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Atomic, Molecular and Optical Physics

2008

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Articles 1 - 30 of 51

Full-Text Articles in Physics

Reconstructing Three-Dimensional Shape Envelopes From Time-Resolved Small-Angle X-Ray Scattering Data, Jessica Lamb, Lisa W. Kwok, Xiangyun Qiu, Kurt Andresen, Hye Yoon Park, Lois Pollack Dec 2008

Reconstructing Three-Dimensional Shape Envelopes From Time-Resolved Small-Angle X-Ray Scattering Data, Jessica Lamb, Lisa W. Kwok, Xiangyun Qiu, Kurt Andresen, Hye Yoon Park, Lois Pollack

Physics and Astronomy Faculty Publications

Modern computing power has made it possible to reconstruct low-resolution, three-dimensional shapes from solution small-angle X-ray scattering (SAXS) data on biomolecules without a priori knowledge of the structure. In conjunction with rapid mixing techniques, SAXS has been applied to time resolve conformational changes accompanying important biological processes, such as biomolecular folding. In response to the widespread interest in SAXS reconstructions, their value in conjunction with such time-resolved data has been examined. The group I intron from Tetrahymena thermophila and its P4–P6 subdomain are ideal model systems for investigation owing to extensive previous studies, including crystal structures. The goal of this …


Material Damage From Ultrashort Bursts Of Light, Jeremy Gulley Oct 2008

Material Damage From Ultrashort Bursts Of Light, Jeremy Gulley

Jeremy R. Gulley

No abstract is currently available.


Direct Observation Of H2 Binding To A Metal Oxide Surface, J. Z. Larese, T. Arnold, L. Frazier, R. J. Hinde, A. J. Ramirez-Cuesta Oct 2008

Direct Observation Of H2 Binding To A Metal Oxide Surface, J. Z. Larese, T. Arnold, L. Frazier, R. J. Hinde, A. J. Ramirez-Cuesta

Chemistry Publications and Other Works

Inelastic neutron scattering is used to probe the dynamical response of H2 films adsorbed on MgO(100) as a function of film thickness. Concomitant diffraction measurements and a reduced-dimensionality quantum dynamical model provide insight into the molecule-surface interaction potential. At monolayer thickness, the rotational motion is strongly influenced by the surface, so that the molecules behave like quasiplanar rotors. These findings have a direct impact on understanding how molecular hydrogen binds to the surface of materials used in catalytic and storage applications.


Dynamics Of Apomyoglobin In The Α-To-Β Transition And Of Partially Unfolded Aggregated Protein, E. Fabiani, A. M. Stadler, D. Madern, M. M. Koza, M. Tehei, M. Hirai, G. Zaccai Oct 2008

Dynamics Of Apomyoglobin In The Α-To-Β Transition And Of Partially Unfolded Aggregated Protein, E. Fabiani, A. M. Stadler, D. Madern, M. M. Koza, M. Tehei, M. Hirai, G. Zaccai

Faculty of Science - Papers (Archive)

Changes of molecular dynamics in the α-to-β transition associated with amyloid fibril formation were explored on apo-myoglobin (ApoMb) as a model system. Circular dichroism, neutron and X-ray scattering experiments were performed as a function of temperature on the protein, at different solvent conditions. A significant change in molecular dynamics was observed at the α-to-β transition at about 55 ˚C, indicating a more resilient high temperature β structure phase. A similar effect at approximately the same temperature was observed in holo-myoglobin, associated with partial unfolding and protein aggregation. A study in a wide temperature range between 20 K and 360 K …


Homogeneous Dbd In N2: 1) Lif, Talif And Electrical Measurements, N. Gherardi, Et. Es-Sebbar, C. Sarra-Bourret, N. Naudé, F. Massines Oct 2008

Homogeneous Dbd In N2: 1) Lif, Talif And Electrical Measurements, N. Gherardi, Et. Es-Sebbar, C. Sarra-Bourret, N. Naudé, F. Massines

Dr. Et-touhami Es-sebbar

In this paper we compare two different discharges that can be obtained in a DBD configuration, that is to say the filamentary discharge (usual regime in atmospheric DBD) with the Atmospheric Pressure Townsend Discharge (APTD), which is a homogeneous regime obtained in nitrogen atmosphere. The aim is to help in the understanding of the processes which control the transition from one regime to the other. To do so, the discharge is characterized through electrical measurements, coupled with optical diagnostics among which Laser Induced Fluorescence (LIF) for radical density measurements. The influence of the addition of small quantities of additives on …


Photoelectron Spectroscopy And Theoretical Studies Of [Com(Pyrene)N]− (M=1,2 And N=1,2) Complexes, Anil K. Kandalam, Puru Jena, Xiang Li, Soren N. Eustis, Kit H. Bowen Oct 2008

Photoelectron Spectroscopy And Theoretical Studies Of [Com(Pyrene)N]− (M=1,2 And N=1,2) Complexes, Anil K. Kandalam, Puru Jena, Xiang Li, Soren N. Eustis, Kit H. Bowen

Physics & Engineering Faculty Publications

No abstract provided.


