Atomic, Molecular and Optical Physics Commons^™

Controlling The Stereodynamics Of Cold Molecular Collisions, Balakrishnan Naduvalath, J. F. E. Croft, Meng Huang, Hua Guo

Chemistry and Biochemistry Faculty Research

We report numerically-exact quantum scattering calculations for low-energy collisions of quantum-state prepared HD with H2. Excellent agreement is obtained with recent measurements of Perreault et al. for the angular distribution of scattered HD at a collision energy of 1 K. By state-preparation of the HD molecules, control of the angular distribution of scattered HD was demonstrated. The stereo-dynamic control is achieved by the ability to choose a single or a coherent superposition of quantum states. We present a first-principles simulation of the experiment which enables us to attribute the main features of the observed angular distribution to a single L …

New Heusler Compounds In Ni-Mn-In And Ni-Mn-Sn Alloys, Xingzhong Li, W.-Y. Zhang, Shah R. Valloppilly, David J. Sellmyer

Nebraska Center for Materials and Nanoscience: Faculty Publications

Rapidly quenched ternary Ni-Mn-T (T = In, Sn) alloys exhibit features associated with magnetic skyrmions, so that XRD, TEM, EDS, SAED and HREM investigations were carried out for structural characterization on the two alloy systems. In this paper, we report a new type of Mn-rich Heusler compound with a cubic unit cell, a = 0.9150 nm in Ni-Mn-In and a = 0.9051 nm in Ni-Mn-Sn, which coexist with a Ni-rich full-Heusler compound with defects, a = 0.6094 nm in Ni-Mn-In and a = 0.6034 nm in Ni-Mn-Sn. A further analysis of the experimental results reveals a close structural relationship between …

Analytic Generalized Description Of A Perturbative Nonparaxial Elegant Laguerre-Gaussian Phasor For Ultrashort Pulses In The Time Domain, Andrew Vikartofsky, Ethan C. Jahns, Anthony F. Starace

Anthony F. Starace Publications

An analytic expression for a polychromatic phasor representing an arbitrarily short elegant Laguerre-Gauss (eLG) laser pulse of any spot size and LG mode is presented in the time domain as a nonrecursive, closed-form perturbative expansion valid to any order of perturbative correction. This phasor enables the calculation of the complex electromagnetic fields for such beams without requiring the evaluation of any Fourier integrals. It is thus straightforward to implement in analytical or numerical applications involving eLG pulses.

Measurement-Induced Dynamics And Stabilization Of Spinor-Condensate Domain Walls, Hilary M. Hurst, I. B. Spielman

Faculty Research, Scholarly, and Creative Activity

Weakly measuring many-body systems and allowing for feedback in real-time can simultaneously create and measure new phenomena in strongly correlated quantum systems. We study the dynamics of a continuously measured two-component Bose-Einstein condensate (BEC) potentially containing a domain wall, and focus on the trade-off between usable information obtained from measurement and quantum backaction. Each weakly measured system yields a measurement record from which we extract real-time dynamics of the domain wall. We show that quantum backaction due to measurement causes two primary effects: domain wall diffusion and overall heating. The system dynamics and signal-to-noise ratio depend on the choice of …

Topics In Three-Dimensional Imaging, Source Localization And Super-Resolution, Zhixian Yu

Physics & Astronomy ETDs

The realization that twisted light beams with helical phasefronts could carry orbital angular momentum (OAM) that is in excess of the photon's spin angular momentum (SAM) has spawned various important applications. One example is the design of novel imaging systems that achieve three-dimensional (3D) imaging in a single snapshot via the rotation of point spread function (PSF).

Based on a scalar-field analysis, a particular simple version of rotating PSF imagery, which was proposed by my advisor Dr. Prasad, furnishes a practical approach to perform 3D source localization using a spiral phase mask that generates a combination of Bessel vortex beams. …

Analytic Description Of High-Order Harmonic Generation In The Adiabatic Limit With Application To An Initial S State In An Intense Bicircular Laser Pulse, M. V. Frolov, N. L. Manakov, A. A. Minina, A. A. Silaev, N. V. Vvedenskii, M. Yu. Ivanov, Anthony F. Starace

Anthony F. Starace Publications

An analytic description of high-order harmonic generation (HHG) is proposed in the adiabatic (low-frequency) limit for an initial s state and a laser field having an arbitrary wave form. The approach is based on the two-state time-dependent effective range theory and is extended to the case of neutral atoms and positively charged ions by introducing ad hoc the Coulomb corrections for HHG. The resulting closed analytical form for the HHG amplitude is discussed in terms of real classical trajectories. The accuracy of the results of our analytic model is demonstrated by comparison with numerical solutions of the time-dependent Schrödinger equation …

Large-Scale Atomistic Simulations Of Complex And Functional Properties Of Ferroic Materials, Raymond Thomas Walter

