Condensed Matter Physics Commons^™

Optical Studies Of Wide Bandgap Photonic Materials, Nikesh Maharjan

Dissertations, Theses, and Capstone Projects

In this dissertation work, optical properties of wide bandgap materials such as hexagonal Boron Nitride (h-BN) and Zinc Oxide (ZnO) have been studied. Deep UV photoluminescence spectroscopy was employed to study the optical properties of bulk h-BN and powder crystals using a laser of wavelength 200 nm, which is the fourth harmonic of Ti:Sapphire laser as excitation source. The properties and chemical compositions of annealed and unannealed bulk h-BN were investigated. The PL spectra from h-BN samples annealed at 900 ºC in ambient air, had strong phonon assisted band edge emissions along with a sharp atomic-like emission line at 4.09 …

Magnetism Of Novel Rare-Earth-Free Intermetallic Compounds, Haohan Wang

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Rare-earth-free magnets have drawn lots of interest because of their low cost, and the production is not limited by the shortage of rare-earth elements. This dissertation focuses on three rare-earth-free materials, Fe-Co-Ti alloys, Fe-Ni-B alloys, and Co-Si. All of them are synthesized by arc melting followed by melt-spinning. Fe_3+xCo_3−xTi₂ (x = 0, 2, 3) alloys exhibit hexagonal crystal structures and show non-collinear spin structures according to neutron diffraction. The magnetic moments have projections on both the c-axis and basal plane, and the corresponding misalignment angle exhibits a nonlinear decrease with …

Investigation Of Topological Phonons In Acoustic Metamaterials, Wenting Cheng

Dissertations

Topological acoustics is a recent and intense area of research. It merges the knowledge of mathematical topology, condensed matter physics, and acoustics. At the same time, it has been pointed out that quasiperiodicity can greatly enhance the periodic table of topological systems. Because quasiperiodic patterns have an intrinsic global degree of freedom, which exists in the topological space called the hull of a pattern, where the shape traced in this topological space is called the phason. The hull augments the physical space, which opens a door to the physics of the integer quantum Hall effect (IQHE) in arbitrary dimensions. In …

Correlations Between The Rotations And Magnetospheres Of The Terrestrial Planets And The Sun's Formation In Our Solar System, Fred J. Cadieu

Publications and Research

Correlations between the rotations of the terrestrial planets in our solar system and the magnetic field of the Sun have been previously noted. These correlations account for the opposite rotation of Venus as a result of the magnetic field of the Sun being dragged across the conducting core of Venus. Currently the Sun’s magnetic field is not sufficiently strong to account for the proposed correlations. But recently meteorite paleomagnetism measurements have indicated that during the Sun’s formation the magnetic field of the Sun was of sufficient strength to have resulted in the observed correlations. As a part of these correlations …

Controlling Magnetic Exchange And Anisotropy By Nonmagnetic Ligand Substitution In Layered M P X 3 ( M = Ni , Mn; X = S , Se), Rabindra Basnet, Kamila M. Kotur, Milosz Rybak, Cory Stephenson, Samuel Bishop, Carmine Autieri, Magdalena Birowska, Jin Hu

Physics Faculty Publications and Presentations

Recent discoveries in two-dimensional magnetism have intensified the investigation of van der Waals magnetic materials and further improved our ability to tune their magnetic properties. Tunable magnetism has been widely studied in antiferromagnetic metal thiophosphates MPX3. Substitution of metal ions M has been adopted as an important technique to engineer the magnetism in MPX3. In this work, we have studied the previously unexplored chalcogen X substitutions in MPX3 (M=Mn/Ni; X=S/Se). We synthesized the single crystals of MnPS3−xSex (0≤x≤3) and NiPS3−xSex (0≤x≤1.3) and investigated the systematic evolution of the magnetism with varying x. Our study reveals the effective tuning of magnetic …

Nonequilibrium And Nonlinear Dynamics In Collective Spin Models And Implementations Using Quantum Feedback Control, Manuel H. Munoz Arias

Physics & Astronomy ETDs

Out-of-equilibrium dynamics generalizes the study of ground states of quantum Hamiltonians at zero temperature, to that of dynamical quasi-steady states of quantum systems far from equilibrium. In this dissertation I discuss dynamical quantum phase transitions and out-of-equilibrium phases of matter in models of collective spins with multi-body interactions. These models, based on collective degrees of freedom, allow an exact description of the thermodynamic limit via the mean-field description. In this limit, the nonequilibrium dynamics of properties of quantum states is mapped to the nonlinear dynamics of classical variables, and thus it can be analyzed using tools from the theory of …

Bio-Based Antibacterial Packaging From Decorated Bagasse Papers With Natural Rosin And Synthesised Go-Ag Nanoparticles, Mohamed Morsy

Nanotechnology Research Centre

No abstract provided.

