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Atomic, Molecular and Optical Physics

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Articles 1 - 30 of 2062

Full-Text Articles in Physics

Synthesizing Viscoelasticity: Living Polymers, Micro-Macro Relations, And Paths For Resolution, Adam M. Hasler Aug 2026

Synthesizing Viscoelasticity: Living Polymers, Micro-Macro Relations, And Paths For Resolution, Adam M. Hasler

Graduate Masters Theses

This thesis investigates the relationship between macroscopic rheological signals and underlying microscopic dynamics in complex fluids, specifically focusing on ”living polymers” within the cetyltrimethylammonium bromide (CTAB) and sodium salicylate (NaSal) surfactant system. The research addresses the inverse parameterization problem, demonstrating how bulk measurements like zero-shear viscosity can mask fundamentally different physical topologies, such as purely cylindrical, reptating micelles versus highly branched networks. Through the successful synthesis of viscoelastically ”degenerate” samples, the study utilizes an array of characterization techniques including frequency sweeps, Large Amplitude Oscillatory Shear (LAOS) to resolve these unique underlying states. Furthermore, the work explores further avenues of study …


Modeling Kinetics Of 5-Aminolevulinic Acid-Induced Protoporphyrin Ix Accumulation For Optimal Photodynamic Therapy, Priscilla Melebor Aug 2026

Modeling Kinetics Of 5-Aminolevulinic Acid-Induced Protoporphyrin Ix Accumulation For Optimal Photodynamic Therapy, Priscilla Melebor

Graduate Masters Theses

Photodynamic therapy (PDT) is a minimally invasive treatment that uses light-activated photosensitizers to selectively destroy diseased tissue through the generation of reactive oxygen species. However, conventional in vitro models often fail to accurately reproduce the pharmacokinetics of photosensitizer accumulation and clearance observed in vivo. This study investigated protoporphyrin IX (PpIX) accumulation following 5-aminolevulinic acid (ALA) exposure under physiologically relevant conditions using two-dimensional (2D) monolayers and three-dimensional (3D) spheroids. By comparing continuous ALA exposure with transient exposure followed by ALA washout, this work provides a more biologically relevant framework for studying PpIX kinetics and optimizing photodynamic therapy.


Symmetry Breaking And Restoration In The Grasshopper Ising Model, Aradh Bisarya Aug 2026

Symmetry Breaking And Restoration In The Grasshopper Ising Model, Aradh Bisarya

Graduate Masters Theses

Distance-selective interactions in Ising systems give rise to a range of rich and unexpected phenomena. A notable example is the so-called Grasshopper Ising model, a conserved spin Ising model with interactions only between spins at a fixed distance. This model is the discrete version of the following mathematical problem: A grasshopper lands at a random point on a planar lawn of area one. It then makes one jump of fixed distance in a random direction. What lawn shape maximizes the probability that the grasshopper lands on the lawn after the jump? The solution to this problem, corresponding to the ground …


Fabrication Of Objectives For Imaging Ultracold Lithium, Danelle Akanova Aug 2026

Fabrication Of Objectives For Imaging Ultracold Lithium, Danelle Akanova

Dartmouth College Master’s Theses

This thesis develops a documented, reproducible procedure for building diffraction-limited microscope objectives entirely from catalog singlets, for imaging ultracold 6Li atoms in a ring-trap experiment. The objectives must resolve micron-scale features through a 5 mm fused-silica vacuum window, operate at multiple wavelengths, fit inside a 48 mm magnet bore, and contain no conductive or magnetic material, because the surrounding coils switch 0.1 T fields on microsecond timescales. Commercial long-working-distance objectives are universally housed in metal, which the eddy-current constraint rules out, and custom fabrication of a suitable non-conductive matched pair is estimated at nearly $200k.

