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Unveiling The Operation Mechanism Of Layered Perovskite Solar Cells, Yun Lin, Yanjun Fang, Jingjing Zhao, Yuchuan Shao, Samuel J. Stuard, Masrur Morshed Nahid, Harald Ade, Qi Wang, Jeffrey E. Shield, Ninghao Zhou, Andrew M. Moran, Jinsong Huang 2019 University of Nebraska-Lincoln

Unveiling The Operation Mechanism Of Layered Perovskite Solar Cells, Yun Lin, Yanjun Fang, Jingjing Zhao, Yuchuan Shao, Samuel J. Stuard, Masrur Morshed Nahid, Harald Ade, Qi Wang, Jeffrey E. Shield, Ninghao Zhou, Andrew M. Moran, Jinsong Huang

Department of Mechanical and Materials Engineering: Faculty Publications

Layered perovskites have been shown to improve the stability of perovskite solar cells while its operation mechanism remains unclear. Here we investigate the process for the conversion of light to electrical current in high performance layered perovskite solar cells by examining its real morphology. The layered perovskite films in this study are found to be a mixture of layered and three dimensional (3D)-like phases with phase separations at micrometer and nanometer scale in both vertical and lateral directions. This phase separation is explained by the surface initiated crystallization process and the competition of the crystallization between 3D-like and layered perovskites. …


Monolithic Heat-Transfer Device, Sidy Ndao, George Gogos, Dennis Alexander, Troy Anderson, Craig Zuhlke 2019 Lincoln, NE

Monolithic Heat-Transfer Device, Sidy Ndao, George Gogos, Dennis Alexander, Troy Anderson, Craig Zuhlke

Department of Mechanical and Materials Engineering: Faculty Publications

A monolithic heat-transfer device can include a container wall configured to retain a working fluid, where the container wall is formed of a single material. The container wall also includes an interior surface configured to be in fluid communication with the working fluid. The monolithic heat-transfer device also includes a channel disposed in the interior surface of the container wall, where the channel comprises a microstructure and a nanostructure. The microstructure and the nanostructure are materially contiguous with the single material forming the container wall. In some embodiments, the nanostructure comprises one or more layers of nanoparticles. The monolithic heat-transfer …


Higher-Order Overtone Thickness-Shear Vibrations Of Multilayered Thin-Film Acoustic Wave Resonators And Angular Rate Sensing, Hui Chen, Ji Wang, Jianke Du, Jiashi Yang 2019 Ningbo University

Higher-Order Overtone Thickness-Shear Vibrations Of Multilayered Thin-Film Acoustic Wave Resonators And Angular Rate Sensing, Hui Chen, Ji Wang, Jianke Du, Jiashi Yang

Department of Mechanical and Materials Engineering: Faculty Publications

We propose a new structure for piezoelectric gyroscopes. It is made from multilayered thin films of AlN or ZnO with alternating c-axes along the film thickness. It is shown theoretically that when such a film is electrically driven into higher-order overtone thickness-shear vibration in one of the two in-plane directions of the film and is rotating about the film normal, the Coriolis force due to the rotation causes a higher-order overtone thicknessshear vibration in a perpendicular direction with an electrical output that can be used to measure the angular rate of the rotation. Different from existing thickness-shear mode piezoelectric gyroscopes …


3d Printing Of Hybrid Mos2-Graphene Aerogels As Highly Porous Electrode Materials For Sodium Ion Battery Anodes, Emery Brown, Pengli Yan, Halil Tekik, Ayyappan Elangovan, Jian Wang, Dong Lin, Jun Li 2019 Kansas State University

3d Printing Of Hybrid Mos2-Graphene Aerogels As Highly Porous Electrode Materials For Sodium Ion Battery Anodes, Emery Brown, Pengli Yan, Halil Tekik, Ayyappan Elangovan, Jian Wang, Dong Lin, Jun Li

Department of Mechanical and Materials Engineering: Faculty Publications

This study reports a 3D freeze-printing method that integrates inkjet printing and freeze casting to control both the microstructure and macroporosity via formation of ice microcrystals during printing. A viscous aqueous ink consisting of a molecular MoS2 precursor (ammonium thiomolybdate) mixed with graphene oxide (GO) nanosheets is used in the printing process. Post-treatments by freeze-drying and reductive thermal annealing convert the printed intermediate mixture into a hybrid structure consisting of MoS2 nanoparticles anchored on the surface of 2D rGO nanosheets in a macroporous framework, which is fully characterized with FESEM, TEM, XRD, Raman spectroscopy and TGA. The resulting …


