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Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

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Full-Text Articles in Atmospheric Sciences

Oco-3 Meets Ecostress: Insights Into Ecosystem Diurnal Water-Use Efficiency From Co-Located Solar-Induced Fluorescence And Thermal Observations, Zoe Amie Pierrat, Thomas P. Kurosu, Abhishek Chatterjee, Joshua B. Fisher, Maggie Johnson, Le Kuai, Kanishka Mallick, Nicholas Parazoo, Benjamin Wiebe, Kerry Cawse-Nicholson Sep 2026

Oco-3 Meets Ecostress: Insights Into Ecosystem Diurnal Water-Use Efficiency From Co-Located Solar-Induced Fluorescence And Thermal Observations, Zoe Amie Pierrat, Thomas P. Kurosu, Abhishek Chatterjee, Joshua B. Fisher, Maggie Johnson, Le Kuai, Kanishka Mallick, Nicholas Parazoo, Benjamin Wiebe, Kerry Cawse-Nicholson

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Terrestrial ecosystem regulation of carbon and water fluxes is critical for constraining climate–biosphere feedbacks but remains poorly quantified across space and time. Here, we evaluate whether co-located observations from NASA's Orbiting Carbon Observatory-3 (OCO-3) and the ECOsystem Spaceborne Thermal Radiometer Experiment on Space Station (ECOSTRESS) can reproduce ecosystem water use efficiency (WUE) dynamics observed at FLUXNET sites across temporal scales, vegetation types, climates, and drought conditions. We created the ECOCO3 data set, which harmonizes OCO-3 and ECOSTRESS observations in space and time. ECOCO3 captures broad seasonal and diurnal carbon and water flux patterns including midday drought responses. Sampling sensitivity analysis …


Evapotranspiration Everywhere, All The Time: Towards A Unified View From Earth Observation, Joshua B. Fisher, Martha C. Anderson, Diego G. Miralles, Kanishka Mallick, Paul C. Stoy, Youngryel Ryu, Wim G. M. Bastiaanssen May 2026

Evapotranspiration Everywhere, All The Time: Towards A Unified View From Earth Observation, Joshua B. Fisher, Martha C. Anderson, Diego G. Miralles, Kanishka Mallick, Paul C. Stoy, Youngryel Ryu, Wim G. M. Bastiaanssen

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Scientists want to know everything, everywhere, and all the time. This is particularly true in Earth science, where we seek to understand processes that span from the molecular to the planetary scale in how the world works, how it affects us, and how we impact it—especially the water cycle. Evapotranspiration (ET) was the last component to be measured in closing the water cycle: for decades, closing the water budget meant adding up all the measurable components, then inferring ET as the residual. Early measurements relied on water loss from pans and weighing lysimeters, followed by sensors inserted into plants to …


Warming Climate Amplifies Vapor Pressure Deficit Limits On Gross Primary Productivity, Shiqin Xu, Nate G. Mcdowell, Tim R. Mcvicar, Diego G. Miralles, Stephen Sitch, Pablo Sanchez-Martinez, Joshua B. Fisher, Pierre Friedlingstein, Hylke E. Beck, Matthew F. Mccabe Apr 2026

Warming Climate Amplifies Vapor Pressure Deficit Limits On Gross Primary Productivity, Shiqin Xu, Nate G. Mcdowell, Tim R. Mcvicar, Diego G. Miralles, Stephen Sitch, Pablo Sanchez-Martinez, Joshua B. Fisher, Pierre Friedlingstein, Hylke E. Beck, Matthew F. Mccabe

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Ongoing climate warming may profoundly impact terrestrial gross primary productivity (GPP), a key component of the global carbon cycle. However, uncertainty in the relative roles of atmospheric water demand (vapor pressure deficit, VPD) and root-zone soil moisture (SM) limits predictions of drought impacts on GPP. Here, we show that growing-season GPP was more strongly constrained by VPD than SM globally, based on observation-constrained model estimates, satellite retrievals and Dynamic Global Vegetation Model simulations. The importance of VPD increased with higher temperatures and more severe and prolonged droughts. This pattern reflects VPD’s critical role in regulating stomatal conductance and plant hydraulic …


Climate Change Has Increased Global Evaporative Demand Except In South Asia, Saeed Karimzadeh, Arman Ahmadi, Dennis Baldocchi, Joshua B. Fisher Nov 2025

Climate Change Has Increased Global Evaporative Demand Except In South Asia, Saeed Karimzadeh, Arman Ahmadi, Dennis Baldocchi, Joshua B. Fisher

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Climate change alters how strongly the atmosphere draws water from the land, yet a consistent global assessment of this evaporative demand has been lacking. Here, we analyze 45 years of climate data and global models to quantify trends in the key drivers—air temperature, humidity, radiation, wind speed, and cloud cover—that determine the atmosphere’s drying power. We find that evaporative demand has increased worldwide, indicating a stronger atmospheric thirst, except in South Asia, where it has declined. There, widespread irrigation has increased soil and air moisture, enhanced cloud formation, and reduced sunlight reaching the surface, counteracting the global signal. These contrasting …


A Novel Approach To Increase Accuracy In Remotely Sensed Evapotranspiration Through Basin Water Balance And Flux Tower Constraints, Kul Khand, Gabriel B. Senay, Mackenzie Friedrichs, Koong Yi, Joshua B. Fisher, Lixin Wang, Kosana Suvočarev, Arman Ahmadi, Housen Chu, Stephen Good, Kanishka Mallick, Justine Missik, Jacob A. Nelson, David E. Reed, Tianxin Wang, Xiangming Xiao Jul 2025

