser Measurements Of Formaldehyde During The Topse 2000 Study: Distributions, Trends, And Model Comparisons, A Fried, Yuhang Wang, C A. Cantrell, B Wert, J Walega, Brian Ridley, Elliot Atlas, R E. Shetter, Barry Lefer, Michael T. Coffey, James W. Hannigan, D R. Blake, N J. Blake, Simone Meinardi, R. Talbot, Jack E. Dibb, Eric Scheuer, Oliver Wingenter, J Snow, B J. Heikes, Dieter Ehhalt
Earth Sciences
Airborne measurements of formaldehyde (CH2O) were acquired employing tunable diode laser absorption spectroscopy (TDLAS) during the 2000 Tropospheric Ozone Production About the Spring Equinox (TOPSE) study. This study consisted of seven deployments spanning the time period from 4 February to 23 May 2000 and covered a wide latitudinal band from 40°N to 85°N. The median measured CH2O concentrations, with a few exceptions, did not show any clear temporal trends from February to May in each of five altitude and three latitude bins examined. Detailed measurement–model comparisons were carried out using a variety of approaches employing two …
An Estimate Of The Stratospheric Contribution To Springtime Tropospheric Ozone Maxima Using Topse Measurements And Beryllium-7 Simulations, Dale J. Allen, Jack E. Dibb, Brian Ridley, Kenneth E. Pickering, R. Talbot
An Estimate Of The Stratospheric Contribution To Springtime Tropospheric Ozone Maxima Using Topse Measurements And Beryllium-7 Simulations, Dale J. Allen, Jack E. Dibb, Brian Ridley, Kenneth E. Pickering, R. Talbot
Earth Sciences
Measurements of tropospheric ozone (O3) between 30°N and 70°N show springtime maxima at remote locations. The contribution of seasonal changes in stratosphere–troposphere exchange (STE) to these maxima was investigated using measurements from the Tropospheric Ozone Production about the Spring Equinox Experiment (TOPSE) campaign and the beryllium-7 (7Be) distribution from a calculation driven by fields from the Goddard Earth Observing System Data Assimilation System (GEOS DAS). Comparison with TOPSE measurements revealed that upper tropospheric model-calculated 7Be mixing ratios were reasonable (a change from previous calculations) but that lower tropospheric mixing ratios were too low most likely …
Coupled Evolution Of Brox-Clox-Hox-Nox Chemistry During Bromine-Catalyzed Ozone Depletion Events In The Arctic Boundary Layer, M J. Evans, D J. Jacob, E L. Atlas, C A. Cantrell, Fred Eisele, F Flocke, A Fried, R L. Mauldin, Brian Ridley, B Wert, R. Talbot, D R. Blake, B J. Heikes, J Snow, J Walega, Andrew Weinheimer, Jack E. Dibb
Coupled Evolution Of Brox-Clox-Hox-Nox Chemistry During Bromine-Catalyzed Ozone Depletion Events In The Arctic Boundary Layer, M J. Evans, D J. Jacob, E L. Atlas, C A. Cantrell, Fred Eisele, F Flocke, A Fried, R L. Mauldin, Brian Ridley, B Wert, R. Talbot, D R. Blake, B J. Heikes, J Snow, J Walega, Andrew Weinheimer, Jack E. Dibb
Earth Sciences
Extensive chemical characterization of ozone (O3) depletion events in the Arctic boundary layer during the TOPSE aircraft mission in March–May 2000 enables analysis of the coupled chemical evolution of bromine (BrOx), chlorine (ClOx), hydrogen oxide (HOx) and nitrogen oxide (NOx) radicals during these events. We project the TOPSE observations onto an O3 chemical coordinate to construct a chronology of radical chemistry during O3 depletion events, and we compare this chronology to results from a photochemical model simulation. Comparison of observed trends in ethyne (oxidized by Br) and ethane …
Investigations Into Free Tropospheric New Particle Formation In The Central Canadian Arctic During The Winter/Spring Transition As Part Of Topse, R J. Weber, D A. Orsini, B Wang, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, R L. Mauldin, E Kosciuch, C A. Cantrell, Fred Eisele
Investigations Into Free Tropospheric New Particle Formation In The Central Canadian Arctic During The Winter/Spring Transition As Part Of Topse, R J. Weber, D A. Orsini, B Wang, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, R L. Mauldin, E Kosciuch, C A. Cantrell, Fred Eisele
