High-Latitude Short-Period Mesospheric Gravity Wave Dynamics And Winter Climatology,
2013
Utah State University
High-Latitude Short-Period Mesospheric Gravity Wave Dynamics And Winter Climatology, Michael Negale, Kim Nielsen, Michael J. Taylor, Dominique Pautet, Margit Dyrland
Physics Student Research
Short-period gravity wave observations over the Arctic region are few and their impact on the Arctic mesosphere lower thermosphere region via momentum deposition is of high interest. The Mesospheric Airglow Imaging and Dynamics project was initiated in January 2011 to investigate the presence and dynamics of these waves over the interior of Alaska. Observations were made from Poker Flat Research Range (PFRR) using an all-sky imager. This site provides an exceptional opportunity to establish a long-term climatology of short-period gravity waves in the Arctic Region. We present summary measurements of prominent gravity waves over two consecutive winters and compare their …
Cave Ventilation Is Influenced By Variations In The Co2-Dependent Virtual Temperature,
2013
Departamento de Desertificación y Geoecología, Estación Experimental de Zonas Áridas, CSIC, Almería, Spain
Cave Ventilation Is Influenced By Variations In The Co2-Dependent Virtual Temperature, Enrique P. Sánchez-Cañete, Penélope Serrano-Ortiz, Francisco Domingo, Andrew S. Kowalski
International Journal of Speleology
Dynamics and drivers of ventilation in caves are of growing interest for different fields of science. Accumulated CO2 in caves can be exchanged with the atmosphere, modifying the internal CO2 content, affecting stalagmite growth rates, deteriorating rupestrian paintings or creating new minerals. Current estimates of cave ventilation neglect the role of high CO2 concentrations in determining air density – approximated via the virtual temperature (Tv) –, affecting buoyancy and therefore the release or storage of CO2. Here we try to improve knowledge and understanding of cave ventilation through the use of T …
Analyzing Experimental Data And Model Parameters: Implications For Predictions Of Soa Using Chemical Transport Models,
2013
Portland State University
Analyzing Experimental Data And Model Parameters: Implications For Predictions Of Soa Using Chemical Transport Models, Kelley Barsanti, Annmarie G. Carlton, Serena H. Chung
Civil and Environmental Engineering Faculty Publications and Presentations
Despite critical importance for air quality and climate predictions, accurate representation of secondary organic aerosol (SOA) formation remains elusive. An essential addition to the ongoing discussion of improving model predictions is an acknowledgement of the linkages between experimental conditions, parameter optimization and model output, as well as the linkage between empirically-derived partitioning parameters and the physicochemical properties of SOA they represent in models. In this work, a "best available" set of SOA modeling parameters is selected by comparing predicted SOA yields and mass concentrations with observed yields and mass concentrations from a comprehensive list of published smog chamber studies. Evaluated …
Ace-Fts Observations Of Pyrogenic Trace Species In Boreal Biomass Burning Plumes During Bortas,
2013
Old Dominion University
Ace-Fts Observations Of Pyrogenic Trace Species In Boreal Biomass Burning Plumes During Bortas, K. A. Tereszchuk, G. G. Abad, C. Clerbaux, J. Hadji-Lazaro, D. Hurtmans, P. F. Coheur, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
To further our understanding of the effects of biomass burning emissions on atmospheric composition, the BORTAS campaign (BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) was conducted on 12 July to 3 August 2011 during the boreal forest fire season in Canada. The simultaneous aerial, ground and satellite measurement campaign sought to record instances of boreal biomass burning to measure the tropospheric volume mixing ratios (VMRs) of short- and long-lived trace molecular species from biomass burning emissions. The goal was to investigate the connection between the composition and the distribution of these pyrogenic outflows and …
Ace-Fts Observations Of Acetonitrile In The Lower Stratosphere,
2013
Old Dominion University
Ace-Fts Observations Of Acetonitrile In The Lower Stratosphere, J. J. Harrison, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
This work reports the first infrared satellite remote-sensing measurements of acetonitrile (CH3CN) in the Earth's atmosphere using solar occultation measurements made by the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) between 2004 and 2011. The retrieval scheme uses new quantitative laboratory spectroscopic measurements of acetonitrile (Harrison and Bernath, 2012). Although individual ACE-FTS profile measurements are dominated by measurement noise, median profiles in 10 degrees latitude bins show a steady decline in volume mixing ratio from similar to 150 ppt (parts per trillion) at 11.5 km to < 40 ppt at 25.5-29.5 km. These new measurements agree well with the scant available air-and balloon-borne data in the lower stratosphere. An acetonitrile stratospheric lifetime of 73 ± 20 yr has been determined.