A Novel Approach To Increase Accuracy In Remotely Sensed Evapotranspiration Through Basin Water Balance And Flux Tower Constraints, Kul Khand, Gabriel B. Senay, Mackenzie Friedrichs, Koong Yi, Joshua B. Fisher, Lixin Wang, Kosana Suvočarev, Arman Ahmadi, Housen Chu, Stephen Good, Kanishka Mallick, Justine Missik, Jacob A. Nelson, David E. Reed, Tianxin Wang, Xiangming Xiao

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Remote sensing-derived evapotranspiration (RSET) products capture the spatiotemporal variations of evapotranspiration (ET) from field to basin scales with unprecedented details. However, their accuracy varies across RSET estimation methods and diverse hydroclimate regions. While ET modeling efforts to account for biophysical processes and controlling parameters have made good progress in recent years, a parallel approach of integrating in-situ ET with RSET could reduce biases in RSET products. Basin water balance ET (WBET) and flux tower ET are widely applied to evaluate RSET accuracy, yet such ET measurements are rarely used for RSET bias corrections, especially for large area applications. To address …


Large-Scale Groundwater System Characterization Using Pressure Responses To Barometric Perturbations Caused By The 2022 Hunga Tonga-Hunga Ha'apai Volcanic Eruption, Anhua He, Yang Liu, Fan Zhang, Huamei Zhang, Ramesh P. Singh, Yanzhang Wang May 2025

Large-Scale Groundwater System Characterization Using Pressure Responses To Barometric Perturbations Caused By The 2022 Hunga Tonga-Hunga Ha'apai Volcanic Eruption, Anhua He, Yang Liu, Fan Zhang, Huamei Zhang, Ramesh P. Singh, Yanzhang Wang

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Hunga Tonga-Hunga Ha'apai volcanic erupted on 15 January 2022, causing Lamb waves to propagate throughout the global troposphere. However, reports on volcanic eruptions–pressure fluctuations and water level dynamics are lacking. We quantified the propagation processes of Lamb waves induced by the Tonga volcanic eruption. Barometric pressure data collected at 1-min intervals at 485 meteorological stations in China showed that the eruption induced an atmospheric pressure event with an amplitude of ∼2 hPa over an hour and a wave speed of 295 m/s. Concomitant groundwater levels were available at 338 wells to find the barometric response to the volcanic event. The …


Increasing Atmospheric Evaporative Demand Across The Tibetan Plateau And Implications For Surface Water Resources, Shiqin Xu, Dennis P. Lettenmaier, Tom R. Mcvicar, Pierre Gentine, Hylke E. Beck, Joshua B. Fisher, Zhongbo Yu, Ningpeng Dong, Akash Koppa, Matthew F. Mccabe Jan 2025

Increasing Atmospheric Evaporative Demand Across The Tibetan Plateau And Implications For Surface Water Resources, Shiqin Xu, Dennis P. Lettenmaier, Tom R. Mcvicar, Pierre Gentine, Hylke E. Beck, Joshua B. Fisher, Zhongbo Yu, Ningpeng Dong, Akash Koppa, Matthew F. Mccabe

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The Tibetan Plateau, known as the “Asian water tower,” is a hotspot for complex hydroclimatic changes. We reveal that the previously decreasing atmospheric evaporative demand (Eo) trend at the end of the 20th century has reversed over the last two decades. Although both wind stilling and solar dimming have persisted, their effects on Eo rates have been overshadowed by increasing air temperatures and decreasing relative humidity, leading to a net rise in Eo for 1980−2015. Using the empirical “top-down” Budyko approach, we estimate that across seven sub-catchments draining the Tibetan Plateau, a 10% increase in annual-averaged …


Methane Fluxes In Tidal Marshes Of The Conterminous United States, Ariane Arias-Ortiz, Jaxine Wolfe, Scott D. Bridgham, Sara Knox, Gavin Mcnicol, Brian A. Needelman, Julie Shahan, Ellen J. Stuart-Haëntjens, Lisamarie Windham-Myers, Patty Y. Oikawa, Dennis D. Baldocchi, Joshua S. Caplan, Margaret Capooci, Kenneth M. Czapla, R. Kyle Derby, Heida L. Diefenderfer, Inke Forbrich, Gina Groseclose, Jason K. Keller, Cheryl Kelley, Amir E. Keshta, Helena S. Kleiner, Ken W. Krauss, Robert R. Lane, Sarah Mack, Serena Moseman-Valtierra, Thomas J. Mozdzer, Peter Mueller, Scott C. Neubauer, Genevieve Noyce, Katrina V. R. Schäfer, Rebecca Sanders-Demott, Charles A. Schutte, Rodrigo Vargas, Nathaniel B. Weston, Benjamin Wilson, J. Patrick Megonigal, James R. Homquist Sep 2024

