Condensed Matter Physics Commons^™

Ferroelectric Instability Under Screened Coulomb Interactions, Yong Wang, Xiaohui Liu, John D. Burton, Sitaram S. Jaswal, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

We explore the effect of charge carrier doping on ferroelectricity using density functional calculations and phenomenological modeling. By considering a prototypical ferroelectric material, BaTiO₃, we demonstrate that ferroelectric displacements are sustained up to the critical concentration of 0.11 electron per unit cell volume. This result is consistent with experimental observations and reveals that the ferroelectric phase and conductivity can coexist. Our investigations show that the ferroelectric instability requires only a short-range portion of the Coulomb force with an interaction range of the order of the lattice constant. These results provide a new insight into the origin of ferroelectricity …

Pulse Sharpening Effects Of Thin Film Ferroelectric Transmission Lines, Robert J. Sleezer

Graduate Theses and Dissertations

Advances in material science have resulted in the development of electrically nonlinear high dielectric thin film ferroelectrics, which have led to new opportunities for the creation of novel devices. This dissertation investigated one such device: a low voltage nonlinear transmission line (NLTL). A finite element simulation of ferroelectric transmission lines showed that NLTLs are capable of creating shockwaves. Additionally, if the losses are kept sufficiently low, it was shown that voltage gain should be possible. Furthermore, a method of accounting for material dispersion was developed. Results from simulations including material dispersion showed that temporal solitons might be possible from a …

Electron–Phonon Coupling And Structural Phase Transitions On Au/Mo(112), Keisuke Fukutani

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The electronic structures, many-body interactions and Fermi surface topologies of Au/Mo(112) were investigated in detail and were found to play important roles in the newly discovered order-disorder structural phase transition of the system. First, the high-resolution angle-resolved photoemission spectroscopy was utilized to characterize the electronic band structure of Mo(112) in far greater details than before. This elucidated the existence of several surface-derived states and their dispersion relations in high precisions near the Fermi level, as well as the symmetries of the bulk and surface electronic states, which are in good quantitative agreement with the ab-initio calculations. Such thorough understanding of …

Hohenberg-Kohn Theorem Including Electron Spin, Xiao-Yin Pan, Viraht Sahni

Publications and Research

The Hohenberg-Kohn theorem is generalized to the case of a finite system of N electrons in external electrostatic epsilon(r) = -del nu(r) and magnetostatic B(r) = del x A(r) fields in which the interaction of the latter with both the orbital and spin angular momentum is considered. For a nondegenerate ground state a bijective relationship is proved between the gauge invariant density rho(r) and physical current density j(r) and the potentials {nu(r), A(r)}. The possible many-to-one relationship between the potentials {v(r), A(r)} and the wave function is explicitly accounted for in the proof. With the knowledge that the basic variables …

Equilibrium Magnetic States In Individual Hemispherical Permalloy Caps, Robert Streubel, Volodymyr P. Kravchuk, Denis D. Sheka, Denys Makarov, Florian Kronast, Oliver G. Schmidt, Yuri Gaididei

Robert Streubel Papers

The magnetization distributions in individual soft magnetic permalloy caps on non-magnetic spherical particles with sizes ranging from 50 to 800nm are investigated. We experimentally visualize the magnetic structures at the resolution limit of the x-ray magnetic circular dichroism photoelectron emission microscopy (XMCD-PEEM). By analyzing the so-called tail contrast in XMCD-PEEM, the spatial resolution is significantly enhanced, which allowed us to explore magnetic vortices and their displacement on curved surfaces. Furthermore, cap nanostructures are modeled as extruded hemispheres to determine theoretically the phase diagram of equilibrium magnetic states. The calculated phase diagram agrees well with the experimental observations. © 2012 American …

Nanomechanical Resonator Coupled Linearly Via Its Momentum To A Quantum Point Contact, Latchezar L. Benatov, Miles P. Blencowe

Dartmouth Scholarship

We use a Born-Markov approximated master equation approach to study the symmetrized-in-frequency current noise spectrum and the oscillator steady state of a nanoelectromechanical system where a nanoscale resonator is coupled linearly via its momentum to a quantum point contact (QPC). Our current noise spectra exhibit clear signatures of the quantum correlations between the QPC current and the back-action force on the oscillator at a value of the relative tunneling phase (η=−π/2) where such correlations are expected to be maximized. We also show that the steady state of the oscillator obeys a classical Fokker-Planck equation, but can experience thermomechanical noise squeezing …

