Atmospheric Sciences Commons^™

Verification Of Real-Time Smoke Simulations: A Case Study On Early Summer North American Wildfire Events, Daniel Bonilla

Pitzer Senior Theses

As wildfire intensity and frequency escalate in times of unprecedented climate change and severe droughts, it is important to enhance forecasting models that accurately and efficiently predict wildfire smoke movement. NOAA’s experimental Rapid-Refresh Forecasting System with Smoke and Dust (RRFS-SD) aims to improve upon the High-Resolution Rapid Refresh- Smoke (HRRR-Smoke), by extending the domain to include all of North America and incorporating new developments in physics and wildfire parameterizations. Our work explores the process of adding satellite Aerosol Optical Depth (AOD) data, through AERONET, as an additional method of verification of the RRFS-SD experimental model. Using a case study on …

Collision-Induced Absorption Spectra Of N₂ And Ch₄, Ryan M. Johnson, Peter F. Bernath, Brant Billinghurst, Jianbao Zhao

Chemistry & Biochemistry Faculty Publications

Collision-induced spectra are essential for radiative transfer modeling of Titan's atmosphere. We present experimental spectra of nitrogen–methane mixtures with an accompanying fit of N₂-CH₄ collision-induced absorption in the 30–400 cm⁻¹ region at about 130 K. We found a peak absorption of 2.30 × 10⁻⁵ cm⁻¹ amagat⁻² at 75 cm⁻¹ and a secondary peak of 1.35 × 10⁻⁵ c⁻¹ amagat⁻² at 206.5 cm⁻¹, which agrees with previous studies. Our work does not support the suggestion that N₂-CH₄ CIA in the far-infrared should be increased by about 50%, as suggested by spectroscopic modeling of Titan using data from A. Borysow & C. …

Atmospheric Chemistry Experiment (Ace) Winds, Matthew Wyatt, Peter F. Bernath, Chris Boone, Léo Lavy, Ryan Johnson

Chemistry & Biochemistry Faculty Publications

The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) uses limb geometry to measure transmittance spectra of Earth's atmosphere by solar occultation. Line-of-sight wind speeds can be derived via Doppler shifts of molecular lines in infrared spectra. The wind look direction angles relative to geodetic North are derived from geometry. We validate the new ACE version 5.3 (v.5.3) line-of-sight winds with MIGHTI and meteor radar vector wind observations and find a ±15 m/s sunrise/sunset shift above 80 km. We also compare line-of-sight winds from ACE-FTS v.5.2 and v.5.3 with vector winds from the MERRA-2, HWM14, and WACCM-X models. A ±15 m/s …

Cloud Condensation Nuclei Activity Of Fresh And Aged Phenolic Acid Aerosol Particles, Emily A. Nortmann

Honors Undergraduate Theses

In recent years, the incidence of wildfires has considerably increased, with fire seasons starting earlier and ending later than usual due to changes in snowpack, precipitation, and temperature, which are attributed in part to climate change. Wildfires are responsible for the emission of a variety of gases and organic aerosol particles in the atmosphere with profound impacts on air quality, visibility, and human health. The aerosol particles produced by wildfires can contribute to climate change by scattering or absorbing solar radiation, affecting the radiative balance of the planet through cooling or warming effects, or by acting as cloud condensation nuclei …

High-Altitude Balloon-Launched Uncrewed Aircraft System Measurements Of Atmospheric Turbulence And Qualitative Comparison With Infrasound Microphone Response, Anisa Haghighi

Theses and Dissertations--Mechanical and Aerospace Engineering

This study explores the use of a balloon-launched uncrewed aircraft system (UAS) to measure atmospheric turbulence in the troposphere and lower stratosphere using both wind velocity measurements and infrasonic acoustic energy. The UAS, a glider configured for autonomous descent along a predefined trajectory, had on board, in situ sensors to capture thermodynamic and kinematic atmospheric parameters. Additionally, it carried an infrasonic microphone to evaluate its potential for remotely detecting clear-air turbulence by capturing infrasonic waves. The system’s performance was assessed over the course of three test flights conducted in New Mexico, USA, in 2021. The descent enabled high-resolution profiling, with …

