Atomic, Molecular and Optical Physics Commons^™

Gas-Phase Electron Diffraction From Laser-Aligned Molecules, Jie Yang, Martin Centurion

Martin Centurion Publications

Electron diffraction is a valuable tool to capture structural information from molecules in the gas phase. However, the information contained in the diffraction patterns is limited due to the random orientation of the molecules. Additional structural information can be retrieved if the molecules are aligned. Molecules can be impulsively aligned with femtosecond laser pulses, producing a transient alignment. The alignment persists only for a time on the order of a picosecond, so a pulsed electron gun is needed to record the diffraction patterns. In this manuscript, we describe the alignment process and show the changes in the diffraction pattern as …

Dynamics Of Optically-Generated Carriers In Si (100) And Si (111) Substrate-Grown Gaas/Algaas Core-Shell Nanowires, Ramon M. Delos Santos, Jasher John Ibañes, Maria Herminia Balgos, Rafael Jaculbia, Jessica Pauline Afalla, Michelle Bailon-Somintac, Elmer Estacio, Arnel Salvador, Armando Somintac, Christopher Que, Satoshi Tsuzuki, Kohji Yamamoto, Masahiko Tani

Physics Faculty Publications

GaAs/Al0.1Ga0.9As core-shell nanowires (CSNWs), with average lateral size of 125 nm, were grown on gold nanoparticle-activated Si (100) and Si (111) substrates via molecular beam epitaxy. Room temperature-photoluminescence (RT-PL) from the samples showed bulk-like GaAs and Al0.1Ga0.9As bandgap emission peaks at 1.43 and 1.56 eV, respectively. Higher PL emission intensity of the sample on Si (111) compared to that on Si (100) is attributed to uniform Al0.1Ga0.9As shell passivation of surface states on Si (111)-grown CSNWs. Carrier dynamics in two different temporal regimes were studied. In the sub-nanosecond time scale (300–500 ps), time-resolved radiative recombination efficiency of carriers was examined. …

Simulations Of The Angular Dependence Of The Dipole-Dipole Interaction, Jacob T. Paul, Matan Peleg

Physics and Astronomy Summer Fellows

In our project we ran computations on a supercomputer to simulate experiments performed on highly excited atoms at μK temperatures. At μK temperatures the atoms are moving slowly so there are essentially no collisions of the atoms on the time scales at which we perform our experiments. In the absence of collisions the atoms exchange energy through long range dipole-dipole interactions. This exchange depends on the distances between and relative orientation of the atoms. The angular dependence between two atoms has recently been studied experimentally¹ . We simulate experimentally accessible spatial arrangements to see if the effect of the …

Simulations Of The Angular Dependence Of The Dipole-Dipole Interaction, Matan Peleg, Jacob T. Paul

Physics and Astronomy Summer Fellows

We conducted simulations of Rydberg atoms in a magneto-optical trap using the supercomputer available on campus and the COMET supercomputer provided by the NSF. Our research focused on the angular dependence of the long range interaction between Rydberg atoms. We simulated randomly distributed atoms alligned with a magnetic and electric field. We compared the simulated interaction rates for different electric field directions.

Toward Quantum Analog Computing: Simulating Designer Atomic Systems, Veronica L. Sanford, Jacob L. Bigelow

Physics and Astronomy Summer Fellows

We use a magneto-optical trap to cool rubidium atoms to temperatures in the _µK range. On the _µs timescales of our experiment, the atoms are moving slowly enough that they appear stationary. We then excite them to a Rydberg state, where the outer electron is loosely bound. In these high energy states, the atoms can exchange energy with each other. Since the energy exchange depends on the separation and the relative orientation of the atoms, we can potentially control their interactions by controlling the spatial arrangements of the atoms. We model this system using simulations on a supercomputer …

Toward Analog Quantum Computing: Simulating Designer Atomic Systems, Jacob L. Bigelow, Veronica L. Sanford

Physics and Astronomy Summer Fellows

We use a magneto-optical trap to cool rubidium atoms to temperatures in the _µK range. On the _µs timescales of our experiment, the atoms are moving slowly enough that they appear stationary. We then excite them to a Rydberg state, where the outer electron is loosely bound. In these high energy states, the atoms can exchange energy with each other. Since the energy exchange depends on the separation and the relative orientation of the atoms, we can potentially control their interactions by controlling the spatial arrangements of the atoms. We model this system using simulations on a supercomputer …

High Precision Optical Cavity Length And Width Measurements Using Double Modulation, A. Staley, D. Hoak, A. Effler, K. Izumi, S. Dwyer, K. Kawabe, E. J. King, Malik Rakhmanov, R. L. Savage, D. Sigg

