Plasma and Beam Physics Commons^™

X-Ray Second Harmonic Generation, S. Shwartz, Matthias Fuchs, J. B. Hastings, Y. Inubushi, T. Ishikawa, T. Katayama, D. A. Reis, T. Sato, K. Tono, M. Yabashi, S. Yudovich, S. E. Harris

Matthias Fuchs Publications

We report clear experimental evidence for second harmonic generation at hard x-ray wavelengths. Using a 1.7 Å pumping beam generated by a free electron laser, we observe second harmonic generation in diamond. The generated second harmonic is of order 10 times the background radiation, scales quadratically with pump pulse energy, and is generated over a narrow phase-matching condition. Of importance for future experiments, our results indicate that it is possible to observe nonlinear x-ray processes in crystals at pump intensities exceeding 10¹⁶ W/cm².

In-Package Atmospheric Pressure Cold Plasma Treatment Of Cherry Tomatoes, N. Misra, Kevin Keener, Paula Bourke, J Mosnier, Patrick J. Cullen

Articles

Cold plasma is increasingly under research for decontamination of foods, especially fresh fruits and vegetables. The effect of cold plasma on food quality, however, remains under researched. This study investigates the effects of cold plasma generated within a sealed package from a dielectric barrier discharge on the physical quality parameters and respiration rates of cherry tomatoes. Respiration rates and weight loss were monitored continuously, while other parameters are reported at the end of storage period. Differences among weight loss, pH and firmness for control and treated cherry tomatoes were insignificant towards the end of storage life. Changes in respiration rates …

In-Package Nonthermal Plasma Degradation Of Pesticides On Fresh Produce, N. Misra, Shashi Pankaj, Tony Walsh, Finbarr O'Regan, Paula Bourke, Patrick J. Cullen

Articles

In-package nonthermal plasma (NTP) technology is a novel technology for the decontamination of foods and biological materials. This study presents the first report on the potential of the technology for the degradation of pesticide residues. A cocktail of pesticides, namely Azoxystrobin, Cyprodinil, Fludioxonil and Pyriproxyfen was tested on strawberries. The concentrations of these pesticides were monitored in priori and post- plasma treatment using GC-MS/MS. An applied voltage and time dependent degradation of the pesticides was observed for treatment voltages of 60, 70 and 80 kV and treatment durations ranging from 1 to 5 min, followed by 24 h in-pack storage. …

Resonant Electron-Atom Bremsstrahlung In An Intense Laser Field, A. N. Zheltukhin, A. V. Flegel, M. V. Frolov, N. L. Manakov, Anthony F. Starace

Anthony F. Starace Publications

We analyze a resonant mechanism for spontaneous laser-assisted electron bremsstrahlung (BrS) involving the resonant transition (via either laser-assisted electron-ion recombination or electron-atom attachment) into a laser-dressed intermediate quasibound state (corresponding, respectively, to either a field-free neutral atom or a negative-ion bound state) accompanied by ionization or detachment of this state by the laser field. This mechanism leads to resonant enhancement (by orders of magnitude) of the BrS spectral density for emitted photon energies corresponding to those for laser-assisted recombination or attachment. We present an accurate parametrization of the resonant BrS amplitude in terms of the amplitudes for nonresonant BrS, for …

Characterization Of Polarized Synchrotron Light, Britny N. Delp, Jeff Corbett

STAR Program Research Presentations

The Stanford Synchrotron Radiation Light accelerates electrons around a 234-meter circumference ring at relativistic speeds. The x-ray radiation produced by this process is used in many fields of science ranging from materials science to medicine.

This project seeks to measure the polarization of the 532 nanometer wavelength component in the visible light beam emitted from the SPEAR-3 synchrotron as a function of vertical position. The beam was focused through a lens, then passed through a 532 nm band pass filter and a polarizer mounted on a rotating stand. The beam power was measured as a function of vertical position and …

Diagnostics Of An O2–He Rf Atmospheric Plasma Discharge By Spectral Emission, Vladimir Milosavljevic, Mick Donegan, Patrick J. Cullen, Denis Dowling

Articles

In this paper optical emission spectroscopy (OES) is used as a Diagnostic technique for the measurement of atomic and molecular spectral emissions generated using a helium rf industrial atmospheric plasma jet system. The OES of neutral atomic spectral lines and molecular bands are investigated over a range of plasma process parameters.
/="/">Wavelength resolve optical emission profiles suggest that the emission of helium’s spectral lines shows that the high energy electrons have a larger influence than helium metastables on the overall spectral emission. Furthermore, the experimental data indicates that the use of high helium flow rates, in any confined open …

