Plasma and Beam Physics Commons^™

Characterizing Plasma With Emission Tomography-Feasibility Study On Synthetic And Experimental Data, M. Nikolić, A. Samolov, A. Godunov, L. Vušković,, S. Popović

Physics Faculty Publications

We present a feasibility study on different tomographic algorithms to overcome the issues of finite sets of projection data, limited viewing angles, and noisy data, which cause the tomographic reconstruction to be an ill-posed inversion problem. We investigated three approaches: single angle Abel inversion, two angle approach, and multiple angle 2D plasma tomography. These methods were tested on symmetric and asymmetric sample functions and on experimental results from a supersonic flowing argon microwave plasma sustained in a cylindrical quartz cavity. The analysis focused on the afterglow region of the microwave flow where a plasmoid-like formation was observed. We investigated the …

Characterization Of Argon And Ar/Cl2 Plasmas Used For The Processing Of Niobium Superconducting Radio-Frequency Cavities, Jeremy J. Peshl

Physics Theses & Dissertations

The plasma processing of superconducting radio-frequency (SRF) cavities has shown significant promise as a complementary or possible replacement for the current wet etch processes. Empirical relationships between the user-controlled external parameters and the effectiveness of Reactive Ion Etching (RIE) for the removal of surface layers of bulk niobium have been previously established. However, a lack of a physical description of the etching discharge, particularly as the external parameters are varied, limits the development of this technology. A full understanding of how these external parameters affect both the amount of material removed and the physical properties of the plasma would aid …

Plasma Spectroscopy Of Titanium Monoxide For Characterization Of Laser Ablation, Todd A. Van Woerkom, Glen P. Perram, Christian G. Parigger, Brian D. Dolasinski, Charles D. Phelps, Patrick A. Berry

Faculty Publications

Ablation of titanium wafers in air is accomplished with 60 µs pulsed, 2.94 µm laser radiation. Titanium monoxide spectra are measured in the wavelength range of 500 nm to 750 nm, and molecular signatures include bands of the C3 Δ → X3 Δ α, B3 Π → X3 Δ γ', and A3 Φ → X3 Δ γ transitions. The spatially and temporally averaged spectra appear to be in qualitative agreement with previous temporally resolved studies that employed shorter wavelengths and shorter pulse durations than utilized in this work. The background signals in the current study are possibly due to particulate …

The Population Densities Of Argon Metastable Levels, Nada Khogeer, Chelsy Gonzalez, Milka Nikolic

Physics and Astronomy

In this experiment, we used the optical emission spectroscopy (OES) method to obtain the main properties of low temperature Argon plasma. The experiment was sustained in powers and pressures that ranges from 30-100 W and 15-100 mTorr. We used numerical methods for the Argon kinetic model to calculate metastable levels and resonant states for the first excited states in low temperature Argon plasma. By finding the ratio of two spectral lines and finding another ratio from a different upper energy level that goes down to the same two lower energy levels, we can construct a system of two nonlinear equations. …

Spectroscopy Of Neon For The Advanced Undergraduate Laboratory, H. C. Busch, M. B. Cooper, C. I. Sukenik

Physics Faculty Publications

We describe a spectroscopy experiment, suitable for upper-division laboratory courses, that investigates saturated absorption spectroscopy and polarization spectroscopy in a neon discharge. Both experiments use nearly identical components, allowing students to explore both techniques in a single apparatus. Furthermore, because the wavelength of the laser is in the visible part of the spectrum (640 nm), the experiment is well-suited for students with limited experience in optical alignment. The labs nicely complement a course in atomic or plasma physics, provide students with the opportunity to gain important technical skills in the area of optics and lasers, and can provide an introduction …

Argon Metastable And Resonant Level Densities In Ar And Ar/Cl² Discharges Used For The Processing Of Bulk Niobium, Jeremy Peshl, Roderick Mcneill, Charles I. Sukenik, Milka Nikolić, Svetozar Popović, Leposava Vŭsković

Physics Faculty Publications

A comparative analysis of two popular spectroscopy techniques is conducted in a coaxial cylindrical capacitively coupled discharge designed for the plasma processing of superconducting radio frequency (SRF) cavities. The density of the metastable and resonant levels in Ar is measured in both Ar and Ar/Cl₂ discharges to properly characterize the unique discharge system and aid in the development of a cavity etching routine. The first method, deemed the “branching fraction method,” utilizes the sensitivity of photon reabsorption of radiative decay to measure the lower state (metastable and resonant) densities by taking ratios of spectral lines with a common upper …