Hci And Cio Profiles Inside The Antarctic Vortex As Observed By Smiles In November 2009: Comparisons With Mls And Ace-Fts Instruments,
2013
Old Dominion University
Hci And Cio Profiles Inside The Antarctic Vortex As Observed By Smiles In November 2009: Comparisons With Mls And Ace-Fts Instruments, T. Sugita, Y. Kasai, Y. Terao, S. Hayashida, G. L. Manney, W. H. Daffer, H. Sagawa, M. Suzuki, M. Shiotani, K. A. Walker, C. D. Boone, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
We present vertical profiles of hydrogen chloride (HCl) and chlorine monoxide (ClO) as observed by the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) on the International Space Station (ISS) inside the Antarctic vortex on 19-24 November 2009. The SMILES HCl value reveals 2.8-3.1 ppbv between 450K and 500K levels in potential temperature (PT). The high value of HCl is highlighted since it is suggested that HCl is a main component of the total inorganic chlorine Cly, defined as Cly similar or equal to HCl + ClO + chlorine nitrate ClONO2, inside the Antarctic vortex in spring, owing …
Uncertainties In Modelling Heterogeneous Chemistry And Arctic Ozone Depletion In The Winter 2009/2010,
2013
Old Dominion University
Uncertainties In Modelling Heterogeneous Chemistry And Arctic Ozone Depletion In The Winter 2009/2010, I. Wohltmann, T. Wegner, R. Müller, R. Lehmann, M. Rex, G. L. Manney, M. L. Santee, P. Bernath, O. Suminska-Ebersoldt
Chemistry & Biochemistry Faculty Publications
Stratospheric chemistry and denitrification are simulated for the Arctic winter 2009/2010 with the Lagrangian Chemistry and Transport Model ATLAS. A number of sensitivity runs is used to explore the impact of uncertainties in chlorine activation and denitrification on the model results. In particular, the efficiency of chlorine activation on different types of liquid aerosol versus activation on nitric acid trihydrate clouds is examined. Additionally, the impact of changes in reaction rate coefficients, in the particle number density of polar stratospheric clouds, in supersaturation, temperature or the extent of denitrification is investigated. Results are compared to satellite measurements of MLS and …
Validation Of Stratospheric And Mesospheric Ozone Observed By Smiles From International Space Station,
2013
Old Dominion University
Validation Of Stratospheric And Mesospheric Ozone Observed By Smiles From International Space Station, Y. Kasai, H. Sagawa, D. Kreyling, E. Dupuy, P. Baron, J. Mendrok, K Suzuki, T. O. Sato, T. Nishibori, S. Mizobuchi, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
We observed ozone O3 in the vertical region between 250 and 0.0005 hPa (~ 12-96 km) using the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) on the Japanese Experiment Module (JEM) of the International Space Station (ISS) between 12 October 2009 and 21 April 2010. The new 4K superconducting heterodyne receiver technology of SMILES allowed us to obtain a one order of magnitude better signal-to-noise ratio for the O3 line observation compared to past spaceborne microwave instruments. The non-sun-synchronous orbit of the ISS allowed us to observe O3 at various local times. We assessed the quality of the vertical …
Hydrocarbons In The Upper Troposphere And Lower Stratosphere Observed From Ace-Fts And Comparisons With Waccm,
2013
Old Dominion University
Hydrocarbons In The Upper Troposphere And Lower Stratosphere Observed From Ace-Fts And Comparisons With Waccm, Mijeong Park, William J. Randel, Douglas E. Kinnison, Louisa K. Emmons, Peter F. Bernath, Kaley A. Walker, Chris D. Boone, Nathaniel J. Livesey
Chemistry & Biochemistry Faculty Publications