High Frequency Study Of Magnetic Nanostructures, Abhishek Srivastava

LSU New Orleans Theses and Dissertations

The work in this thesis is divided in three parts. In part one we developed electrodeposition method of Nickel Nanowire in commercial AAO template in constant current (Galvanostatic) mode, further we tried to estimate the growth rate from theory, from saturation magnetization and direct measurement from SEM image.

In part two we focused on using the Vector Network Analyzer (VNA) to measure the Ferromagnetic Resonance (FMR))of various magnetic Nanowire arrays. We employed different measurement geometries using microstripline and coplanar waveguide as microwave transmission lines.

In part three our aim was to study the magnetic properties of complex ferromagnetic system, especially …

Electronic Transport In Thermoelectric Bismuth Telluride, Westly Nolting

LSU New Orleans Theses and Dissertations

An experimental investigation of the electronic transport properties of bismuth telluride nanocomposite materials is presented. The primary transport measurements are electrical conductivity, Seebeck coefficient and Hall effect. An experimental apparatus for measuring Hall effect and electrical conductivity was designed, constructed and tested. Seebeck coefficient measurements were performed on a commercial instrument. The Hall effect and Seebeck coefficient measurements are two of the most important tools for characterizing thermoelectric materials and are widely used in the semiconductor industry for determining carrier types, carrier concentration and mobility. Further, these transport parameters are used to determine the thermal to electrical conversion efficiency of …

Characterization Of Magnetic Nanostructured Materials By First Order Reversal Curve Method, Denny R. Lenormand

LSU New Orleans Theses and Dissertations

The Interactions and magnetization reversal of Ni nanowire arrays and synthetic anit-ferromagnetic coupled thin film trilayers have been investigated through first order reversal curve (FORC) method. By using a quantitative analysis of the local interaction field profile distributions obtained from FORC, it has proven to be a powerful characterization tool that can reveal subtle features of magnetic interactions.

Ii-Vi Core-Shell Nanowires: Synthesis, Characterizations And Photovoltaic Applications, Kai Wang

LSU New Orleans Theses and Dissertations

The emergence of semiconducting nanowires as the new building blocks for photovoltaic (PV) devices has drawn considerable attention because of the great potential of achieving high efficiency and low cost. In special, nanowires with a coaxial structure, namely, core-shell structures have demonstrated significant advantages over other device configurations in terms of radial charge collection and cost reduction. In this dissertation, several core-shell nanowire structures, including ZnO/ZnSe, ZnO/ZnS, and CdSe/ZnTe, have been synthesized and the photovoltaic devices processed from a ZnO/ZnS core-shell nanowire array and a single CdSe/ZnTe core-shell nanowire have been demonstrated.

By combining the chemical vapor deposition and pulsed …

Information Content Of Spontaneous Symmetry Breaking, Marcelo Gleiser, Nikitas Stamatopoulos

Dartmouth Scholarship

We propose a measure of order in the context of nonequilibrium field theory and argue that this measure, which we call relative configurational entropy (RCE), may be used to quantify the emergence of coherent low-entropy configurations, such as time-dependent or time-independent topological and nontopological spatially extended structures. As an illustration, we investigate the nonequilibrium dynamics of spontaneous symmetry breaking in three spatial dimensions. In particular, we focus on a model where a real scalar field, prepared initially in a symmetric thermal state, is quenched to a broken-symmetric state. For a certain range of initial temperatures, spatially localized, long-lived structures known …

Dynamical Properties Of Ferroelectric Perovskites (Ba,Sr)Tio3 And Pb(Zr,Ti)O3 Systems From First Principles, Jeevaka Weerasinghe