The procedure is developed and …


Electronic Structure Discretization And Compression Using Diagonal Basis Sets, Casey Lee Dowdle Aug 2026

Electronic Structure Discretization And Compression Using Diagonal Basis Sets, Casey Lee Dowdle

Dartmouth College Ph.D Dissertations

Numerically solving the electronic structure problem is a fundamentally difficult problem due to the exponential growth in the dimension of the Hilbert space as the system size increases. In order to solve problems at a chemically relevant accuracy, both the choice of basis set and numerical method are important factors that are intrinsically connected.

In this thesis, we study the discretization and resulting compression of electronic Hamiltonians using diagonal basis sets. A diagonal basis set approximately diagonalizes the matrix and tensor representations of the one- and two-body potentials. This can reduce storage, simplify matrix-vector products, and lower the complexity of …


Bounded Thunderstorm Tracking Of Lightning Events With Muon Detection, Skylar Wardlaw, Ainsley Helgerson, Maria Kaminska, Logan Velvet, Georgii Dubrov, Jackson Stewart, Aaron Jung, Nathaniel O’Hara, Amelia Koth, Nash Mcleod, Emaleth Wyckoff Aug 2026

Bounded Thunderstorm Tracking Of Lightning Events With Muon Detection, Skylar Wardlaw, Ainsley Helgerson, Maria Kaminska, Logan Velvet, Georgii Dubrov, Jackson Stewart, Aaron Jung, Nathaniel O’Hara, Amelia Koth, Nash Mcleod, Emaleth Wyckoff

Discovery Day - Daytona Beach

The muon is a high-energy particle that can be produced by cosmic rays and trigger upper-atmospheric particle cascades and energetic processes. It has been hypothesized that such cascades are at the onset of lightning. As such, muons serve as a valuable probe for investigating the underlying mechanisms of its initiation, whose full governing dynamics remain vastly unknown despite extensive research. Traditional approaches to lightning research involve simulations and observations of the discharge itself, but the role of high-energy particle interactions has yet to be fully constrained. The CosmicWatch Muon Detector design enables the detection of atmospheric muons through scintillation events, …


Coherent Two-Photon Backscattering And Induced Angular Quantum Correlations In Multiple-Scattered Two-Photon States Of The Light, Nooshin M. Estakhri, Theodore B. Norris Jul 2026

Coherent Two-Photon Backscattering And Induced Angular Quantum Correlations In Multiple-Scattered Two-Photon States Of The Light, Nooshin M. Estakhri, Theodore B. Norris

Engineering Faculty Articles and Research

We present the emergence of coherent two-photon backscattering, a manifestation of weak localization, in multiple scattering of maximally entangled pure and fully mixed two-photon states and examine the effect of entanglement and classical correlations. Quantum correlations in backscattering are investigated for finite three-dimensional disordered structures in the weak localization regime, as well as systems of a small number of scatterers with specified spatial arrangements. No assumptions are made about the statistical behavior of the scattering matrix elements. Furthermore, we study the interplay between quantum correlations induced by multiple scattering and the correlations that may be present in the illumination fields, …


Lafe0.925ti0.075o3 Perovskite Coated With Ethyl Cellulose: A High-Stability, Low-Hysteresis Platform For Advanced Humidity Sensing, Akhmad Futukhillah Fataba Alaih, Djoko Triyono, Rifqi Almusawi Rafsanjani Jun 2026

Lafe0.925ti0.075o3 Perovskite Coated With Ethyl Cellulose: A High-Stability, Low-Hysteresis Platform For Advanced Humidity Sensing, Akhmad Futukhillah Fataba Alaih, Djoko Triyono, Rifqi Almusawi Rafsanjani

Makara Journal of Science

Humidity sensors are pivotal in numerous sectors, such as environmental monitoring, industrial automation, and health-care. This study presents the fabrication and detailed evaluation of an advanced humidity sensor using ethyl cellulose (EC)-coated LaFe0.925Ti0.075O3 (LFTO) perovskite nanoparticles synthesized via the sol-gel method. The LFTO nanopar-ticles exhibited a mesoporous structure with an enhanced surface area, which significantly improved their moisture adsorption capabilities. The innovative application of EC coating addresses critical substrate adhesion issues, enhancing mechanical stability without compromising sensor sensitivity. Comprehensive performance evaluations revealed minimal hysteresis (