Earth Sciences
In this paper, we investigate the role of in situ new particle production in the central Canadian sub-Arctic and Arctic as part of the TOPSE experiment. Airborne measurements conducted primarily in the free troposphere were made from 50° to 90°W longitude and 60° to 85°N latitude during the period from February to May 2000. Data pertinent to this paper include 3–4 nm diameter (Dp) particles, ultrafine condensation nuclei (Dp > 3 nm), fine particles (0.2 < Dp < 3 μm), and the possible nucleation precursor, sulfuric acid, and its precursor, sulfur dioxide. For data averaged over this period, most species showed little evidence for a latitudinal trend. Fine aerosol number concentrations, however, showed a slight increase with latitude. The evolution of various species concentrations over the period of the study show that fine particles also had a consistent temporal trend, increasing at all altitudes from February to May, whereas sulfur dioxide at the surface tended to peak in late March. Ultrafine condensation nuclei and 3–4 nm particles showed no temporal trends. Little evidence for in situ new particle production was observed during the study, except for one atypical event where SO2concentrations were 3.5 ppbv, 2 orders of magnitude higher than typical levels. This paper cannot address the question of whether the observed condensation nuclei were …
Ozone Depletion Events Observed In The High Latitude Surface Layer During The Topse Aircraft Program, Brian Ridley, Elliot Atlas, D Montzka, Edward V. Browell, C A. Cantrell, D R. Blake, N J. Blake, L Cinquini, Michael T. Coffey, L K. Emmons, Ronald C. Cohen, Russell J. Deyoung, Jack E. Dibb, Fred Eisele, F Flocke, A Fried, F E. Grahek, William B. Grant, Jonathan Hair, James W. Hannigan, B J. Heikes, Barry Lefer, R L. Mauldin, Jennie Moody, R E. Shetter, J Snow, R. Talbot, J A. Thornton, J Walega, Andrew Weinheimer, B Wert, Anthony Wimmers
Ozone Depletion Events Observed In The High Latitude Surface Layer During The Topse Aircraft Program, Brian Ridley, Elliot Atlas, D Montzka, Edward V. Browell, C A. Cantrell, D R. Blake, N J. Blake, L Cinquini, Michael T. Coffey, L K. Emmons, Ronald C. Cohen, Russell J. Deyoung, Jack E. Dibb, Fred Eisele, F Flocke, A Fried, F E. Grahek, William B. Grant, Jonathan Hair, James W. Hannigan, B J. Heikes, Barry Lefer, R L. Mauldin, Jennie Moody, R E. Shetter, J Snow, R. Talbot, J A. Thornton, J Walega, Andrew Weinheimer, B Wert, Anthony Wimmers
Earth Sciences
During the Tropospheric Ozone Production about the Spring Equinox (TOPSE) aircraft program, ozone depletion events (ODEs) in the high latitude surface layer were investigated using lidar and in situ instruments. Flight legs of 100 km or longer distance were flown 32 times at 30 m altitude over a variety of regions north of 58° between early February and late May 2000. ODEs were found on each flight over the Arctic Ocean but their occurrence was rare at more southern latitudes. However, large area events with depletion to over 2 km altitude in one case were found as far south as …
Seasonal Distributions Of Fine Aerosol Sulfate In The North American Arctic Basin During Topse, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, Barry Lefer
Seasonal Distributions Of Fine Aerosol Sulfate In The North American Arctic Basin During Topse, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, Barry Lefer
Earth Sciences
