Quantum Physics Commons^™

Tip-Enhanced Nano-Optical Imaging Of Superacid Treated Bilayer Mos2-Ws2 2d Lateral Heterostructures, Amala Dixit

USF Tampa Graduate Theses and Dissertations

Nanoscale optical characterization of two-dimensional (2D) materials and heterostructures is important for the design of novel optoelectronic flexible nano-devices. Nano-optical photoluminescence (PL) and Raman imaging of bilayer 2D materials has been a challenging problem due to weak signals. The exciton-dominated light emission of two-dimensional (2D) transition metal dichalcogenide (TMDC) materials is affected by the formation of defects and doping states. Previous studies have shown that chemical treatment modifies the defect and doping states of chemical vapor deposition (CVD)-grown monolayers of MoS₂ and WS₂, which provides a promising possibility for engineering the optoelectronic properties of these 2D TMDCs. …

Control Of Light-Matter Interactions Via Nanostructured Photonic Materials, Nicholas Proscia

Dissertations, Theses, and Capstone Projects

The thesis here investigates the manipulation of light-matter interactions via nanoscale engineering of material systems. When material systems are structured on the nanoscale, their optical responses can be dramatically altered. In this thesis, this is done in two primary ways: One method is by changing the geometry of nanostructures to induce a resonant behavior with incident electromagnetic field of optical wavelengths. This allows field enhancement in highly localized areas to strengthen exotic light-matter interactions that would otherwise be too weak to measure or for practical use. In this regard, the work presented here studies a voltage produced in a metal …

Physics And Applications Of Exceptional Points, Qi Zhong

Dissertations, Master's Theses and Master's Reports

Exceptional points (EPs) are singularities that arise in non-Hermitian physics. Crossing EPs is believed to be related with phase transitions between parity-time-(PT-)symmetric phase and broken PT phase. Owing to their peculiar topology, EPs can remotely induce observable effects when encircled by closed trajectories in the parameter space. In this dissertation, first of all, we investigate the extreme dynamics of non-Hermitian systems near higher order EPs constructed using the bosonic algebra method. The strong power oscillations for certain initial conditions can occur as a result of the peculiar eigenspace geometry and its dimensionality collapse near these singularities. And in the PT …

Using Fundamental Properties Of Light To Investigate Photonic Effects In Condensed Matter And Biological Tissues, Laura A. Sordillo

Dissertations and Theses

Light possesses characteristics such as polarization, wavelength and coherence. The interaction of light and matter, whether in a semiconductor or in a biological sample, can reveal important information about the internal properties of a system. My thesis focuses on two areas: photocarriers in gallium arsenide and biomedical optics. Varying the excitation wavelength can be used to study both biological tissue and condensed matter. I altered the excitation wavelengths to be in the longer near-infrared (NIR) optical windows, in the shortwave infrared (SWIR) range, a wavelength region previously thought to be unusable for medical imaging. With this method, I acquired high …

Plasmonic Enhancement Of Photoluminescence And Photobrightening In Cdse Quantum Dots, David Alan French

Graduate Theses and Dissertations

Quantum dots are gaining recognition not just in the physics and chemistry community, but in the public eye as well. Quantum dot technologies are now being used in sensors, detectors, and even television displays. By exciting quantum dots with light or electricity, they can be made to emit light, and by altering the quantum dot characteristics the wavelength can be finely tuned. The light emitted can be also be made more intense by an increase in the excitation energy. The excitation light can be increased via plasmonic enhancement, leading to increased luminescence. Aside from the relatively steady-state response, quantum dots …

Beam Theory For Classical And Quantum Nonlinear Optics---Exposing Classical And Quantum Correlations Of Transverse-Spatial Modes, Robert Nicholas Lanning

LSU Doctoral Dissertations

Optics is arguably the most important branch of physics that has ever been studied. It is not only an essential ingredient of many other branches of physics that we study, it governs how we see, how we measure, and how we communicate in the modern world. And as the world continues to change, so do our tools and resources. In a relatively short amount of time, we have progressed from rudimentary tools that shape the world around us, to tools that harness the fundamental laws of nature. Unsurprisingly, the laws of nature governing optics remain paramount. This is because many …

