Optics Commons^™

Applications Of The Negatively-Charged Silicon Vacancy Color Center In Diamond, Forrest A. Hubert

Optical Science and Engineering ETDs

The spatial resolution and fluorescence signal amplitude in stimulated emission depletion (STED) microscopy is limited by the photostability of available fluorophores. Here, we show that negatively-charged silicon vacancy (SiV) centers in diamond are promising fluorophores for STED microscopy, owing to their photostable, near-infrared emission and favorable photophysical properties. A home-built pulsed STED microscope was used to image shallow implanted SiV centers in bulk diamond at room temperature. We performed STED microscopy on isolated SiV centers and observed a lateral full-width-at-half-maximum spot size of 89 ± 2 nm, limited by the low available STED laser pulse energy (0.4 nJ). For a …

Mid-Ir Optical Refrigeration And Radiation Balanced Lasers, Saeid Rostami

Optical Science and Engineering ETDs

This dissertation reports recent advances in mid-infrared (mid-IR) optical refrigeration and Radiation Balanced Lasers (RBLs). The first demonstration of optical refrigeration in Ho:YLF and Tm:YLF crystals as promising mid-IR laser cooling candidates is reported. Room temperature laser cooling efficiency of Tm- and Ho-doped crystals at different excitation polarization is measured and their external quantum efficiency and background absorption are extracted. Complete characterization of laser cooling samples is obtained via performing detailed low-temperature spectroscopic analysis, and their minimum achievable temperature as well as conditions to achieve laser cooling efficiency enhancement in mid-IR are investigated. By developing a Thulium-doped fiber amplifier, seeded …

Integrated Chirped-Grating Spectrometer-On-A-Chip, Shima Nezhadbadeh

Optical Science and Engineering ETDs

In this dissertation we demonstrate a new structure based on waveguide coupling atop a silicon wafer using a chirped grating to provide the dispersion that leads to a high-resolution, compact, fully integrable and CMOS-compatible spectrometer. Light is both analyzed and detected in a single, completely monolithic component which enables realizing a high-resolution portable spectrometer with an extremely compact footprint. The structure is comprised of a SiO₂/Si₃N₄/SiO₂ waveguide on top of a silicon wafer. Grating regions are fabricated on the top cladding of the waveguide. The input light is incident on a chirped grating …

Near-Field And Far-Field Microscopic And Spectroscopic Characterizations Of Coupled Plasmonic, Excitonic And Polymeric Materials, Chih-Feng Wang

Optical Science and Engineering ETDs

The properties of localized surface plasmons (LSP) have been broadly utilized for chemical sensing, surface enhanced Raman spectroscopy, biomedical imaging and photothermal treatments. By exploiting well-established plasmonic effects, the spectroscopic investigation of intriguing quantum phenomena, such as excitonic interband and intersubband (ISB) transitions in semiconductor heterostructures, was examined and extended in both far- and near-field optical measurements. For far-field characterization, we used colloidal plasmonic Au nanorods (AuNRs) to increase the quantum efficiency of InGaAs/GaAs single quantum well. By analyzing the temperature-dependent photoluminescence enhancement as a function of GaAs capping layer thickness, we attributed the mechanism of the LSP enhancement to …

Electromagnetic Analysis Of Bidirectional Reflectance From Roughened Surfaces And Applications To Surface Shape Recovery, Julian Antolin Camarena

Physics & Astronomy ETDs

Scattering from randomly rough surfaces is a well-established sub area of electrodynamics. There remains much to be done since each surface and optical processes that may occur in within the scattering medium, and countless other scenarios, is different. There are also illumination models that describe lighting in a scene on the macroscopic scale where geometrical optics can be considered adequate. Of particular interest for us is the intersection of the physical scattering theories and the illumination models. We present two contributions: 1) A minimum of two independent images are needed since any opaque surface can be uniquely specified in terms …