We used the mist chamber/ion chromatography technique to quantify fine aerosol SO4=(<2.7 μm) in the Arctic during the Tropospheric Ozone Production about the Spring Equinox Experiment (TOPSE) with about 2.5 min time resolution. Our effective sample area ranged from 50° to 86°N and 53° to 100°W. The seasonal evolution of fine aerosol sulfate in the Arctic troposphere during TOPSE was consistent with the phenomenon of Arctic haze. Arctic haze has been attributed to pollution from sources in the Arctic and pollution transported meridionally along stable isentropes into the Arctic in geographically broad but vertically narrow bands. These layers became more prevalent at higher altitudes as the season progressed toward summer, and the relevant isentropes are not held so close to the surface. Mean fine particle SO4= mixing ratios during TOPSE in February below 1000 m were elevated (112 pptv) and highly variable (between 28 and 290 pptv) but were significantly lower at higher altitudes (about 40 pptv). As the season progressed, elevated mixing ratios and higher variability were observed at higher altitudes, up to 7 km. In May, mixing ratios at the lowest altitudes declined but still remained higher than in February at all altitudes. The high variability in our measurements likely reflects the vertical heterogeneity of the wintertime …2.7>
Steady State Free Radical Budgets And Ozone Photochemistry During Topse, C A. Cantrell, Lee Mauldin, M Zondlo, Fred Eisele, E Kosciuch, R E. Shetter, Barry Lefer, S R. Hall, T L. Campos, Brian Ridley, J Walega, A Fried, B Wert, F Flocke, Andrew Weinheimer, James W. Hannigan, Michael T. Coffey, Elliot Atlas, S Stephens, B J. Heikes, J Snow, D R. Blake, N J. Blake, A Katzenstein, J Lopez, Edward V. Browell, Jack E. Dibb, Eric Scheuer, Garry Seid, R. Talbot
Steady State Free Radical Budgets And Ozone Photochemistry During Topse, C A. Cantrell, Lee Mauldin, M Zondlo, Fred Eisele, E Kosciuch, R E. Shetter, Barry Lefer, S R. Hall, T L. Campos, Brian Ridley, J Walega, A Fried, B Wert, F Flocke, Andrew Weinheimer, James W. Hannigan, Michael T. Coffey, Elliot Atlas, S Stephens, B J. Heikes, J Snow, D R. Blake, N J. Blake, A Katzenstein, J Lopez, Edward V. Browell, Jack E. Dibb, Eric Scheuer, Garry Seid, R. Talbot
Earth Sciences
A steady state model, constrained by a number of measured quantities, was used to derive peroxy radical levels for the conditions of the Tropospheric Ozone Production about the Spring Equinox (TOPSE) campaign. The analysis is made using data collected aboard the NCAR/NSF C-130 aircraft from February through May 2000 at latitudes from 40° to 85°N, and at altitudes from the surface to 7.6 km. HO2 + RO2 radical concentrations were measured during the experiment, which are compared with model results over the domain of the study showing good agreement on the average. Average measurement/model ratios are 1.04 (σ …
Springtime Photochemistry At Northern Mid And High Latitudes, Yuhang Wang, Brian Ridley, A Fried, C A. Cantrell, D D. Davis, Gao Chen, J Snow, B J. Heikes, R. Talbot, Jack E. Dibb, F Flocke, Andrew Weinheimer, N J. Blake, D R. Blake, R E. Shetter, Barry Lefer, Elliot Atlas, Michael T. Coffey, J Walega, B Wert
Springtime Photochemistry At Northern Mid And High Latitudes, Yuhang Wang, Brian Ridley, A Fried, C A. Cantrell, D D. Davis, Gao Chen, J Snow, B J. Heikes, R. Talbot, Jack E. Dibb, F Flocke, Andrew Weinheimer, N J. Blake, D R. Blake, R E. Shetter, Barry Lefer, Elliot Atlas, Michael T. Coffey, J Walega, B Wert
Earth Sciences
Physical and chemical properties of the atmosphere at 0–8 km were measured during the Tropospheric Ozone Production about the Spring Equinox (TOPSE) experiments from February to May 2000 at mid (40°–60°N) and high latitudes (60°–80°N). The observations were analyzed using a diel steady state box model to examine HOx and O3 photochemistry during the spring transition period. The radical chemistry is driven primarily by photolysis of O3 and the subsequent reaction of O(1D) and H2O, the rate of which increases rapidly during spring. Unlike in other tropospheric experiments, observed H2O2 …
Near-Surface Currents In Desoto Canyon (1997–99): Comparison Of Current Meters, Satellite Observation, And Model Simulation, Dong-Ping Wang, Lie-Yauw Oey, Tal Ezer, Peter Hamilton
Near-Surface Currents In Desoto Canyon (1997–99): Comparison Of Current Meters, Satellite Observation, And Model Simulation, Dong-Ping Wang, Lie-Yauw Oey, Tal Ezer, Peter Hamilton
