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- Aerosol equilibrium; dust; chemical transport model (1)
- Aerosol transport; aerosol radiative forcing; rural New England (1)
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- Aerosols; PM2.5; MODIS (1)
- Aerosols; TRACE-P; Asia (1)
- Aerosols; radioisotopes; beryllium; stratosphere-troposphere exchange (1)
- Aerosols; special field campaigns; instrument comparison (1)
- Airborne aerosol sampling; inlet passing efficiency; tropical Pacific; PEM Tropics B (1)
- Airborne aerosol; chemical composition; intercomparison (1)
- Airborne formaldehyde measurements; tunable diode laser measurements; formaldehyde measurements at high latitudes; formaldehyde during TOPSE (1)
- Aircraft measurement intercomparison; chemistry instruments (1)
- Asian outflow; TRACE-P; aerosol-associated soluble ions; beryllium-7; lead-210 (1)
- Atmospheric chemistry; bromine; Arctic (1)
- Atmospheric composition and structure; troposphere; composition and chemistry; constituent transport and chemistry (1)
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- Beryllium-7; Be-7; 7Be; ozone; stratosphere/troposphere exchange; polar sunrise (1)
- Biomass burning (1)
- Carbonyl sulfide (OCS); carbon disulfide (CS2); Asian emissions; emission inventories (1)
- Carrington event; ice core; nitrate; sep (1)
- Chemical data assimilation; ozone; ozone and reactive nitrogen budget (1)
- Chemical transport model; lateral boundary condition; ICARTT (1)
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- Firn densification; ice sheet; mass balance; satellite altimetry (1)
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Articles 61 - 90 of 155
Full-Text Articles in Atmospheric Sciences
Biomass Burning And Pollution Aerosol Over North America: Organic Components And Their Influence On Spectral Optical Properties And Humidification Response, A D. Clarke, Cameron Mcnaughton, V Kapustin, Yohei Shinozuka, S G. Howell, Jack E. Dibb, J Zhou, B Anderson, V Brekhovskikh, H Turner, M Pinkerton
Biomass Burning And Pollution Aerosol Over North America: Organic Components And Their Influence On Spectral Optical Properties And Humidification Response, A D. Clarke, Cameron Mcnaughton, V Kapustin, Yohei Shinozuka, S G. Howell, Jack E. Dibb, J Zhou, B Anderson, V Brekhovskikh, H Turner, M Pinkerton
Earth Sciences
Thermal analysis of aerosol size distributions provided size resolved volatility up to temperatures of 400°C during extensive flights over North America (NA) for the INTEX/ICARTT experiment in summer 2004. Biomass burning and pollution plumes identified from trace gas measurements were evaluated for their aerosol physiochemical and optical signatures. Measurements of soluble ionic mass and refractory black carbon (BC) mass, inferred from light absorption, were combined with volatility to identify organic carbon at 400°C (VolatileOC) and the residual or refractory organic carbon, RefractoryOC. This approach characterized distinct constituent mass fractions present in biomass burning and pollution plumes every 5–10 min. Biomass …
Surface And Lightning Sources Of Nitrogen Oxides Over The United States: Magnitudes, Chemical Evolution, And Outflow, R C. Hudman, D J. Jacob, S Turquety, Eric M. Leibensperger, L T. Murray, S Wu, A B. Gilliland, M A. Avery, T H. Bertram, William H. Brune, Ronald C. Cohen, Jack E. Dibb, F Flocke, A Fried, J S. Holloway, J A. Neuman, R Orville, A E. Perring, Xinrong Ren, G W. Sachse, H B. Singh, Aaron L. Swanson, Paul J. Wooldridge
Surface And Lightning Sources Of Nitrogen Oxides Over The United States: Magnitudes, Chemical Evolution, And Outflow, R C. Hudman, D J. Jacob, S Turquety, Eric M. Leibensperger, L T. Murray, S Wu, A B. Gilliland, M A. Avery, T H. Bertram, William H. Brune, Ronald C. Cohen, Jack E. Dibb, F Flocke, A Fried, J S. Holloway, J A. Neuman, R Orville, A E. Perring, Xinrong Ren, G W. Sachse, H B. Singh, Aaron L. Swanson, Paul J. Wooldridge
Earth Sciences
We use observations from two aircraft during the ICARTT campaign over the eastern United States and North Atlantic during summer 2004, interpreted with a global 3-D model of tropospheric chemistry (GEOS-Chem) to test current understanding of regional sources, chemical evolution, and export of NOx. The boundary layer NOx data provide top-down verification of a 50% decrease in power plant and industry NOx emissions over the eastern United States between 1999 and 2004. Observed NOx concentrations at 8–12 km altitude were 0.55 ± 0.36 ppbv, much larger than in previous U.S. aircraft campaigns (ELCHEM, SUCCESS, SONEX) though consistent with data from …
