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Articles 331 - 360 of 369

Full-Text Articles in Condensed Matter Physics

Ferroelectric Properties Of Langmuir-Blodgett Copolymer Films At The Nanoscale, A. Tolstousov, R. V. Gaynutdinov, R. Tadros-Morgane, Herbert Kliem, Stephen Ducharme, Vladimir M. Fridkin Jan 2007

Ferroelectric Properties Of Langmuir-Blodgett Copolymer Films At The Nanoscale, A. Tolstousov, R. V. Gaynutdinov, R. Tadros-Morgane, Herbert Kliem, Stephen Ducharme, Vladimir M. Fridkin

Stephen Ducharme Publications

Langmuir-Blodgett (LB) films are well known structures prepared as a result of successive transfer of monolayers (ML) from the gas-liquid interface onto solid substrates. One impressive possibility of LB method is the opportunity to vary the thickness of the film to an accuracy of one transfer, which could coincide with one ML. The ferroelectric properties of a copolymer of vinylidene fluoride and trifluorethylene P[VDF-TrFE] prepared by LB deposition are investigated in the region of a few monolayers.

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An Evaluation Of Supercritical Drying And Peg/Freeze Drying Of Waterlogged Archaeological Wood, Eric Schindelholz, Robert Blanchette, Desmond C. Cook, Michael Drews, Steve Hand, Benjamin Held, Joel Jurgens, Betty Seifert Jan 2007

An Evaluation Of Supercritical Drying And Peg/Freeze Drying Of Waterlogged Archaeological Wood, Eric Schindelholz, Robert Blanchette, Desmond C. Cook, Michael Drews, Steve Hand, Benjamin Held, Joel Jurgens, Betty Seifert

Physics Faculty Publications

This study was undertaken to evaluate the physical effects of drying waterlogged archaeological wood using supercritical carbon dioxide as compared to air drying and the popular polyethylene glycol (PEG)/freeze drying method. Previous studies have shown supercritical drying to be a potentially advantageous alternative to current methods of drying waterlogged wood through reduced processing time, minimal shrinkage, and increased success for reversibility. Samples in the form of blocks and planks of a few centimeters in size were prepared from two archaeological waterlogged wood sources and grouped into three treatment sets: one for air drying, one for PEG/freeze drying, and the other …

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Transmission Electron Goniometry And Its Relation To Electron Tomography For Materials Science Apoplications, Peter Moeck, P. Fraundorf Nov 2006

Transmission Electron Goniometry And Its Relation To Electron Tomography For Materials Science Apoplications, Peter Moeck, P. Fraundorf

Physics Faculty Publications and Presentations

Aspects of transmission electron goniometry are discussed. Combined with high resolution phase contrast transmission electron microscopy (HRTEM) and atomic resolution scanning TEM (STEM) in the atomic number contrast (Z-STEM) or the phase contrast bright field mode, transmission electron goniometry offers the opportunity to develop dedicated methods for the crystallographic characterization of nanocrystals in three dimensions. The relationship between transmission electron goniometry and electron tomography for materials science applications is briefly discussed. Internet based java applets that facilitate the application of transmission electron goniometry for cubic crystals with calibrated tilt-rotation and double-tilt specimen holders/goniometers are mentioned. The so called cubic-minimalistic tilt …

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Investigation Of The Superconducting Properties Of Niobium Radio-Frequency Cavities, Gianluigi Ciovati Jul 2005

Investigation Of The Superconducting Properties Of Niobium Radio-Frequency Cavities, Gianluigi Ciovati

Physics Theses & Dissertations

Radio-frequency (rf) superconducting cavities are widely used to increase the energy of a charged particle beam in particle accelerators. The maximum gradients of cavities made of bulk niobium have constantly improved over the last ten years and they are approaching the theoretical limit of the material. Nevertheless, rf tests of niobium cavities are still showing some "anomalous" losses (so-called "Q-drop"), characterized by a marked increase of the surface resistance at high rf fields, in absence of field emission. A low temperature "in-situ" baking under ultra-high vacuum has been successfully applied by several laboratories to reduce those losses and …