Graduate Theses and Dissertations

Ferroelectric (FE) nanostructures have attracted considerable attention as our abilities improve to synthesize them and to predict their properties by theoretical means. Depolarizing field effects at interfaces of FE heterostructures are particularly notable for causing topological defects such as FE vortices and negative dielectric responses in superlattices. In this thesis, I employ two large-scale atomistic techniques, the first-principles-based effective Hamiltonian (HEff) method and the linear-scaling three-dimensional fragment (LS3DF) method. I use these methods to explore optical rotation in FE vortices, electro-optic effects in FE vortices and skyrmions, and voltage amplification via negative capacitance in ferroelectric-paraelectric superlattices. We employ HEff in …

Scope Of Self-Interacting Thermal Wimps In A Minimal U(1) D Extension And Its Future Prospects, Rahool Kumar Barman, Biplob Bhattacherjee, Arindam Chatterjee, Arghya Choudhury, Aritra Gupta

Journal Articles

In this work we have considered a minimal extension of Standard Model by a local U(1) gauge group in order to accommodate a stable (fermionic) Dark Matter (DM) candidate. We have focussed on parameter regions where DM possesses adequate self-interaction, owing to the presence of a light scalar mediator (the dark Higgs), alleviating some of the tensions in the small-scale structures. We have studied the scenario in the light of a variety of data, mostly from dark matter direct searches, collider searches and flavor physics experiments, with an attempt to constrain the interactions of the standard model (SM) particles with …

Free Electron Sources And Diffraction In Time, Eric R. Jones

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The quantum revolution of the last century advanced synergistically with technology, for example, with control of the temporal and spatial coherence, and the polarization state of light. Indeed, experimental confirmation of the quirks of quantum theory, as originally highlighted by Einstein, Podolsky, and Rosen, through Bohm, and then Bell, have been performed with photons, i.e., electromagnetic wave packets prepared in the same quantum states. Experimental tests of quantum mechanics with matter wave packets have been limited due to challenges in preparing all of the packets with similar quantum states. While great strides have been made for trapped atoms and Bose-Einstein …

A Theoretical Investigation Of Small Organic Molecules On Transition Metal Surfaces, Walter Malone

Electronic Theses and Dissertations

With the ever growing number of proposed desnity functional theory (DFT) functionals it becomes necessary to thoroughly screen any new method to determine its merit. Especially relevant methods include a proper description of the van der Waals (vdW) interaction, which can prove vital to a correct description of a myriad of systems of technological importance. The first part of this dissertation explores the utility of several vdW-inclusive DFT functionals including optB86b-vdW, optB88-vdW, optPBE-vdW, revPBE-vdW, rPW86-vdW2, and SCAN+rVV10 by applying them to model systems of small organic molecules, pyridine and thiophene, on transition metal surfaces. Overall, we find the optB88-vdW functional …

Chemistry And Dissipation At Mineral Surfaces In The Space Environment, William Tucker

Electronic Theses and Dissertations

The composition and morphology of mineral surfaces is known to play an important role in various phenomena relevant to planetary science. For example, the synthesis and processing of complex organics likely occurs at mineral surfaces strongly affected by the space environment. Furthermore, the dissipative and adhesive properties of dust grains may depend strongly on the chemical state of the surface including the presence of dangling bonds, adsorbates, and radicals. In this dissertation, experimental results are first presented which demonstrate that mineral grains subjected to high temperatures in a reducing environment lead to iron nanoparticles which are strongly catalytic for the …

The Population Densities Of Argon Metastable Levels, Nada Khogeer, Chelsy Gonzalez, Milka Nikolic

Physics and Astronomy

In this experiment, we used the optical emission spectroscopy (OES) method to obtain the main properties of low temperature Argon plasma. The experiment was sustained in powers and pressures that ranges from 30-100 W and 15-100 mTorr. We used numerical methods for the Argon kinetic model to calculate metastable levels and resonant states for the first excited states in low temperature Argon plasma. By finding the ratio of two spectral lines and finding another ratio from a different upper energy level that goes down to the same two lower energy levels, we can construct a system of two nonlinear equations. …

High Resolution Near-Infrared/Visible Intracavity Laser Spectroscopy Of Small Molecules, Jack Harms

Dissertations

Intracavity laser spectroscopy has been used to study the electronic structure of several small molecules. The molecules studied as part of this dissertation include germanium hydride (GeH), copper oxide (CuO), nickel chloride (NiCl), platinum fluoride (PtF), platinum chloride (PtCl), and copper hydroxide (CuOH). This work encompasses five peer-reviewed publications and two submitted manuscripts.