Influence Of Lateral And Top Boundary Conditions On Regional Air Quality Prediction: A Multiscale Study Coupling Regional And Global Chemical Transport Models, Youhua Tang, Gregory R. Carmichael, Narisara Thongbongchoo, Tianfeng Chai, Larry Horowitz, R B. Pierce, J Al-Saadi, G G. Pfister, Jeffrey Vukovich, Melody A. Avery, Glen Sachse, Thomas B. Ryerson, J S. Holloway, E L. Atlas, F Flocke, Rodney J. Weber, L Gregory Huey, Jack E. Dibb, David G. Streets, William H. Brune
Influence Of Lateral And Top Boundary Conditions On Regional Air Quality Prediction: A Multiscale Study Coupling Regional And Global Chemical Transport Models, Youhua Tang, Gregory R. Carmichael, Narisara Thongbongchoo, Tianfeng Chai, Larry Horowitz, R B. Pierce, J Al-Saadi, G G. Pfister, Jeffrey Vukovich, Melody A. Avery, Glen Sachse, Thomas B. Ryerson, J S. Holloway, E L. Atlas, F Flocke, Rodney J. Weber, L Gregory Huey, Jack E. Dibb, David G. Streets, William H. Brune
Earth Sciences
The sensitivity of regional air quality model to various lateral and top boundary conditions is studied at 2 scales: a 60 km domain covering the whole USA and a 12 km domain over northeastern USA. Three global models (MOZART-NCAR, MOZART-GFDL and RAQMS) are used to drive the STEM-2K3 regional model with time-varied lateral and top boundary conditions (BCs). The regional simulations with different global BCs are examined using ICARTT aircraft measurements performed in the summer of 2004, and the simulations are shown to be sensitive to the boundary conditions from the global models, especially for relatively long-lived species, like CO …
Aerosol Major Ion Record At Mount Washington, E V. Fischer, L D. Ziemba, R. Talbot, Jack E. Dibb, Robert J. Griffin, L Husain, A N. Grant
Aerosol Major Ion Record At Mount Washington, E V. Fischer, L D. Ziemba, R. Talbot, Jack E. Dibb, Robert J. Griffin, L Husain, A N. Grant
Earth Sciences
This study examined the seasonal cycles and regional-scale meteorological controls on the chemical properties of bulk aerosols collected from 1999 to 2004 at Mount Washington, the highest peak in the northeastern United States. The concentrations of NH4+ and SO42− peaked during summer months. The pattern for aerosol NO3− was more complicated with relatively high median concentrations characterizing spring and summer months, but with major elevated events occurring during fall, winter, and spring. The seasonal relationship between NH4+ and SO42− indicated that during warmer months a mixture of (NH4) …
In Situ Evidence For Renitrification In The Arctic Lower Stratosphere During The Polar Aura Validation Experiment (Pave), Jack E. Dibb, Eric Scheuer, Melody A. Avery, G W. Sachse
In Situ Evidence For Renitrification In The Arctic Lower Stratosphere During The Polar Aura Validation Experiment (Pave), Jack E. Dibb, Eric Scheuer, Melody A. Avery, G W. Sachse
Earth Sciences
In-situ measurements of nitric acid (HNO3), ozone (O3), and nitrous oxide (N2O) were made from the NASA DC-8 during the Polar Aura Validation Experiment in January/February 2005. In the lower stratosphere (9–12.5 km, potential temperature 300–350 K) characteristic compact relationships were observed between all three gases. The ratio HNO3/O3 averaged 3.5 (±0.7) ppt/ppb. Samples with enhanced HNO3/O3 (>4.0) were most abundant under the edge of the Arctic Polar vortex in airmasses with enhanced mixing ratios of both gases (>400 ppb O3 and >2000 ppt HNO …
Observations Of Hono By Laser-Induced Fluorescence At The South Pole During Antci 2003, W Liao, A T. Case, J Mastromarino, D Tan, Jack E. Dibb
Observations Of Hono By Laser-Induced Fluorescence At The South Pole During Antci 2003, W Liao, A T. Case, J Mastromarino, D Tan, Jack E. Dibb
Earth Sciences
Observations of nitrous acid (HONO) by laser-induced fluorescence (LIF) at the South Pole taken during the Antarctic Troposphere Chemistry Investigation (ANTCI), which took place over the time period of Nov. 15, 2003 to Jan. 4, 2004, are presented here. The median observed mixing ratio of HONO 10 m above the snow was 5.8 pptv (mean value 6.3 pptv) with a maximum of 18.2 pptv on Nov 30th, Dec 1st, 3rd, 15th, 17th, 21st, 22nd, 25th, 27th and 28th. The measurement uncertainty is ±35%. The LIF HONO observations are compared to concurrent HONO observations performed by mist chamber/ion chromatography (MC/IC). The …
Summertime Ozone At Mount Washington: Meteorological Controls At The Highest Peak In The Northeast, E V. Fischer, R. Talbot, Jack E. Dibb
Summertime Ozone At Mount Washington: Meteorological Controls At The Highest Peak In The Northeast, E V. Fischer, R. Talbot, Jack E. Dibb
Earth Sciences