Structure Functions For The Inclusive Semileptonic B-Quark Decay At Nnlo: A Semi-Analytic Calculation, A. Broggio, B. Capdevila, A. Ferroglia, P. Gambino Jun 2026

Structure Functions For The Inclusive Semileptonic B-Quark Decay At Nnlo: A Semi-Analytic Calculation, A. Broggio, B. Capdevila, A. Ferroglia, P. Gambino

Publications and Research

We present a study of the inclusive charmless semileptonic b decay, bXuℓv at next-to-next-to-leading order (NNLO) in perturbative QCD, with the primary aim of extracting the hadronic structure functions Wi at NNLO. The analysis is based on a numerical calculation of the relevant kinematic distributions using a phase-space slicing method to handle infrared-sensitive contributions from real gluon emissions. We use known results from Heavy Quark Effective Theory and Soft-Collinear Effective Theory to extract the singular terms and construct a model for the regular contributions to the structure functions at NNLO, then perform a fit to the …


30 Db On-Chip Ultra-High Inverse Weak Value Amplification, Yuhan Mei, Meiting Song, Andrew N. Jordan, Jaime Cardenas Jun 2026

30 Db On-Chip Ultra-High Inverse Weak Value Amplification, Yuhan Mei, Meiting Song, Andrew N. Jordan, Jaime Cardenas

Mathematics, Physics, and Computer Science Faculty Articles and Research

Weak value amplification (WVA) has emerged as a powerful technique that enhances measurement precision. However, traditional table-top WVA setups and on-chip demonstrations have not achieved an amplification over 20 dB. The practical limit of the amplification is the fidelity of photon post-selection. To address this limit, we design a weak value device with an over 30 dB interferometer extinction ratio, where the stray light in the dark port is minimized with thermally tunable phase shifters. As a result, the device successfully shows 30 dB WVA, termed ultra-high WVA. This WVA optimization strategy by improving interferometer extinction is extensible to a …


Characterizing Stiffness Dynamics Of Normal And Malignant Breast Spheroids Using Brillouin Microscopy, Razanne Rafat Zaghloul, Karlin Hilai, Chenjun Shi, Jitao Zhang May 2026

Characterizing Stiffness Dynamics Of Normal And Malignant Breast Spheroids Using Brillouin Microscopy, Razanne Rafat Zaghloul, Karlin Hilai, Chenjun Shi, Jitao Zhang

Medical Student Research Symposium

Background: Breast cancer progression and metastasis are closely linked to alterations in the mechanical properties of tumor cells and their microenvironment. Softer, more deformable cells are often associated with higher metastatic potential. While atomic force microscopy (AFM) is the current gold standard for mechanical characterization, it is limited to surface measurements and can damage 3D cultures. It remains unclear how the mechanical properties evolve over time in normal versus malignant spheroids. This study utilizes Brillouin light-scattering microscopy, a non-contact and label-free optical technique, to assess stiffness changes in normal and malignant breast epithelial spheroids over time. Understanding these mechanical signatures …


Optical Nuclear Spin Detection In Diamond And Varifocal Metasurface Optics, Maxwell D. Aiello May 2026

Optical Nuclear Spin Detection In Diamond And Varifocal Metasurface Optics, Maxwell D. Aiello

Physics & Astronomy ETDs

This dissertation presents two experimental investigations at the intersection of quantum sensing and precision optical instrumentation. The primary project demonstrates optically detected nuclear magnetic resonance (NMR) of 13C nuclear spins in diamond, using state-selective Landau-Zener transitions under microwave frequency sweeping to bidirectionally transfer spin polarization between nitrogen-vacancy (NV) electron spins and remote 13C nuclear spins. This enables optical polarization and readout of large ensembles of polarized nuclear spins at low magnetic fields and room temperature, with spin dephasing times limited by longitudinal relaxation of nearby NV electron spins. The secondary project reports the design, fabrication, and characterization of …