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The Effects Of Humidity On The Dielectric Response In Ferroelectric Polymer Films Made By Langmuir-Blodgett Deposition, Kristin L. Kraemer, Alexander V. Sorokin, Christina M. Othon, Stephen Ducharme, Vladimir M. Fridkin Jan 2005

The Effects Of Humidity On The Dielectric Response In Ferroelectric Polymer Films Made By Langmuir-Blodgett Deposition, Kristin L. Kraemer, Alexander V. Sorokin, Christina M. Othon, Stephen Ducharme, Vladimir M. Fridkin

Stephen Ducharme Publications

No abstract provided.

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Condensation On (002) Graphite Of Liquid Bismuth Far Below Its Bulk Melting Point, M. K. Zayed, H. E. Elsayed-Ali Jan 2005

Condensation On (002) Graphite Of Liquid Bismuth Far Below Its Bulk Melting Point, M. K. Zayed, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

Condensation of thermally evaporated Bi on (002) graphite, at temperatures of 300-523K, was studied using in situ reflection high-energy electron diffraction (RHEED) and room temperature ex situ atomic force microscopy (AFM). For deposition at temperatures below 415±5K, transmission RHEED patterns of Bi appeared at an average thickness of ∼0.5 monolayer (ML). AFM images showed that the film consisted of crystallites in the shape of triangular step pyramids with step heights corresponding to single and double Bi layers in the [111] direction. This morphology indicates crystallization from the vapor. For deposition at higher temperatures, diffuse RHEED patterns appeared independent of the …

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Investigation Of Ferroelectricity In Newly Synthesized Nitrile Polymer Systems, Matt Poulsen, Stephen Ducharme, Alexander V. Sorokin, Sahadeva Reddy, James M. Takacs, Y. Wen, Jihee Kim, Shireen Adenwalla Jan 2005

Investigation Of Ferroelectricity In Newly Synthesized Nitrile Polymer Systems, Matt Poulsen, Stephen Ducharme, Alexander V. Sorokin, Sahadeva Reddy, James M. Takacs, Y. Wen, Jihee Kim, Shireen Adenwalla

Stephen Ducharme Publications

The ferroelectric and piezoelectric properties of newly synthesized polymer systems have been studied. To date PVDF and its copolymers P(VDF-TrFE) have provided the bulk of the knowledge pertaining to ferroelectricity in polymers. Recently, ultrathin ferroelectric films of P(VDF-TrFE) 70:30 have been fabricated using the Langmuir-Blodgett technique [4]. In this study, various new polymers have been synthesized by chemically altering the PVDF structure. This alteration was performed in order to enhance the amphiphilic nature of the polymer and thus improve the LB film quality and control. Various chemical groups have been used to replace the electropositive hydrogen and electronegative fluorine found …

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Boron-Rich Semiconducting Boron Carbide Neutron Detector, Andrew D. Harken, Ellen E. Day, Brian W. Robertson, Shireen Adenwalla Jan 2005

Boron-Rich Semiconducting Boron Carbide Neutron Detector, Andrew D. Harken, Ellen E. Day, Brian W. Robertson, Shireen Adenwalla

Shireen Adenwalla Papers

Data on the neutron detection capabilities of a variety of boron carbide/Si heterojunction diodes is presented. The pulse height spectra are compared with previously measured conversion layer devices and the variations in shape and position of the peaks are discussed.