Graduate Theses and Dissertations

A first-principles-based effective Hamiltonian scheme which incorporates coupling between ferroelectric (FE) and antiferrodistortive (AFD) motions is applied to Pb(Zr,Ti)O₃ alloys. It validates the existence of two modes of E symmetry (rather than the single E(1TO) soft mode) in the 50-75 cm^-1 range for temperatures smaller than 200 K and for compositions falling within the Rhombohedral R3c phase. Coupling between long-range-ordered FE and AFD motions is shown to be the cause of the additional mode and more insight into its nature is provided. This scheme is further used to reveal a field-induced anticrossing involving FE and AFD degrees of …

The Effect Of Polarization And Ingan Quantum Well Shape In Multiple Quantum Well Light Emitting Diode Heterostructures, Patrick M. Mcbride

Master's Theses

Previous research in InGaN/GaN light emitting diodes (LEDs) employing semi-classical drift-diffusion models has used reduced polarization constants without much physical explanantion. This paper investigates possible physical explanations for this effective polarization reduction in InGaN LEDs through the use of the simulation software SiLENSe. One major problem of current LED simulations is the assumption of perfectly discrete transitions between the quantum well (QW) and blocking layers when experiments have shown this to not be the case. The In concentration profile within InGaN multiple quantum well (MQW) devices shows much smoother and delayed transitions indicative of indium diffusion and drift during …

Magnetic Vortices On Closely Packed Spherically Curved Surfaces, Robert Streubel, Denys Makarov, Florian Kronast, Volodymyr Kravchuk, Manfred Albrecht, Oliver G. Schmidt

Robert Streubel Papers

We investigate the change of magnetic vortex states driven by curvature. The equilibrium state and magnetization reversal of soft magnetic permalloy (Py, Ni ₈₀Fe ₂₀) caps on self-assembled spherical particles with diameters of 100, 330, and 800 nm are investigated, revealing the vortex ground state for individual caps and closely packed cap arrays. The magnetic coupling between vortices is substantially reduced due to the shape of the cap as apparent in a much weaker dependence of the magnetization reversal process on the separation distance. Interestingly, the remaining coupling is still sufficiently large to introduce chirality frustrated vortex states …

Magnetic Ordering And Structural Phase Transition In Strained Ultrathin Srruo3/Srtio3 Superlattice, Mingquiang Gu, Xiaoshan Wu, Guoping Zhang

Symposium 2012

No abstract provided.

Charging Effects Of Multilayered Dielectric Spacecraft Materials: Surface Voltage, Discharge And Arcing, Gregory Wilson, Amberly Evans Jensen, Justin Dekany, Jr Dennison

Conference Proceedings

Charging of thin-film, multilayer dielectric materials subject to electron bombardment was found to evolve with time. The charging behavior was also highly dependent on the incident energy of the monoenergetic electron beams; this is driven by energy dependant processes including the electron penetration depth, electron emission, and material conductivity. The electron penetration depth is the average range to which incident electrons at a given incident energy penetrate into the material, thus defining the mean depth of an embedded charge layer. The secondary electron yield is the ratio of electrons emitted from the surface to the number of incident electrons; this …

Low Temperature Cathodoluminescence Of Space Observatory Materials, Amberly Evans Jensen, Gregory Wilson, Justin Dekany, Jr Dennison

Conference Proceedings

In recent charging studies, a discernable glow was detected emanating from sample surfaces undergoing electron beam bombardment that resulted from a luminescent effect termed cathodoluminescence. This suggests that some of the materials used as optical elements, structural components, and thermal control surfaces in the construction of space-based observatories might luminesce when exposed to sufficiently energetic charged particle fluxes from the space plasma environment. If these visible, infrared and ultraviolet emissions are intense enough, they can potentially produce optical contamination detrimental to the performance of the observatory optical elements and sensors, and act to limit their sensitivity and performance windows. As …

Hohenberg-Kohn And Percus-Levy-Lieb Proofs Of Density-Functional Theory, Viraht Sahni, Xiao-Yin Pan

Publications and Research

The premise of density-functional theory is that knowledge of the ground-state density uniquely determines the Hamiltonian, and thereby, via solution of the corresponding time-independent Schrodinger equation, all the properties of the system. The density therefore constitutes a basic variable of quantum mechanics. There are at present two paths from the density to the Hamiltonian: the Hohenberg and Kohn proof of the bijectivity between the external potential and the basic variable, and the Percus, Levy, and Lieb constrained-search proof. We argue the Hohenberg- and Kohn-type proof to be the more fundamental, and that this is the case in general when both …

