Nuclear Commons^™

Experimental Investigation Of Steel Corrosion In Lead Bismuth Eutectic (Lbe): Characterization, Species Identification, And Chemical Reactions, John Farley, Dale L. Perry, Allen L. Johnson

Transmutation Sciences Materials (TRP)

The goal of the present research is to achieve a basic understanding of corrosion of steels by Lead Bismuth Eutectic (LBE). Liquid LBE is under consideration in the transmuter as both a spallation target and as a blanket coolant. There have been previous studies of LBE, especially by the Russians, who have over 80 reactor-years experience with LBE coolant in their Alpha-class submarine reactors. The Russians found that the presence of small amounts (ppm) of oxygen in the LBE significantly reduced corrosion. However, a fundamental understanding and verification of its role in the corrosion of steels is still very incomplete. …

University Of Nevada, Las Vegas Transmutation Research Program: Quarterly Report, Second Quarter Year 2 (June 2002 To August 2002), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Transmutation Research Program (TRP) Director to the U.S. Department of Energy (DOE) as described in the UNLV Advanced Accelerator Applications (AAA) proposal, and AAA FY02 Work Package. Note: during this quarter, the AAA national program changed names to the Advanced Fuel Cycle Initiative (AFCI) and the UNLV AAA University Participation Program changed its name to the Transmutation Research Program. The new names will be used in future references.

The TRP Director implements the program’s administration using staff from the Harry Reid Center for Environmental Studies …

Corrosion Of Steel By Lead Bismuth Eutectic: Quarterly Report November- December 2002 January 2003, John Farley

Transmutation Sciences Materials (TRP)

We continue to get valuable data from sputter depth profiling of steel samples. We meet weekly to discuss progress. We took depth-profiling data on D9 steel that had been exposed to LBE. This the first time we have examined this type of steel. This is important because it will enable us to separate out two effects and determine their effect on corrosion: composition of the steel vs surface preparation.

We started to plan a small experiments using a crucible of heated LBE, with the research program to be conducted at UNLV, on basic aspects of corrosion in this system. The …

An Analysis Of The Melt Casting Of Metallic Fuel Pins, Xiaolong Wu, Randy Clarksean, Yitung Chen [email protected], Darrell Pepper, Mitchell K. Meyer

Fuels Campaign (TRP)

• Background

– Casting Volatile Actinides

– Need to Contain Americium

– Overview of Project

• Fuel Rod Model

– Physical System

– Governing Equations

• Preliminary Modeling Results

– Mold Materials

– Injection Casting Velocity

Precision Measurement Of The Proton And Deuteron Spin Structure Functions G2 And Asymmetries A2, P. L. Anthony, R. G. Arnold, T. Averett, H. R. Band, N. Benmouna, W. Boeglin, H. Borel, P. E. Bosted, S. L. Bültmann, G. R. Court, C. E. Hyde-Wright, S. E. Kuhn, F. Sabatie, F. R. Wesselmann

Physics Faculty Publications

We have measured the spin struction functions g2(p) and g(2)(d) and the virtual photon asymmetries A(2)(p) and A(2)(d) over the kinetmatic range 0.02 less than or equal to x less than or equal to 0.8 and 0.7 less than or equal to Q² less than or equal to 20 GeV2 by scattering 29.1 and 32.3 GeV longitudinally polarized electrons from transversely polarized NH3 and (LiD)-Li-6 targets. Our measured g² approximately follows the twist-2 Wandzura-Wilczek calculation. The twist-3 reduced matrix elements d(2)(p) and d(2)(n) are less than two standard deviations from zero. The data are inconsistent with the Burkhardt-Cottingham …

The Neutron Charge Form Factor And Target Analyzing Powers From 3He (E→, E 'N) Scattering, J. Bermuth, P. Merle, C. Carasco, D. Baumann, R. Böhm, D. Bosnar, M. Ding, M. O. Distler, J. Friedrich, A. Klein

Physics Faculty Publications

The charge form factor of the neutron has been determined from asymmetries measured in quasi-elastic ³He(e→, e 'n) at a momentum transfer of 0.67 (GeV/c)². In addition, the target analyzing power, Ayo has been measured to study effects of final state interactions and mespn exchange currents.

