Atmospheric Sciences Commons^™

Atmospheric Chemistry Experiment (Ace) Winds, Matthew Wyatt, Peter F. Bernath, Chris Boone, Léo Lavy, Ryan Johnson

Chemistry & Biochemistry Faculty Publications

The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) uses limb geometry to measure transmittance spectra of Earth's atmosphere by solar occultation. Line-of-sight wind speeds can be derived via Doppler shifts of molecular lines in infrared spectra. The wind look direction angles relative to geodetic North are derived from geometry. We validate the new ACE version 5.3 (v.5.3) line-of-sight winds with MIGHTI and meteor radar vector wind observations and find a ±15 m/s sunrise/sunset shift above 80 km. We also compare line-of-sight winds from ACE-FTS v.5.2 and v.5.3 with vector winds from the MERRA-2, HWM14, and WACCM-X models. A ±15 m/s …

Co₂ Isotopologues From The Ace Satellite, D. English, P. Bernath, C. Boone

Chemistry & Biochemistry Faculty Publications

Carbon dioxide isotopologues have been studied thoroughly in the troposphere. In the stratosphere, the minor oxygen CO₂ isotopologues have anomalous abundances due to their exchange reactions with isotopically fractionated ozone, differentiating them from tropospheric CO₂. Previously a model predicted that this anomalous isotopic abundance continues into the mesosphere but lacked verification from experimental observations. Here we use the Atmospheric Chemistry Experiment Fourier Transform Spectrometer which records infrared transmittance spectra of the Earth's limb from low Earth orbit using solar occultation. These infrared spectra provide measurements of global CO₂ isotopologue volume mixing ratios (VMRs) from the upper troposphere to the lower …

Analysis Of Aerosols In The Asian Monsoon Anticyclone As Observed By The Atmospheric Chemistry Experiment, M. Lecours, R. Dodangodage, C. D. Boone, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

During the Asian summer monsoon season, pollutants from the lower troposphere are transported through deep convection to the upper troposphere and lower stratosphere. Surface pollutants such as CO are transported upward and trapped in the anticyclone during this unique atmospheric phenomenon. Associated with the anticyclone is a layer of enhanced aerosols located near the tropopause often referred to as the Asian tropopause aerosol layer (ATAL). The chemical and physical properties of aerosols in the ATAL are not yet fully understood as direct observations of the aerosols are limited. The Atmospheric Chemistry Experiment (ACE) is a satellite mission that provides high-resolution …

Twenty Years Of Global Stratospheric Fluorine Inventories From Atmospheric Chemistry Experiment Fourier Transform Spectrometer (Ace-Fts) Measurements, N. Raymond, P. Bernath, C. Boone, M. Chipperfield

Chemistry & Biochemistry Faculty Publications

We present fluorine inventories calculated for twenty years (2004–2023) and five latitude bands (82°–60°N, 60°–30°N, 30°N–30°S, 30°–60°S, and 60°–82°S) at altitudes from the surface up to 55 km. The inventories were calculated using the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE‐FTS) version 5.2 retrievals of the volume mixing ratios (VMRs) of 15 fluorine‐containing species. Of these 15 species, 3 are product gases: HF, COF₂, COCIF, and 12 are source gases: SF₆, PFC-14 (CF₄), CFC-11 (CCl₃F), CFC-12 (CCl₂F₂), CFC-113 (CCIF₂CCl₂F), HCFC-22 (CHF₂CL), HCFC-141b(C₂H₃Cl₂F), HCFC-142b ( …

High-Altitude Balloon-Launched Uncrewed Aircraft System Measurements Of Atmospheric Turbulence And Qualitative Comparison With Infrasound Microphone Response, Anisa Haghighi

Theses and Dissertations--Mechanical and Aerospace Engineering

This study explores the use of a balloon-launched uncrewed aircraft system (UAS) to measure atmospheric turbulence in the troposphere and lower stratosphere using both wind velocity measurements and infrasonic acoustic energy. The UAS, a glider configured for autonomous descent along a predefined trajectory, had on board, in situ sensors to capture thermodynamic and kinematic atmospheric parameters. Additionally, it carried an infrasonic microphone to evaluate its potential for remotely detecting clear-air turbulence by capturing infrasonic waves. The system’s performance was assessed over the course of three test flights conducted in New Mexico, USA, in 2021. The descent enabled high-resolution profiling, with …

Characterizing The Earth's Magnetosheath With In Situ Measurements, Hector A. Salinas

Physics Dissertations - Archive

Earth’s magnetosheath is a region of shocked plasma that mediates energy and momentum transfer from the solar wind to the magnetosphere. The dynamics and thus the plasma structures of this region are highly dependent on upstream solar wind conditions. As such, the region is often characterized as a turbulent environment, with the most intense periods of turbulence occurring often under quasi-parallel bow shock conditions. This magnetosheath turbulence displays as variable and large-scale fluctuations with in-situ measurements. Given that turbulence is a characteristic feature of the magnetosheath, this dissertation asks two questions: (1) How are plasma structures inside the sheath affected …

Light Absorbing Aerosol Interactions With Warm Clouds, Shreya Joshi

Dissertations, Master's Theses and Master's Reports

Atmospheric particles such as biomass-burning aerosols, including black carbon - are critical in altering the Earth's energy balance through interactions with light and clouds. Biomass-burning aerosols also contain organic carbon, a diverse mix of organic compounds. As these aerosols age, they evolve by interacting with other atmospheric species, including cloud water, leading to changes in particle morphology and the development of coatings that impact their lifetime and ability to interact with clouds and light.