Methane Fluxes In Tidal Marshes Of The Conterminous United States, Ariane Arias-Ortiz, Jaxine Wolfe, Scott D. Bridgham, Sara Knox, Gavin Mcnicol, Brian A. Needelman, Julie Shahan, Ellen J. Stuart-Haëntjens, Lisamarie Windham-Myers, Patty Y. Oikawa, Dennis D. Baldocchi, Joshua S. Caplan, Margaret Capooci, Kenneth M. Czapla, R. Kyle Derby, Heida L. Diefenderfer, Inke Forbrich, Gina Groseclose, Jason K. Keller, Cheryl Kelley, Amir E. Keshta, Helena S. Kleiner, Ken W. Krauss, Robert R. Lane, Sarah Mack, Serena Moseman-Valtierra, Thomas J. Mozdzer, Peter Mueller, Scott C. Neubauer, Genevieve Noyce, Katrina V. R. Schäfer, Rebecca Sanders-Demott, Charles A. Schutte, Rodrigo Vargas, Nathaniel B. Weston, Benjamin Wilson, J. Patrick Megonigal, James R. Homquist

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Methane (CH4) is a potent greenhouse gas (GHG) with atmospheric concentrations that have nearly tripled since pre-industrial times. Wetlands account for a large share of global CH4 emissions, yet the magnitude and factors controlling CH4 fluxes in tidal wetlands remain uncertain. We synthesized CH4 flux data from 100 chamber and 9 eddy covariance (EC) sites across tidal marshes in the conterminous United States to assess controlling factors and improve predictions of CH4 emissions. This effort included creating an open-source database of chamber-based GHG fluxes (https://doi.org/10.25573/serc.14227085). Annual fluxes across chamber and EC sites averaged 26 ± 53 g CH4 …


The Ecosystem As Super-Organ/Ism, Revisited: Scaling Hydraulics To Forests Under Climate Change, Jeffrey D. Wood, Matteo Detto, Marvin Browne, Nathan J.B. Kraft, Alexandra G. Konings, Joshua B. Fisher, Gregory R. Quetin, Anna T. Trugman, Troy S. Magney, Camila D. Medeiros, Nidhi Vinod, Thomas N. Buckley, Lawren Sack Jun 2024

The Ecosystem As Super-Organ/Ism, Revisited: Scaling Hydraulics To Forests Under Climate Change, Jeffrey D. Wood, Matteo Detto, Marvin Browne, Nathan J.B. Kraft, Alexandra G. Konings, Joshua B. Fisher, Gregory R. Quetin, Anna T. Trugman, Troy S. Magney, Camila D. Medeiros, Nidhi Vinod, Thomas N. Buckley, Lawren Sack

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Classic debates in community ecology focused on the complexities of considering an ecosystem as a super-organ or organism. New consideration of such perspectives could clarify mechanisms underlying the dynamics of forest carbon dioxide (CO2) uptake and water vapor loss, important for predicting and managing the future of Earth's ecosystems and climate system. Here, we provide a rubric for considering ecosystem traits as aggregated, systemic, or emergent, i.e., representing the ecosystem as an aggregate of its individuals, or as a metaphorical or literal super-organ or organism. We review recent approaches to scaling-up plant water relations (hydraulics) concepts developed for …


Dynamic And Thermodynamic Influences On Precipitation In Northeast Mexico On Orbital To Millennial Timescales, Kevin T. Wright, Kathleen R. Johnson, Gabriela Serrato Marks, David Mcgee, Tripti Bhattacharya, Gregory R. Goldsmith, Clay R. Tabor, Jean-Louis Lacaille-Muzquiz, Gianna Lum, Laura Beramendi-Orosco Apr 2023

Dynamic And Thermodynamic Influences On Precipitation In Northeast Mexico On Orbital To Millennial Timescales, Kevin T. Wright, Kathleen R. Johnson, Gabriela Serrato Marks, David Mcgee, Tripti Bhattacharya, Gregory R. Goldsmith, Clay R. Tabor, Jean-Louis Lacaille-Muzquiz, Gianna Lum, Laura Beramendi-Orosco

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The timing and mechanisms of past hydroclimate change in northeast Mexico are poorly constrained, limiting our ability to evaluate climate model performance. To address this, we present a multiproxy speleothem record of past hydroclimate variability spanning 62.5 to 5.1 ka from Tamaulipas, Mexico. Here we show a strong influence of Atlantic and Pacific sea surface temperatures on orbital and millennial scale precipitation changes in the region. Multiple proxies show no clear response to insolation forcing, but strong evidence for dry conditions during Heinrich Stadials. While these trends are consistent with other records from across Mesoamerica and the Caribbean, the relative …


Dynamic Characteristics Of Aerosol Optical Properties Over Dibrugarh City In The North-Eastern Indian Region During 2018–2021, Akshansa Chauhan, Shukla Acharjee, Ramesh P. Singh, Brent N. Holben Mar 2023

Dynamic Characteristics Of Aerosol Optical Properties Over Dibrugarh City In The North-Eastern Indian Region During 2018–2021, Akshansa Chauhan, Shukla Acharjee, Ramesh P. Singh, Brent N. Holben

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Aerosols play an important role in the earth's environment across the globe through their involvement in various earth system cycles. The change in the aerosol properties may cause short and long-term impacts, the knowledge of such changes is useful in the estimation of the pollution sources of any region. We have carried out the analysis of the aerosols' optical and radiative properties using AERONET station data from 2018 to 2021 in Dibrugarh City. The higher Aerosol Optical Depth (AOD) values during winter and pre-monsoon months indicate high anthropogenic activities, and biomass burning in Dibrugarh. The impact of various sources and …


