Atomic, Molecular and Optical Physics Commons^™

Quantitative, Photocurrent Multidimensional Coherent Spectroscopy, Adam Halaoui

Electronic Theses and Dissertations

Multidimensional coherent spectroscopy (MDCS) is a quickly growing field that has a lot of advantages over more conventional forms of spectroscopy. These advantages all come from the fact that MDCS allows us to get time resolved correlated emission and absorption spectra using very precisely chosen interactions between the density matrix and the excitation laser. MDCS spectra gives the researcher a lot of information that can be extracted purely through qualitative analysis. This is possible because state couplings are entirely separated on the spectra, and once we know how to read the data, we can see how carriers transport in the …

Equilibrium And Quench-Dynamical Studies Of Ultracold Fermions In Ring-Shaped Optical Traps, Daniel Gordon Allman

Dartmouth College Ph.D Dissertations

The unique capability to precisely tune the few and many-body configurations of
ultracold Fermi gases provides a multi-dimensional platform for studying novel, ex-
otic aspects of quantum systems. These aspects include superfluid/superconducting
phenomena supported by potentially exotic pairing mechanisms, non-equilibrium and
critical dynamics, and proposed quantum sensing or computing applications based on
atomtronics.
Ring geometries provide natural arenas for probing transport properties of super-
fluids. Metastable states of quantized superfluid flow —persistent currents— exhibit
remarkable properties, and the manner in which they form is an incredibly rich sub-
ject. Studies of quenched superfluids demonstrate that persistent currents can form
from …

Time-Symmetry And Topology Of The Aharonov-Bohm Effect, Yakir Aharonov, Ismael L. Paiva, Zohar Schwartzman-Nowik, Avshalom C. Elitzur, Eliahu Cohen

Mathematics, Physics, and Computer Science Faculty Articles and Research

The Aharonov–Bohm (AB) effect has been highly influential in fundamental and applied physics. Its topological nature commonly implies that an electron encircling a magnetic flux source in a field-free region must close the loop in order to generate an observable effect. In this paper, we study a variant of the AB effect that apparently challenges this concept. The significance of weak values and nonlocal equations of motion is discussed as part of the analysis, shedding light on and connecting all these fundamental concepts.

Non-Hermitian Gauged Laser Arrays With Localized Excitations: Anomalous Threshold And Generalized Principle Of Selective Pumping, Li Ge, Zihe Gao, Liang Feng

Publications and Research

We investigate non-Hermitian skin modes in laser arrays with spatially localized excitation. Intriguingly, we observe an unusual threshold behavior when selectively pumping either the head or the tail of these modes: both cases exhibit the same lasing threshold and hence defy the conventional principle of selective pumping, which aims to maximize the overlap between the pump profile and the target lasing mode. To shed light on this enigma, we reveal a previously overlooked phenomenon, i.e., energy exchange at non-Hermitian coupling junctions with the photonic environment, which does not occur with uniform gain or loss. Utilizing a transfer matrix approach, we …

Ferroelectric Hafnia Surface In Action, Xia Hong

Nebraska Center for Materials and Nanoscience: Faculty Publications

Piezoresponse microscopy and spectroscopy reveal the inextricable role of surface electrochemistry in stabilizing and controlling ferroelectricity in doped hafnia.

Doped hafnia (HfO₂), a relatively new member of the ferroelectric family, has challenged in many ways our conventional perception of ferroelectric oxides. It possesses extremely localized electric dipoles that are independently switchable,¹ making it immune to finite size effects — the loss of long-range dipole order in ferroic materials due to size scaling. While polycrystalline grains and microstructures can yield lower polarization and poorer cycling behavior in canonical ferroelectrics such as Pb(Zr,Ti)O₃ and BaTiO₃, in …

Improving And Evaluating Performance Of The Proton Prediction System Through An Expanded Solar Proton Event Catalog, Samantha R. Howard

Theses and Dissertations

Solar energetic particles (SEPs) are especially high energy protons (≥ 5 or 10MeV kinetic energies) originating from the Sun that are known to have significant effects on space-based military operations. The Air Force’s current forecast model, the Proton Prediction System (PPS), forecasts less than half of SEP events that are observed, motivating the need for an update to the operational model. To develop the updated PPS model, PPS2.0, an expanded SEP catalog was produced, which includes 103 previously unidentified events and specification of the proton flux response above background levels or prior events. Event detection and source association were initially …

Non-Contact Optical Spectroscopy For Tumor-Sensitive Diffuse Reflectance And Fluorescence Measurements On Murine Subcutaneous Tissue Models: Monte Carlo Modeling And Experimental Validations, Zahid Hasan, Pranto Soumik Saha, Madison O. Korfhage, Caigang Zhu