Final State Interaction Effects In 3He (E→, E' P), C. Carasco, J. Bermuth, P. Merle, P. Bartsch, D. Baumann, R. Böhm, D. Bosnar, M. Ding, M. O. Distler, A. Klein

Physics Faculty Publications

Asymmetries in quasi-elastic ³He(e→, e 'p) have been measured at a momentum transfer of 0.67 (GeV/c)² and are compared to a calculation which takes into account relativistic kinematics in the final state and a relativistic one-body current operator. With an exact solution of the Faddeev equation for the ³He-ground state and an approximate treatment offinal state interactions in the continuum good agreement is found with the experimental data.

Ep → Ep Π⁰ Reaction Studied In The Δ(1232) Mass Region Using Polarization Asymmetries, M. Bektasoglu, L. Ciciani, K.V. Dharmawardane, G. E. Dodge, T.A. Forest, C.E. Hyde-Wright, A. Klein, A. V. Klimenko, S. E. Kuhn, S. Stepanyan, L. B. Weinstein, Et Al., Clas Collaboration

Physics Faculty Publications

Measurements of the angular distributions of target and double-spin asymmetries for the Δ⁺(1232) in the exclusive channel ^→ p(^→e,e'p)π⁰ obtained at the Jefferson Lab in the Q² range from 0.5 to 1.5 GeV²/c² are presented. Results of the asymmetries are compared with the unitary isobar model [D. Drechsel , Nucl. Phys. A645, 145 (1999)], dynamical models [T. Sato and T. S. Lee, Phys. Rev. C 54, 2660 (1996); S. S. Kamalov , Phys. Lett. B 27, 522 (2001)], and the effective Lagrangian theory [R. M. Davidson , Phys. Rev. …

First Measurement Of Transferred Polarization In The Exclusive →E P → E'K+ →Λ, M. Bektasoglu, K. V. Dharmawardane, G. E. Dodge, T. A. Forest, C. E. Hyde-Wright, A. V. Klimenko, S. E. Kuhn, R. A. Niyazov, L. M. Qin, L. B. Weinstein, J. Yun

Physics Faculty Publications

The first measurements of the transferred polarization for the exclusive ^→ep → e'K+ ^→Λ over right arrow reaction have been performed at Jefferson Laboratory using the CLAS spectrometer. A 2.567 GeV beam was used to measure the hyperon polarization over Q² from 0.3 to 1.5 (GeV/c)², W from 1.6 to 2.15 GeV, and over the full K⁺ center-of-mass angular range. Comparison with predictions of hadrodynamic models indicates strong sensitivity to the underlying resonance contributions. A nonrelativistic quark-model interpretation of our data suggests that the s ^-s quark pair is produced with spins predominantly …

Radiation Transport Modeling Using Parallel Computational Techniques, William Culbreth

Reactor Campaign (TRP)

The Advanced Fuel Cycle Initiative (AFCI) program will rely on the use of accurate calculations and simulations of criticality and shielding for the separation process of the longlived isotopes that present a significant safety hazard in commercial spent fuel. To help design and verify the safety of the separation process, the neutronics code MCNPX will be used to model the distribution of neutron flux within the fuel blanket and to determine the neutron multiplication, k_eff. However, the cross section libraries and computational methods used by MCNPX at these neutron energies still have some uncertainty and will require validation. …

Radiation Transport Modeling Using Parallel Computational Techniques, William Culbreth, Denis Beller

Reactor Campaign (TRP)

The second year of this project involved modeling several aspects of the LANCSE beam experiments:

• Modeling targets of varying diameter in air, in a vacuum, and in the presence of humid air;
• Modeling various proton beam profiles;
• Modeling the effects of off-axis proton beam impingement on the target;
• Modeling the asymmetry introduced by the steel table below the target;
• Modeling the effect of varying ratios of Pb to Bi and the effect of impurities; and
• Modeling the system, including other structures within the test room.