Neutron Spin Struccture With Polarized Deuterons And Spectator Proton Tagging At Eic, W. Cosyn, V. Guzey, D. W. Higinbotham, C. Hyde, S. Kuhn, P. Nadel-Turonski, K. Park, M. Sargsian, M. Strikman, C. Weiss

Physics Faculty Publications

The neutron's deep-inelastic structure functions provide essential information for the flavor separation of the nucleon parton densities, the nucleon spin decomposition, and precision studies of QCD phenomena in the flavor-singlet and nonsinglet sectors. Traditional inclusive measurements on nuclear targets are limited by dilution from scattering on protons, Fermi motion and binding effects, final-state interactions, and nuclear shadowing at x ≪ 0.1. An Electron-Ion Collider (EIC) would enable next-generation measurements of neutron structure with polarized deuteron beams and detection of forward-moving spectator protons over a wide range of recoil momenta (0 < pR < several 100MeV in the nucleus rest frame). The free neutron structure functions could be obtained by extrapolating the measured recoil momentum distributions to the on-shell point. The method eliminates nuclear modifications and can be applied to polarized scattering, as well as to semi-inclusive and exclusive final states. We review the prospects for neutron structure measurements with spectator tagging at EIC, the status of R&D efforts, and the accelerator and detector requirements.

Resonant Enhancement Of The Harmonic-Generation Spectrum Of Beryllium, Jean Marcel Ngoko Djiokap, Anthony F. Starace

Anthony F. Starace Publications

The high-order harmonic-generation (HHG) spectrum of Be is investigated in the multiphoton regime by solving the full-dimensional, two-active-electron, time-dependent Schr¨odinger equation in an intense (≈10¹³ W/cm²), 30-cycle laser field. As the laser frequency ω_L varies from 1.7 to 1.8 eV (which is in the tunable range of a Ti:sapphire laser), the seventh harmonic becomes resonant sequentially with the transition between the ground state and two doubly excited autoionizing states, 2p4s(¹P) (at ω_L = 1.734 eV) and 2p5s …

Carrier-Envelope-Phase-Induced Asymmetries In Double Ionization Of Helium By An Intense Few-Cycle Xuv Pulse, Jean Marcel Ngoko Djiokap, N. L. Manakov, A. V. Meremianin, Anthony F. Starace

Anthony F. Starace Publications

The carrier-envelope-phase (CEP) dependence of electron angular distributions in double ionization of He by an arbitrarily polarized, few-cycle, intense XUV pulse is formulated using perturbation theory (PT) in the pulse amplitude. Owing to the broad pulse bandwidth, interference of first- and second-order PT amplitudes produces asymmetric angular distributions sensitive to the CEP. The PT parametrization is shown to be valid by comparing with results of solutions of the full-dimensional, two-electron time-dependent Schrödinger equation for the case of linear polarization.

Harmonic Generation Spectroscopy With A Two-Colour Laser Field Having Orthogonal Linear Polarizations, T. S. Sarantseva, M. V. Frolov, N. L. Manakov, M. Yu. Ivanov, Anthony F. Starace

Anthony F. Starace Publications

The interpretation of many high-order harmonic generation (HHG) experiments is based on the assumption that the HHG yield of an atom can be factorized into (i) a laser-dependent ‘electron wave packet’ with rather simple properties, including a nearly universal shape, and (ii) an atomic photorecombination cross section. We show that this factorization is restricted to linearly polarized laser fields and fails in two-colour laser fields with orthogonal polarizations. At the same time, we show how two-colour HHG spectroscopy using orthogonally polarized intense fundamental and relatively weak second harmonic fields makes a complete experiment possible that enables the retrieval of the …

Asymmetries In Production Of He+(N = 2) With An Intense Few-Cycle Attosecond Pulse, Jean Marcel Ngoko Djiokap, S. X. Hu, Wei-Chao Jiang, Liang-You Peng, Anthony F. Starace

Anthony F. Starace Publications

By solving the two-electron time-dependent Schrödinger equation, we study carrier-envelope-phase (CEP) effects on ionization plus excitation of He to He⁺(n = 2) states by a few-cycle attosecond pulse with a carrier frequency of 51 eV. For most CEPs the asymmetries in the photoelectron angular distributions with excitation of He⁺(2s) or He⁺(2p) have opposite signs and are two orders of magnitude larger than for ionization without excitation. These results indicate that attosecond pulse CEP effects may be significantly amplified in correlated two-electron ionization processes.