Tailored Frequency Comb Structures And Their Sensing Applications, James Hendrie

Optical Science and Engineering ETDs

The focus of this dissertation is the development and investigation of nested cavity mode-locked lasers and their resultant tailored frequency combs. A nested cavity is made up of two cavities, known as parents. One parent is a larger, active, 100MHz Ti:Saph oscillator and the other is a smaller, passive, 7GHz Fabry-Perot Etalon (FPE). Unlike standard frequency combs that are continuous, a tailored comb’s teeth are distributed in equally spaced groups where the center of each group corresponds to the resonance of the FPE and the side bands are determined by the resonances of the Ti:Saph. This unique coupling of the …

Symmetry And Dopant Diffusion In Inverted Nanopyramid Arrays For Thin Crystalline Silicon Solar Cells, Seok Jun Han

Chemical and Biological Engineering ETDs

In this dissertation, we enhance the efficiency of thin flexible monocrystalline silicon solar cells by breaking symmetry in light trapping nanostructures and improving homogeneity in dopant concentration profile. These thin cells are potentially less expensive than conventional thick silicon cells by using less silicon material and making the cells more convenient to be handled when supported on polymer films. Moreover, these cells are widely applicable due to their flexibility and lightweight. However, for high efficiencies, these cells require effective light trapping and charge collection. We achieve these in cells based on 14-mm-thick free-standing silicon films with light-trapping arrays of nanopyramidal …

Topics In Three-Dimensional Imaging, Source Localization And Super-Resolution, Zhixian Yu

Physics & Astronomy ETDs

The realization that twisted light beams with helical phasefronts could carry orbital angular momentum (OAM) that is in excess of the photon's spin angular momentum (SAM) has spawned various important applications. One example is the design of novel imaging systems that achieve three-dimensional (3D) imaging in a single snapshot via the rotation of point spread function (PSF).

Based on a scalar-field analysis, a particular simple version of rotating PSF imagery, which was proposed by my advisor Dr. Prasad, furnishes a practical approach to perform 3D source localization using a spiral phase mask that generates a combination of Bessel vortex beams. …

Generation And Use Of Femtosecond, Gigawatt, Near Infrared Laser Pulses From An Amplified, Mode-Locked, Ti:Sapphire Laser, David Anthony Valdés

Optical Science and Engineering ETDs

This work modeled the early to middle successes achieved in the field of ultrafast, high peak power optics, beginning with the work of Nobel Prize winners Donna Strickland and Gérard Mourou in 1985. In our work, 100 fs light pulses of around 800 nm were generated by a Ti:Sapphire oscillator, then amplified to approximately 30 GW peak power using a chirped pulse amplification system that included regenerative and multi-pass amplifiers. As a verification of our pulses having high peak powers and ultrashort durations, they were then used to strike water, glass, and a Kerr Cell. Supercontinuum generation was observed as …

Transverse Anderson Localization In Optical Fibers: High-Quality Wave Transmission And Novel Lasing Applications, Behnam Abaie

Optical Science and Engineering ETDs

In this dissertation, transverse Anderson localization (TAL) of light mediated by disordered optical fibers is exploited for high-quality optical wave transmission and novel random lasing applications. En route, we first establish a powerful numerical platform for detailed investigation of TAL optical fibers (TALOF). Our approach is based on a modal perspective as opposed to beam propagation method (BPM) which was primarily used in the previous studies of TAL in disordered optical fibers. The versatile numerical tools developed in our simulations result in a potent methodology for simulation of TALOFs; the result is a fast and effective algorithm which can be …

Genetic Algorithm Design Of Photonic Crystals For Energy-Efficient Ultrafast Laser Transmitters, Troy A. Hutchins-Delgado

Shared Knowledge Conference

Photonic crystals allow light to be controlled and manipulated such that novel photonic devices can be created. We are interested in using photonic crystals to increase the energy efficiency of our semiconductor whistle-geometry ring lasers. A photonic crystal will enable us to reduce the ring size, while maintaining confinement, thereby reducing its operating power. Photonic crystals can also exhibit slow light that will increase the interaction with the material. This will increase the gain, and therefore, lower the threshold for lasing to occur. Designing a photonic crystal for a particular application can be a challenge due to its number of …