Origin Of Enhanced Anisotropy In Fept-C Granular Films Revealed By Xmcd, Robert Streubel, Alpha T. N'Diaye, Kumar Srinivasan, Antony Ajan, Peter Fischer

Robert Streubel Papers

We study the effect of carbon segregants on the spin and orbital moments of L10 FePt granular media using x-ray magnetic circular dichroism (XMCD) spectroscopy and report an effective decoupling of the structural film properties from the magnetic parameters of the grains. The carbon concentration reduces the grain size from (200 ± 160) nm2 down to (50 ± 20) nm2 for 40 mol. %C and improves sphericity and the order of grains, while preserving the crystalline order, spin and orbital moments, and perpendicular magnetocrystalline anisotropy. We identify the primary cause of enhanced saturation and coercive fields as the reduced demagnetization …

Roadmap On Superoscillations, Michael Berry, Nicolay Zheludev, Yakir Aharonov, Fabrizio Colombo, Irene Sabadini, Daniele C. Struppa, Jeff Tollaksen, Edward T. F. Rogers, Fei Qin, Minghui Hong, Xiangang Luo, Roei Remez, Ady Arie, Jörg B. Götte, Mark R. Dennis, Alex M. H. Wong, George V. Eleftheriades, Yaniv Eliezer, Alon Bahabad, Gang Chen, Zhongquan Wen, Gaofeng Liang, Chenglong Hao, C-W Qiu, Achim Kempf, Eytan Katzav, Moshe Schwartz

Mathematics, Physics, and Computer Science Faculty Articles and Research

Superoscillations are band-limited functions with the counterintuitive property that they can vary arbitrarily faster than their fastest Fourier component, over arbitrarily long intervals. Modern studies originated in quantum theory, but there were anticipations in radar and optics. The mathematical understanding—still being explored—recognises that functions are extremely small where they superoscillate; this has implications for information theory. Applications to optical vortices, sub-wavelength microscopy and related areas of nanoscience are now moving from the theoretical and the demonstrative to the practical. This Roadmap surveys all these areas, providing background, current research, and anticipating future developments.

Single Metalens For Generating Polarization And Phase Singularities Leading To A Reverse Flow Of Energy, Victor V. Kotlyar, Anton G. Nalimov, Sergey S. Stafeev, Liam O'Faolain

Cappa Publications

Using Jones matrices and vectors, we show that a metasurface-based optical element composed of a set of subwavelength diffraction gratings, whose anisotropic transmittance is described by a matrix of polarization rotation by angle m, where is the polar angle, generate an mth order azimuthally or radially polarized beam, when illuminated by linearly polarized light, or an optical vortex with topological charge m, when illuminated by circularly polarized light. Such a converter performs a spin–orbit transformation, acting similarly to a liquid-crystal half-wave plate. Using the FDTD-aided numerical simulation, we show that uniform linearly or circularly polarized light passing through the …

Subwavelength Grating-Based Spiral Metalens For Tight Focusing Of Laser Light, Victor V. Kotlyar, Sergey S. Stafeev, Anton G. Nalimov, Liam O'Faolain

Cappa Publications

In this paper, we investigate a 16-sector spiral metalens fabricated on a thin film (130 nm) of amorphous silicon, consisting of a set of subwavelength binary diffractive gratings and with a numerical aperture that is close to unity. The metalens converts linearly polarized incident light into an azimuthally polarized optical vortex and focuses it at a distance approximately equal to the wavelength of the incident light, k ¼ 633 nm. Using a scanning near-field optical microscope, it is shown experimentally that the metalens forms an elliptical focal spot with diameters smaller than the diffraction limit: FWHMx ¼ 0.32k (60.03k) and …

Testing Quantum Coherence In Stochastic Electrodynamics With Squeezed Schrödinger Cat States, Wayne Cheng-Wei Huang, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

The interference pattern in electron double-slit diffraction is a hallmark of quantum mechanics. A long-standing question for stochastic electrodynamics (SED) is whether or not it is capable of reproducing such effects, as interference is a manifestation of quantum coherence. In this study, we used excited harmonic oscillators to directly test this quantum feature in SED. We used two counter-propagating dichromatic laser pulses to promote a ground-state harmonic oscillator to a squeezed Schrödinger cat state. Upon recombination of the two well-separated wavepackets, an interference pattern emerges in the quantum probability distribution but is absent in the SED probability distribution. We thus …

Novel Data Analysis Methods In Multi-Channel And Multi-State Binding Experiments, Joseph Tibbs, Elizabeth Boehm, Wayne Bowie, Todd Washington, Maria Spies, Ali Tabei

Research in the Capitol

Single-Molecule studies use advanced microscopy techniques to view biomolecules, such as proteins and DNA, individually. On a slide, fluorescently-labeled molecules are immobilized and imaged using lasers, and the patterns of fluorescence can give important information about the interactions of multiple molecules. To extract this information, advanced, customizable data analysis tools must be created. The first goal is to create a method to robustly normalize (correct for brightness) single-channel fluorescence data. The second goal is to extend pattern recognition of binding order to multi-state and multi-channel binding patterns. The KERA 3.0 suite links creative pattern-recognition and normalization techniques with the abilities …

Investigating The Talbot Effect In Arrays Of Optical Dipole Traps For Neutral Atom Quantum Computing, Sergio Aguayo

Physics

Quantum computers are devices that are able to perform calculations not achievable for classical computers. Although there are many methods for creating a quantum computer, using neutral atoms offers the advantage of being stable when compared to other methods. The purpose of this investigation is to explore possible optical dipole trap configurations that would be useful for implementing a quantum computer with neutral atoms. Specifically, we computationally investigate arrays of pinholes, the diffraction pattern generated by them, and the onset of the Talbot effect in these traps. We manipulate the radius of the pinholes, the number of pinholes in the …