Physics & Astronomy Faculty Publications

We use doubly phase modulated light to measure both the length and the linewidth of an optical resonator with high precision. The first modulation is at RF frequencies and is set near a multiple of the free spectral range, whereas the second modulation is at audio frequencies to eliminate offset errors at DC. The light in transmission or in reflection of the optical resonator is demodulated while sweeping the RF frequency over the optical resonance. We derive expressions for the demodulated power in transmission, and show that the zero crossings of the demodulated signal in transmission serve as a precise …

Retrieving Spin Textures On Curved Magnetic Thin Films With Full-Field Soft X-Ray Microscopies, Robert Streubel, Florian Kronast, Peter Fischer, Dula Parkinson, Oliver G. Schmidt, Denys Makarov

Robert Streubel Papers

X-ray tomography is a well-established technique to characterize 3D structures in material sciences and biology; its magnetic analogue - magnetic X-ray tomography - is yet to be developed. Here we demonstrate the visualization and reconstruction of magnetic domain structures in a 3D curved magnetic thin films with tubular shape by means of full-field soft X-ray microscopies. The 3D arrangement of the magnetization is retrieved from a set of 2D projections by analysing the evolution of the magnetic contrast with varying projection angle. Using reconstruction algorithms to analyse the angular evolution of 2D projections provides quantitative information about domain patterns and …

Plotting The Van Der Waals Fluid In Pseudo-3d And The Maxwell Construction, Carl W. David

Chemistry Education Materials

The van der Waals (from his thesis of 1873) equation is a cubic in the molar volume. Plotting the equation in pseudo 3 dimensions is quite simple to do, but including tie lines is quite difficult. Employing the solutions to the cubic van der Waals equation, the tie lines are readily available and can be easily incorporated into the aforementioned 3D plots.

Photodetachment Of A Model Molecular System By An Elliptically Polarized Field, M. V. Frolov, N. L. Manakov, S. S. Marmo, Anthony F. Starace

Anthony F. Starace Publications

The differential cross section for one-photon molecular detachment by an elliptically polarized field is analyzed for a one-electron molecular model comprised of an electron in the field of two (generally nonequivalent) attractive zero-range potentials (ZRPs) separated by the distance R. A phenomenological parametrization of the photodetachment cross section for a fixed-in-space molecular system in terms of two scalar dynamical parameters is presented and circular dichroism effects are discussed. Analytic results for the dynamical molecular parameters within the ZRP molecular model are used to analyze interference phenomena (including two-center interference) and dichroic effects in the detached electron angular distributions and …

Coupling Nuclear Induced Phonon Propagation With Conversion Electron Mössbauer Spectroscopy, Michael J. Parker

Theses and Dissertations

Mössbauer spectroscopy is a very sensitive measurement technique (10^-8 eV) which prompted motivation for the experiment described in this thesis. Namely, can a sensitive detection system be developed to detect nuclear recoils on the order of 10 to 100 of eVs? The hypothesis that this thesis tests is: Nuclear induced phonon bursts caused by Rutherford scattered alphas, decayed from ²⁴¹Am, in a type-310 stainless steel material can couple with 7.3 keV conversion electron Mössbauer events at the other end of the material which will have a statistically significant effect on a Mössbauer spectrum. The phonon bursts produced by …

Comparison Of Absorption, Fluorescence, And Polarization Spectroscopy Of Atomic Rubidium, Seth T. Ashman, Cayla Stifler, Joaquin Romero

Engineering & Physics Faculty Publications

An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and …

Imaging The Dipole-Dipole Energy Exchange Between Ultracold Rubidium Rydberg Atoms, Donald P. Fahey, Thomas J. Carroll, Michael W. Noel

Physics and Astronomy Faculty Publications

The long-range, anisotropic nature of the interaction among atoms in an ultracold dipolar gas leads to a rich array of possibilities for studying many-body physics. In this work, an ultracold gas of highly excited atoms is used to study energy transport due to the long-range dipole-dipole interaction. A technique is developed to measure both the internal energy states of the interacting Rydberg atoms and their positions in space. This technique is demonstrated by observing energy exchange between two spatially separated groups of Rydberg atoms excited to two different internal states. Simulations confirm the general features of the energy transport in …

Electron Transmission Through Micrometer Sized Funnelshaped Tapered Glass Capillaries And Electron Micro-Beam Production, Samanthi Jayamini Wickramarachchi

Dissertations

The prime motivation of this work is to understand the fundamental transmission process of an electron beam through a funnel-shaped capillary taking into account its shape together with the energy, angular and time dependence of the transmitted electrons produce a microsized electron beam. The utilized capillaries had inlet/outlet diameters of 800/16 μm, 800/100 μm and lengths of 35 mm. Considerable transmission of 800 and 1000 eV electrons for tilt angles up to 1.5^o and only small transmission for 500 eV electrons was observed for the capillary with the smaller outlet diameter of 16 μm. Incident electrons with energies of …