A Wall Of Smoke: Understanding The Drivers Of The June 2023 Canadian Wildfire Smoke Event For New York City, Gregory S. Randazzo

Dissertations and Theses

The 2023 Canadian wildfire season was notable for its extent and the dense smoke it produced. Motivated by the resulting air quality impacts in the New York City region, we explore how the total particulate matter output from the Quebec fires influenced PM2.5 concentrations downstream in New York City. Using injection height data from the Regional Advanced Baseline Imager + VIIRS Emissions dataset, we relate the tropospheric injection heights of the fires with the broader synoptic context and surface PM2.5 concentrations. Using data from the NYS Mesonet Profiler Network, radiosondes, and ERA5 reanalysis, we document the connection between an anomalous …

Development Of An Quadcopter Unmanned Aerial Vehicle For Atmospheric Remote Sensing, Omar J. Addasi

Dissertations and Theses

This paper explores the development of a quadcopter unmanned aerial vehicle (UAV, a.k.a. drone) for atmospheric remote sensing of temperature, pressure, humidity, and PM2.5 particulate matter quantities. A 3-D printed drone body is designed and flight tuning is performed. An optimal length for an upward extending mast for the drone body is determined. Low cost, lightweight sensors are compared against higher precision sensors in both static and dynamic conditions. In addition, an initial investigation into the design of a pressure sensor based anemometer is performed.

Evaluation Of Practical Methods To Determine If A Karst Creek Is Gaining Or Losing: Case Study Of Leith Creek, Elizabeth Jones

Graduate Theses/Dissertations

Karst landscapes are abundant in Missouri, with features such as caves, springs, and sinkholes that form through the dissolution of limestone. Leith Creek is a small stream in Polk County, Missouri fed by two springs and the shallow unconfined Springfield Plateau aquifer, a highly karstified aquifer which is made up of limestone and minor interbedded shale-mudstone units. To determine if Leith Creek is gaining or losing, stream flow, water chemistry and temperature sensors were monitored. Stream flow results required multiple visits to take measurements while temperature sensors required two visits, one to install the dataloggers and another to remove the …

Light Absorbing Aerosol Interactions With Warm Clouds, Shreya Joshi

Dissertations, Master's Theses and Master's Reports

Atmospheric particles such as biomass-burning aerosols, including black carbon - are critical in altering the Earth's energy balance through interactions with light and clouds. Biomass-burning aerosols also contain organic carbon, a diverse mix of organic compounds. As these aerosols age, they evolve by interacting with other atmospheric species, including cloud water, leading to changes in particle morphology and the development of coatings that impact their lifetime and ability to interact with clouds and light.

Some biomass-burning aerosols serve as cloud condensation nuclei. When cloud water droplets form, the properties of the nucleating particles can change. Many clouds evaporate before precipitating, …

Analysis Of Aerosols In The Asian Monsoon Anticyclone As Observed By The Atmospheric Chemistry Experiment, M. Lecours, R. Dodangodage, C. D. Boone, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

During the Asian summer monsoon season, pollutants from the lower troposphere are transported through deep convection to the upper troposphere and lower stratosphere. Surface pollutants such as CO are transported upward and trapped in the anticyclone during this unique atmospheric phenomenon. Associated with the anticyclone is a layer of enhanced aerosols located near the tropopause often referred to as the Asian tropopause aerosol layer (ATAL). The chemical and physical properties of aerosols in the ATAL are not yet fully understood as direct observations of the aerosols are limited. The Atmospheric Chemistry Experiment (ACE) is a satellite mission that provides high-resolution …