Theoretical Top Quark Cross Section At The Fermilab Tevatron And The Cern Lhc, Nikolaos Kidonakis, Ramona Vogt Oct 2008

Theoretical Top Quark Cross Section At The Fermilab Tevatron And The Cern Lhc, Nikolaos Kidonakis, Ramona Vogt

Faculty and Research Publications

We present results for the top quark pair cross section at the Tevatron and the LHC. We use the resummed double differential cross section, employing the fully kinematics-dependent soft-anomalous-dimension matrices, to calculate the soft-gluon contributions at next-to-next-to-leading order (NNLO). We improve and update our previous estimates by refining our methods, including further subleading terms, and employing the most recent parton distribution function sets. The NNLO soft corrections significantly enhance the NLO cross section while considerably reducing the scale dependence. We provide a detailed discussion of all theoretical uncertainties in our calculation, including kinematics, scale, and parton distribution uncertainties, and clarify …


Photoelectron Spectroscopic Study Of The Anionic Transition Metalorganic Complexes [Fe1,2(Cot)]− And [C(Cot)]−, Xiang Li, Soren N. Eustis, Kit H. Bowen, Anil K. Kandalam Sep 2008

Photoelectron Spectroscopic Study Of The Anionic Transition Metalorganic Complexes [Fe1,2(Cot)]− And [C(Cot)]−, Xiang Li, Soren N. Eustis, Kit H. Bowen, Anil K. Kandalam

Physics & Engineering Faculty Publications

No abstract provided.


Active Species Generation Of Homogeneous Dbd In N2: Experiment And Modelling, N. Gherardi, Et. Es-Sebbar, C. Sarra-Bourret, N. Naudé, F. Massines, D. Tzyganov, P. Ségur, S. Pancheshnyi Sep 2008

Active Species Generation Of Homogeneous Dbd In N2: Experiment And Modelling, N. Gherardi, Et. Es-Sebbar, C. Sarra-Bourret, N. Naudé, F. Massines, D. Tzyganov, P. Ségur, S. Pancheshnyi

Dr. Et-touhami Es-sebbar

No abstract provided.


A Study Of The Irradiance-And-Temperature-Dependence Of Mid-Wave-Infrared (Mwir)Absorption In Indium Antimonide (Insb), John M. Callahan Sep 2008

A Study Of The Irradiance-And-Temperature-Dependence Of Mid-Wave-Infrared (Mwir)Absorption In Indium Antimonide (Insb), John M. Callahan

Theses and Dissertations

This work entails further investigation of the absorption of photons in indium antimonide (InSb). Previously work at the Air Force Institute of Technology (AFIT) attributed laser blooming effects in InSb focal plane arrays (FPA’s) to the Burstein-Moss effect. The contributing effect is from a decrease in the absorption of the InSb material, such that the transmitted optical energy scatters off the integrated circuitry beneath the InSb thin film back into the optical system. To evaluate this, irradiance-dependent laser-absorption experiments were performed on thinned, InSb wafers prior to their FPA fabrication. The samples were illuminated with a focused CO2 laser at …


Linear Dichroism In Resonant Inelastic X-Ray Scattering To Molecular Spin-Orbit States, Renaud Guillemin, Stephane Carniato, Wayne C. Stolte, Loic Journel, Richard Taieb, Dennis W. Lindle, Marc Simon Sep 2008

Linear Dichroism In Resonant Inelastic X-Ray Scattering To Molecular Spin-Orbit States, Renaud Guillemin, Stephane Carniato, Wayne C. Stolte, Loic Journel, Richard Taieb, Dennis W. Lindle, Marc Simon

Chemistry and Biochemistry Faculty Research

Polarization-dependent resonant inelastic x-ray scattering (RIXS) is shown to be a new probe of molecular-field effects on the electronic structure of isolated molecules. A combined experimental and theoretical analysis explains the linear dichroism observed in Cl 2p RIXS following Cl 1s excitation in HCl and CF3Cl as due to molecular-field effects, including singlet-triplet exchange, indicating polarized-RIXS provides a direct probe of spin-orbit-state populations applicable to any molecule.


