Atmospheric Sciences Commons^™

Data Supporting The Paper "Enhancing Turbulent Mixing And Microphysical Uniformity In A Tall Convection-Cloud Chamber Through Idealized Heterogeneity Of Boundaries", Lois Thomas, Fan Yang, Aaron Wang, Mikhail Ovchinnikov, Kyle G. Pressel, Raymond Shaw

Michigan Tech Research Data

A large convection cloud chamber has been proposed for exploring aerosol–cloud–drizzle interactions under well-controlled turbulent conditions. Recent theoretical and numerical studies suggest that a convection cloud chamber with two heated and two cooled sidewalls can significantly enhance the liquid water content and thus benefit drizzle initiation. However, a chamber with such a sidewall configuration develops stable stratification and extremely weak turbulence therein. In this study, we conduct large-eddy simulations of a tall convection chamber with five different sidewall configurations consisting of alternating warm and cold patches. For each configuration, the total surface area of warm patches equals that of cold …

High-Resolution Temperature Profiling In The Pi Chamber: Variability Of Statistical Properties Of Temperature Fluctuations, Robert Grosz, Kamal Kant Chandrakar, Raymond A. Shaw, Jesse C. Anderson, Will Cantrell, Szymon P. Malinowski

Michigan Tech Research Data

This study delves into the small-scale temperature structure inside the turbulent convection Pi Chamber under three temperature differences (10, 15, and 20 K) at Rayleigh number Ra ~ 10^9 and Prandtl number Pr = 0.7. We performed high-frequency measurements (2 kHz) with the UltraFast Thermometer (UFT) at selected points along the vertical axis. The miniaturized design of the sensor with a resistive platinum-coated tungsten wire, 2.5 μm thick and 3 mm long, mounted on a miniature wire probe, allowed for vertically undisturbed temperature
profiling through the chamber’s depth spanning from 8 cm above the bottom to 5 cm below the …

Vertical Gradient In Atmospheric Particle Phase State: A Case Study Over The Alaskan Arctic Oil Fields, Nurun Nahar Lata, Zezhen Cheng, Darielle Dexheimer, Susan Mathai, Matthew A. Marcus, Kerri A. Pratt

Michigan Tech Publications

The phase state of atmospheric particles impacts atmospheric processes like heterogeneous reactions, cloud droplet activation, and ice nucleation, influencing Earth's climate. Factors like chemical composition, temperature, and relative humidity govern particle phase states. The Arctic atmosphere is stratified, with varying particle compositions, but vertical profiles of submicron phase states remain poorly understood due to limited aloft measurements. To address this, particle samples were collected via a tethered balloon system (TBS) at the U.S. Department of Energy Atmospheric Radiation Measurement Program's facility at Oliktok Point, Alaska, on November 19, 2020. Using an environmental scanning electron microscope with a tilted Peltier stage …

Coupled Lake-Atmosphere-Land Physics Uncertainties In A Great Lakes Regional Climate Model, William J. Pringle, Chenfu Huang, Pengfei Xue, Jiali Wang, Khachik Sargsyan, Miraj Kayastha, Et. Al.

Michigan Tech Publications

This study develops a surrogate-based method to assess the uncertainty within a convective permitting integrated modeling system of the Great Lakes region, arising from interacting physics parameterizations across the lake, atmosphere, and land surface. Perturbed physics ensembles of the model during the 2018 summer are used to train a neural network surrogate model to predict lake surface temperature (LST) and near-surface air temperature (T2m). Average physics uncertainties are determined to be 1.5°C for LST and T2m over land, and 1.9°C for T2m over lake, but these have significant spatiotemporal variations. We find that atmospheric physics parameterizations alone are the dominant …

Light Absorbing Aerosol Interactions With Warm Clouds, Shreya Joshi

Dissertations, Master's Theses and Master's Reports

Atmospheric particles such as biomass-burning aerosols, including black carbon - are critical in altering the Earth's energy balance through interactions with light and clouds. Biomass-burning aerosols also contain organic carbon, a diverse mix of organic compounds. As these aerosols age, they evolve by interacting with other atmospheric species, including cloud water, leading to changes in particle morphology and the development of coatings that impact their lifetime and ability to interact with clouds and light.

