Optics Commons^™

Algorithmic Sculpting Of Complex Fused Silica Surfaces For Nondestructive, Mode-Matched Cavity Quantum Electrodynamics: Adaptive Co2 Milling And Simulation-Guided Ultrafast Inscription, From Fiber Fabry-Perot Cavities To Monolithic Architectures, Meagan E. Parker

Optical Science and Engineering ETDs

Quantum sensors achieve exceptional measurement sensitivity through coherent, well-isolated quantum systems, but practical deployment is hindered by destructive readouts that require repeated state preparation and create long system dead times. Optical cavities enable continuous, nondestructive measurements with minimal back-action, yet integrating high-finesse cavities into scalable quantum devices remains limited by existing fabrication methods. To overcome these constraints, an adaptive CO₂ laser-milling platform was developed. Guided by glass thermodynamics and melt dynamics, this closed-loop system uses in-situ phase-shifting interferometry to sculpt complex fused-silica surfaces with sub-nanometer root-mean-square roughness. The platform was validated by fabricating extended-length fiber Fabry–Pérot cavities and monolithic micro-cavity …

Non-Traditional Rare-Earth-Doped Oxide Glass As A Gain Medium, Jared S. Tolliver

Optical Science and Engineering ETDs

There is a need for mid-infrared(MIR) lasers in defense, medical, and environmental monitoring. A large part of this technological development is the study of gain media. One class of materials of special interest is glasses with a low maximum phonon energy. These have the fiberization and broad spectral features of glass, whereas glasses with high maximum phonon energy exhibit higher rates of multi-phonon relaxation and can be opaque in the MIR, both of which are detrimental to laser operation. Recent advances in container-less processing have allowed for the study of new glasses that aren’t possible with conventional fabrication techniques. One …

Optical Nuclear Spin Detection In Diamond And Varifocal Metasurface Optics, Maxwell D. Aiello

Physics & Astronomy ETDs

This dissertation presents two experimental investigations at the intersection of quantum sensing and precision optical instrumentation. The primary project demonstrates optically detected nuclear magnetic resonance (NMR) of ¹³C nuclear spins in diamond, using state-selective Landau-Zener transitions under microwave frequency sweeping to bidirectionally transfer spin polarization between nitrogen-vacancy (NV) electron spins and remote ¹³C nuclear spins. This enables optical polarization and readout of large ensembles of polarized nuclear spins at low magnetic fields and room temperature, with spin dephasing times limited by longitudinal relaxation of nearby NV electron spins. The secondary project reports the design, fabrication, and characterization of …

Design, Fabrication, And Characterization Of Silicon Nitride Microresonator Optical Frequency Combs, Lala Rukh

Optical Science and Engineering ETDs

Optical frequency combs consist of equidistant optical frequencies and have numerous applications ranging from optical metrology to medical diagnostics. Initially, frequency combs were based on bulky mode-locked lasers, but advancements in integrated photonics enabled the generation of frequency combs in chip-scale resonators (microcombs) using Kerr nonlinearity. These miniaturized systems present various challenges, including increased propagation losses, enhanced thermal effects, and the extension of microcombs to visible wavelengths. In this dissertation, I will focus on addressing these challenges in silicon nitride (SiN) resonators. First, this thesis focuses on the fabrication of high-Q SiN resonators and the impact of fabrication parameters on …

Volumetric Imaging Of Cellular Dynamics Using Light-Sheet Microscopy: From Subcellular Structures To Whole Organisms, Md Nasful Huda Prince

Optical Science and Engineering ETDs

Advancing biomedical imaging requires platforms that combine high-resolution, speed, and stability across biological scales. This dissertation presents three innovations designed to address limitations of conventional light-sheet and oblique plane imaging. First, we introduce Reflected Inline Detection in Epi-Oblique Plane Microscopy (RIDE-OPM), a compact and drift-resistant system that eliminates a tertiary detection path while maintaining alignment flexibility, enabling robust long-term live imaging. Second, we present a high-speed Axially Swept Light-Sheet Microscopy (ASLM) platform for cleared tissues, using dual foci and synchronized sweeping to achieve isotropic sub-micron resolution at up to 40 frames-per-second, a fourfold improvement over standard ASLM. Integrated with a …

