Atmospheric Sciences Commons^™

An Analysis Of Surface Air Temperature Trends And Variability Along The Andes, Eric Franquist

Legacy Theses & Dissertations (2009 - 2024)

Climate change is difficult to study in mountainous regions such as the Andes since steep changes in elevation cannot always be resolved by climate models. However, it is important to examine temperature trends in this region as rises in surface air temperature are leading to the melting of tropical glaciers. Local communities rely on the glacier-fed streamflow to get their water for drinking, irrigation, and livestock. Moreover, communities also rely on the tourism of hikers who come to the region to view the glaciers. As the temperatures increase, these glaciers are no longer in equilibrium with their current climate and …

The Motion Of Mesoscale Snowbands In Northeast U.S. Winter Storms, Jaymes Kenyon

Legacy Theses & Dissertations (2009 - 2024)

The distribution of snowfall accumulation attending winter storms is a product of both precipitation intensity and duration. Many heavy snowfall events are associated with distinct mesoscale snowbands that strongly modulate snowfall accumulation. Mesoscale snowbands are known to be favored within environments characterized by frontogenesis in the presence of weak moist symmetric or gravitational stabilities. Although the development of mesoscale snowbands often can be anticipated at 24–36-h ranges, anticipating band residence time at a fixed location remains a forecasting challenge. However, given that snowband residence time is related to characteristics of band motion, improved understanding of band motion presents an opportunity …

Solar Radiation Measurements And Their Applications In Climate Research, Bangsheng Yin

Legacy Theses & Dissertations (2009 - 2024)

Aerosols and clouds play important roles in the climate system through their radiative effects and their vital link in the hydrological cycle. Accurate measurements of aerosol and cloud optical and microphysical properties are crucial for the study of climate and climate change. This study develops/improves retrieval algorithms for aerosol single scattering albedo (SSA) and low liquid water path (LWP) cloud optical properties, evaluates a new spectrometer, and applies long-term measurements to establish climatology of aerosol and cloud optical properties. The following results were obtained.

Interactions Between African Easterly Waves And Moist Convection, Matthew Adam Janiga

Legacy Theses & Dissertations (2009 - 2024)

African easterly waves (AEWs) over tropical Africa and the East Atlantic influence and are themselves influenced by moist convection. Data from the Tropical Rainfall Measuring Mission (TRMM) satellite, reanalyses, and in-situ observations are used to examine both directions of this two-way interaction.

Study Of Key Factors Influencing Dust Emission : An Assessment Of Geos-Chem And Dead Simulations With Observations, Kevin Scott Bartlett

Legacy Theses & Dissertations (2009 - 2024)

Mineral dust aerosols can impact air quality, climate change, biological cycles, tropical cyclone development and flight operations due to reduced visibility. Dust emissions are primarily limited to the extensive arid regions of the world, yet can negatively impact local to global scales, and are extremely complex to model accurately. Within this dissertation, the Dust Entrainment And Deposition (DEAD) model was adapted to run, for the first known time, using high temporal (hourly) and spatial (0.3°x0.3°) resolution data to methodically interrogate the key parameters and factors influencing global dust emissions. The dependence of dust emissions on key parameters under various conditions …

Evaluating Drought In The United States Using The Emissivity Difference Vegetation Index, Hanisha Hirani

Legacy Theses & Dissertations (2009 - 2024)

As monitoring vegetation and crops becomes increasingly important due to climate change, there arises the need for a monitoring scheme that places more weight on water availability as an indication of vegetation health and vitality. The Emissivity Difference Vegetation Index (EDVI) is the first step towards that type of monitoring scheme. With the potential for diurnal studies, there are applications towards agriculture monitoring, wildfire monitoring, and much more. EDVI is a synergetic product retrieved from microwave, visible, and infrared satellite measurements, as well as reanalysis. Since microwave measurements are more sensitive to vegetation water content, EDVI has the potential to …