Some biomass-burning aerosols serve as cloud condensation nuclei. When cloud water droplets form, the properties of the nucleating particles can change. Many clouds evaporate before precipitating, …

Investigating Microphysical Variability And Entrainment In Clouds Using Airborne Digital Holography, Machine Learning, And Large Eddy Simulations, Nithin Allwayin

Dissertations, Master's Theses and Master's Reports

Advancing our understanding of cloud microphysics—the processes governing cloud particles' formation, growth, and interactions—is essential for accurate weather and climate modeling. In this work, we investigate how droplet size distributions vary in a cloud and explore how microphysical properties such as droplet size and number concentration respond to entrainment and mixing.

In the first part of the work, a novel algorithm is developed combining hypothesis testing with density-based clustering to identify characteristic cloud droplet size distribution types in marine stratocumulus clouds. Applied to data from the airborne Holographic Detector for Clouds (HOLODEC), the algorithm successfully identifies a relatively small set …

Cloud Microphysical Response To Entrainment And Mixing Is Locally Inhomogeneous And Globally Homogeneous: Evidence From The Lab, Jaemin Yeom, Ian Helman, Prasanth Prabhakaran, Jesse Anderson, Fan Yang, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

The effects of entrainment-mixing on the cloud droplet size distribution are examined in the Pi cloud chamber that creates a turbulent supersaturated environment for cloud formation. The experiments are conducted with a temperature-controlled flange to mimic the entrainment-mixing process. The entrainment zone is created at the center of the top surface of the chamber, allowing dry air of controlled temperature (T_e) and flow rate (Q_e) to flow into the mixing cloud region. Due to the large-scale circulation, the downwind region is directly affected by entrained dry air from the flange, whereas the upwind region is representative …

Molecular Dynamics Simulation Data: Mw And Mlmw Water Model Ice Nucleation On A Hydrophilic Substrate With Negative Pressure, Will Cantrell, Tianshu Li, Issei Nakamura, Elise Rosky, Raymond Shaw

Michigan Tech Research Data

This dataset contains the data supporting Figures in the study by Rosky et al., "Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension", submitted for publication in Atmospheric Chemistry and Physics in February 2023. Input files for reproducing the molecular dynamics simulations are included.

The abstract from the paper reads: Using a molecular model of water freezing on a hydrophilic substrate, it is found that heterogeneous ice nucleation rates occur at higher temperatures in water that is under tension, in other words under negative pressure. For pressures ranging from from 1 atm to …

An Exploration Of Cloud Droplet Growth By Condensation And Collision-Coalescence In A Convection-Cloud Chamber, Jacob T. Kuntzleman

Dissertations, Master's Theses and Master's Reports

Atmospheric clouds are crucial to weather and climate, and the rate at which droplets collide and coalesce to form precipitation is one of the fundamental controlling processes. The convection-cloud chamber allows the interactions between aerosols and cloud droplets produced by condensation to be investigated within a turbulent environment. Studying the full range of microphysical conditions in atmospheric clouds is not possible, however, unless conditions for droplet growth by collision and coalescence are also achieved. In this study, we explore the conditions favorable to collision-coalescence growth in convection-cloud chambers, extending previous work on steady-state droplet size distributions due to condensation alone. …

Physical, Optical, And Chemical Properties Of Light Absorbing Aerosols And Their Climatic Impacts, Susan Mathai

Dissertations, Master's Theses and Master's Reports

Aerosols are particles suspended in the atmosphere; they are emitted during natural phenomena such as dust storms, wildfires, and volcanic eruptions, and during anthropogenic activities like household wood burning, vehicles operations, and industrial productions, or they can form in the atmosphere from gas to particle partition. Aerosols impact earth’s weather and climate by absorbing and scattering the incoming solar and the outgoing earth thermal radiation and interacting with clouds. The optical properties of aerosols evolve as the chemical and physical properties vary during their residence in the atmosphere. In addition, the aerosols’ properties strongly depend on the vertical distribution in …

Large Cloud Droplets And The Initiation Of Ice By Pressure Fluctuations: Molecular Simulations And Airborne In-Situ Observations, Elise Rosky

Dissertations, Master's Theses and Master's Reports

From the molecular dynamics of water molecules to the global processes that control atmospheric circulation: describing the evolution of atmospheric clouds necessitates physics that spans vast spatial scales. In this work, steps are taken towards connecting the molecular physics of ice-nucleation to the growth and subsequent freezing of cloud droplets in convective cumulus clouds. Motivated by experimental evidence of ice nucleation triggered by agitation and distortion of a water droplet surface, the first study in this dissertation uses molecular dynamics simulations to demonstrate that negative Laplace pressure from a curved water surface leads to heterogeneous ice nucleation at higher temperatures. …

