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2012

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Articles 1201 - 1220 of 1220

Full-Text Articles in Physics

Structure, Stability, Vibrational, Thermodynamic, And Catalytic Properties Of Metal Nanostructures: Size, Shape, Support, And Adsorbate Effects, Farzad Behafarid Jan 2012

Structure, Stability, Vibrational, Thermodynamic, And Catalytic Properties Of Metal Nanostructures: Size, Shape, Support, And Adsorbate Effects, Farzad Behafarid

Electronic Theses and Dissertations

Recent advances in nanoscience and technology have provided the scientific community with new exciting opportunities to rationally design and fabricate materials at the nanometer scale with drastically different properties as compared to their bulk counterparts. A variety of challenges related to nanoparticle (NP) synthesis and materials characterization have been tackled , allowing us to make more homogenous, well defined, size- and shape-selected NPs, and to probe deeper and more comprehensively into their distinct properties. In this dissertation, a variety of phenomena relevant to nanosized materials are investigated, including the thermal stability of NPs and coarsening phenomena in different environments, the …

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High-Efficiency Blue Phase Liquid Crystal Displays, Yan Li Jan 2012

High-Efficiency Blue Phase Liquid Crystal Displays, Yan Li

Electronic Theses and Dissertations

Blue phase liquid crystals (BPLCs) have a delicate lattice structure existing between chiral nematic and isotropic phases, with a stable temperature range of about 2 K. But due to short coherent length, these self-assembled nano-structured BPLCs have a fast response time. In the past three decades, the application of BPLC has been rather limited because of its narrow temperature range. In 2002, Kikuchi et al. developed a polymer stabilization method to extend the blue-phase temperature range to more than 60 K. This opens a new gateway for display and photonic applications. In this dissertation, I investigate the material properties of …

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Laser Filamentation Interaction With Materials For Spectroscopic Applications, Matthew Weidman Jan 2012

Laser Filamentation Interaction With Materials For Spectroscopic Applications, Matthew Weidman

Electronic Theses and Dissertations

Laser filamentation is a non-diffracting propagation regime consisting of an intense core that is surrounded by an energy reservoir. For laser ablation based spectroscopy techniques such as Laser Induced Breakdown Spectroscopy (LIBS), laser filamentation enables the remote delivery of high power density laser radiation at long distances. This work shows a quasiconstant filament-induced mass ablation along a 35 m propagation distance. The mass ablated is sufficient for the application of laser filamentation as a sampling tool for plasma based spectroscopy techniques. Within the scope of this study, single-shot ablation was compared with multi-shot ablation. The dependence of ablated mass on …

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Entropy And Information Causality In General Probabilistic Theories (Addendum), Howard Barnum, Jonathan Barrett, Lisa Orloff Clark, Matthew S. Leifer, Robert Spekkens, Nicholas Stepanik, Alex Wilce, Robin Wilke Jan 2012

Entropy And Information Causality In General Probabilistic Theories (Addendum), Howard Barnum, Jonathan Barrett, Lisa Orloff Clark, Matthew S. Leifer, Robert Spekkens, Nicholas Stepanik, Alex Wilce, Robin Wilke

Mathematics, Physics, and Computer Science Faculty Articles and Research

In this addendum to our paper (2010 New J. Phys. 12 033024), we point out that an elementary consequence of the strong subadditivity inequality allows us to strengthen one of the main conclusions of that paper.

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Pbr, Epr, And All That Jazz, Matthew S. Leifer Jan 2012

Pbr, Epr, And All That Jazz, Matthew S. Leifer

Mathematics, Physics, and Computer Science Faculty Articles and Research

"In the past couple of months, the quantum foundations world has been abuzz about a new preprint entitled "The Quantum State Cannot be Interpreted Statistically" by Matt Pusey, Jon Barrett and Terry Rudolph (henceforth known as PBR). Since I wrote a blog post explaining the result, I have been inundated with more correspondence from scientists and more requests for comment from science journalists than at any other point in my career. Reaction to the result amongst quantum researchers has been mixed, with many people reacting negatively to the title, which can be misinterpreted as an attack on the Born rule. …

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Review Of Elegance And Enigma: The Quantum Interviews, Matthew S. Leifer Jan 2012

Review Of Elegance And Enigma: The Quantum Interviews, Matthew S. Leifer

Mathematics, Physics, and Computer Science Faculty Articles and Research

A review of Elegance and Enigma: The Quantum Interviews, edited by Maximilian Schlosshauer.