Photoelectron Spectroscopic And Theoretical Studies Of Fem − (Coronene)N (M=1,2, N=1,2) Complexes, Xiang Li, Soren Eustis, Kit H. Bowen, Anil K. Kandalam, Puru Jena Aug 2008

Photoelectron Spectroscopic And Theoretical Studies Of Fem − (Coronene)N (M=1,2, N=1,2) Complexes, Xiang Li, Soren Eustis, Kit H. Bowen, Anil K. Kandalam, Puru Jena

Physics & Engineering Faculty Publications

No abstract provided.


Surface Ion-Electron Recombination As The Main Source Of Atoms In Flowing N2 Dbd, D. Tsyganov, Et. Es-Sebbar, S. Pancheshnyi, N. Gherardi, P. Ségur, F. Massines Jul 2008

Surface Ion-Electron Recombination As The Main Source Of Atoms In Flowing N2 Dbd, D. Tsyganov, Et. Es-Sebbar, S. Pancheshnyi, N. Gherardi, P. Ségur, F. Massines

Dr. Et-touhami Es-sebbar

No abstract provided.


Talif Quantification Of Nitrogen Atoms Applied To Experimental Simulation Of Titan’S Atmosphere, Et. Es-Sebbar, Y. Benilan, E. Arzoumanian, M.-C. Gazeau Jul 2008

Talif Quantification Of Nitrogen Atoms Applied To Experimental Simulation Of Titan’S Atmosphere, Et. Es-Sebbar, Y. Benilan, E. Arzoumanian, M.-C. Gazeau

Dr. Et-touhami Es-sebbar

No abstract provided.


S.E.T.U.P., A New Program Of Representative Simulations Of Titan’S Atmosphere: Current Status, M-C. Gazeau, E. Arzoumanian, Y. Benilan, Et. Es-Sebbar, A. Jolly, S. Perrier, C. Romanzin Jul 2008

S.E.T.U.P., A New Program Of Representative Simulations Of Titan’S Atmosphere: Current Status, M-C. Gazeau, E. Arzoumanian, Y. Benilan, Et. Es-Sebbar, A. Jolly, S. Perrier, C. Romanzin

Dr. Et-touhami Es-sebbar

No abstract provided.


Investigation Of (E, 2e) Collisions And Related Phenomena, Jason Manuel Martinez Jul 2008

Investigation Of (E, 2e) Collisions And Related Phenomena, Jason Manuel Martinez

Physics Theses & Dissertations

In this thesis I investigate (e, 2e) processes, or electron impact ionization, using several theoretical methods. I first examine the problem using the Born approximations, particularly the Distorted Wave Born Approximation (DWBA), focusing on the underlying processes that dominate for ionization of the 2p state of Argon and Magnesium. I investigate as well the ionization of helium and hydrogen and use the simplicity of the approximation to probe the incident particle effects on the Helium cross section. In both cases the results are compared with experiment. I also produce cross section results for ions near threshold, a regime that …


The Study Of Optogalvanic Effect Associated With The 1s States Of Neon, Naveed Piracha, K. Nesbett, S. Marotta Jun 2008

The Study Of Optogalvanic Effect Associated With The 1s States Of Neon, Naveed Piracha, K. Nesbett, S. Marotta

Naveed K. Piracha

We report on the temporal evolution of the optogalvanic signals in neon using a commercial hollow cathode lamp in conjunction with a Nd:YAG pumped dye laser system. We have recorded transitions excited from each of the neon 1s states over a range of discharge current to investigate the dominant physical processes responsible for the optogalvanic effect in neon discharges. The decay rates associated with the four 1s levels have been obtained using a mathematical rate equation model. A linear relationship between the decay rates and the discharge current has been found and the effective lifetimes and the electron collisional rate …


Oxidation Resistance Studies Of Crain Coatings On 430 Stainless Steel, Kurtis Wickey Jun 2008

Oxidation Resistance Studies Of Crain Coatings On 430 Stainless Steel, Kurtis Wickey