Modelling Transient Terahertz Magneto-Spectroscopy Measurements Of P-Type Cvd Graphene Leading To A Negative Photoconductivity., Rhyan Foo Kune

Macalester Journal of Physics and Astronomy

Ultrafast Terahertz (THz) Magneto-Spectroscopy (UTMS) measurements were performed on p-type CVD graphene sample to investigate the intrinsic carrier dynamics of the material. We investigated static and time-resolved THz transmission measurements, in which the sample was photo-excited by a near infrared (NIR) pump pulse, in order to study its behavior in a magnetic field. In these measurements the free carriers were probed to independently measure the carrier density and scattering rate in this film. We observed, in our graphene sample, an increase in transmission related to a negative photoconductivity (decrease in conductivity after photoexcitation) consistent with previous research. This decrease is …

Modeling The Optical Response To A Near-Field Probe Tip From A Generalized Multilayer Thin Film, A.J. Lawrence

Dissertations and Theses

The contrast mechanism in Kerr imaging is the apparent angle through which the plane of polarization is rotated upon reflection from a magnetic surface. This can be calculated for a well characterized surface given the polarization state of the incident light. As in traditional optical microscopy, the spatial resolution is limited by diffraction to roughly half the wavelength of the illumination light.

The diffraction limit can be circumvented through the use of near-field scanning optical microscopy, in which the illumination source is an evanescent field at the tip of a tapered optical fiber. A novel probe design for near-field optical …

A Slow Neutron Polarimeter For The Measurement Of Parity-Odd Neutron Rotary Power, W. M. Snow, E. Anderson, L. Barron-Palos, C. D. Bass, T. D. Bass, Bret E. Crawford, C. Crawford, J. M. Dawkins, D. Esposito, J. Fry, H. Gardiner, K. Gan, C. Haddock, B. R. Heckel, A. T. Holley, J. C. Horton, C. Huffer, J. Lieffers, D. Luo, M. Maldonado-Velazquez, D. M. Markoff, A. M. Micherdzinska, H. P. Mumm, J. S. Nico, M. Sarsour, S. Santra, E. I. Sharapov, H. E. Swanson, S. B. Walbridge, V. Zhumabekova

Physics and Astronomy Faculty Publications

We present the design, description, calibration procedure, and an analysis of systematic effects for an apparatus designed to measure the rotation of the plane of polarization of a transversely polarized slow neutron beam as it passes through unpolarized matter. This device is the neutronoptical equivalent of a crossed polarizer/analyzer pair familiar from light optics. This apparatus has been used to search for parity violation in the interaction of polarized slow neutrons in matter. Given the brightness of existing slow neutron sources, this apparatus is capable ofmeasuring a neutron rotary power of dϕ/dz = 1 × 10⁻⁷ rad/m.

Interstitial Silicon Ions In Rutile Tio2 Crystals, Eric M. Golden, Nancy C. Giles, Shan Yang, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) is used to identify a new and unique photoactive silicon-related point defect in single crystals of rutile TiO₂. The importance of this defect lies in its assignment to interstitial silicon ions and the unexpected establishment of silicon impurities as a major hole trap in TiO₂. Principal g values of this new S=1/2 center are 1.9159, 1.9377, and 1.9668 with principal axes along the [¯110],[001], and [110] directions, respectively. Hyperfine structure in the EPR spectrum shows the unpaired spin interacting equally with two Ti nuclei and unequally with two Si nuclei. These silicon …

Measuring The Hyperfine Splittings Of Lowest Energy Atomic Transitions In Rubidium, Benjamin D. Graber

Undergraduate Honors Thesis Projects

The goal of this experiment was to measure the hyperfine energy splittings of the ground to first excited state transitions in rubidium using saturated absorption spectroscopy. Using this technique, we measured these transition energy spectra by taking the difference of two photodiode outputs due to multiple beams of a single laser scanned over a range of frequencies and shone through a cell of Rb vapor. When the laser frequency was resonant with an atomic transition, photons of those frequencies were absorbed, leaving a dip in intensity of the beam measured at the photodiode. One of the two laser beams had …

Experimental Constraints On Exotic Spin-Dependent Interactions Using Specialized Materials, Rakshya Khatiwada

Open Access Dissertations

Various theories predict the possible existence of symmetry violating forces with mesoscopic range interactions from mm-m [1]. These forces can arise from the coupling of a spin 0 boson to spin 1/2 fermions through scalar (gs) and pseudoscalar (gp) couplings. We discuss two experiments that can investigate these interactions using nucleon rich, impressively low magnetic susceptibility (5-100 times lower than pure water) test masses and electron-spin rich, polarized test masses (spin density: 10^20 h/cm3 ). The first experiment looks for a P-odd, T-odd interaction potential proportional to (S.r) where S is the spin of one particle and r is the …