With the experience gained through modeling these systems, the UNLV researchers plan, with the assistance …

Monte Carlo Verification And Modeling Of Lead-Bismuth Spallation Targets, Daniel R. Lowe

Reactor Campaign (TRP)

No abstract provided.

University Of Nevada, Las Vegas Transmutation Research Program Annual Report 2002, Anthony Hechanova, Elizabeth Johnson, Gary Cerefice

Transmutation Research Program Reports (TRP)

The UNLV Transmutation Research Program consists of four components: Program Support, Research Infrastructure Augmentation, International Collaboration, and Student Research.

In the first year of the program, the student research component was supported by the infrastructure augmentation and the program support components. In the second year of the program, the fourth leg of the support system, international collaborations, was added to the research support system.

Corrosion Of Steel By Lead Bismuth Eutectic, John Farley, Allen L. Johnson, Dale L. Perry

Transmutation Sciences Materials (TRP)

Materials for transmuter systems must be able to tolerate high neutron fluxes, great temperatures, and chemical corrosion. For lead bismuth eutectic (LBE) systems, there is an additional challenge in that the corrosive behaviors of materials in LBE are not well understood. Most of the available information on LBE systems has come from the Russians, who have over 80 reactor-years experience with LBE coolant in their Alpha-class submarine reactors. The Russians found that the presence of small amounts of oxygen (on the order of parts per million) in the LBE significantly reduced corrosion. However, a fundamental understanding and verification of its …

Surface Studies Of Corrosion Of Stainless Steel By Lead Bismuth Eutectic, Daniel Koury, Brian D. Hosterman, John Farley, Dale L. Perry, D. Parsons, J. Manzerova, Allen L. Johnson

Transmutation Sciences Materials (TRP)

Why is Lead Bismuth Eutectic Important?

• Changing national security stances have led to reexamination of nuclear waste reprocessing

• Dangerous actinides can be separated and

• Transmuted into safer products, creating a waste form dangerous for only hundreds of years, in addition to the production (up to 1/3 of the original fission energy) of useful energy

• Non-moderating coolants or spallation targets for production of fast neutrons is required for transmutation

• Russian experience with LBE coolants in their nuclear submarine fleet makes LBE an attractive possible transmutation coolant technology

• Corrosion of steel by LBE is an important …

Neutron Multiplicity Measurements Of Target/Blanket Materials, Carter D. Hull, Denis Beller

Transmutation Sciences Physics (TRP)

To optimize the performance of accelerator driven transmutation systems (ADS), engineers will need to design the system to operate with a neutron multiplication factor just below that of a critical, or self-sustaining, system. This design criteria requires particle transport codes that instill the highest level of confidence with minimal uncertainty, because the larger the uncertainties in the codes, the larger the safety margin required in the design and the lower the efficiency of the ADS transmuter. For current design efforts, the MCNPX code is used to determine neutron production and transport for spallation neutron systems.

While providing a very useful …

Development Of Dose Coefficients For Radionuclides Produced In Spallation Targets, Phillip W. Patton, Mark Rudin

Transmutation Sciences Physics (TRP)

Dose coefficients permit simple determination of radiation dose associated with various exposure scenarios, and ultimately permit radiation safety personnel to assess the health risks to workers in a nuclear facility. Specifically, radiation safety personnel use dose coefficients to determine the radiation dose incurred to a tissue or organ system from a given exposure. These parameters are often expressed in terms of Annual Limits on Intake (ALIs) and Derived Air Concentrations (DACs).

Results from this study will be used to produce ALIs and DACs for these rare radionuclides created by spallation target systems that are not included in Federal Guidance Report …

Development Of Dose Coefficients For Radionulides Produced In Spallation Neutron Sources: Annual Report, Phillip W. Patton, Mark Rudin

Transmutation Sciences Physics (TRP)

The University of Nevada, Las Vegas (UNLV) Transmutation Research Program has been tasked to support U.S. Department of Energy (DOE) efforts to assess the health risks associated with the operation of each of their accelerator-driven nuclear facilities for both NEPA and PSAR development. Quantifying the radiological risks to workers will have to be addressed during the design and siting of each of these facilities. U.S. Environmental Protection Agency (EPA) Federal Guidance Report No. 11 “Limiting Values of Intake and Air Concentration and Dose Conversion Factors for Inhalation, Submersion, and Ingestion”, developed two derived guides, Annual Limit on Intake (ALI) and …