The Effects Of Surface Roughness On Diffuse Optical Reflection And Photoyields On Spacecraft Materials, Amberly Evans Jensen

Senior Theses and Projects

The goal of this project was to measure the change in the absorbance of spacecraft materials due to changes in the surface of the material. The absorbance was obtained by measuring reflectance and transmittance. We found that modifying the surface of a material did affect the material’s specular reflectance. However, the change may not have been entirely due to an increase in absorbance, but may also imply an increase in the diffuse reflection. To understand the affect on absorbance, diffuse reflectance and transmission will need to be measured. This will lead to a prediction of how surface modification affects the …

Evaluation Of The Temperature Dependence Of Endurance Models Of Electrostatic Breakdown, Charlie Sim, Jr Dennison

Senior Theses and Projects

The goal of this research was to investigate temperature and time dependent models for the electrostatic breakdown of polymeric spacecraft insulators. Temperature dependent breakdown was found by inducing an electrostatic breakdown in the prototypical polymer Low Density Polyethylene (LDPE) at various temperatures. Time dependent breakdown was found by applying a static voltage to LDPE and measuring the time to electrostatic breakdown. No significant temperature dependence of the electrostatic breakdown of LDPE was observed in a temperature range of 150 K to 300 K. The time dependent results show that the time to electrostatic breakdown is modeled by a negative logarithmic …

Highly Charged Ion Interactions With Ultrathin Dielectric Films, Russell Lake

All Dissertations

The excitations occurring at a solid surface due to slow highly charged ion (HCI) impacts are interesting from the perspective of fundamental processes in atomic collisions and materials science. This thesis focuses on two questions: 1) How much HCI potential energy deposition is required to form permanent surface modifications?, 2) How does the presence of a thin dielectric surface film change the classical over-the-barrier picture for neutralization above a clean metal?
I describe a measurement of craters in thin dielectric films formed by XeQ+ (26 ≤ Q ≤ 44) projectiles. Tunnel junction devices with ion-irradiated barriers were used to amplify …

Synthesis And High-Pressure Structural Studies Of Aux2 (X= Al, Ga, In) Compounds, Jason Lee Baker

UNLV Theses, Dissertations, Professional Papers, and Capstones

Three intermetallic compounds, AuX₂ (X = Al, Ga, In), were synthesized by arc-melting proper stoichiometric ratios of high purity Au, Al, Ga, and In. They were found to be single-phase in the CaF₂ type Fm3m crystalline structure. Interest in these particular intermetallic materials is due to intriguing pressure-induced behavior such as electronic topological transitions (ETTs), and structural phase transitions as well as their use in a variety of practical applications such as a solar spectral absorber and in electronic circuitry. In this study, the high-pressure structure of these materials was studied using high resolution synchrotron x-ray diffraction (XRD) …

Mott Transition And Electronic Structure In Complex Oxide Heterostructures, Jian Liu

Graduate Theses and Dissertations

Strongly correlated electron systems, particularly transition metal oxides, have been a focus of condensed matter physics for more than two decades since the discovery of high-temperature superconducting cuprates. Diverse competing phases emerge, spanning from exotic magnetism to unconventional superconductivity, in proximity to the localized-itinerant transition of Mott insulators. While studies were concentrated on bulk crystals, the recent rapid advance in synthesis has enabled fabrication of high-quality oxide heterostructures, offering a new route to create novel artificial quantum materials.

This dissertation details the investigation on ultrathin films and heterostructures of 3d⁷(t_2g⁶e_g¹) systems with …

Use Of Ultra High Vacuum Plasma Enhanced Chemical Vapor Deposition For Graphene Fabrication, Shannen Adcock

Graduate Theses and Dissertations

Graphene, what some are terming the "new silicon", has the possibility of revolutionizing technology through nanoscale design processes. Fabrication of graphene for device processing is limited largely by the temperatures used in conventional deposition. High temperatures are detrimental to device design where many different materials may be present. For this reason, graphene synthesis at low temperatures using plasma-enhanced chemical vapor deposition is the subject of much research. In this thesis, a tool for ultra-high vacuum plasma-enhanced chemical vapor deposition (UHV-PECVD) and accompanying subsystems, such as control systems and alarms, are designed and implemented to be used in future graphene growths. …