Air-Sea Dimethylsulfide (Dms) Gas Transfer In The North Atlantic: Evidence For Limited Interfacial Gas Exchange At High Wind Speed, T. G. Bell, Warren J. De Bruyn, S. D. Miller, B. Ward, K. Christensen, E. S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Shipboard measurements of eddy covariance dimethylsulfide (DMS) air-sea fluxes and seawater concentration were carried out in the North Atlantic bloom region in June/July 2011. Gas transfer coefficients (k(660)) show a linear dependence on mean horizontal wind speed at wind speeds up to 11 m s(-1). At higher wind speeds the relationship between k(660) and wind speed weakens. At high winds, measured DMS fluxes were lower than predicted based on the linear relationship between wind speed and interfacial stress extrapolated from low to intermediate wind speeds. In contrast, the transfer coefficient for sensible heat did not exhibit this effect. The apparent …

Multi-Instrument Comparisons Of D-Region Plasma Measurements, M. Friedrich, K. M. Torkar, U. P. Hoppe, T. A. Bekkeng, A. Barjatya, M. Rapp

Publications

The ECOMA (Existence and Charge state Of Meteoric dust grains in the middle Atmosphere) series of sounding rocket flights consisted of nine flights with almost identical payload design and flight characteristics. All flights carried a radio wave propagation experiment together with a variety of plasma probes. Three of these measured electron densities, two ion densities. The rockets were all launched from the Andøya Rocket Range, Norway, in four campaigns between 2006 and 2010. Emphasis is on the final three flights from 2010 where the payloads were equipped with four instruments capable of measuring plasma densities in situ, among them a …

Black Carbon Measurements Of Snow And Ice Using The Single Particle Soot Photometer: Method Development And An Ad 1852-1999 Record Of Atmospheric Black Carbon From A Mount Logan Ice Core, James Andrew Menking

All Master's Theses

Black carbon (BC), produced by the combustion of fossil and biofuels, warms the climate by absorbing solar radiation when in the atmosphere and by reducing the albedo of snow and ice when deposited. Measuring BC in snow and ice is important for estimating albedo reduction and developing historical records of BC concentration. Experiments were conducted to further develop a method for measuring BC in snow and ice using the Single Particle Soot Photometer (SP2). Results suggest the optimal procedures for sample storage, treatment, and nebulization, and analysis and calibration of BC concentrations measured using the SP2 coupled to a CETAC …

Carbon Farming In Wa, Department Of Agriculture And Food, Western Australia, Department Of Regional Development And Lands, Western Australia

Natural resources published reports

Fact sheets:

1. Applying biochar to improve soil quality and crop productivity

2. Reducing methane emissions from cattle using feed additives

3. Cattle breeding for lower greenhouse gas emissions

4. Managing genetic codes to reduce methane emissions from cattle

5. Managing pastures and stocking rate to reduce methane emissions from cattle

6. Claying as a method of increasing soil carbon content

7. Green and brown manuring as part of carbon farming

8. Permanent environmental plantings to earn carbon credits

9. Nitrous oxide emissions from agricultural soils

10. Sheep genetics in methane reduction

11. Managing sheep pastures to reduce methane production …

Tropical Cyclone Intensity Estimation Using Temporal And Spatial Features From Satellite Data, Gholamreza Fetanat Haghighi

Dissertations

Accurate intensity estimation of tropical cyclones (TC) is an important topic of research due to its economic impact and public safety concerns. An accurate measure of the current wind strength is necessary to accurately predict TC intensity. We have developed and tested automated method to estimate TC intensity based on the existing historical satellite images alone. The Hurricane Satellite data (HURSAT-B1) is used to develop the algorithm, which focuses on the North Atlantic from 1978-2009. The algorithm is trained and validated using aircraft reconnaissance-based data. Here, the data is restricted to include only fixes that are over water and are …

Production Mechanisms, Number Concentration, Size Distribution, Chemical Composition, And Optical Properties Of Sea Spray Aerosols, Nicholas Meskhidze, Markus D. Petters, Kostas Tsigaridis, Tim Bates, Colin O'Dowd, Jeff Reid, Ernie R. Lewis, Brett Gantt, Magdalena D. Anguelova, Prakash V. Bhave, Andrew Wozniak