Markey Cancer Center Faculty Publications

Fiber-optic probes are commonly used in biomedical optical spectroscopy platforms for light delivery and collection. At the same time, it was reported that the inconsistent probe- sample contact could induce significant distortions in measured optical signals, which consequently cause large analysis errors. To address this challenge, non-contact optical spectroscopy has been explored for tissue characterizations. However, existing non-contact optical spectroscopy platforms primarily focused on diffuse reflectance measurements and may still use a fiber probe in which the probe was imaged onto the tissue surface using a lens, which serves as a non-contact probe for the measurements. Here, we report a …

Brdf Measurements And Physical Optics Modeling Applied To Anisotropic Satellite Solar Cells, Madilynn E. Compean

Theses and Dissertations

Light curve analysis is often used to discern information about satellites in geosynchronous orbits, and since solar panels comprise relatively large surface areas, their reflected energy can contribute greatly to observed light curves. Data was collected using a space qualified solar cell interrogated by a green HeNe laser. The data validated certain aspects from previous work, but also identified multi-slit behavior, showed that the specular term was a second diffraction pattern, and diagnosed the out-of-plane diffraction curvature as the conical diffraction phenomenon. Two physical-optics-based models were developed to incorporate these new features and better predict solar cell BRDF solely from …

Theoretical Framework Of Exchange Coupled Tripartite Spin Systems With Magnetic Anisotropy And Predictions Of Spin And Electronic Transport Properties For Their Use In Quantum Architectures, Eric Switzer

Electronic Theses and Dissertations, 2020-2023

There has been significant interest in spin systems involving two or more coupled spins as a single logical qubit, particularly for scalable quantum computing architectures. Recent realizations include the so-called singlet-triplet qubits and coupled magnetic molecules. An important class of coupled-spin systems, the three-spin paradigm for spin greater than 1/2, has not yet been fully realized in scalable qubit architectures. In this thesis, I develop the theoretical framework to investigate a class of tripartite spin models for realistic systems. First, I model a spin 1/2 particle (e.g., an electron) and two spin 1 particles (in a dimer arrangement) coupled with …

Anomaly Detection In The Molecular Structure Of Gallium Arsenide Using Convolutional Neural Networks, Timothy Roche, Aihua W. Wood, Philip Cho, Chancellor Johnstone

Faculty Publications

This paper concerns the development of a machine learning tool to detect anomalies in the molecular structure of Gallium Arsenide. We employ a combination of a CNN and a PCA reconstruction to create the model, using real images taken with an electron microscope in training and testing. The methodology developed allows for the creation of a defect detection model, without any labeled images of defects being required for training. The model performed well on all tests under the established assumptions, allowing for reliable anomaly detection. To the best of our knowledge, such methods are not currently available in the open …

Spectroscopy Of Highly Charged Ions For Astrophysical And Laboratory Plasma Diagnostics, Yang Yang

All Dissertations

Electron beam ion traps (EBITs) are small-scale laboratory devices that create and trap highly charged ions (HCI) for spectroscopic studies. These devices create plasma conditions resembling astrophysical environments like stellar winds and supernova remnants, providing valuable insights into astrophysical plasma. Theoretical models for such systems require incorporating relativistic and quantum electrodynamics effects, making experimental studies of HCIs essential for benchmarking these theories.

Spectral analysis of astrophysical and laboratory plasma requires understanding the ionization balance. Accurate atomic data, including excitation, ionization, and recombination cross sections, along with precise knowledge of operating conditions such as electron beam density, electron beam energy, and …

Study Of Highly Charged Ion Charge Exchange With Applications To X-Ray Astrophysics, Richard Mattish

All Dissertations

Highly charged ions (HCIs) exist in many hot astrophysical environments where they play an important role in plasma dynamics. Charge exchange involving highly charged ions has been shown to be responsible for many observed X-ray emissions from a variety of astrophysical sources. Proper modeling of these environments requires an understanding of this process, including the electronic structure of each ion species as well as their charge exchange cross sections. This dissertation investigates charge exchange processes with highly charged ions which are present in astrophysical environments via a laboratory-based study.

The Clemson University electron beam ion trap (CUEBIT) laboratory was utilized …

High-Power Laser Cooling And Temperature-Dependent Fluorescence Studies Of Ytterbium Doped Silica, Brian Topper

Optical Science and Engineering ETDs

Experimental observation of optical refrigeration using ytterbium doped silica glass in recent years has created a new solution for heat mitigation in high-power laser systems, nonlinear fiber experiments, integrated photonics, and precision metrology. Current efforts of different groups focus on compositional optimization, fiber fabrication, and investigating how much silica can be cooled with a laser. At the start of this work, the best effort in laser cooling ytterbium doped silica saw cooling by 6 K from room temperature. This dissertation follows the experimental efforts that culminated in the increase of this initial record by one order of magnitude. Comprehensive spectroscopic …

Portable Optical Spectroscopic Assay For Non-Destructive Measurement Of Key Metabolic Parameters On In Vitro Cancer Cells And Organotypic Fresh Tumor Slices, Jing Yan, Carlos Frederico Lima Goncalves, Madison O. Korfhage, Zahid Hasan, Teresa Whei-Mei Fan, Xiaoqin Wang, Caigang Zhu