CCPO Publications
This study evaluates a data-assimilated model simulation of near-surface circulation in DeSoto Canyon (DSC), Gulf of Mexico, with emphasis on analyzing moored current-meter observations and comparing them with satellite data and model results. The study period is for two years from April 1997 to April 1999. The model results are from a high-resolution Gulf of Mexico model forced by analyzed wind and surface heat flux. Two types of data are used to deduce near-surface circulation: moored current meters at 13 locations in the DSC, and satellite sea level anomaly. The moored currents are mapped through multivariate objective analysis to produce …
Ozone, Aerosol, Potential Vorticity, And Trace Gas Trends Observed At High-Latitudes Over North America From February To May 2000, Edward V. Browell, Jonathan Hair, Carolyn Butler, William B. Grant, Russell J. Deyoung, Marta Fenn, Vincent G. Brackett, Marian B. Clayton, Lorraine A. Brasseur, David B. Harper, Brian Ridley, Andrzej Klonecki, Peter Hess, L K. Emmons, Xuexi Tie, Elliot Atlas, C A. Cantrell, Anthony Wimmers, D R. Blake, Michael T. Coffey, James W. Hannigan, Jack E. Dibb, R. Talbot, F Flocke, Andrew Weinheimer, A Fried, B Wert, J Snow, Barry Lefer
Ozone, Aerosol, Potential Vorticity, And Trace Gas Trends Observed At High-Latitudes Over North America From February To May 2000, Edward V. Browell, Jonathan Hair, Carolyn Butler, William B. Grant, Russell J. Deyoung, Marta Fenn, Vincent G. Brackett, Marian B. Clayton, Lorraine A. Brasseur, David B. Harper, Brian Ridley, Andrzej Klonecki, Peter Hess, L K. Emmons, Xuexi Tie, Elliot Atlas, C A. Cantrell, Anthony Wimmers, D R. Blake, Michael T. Coffey, James W. Hannigan, Jack E. Dibb, R. Talbot, F Flocke, Andrew Weinheimer, A Fried, B Wert, J Snow, Barry Lefer
Earth Sciences
Ozone (O3) and aerosol scattering ratio profiles were obtained from airborne lidar measurements on thirty-eight flights over seven deployments covering the latitudes of 40°–85°N between 4 February and 23 May 2000 as part of the Tropospheric Ozone Production about the Spring Equinox (TOPSE) field experiment. Each deployment started from Broomfield, Colorado, with bases in Churchill, Canada, and on most deployments, Thule Air Base, Greenland. Nadir and zenith lidar O3 measurements were combined with in situ O3measurements to produce vertically continuous O3 profiles from near the surface to above the tropopause. Potential vorticity (PV) distributions …
New Evidence For Enhanced Ocean Primary Production Triggered By Tropical Cyclone, I. Lin, W. Timothy Liu, Chun-Chieh Wu, George T. F. Wong, Chuanmin Hu, Zhiqiang Chen, Wen-Der Liang, Yih Yang, Kon-Kee Liu
New Evidence For Enhanced Ocean Primary Production Triggered By Tropical Cyclone, I. Lin, W. Timothy Liu, Chun-Chieh Wu, George T. F. Wong, Chuanmin Hu, Zhiqiang Chen, Wen-Der Liang, Yih Yang, Kon-Kee Liu
OES Faculty Publications
[1] New evidence based on recent satellite data is presented to provide a rare opportunity in quantifying the long-speculated contribution of tropical cyclones to enhance ocean primary production. In July 2000, moderate cyclone Kai-Tak passed over the South China Sea (SCS). During its short 3-day stay, Kai-Tak triggered an average 30-fold increase in surface chlorophyll-a concentration. The estimated carbon fixation resulting from this event alone is 0.8 Mt, or 2-4% of SCS's annual new production. Given an average of 14 cyclones passing over the SCS annually, we suggest the long-neglected contribution of tropical cyclones to SCS's annual new production may …
Net Surface Flux Budget Over Tropical Oceans Estimated From The Tropical Rainfall Measuring Mission (Trmm), Tai-Fang Fan
Net Surface Flux Budget Over Tropical Oceans Estimated From The Tropical Rainfall Measuring Mission (Trmm), Tai-Fang Fan
Dissertations, Theses, and Masters Projects
No abstract provided.
