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Articles 991 - 999 of 999

Full-Text Articles in Elementary Particles and Fields and String Theory

Anisotropy Of Polarized X-Ray Emission From Molecules, S. H. Southworth, Dennis W. Lindle, R. Mayer, P. L. Cowan Aug 1991

Anisotropy Of Polarized X-Ray Emission From Molecules, S. H. Southworth, Dennis W. Lindle, R. Mayer, P. L. Cowan

Chemistry and Biochemistry Faculty Research

Strongly anisotropic, polarized Cl K-V x-ray emission from gas-phase CF3Cl has been observed following resonant excitation with a linearly polarized x-ray beam. Distinctively different angular distributions are observed for x-ray emission involving molecular orbitals of different symmetries. A classical model of the x-ray absorption-emission process accurately describes the observed radiation patterns.

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Molecular-Orbital Studies Via Satellite-Free X-Ray Fluorescence: Cl-K Absorption And K–Valence-Level Emission Spectra Of Chlorofluoromethanes, Rupert C. Perera, P. L. Cowan, Dennis W. Lindle, R. E. Lavilla, T. Jach, R. D. Deslattes Apr 1991

Molecular-Orbital Studies Via Satellite-Free X-Ray Fluorescence: Cl-K Absorption And K–Valence-Level Emission Spectra Of Chlorofluoromethanes, Rupert C. Perera, P. L. Cowan, Dennis W. Lindle, R. E. Lavilla, T. Jach, R. D. Deslattes

Chemistry and Biochemistry Faculty Research

X-ray absorption and emission measurements in the vicinity of the chlorine K edge of the three chlorofluoromethanes have been made using monochromatic synchrotron radiation as the source of excitation. By selectively tuning the incident radiation to just above the Cl 1s single-electron ionization threshold for each molecule, less complex x-ray-emission spectra are obtained. This reduction in complexity is attributed to the elimination of multielectron transitions in the Cl K shell, which commonly produce satellite features in x-ray emission. The resulting "satellite-free" x-ray-emission spectra exhibit peaks due only to electrons in valence molecular orbitals filling a single Cl 1s vacancy. These …

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Polarized X-Ray-Emission Studies Of Methyl Chloride And The Chlorofluoromethanes, Dennis W. Lindle, P. L. Cowan, T. Jach, R. E. Lavilla, R. D. Deslattes, Rupert C. Perera Mar 1991

Polarized X-Ray-Emission Studies Of Methyl Chloride And The Chlorofluoromethanes, Dennis W. Lindle, P. L. Cowan, T. Jach, R. E. Lavilla, R. D. Deslattes, Rupert C. Perera

Chemistry and Biochemistry Faculty Research

A new technique sensitive to molecular orientation and geometry, and based on measuring the polarization of x-ray emission, has been applied to the Cl-containing molecules methyl chloride (CH3Cl) and the chlorofluoromethanes (CF3Cl, CF2Cl2, and CFCl3) in the gas phase. Upon selective excitation using monochromatic synchrotron radiation in the Cl K-edge (Cl 1s) near-threshold region, polarization-selective x-ray emission studies reveal highly polarized molecular valence x-ray fluorescence for all four molecules. The degree and the orientation of the polarized emission are observed to be sensitive to the incident excitation energy near …

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Direct Determination Of Molecular-Orbital Symmetry Of H2s Using Polarized X-Ray Emission, R. Mayer, Dennis W. Lindle, S. H. Southworth, P. L. Cowan Jan 1991

Direct Determination Of Molecular-Orbital Symmetry Of H2s Using Polarized X-Ray Emission, R. Mayer, Dennis W. Lindle, S. H. Southworth, P. L. Cowan

Chemistry and Biochemistry Faculty Research

X-ray emission from the molecule H2S is strongly polarized following excitation of a sulfur K-shell electron to an unoccupied subthreshold molecular orbital with a polarized x-ray beam. Changes in the polarization of the emission spectrum are observed as the incident beam's energy is swept across the subthreshold absorption resonance. The previously unresolved absorption resonance is shown experimentally to be primarily associated with a molecular orbital of b2 symmetry, but with a high-excitation-energy component due to an orbital with a1 symmetry. Satellite emission intensity is shown to depend on the primary photon energy and is therefore associated …