The Interaction Of Topological Defects In Anisotropically-Elastic Nematic Liquid Crystals, Carter J. Swift

Macalester Journal of Physics and Astronomy

Topological defects are very well understood so long as the medium in which they exist is isotropically-elastic. They lead to director fields which are easy to calculate and superpose linearly so that a system with any number of defects is analytically treatable. They also have an interaction which is simple in form and can be accurately described by the Peach-Koehler force. In an anisotropically-elastic medium, however, such defects are very poorly understood outside of the single-defect case which was solved by Dzyaloshinskii. In this project, numerical and approximate analytical techniques are applied in order to better understand the interaction between …

Finite-Difference-Time-Domain Simulation Of Ultrafast Experiments, Alpha Ma

Macalester Journal of Physics and Astronomy

The Finite-Difference-Time-Domain (FDTD) method is a numerical method that calculates electric fields or magnetic fields by interleaving them in space and time. Using a python package called “MEEP”, I was able to write optical simulations of ultrafast experiments, especially the Terahertz Pump-Probe experiments. The goal of this project was to use FDTD simulation to measure the transmission of an electro-magnetic pulse passing through a thin film of conducting material on a dielectric substrate in order to study the characteristic conductivity of potential solar cell materials.

Approaching Quantum-Limited Electrometry In The Single-Photon Regime, Sisira Kanhirathingal

Dartmouth College Ph.D Dissertations

Mesoscopic quantum systems currently serve as essential building blocks in many quantum information and metrology devices. This thesis investigates the potential of quantum-limited detection in a mesoscopic electrometer named the cavity-embedded Cooper pair transistor (cCPT). As one application, this charge detector can act as the basis for an optomechanical system in the single-photon strong coupling regime. The realization of this scheme would entail near quantum-limited, ultra-sensitive electrometry at the single-photon level, the feasibility of which is studied at length in this thesis.

On the one hand, we approach this question using a fundamental, first-principles study, where an operator scattering model …

Synthesis, Characterization, And Functionality Of Novel 2d Material Sn3p2, Cory Stephenson

Physics Undergraduate Honors Theses

In recent years, two-dimensional (2D) materials have gained a lot of attention due to their potential applications in devices and their promise to revolutionize technology. In our group, we are capable of synthesizing such materials and study their properties. I have discovered a new material of the tin-phosphorus family that displays the 2D layered structure and therefore shows potential to be used in future devices due to this reduced dimensionality from the typical three-dimensional counterpart. This 2D structure may allow for new phenomena to emerge as there is no longer any interatomic interactions along the z- axis. Under this motivation, …

Towards Highly Sensitive Capacitance Measurements Of A Quantum Anomalous Hall Phase In Van Der Waal Heterostructures, Kayla Cerminara

UNLV Theses, Dissertations, Professional Papers, and Capstones

One of the pioneering achievements in condensed matter physics of the 20th century is the observation of the quantum Hall e↵ect (QHE) in which the Hall resistance in a two-dimensional (2D) sample takes on quantized values in the presence of a strong perpendicular magnetic field. The precise quantization of the hall resistance to one part in a billion has provided a practical, worldwide resistance standard. A long-standing goal has been to realize a similar state of matter but without the need of a strong quantizing magnetic field. The quantum anomalous Hall e↵ect (QAHE) is such a state that is predicted …

Exploring Tunable Magnetization And High-Temperature Ferromagnetism In Ternary Transition Metal-Based Chalcogenides, Hector Iturriaga

Open Access Theses & Dissertations

The discovery of long-range magnetic ordering in ultrathin transition metal-based compounds shows great promise for the development of nanoscale memory and spintronic devices. Composed of cost-effective materials and boasting from strong chemical and thermal stability at low dimensions, van der Waals (vdW) ternary transition metal chalcogenide magnets like CrSiTe3 (CST), Fe2.7GeTe2 (FGT), and Mn3Si2Te6 (MST), provide not only possible energy solutions, but also a broad platform to explore the versatile magnetic character of this family of compounds. Although they have great potential, it has been found that their long-range magnetic ordering exists at temperatures far too low (the highest of …

Evolution Of The Magnetic Properties On Van Der Waals Layered Magnets Via Pressure And Proton Irradiation, Rubyann Olmos

Open Access Theses & Dissertations

Probing the magnetism in quasi two-dimensional materials has the potential in driving their properties towards future use in spin electronic based devices. Studying such layered magnets will enable the scientific community to uncover tunable exotic phases such as superconductivity, quantum paramagnetism, etc. This work examines the influence of two types of external perturbations, namely, the pressure and proton irradiation, on the magnetic properties of several compounds in the van der Waals crystal family.