Honors Theses

The requirements of low cost and high-cost temperature corrosion resistance for interconnect plates in solid oxide fuel cell stacks has directed attention to the use of metal plates with oxidation resistant coatings. We have investigated the performance of stainless steel plates with homogenous coatings of CrAIN. The coatings were deposited using RF magnetron sputtering, with Ar as a sputtering gas and N as reactive gas. The Cr/A1 composition ratio in the coatings was varied in a combinatorial approach. The coatings were subsequently annealed in air for up to 25 hours at 800°C. The composition of the coated plates and the …


Comparison Of Townsend Dielectric Barrier Discharge In N2, N2/O2 And N2/N2o: Behavior And Density Of Radicals, F. Massines, Et. Es-Sebbar, N. Gherardi, N. Naudé, D. Tsyganov, P. Ségur, S. Pancheshnyi Jun 2008

Comparison Of Townsend Dielectric Barrier Discharge In N2, N2/O2 And N2/N2o: Behavior And Density Of Radicals, F. Massines, Et. Es-Sebbar, N. Gherardi, N. Naudé, D. Tsyganov, P. Ségur, S. Pancheshnyi

Dr. Et-touhami Es-sebbar

No abstract provided.


Higgs Production Via B Bbar -> H In Hadron Colliders, Nikolaos Kidonakis May 2008

Higgs Production Via B Bbar -> H In Hadron Colliders, Nikolaos Kidonakis

Faculty and Research Publications

I present NNNLO collinear and soft gluon corrections for Higgs production via the process b bbar -> H. I show that the collinear corrections dominate and contribute large enhancements to the cross section at both the Tevatron and the LHC.


Simulation And Analysis Of Ultrafast-Laser-Pulse-Induced Plasma Generation In Fused Silica, Jeremy Gulley, Sebastian Winkler, W. M. Dennis May 2008

Simulation And Analysis Of Ultrafast-Laser-Pulse-Induced Plasma Generation In Fused Silica, Jeremy Gulley, Sebastian Winkler, W. M. Dennis

Jeremy R. Gulley

Recent experiments on optical damage by ultrashort laser pulses have demonstrated that the temporal pulse shape can dramatically influence plasma generation in fused silica. We use a modified 3+1D nonlinear Schrödinger equation for the pulse propagation coupled to a rate equation for the plasma density in the dielectric material to simulate pulse propagation and plasma formation in fused silica. We use these simulations to analyze the influence of pulse shape and beam geometry on the formation of the electron plasma and hence modification in the bulk material. In particular, we simulate the effect of pulses reconstructed from experimental data. It …


Status Of Eikonal Two-Loop Calculations With Massive Quarks, Nikolaos Kidonakis, Philip Stephens May 2008

Status Of Eikonal Two-Loop Calculations With Massive Quarks, Nikolaos Kidonakis, Philip Stephens

Faculty and Research Publications

We present results for two-loop diagrams with massive quarks in the eikonal approximation. Explicit expressions are given for the UV poles in dimensional regularization of several of the required integrals.


Dielectric Relaxation Behaviour Of Glycine In Acqueous Solution Medium In The Microwave Frequency Region, Ajaya Kumar Kavala Apr 2008

Dielectric Relaxation Behaviour Of Glycine In Acqueous Solution Medium In The Microwave Frequency Region, Ajaya Kumar Kavala

Mr Ajaya Kumar Kavala

No abstract provided.


Real-Time Plasma Controlled Chemistry In A Two-Frequency, Confined Plasma Etcher, Vladimir Milosavljevic, Albert R. Ellingboe, Cezar Gaman, John V. Ringwood Apr 2008

Real-Time Plasma Controlled Chemistry In A Two-Frequency, Confined Plasma Etcher, Vladimir Milosavljevic, Albert R. Ellingboe, Cezar Gaman, John V. Ringwood

Articles

The physics issues of developing model-based control of plasma etching are presented. A novel methodology for incorporating real-time model-based control of plasma processing systems is developed. The methodology is developed for control of two dependent variables (ion flux and chemical densities) by two independent controls (27 MHz power and O2flow). A phenomenological physics model of the nonlinear coupling between the independent controls and the dependent variables of the plasma is presented. By using a design of experiment, the functional dependencies of the response surface are determined. In conjunction with the physical model, the dependencies are used to deconvolve the sensor …


Investigation Of Loading Of Pulsed And Continuous-Wave Optical Dipole Force Traps, M. Shiddiq, E. M. Ahmed, M. D. Havey, C. I. Sukenik Apr 2008

Investigation Of Loading Of Pulsed And Continuous-Wave Optical Dipole Force Traps, M. Shiddiq, E. M. Ahmed, M. D. Havey, C. I. Sukenik