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Everything Is Entangled, Roman V. Buniy, Stephen D. H. Hsu Jan 2012

Everything Is Entangled, Roman V. Buniy, Stephen D. H. Hsu

Mathematics, Physics, and Computer Science Faculty Articles and Research

We show that big bang cosmology implies a high degree of entanglement of particles in the universe. In fact, a typical particle is entangled with many particles far outside our horizon. However, the entanglement is spread nearly uniformly so that two randomly chosen particles are unlikely to be directly entangled with each other - the reduced density matrix describing any pair is likely to be separable.

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An Algebraic Classification Of Entangled States, Roman V. Buniy, Thomas W. Kephart Jan 2012

An Algebraic Classification Of Entangled States, Roman V. Buniy, Thomas W. Kephart

Mathematics, Physics, and Computer Science Faculty Articles and Research

We provide a classification of entangled states that uses new discrete entanglement invariants. The invariants are defined by algebraic properties of linear maps associated with the states. We prove a theorem on a correspondence between the invariants and sets of equivalent classes of entangled states. The new method works for an arbitrary finite number of finite-dimensional state subspaces. As an application of the method, we considered a large selection of cases of three subspaces of various dimensions. We also obtain an entanglement classification of four qubits, where we find 27 fundamental sets of classes.

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Characterization Of Online Archives Of Astronomical Imaging Vis-A-Vis Serendipitous Asteroids, And Their Astrometric Properties, Jean Marc Denis Jan 2012

Characterization Of Online Archives Of Astronomical Imaging Vis-A-Vis Serendipitous Asteroids, And Their Astrometric Properties, Jean Marc Denis

Electronic Theses and Dissertations

The identification of known asteroids on existing CCD pictures would allow us to obtain accurate astrometric and photometric asteroid properties. Some asteroids might have ambiguous orbital elements, thus their identification along with their exact positions on multiple picture frames could significantly improve their orbital elements. Furthermore, the possibility of identifying known asteroids on older pictures, sometimes preceding their discovery date, might allow the study of non-gravitational effects like the Yarkovsky effect. Identifying a potential Yarkovsky effect on asteroids is challenging because it is extremely weak. However, this effect cumulates with time, therefore, it is necessary to find astronomical pictures that …

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Fundamental Properties Of Functional Zinc Oxide Nanowires Obtained By Electrochemical Method And Their Device Applications, Athavan Nadarajah Jan 2012

Fundamental Properties Of Functional Zinc Oxide Nanowires Obtained By Electrochemical Method And Their Device Applications, Athavan Nadarajah

Dissertations and Theses

We report on the fundamental properties and device applications of semiconductor nanoparticles. ZnO nanowires and CdSe quantum dots were used, prepared, characterized, and assembled into novel light-emitting diodes and solar cells. ZnO nanowire films were grown electrochemically using aqueous soluble chloride-based electrolytes as precursors at temperatures below 90° C. Dopants were added to the electrolyte in the form of chloride compounds, which are AlCl3, CoCl2, CuCl2, and MnCl2. The optical, magnetic, and structural properties of undoped and transition-metal-ion doped ZnO nanowires were explored. Our results indicate that the as-grown nanowire structures have …

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Analysis Of Human Skin Tissue By Raman Microspectroscopy: Dealing With The Background, Franck Bonnier, Syed Mehmood Ali, Peter Knief, Helen Lambkin, Kathleen Flynn, Vincent Mcdonagh, Claragh Healy, Thomas Lee, Fiona Lyng, Hugh Byrne Jan 2012

Analysis Of Human Skin Tissue By Raman Microspectroscopy: Dealing With The Background, Franck Bonnier, Syed Mehmood Ali, Peter Knief, Helen Lambkin, Kathleen Flynn, Vincent Mcdonagh, Claragh Healy, Thomas Lee, Fiona Lyng, Hugh Byrne

Articles

Raman microspectroscopy is widely used for molecular characterisation of tissue samples. Nevertheless, when working in vitro on tissue sections, the presence of a broad background to the spectra remains problematic and its removal requires advanced methods for pre-processing of the data. To date, research efforts have been primarily devoted to development of techniques of statistical analysis to extract the relevant information contained in the spectra. However, few attempts have been made to understand the origin of the background and to improve the protocols used for the collection of Raman spectra that could lead to the reduction or elimination of the …