Some biomass-burning aerosols serve as cloud condensation nuclei. When cloud water droplets form, the properties of the nucleating particles can change. Many clouds evaporate before precipitating, …

Cloud Condensation Nuclei Activity Of Fresh And Aged Phenolic Acid Aerosol Particles, Emily A. Nortmann

Honors Undergraduate Theses

In recent years, the incidence of wildfires has considerably increased, with fire seasons starting earlier and ending later than usual due to changes in snowpack, precipitation, and temperature, which are attributed in part to climate change. Wildfires are responsible for the emission of a variety of gases and organic aerosol particles in the atmosphere with profound impacts on air quality, visibility, and human health. The aerosol particles produced by wildfires can contribute to climate change by scattering or absorbing solar radiation, affecting the radiative balance of the planet through cooling or warming effects, or by acting as cloud condensation nuclei …

Cover Crops Can Reduce Greenhouse Gas Emissions From No-Till Maize In Southern Brazil: Insights From A Long-Term Field Experiment, Guilherme Rosa Da Silva, Adam J. Liska, Cimélio Bayer

Adam Liska Papers

Brazil is one of the countries that has the most agricultural area under no-till (NT) management. This research study aims to evaluate life-cycle greenhouse gas (GHG) emissions from maize (M) grain production in agroecosystems that used different cover crops under NT management in southern Brazil. The data for this study were from a long-term 41-year field experiment in southern Brazil. The long-term experiment evaluated the effects of fallow (F) and cover crops (oat (O), vetch (V), cowpea (B), pigeon pea (P), and lablab (L)) on nitrous oxide and methane emissions and soil carbon (C) sequestration in maize agroecosystems. Five cropping …

Development Of An Quadcopter Unmanned Aerial Vehicle For Atmospheric Remote Sensing, Omar J. Addasi

Dissertations and Theses

This paper explores the development of a quadcopter unmanned aerial vehicle (UAV, a.k.a. drone) for atmospheric remote sensing of temperature, pressure, humidity, and PM2.5 particulate matter quantities. A 3-D printed drone body is designed and flight tuning is performed. An optimal length for an upward extending mast for the drone body is determined. Low cost, lightweight sensors are compared against higher precision sensors in both static and dynamic conditions. In addition, an initial investigation into the design of a pressure sensor based anemometer is performed.

A Wall Of Smoke: Understanding The Drivers Of The June 2023 Canadian Wildfire Smoke Event For New York City, Gregory S. Randazzo

Dissertations and Theses

The 2023 Canadian wildfire season was notable for its extent and the dense smoke it produced. Motivated by the resulting air quality impacts in the New York City region, we explore how the total particulate matter output from the Quebec fires influenced PM2.5 concentrations downstream in New York City. Using injection height data from the Regional Advanced Baseline Imager + VIIRS Emissions dataset, we relate the tropospheric injection heights of the fires with the broader synoptic context and surface PM2.5 concentrations. Using data from the NYS Mesonet Profiler Network, radiosondes, and ERA5 reanalysis, we document the connection between an anomalous …

Stratospheric Variability And Its Relationship To Cold Air Outbreaks In The United States, Paul T. Panhans

Electronic Theses & Dissertations (2024 - present)

Only since the early 2000s, has there been a growing body of work linking extreme winter temperature anomalies to the variability of the Northern Hemisphere stratospheric polar vortex (SPV). However, the understanding behind stratosphere-troposphere coupling and cold air outbreaks (CAOs) remain occasionally contradictory in the literature, making it difficult to properly articulate societal risks. Studies often focused on broad stratospheric influences, but this research directly compared stratospheric variability according to their respective tropospheric impacts. This dissertation filled a knowledge gap, as there has yet to be a comprehensive analysis to quantify the differences in stratospheric variability with and without CAOs …

Understanding The Dynamical Mechanisms Governing Northern Hemisphere Wintertime Persistent Flow Regimes And Their Associated Extreme Weather Events, Tyler Christopher Leicht

Electronic Theses & Dissertations (2024 - present)

Weather regimes are characterized as patterns of low-frequency variability in the middle to upper troposphere of the extratropics. Weather regimes can also be linked to variations in surface weather, making the study of weather regimes a bridge between traditional synoptic-dynamic meteorology and subseasonal-to-seasonal variability. This dissertation identifies and categorizes persistent flow regimes (PFRs), analyzes the dynamics underpinning PFR formation, identifies the linkages to atmospheric teleconnections, and examines the occurrence of surface weather extremes before and during PFRs.

