Atomic, Molecular and Optical Physics Commons^™

Theoretical Calculations For Electron Impact Ionization Of Atoms And Molecules, Sadek Mohamed Fituri Amami

Doctoral Dissertations

"In the last twenty years, significant progress has been made for the theoretical treatment of electron impact ionization (e,2e) of atoms and molecules and, for some cases, very nice agreement between experiment and theory has been achieved. In particular, excellent agreement between theory and experiment and theory has been achieved for ionization of hydrogen and helium. However, agreement between experiment and theory is not nearly as good for ionization of larger atoms and molecules. In the first part of this dissertation, different theoretical approaches will be employed to study the triply differential cross section (TDCS) for low and intermediate energy …

Coincidence Charged-Current Neutrino-Induced Deuteron Disintegration For 2H216O, J. W. Van Orden, T. W. Donnelly, O. Moreno

Physics Faculty Publications

Semi-inclusive charge-changing neutrino reactions on targets of heavy water are investigated with the goal of determining the relative contributions to the total cross section of deuterium and oxygen in kinematics chosen to emphasize the former. The study is undertaken for conditions where the typical neutrino beam energies are in the few GeV region, and hence relativistic modeling is essential. For this, the previous relativistic approach for the deuteron is employed, together with a spectral function approach for the case of oxygen. Upon optimizing the kinematics of the final-state particles assumed to be detected (typically a muon and a proton) it …

Transverse Parton Momenta In Single Inclusive Hadron Production In E+E- Annihilation Process., M. Boglione, J. O. Gonzalez-Hernandez, R. Taghavi

Physics Faculty Publications

We study the transverse momentum distributions of single inclusive hadron production in e⁺e⁻ annihilation processes. Although the only available experimental data are scarce and quite old, we find that the fundamental features of transverse momentum dependent (TMD) evolution, historically addressed in Drell–Yan processes and, more recently, in Semi-inclusive deep inelastic scattering processes, are visible in e⁺e⁻ annihilations as well. Interesting effects related to its non-perturbative regime can be observed.

We test two different parameterizations for the p⊥ dependence of the cross section: the usual Gaussian distribution and a power-law model. We find the latter …

Ruo2 Ph Sensor With Super-Glue-Inspired Reference Electrode, Wade Lonsdale, Magdalena Wajrak, Kamal Alameh

Research outputs 2014 to 2021

A pH-sensitive RuO2 electrode coated in a commercial cyanoacrylate adhesive typically exhibits very low pH sensitivity, and could be paired with a RuO2 working electrode as a differential type pH sensor. However, such sensors display poor performance in real sample matrices. A pH sensor employing a RuO2 pH-sensitive working electrode and a SiO2-PVB junction-modified RuO2 reference electrode is developed as an alternative high-performance solution. This sensor exhibits a performance similar to that of a commercial glass pH sensor in some common sample matrices, particularly, an excellent pH sensitivity of 55.7 mV/pH, a hysteresis as low as 2.7 mV, and a …

Schrödinger Theory Of Electrons In Electromagnetic Fields: New Perspectives, Viraht Sahni, Xiao-Yin Pan

Publications and Research

The Schrödinger theory of electrons in an external electromagnetic field is described from the new perspective of the individual electron. The perspective is arrived at via the time-dependent "Quantal Newtonian" law (or differential virial theorem). (The time-independent law, a special case, provides a similar description of stationary-state theory). These laws are in terms of "classical" fields whose sources are quantal expectations of Hermitian operators taken with respect to the wave function. The laws reveal the following physics: (a) in addition to the external field, each electron experiences an internal field whose components are representative of a specific property of the …

Real-Space Mean-Field Theory Of A Spin-1 Bose Gas In Synthetic Dimensions, Hilary M. Hurst, Justin H. Wilson, J. H. Pixley, I. B. Spielman, Stefan S. Natu

Faculty Research, Scholarly, and Creative Activity

The internal degrees of freedom provided by ultracold atoms give a route for realizing higher dimensional physics in systems with limited spatial dimensions. Non-spatial degrees of freedom in these systems are dubbed "synthetic dimensions". This connection is useful from an experimental standpoint but complicated by the fact that interactions alter the condensate ground state. Here we use the Gross-Pitaevskii equation to study ground state properties of a spin-1 Bose gas under the combined influence of an optical lattice, spin-orbit coupling, and interactions at the mean field level. The associated phases depend on the sign of the spin-dependent interaction parameter and …

Linear Feedback Stabilization For A Continuously Monitored Qubit, Taylor Lee Patti, A. Chantasri, Justin Dressel, A. N. Jordan

Student Scholar Symposium Abstracts and Posters

In quantum mechanics, standard or strong measurement approaches generally result in the collapse of an ensemble of wavefunctions into a stochastic mixture of eigenstates. On the other hand, continuous or weak measurements have the propensity to dynamically control the evolution of quantum states over time, guiding the trajectory of the state into non-trivial superpositions and maintaining state purity. This kind of measurement-induced state steering is of great theoretical and experimental interest for the harnessing of quantum bits or "qubits", which are the fundamental unit of the emerging quantum computer. We explore continuous measurement-based quantum state stabilization through linear feedback control …