Catalysis Of Stark-Tuned Interactions Between Ultracold Rydberg Atoms, A. L. Win, W. D. Williams, T. J. Carroll, C. I. Sukenik

Physics Faculty Publications

We have experimentally investigated a catalysis effect in the resonant energy transfer between ultracold ⁸⁵Rb Rydberg atoms. We studied the time dependence of the process, 34p + 34p → 34s + 35s, and observed an enhancement of 34s state population when 34d state atoms are added. We have also performed numerical model simulations, which are in qualitative agreement with experiment and indicate that the enhancement arises from a redistribution of p-state atoms due to the presence of the d-state atoms.

Charge State Dynamics And Quantum Sensing With Defects In Diamond, Jacob D. Henshaw

Dissertations, Theses, and Capstone Projects

In recent years, defect centers in wide band gap semiconductors such as diamond, have received significant attention. Defects offer great utility as single photon emitters, nanoscale sensors, and quantum memories and registers for quantum computation. Critical to the utility of these defects, is their charge state.

In this dissertation, experiments surrounding the charge state dynamics and the carrier dynamics are performed and analyzed. Extensive studies of the ionization and recombination processes of defects in diamond, specifically, the Nitrogen Vacancy (NV) center, have been performed. Diffusion of ionized charge carriers has been imaged indirectly through the recapture of said carriers by …

Scattering Of Few Photon Fields By Two Level Systems In A One Dimensional Geometry, William Konyk

Graduate Theses and Dissertations

Recent experimental progress has realized strong, efficient coupling of effective two level systems to waveguides. We study the scattering of multimode photons from such emitters coupled losslessly to the confined geometry of a one dimensional waveguide. We develop novel techniques for describing the scattered state of both single and multi-photon wavepackets and explore how such wavepackets interact with arrays of emitters coupled to a one dimensional waveguide. Finally, we apply these techniques and analyze the capability of two particular systems to act as a quantum conditional logic gate.

Broadband Measurement And Reduction Of Quantum Radiation Pressure Noise In The Audio Band, Jonathan Daniel Cripe

LSU Doctoral Dissertations

One hundred years after Albert Einstein predicted the existence of gravitational waves in his general theory of relativity, the Laser Interferometer Gravitational-Wave Observatory (LIGO) made the first direct detection of gravitational waves. Since the first detection of gravitational waves from a binary black hole merger, LIGO has gone on to detect gravitational waves from multiple binary black hole mergers, and more recently from a binary neutron star merger in collaboration with telescopes around the world. The detection of gravitational waves has opened a new window to the universe and has launched the era of gravitational wave astronomy.

With the first …

Precision Spectroscopy Of Beryllium, Advik D. Vira

Theses, Dissertations, and Projects

We report on the calibration and absolute frequency results for the 2s2p1P1 state in neutral atomic beryllium-9. We start off with a discussion of the method used to calibrate the laser, which includes a detailed explanation of the basic physics involved, and then discuss the results for the lowest singlet state in neutral beryllium-9. We discuss a way to predict the spectra using optical Bloch equations and then present and analyze the experimental results. We found the absolute frequency for the 1P1 state to be 42565.4487(30) cm-1, which is in agreement with the current best theoretical estimateof42565.441(11)cm-1 [49]. Amoresophisticatedanalyticaltechniqueisproposed; however, …

Dispersive Quantum Interface With Atoms And Nanophotonic Waveguides, Xiaodong Qi

Physics & Astronomy ETDs

Strong coupling between atoms and light is critical for quantum information processing and precise sensing. A nanophotonic waveguide is a promising platform for realizing an atom-light interface that reaches the strong coupling regime. In this dissertation, we study the dispersive response theory of the nanowaveguide system as the means to create an entangling atom-light interface, with applications to quantum non-demolition (QND) measurement and spin squeezing.

