Atomic, Molecular and Optical Physics Commons^™

Chiral Spin Textures In Amorphous Iron–Germanium Thick Films, Robert Streubel, D. Simca Bouma, Frank Bruni, Xiaoqian Chen, Peter Ercius, Jim Ciston, Alpha T. N'Diaye, Sujoy Roy, Steve D. Kevan, Peter Fischer, Frances Hellman

Robert Streubel Papers

Topological solitary fields, such as magnetic and polar skyrmions, are envisioned to revolutionize microelectronics. These configurations have been stabilized in solid-state materials with a global inversion symmetry breaking, which translates in magnetic materials into a vector spin exchange known as the Dzyaloshinskii–Moriya interaction (DMI), as well as spin chirality selection and isotropic solitons. This work reports experimental evidence of 3D chiral spin textures, such as helical spins and skyrmions with different chirality and topological charge, stabilized in amorphous Fe–Ge thick films. These results demonstrate that structurally and chemically disordered materials with a random DMI can resemble inversion symmetry broken systems …

Photoinduced Trapping Of Charge At Sulfur Vacancies And Copper Ions In Photorefractive Sn2P2S6 Crystals, Timothy D. Gustafson, Eric M. Golden, Elizabeth M. Scherrer, Nancy C. Giles, A. A. Grabar, Sergey A. Basun, Jonathan E. Slagle [*], Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) is used to monitor photoinduced changes in the charge states of sulfur vacancies and Cu ions in tin hypothiodiphosphate. A Sn₂P₂S₆ crystal containing Cu+ (3d10) ions at Sn²⁺ sites was grown by the chemical vapor transport method. Doubly ionized sulfur vacancies (V²⁺S) are also present in the as-grown crystal (where they serve as charge compensators for the Cu+ ions). For temperatures below 70 K, exposure to 532 or 633 nm laser light produces stable Cu²⁺ (3d⁹) ions, as electrons move from Cu⁺ ions to …

Interactions Of Organic Fluorophores With Plasmonic Surface Lattice Resonances, Robert J. Collison

Dissertations, Theses, and Capstone Projects

It is common knowledge that metals, alloys and pure elements alike, are lustrous and reflective, the more so when a metal surface is flat, polished, and free from oxidation and surface fouling. However, some metals reflect visible light, in the 380 nm to 740 nm range of wavelengths, much more strongly than others. In particular, some metals reflect wavelengths in certain portions of the ultraviolet (UV), visible, and near-infrared (NIR) regime, let us say 200 nm to 2000 nm, while absorbing light strongly in other segments of this range. There are several factors that account for this difference between various …

Characterization Of Spatial-Mode Properties In Few-Mode Fiber Bragg Gratings And Its Applications, Muhammad Khairol Annuar Zaini

Student Works (2020-2029)

Recently, few-mode fiber (FMF) has gained much research attention compared to single mode fiber (SMF) due to its capability to overcome the capacity limit. FMF based fiber sensors have many distinctive advantages such as cost efficiency, great sensitivity, and have the ability to employ the spatial dimension for multi-parameter sensing with discrimination capability. In this work, an analytical model has been proposed to investigate the relationship of the resonant wavelength shift of a few-mode FBG (FMFBG) to the axial stress of the FMF. By applying the proposed model, the axial stress of an FMFs was determined. Besides, the polariscopic technique …

Development Of A Modular Mixed-Radiation Directional Rotating Scatter Mask Detection System, Bryan V. Egner, Darren E. Holland, Larry W. Burggraf, James E. Bevins

Faculty Publications

The ability to simultaneously identify the direction of both fast neutrons, above 1 MeV, and gamma rays using a light-weight system consisting of a single 1” EJ-309 organic liquid scintillator and a plastic Spartan rotating scatter mask (RSM) is demonstrated computationally through Monte Carlo simulations and validated with experimental measurements. Two sets of directional measurements were performed with an americium–beryllium source, emitting both neutrons and gamma rays. The RSM identified the direction of the source within one 10° rotational increment in the azimuthal and polar directions based on both the neutron and gamma-ray induced signals discriminated by charge integration pulse-shape …

Structure Retrieval In Liquid-Phase Electron Scattering, Jie Yang, J. Pedro F. Nunes, Kathryn Ledbetter, Elisa Biasin, Martin Centurion, Zhijiang Chen, Amy A. Cordones, Christopher Crissman, Daniel P. Deponte, Siegfried H. Glenzer, Ming Fu Lin, Mianzhen Mo, Conor D. Rankine, Xiaozhe Shen, Thomas J.A. Wolf, Xijie Wang

Martin Centurion Publications

Electron scattering on liquid samples has been enabled recently by the development of ultrathin liquid sheet technologies. The data treatment of liquid-phase electron scattering has been mostly reliant on methodologies developed for gas electron diffraction, in which theoretical inputs and empirical fittings are often needed to account for the atomic form factor and remove the inelastic scattering background. In this work, we present an alternative data treatment method that is able to retrieve the radial distribution of all the charged particle pairs without the need of either theoretical inputs or empirical fittings. The merits of this new method are illustrated …