Nuclear Criticality, Shielding, And Thermal Analyses Of Separations Processes For The Transmutation Fuel Cycle, William Culbreth, Denis Beller

Separations Campaign (TRP)

The first step in any transmutation strategy is the separation of radionuclides in used nuclear fuel. The current separation strategy supporting the Advanced Fuel Cycle Initiative (AFCI) program is based on the use of a solvent extraction separation process to separate the actinides, fission products, and uranium from used commercial nuclear fuel, and on the use of pyrochemical separation technologies to process used transmuter fuels. To separate the fission products and transuranic elements from the uranium in used fuel, the national program is developing a new solvent extraction process, the Uranium Extraction Plus, or UREX+, process, based on the traditional …

Design And Analysis Of A Process For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides, Yitung Chen, Darrell Pepper, Randy Clarksean

Fuels Campaign (TRP)

The goal of this project is to investigate the casting processes for metallic fuels to help design a process that minimizes the loss of the volatile actinide elements from the fuel.

The research effort centers on the development of advanced numerical models to assess conditions that significantly impact the transport of volatile actinides during the melt casting process and represents a joint effort between researchers at the University of Nevada, Las Vegas (UNLV) and Argonne National Laboratory (ANL).

Corrosion Of Steel By Lead Bismuth Eutectic: Quarterly Report August September October 2002, John Farley

Transmutation Sciences Materials (TRP)

We continued with sputter depth profiling of 316 and 316L steel samples that have been exposed to LBE. We also calibrated the sputter depth profiling using a sample of SiO₂ on Si, and the SEM. This is a valuable independent determination of the thickness of oxide layers.

In the laboratory, progress continues using the XPS machine. Experiments have been performed on steel samples using Argon ions to mill away the surface of the sample, thereby making measurements as a function of depth. This "ion beam milling" proceeds slowly through the oxide layer that covers the steel sample. We are …

University Of Nevada, Las Vegas Advanced Accelerator Applications University Participation Program: Quarterly Report, First Quarter Year 2 (March 2002 To May 2002), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Advanced Accelerator Applications (AAA) University Participation Program (UPP) Director to the U.S. Department of Energy (DOE) as described in the UNLV AAA proposal, and Statement of Work for the First Quarter Year 2 and AAA FY02 Work Package.

The UNLV AAA UPP Director implements the program’s administration using staff from the Harry Reid Center for Environmental Studies (HRC) to ensure that work conducted under the UNLV AAA UPP meets program objectives. The UNLV AAA program consists of four components: Program Support, Research Infrastructure Augmentation, International …

University Of Nevada, Las Vegas Advanced Accelerator Applications University Participation Program: Quarterly Report, Third Quarter Year 2 (Sept. 2002 To Nov. 2002), Anthony Hechanova

Transmutation Research Program Reports (TRP)

This Quarterly Report is a primary deliverable from the University of Nevada, Las Vegas (UNLV) Advanced Accelerator Applications (AAA) University Participation Program (UPP) Director to the U.S. Department of Energy (DOE) as described in the UNLV AAA proposal and Statement of Work for the Fourth Quarter.

The UNLV AAA UPP Director implements the program’s administration using staff from the Harry Reid Center for Environmental Studies (HRC) to ensure that work conducted under the UNLV AAA UPP meets program objectives. The UNLV AAA program consists of three components: Program Support, Research Infrastructure Augmentation, and Student Research.

Radiation Transport Modeling Of Beam-Target Experiments For The Aaa Project: Quaterly Report, June 01- August 31, 2002, William Culbreth

Reactor Campaign (TRP)

The national development of technology to transmute nuclear waste depends upon the generation of high-energy neutrons produced by proton spallation. Proton accelerators, such as LANSCE at the Los Alamos National Laboratory, are capable of producing 800 MeV protons. By bombarding a lead /bismuth target, each proton may generate up to 25 neutrons that can activate fission of transuranic isotopes. Students at UNLV have been involved in radiation transport calculations in collaboration with researchers at the Los Alamos National Laboratory and at the Argonne National Laboratory.