Constructing A Laser Stabilization System For Frequency Metrology, Stephanie Letourneau May 2026

Constructing A Laser Stabilization System For Frequency Metrology, Stephanie Letourneau

UNLV Theses, Dissertations, Professional Papers, and Capstones

Frequency metrology and quantum control, which uses light as a tool for measurement and manipulation, relies on spectrally narrow, stable lasers. Often thought of as being perfectly monochromatic and coherent, in reality, the free-running instantaneous linewidth of lasers can be on the order of hundreds of kHz in the millisecond time-frame and drift on the order of tens of MHz over hours. To correct for these instabilities in real-time, a variety of laser stabilization methods have been implemented, including the Pound-Drever-Hall (PDH) method, saturation absorption spectroscopy (SAS), and dichroic atomic vapor laser locking (DAVLL). All of these methods rely on …


Designing Enhanced Nonlinearity In Plasmonic Devices With Epsilon-Near-Zero Films, Kevin Tran Le May 2026

Designing Enhanced Nonlinearity In Plasmonic Devices With Epsilon-Near-Zero Films, Kevin Tran Le

Electrical Engineering and Computer Science (MS) Theses

The growing demand for energy-efficient optical information processing motivates compact nonlinear photonic devices that can operate at low power. Silicon photonics is a mature platform for linear optical functions, but nonlinear operation remains challenging because of its weak Kerr response, two-photon absorption at telecommunication wavelengths, and limited compatibility with deeply subwavelength plasmonic confinement. This thesis computationally investigates epsilon-near-zero thin films integrated into plasmonic waveguide architectures as a route toward stronger light–matter interaction in compact nonlinear devices.

Two waveguide geometries are examined: a hybrid metal-insulator-metal plasmonic slab waveguide incorporating an ultrathin indium tin oxide epsilon-near-zero layer (5–50 nm), and a dielectric-loaded …


Comparison Of Anomaly Detection Methods On Event-Based Vision Sensor Data In A High Noise Environment, Will Johnston, Anthony L. Franz, Shannon R. Young, Rachel Oliver, Zachary Theis, Brian Mcreynolds, Michael L. Dexter Apr 2026

Comparison Of Anomaly Detection Methods On Event-Based Vision Sensor Data In A High Noise Environment, Will Johnston, Anthony L. Franz, Shannon R. Young, Rachel Oliver, Zachary Theis, Brian Mcreynolds, Michael L. Dexter

Faculty Publications

Event-based vision sensors (EVSs) provide unique frequency analysis opportunities due to their event data output and high temporal resolution. Anomaly detection methods used in hyperspectral analysis can be used on the event frequency spectra to detect targets. However, the introduction of a strong, flickering interfering source can reduce the EVS sensitivity and obscure targets of interest. Previous work presented a method showing that targets could still be detected through an overwhelming source using frequency analysis, background suppression, and statistical filtering. This paper extends that research and compares the ability of five different eigenanalysis anomaly detection methods (principal component background suppression …


Calculating Potential Energy Curves Of Molecular Hydrogen And Its Ion Using Psi4 For Blinc Fusion Applications*, Angelina Castillo, Oscar Coral, Canaan Hercules, Blake Laing, Vola Andrianarijaona Apr 2026

Calculating Potential Energy Curves Of Molecular Hydrogen And Its Ion Using Psi4 For Blinc Fusion Applications*, Angelina Castillo, Oscar Coral, Canaan Hercules, Blake Laing, Vola Andrianarijaona

Campus Research Month

Southern Adventist University’s Beamline for Ionic and Neutral Collisions (BLINC) is investigating the interactions between hydrogen molecules and fusion particles. To perform in-house theoretical calculations, the BLINC Theory and Analysis Group is testing Psi4 as a viable computational method for BLINC fusion research. Successful calculations of the potential energy curves and dissociation energies of H2 and H2+ have been completed and compared to known values. Preliminary results align with known values, demonstrating Psi4’s potential for BLINC research. Future work will focus on the vibrational energies, wavefunctions, and transition probabilities of H2 and H2+.