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Anisotropy Of Exchange Stiffness And Its Effect On The Properties Of Magnets, K. D. Belashchenko Apr 2004

Anisotropy Of Exchange Stiffness And Its Effect On The Properties Of Magnets, K. D. Belashchenko

Kirill Belashchenko Publications

Using the spin-spiral formulation of the tight-binding linear muffin-tin orbital method, the principal components of the exchange stiffness tensor are calculated for typical hard magnets including tetragonal CoPt-type and hexagonal YCo5 alloys. The exchange stiffness is strongly anisotropic in all studied alloys. This anisotropy makes the domain wall surface tension anisotropic. Competition between this anisotropic surface tension and magnetostatic energy controls the formation and dynamics of nanoscale domain structures in hard magnets. Anisotropic domain wall bending is described in detail from the general point of view and with application to cellular Sm–Co magnets. It is shown that the repulsive …

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Mapping Surface Polarization In Thin Films Of The Ferroelectric Polymer P(Vdf-Trfe)., Bradley W. Peterson, Stephen Ducharme, Vladimir M. Fridkin, Timothy J. Reece Jan 2004

Mapping Surface Polarization In Thin Films Of The Ferroelectric Polymer P(Vdf-Trfe)., Bradley W. Peterson, Stephen Ducharme, Vladimir M. Fridkin, Timothy J. Reece

Stephen Ducharme Publications

Pyroelectric Scanning Microscopy (PSM) has been developed to enable mapping of surface polarization in ferroelectric thin films, in particular the copolymer polyvinylidene fluoride trifluororethylene, or P(VDF-TrFE). The Chynoweth method for dynamically measuring pyroelectric current is employed in conjunction with a micropositioning system to construct two-dimensional images of the film polarization. These images have revealed enhancement of the polarization near the edges of the film below the average coercive field, with the center's polarization increasing thereafter to meet the edge value at saturation.

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Electron Irradiation Effects On Ferroelectric Copolymer Langmuir-Blodgett Films, Christina M. Othon, Stephen Ducharme Jan 2004

Electron Irradiation Effects On Ferroelectric Copolymer Langmuir-Blodgett Films, Christina M. Othon, Stephen Ducharme

Stephen Ducharme Publications

The effect of irradiation on the ferroelectric properties of Langmuir-Blodgett films of the copolymer poly(vinylidene fluoride-trifluorethelene) is investigating using 1.26 MeV electrons with dosages from 16 to 110 Mrad. Irradiation causes a systematic decrease in the phase transition temperature, coercive field and polarization of these thin films.

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Ferroelectricity At Molecular Level, L. M. Blinov, A. V. Bune, Peter A. Dowben, Stephen Ducharme, Vladimir M. Fridkin, S. P. Palto, K. A. Verkhovskaya, G. V. Vizdrik, S. G. Yudin Jan 2004

Ferroelectricity At Molecular Level, L. M. Blinov, A. V. Bune, Peter A. Dowben, Stephen Ducharme, Vladimir M. Fridkin, S. P. Palto, K. A. Verkhovskaya, G. V. Vizdrik, S. G. Yudin

Stephen Ducharme Publications

he synthesis of ultrathin ferroelectric nanostructures by the Langmuir-Blodgett method and their properties are reviewed. It is shown that ferroelectricity exists in one monolayer of the ferroelectric P(VDF-TrFE) copolymer, i.e., at the molecular level. The specific characteristics of switching of ultrathin ferroelectric films are established.

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Comment On: 'Depolarization Corrections To The Coercive Field In Thin-Film Ferroelectrics', Stephen Ducharme, Vladimir Fridkin Jul 2003

Comment On: 'Depolarization Corrections To The Coercive Field In Thin-Film Ferroelectrics', Stephen Ducharme, Vladimir Fridkin

Stephen Ducharme Publications

The Letter by Dawber et al. [J. Phys.: Condens. Matter 15 L393 (2003)] notes that incomplete screening in the electrodes of a ferroelectric capacitor can result in an underestimate for the true coercive field in films of nanometer thickness. We show that their estimate of the magnitude of this correction it too large in the case of ferroelectric copolymer Langmuir- Blodgett films and, as a result, invalidates the claim that finite-size scaling of the ferroelectric coercive field is evident in films thinner than 15 nm.