PFRs are identified from 1979–2022 and grouped into five clusters using k-means clustering, which then allows for time-lag composite analysis to determine the …

Dynamics Of Mesoscale Offshore Wind Flows From An Observational And Modeling Perspective: Implications For Offshore Wind Energy, Elizabeth J. Mccabe

Electronic Theses & Dissertations (2024 - present)

Mid-latitude coastal regions of the United States, such as the New York Bight (NYB), are playing a major role in the development of offshore wind energy. However, mesoscale dynamics of local and regional circulations in these offshore waters are poorly understood. The sea breeze, especially in the NYB, will play a key role in the development of offshore wind energy, given the favorable wind speeds and high capacity factors during periods of peak demand. With limited vertical wind profile observations available offshore, the ability to accurately forecast and understand the spatiotemporal extent of the sea breeze and often associated low-level …

Analysis Of Extreme Rainfall And Streamflow Events In The Catskill/Delaware Catchment Using The New York State Mesonet, Ada Ellingworth

Electronic Theses & Dissertations (2024 - present)

Extreme rainfall and streamflow often lead to increased turbidity in reservoirs in the Catskill/Delaware catchment, which is part of the New York City water supply system. To better understand extreme events that lead to increased turbidity, this study takes a dual approach: first, we identify hydrologic conditions during extremes to understand when and why extremes occur. Next, we evaluate an identified extreme case to evaluate mesoscale model skill in this region. Measurements from the New York State Mesonet and United States Geological Survey are used to identify hydrologic conditions from 2017-2024 associated with three extreme event types: rainfall, streamflow, and …

Convective Modes Associated With Precipitation Exceeding Postfire Debris Flow Thresholds In The Southwestern United States, Anya M. Aponte Torres

Graduate Research Theses & Dissertations

Postfire debris flows can occur when surface-water runoff dislodges and carries a slurry of loose sediment and vegetation downslope, usually in steep, recently burned terrain. Short-duration, high-intensity rainfall embedded within short or long-duration rainstorms (e.g., thunderstorms and atmospheric rivers) is most commonly associated with this mode of debris-flow initiation. The typical horizontal grid spacings of global numerical weather prediction and general circulation models are too coarse to resolve these convective precipitation features, which poses an obstacle to short-term forecasting and investigating future trends in the frequency, magnitude, and characteristics of debris-flow generating rainfall. For this study, 15-minute precipitation and simulated …

The Response Of Tropopause Phenomena To Stratospheric Variability: Rossby Wave Breaking And Tropopause Polar Vortices, Cameron R. Paquette

Electronic Theses & Dissertations (2024 - present)

Variability in the high-latitude wintertime stratospheric flow, often referred to as the stratospheric polar vortex, can precede anomalous conditions in tropospheric flow on subseasonal-to-seasonal (S2S) timescales and impact surface weather. The range of stratospheric impacts on tropospheric conditions range from shifts in the North Atlantic storm tracks, formation of cold spells, and development of extreme precipitation. Impacts of stratospheric variability are known to persist for up to 60 days, providing ample windows of opportunity in forecasting on S2S timescales. This dissertation focuses on the stratospheric impacts on tropopause-level processes, such as Rossby wave breaking (RWB) events and tropopause polar vortices …

Limitations Of The High-Resolution Rapid Refresh Gust Algorithm, Alex M. Glasser

Electronic Theses & Dissertations (2024 - present)

ABSTRACT:

Accurate wind and gust forecasts are crucial in operational meteorology, yet there is a distinct gap in the literature regarding the verification of operational gust forecasts. In the present work, we assess the performance of the High-Resolution Rapid Refresh's (HRRR) gust potential, verifying it against the Automated Surface Observing System's (ASOS) observed gusts across the Continental United States (CONUS). The HRRR gust's diurnal cycle reveals a significant underprediction of the gust during daylight hours and a slight overprediction of the gust during hours of darkness. The daytime underprediction undermines the assumption that forecasts represent a potential that tends to …

A Dynamically Adapting Forecast Cone Based On Ensemble Spread, Michael N. Barletta

Electronic Theses & Dissertations (2024 - present)

Dynamically based ensemble prediction systems have gained considerable attention because they can provide a greater range of possible forecast outcomes and quantify the uncertainty in forecasts. In turn, forecasters can convey clearer messages to the public on the range of forecast scenarios and display inherent uncertainty in weather forecasts, which can be difficult to do with deterministic forecasts. Although global ensemble prediction systems have demonstrated skill in their probabilistic track predictions, the information contained within them is not always fully utilized beyond the mean forecast and standard deviation (i.e., spread). One way that these ensembles could be better employed is …

Using The High Resolution Rapid Refresh To Validate A Novel Forecast Methodology, Sylvia M. Garmong

Electronic Theses & Dissertations (2024 - present)

NOAA’s High-Resolution Rapid Refresh (HRRR) is frequently used by forecasters for short term predictions and although the model performs well in many metrics, previous study (Fovell and Gallagher 2020) identified temperature and windspeed biases within the boundary layer using radiosonde and surface observations. The current work uses a forecast drift metric to study how model forecasts evolve with time and distance to radiosonde sites. The metric is calculated by subtracting model analysis from forecasts at the same valid time, creating a proxy for bias. HRRR data on native model levels are obtained from the Google Cloud and Amazon Web Services …