Construction Of Alkali Oven For Charge Transfer Collisions In Beamline Applications*, Benjamin D. Chun, Oscar T. Coral, Gabriella Kim, Naomi Munyaka, Vola Andrianarijaona Apr 2026

Construction Of Alkali Oven For Charge Transfer Collisions In Beamline Applications*, Benjamin D. Chun, Oscar T. Coral, Gabriella Kim, Naomi Munyaka, Vola Andrianarijaona

Campus Research Month

This work presents the desig and development of an alkali metal oven used for charge-transfer collision experiments within the Beamline for Ionic and Neutral Collisions (BLINC) at Southern Adventist University. This oven is engineered to produce a stable and controllable alkali vapor source (K/Cs), enabling interactions between the H2+ ions and neutral alkali atoms for the study of rovibrational energy transfer.

The alkali metal oven was designed to be modular to switch out different capillary designs for diverse vapor release into the beamline. This system was designed using SolidWorks and fabricated through CNC machining, with particular emphasis on thermal wiring …


Exclusive Neutral Pion Electroproduction Cross Section Measurements With A Neutral Particle Spectrometer, Mitchell R. Kerver Apr 2026

Exclusive Neutral Pion Electroproduction Cross Section Measurements With A Neutral Particle Spectrometer, Mitchell R. Kerver

Physics Theses & Dissertations

Deep Virtual Compton Scattering (DVCS), the exclusive electron-proton scattering process ep →e′p′γ, provides access to generalized parton distributions (GPDs), which correlate informa tion about the longitudinal momentum and transverse spatial structure of quarks inside the nucleon. Experiment E12-13-010 in Hall C at Jefferson Lab was designed to take high-precision measure ments of the DVCS cross section over an extended kinematic range using the newly commis sioned Neutral Particle Spectrometer (NPS). The NPS features a high-resolution electromagnetic calorimeter and a streaming data acquisition system optimized for operation at high luminosities. This thesis presents the detector and analysis work carried out to …


Investigation Of Molecular Footprints In Ultra-High Diluted Homoeopathic Solutions Of Arnica Montana And Rhus Toxicodendron Through Combined Infrared And Impedance Spectroscopy, Sharbadeb Kundu, Usha Rani Dash, Chirasree Roychaudhuri, Aindrila Roy, Sanatan Chattopadhyay, Rathin Chakravarty, Debadatta Nayak, Subhash Kaushik, Amit Roy Chowdhury, Ananya Barui, Subhadip Chakraborty Mar 2026

Investigation Of Molecular Footprints In Ultra-High Diluted Homoeopathic Solutions Of Arnica Montana And Rhus Toxicodendron Through Combined Infrared And Impedance Spectroscopy, Sharbadeb Kundu, Usha Rani Dash, Chirasree Roychaudhuri, Aindrila Roy, Sanatan Chattopadhyay, Rathin Chakravarty, Debadatta Nayak, Subhash Kaushik, Amit Roy Chowdhury, Ananya Barui, Subhadip Chakraborty

Indian Journal of Research in Homoeopathy

Background: The study of ultra-high diluted (UHD) solutions is a compelling and controversial domain in modern science. Despite numerous investigations and hypotheses, there is a lack of rigorous, reproducible empirical evidence supporting the existence of molecular footprints beyond the Avogadro's limit. Objective: This study conducted a detailed investigation of the molecular and electrical properties, focusing on hydrogen bonding and impedance to understand the fundamental nature of UHD solutions. Materials and methods: Combined impedance and infrared spectroscopic investigations were performed to probe the structural behaviour of relevant water networks at the molecular level of UHD alcoholic extract of Arnica montana (AM) …


Guiding Fast Ion Beam By Suppressing Secondary Ions, Yingli Xue, Junliang Liu, Mingwu Zhang, Daniel Fischer, Guoxing Xia, Nikolaus Stolterfoht, Reinhold Schuch, Yehong Wu, Bian Yang, Xiaoxiao Li, Caojie Shao, Wei Wang, Zhangyong Song, Xing Fang Mar 2026