Phase Nanoscopy With Correlated Frequency Combs, Xiaobing Zhu

Optical Science and Engineering ETDs

In this dissertation a sensing method applying to any physical quantity that modifies optical phase is developed. Two pulses are produced inside a synchronously pumped Optical Parametric Oscillator, generating two identical, undistinguishable frequency combs. The physical quantity to be measured applies a small phase shift/round trip to one of the pulses, resulting in a frequency shift of the corresponding comb. The latter frequency is measured as a beat by interfering the two combs on a detector. A world record resolution, close to the quantum limit, of 0.033 nanoradian (corresponding to 0.006 fm in displacement) is achieved. A detailed analysis of …

Advancing Diamond Quantum Sensors: Isotropic Flux Concentrators And Phase Noise Mitigation, Maziar Saleh Ziabari

Optical Science and Engineering ETDs

Two methods for improving the sensitivity of nitrogen vacancy quantum sensors in diamond are explored. First, by passively concentrating the magnetic flux, three orthogonally oriented ferrite truncated cone pairs amplify the field isotropically by 19 times, allowing measurement of Earth's field without a bias field and increasing sensitivity. Through thorough analysis, modeling and tuning a novel 3-dimensional flux concentrator system, we achieve a fractional standard deviation of less than 1% anisotropy and quantify minimal deadzones and ambient temperature-limited variations below 40 nT/hour. Second, we characterize, model and calculate phase noise in NV experiments, which in NV sensors is effectively indistinguishable …

Yb:Ylf Optical Cryocoolers: Saturation Effects, Pump Management, Robust Thermometry, And Novel Architectures, Jackson Kock

Optical Science and Engineering ETDs

Solid-state optical refrigeration using anti-Stokes fluorescence offers a compact, vibration-free route to cryogenic cooling. This dissertation advances ytterbium-doped yttrium lithium fluoride (Yb:YLF) refrigerators, achieving a world record payload cooling temperature of 124 K by addressing key limitations due to absorption saturation. An expanded theoretical model incorporating saturation effects enables accurate predictions of cooling performance under high pump intensities. To improve pump control, a modeling framework for astigmatic Herriott cells was developed, revealing how beam clipping and intensity impact coupling efficiency. A novel fluorescence-based thermometry method was also established, providing accurate, orientation-independent temperature sensing by overcoming reabsorption and crystal orientation. Finally, …

Super-Resolution Magnetic Microscopy And Earth’S Field Magnetometry With Color Centers In Diamond, Nazanin Mosavian

Optical Science and Engineering ETDs

In recent years, the negatively charged nitrogen- vacancy (NV) center has emerged as a promising solid-state color center capable of measuring magnetic fields with high sensi- tivity and spatial resolution under ambient conditions. In this thesis I will discuss how we perform super resolution magnetic microscopy and acquire magnetic field images of nanoparticle samples at 100 nm resolution. I will explain how 3D flux concentrators increase magnetic field amplitude and allows us to measure vector component magnetic fields as low as 50 µT with a diamond magnetometer, without the use of an additional bias magnetic field. I also describe how …

Exploration Of Semiconductor Gain Medium, Resonator, Pump, And Frequency Stabilization For Laser Guide Star Applications, Mingyang Zhang

Optical Science and Engineering ETDs

Laser Guide Star (LGS) systems are essential for adaptive optics in ground-based astronomical observation. This dissertation demonstrates the feasibility of semiconductor-based LGS systems using the membrane external-cavity surface-emitting laser (MECSEL) platform, employing multiple quantum wells. Various laser cavity configurations were analyzed through simulations and experiments. The in-well pumping method was explored to reduce the quantum defect and address thermal limitations. Multi-pass pumping schemes were designed with Zemax modeling and demonstrated experimentally. To simplify multi-pass pumping, the hybrid-MECSEL (H-MECSEL) design was introduced. COMSOL modeling studied thermal management and thermal lensing effect.

The H-MECSEL achieved approximately 30 W of output power at …

Volumetric Imaging Using The Pupil-Matched Remote Focusing Technique In Light-Sheet Microscopy, Sayed Hassan Dibaji Foroushani

Optical Science and Engineering ETDs

ABSTRACT

The dissertation explores innovative techniques in light sheet microscopy, a pivotal tool in biomedical imaging, to enhance its speed, resolution, and efficiency in capturing dynamic biological processes. Light sheet microscopy allows for quick 3D imaging of biological specimens ranging from cells to organs with high spatiotemporal resolution, large field-of-view, and minimal damage, making it vital for in vivo imaging.