Cavity Ringdown Spectroscopy In Nitrogen/Oxygen Mixtures In The Presence Of Alpha Radiation, Sidney John Gautrau

Master's Theses

This research was part of an effort to experimentally validate computational models under development for radiation-induced atmospheric effects. Cavity Ringdown Spectroscopy (CRDS) was used to measure the concentration of chemical products generated as a result of radiation interactions in a controlled atmosphere. Experiments were conducted in a vacuum chamber interfaced with a gas introduction system that controlled the initial atmospheric composition. A quadrupole mass spectrometer and tunable dye laser were integrated to confirm initial atmospheric composition, and provide wavelength flexibility for detecting a variety of chemical products generated by radiation interactions. CRDS measurements were made for ozone production resulting from …

All-Optical Cooling Of Fermi Gases Via Pauli Inhibition Of Spontaneous Emission, Roberto Onofrio

Dartmouth Scholarship

A technique is proposed to cool Fermi gases to the regime of quantum degeneracy based on the expected inhibition of spontaneous emission due to the Pauli principle. The reduction of the linewidth for spontaneous emission originates a corresponding reduction of the Doppler temperature, which under specific conditions may give rise to a runaway process through which fermions are progressively cooled. The approach requires a combination of a magneto-optical trap as a cooling system and an optical dipole trap to enhance quantum degeneracy. This results in expected Fermi degeneracy factors T/TF comparable to the lowest values recently achieved, with potential for …

Properties Of The Schrödinger Theory Of Electrons In Electromagnetic Fields, Viraht Sahni, Xiao-Yin Pan

Publications and Research

The Schrödinger theory of electrons in an external electromagnetic field can be described from the perspective of the individual electron via the ‘Quantal Newtonian’ laws (or differential virial theorems). These laws are in terms of ‘classical’ fields whose sources are quantal expectations of Hermitian operators taken with respect to the wave function. The laws reveal the following physics: (a) In addition to the external field, each electron experiences an internal field whose components are representative of a specific property of the system such as the correlations due to the Pauli exclusion principle and Coulomb repulsion, the electron density, kinetic effects, …

Selective Growth Of Epitaxial Sr2Iro4 By Controlling Plume Dimensions In Pulsed Laser Deposition, Sung S. Ambrose Seo, J. Nichols, J. Hwang, Jsaminka Terzic, John H. Gruenewald, Maryam Souri, Justin K. Thompson, John G. Connell, Gang Cao

Physics and Astronomy Faculty Publications

We report that epitaxial Sr₂IrO₄ thin-films can be selectively grown using pulsed laser deposition (PLD). Due to the competition between the Ruddlesden-Popper phases of strontium iridates (Sr_n+1Ir_nO_3n+1), conventional PLD methods often result in mixed phases of Sr₂IrO₄ (n = 1), Sr₃Ir₂O₇ (n = 2), and SrIrO₃ (n = ∞). We have discovered that reduced PLD plume dimensions and slow deposition rates are the key for stabilizing pure Sr₂IrO₄ phase thin-films, identified by real-time in-situ monitoring of their optical spectra. …

Neutron Correlations In The Decay Of The First Excited State Of 11li, Jenna K. Smith, Thomas J. Baumann, Daniel Bazin, James Brown, Paul A. Deyoung, Nathan H. Frank, Michael D. Jones, Zack Kohley, Bryan A. Luther, B. S. Marks, Artemis Spyrou, Sharon L. Stephenson, Michael R. Thoennessen, Alexander S. Volya

Physics and Astronomy Faculty Publications

The decay of unbound excited ¹¹Li was measured after being populated by a two-proton removal from a ¹³B beam at 71 MeV/nucleon. Decay energy spectra and Jacobi plots were obtained from measurements of the momentum vectors of the ⁹Li fragment and neutrons. A resonance at an excitation energy of ∼1.2 MeV was observed. The kinematics of the decay are equally well fit by a simple dineutron-like model or a phase-space model that includes final state interactions. A sequential decay model can be excluded.

A Measuring Method For Abundance Of Uranium Components Based On Active Source Of Neutron, Li Li, Gen Hu, Keqi Liu

The 8th International Conference on Physical and Numerical Simulation of Materials Processing

No abstract provided.

Diffractive Imaging Of Coherent Nuclear Motion In Isolated Molecules, Jie Yang, Markus Guehr, Xiaozhe Shen, Renkai Li, Theodore Vecchione, Ryan Coffee, Jeff Corbett, Alan Fry, Nick Hartmann, Carsten Hast, Kareem Hegazy, Keith Jobe, Igor Makasyuk, Joseph Robinson, Matthew S. Robinson, Sharon Vetter, Stephen Weathersby, Charles Yoneda, Xijie Wang, Martin Centurion

Martin Centurion Publications

Observing the motion of the nuclear wave packets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational wave packet in isolated iodine molecules using ultrafast electron diffraction with relativistic electrons. The time-varying interatomic distance was measured with a precision 0.07 Å and temporal resolution of 230 fs full width at half maximum. The method is not only sensitive to the position but also the shape of the nuclear wave packet.