Guiding Fast Ion Beam By Suppressing Secondary Ions, Yingli Xue, Junliang Liu, Mingwu Zhang, Daniel Fischer, Guoxing Xia, Nikolaus Stolterfoht, Reinhold Schuch, Yehong Wu, Bian Yang, Xiaoxiao Li, Caojie Shao, Wei Wang, Zhangyong Song, Xing Fang

Physics Faculty Research & Creative Works

We demonstrate that secondary ions sputtered from a macrocapillary's inner surface by the primary beam induce premature saturation of the guiding field, hindering fast ion guiding. By suppressing secondary ion sputtering with grooved surfaces, we achieve a guiding-field potential difference exceeding 1 kV, 2 orders of magnitude larger than previously achieved in stable ion guiding. This enables stable guiding of a 20-keV/q O5+ beam at offset angles up to 15°, with transmitted ions retaining their initial energy and charge state. A self-consistent field model accurately reproduces these results, revealing that guiding performance relies on managing secondary ions and the channel's …


Uranium Chemical Compound Classification Using Sub-Images And Statistical Machine Learning For Nuclear Forensics, Lee C. Lambert, Brett J. Borghetti, Abigail A. Bickley Feb 2026

Uranium Chemical Compound Classification Using Sub-Images And Statistical Machine Learning For Nuclear Forensics, Lee C. Lambert, Brett J. Borghetti, Abigail A. Bickley

Faculty Publications

Uranium particle analysis from Scanning Electron Microscope (SEM) imagery is a crucial tool in nuclear forensics. The particle morphology lexicon proposed by Tamasi et al. in J Radioanal Nucl Chem 307, 1611–1619 (2016) follows a standardized, manual identification process to identify particle morphology features. The present work seeks to mirror this methodology using computer feature selection from the scikit-image Python library rather than human classification. Using a random forest classifier, a 56% overall uranium true positive classification accuracy (a 39.6% balanced classification accuracy) was achieved on a test set outperforming a naïve (chance) model by 48%. The methodology introduced splits …


Proposed Methodology For Correcting Fourier-Transform Infrared Spectroscopy Field-Of-View Scene-Change Artifacts, Kody A. Wilson, Michael L. Dexter, Benjamin F. Akers, Anthony L. Franz Jan 2026

Proposed Methodology For Correcting Fourier-Transform Infrared Spectroscopy Field-Of-View Scene-Change Artifacts, Kody A. Wilson, Michael L. Dexter, Benjamin F. Akers, Anthony L. Franz

Faculty Publications

Fourier-transform spectrometers are widely used for spectral measurements. Changes in the field of view during measurement introduce oscillations into the measured spectra known as scene-change artifacts. Field-of-view changes also introduce uncertainty about which target the measured spectrum represents. Though scene-change artifacts are often present in dynamic data, their significance is disputed in the current literature. This work presents a theoretical framework and experimental validation for scene-change artifacts. Field-of-view changes introduce variable interferogram offsets, which standard processing techniques assume are constant. The error between the interferogram offset and its estimate is Fourier-transformed, yielding scene-change artifacts, often confused with noise, in the …


A Comparison Of Modeled Daytime E Regions From E-Probed And Pyiri With Ionosonde Observations, Daniel J. Emmons, Cornelius C. J. H. Salinas, Dong L. Wu, Nimalan Swarnalingam, Eugene V. Dao, Jorge L. Chau, Yosuke Yamazaki, Kyle E. Fitch, Victoriya V. Forsythe Jan 2026

A Comparison Of Modeled Daytime E Regions From E-Probed And Pyiri With Ionosonde Observations, Daniel J. Emmons, Cornelius C. J. H. Salinas, Dong L. Wu, Nimalan Swarnalingam, Eugene V. Dao, Jorge L. Chau, Yosuke Yamazaki, Kyle E. Fitch, Victoriya V. Forsythe