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Dynamics Of Phase Transitions On Low-Index Metal Surfaces, Bo Lin Apr 2003

Dynamics Of Phase Transitions On Low-Index Metal Surfaces, Bo Lin

Electrical & Computer Engineering Theses & Dissertations

The surface superheating and phase transitions at the low-index surface of metal were investigated using conventional continuous and 100-ps time-resolved reflection high-energy electron diffraction. Three metal surfaces, In(111), Au(110) and Pb(111), have been investigated in this work. The high temperature behavior of the In(111) surface was investigated using reflection high-energy electron diffraction with 100-ps temporal resolution. The change of surface vacancy density on In(111) is observed from 300 K to near the bulk melting point. The vacancy-formation energy of In(111) surface is estimated from experimental results. The surface vacancy density is observed to increase with temperature; however, the average random …

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Dielectric Properties Of A Ferroelectric Copolymer Langmuir–Blodgett Film, Mahantappa S. Jogad, Stephen Ducharme Aug 2002

Dielectric Properties Of A Ferroelectric Copolymer Langmuir–Blodgett Film, Mahantappa S. Jogad, Stephen Ducharme

Stephen Ducharme Publications

We report measurements of the real (epsilon prime) and imaginary (epsilon double-prime) parts of the relative complex permittivity of a Langmuir–Blodgett film of ferroelectric copolymer of vinylidene fluoride (70%) with trifluoroethylene (30%). The measurements were made in the temperature range of 35 to 125° C, and frequency range of 19 Hz to 5 MHz. The results indicate low frequency loss due to conduction and dielectric loss peak near the ferroelectric–paraelectric phase transition.

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Oxidation-Induced Stacking Fault In (100) And (111) Silicon Wafers, Mei Keat Liang Jan 2002

Oxidation-Induced Stacking Fault In (100) And (111) Silicon Wafers, Mei Keat Liang

Student Works (2000-2009)

Oxidation-induced stacking fault (OISF) dimension and density change on (100) and (111) wafers, as a result of repeated preferential etching were studied using AFM. optical microscope and angular polishing techniques. Density on (100) and (111) wafers is independent of surface removal up to 3.0µm. This indicates the single layer nature of OISF formed from the sand blasted wafer. Besides having higher density, OISFs from (100) wafer were longer than OISF from (111) wafer. OISF width increases linearly with surface removal however the length does not change significantly with surface removal. ln the OISF normal depth studies using angular polishing technique, …

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Effect Of Cr3+ And So42- On The Structure Of Rust Layer Formed On Steels By Atmospheric Corrosion, Masato Yamashita, Hitoshi Uchida,, Desmond C. Cook . Jan 2002

Effect Of Cr3+ And So42- On The Structure Of Rust Layer Formed On Steels By Atmospheric Corrosion, Masato Yamashita, Hitoshi Uchida,, Desmond C. Cook .

Physics Faculty Publications

The effect of chromium ion (Cr3+) and sulfate ion (SO42-) on the structure of the rust layer formed by thin electrolyte-film corrosion of low-alloy steels has been examined. By using X-ray diffraction spectroscopy, it was found that coexistence of Cr3+ and SO42- in the electrolyte film covering the steel surface quickly forms the Cr-goethite (α-(Fe 1-X, CrX)OOH) layer which has been known as the final protective rust layer. Scanning vibrating electrode measurements showed that the rust layer formed under the electrolyte film containing Cr3+ and SO42- …

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The Effect Of Aluminium Oxide And Cerium Oxide As Dispersoids In Chitosan-Lithium Acetate Complexes, Hoi Mien Leow Jan 2001

The Effect Of Aluminium Oxide And Cerium Oxide As Dispersoids In Chitosan-Lithium Acetate Complexes, Hoi Mien Leow

Student Works (2000-2009)