Combined High-Speed Single Particle Tracking Of Membrane Proteins And Super-Resolution Of Membrane-Associated Structures, Hanieh Mazloom Farsibaf, Keith A. Lidke

Shared Knowledge Conference

Many experiments have shown that the diffusive motion of lipids and membrane proteins are slower on the cell surface than those in artificial lipid bilayers or blebs. One hypothesis that may partially explain this mystery is the effect of the cytoskeleton structures on the protein dynamics. A model proposed by Kusumi [1] is the Fence-Picket Model which describes the cell membrane as a set of compartment regions, each ~ 10 to 200 nm in size, created by direct or indirect interaction of lipids and proteins with actin filaments just below the membrane. To test this hypothesis, we have assembled a …

Charge Transfer Plasmon Resonances In Metallic Nanorod-Film Systems, Paul J. Gieri

Shared Knowledge Conference

Understanding how the plasmonic response of colloidally grown metallic nanostructures changes when coupled to a metallic film is an important research problem with significant consequences for a number of applications such as sensing, solar energy harvesting, spectroscopy, and photochemistry, to name a few. In this work we investigate, both through experimental and theoretical approaches, the optical response of ligand coated gold nanorods and their interaction with gold films. We find that the scattering response of these systems is dominated by a charge transfer plasmon, in which charge flows between the particle and film. Additionally, we show that the characteristics of …

Pulsed Fiber Optics Lasers As Highly Sensitive Sensors, Hanieh Afkhamiardakani

Shared Knowledge Conference

An interferometer or resonator is a device in which optical beams of specific frequencies circulate with minimal losses. These losses are completely compensated by the gain inside a laser resonator. A small perturbation introduced inside the laser can affect its frequency, which in turns becomes a metric of that perturbation. The perturbation is usually caused by an electric or magnetic field, rotation, acceleration, nonlinear index of refraction etc. Tiny changes of optical frequency are monitored by superimposing the laser field and a reference field (from the same laser) on a detector. This technique requires creating a laser in which two …

Novel Compact Narrow-Linewidth Mid-Infrared Lasers For Sensing Applications, Behsan Behzadi

Optical Science and Engineering ETDs

The mid-infrared (2-14 μm) spectral region contains the strong absorption lines of many important molecular species, which make this region crucial for several well-know applications such as spectroscopy, chemical and biochemical sensing, security, and industrial monitoring. To fully exploit this region through absorption spectroscopic techniques, compact and low-cost narrow-linewidth (NLW) mid-infrared (MIR) laser sources are of primary importance.

This thesis is focused on three novel compact NLW MIR lasers: demonstration and characterization of a new glass-based spherical microlaser, investigation of the performance of a novel fiber laser, and the design of a monolithic laser on a silicon chip. Starting with …

Dispersive Quantum Interface With Atoms And Nanophotonic Waveguides, Xiaodong Qi

Physics & Astronomy ETDs

Strong coupling between atoms and light is critical for quantum information processing and precise sensing. A nanophotonic waveguide is a promising platform for realizing an atom-light interface that reaches the strong coupling regime. In this dissertation, we study the dispersive response theory of the nanowaveguide system as the means to create an entangling atom-light interface, with applications to quantum non-demolition (QND) measurement and spin squeezing.

We calculate the dyadic Green's function, which determines the scattering of light by atoms in the presence of a nanowaveguide, and thus the phase shift and polarization rotation induced on the guided light. The Green's …

An Exploration Of The Optical Detection Of Ionizing Radiation Utilizing Modern Optics Technology, Sean D. Fournier, Adam Hecht, Cassiano De Oliveira, Jeffrey B. Martin, Richard K. Harrison, Charles Potter