Satellite measurements from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) are used to examine the global, seasonal variations of several hydrocarbons, including carbon monoxide (CO), ethane (C2H6), acetylene (C2H2), and hydrogen cyanide (HCN). We focus on quantifying large-scale seasonal behavior from the middle troposphere to the stratosphere, particularly in the tropics, and furthermore make detailed comparisons with the Whole Atmosphere Community Climate Model (WACCM) chemistry climate model (incorporating tropospheric photochemistry, time-varying hydrocarbon emissions, and meteorological fields nudged from reanalysis). Comparisons with Microwave Limb Sounder (MLS) measurements of CO are also included …
Air-Sea Dimethylsulfide (Dms) Gas Transfer In The North Atlantic: Evidence For Limited Interfacial Gas Exchange At High Wind Speed,
2013
University of California - Irvine
Air-Sea Dimethylsulfide (Dms) Gas Transfer In The North Atlantic: Evidence For Limited Interfacial Gas Exchange At High Wind Speed, T. G. Bell, Warren J. De Bruyn, S. D. Miller, B. Ward, K. Christensen, E. S. Saltzman
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Shipboard measurements of eddy covariance dimethylsulfide (DMS) air-sea fluxes and seawater concentration were carried out in the North Atlantic bloom region in June/July 2011. Gas transfer coefficients (k(660)) show a linear dependence on mean horizontal wind speed at wind speeds up to 11 m s(-1). At higher wind speeds the relationship between k(660) and wind speed weakens. At high winds, measured DMS fluxes were lower than predicted based on the linear relationship between wind speed and interfacial stress extrapolated from low to intermediate wind speeds. In contrast, the transfer coefficient for sensible heat did not exhibit this effect. The apparent …
Modeling Visibility In The El Paso Del Norte (Pdn) Region,
2013
University of Texas at El Paso
Modeling Visibility In The El Paso Del Norte (Pdn) Region, Richard Medina Calderon
Open Access Theses & Dissertations
Poor visibility is a subject of growing public concern throughout the U.S, and an active area of research. Its societal impacts on air quality, aviation transport and traffic are significant. Aerosols play a fundamental role in the attenuation of solar radiation, and also affect visibility. The scattering and extinction coefficients of aerosol particles in the Paso del Norte Region have been calculated using the T- matrix model in conjunction with a laser particle counter. Inter-comparison of the model's results of the scattering and absorption coefficients against the corresponding data from a Photoacustic extinctiometer instrument (which measures in-situ absorption and scattering …
The Relation Between Atmospheric Humidity And Temperature Trends For Stratospheric Water,
2013
Old Dominion University
The Relation Between Atmospheric Humidity And Temperature Trends For Stratospheric Water, S. Fueglistaler, Y. S. Liu, T. J. Flannaghan, P. H. Haynes, D. P. Dee, W. J. Read, E. E. Remsberg, L. W. Thomason, D. F. Hurst, J. R. Lanzante, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
We analyze the relation between atmospheric temperature and water vapor-a fundamental component of the global climate system-for stratospheric water vapor (SWV). We compare measurements of SWV (and methane where available) over the period 1980-2011 from NOAA balloon-borne frostpoint hygrometer (NOAA-FPH), SAGE II, Halogen Occultation Experiment (HALOE), Microwave Limb Sounder (MLS)/Aura, and Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) to model predictions based on troposphere-to-stratosphere transport from ERA-Interim, and temperatures from ERA-Interim, Modern Era Retrospective- Analysis (MERRA), Climate Forecast System Reanalysis (CFSR), Radiosonde Atmospheric Temperature Products for Assessing Climate (RATPAC), HadAT2, and RICHv1.5. All model predictions are dry biased. The interannual …
Long-Term (1951-2007) Rainfall Trends Around Six Indian Cities: Current State, Meteorological, And Urban Dynamics,