Chemistry & Biochemistry Faculty Publications

(First paragraph)

The impact of sea spray aerosols on global climate remains one of the most uncertain components of the aerosol–radiation–climate problem, but has received less attention than the impacts of terrestrial and anthropogenic aerosols. The last decade has produced a large body of information regarding the sources and composition of marine aerosols, resulting in a reassessment of the complex role that sea spray particles play in climate and various geophysical phenomena. As sea spray aerosol contributes substantially to the preindustrial, natural background which provides the baseline on top of which anthropogenic forcing should be quantified, and because the ocean …

Ace-Fts Observations Of Acetonitrile In The Lower Stratosphere, J. J. Harrison, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

This work reports the first infrared satellite remote-sensing measurements of acetonitrile (CH₃CN) in the Earth's atmosphere using solar occultation measurements made by the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) between 2004 and 2011. The retrieval scheme uses new quantitative laboratory spectroscopic measurements of acetonitrile (Harrison and Bernath, 2012). Although individual ACE-FTS profile measurements are dominated by measurement noise, median profiles in 10 degrees latitude bins show a steady decline in volume mixing ratio from similar to 150 ppt (parts per trillion) at 11.5 km to < 40 ppt at 25.5-29.5 km. These new measurements agree well with the scant available air-and balloon-borne data in the lower stratosphere. An acetonitrile stratospheric lifetime of 73 ± 20 yr has been determined.

Quantifying The Impact Of Boreal Forest Fires On Tropospheric Oxidants Over The Atlantic Using Aircraft And Satellites (Bortas) Experiment: Design, Execution And Science Overview, P. I. Palmer, M. Parrington, J. D. Lee, A, C. Lewis, A. R. Rickard, P. F. Bernath, T. J. Duck, D. L. Waugh, D. W. Tarasick, S. Andrews

Chemistry & Biochemistry Faculty Publications

We describe the design and execution of the BORTAS (Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) experiment, which has the overarching objective of understanding the chemical aging of air masses that contain the emission products from seasonal boreal wildfires and how these air masses subsequently impact downwind atmospheric composition. The central focus of the experiment was a two-week deployment of the UK BAe-146-301 Atmospheric Research Aircraft (ARA) over eastern Canada, based out of Halifax, Nova Scotia. Atmospheric ground-based and sonde measurements over Canada and the Azores associated with the planned …

Ace-Fts Observations Of Pyrogenic Trace Species In Boreal Biomass Burning Plumes During Bortas, K. A. Tereszchuk, G. G. Abad, C. Clerbaux, J. Hadji-Lazaro, D. Hurtmans, P. F. Coheur, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

To further our understanding of the effects of biomass burning emissions on atmospheric composition, the BORTAS campaign (BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) was conducted on 12 July to 3 August 2011 during the boreal forest fire season in Canada. The simultaneous aerial, ground and satellite measurement campaign sought to record instances of boreal biomass burning to measure the tropospheric volume mixing ratios (VMRs) of short- and long-lived trace molecular species from biomass burning emissions. The goal was to investigate the connection between the composition and the distribution of these pyrogenic outflows and …

Stratospheric Lifetimes Of Cfc-12, Ccl4, Ch4, Ch3cl And N20 From Measurements Made By The Atmospheric Chemistry Experiment-Fourier Transform Spectrometer, A. T. Brown, C. M. Volk, M. R. Schoebert, C. D. Boone, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

Long lived halogen-containing compounds are important atmospheric constituents since they can act both as a source of chlorine radicals, which go on to catalyse ozone loss, and as powerful greenhouse gases. The long-term impact of these species on the ozone layer is dependent on their stratospheric lifetimes. Using observations from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) we present calculations of the stratospheric lifetimes of CFC-12, CCl₄, CH₄, CH₃Cl and N₂O. The lifetimes were calculated using the slope of the tracer-tracer correlation of these species with CFC-11 at the tropopause. The …