An Intercomparison Of Large-Eddy Simulations Of A Convection Cloud Chamber Using Haze-Capable Bin And Lagrangian Cloud Microphysics Schemes, Fan Yang, Fabian Hoffmann, Raymond Shaw, Mikhail Ovchinnikov, Andrew Vogelmann

Michigan Tech Research Data

Recent in-situ observations show that haze particles exist in a convection cloud chamber. The microphysics schemes previously used for large-eddy simulations of the cloud chamber could not fully resolve haze particles and the associated processes, including their activation and deactivation. Specifically, cloud droplet activation is modeled based on Twomey-type parameterizations, wherein cloud droplets are formed when a critical supersaturation for the available cloud condensation nuclei (CCN) is exceeded and haze particles are not explicitly resolved. Here, we develop and adapt haze-capable bin and Lagrangian microphysics schemes to properly resolve the activation and deactivation processes. Results are compared with the Twomey-type …

Data Supporting The Paper "Is The Water Vapor Supersaturation Distribution Gaussian?", Subin Thomas, Prasanth Prabhakaran, W. Cantrell, Raymond Shaw

Michigan Tech Research Data

The data in this file are from the MTU Pi Cloud Chamber and large eddy simulations. This work was supported by NSF grant AGS-1754244. Data are made available in support of the above publication by Thomas et al.. For any further use, e.g., for publication elsewhere, the authors should be contacted to ensure the appropriate use of the data and proper acknowledgment.

Investigating Ice Nucleation At Negative Pressures Using Molecular Dynamics: A First Order Approximation Of The Dependence Of Ice Nucleation Rate On Pressure, Elise Rosky

Dissertations, Master's Theses and Master's Reports

Atmospheric scientists and climate modelers are faced with uncertainty around the process of ice production in clouds. While significant progress has been made in predicting homogeneous and heterogeneous ice nucleation rates as a function of temperature, recent experiments have shown that ice nucleation rates can be enhanced without decreasing temperature, through various mechanical agitations. One hypothesis for these findings is that mechanisms of stretching water and thereby inducing negative pressure in the liquid could lead to an increase in freezing rate. To better understand the viability of this concept, the effect of negative pressure on ice nucleation rates needs to …

Understanding The Effects Of Water Vapor And Temperature On Aerosol Using Novel Measurement Methods, Tyler Jacob Capek

Dissertations, Master's Theses and Master's Reports

Aerosol and water are inexorably linked, and both are ubiquitous within our atmosphere and required components for cloud formation. Relative humidity (RH), a temperature dependent quantity, can have a significant influence on the size, shape, and ultimately, the optical properties of the aerosol. RH can vary substantially on small spatial and short temporal scales in turbulent conditions due to rapid fluctuations in temperature and water vapor mixing ratio. Accurate assessment of optical enhancements due to an increase in RH is key for determining the particles’ impact on the climate and visibility.

A humidity-controlled cavity attenuated phase-shift albedometer (H-CAPS-PM_SSA) …

Modeling And Numerical Simulations Of The Michigan Tech Convection Cloud Chamber, Subin Thomas

Dissertations, Master's Theses and Master's Reports

Understanding atmospheric clouds is essential for human progress, ranging from short-term effects such as when and how much it rains to long-term effects such as how much temperatures would rise due to global climate change. Clouds vary globally and seasonally; also they have length scales ranging from a few nanometers to a few kilometers and timescales from a few nanoseconds to a few weeks. Knowledge gaps in aerosol-cloud-turbulence interactions and a lack of sufficient resolution in observations pose a challenge in understanding cloud systems.

Experimental facilities like the Michigan Tech Cloud Chamber can provide a suitable platform for studying aerosol-cloud …

Activation Scavenging Of Aerosol : Effect Of Turbulence And Aerosol-Composition, Abu Sayeed Md Shawon

Dissertations, Master's Theses and Master's Reports

The interaction of aerosol particles with solar radiation significantly contributes to the global radiation balance. The magnitude of this aerosol-radiation interaction, among other parameters, depends on different aerosol properties, including how readily these particles would act as cloud condensation nuclei (CCN). These properties are governed by the formation and scavenging processes of aerosol. This dissertation explores some of these scavenging processes.

Favorable humidity and preexisting aerosol particles acting as CCN are the sine qua non conditions to form cloud droplets in Earth’s atmosphere. Forming cloud droplets (known as activation), meanwhile, acts as a wet scavenging mechanism for those CCN. Given …

Data In Support Of The Paper "Dependence Of Aerosol-Droplet Partitioning On Turbulence In A Laboratory Cloud", Abu Sayeed Md Shawon, Prasanth Prabhakaran, Gregory Kinney, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

No abstract provided.