The first project introduces a novel optical concept designed to optimize Axially Swept Light Sheet Microscopy (ASLM). This technique is crucial for imaging specimens ranging from live cells to chemically cleared organs due to its versatility across different immersion media. …

High-Power Laser Cooling And Temperature-Dependent Fluorescence Studies Of Ytterbium Doped Silica, Brian Topper

Optical Science and Engineering ETDs

Experimental observation of optical refrigeration using ytterbium doped silica glass in recent years has created a new solution for heat mitigation in high-power laser systems, nonlinear fiber experiments, integrated photonics, and precision metrology. Current efforts of different groups focus on compositional optimization, fiber fabrication, and investigating how much silica can be cooled with a laser. At the start of this work, the best effort in laser cooling ytterbium doped silica saw cooling by 6 K from room temperature. This dissertation follows the experimental efforts that culminated in the increase of this initial record by one order of magnitude. Comprehensive spectroscopic …

Super-Resolution Microscopy With Color Centers In Diamond, Forrest A. Hubert

Optical Science and Engineering ETDs

This dissertation explores the development and application of diamond color centers, specifically the silicon-vacancy (SiV) and nitrogen-vacancy (NV) centers, in super-resolution microscopy and magnetic imaging techniques. It demonstrates the potential of SiV centers as photostable fluorophores in stimulated emission depletion (STED) microscopy, with a resolution of approximately 90 nm. The research also presents a method for nanoscale magnetic microscopy using NV centers by combining charge state depletion (CSD) microscopy with optically detected magnetic resonance (ODMR) to image magnetic fields produced by 30 nm iron-oxide nanoparticles. The individual magnetic feature width reaches ~100 nm while resolving magnetic field patterns from nanoparticles …

Filaments And Their Application To Air Lasing, Spectroscopy, And Guided Discharge, Ali Rastegari

Optical Science and Engineering ETDs

Laser filamentation is a fascinating phenomenon that occurs when an intense laser beam travels through transparent materials, in particular air. At sufficiently high power (TW in the near IR, GW in the UV), instead of spreading out like a regular laser beam, something remarkable happens: the laser beam becomes tightly focused, creating a thin and intense column of light called a laser filament. Laser filamentation is characterized by two main properties: (I) a high-intensity core that remains narrow over long distances beyond the Rayleigh range and (II) a low-density plasma channel within the core. In recent years, laser filamentation has …

Femtotesla Magnetometry And Nanoscale Imaging With Color Centers In Diamond, Yaser Silani

Optical Science and Engineering ETDs

Intriguing photophysical properties of color centers in diamond make them ideal candidates for many applications from imaging and sensing to quantum networking. In the first part of this work, we have studied the silicon vacancy (SiV) centers in diamond for nanoscale imaging applications. We showed that these centers are promising fluorophores for Stimulated Emission Depletion (STED) microscopy, owing to their photostable, near-infrared emission and favorable photophysical properties. In the second part, we built a femtotesla Radio-Frequency (RF) magnetometer based on the diamond nitrogen vacancy (NV) centers and magnetic flux concentrators. We used this sensor to remotely detect Nuclear Quadrupole Resonance …

Investigation Of Gaas Double Heterostructures For Photonic Heat Engines, Nathan Giannini-Hutchin

Optical Science and Engineering ETDs

The creation of a laser cooled semiconductor device has been a long sought achievement. GaAs-based devices have emerged as a promising candidate for the realization of this goal. Efforts to improve the efficiency of such devices have enabled the material to exhibit external quantum efficiencies (EQE, a measure of the probability that an excitation leads to the emission of a photon) of 99.5\%. Despite this impressive feat, a laser coolable device remains elusive.

To investigate the obstacles to such a device, the material characteristics of GaAs-based double heterostructures (DHS) are theoretically and experimentally examined. Through this study, a GaAs $\vert$ …

Investigation Of Laser And Nonlinear Properties Of Anderson Localizing Optical Fibers, Cody Ryan Bassett

Optical Science and Engineering ETDs

In this dissertation, I investigate the possibility of lasing and nonlinear phenomena in completely solid-state transverse Anderson localizing optical fibers (TALOFs). I examine three areas within this range of topics. The research in nonlinear phenomena focuses on four-wave mixing (FWM). FWM is of high interest in TALOFs due to the fact that guided localized modes of the fiber each have different propagation constants, and thus unique possible FWM pairs can be generated from the same input pump beam. I demonstrate the generation of FWM in the TALOF by pumping it with 532 nm light into a localized mode and observing …

Ultrashort Pulse Laser Filamentation Electrical And Optical Diagnostic Comparison, James E. Wymer