This study examined the synoptic and regional-scale meteorological controls on summertime O3 at Mount Washington, the highest peak (1910 m) in the northeastern United States. Analysis of air mass transport to Mount Washington was conducted for the summers of 1998–2003 using backward trajectories. Distinct patterns in air mass history were revealed using this approach that helped explain extreme variations in O3 mixing ratios. Most enhanced (≥90th percentile) and depleted (≤10th percentile) O3 events were short-lived and spread out over the summer months. Enhanced O3 events at Mount Washington were generally associated with westerly transport, while depleted …
Snow Accumulation, Surface Height Change, And Firn Densification At Summit, Greenland: Insights From 2 Years Of In Situ Observation, Jack E. Dibb, Mark Fahnestock
Snow Accumulation, Surface Height Change, And Firn Densification At Summit, Greenland: Insights From 2 Years Of In Situ Observation, Jack E. Dibb, Mark Fahnestock
Earth Sciences
Weekly measurements of surface height change were made at an accumulation forest of 100 stakes at Summit, Greenland, over a 2-year period (17 August 2000 to 8 August 2002). On average, the surface height relative to the stakes increased 64 (±4.8) cm in the first year and 65 (±5.3) cm in the second, identical to the average (65 ± 4.5 cm yr−1) previously reported for the period 1991–1995 in a similar forest 28 km to the southwest. The continuous 2-year data set indicates that the rate of surface rise was not constant, with the summers of 2001 and …
Ship-Based Nitric Acid Measurements In The Gulf Of Maine During New England Air Quality Study 2002, Jack E. Dibb, Eric Scheuer, Sallie I. Whitlow, Marcy Vozzella, Eric Williams, Brian M. Lerner
Ship-Based Nitric Acid Measurements In The Gulf Of Maine During New England Air Quality Study 2002, Jack E. Dibb, Eric Scheuer, Sallie I. Whitlow, Marcy Vozzella, Eric Williams, Brian M. Lerner
Earth Sciences
Gas phase nitric acid (HNO3) was measured at 5-min resolution on board the National Oceanographic and Atmospheric Administration (NOAA) research vessel Ronald H. Brown during the second leg (29 July to 10 August) of the New England Air Quality Study (NEAQS) 2002 cruise. A primary objective of the cruise was to improve understanding of the oxidation of NOx in, and removal of the oxidation products from, the polluted marine boundary layer east of northeastern North America. For the first 9 days of this leg the ship remained north of Cape Cod, and the cruise track did not …
Three-Dimensional Simulations Of Inorganic Aerosol Distributions In East Asia During Spring 2001, Youhua Tang, Gregory R. Carmichael, John H. Seinfeld, Donald Dabdub, Rodney J. Weber, B J. Huebert, A D. Clarke, Sergio A. Guazzotti, David A. Sodeman, Kimberly A. Prather, Itsushi Uno, Jung -Hun Woo, James J. Yienger, David G. Streets, Patricia K. Quinn, James E. Johnson, Chul-Han Song, Vicki H. Grassian, Adrian Sandu, R. Talbot, Jack E. Dibb
Three-Dimensional Simulations Of Inorganic Aerosol Distributions In East Asia During Spring 2001, Youhua Tang, Gregory R. Carmichael, John H. Seinfeld, Donald Dabdub, Rodney J. Weber, B J. Huebert, A D. Clarke, Sergio A. Guazzotti, David A. Sodeman, Kimberly A. Prather, Itsushi Uno, Jung -Hun Woo, James J. Yienger, David G. Streets, Patricia K. Quinn, James E. Johnson, Chul-Han Song, Vicki H. Grassian, Adrian Sandu, R. Talbot, Jack E. Dibb
Earth Sciences
In this paper, aerosol composition and size distributions in east Asia are simulated using a comprehensive chemical transport model. Three-dimensional aerosol simulations for the TRACE-P and ACE-Asia periods are performed and used to help interpret actual observations. The regional chemical transport model, STEM-2K3, which includes the on-line gas-aerosol thermodynamic module SCAPE II, and explicitly considers chemical aging of dust, is used in the analysis. The model is found to represent many of the important observed features. The Asian outflow during March and April of 2001 is heavily polluted with high aerosol loadings. Under conditions of low dust loading, SO2 …
A Major Regional Air Pollution Event In The Northeastern United States Caused By Extensive Forest Fires In Quebec, Canada, Linsey J. Debell, Jack E. Dibb, R. Talbot, J W. Munger, E V. Fischer, Steve Frolking
A Major Regional Air Pollution Event In The Northeastern United States Caused By Extensive Forest Fires In Quebec, Canada, Linsey J. Debell, Jack E. Dibb, R. Talbot, J W. Munger, E V. Fischer, Steve Frolking
Earth Sciences
During early July 2002, wildfires burned ∼1 × 106 ha of forest in Quebec, Canada. The resultant smoke plume was seen in satellite images blanketing the U.S. east coast. Concurrently, extremely high CO mixing ratios were observed at the Atmospheric Investigation, Regional Modeling, Analysis and Prediction (AIRMAP) network sites in New Hampshire and at the Harvard Forest Environmental Measurement Site (HFEMS) in Massachusetts. The CO enhancements were on the order of 525–1025 ppbv above low mixing ratio conditions on surrounding days. A biomass burning source for the event was confirmed by concomitant enhancements in aerosol K+, NH …