Three-Dimensional Character Of The Deformation Twin In Magnesium, Y. Liu, P.Z. Tang, M.Y. Gong, R.J. McCabe, J. Wang, C.N. Tome 2019 Shanghai Jiao Tong University & Los Alamos National Laboratory

Three-Dimensional Character Of The Deformation Twin In Magnesium, Y. Liu, P.Z. Tang, M.Y. Gong, R.J. Mccabe, J. Wang, C.N. Tome

Department of Mechanical and Materials Engineering: Faculty Publications

Deformation twins are three-dimensional domains, traditionally viewed as ellipsoids because of their two-dimensional lenticular sections. In this work, we performed statistical analysis of twin shapes viewing along three orthogonal directions: the ‘dark side’ (DS) view along the twin shear direction (η1), the twinning plane normal (TPN) view (k1) and the ‘bright side’ (BS) view along the direction λ(=k1 × η1). Our electron back-scatter diffraction results show that twins in the DS and BS views normally exhibit a lenticular shape, whereas they show an irregular shape in the TPN view. Moreover, the findings in the TPN view revealed that twins grow …


Spatiotemporal Characterizations Of Spontaneously Beating Cardiomyocytes With Adaptive Reference Digital Image Correlation, Akankshya Shradhanjali, Brandon D. Riehl, Bin Duan, Ruiguo Yang, Jung Yul Lim 2019 University of Nebraska-Lincoln

Spatiotemporal Characterizations Of Spontaneously Beating Cardiomyocytes With Adaptive Reference Digital Image Correlation, Akankshya Shradhanjali, Brandon D. Riehl, Bin Duan, Ruiguo Yang, Jung Yul Lim

Department of Mechanical and Materials Engineering: Faculty Publications

We developed an Adaptive Reference-Digital Image Correlation (AR-DIC) method that enables unbiased and accurate mechanics measurements of moving biological tissue samples. We applied the AR-DIC analysis to a spontaneously beating cardiomyocyte (CM) tissue, and could provide correct quantifications of tissue displacement and strain for the beating CMs utilizing physiologically-relevant, sarcomere displacement length-based contraction criteria. The data were further synthesized into novel spatiotemporal parameters of CM contraction to account for the CM beating homogeneity, synchronicity, and propagation as holistic measures of functional myocardial tissue development. Our AR-DIC analyses may thus provide advanced non-invasive characterization tools for assessing the development of spontaneously …


Insulating Tunneling Contact For Efficient And Stable Perovskite Solar Cells, Jinsong Huang, Xiaopeng Zheng, Qi Wang, Yang Bai, Qingfeng Dong 2019 Lincoln, NE

Insulating Tunneling Contact For Efficient And Stable Perovskite Solar Cells, Jinsong Huang, Xiaopeng Zheng, Qi Wang, Yang Bai, Qingfeng Dong

Department of Mechanical and Materials Engineering: Faculty Publications

Perovskite-based photoactive devices, such as solar cells, include an insulating tunneling layer inserted between the perovskite photoactive material and the electron collection layer to reduce charge recombination and concomitantly provide water resistant properties to the device.


Beyond The Toolpath: Site-Specific Melt Pool Size Control Enables Printing Of Extra-Toolpath Geometry In Laser Wire-Based Directed Energy Deposition, Brian T. Gibson, Bradley S. Richardson, Tayler W. Undermann, Lonnie J. Love 2019 Oak Ridge National Laboratory

Beyond The Toolpath: Site-Specific Melt Pool Size Control Enables Printing Of Extra-Toolpath Geometry In Laser Wire-Based Directed Energy Deposition, Brian T. Gibson, Bradley S. Richardson, Tayler W. Undermann, Lonnie J. Love

Department of Mechanical and Materials Engineering: Faculty Publications

A variety of techniques have been utilized in metal additive manufacturing (AM) for melt pool size management, including modeling and feed-forward approaches. In a few cases, closed-loop control has been demonstrated. In this research, closed-loop melt pool size control for large-scale, laser wire-based directed energy deposition is demonstrated with a novel modification, i.e., site-specific changes to the controller setpoint were commanded at trigger points, the locations of which were generated by the projection of a secondary geometry onto the primary three-dimensional (3D) printed component geometry. The present work shows that, through this technique, it is possible to print a specific …