Ecological Protection Alone Is Not Enough To Conserve Ecosystem Carbon Storage: Evidence From Guangdong, China, Lihan Cui, Wenwen Tang, Sheng Zheng, Ramesh P. Singh Dec 2022

Ecological Protection Alone Is Not Enough To Conserve Ecosystem Carbon Storage: Evidence From Guangdong, China, Lihan Cui, Wenwen Tang, Sheng Zheng, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The increase in atmospheric CO2 caused by land use and land cover change (LUCC) is one of the drivers of the global climate. As one of the most typical high-urbanization areas, the ecological conflicts occurring in Guangdong Province warrant urgent attention. A growing body of evidence suggests LUCC could guide the future ecosystem carbon storage, but most LUCC simulations are simply based on model results without full consistency with the actual situation. Fully combined with the territorial spatial planning project and based on the land use pattern in 2010 and 2020, we have used the Markov and Patch-generating Land …


Possible Overestimation Of Nitrogen Dioxide Outgassing During The Beirut 2020 Explosion, Ashraf Farahat, Nayla El-Kork, Ramesh P. Singh, Feng Jing Dec 2022

Possible Overestimation Of Nitrogen Dioxide Outgassing During The Beirut 2020 Explosion, Ashraf Farahat, Nayla El-Kork, Ramesh P. Singh, Feng Jing

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

On 4 August 2020, a strong explosion occurred near the Beirut seaport, Lebanon and killed more than 200 people and damaged numerous buildings in the vicinity. As Amonium Nitrate (AN) caused the explosion, many studies claimed the release of large amounts of NO2 in the atmosphere may have resulted in a health hazard in Beirut and the vicinity. In order to reasonably evaluate the significance of NO2 amounts released in the atmosphere, it is important to investigate the spatio-temporal distribution of NO2 during and after the blast and compare it to the average day-to-day background emissions from …


Increased Aerosols Can Reverse Twomey Effect In Water Clouds Through Radiative Pathway, Pradeep Khatri, Tadahiro Hayasaka, Brent N. Holben, Ramesh P. Singh, Husi Letu, Sachchida N. Tripathi Nov 2022

Increased Aerosols Can Reverse Twomey Effect In Water Clouds Through Radiative Pathway, Pradeep Khatri, Tadahiro Hayasaka, Brent N. Holben, Ramesh P. Singh, Husi Letu, Sachchida N. Tripathi

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Aerosols play important roles in modulations of cloud properties and hydrological cycle by decreasing the size of cloud droplets with the increase of aerosols under the condition of fixed liquid water path, which is known as the first aerosol indirect effect or Twomey-effect or microphysical effect. Using high-quality aerosol data from surface observations and statistically decoupling the influence of meteorological factors, we show that highly loaded aerosols can counter this microphysical effect through the radiative effect to result both the decrease and increase of cloud droplet size depending on liquid water path in water clouds. The radiative effect due to …


Response Of Surface And Atmospheric Parameters Associated With The Iran M 7.3 Earthquake, Feng Jing, Ramesh P. Singh Jul 2022

Response Of Surface And Atmospheric Parameters Associated With The Iran M 7.3 Earthquake, Feng Jing, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Multiparameter observed from satellite, including microwave brightness temperature, skin temperature, air temperature, and carbon monoxide, have been analyzed to identify the anomalous signals associated with the M 7.3 Iran earthquake of November 12, 2017. Besides removing the multiyear variability of parameters as background, the effect of surface and atmosphere of a dust storm event in Middle East region during October 29–November 1 is considered to distinguish the possible anomalies associated with the earthquake. The characteristic behaviors of surface and atmospheric parameters clearly show the signals associated with the M 7.3 earthquake and the dust storm event. The multiple parameters at …


A General Pattern Of Trade-Offs Between Ecosystem Resistance And Resilience To Tropical Cyclones, Christopher J. Patrick, John S. Kominoski, William H. Mcdowell, Benjamin Branoff, David Lagomasino, Miguel Leon, Enie Hensel, Marc J. S. Hensel, Bradley A. Strickland, T. Mitchell Aide, Anna Armitage, Marconi Campos-Cerqueira, Victoria M. Congdon, Todd A. Crowl, Donna J. Devlin, Sarah Douglas, Brad E. Erisman, Rusty A. Feagin, Simon J. Geist, Nathan S. Hall, Amber K. Hardison, Michael R. Heithaus, J. Aaron Hogan, J. Derek Hogan, Sean Kinard, Jeremy J. Kiszka, Teng-Chiu Lin, Kaijun Lu, Christopher J. Madden, Paul A. Montagna, Christine S. O'Connell, C. Edward Proffitt, Brandi Kiel Reese, Joseph W. Reustle, Kelly L. Robinson, Scott A. Rush, Rolando O. Santos, Astrid Schnetzer, Delbert L. Smee, Rachel S. Smith, Gregory Starr, Beth A. Stauffer, Lily M. Walker, Carolyn A. Weaver, Michael S. Wetz, Elizabeth R. Whitman, Sara S. Wilson, Jianhong Xue, Xiaoming Zou Mar 2022