Analytic Description Of Elastic Electron-Atom Scattering In An Elliptically Polarized Laser Field, A. V. Flegel, M. V. Frolov, N. L. Manakov, Anthony F. Starace, A. N. Zheltukhin

Anthony F. Starace Publications

An analytic description of laser-assisted electron-atom scattering (LAES) in an elliptically polarized field is presented using time-dependent effective range (TDER) theory to treat both electron-laser and electron-atom interactions nonperturbatively. Closed-form formulas describing plateau features in LAES spectra are derived quantum mechanically in the low-frequency limit. These formulas provide an analytic explanation for key features of the LAES differential cross section. For the low-energy region of the LAES spectrum, our result generalizes the Kroll-Watson formula to the case of elliptic polarization. For the high-energy (rescattering) plateau in the LAES spectrum, our result generalizes prior results for a linearly polarized field valid …

Hybrid Plasmonic Nanoantennas: Fabrication, Characterization, And Application, Shengjie Zhai

UNLV Theses, Dissertations, Professional Papers, and Capstones

As optical counterpart of microwave antennas, plasmonic nanoantennas are important nanoscale devices for converting propagating optical radiation into confined/enhanced electromagnetic fields. Presently, nanoantennas, with a typical size of 200-500 nm, have found their applications in bio-sensing, bio-imaging, energy harvesting, and disease cure and prevention. With the device feature size of next generation IC goes down to 22 nm or smaller, and biological/chemical sensing reaches the Gene’s level, the sizes of the corresponding nanoantennas have to be scaled down to sub-100nm level. In the literature, these sub-100nm nanoantennas are referred as deep subwavelength nanoantennas as size of such miniaturized nanoantennas is …

Threshold Effects In Strong-Field Ionization: Energy Shifts And Rydberg Structures, Katarzyna Krajewska, Ilya I. Fabrikant, Anthony F. Starace

Anthony F. Starace Publications

The behavior of strong-field ionization rates of neutral atoms in the vicinity ofmultiphoton ionization thresholds is analyzed using formal collision theory.Our approach,which accounts nonperturbatively for effects of an intense laser field, shows that the ionization rates have a nearly constant behavior below and above each multiphoton threshold and that between such thresholds there are an apparently finite number of rapid oscillations due to resonances with laser-field-modified Rydberg states. This pattern is typical for any atomic target, as we illustrate specifically for hydrogen and neon atoms. The flat behavior of the ionization yield near multiphoton thresholds gives the appearance of an …

Gaussian Beam Steering On A Target Plane Via High Speed Orthogonal Mirror-Mounted Galvanometers, Keith Gresiak

Physics

No abstract provided.

Case Studies In Many-Body Physics, Ana Samolov

Physics Theses & Dissertations

The many-body problem refers to any physical problem made of more than two interacting particles. With increasing number of particles in a system, their coupling and entanglement becomes more complex, and there is no general analytic solution even for a three-body classical or quantum systems. However, some of the most fascinating phenomena in nature are products of collective effects. Therefore, significant efforts have been made in both experiment and theory to unravel some specific many-body problems. If we look at still unanswered physics questions we see that for most of these problems addressing the many-body interactions is a key issue. …

Observation And Identification Of Metastable Excited States In Ultrafast Laser-Ionized Pyridine, David B. Foote, Timothy D. Scarborough, Cornelis J. Uiterwaal

C.J.G.J. Uiterwaal Publications

We report on the fragmentation of ionized pyridine (C₅H₅N) molecules by focused 50 fs, 800 nm laser pulses. Such ionization produces several metastable ionic states that fragment within the field-free drift region of a reflectron- type time of flight mass spectrometer, with one particular metastable dissociation being the leading fragmentation process. Because the time of flight is no longer dependent in a simple way on the mass of the ion, the metastable decay is manifested as an unfocused peak on the mass spectrum that appears at a time of flight not corresponding to an integer mass. …

Dc Pulsed Atmospheric Pressure Plasma Jet Image Information, Denis P. Dowling, F T. O'Neill, Vladimir Milosavljevic, Victor J. Law

Articles

This paper presents optical imaging and optical emission spectroscopy (OES) data of an atmospheric-pressure plasma jet. It is shown how the visual information and OES information of the air discharge are related as the blown arc extends from the nozzle (2-4 mm) with a molecular nitrogen rotational temperature on the order of 1700 K and the flowing afterglow beyond this region is dominated by the cooler (300-K) NO-O chemiluminescent reaction that produces NO₂ species.