Disposable Fluidic Self-Propelling Robot For Traversing A Tubular Passage, Carl Nelson, Benjamin Terry, Abolfazl Pourghodrat, Hossein Dehghani, Dmitry Oleynikov, Prithviraj Dasgupta 2019 Lincoln, Ne

Disposable Fluidic Self-Propelling Robot For Traversing A Tubular Passage, Carl Nelson, Benjamin Terry, Abolfazl Pourghodrat, Hossein Dehghani, Dmitry Oleynikov, Prithviraj Dasgupta

Department of Mechanical and Materials Engineering: Faculty Publications

A probe for traversing a tubular passage includes an introducer to be supported at an entrance to the tubular passage. The probe also includes a probe tip to traverse the tubular passage, and a tube with an inflatable tube segment. In some embodiments, the inflatable tube segment is storable in the probe tip. The inflatable tube segment is configured to be inflated to push the probe tip away from the introducer toward an end on the tubular passage. In some embodiments, the probe includes a sealing mechanism, whre the sealing mechanism can be positioned between the inflatable tube segment of …


Mechanical Stresses Associated With Flattening Of Human Femoropopliteal Artery Specimens During Planar Biaxial Testing And Their Effects On The Calculated Physiologic Stress-Stretch State, Majid Jadidi, Anastasia Desyatova, Jason N. MacTaggart, Alexey Kamenskiy 2019 University of Nebraska-Lincoln

Mechanical Stresses Associated With Flattening Of Human Femoropopliteal Artery Specimens During Planar Biaxial Testing And Their Effects On The Calculated Physiologic Stress-Stretch State, Majid Jadidi, Anastasia Desyatova, Jason N. Mactaggart, Alexey Kamenskiy

Department of Mechanical and Materials Engineering: Faculty Publications

Planar biaxial testing is commonly used to characterize the mechanical properties of arteries, but stresses associated with specimen flattening during this test are unknown. We quantified flattening effects in human femoropopliteal arteries (FPAs) of different ages, and determined how they affect the calculated arterial physiologic stress-stretch state. Human FPAs from 472 tissue donors (age 12-82 years, mean 53±16 years) were tested using planar biaxial extension, and morphometric and mechanical characteristics were used to assess the flattening effects. Constitutive parameters for the invariant-based model were adjusted to account for specimen flattening, and used to calculate the physiologic stresses, stretches, axial force, …


Correlation Microanalysis Of Localized Molecular Structure And Nano-Mechanical Property Of Pvdf Based Copolymer, Wen Qian, Shuo Sun, Charles Nguyen, Stephen Ducharme, Joesph A. Turner 2019 University of Nebraska-Lincoln

Correlation Microanalysis Of Localized Molecular Structure And Nano-Mechanical Property Of Pvdf Based Copolymer, Wen Qian, Shuo Sun, Charles Nguyen, Stephen Ducharme, Joesph A. Turner

Department of Mechanical and Materials Engineering: Faculty Publications

Poly (vinylidenefluoride) (PVDF) and its copolymers, are well-recognized electroactive polymers. The PVDF polymer can crystallize in a quasi-hexagonal close-packed “β-phase” structure with the dipoles of all chains aligned with maximum spontaneous polarization [1-3]. Due to the limited availability of quantitative methods for nanoscale molecular structure and mechanical analysis, the polymer organization has not been fully optimized. For such ferroelectric polymers, the influence of nanoscale molecular structure on mechanical response is not well understood. In this paper, we demonstrate nanoscale characterization and measurement techniques, by comprehensive integrating atomic force microscopy (AFM), X-ray diffraction (XRD), nano-infrared (nanoIR) spectroscopy, nanoindentation, chemical nanoIR mapping, …


Mechanical Characterizations Of 3d-Printed Plla/Steel Particle Composites, Hozhabr Mozafari, Pengfei Dong, Haitham Hadidi, Michael P. Sealy, Linxia Gu 2019 University of Nebraska-Lincoln

Mechanical Characterizations Of 3d-Printed Plla/Steel Particle Composites, Hozhabr Mozafari, Pengfei Dong, Haitham Hadidi, Michael P. Sealy, Linxia Gu