Ultrafast Thermal Modification Of Strong Coupling In An Organic Microcavity, Bin Liu, Vinod M. Menon, Matthew Y. Sfeir

Advanced Science Research Center

There is growing interest in using strongly coupled organic microcavities to tune molecular dynamics, including the electronic and vibrational properties of molecules. However, very little attention has been paid to the utility of cavity polaritons as sensors for out-of-equilibrium phenomena, including thermal excitations. Here, we demonstrate that non-resonant infrared excitation of an organic microcavity system induces a transient response in the visible spectral range near the cavity polariton resonances. We show how these optical responses can be understood in terms of ultrafast heating of electrons in the metal cavity mirror, which modifies the effective refractive index and subsequently the strong …

Visualizing The Electronic Structure Of Atoms, Ryan J. Bouman, Roger Dekock

Summer Research

There are three aspects of the electronic structure of atoms that confront the university student. All three arise in Hartree-Fock (HF) theory, which is foundational to understanding the periodic table. These aspects are: 1) Electron probability distributions of oneelectron atomic orbitals. 2) One-electron orbital energies. 3) How 1) and 2) relate to the total atomic energy and the total electron probability distribution. The goal of our work is to build a website that will employ a long-neglected model, first introduced by Slater and Zener (SZ). HF theory requires a knowledge of calculus, differential equations, and the ability to solve many …

Mot-Based Lifetime Measurements Of Potassium-39 5p1/2 And 5p3/2 States, Huan Q. Bui

Honors Theses

This thesis presents measurements of the lifetimes of 5p1/2 and 5p3/2 of K39 via exciting a cloud of K39 atoms in a magneto-optical trap by a linearly-polarized pulse of 405 nm light followed polarization-specific, time-resolved fluorescence detection. We find that $\tau_{5p1/2} = $ 138.8 $\pm$ 1.6 ns, which is consistent with past measurements \cite{triumf}, \cite{berends} and calculations \cite{safranova}. The $\tau_{5p3/2}$ measurement is naturally more involved since quantum beats due to hyperfine and Zeeman effect are present. Our observation of $\tau_{5p3/2} =$ 137.6 $\pm$ 3.1 ns and $\tau_{5p3/2} =$ 136.0 $\pm$ 2.4 ns, obtained from two slightly different approaches, are compared …

Transmission Zeros With Topological Symmetry In Complex Systems, Yuhao Kang, Azriel Genack

Publications and Research

Understanding vanishing transmission in Fano resonances in quantum systems and metamaterials and perfect and ultralow transmission in disordered media, has advanced the understanding and applications of wave interactions. Here we use analytic theory and numerical simulations to understand and control the transmission and transmission time in complex systems by deforming a medium and by adjusting the level of gain or loss. Unlike the zeros of the scattering matrix, the position and motion of the zeros of the determinant of the transmission matrix in the complex plane of frequency and field decay rate have robust topological properties. In systems without loss …

Molecular Spectroscopy For Innovative Physics: Alcl & Baf, Alex Preston

Pomona Senior Theses

This thesis is inspired by recent developments in the realm of fundamental physics. Spectroscopic studies on diatomic molecules are at the forefront of such endeavors. High-precision microwave spectroscopy probing the rotational energy level transitions of the molecules AlCl and BaF are analyzed at length in this work. The frequency data for these molecules are evaluated using the programs SPFIT and SPCAT in order to develop a “global fit” numerical model of the rotational, vibrational, nuclear, and hyperfine parameters characterizing the systems. Born-Oppenheimer breakdown terms used to amend inconsistencies in the spectral coefficients are determined for both systems. Previously published data …

One-Dimensional Lateral Force Anisotropy At The Atomic Scale In Sliding Single Molecules On A Surface, Yuan Zhang, Daniel J. Trainer, Badri Narayanan, Yang Li, Anh T. Ngo, Sushila Khadka, Arnab Neogi, Brandon Fisher, Larry A. Curtiss, Subramanian K.R.S. Sankaranarayanan, Saw Wai Hla

Physics Faculty Publications

Using a q+ atomic force microscopy at low temperature, a sexiphenyl molecule is slid across an atomically flat Ag(111) surface along the direction parallel to its molecular axis and sideways to the axis. Despite identical contact area and underlying surface geometry, the lateral force required to move the molecule in the direction parallel to its molecular axis is found to be about half of that required to move it sideways. The origin of the lateral force anisotropy observed here is traced to the one-dimensional shape of the molecule, which is further confirmed by molecular dynamics simulations. We also demonstrate that …

Laser Chirping In Inverse Compton Sources At High Electron Beam Energies And High Laser Intensities, Balŝa Terzić, Jeffrey Mckaig, Erik Johnson, Tabin Dharanikota, Geoffrey A. Krafft

Physics Faculty Publications

The onset of nonlinear effects, such as ponderomotive broadening, increases the radiation bandwidth and thereby places a stringent limitation on the laser intensity used in inverse Compton sources. Recently, we have shown that a judicious longitudinal laser frequency modulation ("chirping") can perfectly compensate for this ponderomotive broadening and restore the narrow band property of scattered radiation in the Thomson regime, when electron recoil during the collision with the laser can be neglected. Consequently, using QED, the laser chirping has been extended to the Compton regime, where electron recoil is properly accounted for. Here we present a new, semiclassical model for …