Optical Science and Engineering ETDs

Results presented here examine the effect of changing gas pressure on the radio frequency (RF) emissions of an ultrashort pulse laser filament plasma and how those emissions vary longitudinally in the laser focal region. We use a WR284 rectangular waveguide with a 1.5 cm hole that allows the beam through. A 3.2 GHz microwave signal is emitted in the waveguide, and signals are received through a waveguide-to-coax antenna connected to an HP8470B Schottky diode. By enabling and disabling the 3.2 GHz signal, we measure both the self-emitted RF from a USPL filament and subsequently the degree of attenuation a filament …

Atomic Gradiometry Based On The Interference Of Microwave Optical Sidebands, Kaleb L. Campbell

Optical Science and Engineering ETDs

We describe a novel pulsed magnetic gradiometer based on the optical interference of sidebands generated using two spatially separated alkali vapor cells. The sidebands are produced with high efficiency using parametric frequency conversion of a probe beam interacting with Rubiduim 87 atoms in a coherent superposition of magnetically sensitive hyperfine ground states. First, experimental evidence of the sideband process is described for both steady-state and pulsed operation. Then, a theoretical framework is developed that accurately models sideband generation based on density matrix formalism. The gradiometer is then constructed using two spatially separated vapor cells, and a beat-note is generated. The …

Examination Of Ionization In Cesium Diode Pumped Alkali Lasers With An Ion Chamber Diagnostic, Benjamin Oliker

Optical Science and Engineering ETDs

Diode pumped alkali lasers (DPALs) are leading candidates for future high power applications, with many potential utilities for the military, aerospace, communications, and scientific diagnostics. A critical step in their development is measurement and understanding of unwanted ionization processes that occur inside the laser, which decrease efficiency, reduce the usable alkali population, and increase heat load. In this dissertation, direct measurement of the ionization rate of a cesium DPAL gain medium are made for the first time, via application of an ion chamber diagnostic. Results will demonstrate that the rate of ionization is slow compared to pump absorption, with a …

Design And Characterization Of Frequency Tripling Mirrors, Amir Khabbazi Oskouei

Optical Science and Engineering ETDs

Aperiodic stacks of dielectric low- and high-index films can be designed to enhance third-harmonic generation (THG) in reflection of near infrared laser pulses using computer optimization. Numerical and analytical results suggest that the TH energy increases rapidly with increasing number of films and the ratio of the high and low index.

Our optical matrix based THG model that takes into account the full pulse bandwidth predicts conversion efficiencies of about 7% for transform-limited Gaussian pulse bandwidths of 16 nm for mirrors with 45 layers, which exceed those expected from periodic designs. Stability against film thickness fluctuations expected from the deposition …

Intracavity Phase Interferometry Based Fiber Sensors, Luke Jameson Horstman

Optical Science and Engineering ETDs

Intracavity Phase Interferometry (IPI) is a detection technique that exploits the inherent sensitivity of a laser's frequency to the parameters of its cavity. Intracavity interferometry is orders of magnitude more sensitive than its extracavity alternatives. This dissertation improves on previous free-space proof-of-concept designs. By implementing the technique in fiber optics, using optical parametric oscillation, and investigating non-Hermitian quantum mechanics and dispersion tailoring enhancement techniques, IPI has become more applicable and sensitive. Ring and linear IPI configurations were realized in this work, both operating as bidirectional fiber optical parametric oscillators. The benefit of using externally pumped synchronous optical parametric oscillation is …

Ultrafast Spectroscopy Of Air Lasing In Filaments, Brian Robert Kamer

Optical Science and Engineering ETDs

Filamentation in air is a phenomenon that has been extensively investigated for the last two decades. At sufficiently high intensity, even air is a nonlinear medium. These intensities are reached with ultrashort pulses (50 to 100 fs) of more than 1 J energy, which self-focus in air, reach ionizing intensities of oxygen and nitrogen, creating a plasma that defocuses the beam. The air filament is a self-induced waveguide resulting from a balance of focusing and defocusing. In this work new techniques were developed to visualize and analyze this phenomenon through its emission, in particu- lar the UV emission of the …

Interferometric Lithography- An Approach To Large Area And Cost Effective Nanopatterning, Vineeth Sasidharan

Optical Science and Engineering ETDs

In this dissertation interferometric lithography is approached in two different ways to address two important constraints of nanopatterning. One approach solves the problem of scaling up interferometric lithography to wafer scale (4 inch or larger) area. Through the second approach we have developed a nanopatterning technique based on interferometric lithography by using an inexpensive (~$100) diode laser as source, making interferometric lithography a very cost-effective technique.