Department of Mechanical and Materials Engineering: Faculty Publications

The objective of this study is to characterize the micromechanical properties of poly-L-lactic acid (PLLA) composites reinforced by grade 420 stainless steel (SS) particles with a specific focus on the interphase properties. The specimens were manufactured using 3D printing techniques due to its many benefits, including high accuracy, cost effectiveness and customized geometry. The adopted fused filament fabrication resulted in a thin interphase layer with an average thickness of 3 μm. The mechanical properties of each phase, as well as the interphase, were characterized by nanoindentation tests. The effect of matrix degradation, i.e., imperfect bonding, on the elastic modulus of …


Hemodynamic Interference Of Serial Stenoses And Its Impact On Ffr And Ifr Measurements, Siyeong Ju, Linxia Gu 2019 University of Nebraska-Lincoln

Hemodynamic Interference Of Serial Stenoses And Its Impact On Ffr And Ifr Measurements, Siyeong Ju, Linxia Gu

Department of Mechanical and Materials Engineering: Faculty Publications

The hemodynamic interference of serial stenoses poses challenges for identifying the functional severity using the fractional flow reserve (FFR) method. The instantaneous wave-free ratio (iFR), i.e., the distal-to-proximal pressure ratio at 75% of diastole, was recently proposed to overcome the disadvantages of the FFR. However, the underlying mechanism remained ambiguous due to the lack of quantitative definition of hemodynamic interference. The objective of this study is to quantitatively define the hemodynamic interference and then examine its role on the FFR and iFR measurements. Pressure distributions, velocity fields, and Q-criterion which identifies vortices, were obtained through the computational fluid dynamics (CFD) …


Hemodynamics And Wall Mechanics After Surgical Repair Of Aortic Arch: Implication For Better Clinical Decisions, Siyeong Ju, Ibrahim Abdullah, Shengmao Lin, Linxia Gu 2019 University of Nebraska-Lincoln

Hemodynamics And Wall Mechanics After Surgical Repair Of Aortic Arch: Implication For Better Clinical Decisions, Siyeong Ju, Ibrahim Abdullah, Shengmao Lin, Linxia Gu

Department of Mechanical and Materials Engineering: Faculty Publications

Graft repair of aortic coarctation is commonly used to mimic the physiological aortic arch shape and function. Various graft materials and shapes have been adopted for the surgery. The goal of this work is to quantitatively assess the impact of graft materials and shapes in the hemodynamics and wall mechanics of the restored aortic arch and its correlation with clinical outcomes. A three-dimensional aortic arch model was reconstructed from magnetic resonance images. The fluid–structure interaction (FSI) analysis was performed to characterize the hemodynamics and solid wall mechanics of the repaired aortic arch. Two graft shapes (i.e., a half-moon shape and …


Interface Facilitated Reorientation Of Mg Nanolayers In Mg-Nb Nanolaminates, Y. CHen, Mingyu Gong, N. A. Mara, Jian Wang 2019 University of Minnesota, Minneapolis

Interface Facilitated Reorientation Of Mg Nanolayers In Mg-Nb Nanolaminates, Y. Chen, Mingyu Gong, N. A. Mara, Jian Wang

Department of Mechanical and Materials Engineering: Faculty Publications

Mg/Nb nanolaminates synthesized through vapor deposition techniques exhibit high flow strength without conventional twinning in Mg. In this work, we investigated the influence of laminated microstructures on deformation mechanisms of Mg nanolayers. Using molecular dynamics simulations, we explored that (0001)-oriented Mg layers transform or re-orient to {10¯10}-oriented Mg layers through nucleation and growth of {10¯12} twins by atomic shuffling, instead of conventional {10¯12} twinning shear. Such a reorientation accommodates in-plane compressive strain and out-of-plane tensile strain when Mg/Nb laminates are subjected to compression parallel to the Mg/Nb interfaces. The nucleation of {10¯12} twins is promoted at the Mg/Nb interface due …


Predictive Peridynamic 3d Models Of Pitting Corrosion In Stainless Steel With Formation Of Lacy Covers, Siavash Jafarzadeh, Florin Bobaru, Ziguang Chen 2019 University of Nebraska-Lincoln

Predictive Peridynamic 3d Models Of Pitting Corrosion In Stainless Steel With Formation Of Lacy Covers, Siavash Jafarzadeh, Florin Bobaru, Ziguang Chen

Department of Mechanical and Materials Engineering: Faculty Publications

In this work, the peridynamic corrosion model is used for 3D simulation of pitting corrosion in stainless steel. Models for passivation and salt layer formation are employed to predict detailed characteristics of pit growth kinetic in stainless steels, such as lacy cover formation on top of the pit, and the diffusion-controlled regime at the pit bottom. The model is validated against an experimentally grown pit on 316L stainless steel in NaCl solution. Lacy covers in this model are formed autonomously during the simulation process. They are remarkably similar to the covers observed on top of the real pits.