Laboratory Astrophysics: Using Ebit Measurements To Interpret High Resolution Spectra From Celestial Sources, Carey Scott, Joshua Thompson, N. Hell, Greg V. Brown

STAR Program Research Presentations

Astrophysicists use radiation to investigate the physics controlling a variety of celestial sources, including stellar atmospheres, black holes, and binary systems. By measuring the spectrum of the emitted radiation, astrophysicists can determine a source’s temperature and composition. Accurate atomic data are needed for reliably interpreting these spectra. Here we present an overview of how LLNL’s EBIT facility is used to put the atomic data on sound footing for use by the high energy astrophysics community.

Laser-Wakefield Accelerators: Glass-Guiding Benefits, Donald P. Umstadter

Donald Umstadter Publications

A main attraction of laser-driven electron accelerators is their absence of cavity walls, which can break down in the presence of intense electric fields. Now it seems that the inclusion of a hollow glass fibre cavity could lead to more efficient acceleration at lower laser intensities. ... Further research will reveal which of the above methods for guiding light will ultimately prove best for future accelerator designs. In any case, although it is perhaps ironic that the relatively old technology of glass waveguides may benefit next-generation accelerators, it is nonetheless satisfying to see such a classic photonic solution come to …

Laser-Induced Breakdown Spectroscopy, Connor Drake

Physics

The goal of this work is to use a Neodymium-Doped Yttrium Aluminum Garnet (Nd:YAG) Laser, spectrometer, and computer to create a Laser Induced Breakdown Spectroscopy (LIBS) system. LIBS utilizes a focused, high-powered, pulsed laser whose peak electric field ionizes materials at the beam focal point, creating localized plasma.  The plasma state includes broken molecular bonds, atom/electron-ionization, and excited electrons, which on the macroscopic level is a loud “snap” and a bright spark. In this project, a fiber optic cable is used to capture light emitted from the spark, and direct it into a spectrometer which tallies the number of photons …

Raman Scattering Analysis Of Silicon Dioxide Single Crystal Treated By Direct Current Plasma Discharge, Dusan M. Poparic, Vladimir Milosavljevic, Andrijana Zekic, N Romcevic, Steven Daniels

Articles

Low-k materials such as silicon dioxide (SiO2) play an important role in the semiconductor industry. Plasma has become indispensable for advanced materials processing. In this work a treatment of SiO2single crystal by direct current plasma discharge is studied in detail. Offline metrology is conducted for silicon dioxide wafers by Raman scattering, energy-dispersive x-ray spectroscopy, and ellipsometry. Broad Raman peak at around 2800 cm−1 is observed for the treatedSiO2 wafers. Effects of plasma treatment on position of this peak are reported in the paper. An analysis of this correlation could be a framework for creating virtual etch rate sensors, which might …

Oscillator Strength Measurements In Singly-Ionized, Doubly-Ionized And Neutral Lanthanides And Transition Elements (Sm, Nd, Pr, Gd, Cu, And Fe) Using Laser-Induced Breakdown Spectroscopy., Caleb Ryder

Wayne State University Dissertations

Models for stellar nucleosynthesis, age determinations for stars in the Milky Way's galactic halo, and stellar chemical abundance determinations are dependent upon accurate atomic spectroscopic data to allow the correct interpretation of stellar absorption and emission spectra. It is well known that calculations of many astrophysically important atomic parameters are limited due to line blending, insufficient spectral resolution of some key spectral lines, and also the complicated electronic structure of the important heavy elements. Astrophysicists have therefore looked to laboratory astrophysics experiments to provide accurate atomic data to help resolve these limiting issues. In this dissertation, laser-induced breakdown spectroscopy (LIBS) …

Electron Transmission Characteristics And The Production Of Narrow Beams Using Glass Optics, Buddhika Senarath Dassanayake

Dissertations

Transmission of electrons through an insulating single cylindrically-shaped glass capillary of microscopic dimension has been investigated. Samples made with Borosilicate glass (PYREX 7740) were subjected to bombardment of 300-1000 eV electrons. Transmitted electrons were analyzed using a parallel-plate spectrometer coupled to a channel electron multiplier.