Extensive Soot Compaction By Cloud Processing From Laboratory And Field Observations, Janarjan Bhandari, Swarup China, Kamal Kant Chandrakar, Greg Kinney, Will Cantrell, Raymond Shaw, Lynn Mazzoleni, Giulia Girotto, Noopur Sharma, Kyle Gorkowski, Stefania Gilardoni, Stefano Decesari, Maria Cristina Facchini, Nicola Zanca, Giulia Pavese, Francesco Esposito, Manvendra K Dubey, Allison C Aiken, Rajan K Chakrabarty, Hans Moosmüller, Timothy B Onasch, Rahul A Zaveri, Barbara V Scarnato, Paulo Fialho, Claudio Mazzoleni

Michigan Tech Publications, Part 1

Soot particles form during combustion of carbonaceous materials and impact climate and air quality. When freshly emitted, they are typically fractal-like aggregates. After atmospheric aging, they can act as cloud condensation nuclei, and water condensation or evaporation restructure them to more compact aggregates, affecting their optical, aerodynamic, and surface properties. Here we survey the morphology of ambient soot particles from various locations and different environmental and aging conditions. We used electron microscopy and show extensive soot compaction after cloud processing. We further performed laboratory experiments to simulate atmospheric cloud processing under controlled conditions. We find that soot particles sampled after …

Data Supporting The Paper "Extensive Soot Compaction By Cloud Processing From Laboratory And Field Observations", Janarjan Bhandari, Swarup China, Kamal Kant Chandrakar, Greg Kinney, Will Cantrell, Raymond Shaw, Lynn R. Mazzoleni, Giulia Girotto, Noopur Sharma, Kyle Gorkowski, Stefania Gilardoni, Stefano Decesari, Maria Cristina Facchini, Nicola Zanca, Giulia Pavese, Francesco Esposito, Manvendra Dubey, Allison Aiken, Rajan K. Chakrabarty, Hans Moosmüller, Timothy B. Onasch, Rahul A. Zaveri, Barbara Scarnato, Paolo Fialho, Claudio Mazzoleni

Department of Physics Publications

No abstract provided.

Data Supporting The Paper "Scaling Of An Atmospheric Model To Simulate Turbulence And Cloud Microphysics In The Pi Chamber", Subin Thomas, Mikhail S. Ovchinnikov, Fan Yang, Dennis Van Der Voort, Will Cantrell, Steven K. Krueger, Raymond Shaw

Department of Physics Publications

No abstract provided.

Extreme Molecular Diversity In Biomass Burning Atmospheric Organic Aerosol Observed Through Ultrahigh Resolution Mass Spectrometry, Matthew Brege

Dissertations, Master's Theses and Master's Reports

Ambient atmospheric aerosol is ubiquitous in the atmosphere, originating from a variety of natural and man-made sources. These microscopic particles have profound impacts on the global climate system as well as human health. The organic fraction of atmospheric aerosol is an extremely complex mixture which is not yet fully characterized. These unknown organic aerosol species contribute to the uncertainty in the effect of aerosol on climate and uncertainty in overall ambient aerosol toxicity. Light absorbing organic aerosol can interact with incoming solar radiation and contribute to atmospheric heating; however, the source apportionment and overall fate of these absorbing organic aerosol …

Molecular Characterization Of Free Tropospheric Organic Aerosol And The Development Of Computational Tools For Molecular Formula Assignment, Simeon Schum

Dissertations, Master's Theses and Master's Reports

Organic aerosol affects human health and climate. These effects are largely determined by the composition of the organic aerosol, which is a complex mixture of species. Understanding the complexity of organic aerosol is critical to determining its effect on human health and climate. In this study, long range transported organic aerosol collected at the Pico Mountain Observatory was analyzed using ultrahigh resolution mass spectrometry. Organic aerosol transported in the free troposphere had an overall lower extent of oxidation than aerosol transported in the boundary layer. It was hypothesized that the lower oxidation was related to a more viscous phase state …

Aerosol-Cloud Interactions In Turbulent Clouds: A Combined Cloud Chamber And Theoretical Study, Kamal Kant Chandrakar

Dissertations, Master's Theses and Master's Reports

The influence of aerosol concentration on the cloud droplet size distribution is investigated in a laboratory chamber that enables turbulent cloud formation through moist convection. In chapter 2, moist Rayleigh-Bénard convection with water saturated boundaries is explored using a one-dimensional-turbulence model. This study provides some background about supersaturation statistics in moist convection. Chapters 3 - 7 discuss the experimental and theoretical investigation of aerosol-cloud interactions and cloud droplet size-distributions in turbulent conditions. The experiments are performed in a way so that steady-state microphysics are achieved, with aerosol input balanced by cloud droplet growth and fallout. As aerosol concentration is increased …