Faculty Publications

While the F region is the primary focus of many ionospheric models because it contains the peak electron density, the E region is an important region for ionospheric conductivities and high-frequency radio propagation. This study analyzes modeled E regions from the newly developed PyIRI and E-PROBED models. A long-term comparison of E region predictions from E-PROBED and PyIRI with ionosonde observations is performed for three sites spanning low- (Fortaleza, Brazil), mid- (El Arenosillo, Spain), and high-latitudes (Gakona, Alaska). Modeled foE and hmE trends are compared against a combination of manually-scaled and automatically-scaled ionograms using ARTIST-5 for the period 2009–2024 for …


Frequency Stabilization Of An Affordable Adjustable Repetition Rate Dual Frequency Comb Spectrometer, Michael Moran Jan 2026

Frequency Stabilization Of An Affordable Adjustable Repetition Rate Dual Frequency Comb Spectrometer, Michael Moran

Physics, Astronomy and Geophysics Honors Papers

Two affordably home-built optical frequency combs are stabilized for use in molecular spectroscopy. Each comb is paired with a multi-tiered stabilization scheme that will enable the dual-comb spectrometer to perform precision measurements. The two degrees of freedom for an optical frequency comb, the repetition rate frequency and offset frequency, are accounted for in this stabilization scheme. The repetition rate is directly stabilized through control of the laser enclosure temperature and the fiber laser cavity length. The offset frequency is controlled indirectly via the stabilization of an optical beat note, the heterodyned signal resulting from a narrow linewidth laser and the …


Fully Differential Studies On Dissociative Capture In P + D2 Collisions And On Ionization In P + He Collisions, Shruti Majumdar Jan 2026

Fully Differential Studies On Dissociative Capture In P + D2 Collisions And On Ionization In P + He Collisions, Shruti Majumdar

Doctoral Dissertations

Advancing our understanding of few-body dynamics in simple atomic systems is a fundamental objective in atomic scattering research. The underlying problem is that the Schrödinger equation is not analytically solvable for more than two mutually interacting particles. This involves a comprehensive exploration of various channels, such as ionization, capture, and excitation. A common theoretical approach to describe ion-atom collisions is based on perturbation theory, where the scattering amplitude is expanded in powers of the interaction potential. Here, understanding the few-body problem means accurately describing the relative importance of the higher- vs the first order terms.

In the case of ionization, …


Shock-Wave Structure In A Monatomic Gas Mixture With Rydberg Atoms, Anna Markhotok Jan 2026

Shock-Wave Structure In A Monatomic Gas Mixture With Rydberg Atoms, Anna Markhotok

Physics Faculty Publications

The effect of atom size on the shock-wave structure in a binary monatomic gas mixture with Rydberg atoms has been investigated. The problem was solved numerically using the system of hydrodynamic equations in argon gas for the atom-size ratios between 2 and 100, T = 1500 K, and the density between 10¹⁷ and 10²⁰ m−³. It was found that the presence of larger-sized atoms in the mixture results in shock front splitting that is on the order of the mean free path for this component. The results could be of interest in supersonic plasma dynamics and in astrophysics, studying shock …


First Remi Experiments At A Cryogenic Ion Storage Ring, M. Schulz, F. Herrmann, W. Zhang, A. Dorn, M. Grieser, F. Grussie, H. Kreckel, O. Novotny, A. Wolf, T. Pfeifer, C. D. Schröter, R. Moshammer Jan 2026

First Remi Experiments At A Cryogenic Ion Storage Ring, M. Schulz, F. Herrmann, W. Zhang, A. Dorn, M. Grieser, F. Grussie, H. Kreckel, O. Novotny, A. Wolf, T. Pfeifer, C. D. Schröter, R. Moshammer

Civil, Architectural and Environmental Engineering Faculty Research & Creative Works