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Comparison Of Micro- And Nanoscale Fe+3-Containing (Hematite) Particles For Their Toxicological Properties In Human Lung Cells In Vitro, Kunal Bhattacharya, Eik Hoffmann, Roel Schins, Jens Boertz, Eva-Maria Prantl, Gerrit Alink, Hugh Byrne, Thomas Kuhlbusch, Qamar Rahman, Hartmut Wiggers, Christof Schulz, Elke Dopp Jan 2012

Comparison Of Micro- And Nanoscale Fe+3-Containing (Hematite) Particles For Their Toxicological Properties In Human Lung Cells In Vitro, Kunal Bhattacharya, Eik Hoffmann, Roel Schins, Jens Boertz, Eva-Maria Prantl, Gerrit Alink, Hugh Byrne, Thomas Kuhlbusch, Qamar Rahman, Hartmut Wiggers, Christof Schulz, Elke Dopp

Articles

The specific properties of nanoscale particles, large surface-to-mass ratio and highly reactive surfaces, have increased their commercial application in many fields. However, the same properties are also important for the interaction and bio-accumulation of the non-/biodegradable nanoscale particles in a biological system and are a cause for concern. Hematite (α-Fe2O3), being a mineral form of Fe(III) oxide, is one of the most used iron oxides besides magnetite. The aim of our study was the characterization and comparison of biophysical reactivity and toxicological effects of α-Fe2O3 nano- (d < 100 nm) and microscale (d < 5 μm) particles in human lung cells. Our study demonstrates that the surface reactivity of nanoscale α-Fe2O3 differs to that of microscale particles with respect to the state of agglomeration, radical formation potential, and cellular toxicity. The presence of proteins in culture medium and agglomeration were found to affect the catalytic properties of the hematite nano- and microscale particles. Both the nano- and microscale α-Fe2O3 particles were actively taken up by human lung cells in vitro, although, they were not found in the nuclei and mitochondria. …

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Nonlinear Optical Properties Of Carbon Nanotube Hybrids In Polymer Dispersions, Jun Wang, Kang-Shyang Liao, Daniel Früchtl, Ying Tian, Aisling Gilchrist , T, Nigel Alley, Enrico Andreoli, Brad Aitchison, Albert Nasibulin, Hugh Byrne, Esko I. Kauppinen, Long Zhang, Werner Blau, Seamus Curran Jan 2012

Nonlinear Optical Properties Of Carbon Nanotube Hybrids In Polymer Dispersions, Jun Wang, Kang-Shyang Liao, Daniel Früchtl, Ying Tian, Aisling Gilchrist , T, Nigel Alley, Enrico Andreoli, Brad Aitchison, Albert Nasibulin, Hugh Byrne, Esko I. Kauppinen, Long Zhang, Werner Blau, Seamus Curran

Articles

A series of double-walled carbon nanotubes (DWNTs) and multi-walled nanotubes (MWNTs) functionalized with selected organic chromophores, fluorescein 5(6)-isothiocyanate (FITC), rhodamine B isothiocyanate (RITC) and fullerene (C60) were synthesized by covalently linking these electron-donor groups to the metallic nanotubes. These versatile carbon nanotube composites show remarkable nonlinear optical (NLO) performance, due to a merged effect of the complementary NLO characteristics of the moieties of the composites. The hybrids were characterized by UV-Vis spectroscopy and Raman spectroscopy. Evidence suggests charge transfer species are formed between the chromophores and the nanotubes. The optical limiting performance of the DWNT, MWNT hybrids and …

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Diffuse Optical Imaging Using Decomposition Methods, Binlin Wu, M. Alrubaiee, W. Cai, M. Xu, S. K. Gayen Jan 2012

Diffuse Optical Imaging Using Decomposition Methods, Binlin Wu, M. Alrubaiee, W. Cai, M. Xu, S. K. Gayen

Publications and Research

Diffuse optical imaging (DOI) for detecting and locating targets in a highly scattering turbid medium is treated as a blind source separation (BSS) problem. Three matrix decomposition methods, independent component analysis (ICA), principal component analysis (PCA), and nonnegative matrix factorization (NMF) were used to study the DOI problem. The efficacy of resulting approaches was evaluated and compared using simulated and experimental data. Samples used in the experiments included Intralipid-10% or Intralipid-20% suspension in water as the medium with absorptive or scattering targets embedded.