A Comparison Of Similar Aerosol Measurements Made On The Nasa P3-B, Dc-8, And Nsf C-130 Aircraft During Trace-P And Ace-Asia, K G. Moore, A D. Clarke, V Kapustin, Cameron Mcnaughton, B E. Anderson, E L. Winstead, R J. Weber, Y Ma, Y N. Lee, R. Talbot, Jack E. Dibb, T Anderson, S Dougherty, D Covert, D Rogers
A Comparison Of Similar Aerosol Measurements Made On The Nasa P3-B, Dc-8, And Nsf C-130 Aircraft During Trace-P And Ace-Asia, K G. Moore, A D. Clarke, V Kapustin, Cameron Mcnaughton, B E. Anderson, E L. Winstead, R J. Weber, Y Ma, Y N. Lee, R. Talbot, Jack E. Dibb, T Anderson, S Dougherty, D Covert, D Rogers
Earth Sciences
Two major aircraft experiments occurred off the Pacific coast of Asia during spring 2001: the NASA sponsored Transport and Chemical Evolution over the Pacific (TRACE-P) and the National Science Foundation (NSF) sponsored Aerosol Characterization Experiment-Asia (ACE-Asia). Both experiments studied emissions from the Asian continent (biomass burning, urban/industrial pollution, and dust). TRACE-P focused on trace gases and aerosol during March/April and was based primarily in Hong Kong and Yokota Air Force Base, Japan, and involved two aircraft: the NASA DC-8 and the NASA P3-B. ACE-Asia focused on aerosol and radiation during April/May and was based in Iwakuni Marine Corps Air Station, …
Carbonyl Sulfide And Carbon Disulfide: Large-Scale Distributions Over The Western Pacific And Emissions From Asia During Trace-P, Nicola J. Blake, David G. Streets, Jung -Hun Woo, Isobel J. Simpson, Jonathan Green, Simone Meinardi, Kazuyuki Kita, E L. Atlas, H Fuelberg, Glen Sachse, Melody A. Avery, S Vay, R. Talbot, Jack E. Dibb, A R. Bandy, D C. Thornton, F Sherwood Rowland, D R. Blake
Carbonyl Sulfide And Carbon Disulfide: Large-Scale Distributions Over The Western Pacific And Emissions From Asia During Trace-P, Nicola J. Blake, David G. Streets, Jung -Hun Woo, Isobel J. Simpson, Jonathan Green, Simone Meinardi, Kazuyuki Kita, E L. Atlas, H Fuelberg, Glen Sachse, Melody A. Avery, S Vay, R. Talbot, Jack E. Dibb, A R. Bandy, D C. Thornton, F Sherwood Rowland, D R. Blake
Earth Sciences
An extensive set of carbonyl sulfide (OCS) and carbon disulfide (CS2) observations were made as part of the NASA Transport and Chemical Evolution over the Pacific (TRACE-P) project, which took place in the early spring 2001. TRACE-P sampling focused on the western Pacific region but in total included the geographic region 110°E to 290°E longitude, 5°N to 50°N latitude, and 0–12 km altitude. Substantial OCS and CS2 enhancements were observed for a great many air masses of Chinese and Japanese origin during TRACE-P. Over the western Pacific, mean mixing ratios of long-lived OCS and shorter-lived CS2 …
Intercomparisons Of Airborne Measurements Of Aerosol Ionic Chemical Composition During Trace-P And Ace-Asia, Y Ma, R J. Weber, K Maxwell-Meier, D A. Orsini, Y-N Lee, B J. Huebert, S G. Howell, T H. Bertram, R. Talbot, Jack E. Dibb, Eric Scheuer
Intercomparisons Of Airborne Measurements Of Aerosol Ionic Chemical Composition During Trace-P And Ace-Asia, Y Ma, R J. Weber, K Maxwell-Meier, D A. Orsini, Y-N Lee, B J. Huebert, S G. Howell, T H. Bertram, R. Talbot, Jack E. Dibb, Eric Scheuer
Earth Sciences
As part of the two field studies, Transport and Chemical Evolution over the Pacific (TRACE-P) and the Asian Aerosol Characterization Experiment (ACE-Asia), the inorganic chemical composition of tropospheric aerosols was measured over the western Pacific from three separate aircraft using various methods. Comparisons are made between the rapid online techniques of the particle into liquid sampler (PILS) for measurement of a suite of fine particle a mist chamber/ion chromatograph (MC/IC) measurement of fine sulfate, and the longer time-integrated filter and micro-orifice impactor (MOI) measurements. Comparisons between identical PILS on two separate aircraft flying in formation showed that they were highly …
A 700 Year Record Of Southern Hemisphere Extratropical Climate Variability, Paul A. Mayewski, Kirk A. Maasch, James W.C. White, Eric J. Steig, E A. Meyerson, Ian D. Goodwin, Vin Morgan, Tas D. Van Ommen, Mark Aj Curran, Joseph M. Souney Jr, K Kreutz
A 700 Year Record Of Southern Hemisphere Extratropical Climate Variability, Paul A. Mayewski, Kirk A. Maasch, James W.C. White, Eric J. Steig, E A. Meyerson, Ian D. Goodwin, Vin Morgan, Tas D. Van Ommen, Mark Aj Curran, Joseph M. Souney Jr, K Kreutz