We have recorded double, triple, and quadruple coincidences between neutralized projectiles, recoiling target ions, and two electrons created in collisions of slow anions with neutral atoms. The experiments were performed at the cryogenic storage ring in Heidelberg. The recoil ions and ejected electrons were momentum-analyzed using a Reaction Microscope (ReMi) spectrometer. Various processes involving electron detachment from the projectile accompanied by various transitions in the target were investigated. Detachment without any transition in the target is qualitatively well described by a quasi-free electron model in the case of an Ar target. In detachment with single target ionization, no signatures of …


Real-Space Imaging Of The Electron-Pair Density Hole In Molecular Auger-Meitner Decay, Mats Simmermacher, Nathan Goff, Andres Moreno Carrascosa, Elke Fasshauer, Thomas Northey, Lingyu Ma, Haiwang Yong, Brian Stankus, Asami Odate, Xuan Xu, Wenping Du, Kyle Acheson, Joseph C. Cooper, Daniel Ratner, Mengning Liang, Ruaridh Forbes, Michael P. Minitti, Adam Kirrander, Peter M. Weber Jan 2026

Real-Space Imaging Of The Electron-Pair Density Hole In Molecular Auger-Meitner Decay, Mats Simmermacher, Nathan Goff, Andres Moreno Carrascosa, Elke Fasshauer, Thomas Northey, Lingyu Ma, Haiwang Yong, Brian Stankus, Asami Odate, Xuan Xu, Wenping Du, Kyle Acheson, Joseph C. Cooper, Daniel Ratner, Mengning Liang, Ruaridh Forbes, Michael P. Minitti, Adam Kirrander, Peter M. Weber

Physics Faculty Publications

Electrons in matter can rearrange extremely quickly under external perturbations, underpinning subsequent structural and chemical transformations. Coulomb interactions between neighbouring electrons often shape this response, giving rise to correlated motion and strongly affecting the distribution of electrons in the system. Here we show that non-resonant hard X-ray scattering can directly access changes in the radial electron-pair density during the rapid rearrangement of core and valence electrons. We do this by studying sulfur hexafluoride molecules undergoing Auger–Meitner decay. We exploit a second-order interaction between the X-ray photons and the molecules to trigger and probe the decay dynamics with a single pulse, …


An Application Of Molecular Dynamics To Hed Plasma Physics: Point And Group Defect Diffusion In Coulomb Crystals, Levi Webb Jan 2026

An Application Of Molecular Dynamics To Hed Plasma Physics: Point And Group Defect Diffusion In Coulomb Crystals, Levi Webb

Theses and Dissertations

Molecular dynamics (MD) simulations are used to explore the microscopic behaviors of complex systems that cannot be easily studied experimentally. In particular, the microphysics of high energy density (HED) astrophysical plasma environments remain inaccessible by modern experiment---even in laser facilities, these plasmas exist only on short timescales that do not lend easily to investigation. The diffusion of point and group defects through crystallized plasmas in the cores of white dwarfs and neutron star crusts, called Coulomb crystals, has potentially macroscopic implications for the evolution of these bodies. Thus, I employ the widely-used MD code LAMMPS to simulate small Coulomb crystal …


Design, Fabrication Modeling, And Optical Metrology Of Mwir Silicon Metalenses, Weiyu Chen Jan 2026

Design, Fabrication Modeling, And Optical Metrology Of Mwir Silicon Metalenses, Weiyu Chen

Graduate Studies Theses and Dissertations 2026

Mid-wave infrared (MWIR) optical systems require compact, broadband, manufacturable components whose performance can be predicted and measured reliably. Silicon metalenses are attractive because silicon combines high refractive index, MWIR transparency, and semiconductor-compatible fabrication. This dissertation develops a scale-bridging design–fabrication-modeling–metrology framework for MWIR silicon metalenses.

A shared full-aperture framework connects meta-atom libraries, physical layout generation, angular-spectrum propagation, point-spread-function calculation, and focal-plane energy metrics. Building on this foundation, the Dispersive Sweatt Model (DSM) incorporates meta-atom dispersion into conventional ray-tracing software, enabling broadband co-optimization of metasurfaces and refractive elements. A process-aware design framework then incorporates scanning electron microscopy (SEM)-measured height–radius relationships produced by …