Co₂ Isotopologues From The Ace Satellite, D. English, P. Bernath, C. Boone

Chemistry & Biochemistry Faculty Publications

Carbon dioxide isotopologues have been studied thoroughly in the troposphere. In the stratosphere, the minor oxygen CO₂ isotopologues have anomalous abundances due to their exchange reactions with isotopically fractionated ozone, differentiating them from tropospheric CO₂. Previously a model predicted that this anomalous isotopic abundance continues into the mesosphere but lacked verification from experimental observations. Here we use the Atmospheric Chemistry Experiment Fourier Transform Spectrometer which records infrared transmittance spectra of the Earth's limb from low Earth orbit using solar occultation. These infrared spectra provide measurements of global CO₂ isotopologue volume mixing ratios (VMRs) from the upper troposphere to the lower …

Characterizing The Earth's Magnetosheath With In Situ Measurements, Hector A. Salinas

Physics Dissertations - Archive

Earth’s magnetosheath is a region of shocked plasma that mediates energy and momentum transfer from the solar wind to the magnetosphere. The dynamics and thus the plasma structures of this region are highly dependent on upstream solar wind conditions. As such, the region is often characterized as a turbulent environment, with the most intense periods of turbulence occurring often under quasi-parallel bow shock conditions. This magnetosheath turbulence displays as variable and large-scale fluctuations with in-situ measurements. Given that turbulence is a characteristic feature of the magnetosheath, this dissertation asks two questions: (1) How are plasma structures inside the sheath affected …

Twenty Years Of Global Stratospheric Fluorine Inventories From Atmospheric Chemistry Experiment Fourier Transform Spectrometer (Ace-Fts) Measurements, N. Raymond, P. Bernath, C. Boone, M. Chipperfield

Chemistry & Biochemistry Faculty Publications

We present fluorine inventories calculated for twenty years (2004–2023) and five latitude bands (82°–60°N, 60°–30°N, 30°N–30°S, 30°–60°S, and 60°–82°S) at altitudes from the surface up to 55 km. The inventories were calculated using the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE‐FTS) version 5.2 retrievals of the volume mixing ratios (VMRs) of 15 fluorine‐containing species. Of these 15 species, 3 are product gases: HF, COF₂, COCIF, and 12 are source gases: SF₆, PFC-14 (CF₄), CFC-11 (CCl₃F), CFC-12 (CCl₂F₂), CFC-113 (CCIF₂CCl₂F), HCFC-22 (CHF₂CL), HCFC-141b(C₂H₃Cl₂F), HCFC-142b ( …

The Response Of Tropopause Phenomena To Stratospheric Variability: Rossby Wave Breaking And Tropopause Polar Vortices, Cameron R. Paquette

Electronic Theses & Dissertations (2024 - present)

Variability in the high-latitude wintertime stratospheric flow, often referred to as the stratospheric polar vortex, can precede anomalous conditions in tropospheric flow on subseasonal-to-seasonal (S2S) timescales and impact surface weather. The range of stratospheric impacts on tropospheric conditions range from shifts in the North Atlantic storm tracks, formation of cold spells, and development of extreme precipitation. Impacts of stratospheric variability are known to persist for up to 60 days, providing ample windows of opportunity in forecasting on S2S timescales. This dissertation focuses on the stratospheric impacts on tropopause-level processes, such as Rossby wave breaking (RWB) events and tropopause polar vortices …

Convective Modes Associated With Precipitation Exceeding Postfire Debris Flow Thresholds In The Southwestern United States, Anya M. Aponte Torres

Graduate Research Theses & Dissertations

Postfire debris flows can occur when surface-water runoff dislodges and carries a slurry of loose sediment and vegetation downslope, usually in steep, recently burned terrain. Short-duration, high-intensity rainfall embedded within short or long-duration rainstorms (e.g., thunderstorms and atmospheric rivers) is most commonly associated with this mode of debris-flow initiation. The typical horizontal grid spacings of global numerical weather prediction and general circulation models are too coarse to resolve these convective precipitation features, which poses an obstacle to short-term forecasting and investigating future trends in the frequency, magnitude, and characteristics of debris-flow generating rainfall. For this study, 15-minute precipitation and simulated …