We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of a nanowaveguide, and thus the phase shift and polarization rotation induced on the guided light. The Green's …

Achieving A Stable Magneto-Optical Trap, Chasen S. Himeda

Honors Thesis

The utilization of the Magneto-Optical Trap (MOT) as a method for cooling and confining atoms is a recent development in the field of modern optical physics. Producing an effective MOT relies on a constant magnetic field throughout the trapping region and successful laser cooling, a technique used to achieve optical molasses by slowing particles using a three-dimensional intersection of laser beams. A successful MOT occurs when the trapped atoms slow down to approximately 30 cm/s at a temperature in the microkelvin range and is observable when a small bright orb of atoms is located in the center of the chamber. …

Studies Of Light Generation With Four-Wave Mixing In A Cold Atomic Ensemble, Andrew Ferdinand

Physics & Astronomy ETDs

Correlated light generated from atomic ensembles can have a central role in prominent quantum information protocols, such as long-distance quantum communication. Here we present our studies on three topics involving the generation of correlated light with four-wave mixing (FWM) in a cold atomic ensemble for applications in quantum communications with high capacity. We experimentally investigate the generation of light with seeded FWM in cold cesium atoms and the time correlations of photon pairs generated with spontaneous FWM. We theoretically investigate the correlations in orbital angular momentum of photon pairs generated with spontaneous FWM for a range of experimental geometries. These …

Optimizing An Electron's Path To Ionization Using A Genetic Algorithm, Jason Bennett, Kevin Choice

Physics and Astronomy Summer Fellows

A Rydberg atom is an atom with a highly excited and weakly bound valence electron. A widespread method of studying quantum mechanics with Rydberg atoms is to ionize the electron and measure its arrival time. We use a Genetic Algorithm (GA) to control the electron's path to ionization. The Rydberg electron's energy levels are strongly shifted by the presence of an electric field. The energy levels shift and curve, but never cross. At an avoided crossing the electron can jump from one level to the next. By engineering the electric field's time dependence, we thereby control the path to ionization. …

Quantum Optical Interferometry And Quantum State Engineering, Richard J. Birrittella Jr

Dissertations, Theses, and Capstone Projects

We highlight some of our research done in the fields of quantum optical interferometry and quantum state engineering. We discuss the body of work for which our research is predicated, as well as discuss some of the fundamental tenants of the theory of phase estimation. We do this in the context of quantum optical interferometry where our primary interest lies in the calculation of the quantum Fisher information as it has been shown that the minimum phase uncertainty obtained, the quantum Cramer-Rao bound, is saturated by parity-based detection methods. We go on to show that the phase uncertainty one obtains …

Studies In Mesoscopics And Quantum Microscopies, Zhenghao Ding, Gabriel C. Spalding

Honors Projects

This thesis begins with a foundational section on quantum optics. The single-photon detectors used in the first chapter were obtained through the Advanced Laboratory Physics Association (ALPhA), which brokered reduced cost for educational use, and the aim of the single-photon work presented in Chapter 1 is to develop modules for use in Illinois Wesleyan's instructional labs beyond the first year of university. Along with the American Association of Physics Teachers, ALPhA encourages capstone-level work, such as Chapter 1 of this honors thesis, which is explicitly designed to play the role of passing on, to a next generation of physics majors, …

Key Encryption Through Quantum Optics, Madison Durrance, Zach Galberd, Abbey Savage, Tristan Cabrera, Josh Hoffman

Georgia College Student Research Events

Cryptography has been around since the dawn of human civilization to send private messages for commercial, military, and political purposes. Some of the most important ciphers are the Vigenère cipher, the enigma, and the more modern RSA. Because of the development of the internet, private encryption has also become increasingly more important. The weakest link of encryption is the key creation and key distribution. A key is needed to encrypt and decipher codes and is needed by both the user and sender. A solution to this problem is the generation of quantum key distributions. In our experiment, we are now …

Quantum Foundations With Astronomical Photons, Calvin Leung

HMC Senior Theses

Bell's inequalities impose an upper limit on correlations between measurements of two-photon states under the assumption that the photons play by a set of local rules rather than by quantum mechanics. Quantum theory and decades of experiments both violate this limit.