A General Pattern Of Trade-Offs Between Ecosystem Resistance And Resilience To Tropical Cyclones, Christopher J. Patrick, John S. Kominoski, William H. Mcdowell, Benjamin Branoff, David Lagomasino, Miguel Leon, Enie Hensel, Marc J. S. Hensel, Bradley A. Strickland, T. Mitchell Aide, Anna Armitage, Marconi Campos-Cerqueira, Victoria M. Congdon, Todd A. Crowl, Donna J. Devlin, Sarah Douglas, Brad E. Erisman, Rusty A. Feagin, Simon J. Geist, Nathan S. Hall, Amber K. Hardison, Michael R. Heithaus, J. Aaron Hogan, J. Derek Hogan, Sean Kinard, Jeremy J. Kiszka, Teng-Chiu Lin, Kaijun Lu, Christopher J. Madden, Paul A. Montagna, Christine S. O'Connell, C. Edward Proffitt, Brandi Kiel Reese, Joseph W. Reustle, Kelly L. Robinson, Scott A. Rush, Rolando O. Santos, Astrid Schnetzer, Delbert L. Smee, Rachel S. Smith, Gregory Starr, Beth A. Stauffer, Lily M. Walker, Carolyn A. Weaver, Michael S. Wetz, Elizabeth R. Whitman, Sara S. Wilson, Jianhong Xue, Xiaoming Zou

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Tropical cyclones drive coastal ecosystem dynamics, and their frequency, intensity, and spatial distribution are predicted to shift with climate change. Patterns of resistance and resilience were synthesized for 4138 ecosystem time series from n = 26 storms occurring between 1985 and 2018 in the Northern Hemisphere to predict how coastal ecosystems will respond to future disturbance regimes. Data were grouped by ecosystems (fresh water, salt water, terrestrial, and wetland) and response categories (biogeochemistry, hydrography, mobile biota, sedentary fauna, and vascular plants). We observed a repeated pattern of trade-offs between resistance and resilience across analyses. These patterns are likely the outcomes …


Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer Nov 2021

Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

PM2.5 is a major component of air pollution in China and has a serious threat to public health. It is very important to quantify spatial characteristics of the health effects caused by outdoor PM2.5 exposure. This study analyzed the spatial distribution of PM2.5 concentration (45.9 μg/m3 national average in 2016) and premature mortality attributed to PM2.5 in cities at the prefectural level and above in China in 2016. Using the Global Exposure Mortality Model (GEMM), the total premature mortality in China was estimated to be 1.55 million persons, and the per capita mortality was 11.2 …


Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer Nov 2021

Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

PM2.5 is a major component of air pollution in China and has a serious threat to public health. It is very important to quantify spatial characteristics of the health effects caused by outdoor PM2.5 exposure. This study analyzed the spatial distribution of PM2.5 concentration (45.9 μg/m3 national average in 2016) and premature mortality attributed to PM2.5 in cities at the prefectural level and above in China in 2016. Using the Global Exposure Mortality Model (GEMM), the total premature mortality in China was estimated to be 1.55 million persons, and the per capita mortality was 11.2 …


An Integrative Model For Soil Biogeochemistry And Methane Processes: I. Model Structure And Sensitivity Analysis, Daniel M. Ricciuto, Xiaofeng Xu, Xiaoying Shi, Yihui Wang, Xia Song, Christopher W. Schadt, Natalie A. Griffiths, Jiafu Mao, Jeffrey M. Warren, Peter E. Thornton, Jeff Chanton, Jason K. Keller, Scott D. Bridgham, Jessica Gutknecht, Stephen D. Sebestyen, Adrien Finzi, Randall Kolka, Paul J. Hanson Jul 2021

An Integrative Model For Soil Biogeochemistry And Methane Processes: I. Model Structure And Sensitivity Analysis, Daniel M. Ricciuto, Xiaofeng Xu, Xiaoying Shi, Yihui Wang, Xia Song, Christopher W. Schadt, Natalie A. Griffiths, Jiafu Mao, Jeffrey M. Warren, Peter E. Thornton, Jeff Chanton, Jason K. Keller, Scott D. Bridgham, Jessica Gutknecht, Stephen D. Sebestyen, Adrien Finzi, Randall Kolka, Paul J. Hanson

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Environmental changes are anticipated to generate substantial impacts on carbon cycling in peatlands, affecting terrestrial-climate feedbacks. Understanding how peatland methane (CH4) fluxes respond to these changing environments is critical for predicting the magnitude of feedbacks from peatlands to global climate change. To improve predictions of CH4 fluxes in response to changes such as elevated atmospheric CO2 concentrations and warming, it is essential for Earth system models to include increased realism to simulate CH4 processes in a more mechanistic way. To address this need, we incorporated a new microbial-functional group-based CH4 module into the Energy …


Changes In Tropospheric Ozone Associated With Strong Earthquakes And Possible Mechanism, Feng Jing, Ramesh P. Singh May 2021

Changes In Tropospheric Ozone Associated With Strong Earthquakes And Possible Mechanism, Feng Jing, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The index of ozone anomaly (IOA) has been proposed to detect changes in tropospheric ozone associated with strong earthquakes. The tropospheric ozone prior and after the 2008 Wenchuan earthquake has been analyzed using IOA. Atmospheric infrared sounder ozone volume mixing ratio (O3 VMR) at different pressure levels (600, 500, 400, 300, 200 hPa) for an 18-year period 2003–2020 has been considered to identify the unique behavior associated with the strong earthquakes. Our results show distinct enhancement in tropospheric ozone occurred 5 d (7 May 2008) prior to the main event and distributed along the Longmenshan fault zone. An enhancement in …