Harmonized Dataset Of Ozone Profiles From Satellite Limb And Occultation Measurements, V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. Von Savigny, A Laeng, T. Von Clarmann, P. Bernath, R. J. Hargreaves

Chemistry & Biochemistry Faculty Publications

In this paper, we present a HARMonized dataset of OZone profiles (HARMOZ) based on limb and occultation measurements from Envisat (GOMOS, MIPAS and SCIAMACHY), Odin (OSIRIS, SMR) and SCISAT (ACE-FTS) satellite instruments. These measurements provide high-vertical-resolution ozone profiles covering the altitude range from the upper troposphere up to the mesosphere in years 2001-2012. HARMOZ has been created in the framework of the European Space Agency Climate Change Initiative project. The harmonized dataset consists of original retrieved ozone profiles from each instrument, which are screened for invalid data by the instrument teams. While the original ozone profiles are presented in different …

Validation Of Stratospheric And Mesospheric Ozone Observed By Smiles From International Space Station, Y. Kasai, H. Sagawa, D. Kreyling, E. Dupuy, P. Baron, J. Mendrok, K Suzuki, T. O. Sato, T. Nishibori, S. Mizobuchi, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

We observed ozone O₃ in the vertical region between 250 and 0.0005 hPa (~ 12-96 km) using the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES) on the Japanese Experiment Module (JEM) of the International Space Station (ISS) between 12 October 2009 and 21 April 2010. The new 4K superconducting heterodyne receiver technology of SMILES allowed us to obtain a one order of magnitude better signal-to-noise ratio for the O₃ line observation compared to past spaceborne microwave instruments. The non-sun-synchronous orbit of the ISS allowed us to observe O₃ at various local times. We assessed the quality of the vertical …

The Relation Between Atmospheric Humidity And Temperature Trends For Stratospheric Water, S. Fueglistaler, Y. S. Liu, T. J. Flannaghan, P. H. Haynes, D. P. Dee, W. J. Read, E. E. Remsberg, L. W. Thomason, D. F. Hurst, J. R. Lanzante, P. F. Bernath

Chemistry & Biochemistry Faculty Publications

We analyze the relation between atmospheric temperature and water vapor-a fundamental component of the global climate system-for stratospheric water vapor (SWV). We compare measurements of SWV (and methane where available) over the period 1980-2011 from NOAA balloon-borne frostpoint hygrometer (NOAA-FPH), SAGE II, Halogen Occultation Experiment (HALOE), Microwave Limb Sounder (MLS)/Aura, and Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) to model predictions based on troposphere-to-stratosphere transport from ERA-Interim, and temperatures from ERA-Interim, Modern Era Retrospective- Analysis (MERRA), Climate Forecast System Reanalysis (CFSR), Radiosonde Atmospheric Temperature Products for Assessing Climate (RATPAC), HadAT2, and RICHv1.5. All model predictions are dry biased. The interannual …

Hydrocarbons In The Upper Troposphere And Lower Stratosphere Observed From Ace-Fts And Comparisons With Waccm, Mijeong Park, William J. Randel, Douglas E. Kinnison, Louisa K. Emmons, Peter F. Bernath, Kaley A. Walker, Chris D. Boone, Nathaniel J. Livesey

Chemistry & Biochemistry Faculty Publications

Satellite measurements from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) are used to examine the global, seasonal variations of several hydrocarbons, including carbon monoxide (CO), ethane (C₂H₆), acetylene (C₂H₂), and hydrogen cyanide (HCN). We focus on quantifying large-scale seasonal behavior from the middle troposphere to the stratosphere, particularly in the tropics, and furthermore make detailed comparisons with the Whole Atmosphere Community Climate Model (WACCM) chemistry climate model (incorporating tropospheric photochemistry, time-varying hydrocarbon emissions, and meteorological fields nudged from reanalysis). Comparisons with Microwave Limb Sounder (MLS) measurements of CO are also included …