Nuclear Engineering ETDs

Modern ultraviolet (UV) cameras, when combined with UV-transmitting lenses/filter arrangements, can be used to detect radiation dose in air. Ionizing radiation excites nitrogen molecules in ambient air, the resulting decay includes weak emission of ultraviolet photons. Previous work has proven this phenomenon is detectable using highly-sensitive electronically cooled cameras traditionally used in astronomy for low-background imaging. While the ability to detect the presence of radiation (i.e. qualitative measurement) has been demonstrated at Sandia National Laboratories, there are several challenges in correlating images to known dose-fields (quantitative measurement). These challenges include: a low signal to background ratio, interferences due to electronic …

Studies Of Light Generation With Four-Wave Mixing In A Cold Atomic Ensemble, Andrew Ferdinand

Physics & Astronomy ETDs

Correlated light generated from atomic ensembles can have a central role in prominent quantum information protocols, such as long-distance quantum communication. Here we present our studies on three topics involving the generation of correlated light with four-wave mixing (FWM) in a cold atomic ensemble for applications in quantum communications with high capacity. We experimentally investigate the generation of light with seeded FWM in cold cesium atoms and the time correlations of photon pairs generated with spontaneous FWM. We theoretically investigate the correlations in orbital angular momentum of photon pairs generated with spontaneous FWM for a range of experimental geometries. These …

High Precision Refractive Index Measurement Techniques Applied To The Analysis Of Neutron Damage And Effects In Caf2 Crystals, Joseph P. Morris Ph.D.

Nuclear Engineering ETDs

Neutron irradiation damages material by atomic displacements. The majority of these damage regions are microscopic and difficult to study, though they can cause a change in density and thus a change in refractive index in transparent materials. This work utilized CaF₂ crystals to track refractive index change based on neutron radiation dose. High precision refractive index measurements were performed utilizing a nested-cavity mode-locked laser where the CaF₂ crystal acted as a Fabry-Pérot Etalon (FPE). By comparing the repetition rate of the cavity and the repetition rate of the FPE, refractive index change was determined. Following several irradiation experiments, …

Synchronous Generation And Coherent Control Of Extreme Wavelength Radiation And Ultrafast Spectroscopy, Aram Gragossian

Optical Science and Engineering ETDs

Recent progress in ultrafast laser science has made it possible to synthesize and control complex electromagnetic waveforms down to sub-femtosecond timescales. These tailored ultrashort laser pulses can generate coherent bursts of electromagnetic radiation in the extreme ultraviolet (XUV) and terahertz spectral regions with durations reaching the attosecond regime in the XUV region. This is accomplished by coherently controlling electronic motion in gas plasma targets. With these novel radiation sources, ultrafast time-resolved spectroscopy can be performed on a large variety of materials. Knowledge of the spectral phase of an ultrashort pulse is crucial for many applications. There are a variety of …

Novel Concepts In Semiconductor Disk Lasers, Zhou Yang

Optical Science and Engineering ETDs

Optically-pumped semiconductor disk lasers (SDLs) have received much attention in recent years for a myriad of applications requiring intracavity access, good beam quality, wavelength versatility, and high output powers. The traditional scheme of these lasers feature a semiconductor distributed Bragg reflector (DBR) integrated with the active region, together forming an active mirror in an external free-space cavity. The active mirror component is fabricated by either epitaxial growth or post-growth processing. This places certain restrictions on SDL design, as material system choices become limited. It further viii hinders laser performance with regard to its thermal management and laser bandwidth (tuning range). …

Scatterometry Of 50 Nm Half Pitch Features, Ruichao Zhu

Optical Science and Engineering ETDs

Metrology technologies are an essential adjunct to Integrated Circuit (I.C.) Semiconductor manufacturing. Scatterometry, an optical metrology, was chosen to measure 50 nm half pitch feature structures. A bread-board scatterometry system has been assembled to provide a non-contact, non-destructive, accurate and flexible measurement. A real-time, on-line scatterometry system has also been demonstrated and proven to provide a high throughput measurement.

Three different types of samples have been measured using the scatterometry setup. The wire-grid polarizer (WGP) sample has been made by Jet and Flash Nanoimprint Lithography with ~100 nm pitch and ~50 nm wide ~200 nm tall Al gratings on fused …