Deep Convection, Lightning, And Inertio-Gravity Waves: An Analysis Of Precipitation And Wave Dynamics In The Congo Basin, Stephen L. Solimine

Electronic Theses & Dissertations (2024 - present)

The lack of an extensive in situ observation network throughout equatorial Africa makes it difficult to monitor the Congo climate system. Model and reanalysis products have been used to fill informational gaps but often produce disparate results. To improve model representation of deep convection over the Congo, it’s important to first understand the influence of various thermodynamic and dynamic forces that may be underrepresented. Although satellite based remote sensing retrievals and reanalysis have their own set of limitations, they can offer a great deal of insight into the climate of regions otherwise lacking in observational networks.

The first section of …

A Dynamically Adapting Forecast Cone Based On Ensemble Spread, Michael N. Barletta

Electronic Theses & Dissertations (2024 - present)

Dynamically based ensemble prediction systems have gained considerable attention because they can provide a greater range of possible forecast outcomes and quantify the uncertainty in forecasts. In turn, forecasters can convey clearer messages to the public on the range of forecast scenarios and display inherent uncertainty in weather forecasts, which can be difficult to do with deterministic forecasts. Although global ensemble prediction systems have demonstrated skill in their probabilistic track predictions, the information contained within them is not always fully utilized beyond the mean forecast and standard deviation (i.e., spread). One way that these ensembles could be better employed is …

Analysis Of Extreme Rainfall And Streamflow Events In The Catskill/Delaware Catchment Using The New York State Mesonet, Ada Ellingworth

Electronic Theses & Dissertations (2024 - present)

Extreme rainfall and streamflow often lead to increased turbidity in reservoirs in the Catskill/Delaware catchment, which is part of the New York City water supply system. To better understand extreme events that lead to increased turbidity, this study takes a dual approach: first, we identify hydrologic conditions during extremes to understand when and why extremes occur. Next, we evaluate an identified extreme case to evaluate mesoscale model skill in this region. Measurements from the New York State Mesonet and United States Geological Survey are used to identify hydrologic conditions from 2017-2024 associated with three extreme event types: rainfall, streamflow, and …

Influence Of Cloud-Radiative Forcing On Tropical Cyclone Development In Moderate Vertical Wind Shear, Jannetta C. Richardson

Electronic Theses & Dissertations (2024 - present)

This research seeks to better understand how cloud–radiative forcing (CRF) influences the structural evolution and intensity change of tropical cyclones (TCs) during the organizaional stage, with a particular focus on environments characterized by moderate vertical wind shear. While CRF has been shown to impact TC development during genesis and mature stages, its role during the transitional post-genesis phase—when TCs exhibit disorganized convection and are highly sensitive to environmental influences—remains poorly understood. Moreover, forecasting TC intensity in moderate shear environments continues to present substantial challenges, underscoring the need for focused investigation of TC development in the moderate-shear regime.

The Weather Research …

The Large-Scale Flow Dynamics And Controls On Recurving Eastern North Pacific Tropical Cyclones, Alexander Kyle Mitchell

Electronic Theses & Dissertations (2024 - present)

While eastern North Pacific (EPAC) tropical cyclones (TCs) most often move westward over open water, a subset deviates from this typical path, recurving toward higher latitudes or making landfall along the North American coastline. Because such events are relatively rare, they have received less attention, despite their significant contributions to rainfall and wildfire activity across the southwestern United States. This dissertation identifies and characterizes the spatial variability of EPAC TC tracks, analyzes the synoptic environments associated with TC recurvature near the North American coast, presents a detailed case study of two recurving EPAC TCs from late September to early October …