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Fluids, Anomalies And The Chiral Magnetic Effect: A Group-Theoretic Formulation, V. Parameswaran Nair, Rashmi Ray, Shubho Roy Jan 2012

Fluids, Anomalies And The Chiral Magnetic Effect: A Group-Theoretic Formulation, V. Parameswaran Nair, Rashmi Ray, Shubho Roy

Publications and Research

It is possible to formulate fluid dynamics in terms of group-valued variables. This is particularly suited to the cases where the fluid has nonabelian charges and is coupled to nonabelian gauge fields. We explore this formulation further in this paper. An action for a fluid of relativistic particles (with and without spin) is given in terms of the Lorentz and Poincare (or de Sitter) groups. Considering the case of particles with flavor symmetries, a general fluid action which also incorporates all flavor anomalies is given. The chiral magnetic and chiral vorticity effects as well as the consequences of the mixed …

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Fluid Elasticity Can Enable Propulsion At Low Reynolds Number, Nathan C. Keim, Mike Garcia, Paulo E. Arratia Jan 2012

Fluid Elasticity Can Enable Propulsion At Low Reynolds Number, Nathan C. Keim, Mike Garcia, Paulo E. Arratia

Physics

Conventionally, a microscopic particle that performs a reciprocal stroke cannot move through its environment. This is because at small scales, the response of simple Newtonian fluids is purely viscous and flows are time-reversible. We show that by contrast, fluid elasticity enables propulsion by reciprocal forcing that is otherwise impossible. We present experiments on rigid objects actuated reciprocally in viscous fluids, demonstrating for the first time a purely elastic propulsion set by the object’s shape and boundary conditions. We describe two different artificial “swimmers” that experimentally realize this principle.

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Calibration Of The Hawc Gamma-Ray Observatory, Nathan C. Kelley-Hoskins Jan 2012

Calibration Of The Hawc Gamma-Ray Observatory, Nathan C. Kelley-Hoskins

Dissertations, Master's Theses and Master's Reports - Open

The High-Altitude Water Cherenkov (HAWC) Experiment is a gamma-ray observatory that utilizes water silos as Cherenkov detectors to measure the electromagnetic air showers created by gamma rays. The experiment consists of an array of closely packed water Cherenkov detectors (WCDs), each with four photomultiplier tubes (PMTs). The direction of the gamma ray will be reconstructed using the times when the electromagnetic shower front triggers PMTs in each WCD. To achieve an angular resolution as low as 0.1 degrees, a laser calibration system will be used to measure relative PMT response times. The system will direct 300ps laser pulses into two …

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Charge And Spin Transport In Nanoscale Junction From First Principles, Subhasish Mandal Jan 2012

Charge And Spin Transport In Nanoscale Junction From First Principles, Subhasish Mandal

Dissertations, Master's Theses and Master's Reports - Open

Recently nanoscale junctions consisting of 0-D nanostructures (single molecule) or 1-D nanostructures (semiconducting nanowire) sandwiched between two metal electrodes are successfully fabricated and characterized. What lacks in the recent developments is the understanding of the mechanism behind the observed phenomena at the level of atoms and electrons. For example, the origin of observed switching effect in a semiconducting nanowire due to the influence of an external gate bias is not yet understood at the electronic structure level. On the same context, different experimental groups have reported different signs in tunneling magneto-resistance for the same organic spin valve structure, which has …

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Direct Write Fabrication Of Waveguides And Interconnects For Optical Printed Wiring Boards, Joseph Carl Dingeldein Jan 2012

Direct Write Fabrication Of Waveguides And Interconnects For Optical Printed Wiring Boards, Joseph Carl Dingeldein

Dissertations, Master's Theses and Master's Reports - Open

Current copper based circuit technology is becoming a limiting factor in high speed data transfer applications as processors are improving at a faster rate than are developments to increase on board data transfer. One solution is to utilize optical waveguide technology to overcome these bandwidth and loss restrictions. The use of this technology virtually eliminates the heat and cross-talk loss seen in copper circuitry, while also operating at a higher bandwidth. Transitioning current fabrication techniques from small scale laboratory environments to large scale manufacturing presents significant challenges. Optical-to-electrical connections and out-of-plane coupling are significant hurdles in the advancement of optical …

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Stability Of Diphenylalanine Pepide [I.E. Peptide] Nanotube Studied By Molecular Dynamics Simulation, Haiqing Zhao Jan 2012

Stability Of Diphenylalanine Pepide [I.E. Peptide] Nanotube Studied By Molecular Dynamics Simulation, Haiqing Zhao

Dissertations, Master's Theses and Master's Reports - Open

No abstract provided.

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