Representing Methane Emissions From Wet Tropical Forest Soils Using Microbial Functional Groups Constrained By Soil Diffusivity, Debjani Sihi, Xiaofeng Xu, Mónica Salazar Ortiz, Christine S. O'Connell, Whendee L. Silver, Carla López-Lloreda, Julia M. Brenner, Ryan K. Quinn, Jana R. Phillips, Brent D. Newman, Melanie A. Mayes Mar 2021

Representing Methane Emissions From Wet Tropical Forest Soils Using Microbial Functional Groups Constrained By Soil Diffusivity, Debjani Sihi, Xiaofeng Xu, Mónica Salazar Ortiz, Christine S. O'Connell, Whendee L. Silver, Carla López-Lloreda, Julia M. Brenner, Ryan K. Quinn, Jana R. Phillips, Brent D. Newman, Melanie A. Mayes

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Tropical ecosystems contribute significantly to global emissions of methane (CH4), and landscape topography influences the rate of CH4 emissions from wet tropical forest soils. However, extreme events such as drought can alter normal topographic patterns of emissions. Here we explain the dynamics of CH4 emissions during normal and drought conditions across a catena in the Luquillo Experimental Forest, Puerto Rico. Valley soils served as the major source of CH4 emissions in a normal precipitation year (2016), but drought recovery in 2015 resulted in dramatic pulses in CH4 emissions from all topographic positions. Geochemical parameters …


Air Quality Over Major Cities Of Saudi Arabia During Hajj Periods Of 2019 And 2020, Ashraf Farahat, Akshansha Chauhan, Mohammed Al Otaibi, Ramesh P. Singh Feb 2021

Air Quality Over Major Cities Of Saudi Arabia During Hajj Periods Of 2019 And 2020, Ashraf Farahat, Akshansha Chauhan, Mohammed Al Otaibi, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Mecca and Madinah are two holy cities where millions of people in general, visit throughout the years, during Hajj (Muslim's pilgrimage) time number of people visit these holy cities from different parts of the world is very high. However, the Government of Saudi Arabia only allowed 1000 pilgrims during the 2020 Hajj especially when the world is suffering from COVID-19. In the present paper, a detailed analysis of air quality parameters available from ground measurements have been carried over major cities of Saudi Arabia, Mecca, Madinah, and Jeddah from June to September 2019 and 2020. At Mecca and Jeddah, PM …


Effect Of Lockdown On Hcho And Trace Gases Over India During March 2020, Akshansha Chauhan, Ramesh P. Singh Nov 2020

Effect Of Lockdown On Hcho And Trace Gases Over India During March 2020, Akshansha Chauhan, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

COVID-19 is one of the deadly Epidemics that has impacted people living in more than 200 countries. In order to mitigate the impact of COVID-19, India observed total lockdown in the first phase for a period of 21 days (24 March–13 May 2020), so that social distancing is maintained. However, this sudden decision severely affected the normal life of people. The air quality improved due to lockdown, some relaxation was given in different cities and within some areas in the city where the people were not affected by COVID-19. In this paper, we discuss results of detailed analysis of trace …


Cosore: A Community Database For Continuous Soil Respiration And Other Soil-Atmosphere Greenhouse Gas Flux Data, Ben Bond-Lamberty, Danielle S. Christianson, Avni Malhotra, Stephanie C. Pennington, Debjani Sihi, Amir Aghakouchak, Hassan Anjileli, M. Altaf Arain, Juan J. Armesto, Samaneh Ashraf, Mioko Ataka, Dennis Baldocchi, Thomas Andrew Black, Nina Buchmann, Mariah S. Carbone, Shih-Chieh Chang, Patrick Crill, Peter S. Curtis, Eric A. Davidson, Ankur R. Desai, John E. Drake, Tarek S. El-Madany, Michael Gavazzi, Carolyn-Monika Görres, Christopher M. Gough, Michael Goulden, Jillian Gregg, Omar Gutiérrez Del Arroyo, Jin-Sheng He, Takashi Hirano, Anya Hopple, Holly Hughes, Järvi Järveoja, Rachhpal Jassal, Jinshi Jian, Haiming Kan, Jason Kaye, Yuji Kominami, Naishen Liang, David Lipson, Catriona A. Macdonald, Kadmiel Maseyk, Kayla Mathes, Marguerite Mauritz, Melanie A. Mayes, Steve Mcnulty, Guofang Miao, Mirco Migliavacca, Scott Miller, Chelcy F. Miniat, Jennifer G. Nietz, Mats B. Nilsson, Asko Noormets, Hamidreza Norouzi, Christine S. O'Connell, Bruce Osborne, Cecilio Oyonarte, Zhuo Pang, Matthias Peichl, Elise Pendall, Jorge F. Perez-Quezada, Claire L. Phillips, Richard P. Phillips, James W. Raich, Alexandre A. Renchon, Nadine K. Ruehr, Enrique P. Sánchez-Cañete, Matthew Saunders, Kathleen E. Savage, Marion Schrumpf, Russell L. Scott, Ulli Seibt, Whendee L. Silver, Wu Sun, Daphne Szutu, Kentaro Takagi, Masahiro Takagi, Munemasa Teramoto, Mark G. Tjoelker, Susan Trumbore, Masahito Ueyama, Rodrigo Vargas, Ruth K. Varner, Joseph Verfaillie, Christoph Vogel, Jinsong Wang, Greg Winston, Tana E. Wood, Juying Wu, Thomas Wutzler, Jiye Zeng, Tianshan Zha, Quan Zhang, Junliang Zou Oct 2020