Recent theoretical work in quantum foundations has demonstrated that a local realist model can explain the non-local correlations observed in experimental tests of Bell's inequality if the underlying probability distribution of the local hidden variable depends on the choice of measurement basis, or ``setting choice''. By using setting choices determined by astrophysical events in the distant past, it is …

Discord And Global Discord In Systems Of Coupled Quantum Dots In Driven Cavities With Dissipation, And A Method For The Calculation Of Global Discord, Willa Danielle Rawlinson

Graduate Theses and Dissertations

In the field of quantum information, which is subdivided into quantum computing and quantum cryptography, quantum correlations are essential for a performance or security boost not achievable with classical means. Various quantum correlation measures exist for evaluating a state’s potential to be a qubit (quantum bit). Entanglement, or nonseparability of quantum states, is the older, better known class of measures. However, for a mixed state, quantum entanglement is an incomplete measure of quantumness. Quantum discord, and its multibody extension global discord, encompass all quantum correlations. We study systems of coupled quantum dots using these measures.

We study the discord of …

Resonant Light Scattering From Semiconductor Quantum Dots, Kumarasiri Konthasinghe

USF Tampa Graduate Theses and Dissertations

In this work, resonant laser spectroscopy has been utilized in two major projects --resonance fluorescence measurements in solid-state quantum-confined nanostructures and laser-induced fluorescence measurements in gases. The first project focuses on studying resonant light-matter interactions in semiconductor quantum dots "artificial atoms" with potential applications in quantum information science. Of primary interest is the understanding of fundamental processes and how they are affected by the solid-state matrix. Unlike atoms, quantum dots are susceptible to a variety of environmental influences such as phonon scattering and spectral diffusion. These interactions alter the desired properties of the scattered light and hinder uses in certain …

Quantum Enigma Machine: Experimentally Demonstrating Quantum Data Locking, Daniel J. Lum, John C. Howell, M. S. Allman, Thomas Gerrits, Varun B. Verma, Sae Woo Nam, Cosmo Lupo, Seth Lloyd

Mathematics, Physics, and Computer Science Faculty Articles and Research

Shannon proved in 1949 that information-theoretic-secure encryption is possible if the encryption key is used only once, is random, and is at least as long as the message itself. Notwithstanding, when information is encoded in a quantum system, the phenomenon of quantum data locking allows one to encrypt a message with a shorter key and still provide information-theoretic security. We present one of the first feasible experimental demonstrations of quantum data locking for direct communication and propose a scheme for a quantum enigma machine that encrypts 6 bits per photon (containing messages, new encryption keys, and forward error correction bits) …

Photonicstd-2d: Modeling Light Scattering In Periodic Multilayer Photonic Structures, Alexey Bondarev, Shaimaa Azzam, Zhaxylyk Kudyshev, Alexander V. Kildishev

The Summer Undergraduate Research Fellowship (SURF) Symposium

Efficient modeling of electromagnetic processes in optical and plasmonic metamaterials is important for enabling new and exciting ways to manipulate light for advanced applications. In this work, we put together a tool for numerical simulation of propagation of normally incident light through a nanostructured multilayer composite material. The user builds a unit cell of a given material layer-by-layer starting from a substrate up to a superstrate, splitting each layer further into segments. The segments are defined by width and material -- dielectric, metal or active medium. Simulations are performed with the finite difference time domain (FDTD) method. A database of …

Quantum And Classical Optics–Emerging Links, Joseph H. Eberly, Xiao-Feng Qian, Asma Al Qasimi, Hazrat Ali, M. A. Alonso, R Gutiérrez-Cuevas, Bethany Little, John C. Howell, Tanya Malhotra, A. N. Vamivakas

Mathematics, Physics, and Computer Science Faculty Articles and Research

Quantum optics and classical optics are linked in ways that are becoming apparent as a result of numerous recent detailed examinations of the relationships that elementary notions of optics have with each other. These elementary notions include interference, polarization, coherence, complementarity and entanglement. All of them are present in both quantum and classical optics. They have historic origins, and at least partly for this reason not all of them have quantitative definitions that are universally accepted. This makes further investigation into their engagement in optics very desirable. We pay particular attention to effects that arise from the mere co-existence of …

Spontaneous Parametric Down Conversion Of Photons Through Β-Barium Borate, Luke Horowitz

Physics

An apparatus for detecting pairs of entangled 405nm photons that have undergone Spontaneous Parametric Down Conversion through β-Barium Borate is described. By using avalanche photo-diodes to detect the low-intensity converted beam and a coincidence module to register coincident photons, it is possible to create an apparatus than can be used to perform quantum information experiments under a budget appropriate for an undergraduate physics lab.