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides: Quarterly Progress Report 5/16/02- 8/15/02, Yitung Chen, Randy Clarksean, Darrell Pepper

Fuels Campaign (TRP)

An important aspect of the Advanced Accelerator Applications (AAA) program is the development of a casting process by which volatile actinide element (i.e., americium) can be incorporated into metallic alloy fuel pins. The traditional metal fuel casting process uses an inductively heated crucible.

This process works well for the fabrication of metal fuel pins traditionally composed of alloys of uranium and plutonium, but does not work well when highly volatile actinides are included in the melt. The problem occurs both during the extended time period required to superheat the alloy melt as well as when the chamber must be evacuated. …

Corrosion Of Steel By Lead Bismuth Eutectic: Quarterly Report For May-June-July 2002, John Farley

Transmutation Sciences Materials (TRP)

The goal of this project is to understand the basic science of corrosion in the steel/LBE system.

We are taking more data, typically using the newly installed X-ray Photoelectron Spectrometry (XPS) apparatus, and analyzing our existing data. Undergraduate students Denise Parsons and Julia Manzerova have helped a great deal in the analysis of the data. We can obtain the elemental composition as a function of position within the sample. This gives clues to the migration of materials, the composition of the protective oxide layer, and the basic science of the corrosion process. We found dramatic differences between the exposed and …

Dose Coefficient (Dc) Methodology Report, John P. Shanahan, Phillip W. Patton, Mark Rudin

Transmutation Sciences Physics (TRP)

The purpose of this report is to present the methodology developed to calculate internal and external dose coefficients for radionuclides produced in the spallation process. Much of the information regarding computer codes in this report comes from various technical manuals and professional papers. References are provided at the beginning of each section for documentation and for the user who requires more specific information. The report also includes the results of applying the methodology to determine dose coefficients for five radionuclides. This effort identified potential areas of concern that will need to be addressed when the methodology is used in the …

Efficient And Accurate Computation Of Non-Negative Anisotropic Group Scattering Cross Sections For Discrete Ordinates And Monte Carlo Radiation Transport, David W. Gerts

Theses and Dissertations

A new method for approximating anisotropic, multi-group scatter cross sections for use in discretized and Monte Carlo multi-group neutron transport is presented. The new method eliminates unphysical artifacts such as negative group scatter cross sections and falsely positive cross sections. Additionally, when combined with the discrete elements angular quadrature method, the new cross sections eliminate the lack of angular support in the discrete ordinates quadrature method. The new method generates piecewise-average group-to-group scatter cross sections. The accuracy and efficiency for calculating the discrete elements cross sections has improved by many orders of magnitude compared to DelGrande and Mathews previous implementation. …

Phase I: Design And Analysis Of A Process For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides, Yitung Chen, Randy Clarksean, Darrell Pepper

Fuels Campaign (TRP)

The proposed research would be conducted in 3 phases. Each of the phases would be carried out over a one-year period. Phase I includes model development, analysis, and the selection of a new casting furnace design. The work discussed in this report was completed as Phase I. Phase II of the program will lead to more modeling and validation to evaluate the proposed furnace concept. Phase III would be a joint effort between UNLV and Argonne National Laboratory (ANL) to demonstrate the acceptable use of the new furnace in a simulated remote environment.

The Phase III work would include the …

Non-Dipolar Electron Angular Distributions From Fixed-In-Space Molecules, Renaud Guillemin, Oliver Hemmers, Dennis W. Lindle, E. Shigemasa, K. Le Guen, D. Ceolin, C. Miron, N. Leclercq, P. Morin, Marc Simon, P. W. Langhoff

Environmental Studies Faculty Publications

The first indication of nondipole effects in the azimuthal dependence of photoelectron angular distributions emitted from fixed-in-space molecules is demonstrated in N₂. Comparison of the results with angular distributions observed for randomly oriented molecules and theoretical derivations for the nondipole correction first order in photon momentum suggests that higher orders will be needed to describe distributions measured in the molecular frame.