Investigation Of Light Transport And Scattering In Turbulent Clouds: Simulations And Laboratory Measurements, Corey D. Packard

Dissertations, Master's Theses and Master's Reports

A better understanding of light transport and scattering in turbulent clouds is needed for more accurate remote sensing, improved imaging and signal transmission through atmospheric aerosol and fog, and deeper understanding of cloud optical properties relevant to weather and climate. In this study, we investigate the impact of light scattering in clouds on two problems of atmospheric relevance.

In the first part, we examine deleterious effects of the atmosphere on remotely acquired images including signal attenuation and potential blurring due to forward-scattered light accepted by the imaging system. A prior proposed aerosol scattering model provides a method for calculating the …

Light Propagation Through A Turbulent Cloud: Comparison Of Measured And Computed Extinction, Eduardo Rodriguez-Feo Bermudez

Dissertations, Master's Theses and Master's Reports

Remote sensing techniques used for measurement of atmospheric cloud properties operate under the notion that light extinction caused by scattering and absorption is exponential due to Beer-Lambert law. This is expected to be valid for a uni-form medium with no spatial correlations between particle position. The aim of this research was to show that under turbulent conditions, cloud droplets cannot be interpreted as non-correlated, and in turn will exhibit a lower than exponential light decay from scattering. The research took place at the MTU π-Chamber laboratory. A temperature difference between the floor and ceiling of the chamber was applied to …

Fine-Scale Droplet Clustering In Atmospheric Clouds: 3d Radial Distribution Function From Airborne Digital Holography, Michael L. Larsen, Raymond Shaw, Alexander Kostinski, Susanne Glienke

Department of Physics Publications

The extent of droplet clustering in turbulent clouds has remained largely unquantified, and yet is of possible relevance to precipitation formation and radiative transfer. To that end, data gathered by an airborne holographic instrument are used to explore the three-dimensional spatial statistics of cloud droplet positions in homogeneous stratiform boundary-layer clouds. The three-dimensional radial distribution functions g(r) reveal unambiguous evidence of droplet clustering. Three key theoretical predictions are observed: the existence of positive correlations, onset of correlation in the turbulence dissipation range, and monotonic increase of g(r) with decreasing r. This implies that current theory captures the essential processes contributing …

Turbulence Induced Cloud Voids: Observation And Interpretation, Katarzyna Karpinska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, Eberhard Bodenschatz

Department of Physics Publications

The phenomenon of cloud voids, i.e., elongated volumes inside a cloud that are devoid of droplets, was observed with laser sheet photography in clouds at a mountain-top station. Two experimental cases, similar in turbulence conditions yet with diverse droplet size distributions and cloud void prevalence, are reported. A theoretical explanation is proposed based on the study of heavy inertial sedimenting particles inside a Burgers vortex. A general conclusion regarding void appearance is drawn from theoretical analysis. Numerical simulations of polydisperse droplet motion with realistic vortex parameters and Mie scattering visual effects accounted for can explain the presence of voids with …

Molecular And Physical Characteristics Of Aerosol At A Remote Free Troposphere Site: Implications For Atmospheric Aging, Simeon Schum, Bo Zhang, Katja Džepina, Paolo Fialho, Claudio Mazzoleni, Lynn Mazzoleni

Department of Chemistry Publications

Aerosol properties are transformed by atmospheric processes during long-range transport and play a key role in the Earth's radiative balance. To understand the molecular and physical characteristics of free tropospheric aerosol, we studied samples collected at the Pico Mountain Observatory in the North Atlantic. The observatory is located in the marine free troposphere at 2225m above sea level, on Pico Island in the Azores archipelago. The site is ideal for the study of long-range-transported free tropospheric aerosol with minimal local influence. Three aerosol samples with elevated organic carbon concentrations were selected for detailed analysis. FLEXPART retroplumes indicated that two of …

Data Supporting The Paper "Turbulence Induced Cloud Voids: Observation And Interpretation", Katarzyna Karpinska, Jonathan F. E. Bodenschatz, Szymon P. Malinowski, Jakub L. Nowak, Steffen Risius, Tina Schmeissner, Raymond Shaw, Holger Siebert, Hengdong Xi, Haitao Xu, Eberhard Bodenschatz

Department of Physics Publications

No abstract provided.