Condensed Matter Physics Commons^™

Electron Correlations In An Excited State Of A Quantum Dot In A Uniform Magnetic Field, Marlina Slamet, Viraht Sahni

Publications and Research

Electron correlations in a two-electron two-dimensional ‘artificial atom’ or quantum dot (with harmonic confining potential) in the presence of a uniform magnetic field in an excited singlet state are studied via quantal density functional theory (QDFT). QDFT allows for the separation of the electron correlations due to the Pauli exclusion principle and Coulomb repulsion, as well as the determination of the contribution of these correlations to the kinetic energy. The QDFT mapping is from the excited state of the quantum dot to one of noninteracting fermions in their ground state possessing the same basic variables of the density and physical …

Band-To-Band Transitions, Selection Rules, Effective Mass, And Excitonic Contributions In Monoclinic Β-Ga2o3, Alyssa Mock, Rafal Korlacki, Chad Briley, Vanya Darakchieva, Bo Monemar, Yoshinao Kumagai, Ken Goto, Masataka Higashiwaki, Mathias Schubert

Department of Electrical and Computer Engineering: Faculty Publications

We employ an eigenpolarization model including the description of direction dependent excitonic effects for rendering critical point structures within the dielectric function tensor of monoclinic β-Ga₂O₃ yielding a comprehensive analysis of generalized ellipsometry data obtained from 0.75–9 eV. The eigenpolarization model permits complete description of the dielectric response. We obtain, for single-electron and excitonic band-to-band transitions, anisotropic critical point model parameters including their polarization vectors within the monoclinic lattice. We compare our experimental analysis with results from density functional theory calculations performed using the Gaussian-attenuation-Perdew-Burke-Ernzerhof hybrid density functional. We present and discuss the order of the …

Comment On “Electronic Structure Of Mo(1−X)Rex Alloys Studied Through Resonant Photoemission Spectroscopy”, Prescott Evans, Peter A. Dowben

Peter Dowben Publications

Further analysis of the resonant photoemission data, found within Sundar et al (2016 J. Phys.: Condens. Matter 28 315502), show the intensities do not follow the elemental composition in the Mo_1−xRe_x alloy. Similar trends are observed in the published data for Gd_1−xNi_x alloy films. The analysis of the resonant photoemission intensities suggests that Mo in the Mo_1−xRe_x alloy and Gd in the Gd_1−xNi_x alloy have nearest neighbor bonds to Re and Ni respectively. This means the A–B bond is favored over the average of …

Anomalous Photovoltaic Effect In Organic-Inorganic Hybrid Perovskite Solar Cells, Yongbo Yuan, Tao Li, Qi Wang, Jie Xing, Alexei Gruverman, Jinsong Huang

Alexei Gruverman Publications

Organic-inorganic hybrid perovskites (OIHPs) have been demonstrated to be highly successful photovoltaic materials yielding very-high-efficiency solar cells. We report the room temperature observation of an anomalous photovoltaic (APV) effect in lateral structure OIHP devices manifested by the device’s open-circuit voltage (V_OC) that is much larger than the bandgap of OIHPs. The persistent V_OC is proportional to the electrode spacing, resembling that of ferroelectric photovoltaic devices. However, the APV effect in OIHP devices is not caused by ferroelectricity. The APV effect can be explained by the formation of tunneling junctions randomly dispersed in the polycrystalline films, which allows …

Ch3Nh3Pbi3 Perovskites: Ferroelasticity Revealed, Evgheni Strelcov, Qingfeng Dong, Tao Li, Jungseok Chae, Yuchuan Shao, Yehao Deng, Alexei Gruverman, Jinsong Huang, Andrea Centrone

Alexei Gruverman Publications

Ferroelectricity has been proposed as a plausible mechanism to explain the high photovoltaic conversion efficiency in organic-inorganic perovskites; however, convincing experimental evidence in support of this hypothesis is still missing. Identifying and distinguishing ferroelectricity from other properties, such as piezoelectricity, ferroelasticity, etc., is typically nontrivial because these phenomena can coexist in many materials. In this work, a combination of microscopic and nanoscale techniques provides solid evidence for the existence of ferroelastic domains in both CH₃NH₃PbI₃ polycrystalline films and single crystals in the pristine state and under applied stress. Experiments show that the configuration of CH …

Generalization Of The Schrödinger Theory Of Electrons, Viraht Sahni

Publications and Research

The Schrödinger theory for a system of electrons in the presence of both a static and time-dependent electromagnetic field is generalized so as to exhibit the intrinsic self-consistent nature of the corresponding Schrödinger equations. This is accomplished by proving that the Hamiltonian in the stationary-state and time-dependent cases {\hat{H}; \hat{H}(t)} are exactly known functionals of the corresponding wave functions {\Psi; \Psi(t)}, i.e. \hat{H} = \hat{H}[\Psi] and \hat{H}(t) = \hat{H}[\Psi(t)]. Thus, the Schrödinger equations may be written as \hat{H}[\Psi]\Psi = E[\Psi]\Psi and \hat{H}[\Psi(t)]\Psi(t) = i\partial\Psi(t)/\partial t. As a consequence the eiegenfunctions and energy eigenvalues {\Psi; E} of the stationary-state equation, and …