2013
Dalhousie University, Canada
Long-Term (1951-2007) Rainfall Trends Around Six Indian Cities: Current State, Meteorological, And Urban Dynamics, Shailesh Kumar Kharol, D. G. Kaskaoutis, Anu Rani Sharma, Ramesh P. Singh
Mathematics, Physics, and Computer Science Faculty Articles and Research
The present study focuses on analyzing the precipitation trends over six Indian cities during the summer monsoon (June-September) covering the period 1951-2007 and also attempting to investigate possible urban forcing and dynamics by examining the variation in precipitation in the upwind and downwind directions. The analysis shows negative trends in the total number of rainy days over Hyderabad (-10.4%), Kanpur (-7.1%), Jaipur (-10.5%), and Nagpur (-4.8%) and positive trends over Delhi (7.4%) and Bangalore (22.9%). On the other hand, decreases of -21.3%, -5.9%, -14.2%, and -14.6% in seasonal rainfall are found over Delhi, Hyderabad, Jaipur, and Kanpur, respectively, whereas Bangalore …
Observations Of Peroxyacetyl Nitrate (Pan) In The Upper Troposphere By The Atmospheric Chemistry Experiment-Fourier Transform Spectrometer (Ace-Fts),
2013
Old Dominion University
Observations Of Peroxyacetyl Nitrate (Pan) In The Upper Troposphere By The Atmospheric Chemistry Experiment-Fourier Transform Spectrometer (Ace-Fts), K. A. Tereszchuk, D. P. Moore, J. J. Harrison, C. D. Boone, M. Park, J. J. Remedios, W. J. Randel, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
Peroxyacetyl nitrate (CH3CO·O2NO2, abbreviated as PAN) is a trace molecular species present in the troposphere and lower stratosphere due primarily to pollution from fuel combustion and the pyrogenic outflows from biomass burning. In the lower troposphere, PAN has a relatively short lifetime and is principally destroyed within a few hours through thermolysis, but it can act as a reservoir and carrier of NOx in the colder temperatures of the upper troposphere, where UV photolysis becomes the dominant loss mechanism. Pyroconvective updrafts from large biomass burning events can inject PAN into the upper troposphere …
Stratospheric Lifetimes Of Cfc-12, Ccl4, Ch4, Ch3cl And N20 From Measurements Made By The Atmospheric Chemistry Experiment-Fourier Transform Spectrometer,
2013
Old Dominion University
Stratospheric Lifetimes Of Cfc-12, Ccl4, Ch4, Ch3cl And N20 From Measurements Made By The Atmospheric Chemistry Experiment-Fourier Transform Spectrometer, A. T. Brown, C. M. Volk, M. R. Schoebert, C. D. Boone, P. F. Bernath
Chemistry & Biochemistry Faculty Publications
Long lived halogen-containing compounds are important atmospheric constituents since they can act both as a source of chlorine radicals, which go on to catalyse ozone loss, and as powerful greenhouse gases. The long-term impact of these species on the ozone layer is dependent on their stratospheric lifetimes. Using observations from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) we present calculations of the stratospheric lifetimes of CFC-12, CCl4, CH4, CH3Cl and N2O. The lifetimes were calculated using the slope of the tracer-tracer correlation of these species with CFC-11 at the tropopause. The …
Black Carbon Measurements Of Snow And Ice Using The Single Particle Soot Photometer: Method Development And An Ad 1852-1999 Record Of Atmospheric Black Carbon From A Mount Logan Ice Core,
2013
Central Washington University
Black Carbon Measurements Of Snow And Ice Using The Single Particle Soot Photometer: Method Development And An Ad 1852-1999 Record Of Atmospheric Black Carbon From A Mount Logan Ice Core, James Andrew Menking
All Master's Theses