All Materials
Annually dated ice cores from West and East Antarctica provide proxies for past changes in atmospheric circulation over Antarctica and portions of the Southern Ocean, temperature in coastal West and East Antarctica, and the frequency of South Polar penetration of El Niño events. During the period AD 1700–1850, atmospheric circulation over the Antarctic and at least portions of the Southern Hemisphere underwent a mode switch departing from the out-of-phase alternation of multi-decadal long phases of EOF1 and EOF2 modes of the 850 hPa field over the Southern Hemisphere (as defined in the recent record by Thompson and Wallace, 2000; Thompson …
Nighttime Removal Of Nox In The Summer Marine Boundary Layer, S S. Brown, Jack E. Dibb, H Stark, M Aldener, Marcy Vozzella, Sallie I. Whitlow, E J. Williams, Brian M. Lerner, R Jakoubek, A M. Middlebrook, J A. Degouw, C Warneke, P D. Goldan, W C. Kuster, W M. Angevine, D Sueper, Patricia K. Quinn, Timothy S. Bates, James Meagher, Fred C. Fehsenfeld, A R. Ravishankara
Nighttime Removal Of Nox In The Summer Marine Boundary Layer, S S. Brown, Jack E. Dibb, H Stark, M Aldener, Marcy Vozzella, Sallie I. Whitlow, E J. Williams, Brian M. Lerner, R Jakoubek, A M. Middlebrook, J A. Degouw, C Warneke, P D. Goldan, W C. Kuster, W M. Angevine, D Sueper, Patricia K. Quinn, Timothy S. Bates, James Meagher, Fred C. Fehsenfeld, A R. Ravishankara
Earth Sciences
The nitrate radical, NO3, and dinitrogen pentoxide, N2O5, are two important components of nitrogen oxides that occur predominantly at night in the lower troposphere. Because a large fraction of NO2 reacts to form NO3 and N2O5 during the course of a night, their fate is an important determining factor to the overall fate of NOx (=NO and NO2). As a comprehensive test of nocturnal nitrogen oxide chemistry, concentrations of O3, NO, NO2, NO3, N2O5, HNO3 and a host of other relevant compounds, aerosol abundance and composition, and meteorological conditions were measured in the marine boundary layer from the NOAA research …
Constraints On The Sources Of Tropospheric Ozone From 210pb-7be-O3 Correlations, Hongyu Liu, Daniel Jacob, Jack E. Dibb, Arlene M. Fiore, Robert Yantosca
Constraints On The Sources Of Tropospheric Ozone From 210pb-7be-O3 Correlations, Hongyu Liu, Daniel Jacob, Jack E. Dibb, Arlene M. Fiore, Robert Yantosca
Earth Sciences
The 210Pb-7 Be-O3 relationships observed in three aircraft missions over the western Pacific (PEM-West A and B, TRACE-P) are simulated with a global three-dimensional chemical tracer model (GEOS-CHEM) driven by assimilated meteorological observations. Results are interpreted in terms of the constraints that they offer on sources of tropospheric ozone (O3). Aircraft observations of fresh Asian outflow show strong 210Pb-O3 correlations in September–October, but such correlations are only seen at low latitudes in February–March. Observations further downwind over the Pacific show stronger 210PbO3 correlations in February–March than in September–October. The model reproduces these results and attributes the seasonal contrast to strong …
Asian Dust Storm Events Of Spring 2001 And Associated Pollutants Observed In New England By The Atmospheric Investigation, Regional Modeling, Analysis And Prediction (Airmap) Monitoring Network, Linsey J. Debell, Marcy Vozzella, R. Talbot, Jack E. Dibb
Asian Dust Storm Events Of Spring 2001 And Associated Pollutants Observed In New England By The Atmospheric Investigation, Regional Modeling, Analysis And Prediction (Airmap) Monitoring Network, Linsey J. Debell, Marcy Vozzella, R. Talbot, Jack E. Dibb
Earth Sciences
Between 18 April and 13 May 2001, three statistically extreme dust aerosol events were observed across the entire northeastern United States. High levels of bulk aerosol water-soluble Ca2+ (range = 42–482 pptv) and PM2.5 elemental Ca (range = 19–156 pptv) were observed simultaneously at Atmospheric Investigation, Regional Modeling, Analysis and Prediction (AIRMAP) and Interagency Monitoring of Protected Visual Environments (IMPROVE) stations. On the basis of Ca2+ concentrations, the average bulk dust concentration for all events across all four AIRMAP stations was estimated to be 7.4 μg/m3. There was no evidence of dust outbreaks in North …
Relationships Between Surface And Column Aerosol Radiative Properties And Air Mass Transport At A Rural New England Site, J F. Slater, Jack E. Dibb
Relationships Between Surface And Column Aerosol Radiative Properties And Air Mass Transport At A Rural New England Site, J F. Slater, Jack E. Dibb
Earth Sciences