Evaluation Of X-Ray Spectroscopic Techniques For Determining Temperature And Density In Plasmas, Theodore Scott Lane

Graduate Theses, Dissertations, and Problem Reports

Temperature and density measurements of plasmas are important for understanding various phenomena. For example, equations of state, most scaling arguments for Inertial Confinement Fusion and laboratory astrophysics all rely upon accurate knowledge of temperature and density. Spectroscopy is a non-invasive technique to measure these quantities. In this work we establish a new spectroscopic technique by using it to determine temperature. We also compare and contrast the capability of two codes, PrismSPECT and ATOMIC, to infer electron density from experimentally acquired spectra via Stark broadening.

We compare and contrast the capability of isoelectronic line ratios and inter-stage line ratios in an …

Spectroscopy And Formation Of Lanthanum-Hydrocarbon Radicals Formed By Association And Carbon-Carbon Bond Cleavage Of Isoprene, Wenjin Cao, Dilkrushi Hewage, Dong-Sheng Yang

Chemistry Faculty Publications

La atom reaction with isoprene is carried out in a laser-vaporization molecular beam source. The reaction yields an adduct as the major product and C—C cleaved and dehydrogenated species as the minor ones. La(C₅H₈), La(C₂H₂), and La(C₃H₄) are characterized with mass-analyzed threshold ionization (MATI) spectroscopy and quantum chemical computations. The MATI spectra of all three species exhibit a strong origin band and several weak vibronic bands corresponding to La-ligand stretch and ligand-based bend excitations. La(C₅H₈) is a five-membered metallacycle, whereas La(C₂H_{2 …}

Excited Argon 1s5 Production In Microhollow Cathode Discharges, Richard D. Peterson

Theses and Dissertations

Diode-pumped rare gas lasers (DPRGL) have been in development for their potential to become high energy lasers with excellent beam quality that is typical of gas lasers. DPRGL require metastable densities on the order of 10¹³ cm^-3 at pressures around one atmosphere for efficient operation. Argon 1s5 number densities have been measured in microhollow cathode discharges (MHCD) using tunable diode laser absorption spectroscopy. The MHCD had copper electrodes with gaps of 127 and 254 µm and hole diameters from 100-400 µm. Absorbance was measured at pressures of 37 Torr up to 400 Torr, where absorbance could no longer …

Lanthanum-Mediated Dehydrogenation Of Butenes: Spectroscopy And Formation Of La(C4H6) Isomers, Wenjin Cao, Dilkrushi Hewage, Dong-Sheng Yang

Chemistry Faculty Publications

La atom reactions with 1-butene, 2-butene, and isobutene are carried out in a laser-vaporization molecular beam source. The three reactions yield the same La-hydrocarbon products from the dehydrogenation and carbon-carbon bond cleavage and coupling of the butenes. The dehydrogenated species La(C₄H₆) is the major product, which is characterized with mass-analyzed threshold ionization (MATI) spectroscopy and quantum chemical computations. The MATI spectrum of La(C₄H₆) produced from the La+1-butene reaction exhibits two band systems, whereas the MATI spectra produced from the La+2-butene and isobutene reactions display only a single band system. Each of these …

Pulsed Inductive Plasma Studies By Spectroscopy And Internal Probe Methods, Warner C. Meeks

Doctoral Dissertations

The broad effort of the Missouri Plasmoid Experiment is to elucidate the energy conversion processes in a pulsed inductive discharge due to the presence of plasma. The test article is a 440 to 490 kHz theta-pinch (or solenoidal) geometry coil with a stored energy of around 80 joules. In this work experimental hydrogen, helium, argon and xenon data at back-fill pressures of 10 to 100 mTorr (1.3 to 133.3 Pa) are obtained and interpreted. Spectral and internal probe studies were performed on MPX Mk.I and Mk.II devices, respectively. IR spectra were acquired in the Mk.I device for argon and xenon. …

Optimization Of Plasmon Decay Through Scattering And Hot Electron Transfer, Drew Dejarnette