Zncdmgse As A Materials Platform For Advanced Photonic Devices: Broadband Quantum Cascade Detectors And Green Semiconductor Disk Lasers, Joel De Jesus

Dissertations, Theses, and Capstone Projects

The ZnCdMgSe family of II-VI materials has unique and promising characteristics that may be useful in practical applications. For example they can be grown lattice matched to InP substrates with lattice matched bandgaps that span from 2.1 to 3.5 eV, they can be successfully doped n-type, have a large conduction band offset (CBO) with no intervalley scattering present when strained, they have lower average phonon energies, and the InP lattice constant lies in the middle of the ZnSe and CdSe binaries compounds giving room to experiment with tensile and compressive stress. However they have not been studied in detail for …

Beyond Conventional C-Plane Gan-Based Light Emitting Diodes: A Systematic Exploration Of Leds On Semi-Polar Orientations, Morteza Monavarian

Theses and Dissertations

Despite enormous efforts and investments, the efficiency of InGaN-based green and yellow-green light emitters remains relatively low, and that limits progress in developing full color display, laser diodes, and bright light sources for general lighting. The low efficiency of light emitting devices in the green-to-yellow spectral range, also known as the “Green Gap”, is considered a global concern in the LED industry. The polar c-plane orientation of GaN, which is the mainstay in the LED industry, suffers from polarization-induced separation of electrons and hole wavefunctions (also known as the “quantum confined Stark effect”) and low indium incorporation efficiency that …

Device-Independent Quantum Key Distribution With Generalized Two-Mode Schrödinger Cat States, Curtis J. Broadbent, Kevin Marshall, Christian Weedbrook, John C. Howell

Mathematics, Physics, and Computer Science Faculty Articles and Research

We show how weak nonlinearities can be used in a device-independent quantum key distribution (QKD) protocol using generalized two-mode Schrödinger cat states. The QKD protocol is therefore shown to be secure against collective attacks and for some coherent attacks. We derive analytical formulas for the optimal values of the Bell parameter, the quantum bit error rate, and the device-independent secret key rate in the noiseless lossy bosonic channel. Additionally, we give the filters and measurements which achieve these optimal values. We find that, over any distance in this channel, the quantum bit error rate is identically zero, in principle, and …

Analyzing Major Challenges Of Wind And Solar Variability In Power Systems, Falko Ueckerdt, Robert Brecha, Gunnar Luderer

Physics Faculty Publications

Ambitious policy targets together with current and projected high growth rates indicate that future power systems will likely show substantially increased generation from renewable energy sources. A large share will come from the variable renewable energy (VRE) sources wind and solar photovoltaics (PV); however, integrating wind and solar causes challenges for existing power systems. In this paper we analyze three major integration challenges related to the structural matching of demand with the supply of wind and solar power: low capacity credit, reduced utilization of dispatchable plants, and over-produced generation. Based on residual load duration curves we define corresponding challenge variables …

Spin-Dependent Two-Color Kapitza-Dirac Effects, Scot Mcgregor, Wayne Cheng-Wei Huang, Herman Batelaan, Bradley Allan Shadwick

Department of Physics and Astronomy: Faculty Publications

In this paper we present an analysis of the spin behavior of electrons propagating through a laser field. We present an experimentally realizable scenario in which spin-dependent effects of the interaction between the laser and the electrons are dominant. The laser interaction strength and incident electron velocity are in the nonrelativistic domain. This analysis may thus lead to novel methods of creating and characterizing spin-polarized nonrelativistic femtosecond electron pulses.