Cosore: A Community Database For Continuous Soil Respiration And Other Soil-Atmosphere Greenhouse Gas Flux Data, Ben Bond-Lamberty, Danielle S. Christianson, Avni Malhotra, Stephanie C. Pennington, Debjani Sihi, Amir Aghakouchak, Hassan Anjileli, M. Altaf Arain, Juan J. Armesto, Samaneh Ashraf, Mioko Ataka, Dennis Baldocchi, Thomas Andrew Black, Nina Buchmann, Mariah S. Carbone, Shih-Chieh Chang, Patrick Crill, Peter S. Curtis, Eric A. Davidson, Ankur R. Desai, John E. Drake, Tarek S. El-Madany, Michael Gavazzi, Carolyn-Monika Görres, Christopher M. Gough, Michael Goulden, Jillian Gregg, Omar Gutiérrez Del Arroyo, Jin-Sheng He, Takashi Hirano, Anya Hopple, Holly Hughes, Järvi Järveoja, Rachhpal Jassal, Jinshi Jian, Haiming Kan, Jason Kaye, Yuji Kominami, Naishen Liang, David Lipson, Catriona A. Macdonald, Kadmiel Maseyk, Kayla Mathes, Marguerite Mauritz, Melanie A. Mayes, Steve Mcnulty, Guofang Miao, Mirco Migliavacca, Scott Miller, Chelcy F. Miniat, Jennifer G. Nietz, Mats B. Nilsson, Asko Noormets, Hamidreza Norouzi, Christine S. O'Connell, Bruce Osborne, Cecilio Oyonarte, Zhuo Pang, Matthias Peichl, Elise Pendall, Jorge F. Perez-Quezada, Claire L. Phillips, Richard P. Phillips, James W. Raich, Alexandre A. Renchon, Nadine K. Ruehr, Enrique P. Sánchez-Cañete, Matthew Saunders, Kathleen E. Savage, Marion Schrumpf, Russell L. Scott, Ulli Seibt, Whendee L. Silver, Wu Sun, Daphne Szutu, Kentaro Takagi, Masahiro Takagi, Munemasa Teramoto, Mark G. Tjoelker, Susan Trumbore, Masahito Ueyama, Rodrigo Vargas, Ruth K. Varner, Joseph Verfaillie, Christoph Vogel, Jinsong Wang, Greg Winston, Tana E. Wood, Juying Wu, Thomas Wutzler, Jiye Zeng, Tianshan Zha, Quan Zhang, Junliang Zou

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Globally, soils store two to three times as much carbon as currently resides in the atmosphere, and it is critical to understand how soil greenhouse gas (GHG) emissions and uptake will respond to ongoing climate change. In particular, the soil-to-atmosphere CO2 flux, commonly though imprecisely termed soil respiration (RS), is one of the largest carbon fluxes in the Earth system. An increasing number of high-frequency RS measurements (typically, from an automated system with hourly sampling) have been made over the last two decades; an increasing number of methane measurements are being made with such systems …


Long Term Air Quality Analysis In Reference To Thermal Power Plants Using Satellite Data In Singrauli Region, India, H. K. Romana, Ramesh P. Singh, D. P. Shukla Aug 2020

Long Term Air Quality Analysis In Reference To Thermal Power Plants Using Satellite Data In Singrauli Region, India, H. K. Romana, Ramesh P. Singh, D. P. Shukla

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The exponentially growing population and related anthropogenic activities have led to modifications in local environment. The change in local environment, evolving pattern of land use, concentrations of greenhouse gases and aerosols alter the energy balance of our climate system. This alteration in climate is leading to pre-mature deaths worldwide. This study analyses the air quality of Singrauli region, Madhya Pradesh, India for the past 15 years. Otherwise known as Urjanchal “the energy capital” of India has been declared as critically polluted by CPCB. The study provides an updated list of thermal power plants in the study area and their emission …


Global Atmospheric Budget Of Acetone: Air-Sea Exchange And The Contribution To Hydroxyl Radicals, Siyuan Wang, Eric C. Apel, Rebecca H. Schwantes, Kelvin H. Bates, Daniel J. Jacob, Emily V. Fischer, Rebecca S. Hornbrook, Alan J. Hills, Louisa K. Emmons, Laura L. Pan, Shawn Honomichl, Simone Tilmes, Jean‐François Lamarque, Mingxi Yang, Christa A. Marandino, E. S. Saltzman, Warren J. De Bruyn, Sohiko Kameyama, Hiroshi Tanimoto, Yuko Omori, Samuel R. Hall, Kirk Ullmann, Thomas B. Ryerson, Chelsea R. Thompson, Jeff Peischl, Bruce C. Daube, Róisín Commane, Kathryn Mckain, Colm Sweeney, Alexander B. Thames, David O. Miller, William H. Brune, Glenn S. Diskin, Joshua P. Digangi, Steven C. Wofsy Jul 2020