Environmental Modifications Of Atomic Properties: The Ground And 1s2p Excited States Of Compressed Helium, N. C. Pyper, T. C. Naginey, Colm T. Whelan

Physics Faculty Publications

Atoms remaining as recognizably distinct constituents of bulk condensed phases can have properties modified from those of the isolated species. Dense helium bubbles at high pressures are a common form of radiation damage degrading the mechanical and electrical properties of host materials. Detailed knowledge is critical for predicting their long term performance. Modifications of the ground and first singlet excited states of confined compressed helium are investigated using an entirely non-empirical theory based on the results of ab initio self-consistent field calculations with corrections for the effects of electron correlation. For finite sized portions representing bulk condensed fcc and bcc …

Temporal Coherent Control Of Resonant Two-Photon Double Ionization Of The Hydrogen Molecule Via Doubly Excited States, Jean Marcel Ngoko Djiokap, Anthony F. Starace

Anthony F. Starace Publications

We use time-delayed, counter-rotating, circularly polarized few-cycle attosecond nonoverlapping pulses to study the temporal coherent control of the resonant process of two-photon double ionization (TPDI) of hydrogen molecule via doubly excited states for pulse propagation direction along ˆk either parallel or perpendicular to the molecular axis ˆR. For ˆk ‖ ˆR and a pulse carrier frequency of 36 eV resonantly populating the Q₂ 1∏ ⁺ _u (1) doubly excited state as well as other 1∏ ⁺ _u doubly excited states, we find that the indirect ionization pathway through these doubly excited states changes the character of the kinematical vortex-shaped …

Magnetism In Curved Geometries, Robert Streubel, Evgeny Y. Tsymbal, Peter Fischer

Robert Streubel Papers

Curvature impacts physical properties across multiple length scales, ranging from the macroscopic scale, where the shape and size vary drastically with the curvature, to the nanoscale at interfaces and inhomogeneities in materials with structural, chemical, electronic, and magnetic short-range order. In quantum materials, where correlations, entanglement, and topology dominate, the curvature opens the path to novel characteristics and phenomena that have recently emerged and could have a dramatic impact on future fundamental and applied studies of materials. Particularly, magnetic systems hosting non-collinear and topological states and 3D magnetic nanostructures strongly benefit from treating curvature as a new design parameter to …

Signal-Background Analysis For New Physics At Particle Colliders And The Criteria For Its Discovery, Prudhvi Nikhil Bhattiprolu

Graduate Research Theses & Dissertations

Although the Standard Model (SM) is now complete with the spectacular discovery of the Higgs boson at the Large Hadron Collider (LHC), there are many unsolved puzzles such as the electroweak hierarchy problem, dark matter, neutrino masses, etc., that need to be addressed. Theories proposed to solve these issues often involve new and exotic particles at the TeV scale and beyond. It is therefore of great importance to devise novel strategies to extract new physics signals with small rates lurking in huge backgrounds. My research detailed here is broadly along those lines.

Vectorlike leptons (VLL) are an intriguing possibility for …

Combining Cryo-Em Density Map And Residue Contact For Protein Secondary Structure Topologies, Maytha Alshammari, Jing He

Computer Science Faculty Publications

Although atomic structures have been determined directly from cryo-EM density maps with high resolutions, current structure determination methods for medium resolution (5 to 10 Å) cryo-EM maps are limited by the availability of structure templates. Secondary structure traces are lines detected from a cryo-EM density map for α-helices and β-strands of a protein. A topology of secondary structures defines the mapping between a set of sequence segments and a set of traces of secondary structures in three-dimensional space. In order to enhance accuracy in ranking secondary structure topologies, we explored a method that combines three sources of information: a set …

Complete Experiments On Multi-Photon Ionizations Of Ultra-Cold And Polarized Atoms, Bishnu Prasad Acharya

Doctoral Dissertations

“Fundamental atomic processes such as collision-induced ionization are of relevance in many scientific fields. Describing these reactions can still pose a substantial challenge due to the well-known “few-body problem”, which entails that there is no analytical solution of the equations of motion for systems of more the 2 mutually interacting particle. Novel experimental tools and advancements in theorical methods enable to obtain detailed information on atomic dynamics providing insight into both, the phase as well as the amplitude of the quantum-mechanical wave functions of the particles. In this project, we developed experimental techniques studying multi-photon ionization of lithium in femto-second …

Equations Of State For Warm Dense Carbon From Quantum Espresso, Derek J. Schauss

Theses and Dissertations

Warm dense plasma is the matter that exists, roughly, in the range of 10,000 to 10,000,000 Kelvin and has solid-like densities, typically between 0.1 and 10 grams per centimeter. Warm dense fluids like hydrogen, helium, and carbon are believed to make up the interiors of many planets, white dwarfs, and other stars in our universe. The existence of warm dense matter (WDM) on Earth, however, is very rare, as it can only be created with high-energy sources like a nuclear explosion. In such an event, theoretical and computational models that accurately predict the response of certain materials are thus very …