Schrödinger Theory Of Electrons In Electromagnetic Fields: New Perspectives, Viraht Sahni, Xiao-Yin Pan

Publications and Research

The Schrödinger theory of electrons in an external electromagnetic field is described from the new perspective of the individual electron. The perspective is arrived at via the time-dependent "Quantal Newtonian" law (or differential virial theorem). (The time-independent law, a special case, provides a similar description of stationary-state theory). These laws are in terms of "classical" fields whose sources are quantal expectations of Hermitian operators taken with respect to the wave function. The laws reveal the following physics: (a) in addition to the external field, each electron experiences an internal field whose components are representative of a specific property of the …

Study Of The Photoluminescence Spectra Of Mg-Doped Gan, Puranjan Ghimire

Theses and Dissertations

We have studied luminescence properties of Mg-doped GaN grown by hydride vapor phase epitaxy. Steady state photoluminescence (PL) spectra have been analyzed. Exciton, ultraviolet luminescence (UVL) and blue luminescence (BL) bands are the dominant PL bands in the spectra. At low temperature, Exciton and UVL bands show almost no shift with excitation intensity, whereas the BL band blueshifts by almost 0.4 ���� with increasing excitation intensity by seven orders of magnitude. Such shifting nature of bands with excitation intensity is explained by assuming that the BL band is detected from the region of the sample where potential fluctuations are very …

Dirac Surface States Of Magnetic Topological Insulators, Seng Huat Lee

Doctoral Dissertations

"Magnetic topological insulator (TI) has been theoretically proposed to be a platform for inducing magnetic monopole and exhibit fascinating quantum phenomena, whereas topological superconductor can host Majorana fermions, particles that are their own antiparticles, which can be manipulated for topological quantum computing. In this dissertation, we experimentally demonstrated that by intercalation of different transition metals in the van der Waals gaps of Bi₂Se₃ TI, magnetism and even superconductivity can be induced. In Fe_xBi₂Se₃, antiferromagnetism is induced with a transition temperature at ~ 100 K. Coexistence of the Dirac surface state with …

Femtosecond Laser Induced Structural Dynamics And Melting Of Cu (111) Single Crystal. An Ultrafast Time-Resolved X-Ray Diffraction Study, Runze Li, Omar A. Ashour, Jie Chen, H. E. Elsayed-Ali, Peter M. Rentzepis

Electrical & Computer Engineering Faculty Publications

Femtosecond, 8.04 keV x-ray pulses are used to probe the lattice dynamics of a 150 nm Cu (111) single crystal on a mica substrate irradiated with 400 nm, 100 fs laser pulses. For pump fluences below the damage and melting thresholds, we observed lattice contraction due to the formation of a blast force and coherent acoustic phonons with a period of ∼69 ps. At larger pump fluence, solid to liquid phase transition, annealing, and recrystallization were measured in real time by monitoring the intensity evolution of the probing fs x-ray rocking curves, which agreed well with theoretical simulation results. The …

Light Soaking Phenomena In Organic-Inorganic Mixed Halide Perovskite Single Crystals, Hye Ryung Byun, Dae Young Park, Hye Min Oh, Gon Namkoong, Mun Seok Jeong

Electrical & Computer Engineering Faculty Publications

Recently, organic inorganic mixed halide perovskite (MAPbX₃; MA = CH₃NH₃^+, X = Cl^-, Br^-, or I^-) single crystals with low defect densities have been highlighted as candidate materials for high-efficiency photovoltaics and optoelectronics. Here we report the optical and structural investigations of mixed halide perovskite (MAPbBr_3-xI_x) single crystals. Mixed halide perovskite single crystals showed strong light soaking phenomena with light illumination conditions that were correlated to the trapping and detrapping events from defect sites. By systematic investigation with optical analysis, we found that the …

Tuning The Effective Electron Correlation In Iridate Systems Featuring Strong Spin-Orbit Interaction, John H. Gruenewald

Theses and Dissertations--Physics and Astronomy

The 5d transition metal oxides have drawn substantial interest for predictions of being suitable candidates for hosting exotic electronic and magnetic states, including unconventional superconductors, magnetic skyrmions, topological insulators, and Weyl semimetals. In addition to the electron-electron correlation notable in high-temperature 3d transition metal superconductors, the 5d oxides contain a large spin-orbit interaction term in their ground state, which is largely responsible for the intricate phase diagram of these materials. Iridates, or compounds containing 5d iridium bonded with oxygen, are of particular interest for their spin-orbit split J_eff = 1/2 state, which is partially filled without the presence …

Deconfined Quantum Criticality In 2d Su(N) Magnets With Anisotropy, Jonathan D'Emidio

Theses and Dissertations--Physics and Astronomy

In this thesis I will outline various quantum phase transitions in 2D models of magnets that are amenable to simulation with quantum Monte Carlo techniques. The key player in this work is the theory of deconfined criticality, which generically allows for zero temperature quantum phase transitions between phases that break distinct global symmetries. I will describe models with different symmetries including SU(N), SO(N), and "easy-plane" SU(N) and I will demonstrate how the presence or absence of continuous transitions in these models fits together with the theory of deconfined criticality.