Chemical, physical, and radiative properties of surface and vertical column aerosols were measured at a rural site in southern New Hampshire from July 2000 to September 2001. The primary objective was to determine how intensive and extensive aerosol properties vary in air masses originating in different upwind regions. The data set also allows for an investigation of some of the relationships between surface and column aerosol properties at the site, and provides an estimate of direct radiative forcing by aerosols during the study period. Extensive properties (e.g., optical depth and chemical concentration) were at maximum values during times of south-southwest …
Intercontinental Transport Of Pollution Manifested In The Variability And Seasonal Trend Of Springtime O3 At Northern Middle And High Latitudes, Yuhang Wang, Changsub Shim, Nicola J. Blake, D R. Blake, Yunsoo Choi, Brian Ridley, Jack E. Dibb, Anthony Wimmers, Jennie Moody, F Flocke, Andrew Weinheimer, R. Talbot, Elliot Atlas
Intercontinental Transport Of Pollution Manifested In The Variability And Seasonal Trend Of Springtime O3 At Northern Middle And High Latitudes, Yuhang Wang, Changsub Shim, Nicola J. Blake, D R. Blake, Yunsoo Choi, Brian Ridley, Jack E. Dibb, Anthony Wimmers, Jennie Moody, F Flocke, Andrew Weinheimer, R. Talbot, Elliot Atlas
Earth Sciences
Observations (0–8 km) from the Tropospheric Ozone Production about the Spring Equinox (TOPSE) experiment are analyzed to examine air masses contributing to the observed variability of springtime O3 and its seasonal increase at 40°–85°N over North America. Factor analysis using the positive matrix factorization and principal component analysis methods is applied to the data set with 14 chemical tracers (O3, NOy, PAN, CO, CH4, C2H2, C3H8, CH3Cl, CH3Br, C2Cl4, CFC-11, HCFC-141B, Halon-1211, and 7Be) and one …
Uptake Of Nitrate And Sulfate On Dust Aerosols During Trace-P, C. Jordan, Jack E. Dibb, B E. Anderson, H Fuelberg
Uptake Of Nitrate And Sulfate On Dust Aerosols During Trace-P, C. Jordan, Jack E. Dibb, B E. Anderson, H Fuelberg
Earth Sciences
Aerosol data collected near Asia on the DC-8 aircraft platform during TRACE-P has been examined for evidence of uptake of NO3− and SO4= on dust surfaces. Data is compared between a sector where dust was predominant and a sector where dust was less of an influence. Coincident with dust were higher mixing ratios of anthropogenic pollutants. HNO3, SO2, and CO were higher in the dust sector than the nondust sector by factors of 2.7, 6.2, and 1.5, respectively. The colocation of dust and pollution sources allowed for the uptake of NO3 …
Chemical And Physical Properties Of Bulk Aerosols Within Four Sectors Observed During Trace-P, C. Jordan, B E. Anderson, R. Talbot, Jack E. Dibb, H Fuelberg, Charlie Hudgins, C M. Kiley, R. S. Russo, Eric Scheuer, Garry Seid, K L. Thornhill, E L. Winstead
Chemical And Physical Properties Of Bulk Aerosols Within Four Sectors Observed During Trace-P, C. Jordan, B E. Anderson, R. Talbot, Jack E. Dibb, H Fuelberg, Charlie Hudgins, C M. Kiley, R. S. Russo, Eric Scheuer, Garry Seid, K L. Thornhill, E L. Winstead
Earth Sciences
Chemical and physical aerosol data collected on the DC-8 during TRACE-P were grouped into four sectors based on back trajectories. The four sectors represent long-range transport from the west (WSW), regional circulation over the western Pacific and Southeast Asia (SE Asia), polluted transport from northern Asia with substantial sea salt at low altitudes (NNW) and a substantial amount of dust (Channel). WSW has generally low mixing ratios at both middle and high altitudes, with the bulk of the aerosol mass due to non-sea-salt water-soluble inorganic species. Low altitude SE Asia also has low mean mixing ratios in general, with the …
Aerosol Chemical Composition In Asian Continental Outflow During The Trace-P Campaign: Comparison With Pem-West B, Jack E. Dibb, R. Talbot, Eric Scheuer, Garry Seid, Melody A. Avery, H B. Singh
Aerosol Chemical Composition In Asian Continental Outflow During The Trace-P Campaign: Comparison With Pem-West B, Jack E. Dibb, R. Talbot, Eric Scheuer, Garry Seid, Melody A. Avery, H B. Singh
Earth Sciences
Aerosol associated soluble ions and the radionuclide tracers 7Be and 210Pb were quantified in 414 filter samples collected in spring 2001 from the DC-8 during the Transport and Chemical Evolution over the Pacific (TRACE-P) campaign. Binning the data into near Asia (flights from Hong Kong and Japan) and remote Pacific (all other flights) revealed large enhancements of NO3−, SO4=, C2O4=, NH4+, K+, Mg2+, and Ca2+ near Asia. The boundary layer and lower troposphere were most strongly influenced by continental …