The Web Based Monitoring Project At The Cms Experiment, Juan Antonio Lopez-Perez, Kaori Maeshima, William Badgett, Ulf Behrens, Irakli Chakaberia, Youngkwon Jo, Sho Maruyama, James Patrick, Valdas Rapsevicius, Aron Soha, Mantas Stankevicius, Balys Sulmanas, Sachiko Toda, Zongru Wan

Physics Faculty Research

The Compact Muon Solenoid is a large a complex general purpose experiment at the CERN Large Hadron Collider (LHC), built and maintained by many collaborators from around the world. Efficient operation of the detector requires widespread and timely access to a broad range of monitoring and status information. To the end the Web Based Monitoring (WBM) system was developed to present data to users located anywhere from many underlying heterogeneous sources, from real time messaging systems to relational databases. This system provides the power to combine and correlate data in both graphical and tabular formats of interest to the experimenters, …

Feasibility Of The Use Of Neutron Activation Analysis Techniques In An Underwater Environment, Michael D. Chick

Masters Theses & Specialist Projects

Elements when bombarded with neutrons emit a gamma ray that is characteristic of the isotope that underwent a neutron induced nuclear reaction; this is known as neutron activation. The characteristic gamma energy of an isotope can then be detected and recorded. One can then analyze the gamma energies captured and determine the elemental makeup of the sample. This form of analysis can be used in an underwater environment making it potentially a valuable tool for agencies tasked with maritime security of ports and waterways, or clean-up operations. This thesis will focus on the feasibility of neutron interrogation using pulsed fast/thermal …

Investigation Of Multi-Photon Excitation In Argon With Applications In Hypersonic Flow Diagnostics, Jack L. Mills

Physics Theses & Dissertations

Non-intrusive flow diagnostics are essential for studying the physics of hypersonic flow wake regions. To advance the development of next generation hypersonic vehicles and to improve computational fluid dynamics techniques in the hypersonic regime, NASA needs a suitable non-intrusive diagnostic technique to measure velocity, density, and temperature. We will present our work on developing a seedless, non-intrusive diagnostic technique using excited state argon atoms, prepared via multi-photon excitation. In this dissertation, we report results on the first phase of this hypersonic wake measurement project. In particular, we have redesigned and characterized the performance of a high energy, nanosecond pulsed Ti:Sapphire …

Echocardiography Audit On Patients With Hereditary Haemochromatosis, Lorna Doran

Masters

Background: The European Association for the Study of the Liver (EASL) Guidelines for Hereditary Haemochromatosis (HH) refer specifically to symptomatic Homozygous C282Y patients and provide an algorithm for treating such patients who are predisposed to iron overloading. The British Society of Echocardiography does not make provisions for HH patients per se. Cardiac failure is a known complication of severe iron overload although it is atypical. Aim: To retrospectively investigate if an echocardiogram (echo) was warranted in the HH population at Louth County Hospital (LCH) Venesection Clinic based on the current guidelines. Methods: A cohort of 833 HH patients was reviewed …

Sn Vacancies In Photorefractive Sn2P2S6 Crystals: An Electron Paramagnetic Resonance Study Of An Optically Active Hole Trap, Eric M. Golden, Sergey A. Basun, D. R. Evans, A. A. Grabar, I. M. Stoika, Nancy C. Giles, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) is used to identify the singly ionized charge state of the Sn vacancy (V⁻_Sn) in single crystals of Sn₂P₂S₆ (often referred to as SPS). These vacancies, acting as a hole trap, are expected to be important participants in the photorefractive effect observed in undoped SPS crystals. In as-grown crystals, the Sn vacancies are doubly ionized (V²⁻_Sn) with no unpaired spins. They are then converted to a stable EPR-active state when an electron is removed (i.e., a hole is trapped) during an illumination below 100 K …

Control Of Spontanous Emission From Quantum Emitters Using Hyperbolic Metamaterial Substrates, Tal Galfsky

Dissertations, Theses, and Capstone Projects

Hyperbolic metamaterials (HMMs) are so named for possessing a hyperboloid-shaped dispersion which gives rise to a large photonic density of states. Quantum emitters placed inside or in the near-field of a HMM have been shown to exhibit strong enhancement of spontaneous emission due to the increase in available states. This thesis focuses on enhancing spontaneous emission of quantum emitters in optical frequencies by utilizing multilayered metal/dielectric composites that form these highly anisotropic metamaterials. In conjunction with the enhanced decay rate we experimentally demonstrate two methods for shaping and directing radiation trapped in the HMM into free space by employing a …