Pressure has been found to induce structural and magnetic phase transitions in many of these materials. Using hydrostatic pressure as a disorderless approach to manipulate the interlayer …

Ab Initio Studies Of Structure And Properties Of Group-Iv Monochalcogenide Monolayers, Shiva Prasad Poudel

Graduate Theses and Dissertations

The goal of this dissertation is to study the structure of ferroelectric group-IV monochalcogenide monolayers (MMLs) and their material properties. This work also established a new buckled honeycomb phase of these monolayers. Chapter 1 serves as an introduction where the motivation for these studies is established. In chapter 2, I used eight different exchange-correlation functionals (XC) to study the structure of these 2D ferroelectrics and found that their properties are independent of the choice of XC functionals. These findings reveal that the ground-state ferroelectric unit cell can be described by only five independent parameters, whereas their paraelectric (square or rectangular) …

Crystal Growth And Property Tuning Of Layered Magnetic Topological Semimetals, Krishna Pandey

Graduate Theses and Dissertations

The demand for energy-efficient devices has been growing rapidly due to the need for data-driven technologies and the global energy crisis. As device size approaches the atomic scale, the miniaturization of electronic devices may stop in the near future unless fundamentally new materials or device concepts are developed. The emergent topological materials with exotic properties show remarkable robustness against crystal lattice defects, which are promising for next-generation technology. These materials host exotic properties such as high mobility, large magnetoresistance, chiral anomaly, and surface Fermi arcs, etc. Among various topological materials, the ZrSiS-family materials exhibit two types of Dirac states, which …

Tuning Properties Of Topological Insulators: An Ab-Initio Approach, Karunya Shailesh Shirali

LSU Doctoral Dissertations

This thesis develops a first-principles based approach to explore the tuning of topological properties of the tetradymite topological insulators. We begin by setting up a framework to systematically obtain the bulk and surface properties of topological insulators, treating the structural and electronic properties on an equal footing. We determine a consistent method for including the van der Waals interactions, which are responsible for the weak coupling between sets of atomic layers in this family of layered materials, which is important in obtaining accurate structural properties. We obtain close agreement with experimental values for both the bulk and surface states.

To …

Synthesis And Characterization Of Chiral Magnetic Oxide: Mnmoteo6, Chase Hames, August Meads

Symposium of Student Scholars

The chiral materials lack mirror reflection symmetry in their crystal structures like right and left hands. Such materials often host unique non-collinear or topological magnetic textures such as magnetic skyrmions. If such magnetic textures are formed in insulating oxides with coupled electric and magnetic properties, then such magnetic structures can be controlled and manipulated using electric fields rather than electric current. With this motivation, we are synthesizing and characterizing chiral materials belonging to MMoTeO₆ (M=Mn, Co, Fe, Cu, Ni) family. I will discuss about the phase formation and solid-state synthesis of MnTeMoO₆ along with its structural, electrical and …

Modeling The Effects Of Surface Roughness On Electron Yield, Trace Taylor, Matthew Robertson, Jr Dennison

Conference Proceedings

Surface conditions—including surface morphology, composition, contamination, and oxidation—can significantly affect electron yields and consequently spacecraft charging. The effects of surface roughness on electron yield are modeled in this study by considering four aspects of electron yield calculations: (i) simple models of rough surface geometry, (ii) the angular distributions of electrons emitted from various points on these surfaces, (iii) the likelihood of these emitted electrons escaping the rough surface, and (iv) the relative fractions of smooth and rough surfaces. Three simple periodic one-dimensional surface profiles were considered—namely rectangular, triangular, and sawtooth features; each surface profile was characterized by an aspect ratio …

Laboratory Simulations Of Simultaneous Reduced Gravity And Ionizing Radiation Environments, Achal Duhoon, Jr Dennison

Conference Proceedings

A novel system has been developed to simulate the combined effects of reduced gravity and ionizing radiation present during spaceflight on biological and particulate samples. The miniature rotary cell culture system (mRCCS) was designed to synchronously rotate up to five independent vessels containing particulate samples suspended in fluid media, constructed using radiation tolerant, biocompatible, and vacuum compatible materials. Reduced gravity conditions were achieved when particles (e.g., 200 µm polystyrene microcarrier beads with or without adhered cell clusters) were suspended inside the vessels moving near terminal velocity in viscous fluid media with densities matched to the suspended …