Thermal Conductivities Of Organic Semiconductors, Yulong Yao

Theses and Dissertations--Physics and Astronomy

Organic semiconductors have gained a lot of interest due to their ease of processing, low-cost and inherent mechanical flexibility. Although most of the research has been on their electronic and optical properties, knowledge of the thermal properties is important in the design of electronic devices as well. Our group has used ac-calorimetric techniques to measure both in-plane and transverse thermal conductivities of a variety of organic semiconductors including small-molecule crystals and polymer blends. For layered crystals composed of molecules with planar backbones and silylethynyl (or germylethynyl) sidegroups projecting between the layers, very high interplanar thermal conductivities have been observed, presumably …

How Shape Of Simulated Graphene Sheets Affects Debye Scattering Patterns, Lindsay Lesh

Honors Projects

This research is about understanding the structure of a subset of graphitic stardust found in primitive meteorites (e.g. the Murchison meteorite). The carbon grains of interest exhibit a core-rim structure, where the core – with a density less than that of the graphitic rim – comprises the majority of the grain. Previous studies have shown that the cores are comprised primarily of unlayered graphene, and it has been hypothesized that the cores are the result of the rapid freezing (quenching) of a liquid carbon droplet. Electron diffraction is sensitive to small differences in crystal structure and simulated electron diffraction powder …

Linear Feedback Stabilization For A Continuously Monitored Qubit, Taylor Lee Patti, A. Chantasri, Justin Dressel, A. N. Jordan

Student Scholar Symposium Abstracts and Posters

In quantum mechanics, standard or strong measurement approaches generally result in the collapse of an ensemble of wavefunctions into a stochastic mixture of eigenstates. On the other hand, continuous or weak measurements have the propensity to dynamically control the evolution of quantum states over time, guiding the trajectory of the state into non-trivial superpositions and maintaining state purity. This kind of measurement-induced state steering is of great theoretical and experimental interest for the harnessing of quantum bits or "qubits", which are the fundamental unit of the emerging quantum computer. We explore continuous measurement-based quantum state stabilization through linear feedback control …

Artificial Quantum Many-Body States In Complex Oxide Heterostructures At Two-Dimensional Limit, Xiaoran Liu

Graduate Theses and Dissertations

As the representative family of complex oxides, transition metal oxides, where the lattice,

charge, orbital and spin degrees of freedom are tightly coupled, have been at the forefront

of condensed matter physics for decades. With the advancement of state-of-the-art heteroepitaxial deposition techniques, it has been recognized that combining these oxides on the atomic scale, the interfacial region offers great opportunities to discover emergent phenomena and tune materials' functionality. However, there still lacks general guiding principles for experimentalists, following which one can design and fabricate artificial systems on demand. The main theme of this dissertation is to devise and propose some …

Plasma Processes And Polymers Third Special Issue On Plasma And Cancer, Mounir Laroussi, Annemie Bogaerts, Nazir Barekzi

Electrical & Computer Engineering Faculty Publications

(First paragraph) This issue of Plasma Processes and Polymers is the third in a series on the applications of low temperature plasma (LTP) against cancer, or “plasma oncology.” The papers in this issue are inspired from the talks given at the third International Workshop on Plasma for Cancer Treatment (IWPCT) which took place on April 11–12, 2016 in Washington, DC, USA. IWPCT is an international workshop that was created in 2014 as a venue to share cutting edge plasma oncology research. The first IWPCT was held in Washington DC, under the co-chairmanship of Prof. Mounir Laroussi (Old Dominion University) and …

Avalanche Statistics From Data With Low Time Resolution, Michael Leblanc, Aya Nawano, Wendelin J. Wright, Xiaojun Gu, Jonathan T. Uhl, Karin A. Dahmen

Faculty Journal Articles

Extracting avalanche distributions from experimental microplasticity data can be hampered by limited time resolution. We compute the effects of low time resolution on avalanche size distributions and give quantitative criteria for diagnosing and circumventing problems associated with low time resolution. We show that traditional analysis of data obtained at low acquisition rates can lead to avalanche size distributions with incorrect power-law exponents or no power-law scaling at all. Furthermore, we demonstrate that it can lead to apparent data collapses with incorrect power-law and cutoff exponents. We propose new methods to analyze low-resolution stress-time series that can recover the size distribution …

Properties Of The Schrödinger Theory Of Electrons In Electromagnetic Fields, Viraht Sahni, Xiao-Yin Pan

Publications and Research

The Schrödinger theory of electrons in an external electromagnetic field can be described from the perspective of the individual electron via the ‘Quantal Newtonian’ laws (or differential virial theorems). These laws are in terms of ‘classical’ fields whose sources are quantal expectations of Hermitian operators taken with respect to the wave function. The laws reveal the following physics: (a) In addition to the external field, each electron experiences an internal field whose components are representative of a specific property of the system such as the correlations due to the Pauli exclusion principle and Coulomb repulsion, the electron density, kinetic effects, …