Chemical Composition Of Asian Continental Outflow Over The Western Pacific: Results From Transport And Chemical Evolution Over The Pacific (Trace-P), R. S. Russo, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, C. Jordan, H Fuelberg, G W. Sachse, M A. Avery, S Vay, D R. Blake, N J. Blake, E L. Atlas, A Fried, S T. Sandholm, D Tan, H B. Singh, J Snow, B J. Heikes
Chemical Composition Of Asian Continental Outflow Over The Western Pacific: Results From Transport And Chemical Evolution Over The Pacific (Trace-P), R. S. Russo, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, C. Jordan, H Fuelberg, G W. Sachse, M A. Avery, S Vay, D R. Blake, N J. Blake, E L. Atlas, A Fried, S T. Sandholm, D Tan, H B. Singh, J Snow, B J. Heikes
Earth Sciences
We characterize the chemical composition of Asian continental outflow observed during the NASA Transport and Chemical Evolution over the Pacific (TRACE-P) mission during February–April 2001 in the western Pacific using data collected on the NASA DC-8 aircraft. A significant anthropogenic impact was present in the free troposphere and as far east as 150°E longitude reflecting rapid uplift and transport of continental emissions. Five-day backward trajectories were utilized to identify five principal Asian source regions of outflow: central, coastal, north-northwest (NNW), southeast (SE), and west-southwest (WSW). The maximum mixing ratios for several species, such as CO, C2Cl4, …
Large-Scale Ozone And Aerosol Distributions, Air Mass Characteristics, And Ozone Fluxes Over The Western Pacific Ocean In Late Winter/Early Spring, Edward V. Browell, Marta Fenn, Carolyn Butler, William B. Grant, Vincent G. Brackett, Jonathan Hair, Melody A. Avery, Yuanlong Hu, Reginald E. Newell, H Fuelberg, Daniel J. Jacob, Bruce E. Anderson, Elliot Atlas, D R. Blake, William H. Brune, Jack E. Dibb, A Fried, B J. Heikes, G W. Sachse, S T. Sandholm, Hanwant B. Singh, R. Talbot, S Vay, Rodney J. Weber, Karen B. Bartlett
Large-Scale Ozone And Aerosol Distributions, Air Mass Characteristics, And Ozone Fluxes Over The Western Pacific Ocean In Late Winter/Early Spring, Edward V. Browell, Marta Fenn, Carolyn Butler, William B. Grant, Vincent G. Brackett, Jonathan Hair, Melody A. Avery, Yuanlong Hu, Reginald E. Newell, H Fuelberg, Daniel J. Jacob, Bruce E. Anderson, Elliot Atlas, D R. Blake, William H. Brune, Jack E. Dibb, A Fried, B J. Heikes, G W. Sachse, S T. Sandholm, Hanwant B. Singh, R. Talbot, S Vay, Rodney J. Weber, Karen B. Bartlett
Earth Sciences
Large-scale measurements of ozone (O3) and aerosol distributions were made from the NASA DC-8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) field experiment conducted in February–April 2001. Remote measurements were made with an airborne lidar to provide O3 and multiple-wavelength aerosol backscatter profiles from near the surface to above the tropopause along the flight track. In situ measurements of O3, aerosols, and a wide range of trace gases were made onboard the DC-8. Five-day backward trajectories were used in conjunction with the O3 and aerosol distributions on each flight to …
Summary Of Measurement Intercomparisons During Trace-P, Fred Eisele, Lee Mauldin, C A. Cantrell, M Zondlo, E C. Apel, A Fried, J Walega, R E. Shetter, Barry Lefer, F Flocke, Andrew Weinheimer, M A. Avery, S Vay, G W. Sachse, J Podolske, G S. Diskin, J D. Barrick, H B. Singh, William H. Brune, H Harder, M Martinez, A R. Bandy, D C. Thornton, B J. Heikes, Y Kondo, D Riemer, S T. Sandholm, R. Talbot, Jack E. Dibb
Summary Of Measurement Intercomparisons During Trace-P, Fred Eisele, Lee Mauldin, C A. Cantrell, M Zondlo, E C. Apel, A Fried, J Walega, R E. Shetter, Barry Lefer, F Flocke, Andrew Weinheimer, M A. Avery, S Vay, G W. Sachse, J Podolske, G S. Diskin, J D. Barrick, H B. Singh, William H. Brune, H Harder, M Martinez, A R. Bandy, D C. Thornton, B J. Heikes, Y Kondo, D Riemer, S T. Sandholm, R. Talbot, Jack E. Dibb
Earth Sciences
The NASA DC-8 and P-3B aircraft flew within about a kilometer or less of each other on three occasions during the Transport and Chemical Evolution Over the Pacific (TRACE-P) campaign in order to intercompare similar measurements on the two aircraft. The first and last intercomparisons were in relatively remote marine environments during transits to and from Asia. The first began with a boundary layer measurement followed by an ascent to 3 km. The second set of intercomparisons was at a fixed altitude of about 5.2 km off the coast of Japan, also in relatively clean air. Finally, the third measurement …
Reactive Nitrogen In Asian Continental Outflow Over The Western Pacific: Results From The Nasa Transport And Chemical Evolution Over The Pacific (Trace-P) Airborne Mission, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, R. S. Russo, S T. Sandholm, D Tan, H B. Singh, D R. Blake, N J. Blake, Elliot Atlas, G W. Sachse, C. Jordan, Melody A. Avery