Diurnal Variation In The Basal Emission Rate Of Isoprene, Jennifer L. Funk, Clive G. Jones, Christine J. Baker, Heather M. Fuller, Christian P. Giardina, Manuel T. Lerdau
Diurnal Variation In The Basal Emission Rate Of Isoprene, Jennifer L. Funk, Clive G. Jones, Christine J. Baker, Heather M. Fuller, Christian P. Giardina, Manuel T. Lerdau
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Isoprene is emitted from numerous plant species and profoundly influences tropospheric chemistry. Due to the short lifetime of isoprene in the atmosphere, developing an understanding of emission patterns at small time scales is essential for modeling regional atmospheric chemistry processes. Previous studies suggest that diurnal fluctuations in isoprene emission may be substantial, leading to inaccuracies in emission estimates at larger scales. We examined diurnal patterns in the basal emission rate of isoprene in red oak (Quercus rubra), eastern cottonwood (Populus deltoides), and eucalyptus (Eucalyptus saligna) and the influence of light and temperature on the magnitude of these diurnal patterns. Maximum …
The Chesapeake Bay : A Synopsis, William J. Hargis Jr.
Near-Real-Time Measurement Of Sea-Salt Aerosol During The Seas Campaign: Comparison Of Emission-Based Sodium Detection With An Aerosol Volatility Technique, P. Campuzano-Jost, Catherine D. Clark, H. Maring, D. S. Covert, S. Howell, V. Kapustin, K. A. Clarke, E. S. Saltzman, A. J. Hynes
Near-Real-Time Measurement Of Sea-Salt Aerosol During The Seas Campaign: Comparison Of Emission-Based Sodium Detection With An Aerosol Volatility Technique, P. Campuzano-Jost, Catherine D. Clark, H. Maring, D. S. Covert, S. Howell, V. Kapustin, K. A. Clarke, E. S. Saltzman, A. J. Hynes
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
The first deployment of an emission-based aerosol sodium detector (ASD), designed to chemically characterize marine aerosols on a near-real-time basis, is reported. Deployment occurred as part of the Shoreline Environment Aerosol Study ( SEAS) from 16 April to 1 May 2000 at Bellows Air Force Base on the east side of Oahu, where the University of Hawaii's Department of Oceanography maintains a tower for aerosol measurements. The instrument was operated in size-unsegregated mode and measurements were made that included two extended continuous sampling periods, each of which lasted for 24 h. During this time, the ASD was compared with measurements …
A Simulation Study Of Space-Based Observations Of Gravity Waves In The Airglow Using Observed Aloha-93 Wave Parameters, Michael P. Hickey Ph.D., J. S. Brown
A Simulation Study Of Space-Based Observations Of Gravity Waves In The Airglow Using Observed Aloha-93 Wave Parameters, Michael P. Hickey Ph.D., J. S. Brown
Publications
We use gravity wave parameters derived from the ALOHA-93 campaign to model four gravity waves in airglow emissions as observed from the ground to numerically predict whether these waves could have been observed from space. In spite of encountering critical levels, some waves may still be observed in the airglow provided the critical level lies within the airglow emission region. One of the four waves experiences a critical level in the lower region of an airglow layer such that the disturbance to the volume emission rate would be effectively limited to a short distance along a satellite line of sight. …
A 700-Year Record Of Atmospheric Circulation Developed From The Law Dome Ice Core, East Antarctica, Joseph M. Souney Jr, Paul A. Mayewski, Ian D. Goodwin, David Meeker, Vin Morgan, Mark Aj Curran, Tas D. Van Ommen, Anne S. Palmer
A 700-Year Record Of Atmospheric Circulation Developed From The Law Dome Ice Core, East Antarctica, Joseph M. Souney Jr, Paul A. Mayewski, Ian D. Goodwin, David Meeker, Vin Morgan, Mark Aj Curran, Tas D. Van Ommen, Anne S. Palmer
Earth Systems Research Center
A 700-year, high-resolution, multivariate ice core record from Dome Summit South (DSS) (66°46′S, 112°48′E; 1370 m), Law Dome, is used to investigate sea level pressure (SLP) variability in the region of East Antarctica. Empirical orthogonal function (EOF) analysis reveals that the first EOF (LDEOF1) of the combined glaciochemical, oxygen isotope ratio, and accumulation rate record from DSS represents most of the variability in sea salt seen in the record. LDEOF1 is positively correlated (at least 95% confidence level) to instrumental June mean SLP across most of East Antarctica. Over the last 700 years, LDEOF1 levels at Law Dome were the …