Global Atmospheric Budget Of Acetone: Air-Sea Exchange And The Contribution To Hydroxyl Radicals, Siyuan Wang, Eric C. Apel, Rebecca H. Schwantes, Kelvin H. Bates, Daniel J. Jacob, Emily V. Fischer, Rebecca S. Hornbrook, Alan J. Hills, Louisa K. Emmons, Laura L. Pan, Shawn Honomichl, Simone Tilmes, Jean‐François Lamarque, Mingxi Yang, Christa A. Marandino, E. S. Saltzman, Warren J. De Bruyn, Sohiko Kameyama, Hiroshi Tanimoto, Yuko Omori, Samuel R. Hall, Kirk Ullmann, Thomas B. Ryerson, Chelsea R. Thompson, Jeff Peischl, Bruce C. Daube, Róisín Commane, Kathryn Mckain, Colm Sweeney, Alexander B. Thames, David O. Miller, William H. Brune, Glenn S. Diskin, Joshua P. Digangi, Steven C. Wofsy

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Acetone is one of the most abundant oxygenated volatile organic compounds (VOCs) in the atmosphere. The oceans impose a strong control on atmospheric acetone, yet the oceanic fluxes of acetone remain poorly constrained. In this work, the global budget of acetone is evaluated using two global models: CAM‐chem and GEOS‐Chem. CAM‐chem uses an online air‐sea exchange framework to calculate the bidirectional oceanic acetone fluxes, which is coupled to a data‐oriented machine‐learning approach. The machine‐learning algorithm is trained using a global suite of seawater acetone measurements. GEOS‐Chem uses a fixed surface seawater concentration of acetone to calculate the oceanic fluxes. Both …


Changes In Atmospheric, Meteorological, And Ocean Parameters Associated With The 12 January 2020 Taal Volcanic Eruption, Feng Jing, Akshansa Chauhan, Ramesh P. Singh, Prasanjit Dash Mar 2020

Changes In Atmospheric, Meteorological, And Ocean Parameters Associated With The 12 January 2020 Taal Volcanic Eruption, Feng Jing, Akshansa Chauhan, Ramesh P. Singh, Prasanjit Dash

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The Taal volcano erupted on 12 January 2020, the first time since 1977. About 35 mild earthquakes (magnitude greater than 4.0) were observed on 12 January 2020 induced from the eruption. In the present paper, we analyzed optical properties of volcanic aerosols, volcanic gas emission, ocean parameters using multi-satellite sensors, namely, MODIS (Moderate Resolution Imaging Spectroradiometer), AIRS (Atmospheric Infrared Sounder), OMI (Ozone Monitoring Instrument), TROPOMI (TROPOspheric Monitoring Instrument) and ground observations, namely, Argo, and AERONET (AErosol RObotic NETwork) data. Our detailed analysis shows pronounced changes in all the parameters, which mainly occurred in the western and south-western regions because the …


Methanethiol, Dimethyl Sulfide And Acetone Over Biologically Productive Waters In The Southwest Pacific Ocean, Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. De Bruyn, Eric S. Saltzman Mar 2020

Methanethiol, Dimethyl Sulfide And Acetone Over Biologically Productive Waters In The Southwest Pacific Ocean, Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. De Bruyn, Eric S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Atmospheric methanethiol (MeSHa), dimethyl sulfide (DMSa) and acetone (acetonea) were measured over biologically productive frontal waters in the remote southwest Pacific Ocean in summertime 2012 during the Surface Ocean Aerosol Production (SOAP) voyage. MeSHa mixing ratios varied from below the detection limit (< 10 ppt) up to 65 ppt and were 3 %–36 % of parallel DMSa mixing ratios. MeSHa and DMSa were correlated over the voyage (R2=0.3, slope = 0.07) with a stronger correlation over a coccolithophore-dominated phytoplankton bloom (R2=0.5, slope 0.13). The diurnal cycle for MeSHa shows similar behaviour to DMSa with mixing ratios …


Air/Sea Transfer Of Highly Soluble Gases Over Coastal Waters, J. G. Porter, Warren J. De Bruyn, S. D. Miller, E. S. Saltzman Jan 2020

Air/Sea Transfer Of Highly Soluble Gases Over Coastal Waters, J. G. Porter, Warren J. De Bruyn, S. D. Miller, E. S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The deposition of soluble trace gases to the sea surface is not well studied due to a lack of flux measurements over the ocean. Here we report simultaneous air/sea eddy covariance flux measurements of water vapor, sulfur dioxide (SO2), and momentum from a coastal North Atlantic pier. Gas transfer velocities were on average about 20% lower for SO2 than for H2O. This difference is attributed to the difference in molecular diffusivity between the two molecules (D SO 2/D H 2O = 0.5), in reasonable agreement with bulk parameterizations in air/sea gas …


Global Sinusoidal Seasonality In Precipitation Isotopes, Scott T. Allen, Scott Jasechko, Wouter R. Berghuijs, Jeffrey M. Welker, Gregory R. Goldsmith, James W. Kirchner Aug 2019

Global Sinusoidal Seasonality In Precipitation Isotopes, Scott T. Allen, Scott Jasechko, Wouter R. Berghuijs, Jeffrey M. Welker, Gregory R. Goldsmith, James W. Kirchner

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Quantifying seasonal variations in precipitation δ2H and δ18O is important for many stable isotope applications, including inferring plant water sources and streamflow ages. Our objective is to develop a data product that concisely quantifies the seasonality of stable isotope ratios in precipitation. We fit sine curves defined by amplitude, phase, and offset parameters to quantify annual precipitation isotope cycles at 653 meteorological stations on all seven continents. At most of these stations, including in tropical and subtropical regions, sine curves can represent the seasonal cycles in precipitation isotopes. Additionally, the amplitude, phase, and offset parameters of …