Graduate Theses and Dissertations

Light incident on metal nanoparticles induce localized surface oscillations of conductive electrons, called plasmons, which is a means to control and manipulate light. Excited plasmons decay as either thermal energy as absorbed phonons or electromagnetic energy as scattered photons. An additional decay pathway for plasmons can exist for gold nanoparticles situated on graphene. Excited plasmons can decay directly to the graphene as through hot electron transfer. This dissertation begins by computational analysis of plasmon resonance energy and bandwidth as a function of particle size, shape, and dielectric environment in addition to diffractive coupled in lattices creating a Fano resonance. With …

In-Package Atmospheric Pressure Cold Plasma Treatment Of Cherry Tomatoes, N. Misra, Kevin Keener, Paula Bourke, J Mosnier, Patrick Cullen

Articles

Cold plasma is increasingly under research for decontamination of foods, especially fresh fruits and vegetables. The effect of cold plasma on food quality, however, remains under researched. This study investigates the effects of cold plasma generated within a sealed package from a dielectric barrier discharge on the physical quality parameters and respiration rates of cherry tomatoes. Respiration rates and weight loss were monitored continuously, while other parameters are reported at the end of storage period. Differences among weight loss, pH and firmness for control and treated cherry tomatoes were insignificant towards the end of storage life. Changes in respiration rates …

Steady-State Switching And Dispersion/Absorption Spectroscopy Of Multistate Atoms Inside An Optical Ring Cavity, Jiteng Sheng

Graduate Theses and Dissertations

This thesis mainly focuses on the experimental investigations of electromagnetically induced transparency (EIT) related phenomena in various systems involving multilevel atoms inside an optical ring cavity. Semiclassical methods, e.g. density-matrix equations, are used through out this thesis to simulate the experimental results. First, the cavity transmission spectrum can be significantly modified when multilevel atoms are placed inside an optical ring cavity. Such coupled atom-cavity systems are well explained by the intracavity dispersion/absorption properties. Specifically, three-level lambda-type, four-level N-type and double-lambda-type atoms inside an optical ring cavity are investigated by examining their cavity transmission spectra. Second, optical multistability (OM) has been …

Laboratory Astrophysics: Using Ebit Measurements To Interpret High Resolution Spectra From Celestial Sources, Carey Scott, Joshua Thompson, N. Hell, Greg V. Brown

STAR Program Research Presentations

Astrophysicists use radiation to investigate the physics controlling a variety of celestial sources, including stellar atmospheres, black holes, and binary systems. By measuring the spectrum of the emitted radiation, astrophysicists can determine a source’s temperature and composition. Accurate atomic data are needed for reliably interpreting these spectra. Here we present an overview of how LLNL’s EBIT facility is used to put the atomic data on sound footing for use by the high energy astrophysics community.

Laser-Induced Breakdown Spectroscopy, Connor Drake

Physics

The goal of this work is to use a Neodymium-Doped Yttrium Aluminum Garnet (Nd:YAG) Laser, spectrometer, and computer to create a Laser Induced Breakdown Spectroscopy (LIBS) system. LIBS utilizes a focused, high-powered, pulsed laser whose peak electric field ionizes materials at the beam focal point, creating localized plasma. The plasma state includes broken molecular bonds, atom/electron-ionization, and excited electrons, which on the macroscopic level is a loud “snap” and a bright spark. In this project, a fiber optic cable is used to capture light emitted from the spark, and direct it into a spectrometer which tallies the number of photons …

Inception Of Snapover And Gas Induced Glow Discharges, J. T. Galofaro, B. V. Vayner, D. C. Ferguson, W. A. Degroot, C. D. Thomson, John R. Dennison, R. E. Davies

All Physics Faculty Publications

Ground based experiments of the snapover phenomenon were conducted in the large vertical simulation chamber at the Glenn Research Center (GRC) Plasma Interaction Facility (PIF). Two Penning sources provided both argon and xenon plasmas for the experiments. The sources were used to simulate a variety of ionospheric densities pertaining to a spacecraft in a Low Earth Orbital (LEO) environment. Secondary electron emission is believed responsible for dielectric surface charging, and all subsequent snapover phenomena observed. Voltage sweeps of conductor potentials versus collected current were recorded in order to examine the specific charging history of each sample. The average time constant …