The transmitted electron intensity was found to decrease with increasing sample tilt angle relative to the direction of the primary beam. Two regions of transmission were found: direct where there is no interaction of the beam with the inner capillary wall, and indirect where the beam does interact with the wall. The rate of transmission …

Characterization Of An Inductively Coupled Plasma Produced In Argon At 13.56 Mhz., Lim Ai Nuan

Student Works (2010-2019)

The electrical and plasma characteristics of radio frequency (13.56 MHz) inductively coupled argon plasma (RF ICP) were studied in this project. On the electrical breakdown properties, the breakdown voltage has a general appearance of Paschen’s curve and the minimum is achieved at 0.1 mbar. After ignition, two modes of discharge exist, namely, the E mode at low RF power and H mode at high RF power. Mode transition that occurs is accompanied by abrupt changes in both electrical and plasma characteristics. Hysteresis is observed in the mode transitions and has a minimum at 0.1 mbar. The resistance reflected into the …

Characterization Of Microwave Cavity Discharges In A Supersonic Flow, Dareth Janette Drake

Physics Theses & Dissertations

A partially ionized gas is referred to as either a plasma or a discharge depending on the degree of ionization. The term discharge is usually applied to a weakly ionized gas, i.e. mostly neutrals, where as a plasma usually has a larger degree of ionization. To characterize a discharge the plasma parameters, such as the rotational temperature, vibrational temperature, and electron density, must be determined. Detailed characterization of supersonic flowing discharges is important to many applications in aerospace and aerodynamics. One application is the use of plasma-assisted hydrogen combustion devices to aid in supersonic combustion. In conditions close to the …

Theoretical Model Analysis Of Absorption Of A Three Level Diode Pumped Alkali Laser, Charlton D. Lewis Ii

Theses and Dissertations

This paper models the absorption phenomena of light in a three level diode pumped alkali laser system. Specifically this model calculates for a user defined set of system parameters the attenuation of the input pump beam and characteristics of the bleached wave. Using Wolfram's Mathematical 6.0 software all necessary physics for an accurate description of absorption was modeled from first principles: energy levels, cross sections, spin-orbit kinetic processes, saturation frequencies, pump attenuation, and differential transmittance, which is a representation of the bleached wave. A specific DPAL scenario was simulated, 455K system temperature, alkali concentration of 6.1 - 10¹³, …

Real-Time Plasma Controlled Chemistry In A Two-Frequency, Confined Plasma Etcher, Vladimir Milosavljevic, Albert R. Ellingboe, Cezar Gaman, John V. Ringwood

Articles

The physics issues of developing model-based control of plasma etching are presented. A novel methodology for incorporating real-time model-based control of plasma processing systems is developed. The methodology is developed for control of two dependent variables (ion flux and chemical densities) by two independent controls (27 MHz power and O2flow). A phenomenological physics model of the nonlinear coupling between the independent controls and the dependent variables of the plasma is presented. By using a design of experiment, the functional dependencies of the response surface are determined. In conjunction with the physical model, the dependencies are used to deconvolve the sensor …

A Mode-Locked Vertical Extended Cavity Surface Emitting Laser, Aoife Deburca

Theses

Surface emitting lasers are a competitive and flexible alternative to edge emitting lasers. The surface-emitting laser has many useful characteristics, which make it beneficial for many applications. These characteristics include the ease of testing during the growth and the fundamental mode output that is effortlessly achieved

The thesis is focused on the Vertical External Cavity Surface Emitting Laser due to its increased flexibility beyond that of the Vertical Cavity Surface Emitting Laser. A wide range of possible parameters are detailed allowing for flexibility in design and applications.

Optically pumped pulsed cavity configurations were investigated in relation to intra-cavity devices and …

Practical Sensor For Measurement Of Nitrogen, Dusan Popovic, Vladimir Milosavljevic, Steven Daniels

Articles

This paper presents a method for precise measurement of atomic and molecular nitrogen in an oxygen-nitrogen dc plasma. This is achieved by monitoring the intensities of the atomic nitrogen spectral line at 821.6 nm and the molecular nitrogen bandhead at 337.1 nm, relative to the atomic oxygen spectral line at 844.7 nm. Oxygen is one of the most frequently used gases for surface chemical treatment, including deposition and etching, therefore the ability to measure and control the process and chemical composition of the process is essential. To validate this oxygen actimometry method for N2-xO2 (where x varies from 0 to …