Markey Cancer Center Faculty Publications

To enable non-destructive metabolic characterizations on in vitro cancer cells and organotypic tumor models for therapeutic studies in an easy-to-access way, we report a highly portable optical spectroscopic assay for simultaneous measurement of glucose uptake and mitochondrial function on various cancer models with high sensitivity. Well-established breast cancer cell lines (MCF-7 and MDA-MB-231) were used to validate the optical spectroscopic assay for metabolic characterizations, while fresh tumor samples harvested from both animals and human cancer patients were used to test the feasibility of our optical metabolic assay for non-destructive measurement of key metabolic parameters on organotypic tumor slices. Our optical …

Simulating Strongly Coupled Many-Body Systems With Quantum Algorithms, Manqoba Qedindaba Hlatshwayo

Dissertations

The complexity of the nuclear many-body problem is a severe obstacle to finding a general and accurate numerical approach needed to simulate medium-mass and heavy nuclei. Even with the advent of exascale classical computing, the impediment of exponential growth of the Hilbert space renders the problem intractable for most classical calculations. In the last few years, quantum algorithms have become an attractive alternative for practitioners because quantum computers are more efficient in simulating quantum physics than classical computers. While a fully fault-tolerant universal quantum computer will not be realized soon, this dissertation explores quantum algorithms for simulating nuclear physics suitable …

Study Of Radiation Effects In Gan-Based Devices, Han Gao

Electrical Engineering Theses and Dissertations

Radiation tolerance of wide-bandgap Gallium Nitride (GaN) high-electron-mobility transistors (HEMT) has been studied, including X-ray-induced TID effects, heavy-ion-induced single event effects, and neutron-induced single event effects. Threshold voltage shift is observed in X-ray irradiation experiments, which recovers over time, indicating no permanent damage formed inside the device. Heavy-ion radiation effects in GaN HEMTs have been studied as a function of bias voltage, ion LET, radiation flux, and total fluence. A statistically significant amount of heavy-ion-induced gate dielectric degradation was observed, which consisted of hard breakdown and soft breakdown. Specific critical injection level experiments were designed and carried out to explore …

Density Dependence And Dynamics Of Dipole-Dipole Interactions Among Rydberg Atoms, Hannah Conley

Physics and Astronomy Summer Fellows

After trapping atoms, exciting them to an initial high-energy Rydberg state, and allowing them a brief time to exchange energy with each other through dipole-dipole interactions, we observe how their energies are redistributed among various energy levels. The measurements we make in this physical experiment do not give insight into how individual atoms interact or metrics like fidelity and entanglement entropy, which impact our results. For this reason, it is useful to compare our results from the physical experiment to those of our simulation on a supercomputer, in which we can track the final and initial energy of individual atoms …

Application Of A Diatomic Molecule Model Potential To A Series Of Homo- And Heterodiatomic Molecules, Dorien E. Carpenter, Javier E. Hasbun

Georgia Journal of Science

We apply a one-dimensional classical model of a diatomic molecule model potential with modifications to H₂, HF, LiF, N₂, and CO. We obtain the unknown parameters of this model by digitizing plots of the potential curves for the molecules from a published, Hartree-Fock based theoretical electron correlation calculation (Piris 2017). We then apply the method of successive approximations to the model in order to calculate the wavenumber for each molecule in the series. The wavenumber depends on a parameter which in turn depends on the initial conditions. The value of this parameter for each individual molecule …

Size Effect On The Optical Response Of Cylindrical Palladium Nanoparticles, Salem Marhaba, Mohammed Khalaf

BAU Journal - Science and Technology

In this work, a computational study is carried out to investigate the optical response of palladium nano-cylinders. The Finite Element Method (FEM) is employed using the COMSOL MULTIPHYSICS simulation program to calculate the scattering, absorption, and extinction cross-sections. The influence of the size of the cylindrical nanoparticles on their optical properties is discussed. The results are plotted for a broad spectral range of wavelengths from ultra-violet to infra-red of the incident electromagnetic wave on the cylindrical nanoparticles.

Intrinsic Point Defects (Vacancies And Antisites) In Cdgep2 Crystals, Timothy D. Gustafson, Nancy C. Giles, Peter G. Schunemann, Kevin T. Zawilski, Kent L. Averett, Jonathan E. Slagle, Larry E. Halliburton

Faculty Publications

Cadmium germanium diphosphide (CdGeP₂) crystals, with versatile terahertz-generating properties, belong to the chalcopyrite family of nonlinear optical materials. Other widely investigated members of this family are ZnGeP₂ and CdSiP₂. The room-temperature absorption edge of CdGeP₂ is near 1.72 eV (720 nm). Cadmium vacancies, phosphorous vacancies, and germanium-on-cadmium antisites are present in as-grown CdGeP₂ crystals. These unintentional intrinsic point defects are best studied below room temperature with electron paramagnetic resonance (EPR) and optical absorption. Prior to exposure to light, the defects are in charge states that have no unpaired spins. Illuminating a CdGeP_{2 …}