Out-Of-Surface Vortices In Spherical Shells, Volodymyr P. Kravchuk, Denis D. Sheka, Robert Streubel, Denys Makarov, Oliver G. Schmidt, Yuri Gaididei

Robert Streubel Papers

The interplay of topological defects with curvature is studied for out-of-surface magnetic vortices in thin spherical nanoshells. In the case of an easy-surface Heisenberg magnet it is shown that the curvature of the underlying surface leads to a coupling between the localized out-of-surface component of the vortex with its delocalized in-surface structure, i.e., polarity-chirality coupling. © 2012 American Physical Society.

New View Of The Occupied Band Structure Of Mo(112), Keisuke Fukutani, Hirokazu Hayashi, I. N. Yakovkin, Tula R. Paudel, Takafumi Habuchi, Daisuke Hirayama, Jian Jiang, Hideaki Iwasawa, Kenya Shimada, Ning Wu, Evgeny Y. Tsymbal, Yaroslav B. Losovyj, Peter A. Dowben

Evgeny Tsymbal Publications

We present a comprehensive examination of the occupied surface-weighted band structure of Mo(112) along the two high-symmetry directions of the surface Brillouin zone, both from theoretical and experimental perspectives. The band structures are found to be significantly different for the states along the two high-symmetry directions and for the states with even and odd reflection parities with respect to the mirror planes. The present study suggests the existence of a number of surface-weighted bands along both high-symmetry directions. The complexity of the band structure near the Fermi level may impose potential difficulties in experimental determination of the electronphonon coupling parameters …

Light Vs. Quantum Gravity, Irving Martinez^*

COURI Symposium Abstracts, Spring 2012

No abstract provided.

Demonstration Of The Gunnarsson-Lundqvist Theorem And The Multiplicity Of Potentials For Excited States, Yu-Qi Li, Xiao-Yin Pan, Biao Li, Viraht Sahni

Publications and Research

The Gunnarsson-Lundqvist (GL) theorem of density functional theory states that there is a one-to-one relationship between the density of the lowest nondegenerate excited state of a given symmetry and the external potential. As a consequence, knowledge of this excited state density determines the external potential uniquely. [The GL theorem is the equivalent for such excited states of theHohenberg-Kohn (HK) theorem for nondegenerate ground states.] For other excited states, there is no equivalent of the GL or HK theorem. For these states, there thus exist multiple potentials that generate the excited-state density. We show, by example, the satisfaction that the GL …

Multidimensional Spectroscopy Of Semiconductor Quantum Dots, Jason Michael Bylsma

USF Tampa Graduate Theses and Dissertations

The coherent properties of semiconductor nanostructures are inherently difficult to measure and one-dimensional spectroscopies are often unable to separate inhomogeneous and homogeneous linewidths. We have refined and improved a method of performing multidimensional Fourier transform spectroscopy based on four-wave

mixing (FWM) experiments in the box geometry. We have modified our system with broadband beamsplitters in all interferometer arms, high-resolution translation stages and the ability to work in reflection geometry. By improving the phase-stability of our setup and scanning pulse delays with sub-optical cycle precision, we are able to

reproduce 2DFT spectra of GaAs multiple quantum wells. With the FWM signal …

Electron Drift-Mobility Measurements In Polycrystalline Cuin1-Xgaxse2 Solar Cells, Steluta A. Dinca, Eric A. Schiff, William N. Shafarman, Brian Egaas, Rommel Noufi, David L. Young

Physics - All Scholarship

We report photocarrier time-of-flight measurements of electron drift mobilities for the p-type CuIn_1-xGa_xSe₂ films incorporated in solar cells. The electron mobilities range from 0.02 to 0.05 cm^2/Vs and are weakly temperature-dependent from 100–300 K. These values are lower than the range of electron Hall mobilities (2-1100 cm²/Vs) reported for n-type polycrystalline thin films and single crystals. We propose that the electron drift mobilities are properties of disorder-induced mobility edges and discuss how this disorder could increase cell efficiencies.