Physics Faculty Publications

We have investigated the behavior of an optical dipole force trap realized using a mode-locked Nd:YAG laser and have compared performance to a continuous-wave (cw) trap built using the same laser but running in a cw mode. The traps are used to confine ultracold 85Rb atoms which are loaded from a magneto-optical trap (MOT). In most respects, the two traps behave similarly over a wide range of laser parameters provided that the average potential well depth is the same; however, there is a notable difference in the dipole trap loading efficiency dependence on the detuning of the MOT trap laser …


Extended Tuning Of An Injection-Locked Diode Laser, M. K. Shaffer, G. Ranjit, C. I. Sukenik Apr 2008

Extended Tuning Of An Injection-Locked Diode Laser, M. K. Shaffer, G. Ranjit, C. I. Sukenik

Physics Faculty Publications

We have investigated the application of an electronic feedback technique recently reported by Repasky, et.al. [Appl. Opt. 45, 9013 (2006)] to an injection-locked semiconductor diode laser. We find that without electronic feedback, the injection-locked slave laser will only follow the master for less than 1 GHz, but once the electronic feedback is applied, the slave laser is capable of following for more than 20 GHz, corresponding to the full scan range of the master laser.


Photoassociative Spectroscopy Of Ultracold Metastable Argon And Study Of Dual Species Trap Loss In A Rubidium-Metastable Argon Mot, Michael K. Shaffer Apr 2008

Photoassociative Spectroscopy Of Ultracold Metastable Argon And Study Of Dual Species Trap Loss In A Rubidium-Metastable Argon Mot, Michael K. Shaffer

Physics Theses & Dissertations

This dissertation presents the findings of two experimental investigations in ultracold atomic and molecular physics: The study of the dual species trap loss in a rubidium - metastable argon magneto-optical trap and the photoassociative spectroscopy of ultracold metastable argon. The interspecies trap loss rate coefficients have been measured for ultracold collisions between 85Rb and 40Ar* in a dual-species magneto-optical trap (MOT) and the two rates have been found to be approximately equal over the range of intensities studied with values of β'Rb–Ar* = 3.0 ± 1.3 × 10-11 cm3/s and β'Ar*–Rb = 1.9 …


Cantilever Based Optical Interfacial Force Microscope, Jeremy R. Bonander, Byung I. Kim Mar 2008

Cantilever Based Optical Interfacial Force Microscope, Jeremy R. Bonander, Byung I. Kim

Physics Faculty Publications and Presentations

We developed a cantilever based optical interfacial force microscopy (COIFM) that employs a microactuated silicon cantilever and optical detection method to establish the measurement of the single molecular interactions using the force feedback technique. Through the direct measurement of the COIFM force-distance curves, we have demonstrated that the COIFM is capable of unveiling structural and mechanical information on interfacial water at the single molecular level over all distances between two hydrophilic surfaces.


An Image Based Bidirectional Reflectivity Distribution Function Experiment, Michael T. Hagg Mar 2008

An Image Based Bidirectional Reflectivity Distribution Function Experiment, Michael T. Hagg

Theses and Dissertations

The temperature dependence of Bidirectional Reflectivity Distribution Functions (BRDFs) is not well documented. For the sake of time and customer demand, current measurements are taken at room temperature, but the reflectivity of a material changes as a function of temperature. The assumption is that this change is uniform, and as such, the BRDF will retain its relative angular shape but perhaps be scaled in magnitude as a function of temperature. When BRDFs are to be used at elevated temperatures, a scaling factor is then applied. In addition, BRDF as a function of rate of change of temperature has been identified …


Rabi Oscillations Between Ground And Rydberg States With Dipole-Dipole Atomic Interactions, Todd A. Johnson, E. Urban, T. Henage, L. Isenhower, D. D. Yavuz, T. G. Walker, M Saffman Mar 2008

Rabi Oscillations Between Ground And Rydberg States With Dipole-Dipole Atomic Interactions, Todd A. Johnson, E. Urban, T. Henage, L. Isenhower, D. D. Yavuz, T. G. Walker, M Saffman

Physics Faculty Publications

We demonstrate Rabi oscillations of small numbers of 87Rb atoms between ground and Rydberg states with n≤43. Coherent population oscillations are observed for single atoms, while the presence of two or more atoms decoheres the oscillations. We show that these observations are consistent with van der Waals interactions of Rydberg atoms.