Predictive Peridynamic 3d Models Of Pitting Corrosion In Stainless Steel With Formation Of Lacy Covers, Siavash Jafarzadeh, Florin Bobaru, Ziguang Chen 2019 University of Nebraska-Lincoln

Predictive Peridynamic 3d Models Of Pitting Corrosion In Stainless Steel With Formation Of Lacy Covers, Siavash Jafarzadeh, Florin Bobaru, Ziguang Chen

Department of Mechanical and Materials Engineering: Faculty Publications

In this work, the peridynamic corrosion model is used for 3D simulation of pitting corrosion in stainless steel. Models for passivation and salt layer formation are employed to predict detailed characteristics of pit growth kinetic in stainless steels, such as lacy cover formation on top of the pit, and the diffusion-controlled regime at the pit bottom. The model is validated against an experimentally grown pit on 316L stainless steel in NaCl solution. Lacy covers in this model are formed autonomously during the simulation process. They are remarkably similar to the covers observed on top of the real pits.


Reliability Estimation Of Reciprocating Seals Based On Multivariate Dependence Analysis And It's Experimental Validation, Chao Zhang, Rentong Chen, Shaoping Wang, Yujie Qian, Mileta M. Tomovic 2019 Old Dominion University

Reliability Estimation Of Reciprocating Seals Based On Multivariate Dependence Analysis And It's Experimental Validation, Chao Zhang, Rentong Chen, Shaoping Wang, Yujie Qian, Mileta M. Tomovic

Engineering Technology Faculty Publications

Accurate reliability estimation for reciprocating seals is of great significance due to their wide use in numerous engineering applications. This work proposes a reliability estimation method for reciprocating seals based on multivariate dependence analysis of different performance indicators. Degradation behavior corresponding to each performance indicator is first described by the Wiener process. Dependence among different performance indicators is then captured using D-vine copula, and a weight-based copula selection method is utilized to determine the optimal bivariate copula for each dependence relationship. A two-stage Bayesian method is used to estimate the parameters in the proposed model. Finally, a reciprocating seal degradation …


Deformation Correlations And Machine Learning: Microstructural Inference And Crystal Plasticity Predictions, Michail Tzimas 2019 West Virginia University

Deformation Correlations And Machine Learning: Microstructural Inference And Crystal Plasticity Predictions, Michail Tzimas

Graduate Theses, Dissertations, and Problem Reports (ETD)

The present thesis makes a connection between spatially resolved strain correlations and material processing history. Such correlations can be used to infer and classify prior deformation history of a sample at various strain levels with the use of Machine Learning approaches. A simple and concrete example of uniaxially compressed crystalline thin films of various sizes, generated by two-dimensional discrete dislocation plasticity simulations is examined. At the nanoscale, thin films exhibit yield-strength size effects with noisy mechanical responses which create an interesting challenge for the application of Machine Learning techniques. Moreover, this thesis demonstrates the prediction of the average mechanical responses …


Mechanical Properties And Degradation Of High Capacity Battery Electrodes: Fundamental Understanding And Coping Strategies, Yikai Wang 2019 University of Kentucky

Mechanical Properties And Degradation Of High Capacity Battery Electrodes: Fundamental Understanding And Coping Strategies, Yikai Wang

Theses and Dissertations--Chemical and Materials Engineering

Rechargeable lithium ion and lithium (Li) metal batteries with high energy density and stability are in high demand for the development of electric vehicles and smart grids. Intensive efforts have been devoted to developing high capacity battery electrodes. However, the known high capacity electrode materials experience fast capacity fading and have limited cycle life due to electromechanical degradations, such as fracture of Si-based electrodes and dendrite growth in Li metal electrodes. A fundamental understanding of electromechanical degradation mechanisms of high capacity electrodes will provide insights into strategies for improving their electrochemical performance. Thus, this dissertation focuses on mechanical properties, microstructure …


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