Reactive Nitrogen In Asian Continental Outflow Over The Western Pacific: Results From The Nasa Transport And Chemical Evolution Over The Pacific (Trace-P) Airborne Mission, R. Talbot, Jack E. Dibb, Eric Scheuer, Garry Seid, R. S. Russo, S T. Sandholm, D Tan, H B. Singh, D R. Blake, N J. Blake, Elliot Atlas, G W. Sachse, C. Jordan, Melody A. Avery
Earth Sciences
We present here results for reactive nitrogen species measured aboard the NASA DC-8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE-P) mission. The large-scale distributions total reactive nitrogen (NOy,sum = NO + NO2 + HNO3 + PAN + C1–C5alkyl nitrates) and O3 and CO were better defined in the boundary layer with significant degradation of the relationships as altitude increased. Typically, NOy,sum was enhanced over background levels of ∼260 pptv by 20-to-30-fold. The ratio C2H2/CO had values of 1–4 at altitudes up to 10 …
Be-10/Be-7 Tracer Of Atmospheric Transport And Stratosphere-Troposphere Exchange, C. Jordan, Jack E. Dibb, R C. Finkel
Be-10/Be-7 Tracer Of Atmospheric Transport And Stratosphere-Troposphere Exchange, C. Jordan, Jack E. Dibb, R C. Finkel
Earth Sciences
The 10Be/7Be ratio is a sensitive tracer of atmospheric transport and stratosphere-troposphere exchange (STE). Data from five NASA aircraft field missions (PEM: West A and B, Tropics A; SONEX; and SUCCESS) have been assembled to produce the largest data set of 10Be,7Be, and their ratio collected to date (>300 samples). Ratios near 0.60 are indicative of tropospheric air with little stratospheric influence, while higher ratios are found in stratospheric air. Samples from the lower stratosphere were all collected within 2.5 km of the tropopause and had ratios >1.27. Of these lower stratosphere samples …
Effect Of Sulfate Aerosol On Tropospheric Nox And Ozone Budgets: Model Simulations And Topse Evidence, Xuexi Tie, L K. Emmons, Larry Horowitz, Guy Brasseur, Brian Ridley, Elliot Atlas, Craig Stround, Peter Hess, Andrzej Klonecki, Sasha Madronich, R. Talbot, Jack E. Dibb
Effect Of Sulfate Aerosol On Tropospheric Nox And Ozone Budgets: Model Simulations And Topse Evidence, Xuexi Tie, L K. Emmons, Larry Horowitz, Guy Brasseur, Brian Ridley, Elliot Atlas, Craig Stround, Peter Hess, Andrzej Klonecki, Sasha Madronich, R. Talbot, Jack E. Dibb
Earth Sciences
The distributions of NOx and O3 are analyzed during TOPSE (Tropospheric Ozone Production about the Spring Equinox). In this study these data are compared with the calculations of a global chemical/transport model (Model for OZone And Related chemical Tracers (MOZART)). Specifically, the effect that hydrolysis of N2O5 on sulfate aerosols has on tropospheric NOx and O3 budgets is studied. The results show that without this heterogeneous reaction, the model significantly overestimates NOx concentrations at high latitudes of the Northern Hemisphere (NH) in winter and spring in comparison to the observations during TOPSE; …
Seasonal Distributions Of Fine Aerosol Sulfate In The North American Arctic Basin During Topse, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, Barry Lefer
Seasonal Distributions Of Fine Aerosol Sulfate In The North American Arctic Basin During Topse, Eric Scheuer, R. Talbot, Jack E. Dibb, Garry Seid, Linsey J. Debell, Barry Lefer
Earth Sciences
We used the mist chamber/ion chromatography technique to quantify fine aerosol SO4=(<2.7 μm) in the Arctic during the Tropospheric Ozone Production about the Spring Equinox Experiment (TOPSE) with about 2.5 min time resolution. Our effective sample area ranged from 50° to 86°N and 53° to 100°W. The seasonal evolution of fine aerosol sulfate in the Arctic troposphere during TOPSE was consistent with the phenomenon of Arctic haze. Arctic haze has been attributed to pollution from sources in the Arctic and pollution transported meridionally along stable isentropes into the Arctic in geographically broad but vertically narrow bands. These layers became more prevalent at higher altitudes as the season progressed toward summer, and the relevant isentropes are not held so close to the surface. Mean fine particle SO4= mixing ratios during TOPSE in February below 1000 m were elevated (112 pptv) and highly variable (between 28 and 290 pptv) but were significantly lower at higher altitudes (about 40 pptv). As the season progressed, elevated mixing ratios and higher variability were observed at higher altitudes, up to 7 km. In May, mixing ratios at the lowest altitudes declined but still remained higher than in February at all altitudes. The high variability in our measurements likely reflects the vertical heterogeneity of the wintertime …