Wafer-scale large-area nanopatterning was developed using an amplitude grating mask as a grating beam splitter along with spatial averaging of laser intensity by wobbling. The longitudinal and transverse coherence issues both are eased by …

Fundamental Aspects Of The Interaction Between Light And Nanostructures, Stephen Keith Sanders

Physics & Astronomy ETDs

Recent breakthroughs in nanophotonics have brought new opportunities to control and manipulate light at the nanoscale. The optical properties of metallic nanostructures have attracted particular interest because of their plasmon resonances, which couple strongly with visible light, and generate large near-field enhancements in their vicinity. In the first part of this thesis, we investigate the fundamental limits of the local density of photonic states near nanostructures by analyzing a sum rule relating its spectral integral to the field induced by a static dipole. Next, we analyze how the design of metallic nanoantennas can benefit from incorporating active materials that display …

Optimization And Characterization Of Doped Optical Fibers For Radiation Balanced Fiber Laser And Amplifier, Mostafa Peysokhan

Optical Science and Engineering ETDs

Due to the reliability, compactness, low maintenance costs, superior performance, and versatility of fiber lasers and amplifiers, they are commonly employed in scientific and directed energy applications. Among all kinds of fiber lasers and amplifiers, high-power, Yb-dopped fiber lasers and amplifiers have been extensively researched to achieve higher output powers. One of the major hindrances to achieving higher powers with adequate stability and efficiency in high power performance is heat generated in the fiber lasers and amplifiers' core. The Radiation Balanced Laser (RBL) is a viable technique for heat mitigation has been proposed by S.~Bowman in 1995. RBL technique is …

Heterogeneously Integrated Photonic Modulators And High-Volume Manufacturing Of Related Technologies, Nicholas Adam Boynton

Electrical and Computer Engineering ETDs

Silicon photonics is an attractive approach to cost-effective integrated optics due to the infrastructure established for silicon CMOS electronics. The material properties of silicon however are not ideal for optical devices. Specifically, silicon lacks the ability to easily produce light-emitting devices due to its indirect bandgap, and has a centro-symmetric crystal structure which does not facilitate the Pockels effect required for linear modulation. Conversely, lithium niobate is an excellent optical material due to its strong Pockels effect but, is a notoriously difficult material to process. One method of simultaneously overcoming the material limitations of silicon and the fabrication limitations of …

Development And Demonstration Of A Pico-Watt Calorimeter For Optical Absorption Spectroscopy, Behshad Roshanzadeh

Optical Science and Engineering ETDs

An optical calorimeter for sensitive absorption measurements of non-radiative samples at 4 K was designed, built, and demonstrated. It consists of a cryostat cooled by a commercial pulse tube (PTC) refrigerator, a measurement chamber housing the sample and thermometers, and various fiber-coupled light sources. By employing measures to damp mechanical noise from the environment and active temperature stabilization of critical components of the instrument temperature noise as low as 6 nK/√Hz at 50 mHz was achieved under 15 mW of optical excitation. An optical absorption induced temperature increase of the sample as small as 2.5 nK could be resolved using …

Generation Of Correlated Dual Frequency Combs With Pm Fiber Lasers For High-Precision Metrology, Hanieh Afkhamiardakani

Optical Science and Engineering ETDs

Intracavity Phase Interferometry (IPI) using two correlated, counter-propagating frequency combs (pulse trains) in mode-locked lasers has evolved into a powerful technique for high-precision metrology. In this method a physical parameter to be measured imparts a phase shift onto a pulse circulating in the laser cavity. Inside a laser cavity, that phase shift becomes a frequency shift (phase shift/round-trip time) applied to the whole frequency comb created by this pulse as it exits the cavity at each round-trip. This frequency shift is measured by interfering this comb with a reference comb created by a reference pulse circulating in the same mode-locked …

Radiation-Balanced Fiber Lasers And Amplifiers, Esmaeil Mobini Souchelmaei Mr

Optical Science and Engineering ETDs

Over the past decades, high-power fiber lasers and amplifiers have been extensively under research to achieve higher output powers. However, temperature rise in the core of fiber lasers and amplifiers has been a big issue in power-scaling. Radiation-balancing is a viable technique introduced for effective heat mitigation in lasers and amplifiers by S. Bowman in 1995. Radiation-balancing relies on solid-state laser cooling as a self-cooling mechanism to mitigate the generated heat in lasers and amplifiers. To implement the mentioned idea in fiber lasers and amplifiers, a set of issues should be scrutinized; (i) the amenability of silica glass (as the …