Black carbon (BC), produced by the combustion of fossil and biofuels, warms the climate by absorbing solar radiation when in the atmosphere and by reducing the albedo of snow and ice when deposited. Measuring BC in snow and ice is important for estimating albedo reduction and developing historical records of BC concentration. Experiments were conducted to further develop a method for measuring BC in snow and ice using the Single Particle Soot Photometer (SP2). Results suggest the optimal procedures for sample storage, treatment, and nebulization, and analysis and calibration of BC concentrations measured using the SP2 coupled to a CETAC …
An Analysis Of Surface Air Temperature Trends And Variability Along The Andes,
2013
University at Albany, State University of New York
An Analysis Of Surface Air Temperature Trends And Variability Along The Andes, Eric Franquist
Legacy Theses & Dissertations (2009 - 2024)
Climate change is difficult to study in mountainous regions such as the Andes since steep changes in elevation cannot always be resolved by climate models. However, it is important to examine temperature trends in this region as rises in surface air temperature are leading to the melting of tropical glaciers. Local communities rely on the glacier-fed streamflow to get their water for drinking, irrigation, and livestock. Moreover, communities also rely on the tourism of hikers who come to the region to view the glaciers. As the temperatures increase, these glaciers are no longer in equilibrium with their current climate and …
Evaluating Drought In The United States Using The Emissivity Difference Vegetation Index,
2013
University at Albany, State University of New York
Evaluating Drought In The United States Using The Emissivity Difference Vegetation Index, Hanisha Hirani
Legacy Theses & Dissertations (2009 - 2024)
As monitoring vegetation and crops becomes increasingly important due to climate change, there arises the need for a monitoring scheme that places more weight on water availability as an indication of vegetation health and vitality. The Emissivity Difference Vegetation Index (EDVI) is the first step towards that type of monitoring scheme. With the potential for diurnal studies, there are applications towards agriculture monitoring, wildfire monitoring, and much more. EDVI is a synergetic product retrieved from microwave, visible, and infrared satellite measurements, as well as reanalysis. Since microwave measurements are more sensitive to vegetation water content, EDVI has the potential to …
Interactions Between African Easterly Waves And Moist Convection,
2013
University at Albany, State University of New York
Interactions Between African Easterly Waves And Moist Convection, Matthew Adam Janiga
Legacy Theses & Dissertations (2009 - 2024)
African easterly waves (AEWs) over tropical Africa and the East Atlantic influence and are themselves influenced by moist convection. Data from the Tropical Rainfall Measuring Mission (TRMM) satellite, reanalyses, and in-situ observations are used to examine both directions of this two-way interaction.
The Motion Of Mesoscale Snowbands In Northeast U.S. Winter Storms,
2013
University at Albany, State University of New York
The Motion Of Mesoscale Snowbands In Northeast U.S. Winter Storms, Jaymes Kenyon
Legacy Theses & Dissertations (2009 - 2024)
The distribution of snowfall accumulation attending winter storms is a product of both precipitation intensity and duration. Many heavy snowfall events are associated with distinct mesoscale snowbands that strongly modulate snowfall accumulation. Mesoscale snowbands are known to be favored within environments characterized by frontogenesis in the presence of weak moist symmetric or gravitational stabilities. Although the development of mesoscale snowbands often can be anticipated at 24–36-h ranges, anticipating band residence time at a fixed location remains a forecasting challenge. However, given that snowband residence time is related to characteristics of band motion, improved understanding of band motion presents an opportunity …