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Argon-Photoion–Auger-Electron Coincidence Measurements Following K-Shell Excitation By Synchrotron Radiation, Jon C. Levin, C. Biedermann, N. Keller, L. Liljeby, C.-S. O, R. T. Short, Ivan A. Sellin, Dennis W. Lindle Aug 1990

Argon-Photoion–Auger-Electron Coincidence Measurements Following K-Shell Excitation By Synchrotron Radiation, Jon C. Levin, C. Biedermann, N. Keller, L. Liljeby, C.-S. O, R. T. Short, Ivan A. Sellin, Dennis W. Lindle

Chemistry and Biochemistry Faculty Research

Argon photoion spectra have been obtained for the first time in coincidence with K-LL and K-LM Auger electrons, as a function of photon energy. The simplified charge distributions which result exhibit a much more pronounced photon-energy dependence than do the more complicated noncoincident spectra. In the near-K-threshold region, Rydberg shakeoff of np levels, populated by resonant excitation of K electrons, occurs with significant probability, as do double-Auger processes and recapture of the K photoelectron through postcollision interaction.

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Critical Dimensions For Chiral Bosons, Luca Mezincescu, Rafael I. Nepomechie Jan 1988

Critical Dimensions For Chiral Bosons, Luca Mezincescu, Rafael I. Nepomechie

Physics Articles and Papers

We give the Lagrangian formulation of a Bose model in 1+1 dimensions which describes a free chiral Lie-algebra-valued current. This model is a non-Abelian generalization of the chiral scalar model of Siegel. Both the Abelian and non-Abelian actions have a gauge invariance, which becomes anomalous when the models are quantized. The condition that this anomaly be canceled coincides with the string no-ghost condition.

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The Energy-Dependence Of Polarization Observables In The ²H(D,Γ)⁴He Reaction, H. R. Weller, R. M. Whitton, J. Langenbrunner, Evans Hayward, W. R. Dodge, S. Kuhn, D. R. Tilley Jan 1988

The Energy-Dependence Of Polarization Observables In The ²H(D,Γ)⁴He Reaction, H. R. Weller, R. M. Whitton, J. Langenbrunner, Evans Hayward, W. R. Dodge, S. Kuhn, D. R. Tilley

Physics Faculty Publications

Measurements of the tensor and vector analyzing powers, Ayy(130°) and Ay(130°), have been obtained for the 2H(d,γ )4He reaction for energies ranging from Ed(lab) = 0.3 MeV to Ed(lab) = 50 MeV. The Ayy(130°) data are sensitive to the D-state present in the ground state of 4He and are observed to have their maximum value near Ed = 30 MeV. The vector analyzing power data show a maximum near Ed = 3 MeV. The data are compared to the results of a microscopic …

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Non-Abelian Bosonization: Current Correlation Functions, Lowell S. Brown, Rafael I. Nepomechie Jan 1987

Non-Abelian Bosonization: Current Correlation Functions, Lowell S. Brown, Rafael I. Nepomechie

Physics Articles and Papers

We demonstrate that, in 1+1 dimensions, the effective action produced by massless fermions moving in external gauge potentials is identical with that produced by a suitably defined σ model which includes a Wess-Zumino term. Hence the current correlation functions of the fermion and boson theories are identical.

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Excitation Of Hydrogen Atoms By Fast Protons, Edward Ellis Fitchard Jan 1970

Excitation Of Hydrogen Atoms By Fast Protons, Edward Ellis Fitchard

Physics Theses & Dissertations

In this thesis a theoretical study is made of excitation of hydrogenic atom by charged particles such as protons or electrons. The approximation to the cross section for an inelastic scattering process is obtained under the following radically simplifying assumptions. The projectile is represented in its initial and final state by plane waves. All distortions are neglected whether they originate in an inelastic process or an elastic deflections of the charged particle by the nucleus. The perturbation of the atomic orbits between which the projectile induces transitions is neglected. Nonrelativistic hydrogenic wave functions are used for the electronic states. In …

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