In this study, chitosan with 85% deacetylation was used with Ni(OAc)₂·2H₂O as doping salt and Al₂O₃, or CeO₂ as dispersoid. They were mixed in certain weight percentages and dissolved in 100ml of 0.5% acetic acid solution. These solutions were poured into petri dishes and left at room temperature for film formation. Infrared Spectroscopy has shown that there is interaction between chitosan and LiOAc with and without dispersoid. The peaks are shifted. broadened. split and differs in intensity. The electrical conductivity of all samples was calculated using the bulk resistance value obtained from the complex admittance plot. The highest electrical conductivity …

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Sulphide Based Materials As Potential Anodes In Lithium Ion Cells, Azlin Sanusi Jan 2001

Sulphide Based Materials As Potential Anodes In Lithium Ion Cells, Azlin Sanusi

Student Works (2000-2009)

Sulphides based compounds PbS and SnS have been studied as possible anode material in lithium ion cell. PbS was prepared by the chemical bath deposition technique and SnS by the double decomposition method. Both samples were characterized by the powder X-ray diffraction technique and energy dispersive analysis of X-rays (EDAX). The room temperature electrical conductivity of PbS is 2.6 x 10⁻⁴ S cm⁻¹ and SnS is 5.3 x 10⁻⁷ S cm⁻¹ while at 90°C the electrical conductivity of PbS is 3.3 x 10⁻⁴ S cm⁻¹ and SnS is 2.90 x 10⁻⁶ S cm⁻¹ Cyclic voltammetry determined the potential anode ability …

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Synthesis And Characterization Of Lithiated Mixed Metal Oxides For Lithium Ion Rechargeable Batteries, Seng Gee Tan Jan 2001

Synthesis And Characterization Of Lithiated Mixed Metal Oxides For Lithium Ion Rechargeable Batteries, Seng Gee Tan

Student Works (2000-2009)

Lilhiated mixed metal oxides for lithium ion rechargeable batteries were prepared by the sol gel technique. Samples consisting of lithium acetate, nickel nitrate, cobalt nitrate, manganese acetate and aluminium fluoride were characterised using X-ray Diffraction (XRD), Differential Scanning Calorimetry (DSC), Fourier Transform Infrared Spectroscopy (FTIRS). Energy Dispersive Analysis of X-rays (EDAX) w1d Cyclic Voltammetry (CV). Thermal characterization shows that the acetates, nitrates and fluorides of precursors material deform at temperature between 50° to 100°C and the products begin to form at a temperature between 264°C to 271°C. FTIR studies show that the materials must be heated for a longer time …

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Effects Of Argon Dilution Of Silane On The Optical Properties And Surface Morphology Of Hydrogenated Amorphous Silicon, Choon Kheam Lim Jan 2001

Effects Of Argon Dilution Of Silane On The Optical Properties And Surface Morphology Of Hydrogenated Amorphous Silicon, Choon Kheam Lim

Student Works (2000-2009)

Hydrogenated amorphous silicon (a.Si:H) was prepared using the d.c plasma grow discharge system. Two sets of samples were prepared and studied. The first set of samples referred to as the high argon dilution films were prepared from the discharge of pure silane at flow-rate of 5sccm and silane at the same flow-rate diluted in argon at flow-rates of 5, 10 and 15sccm. Similarly, the second set of sample referred to as the low argon dilution films were prepared from the discharge of pure silane at flow-rate of20sccm and silane at the same flow-rate diluted in argon at the flow-rates mentioned …

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Time-Resolved Structural Study Of Low-Index Surfaces Of Germanium Near Its Bulk Melting Temperature, Xinglin Zeng, H. E. Elsayed-Ali Jan 2001

Time-Resolved Structural Study Of Low-Index Surfaces Of Germanium Near Its Bulk Melting Temperature, Xinglin Zeng, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The structure of the low-index surfaces of germanium near its bulk melting temperature is investigated using 100-ps time-resolved reflection high-energy electron diffraction. The surface is heated by 100-ps laser pulses while a synchronized electron beam probes the structure. Ge(111)was observed to remain in its incomplete melting structure up to at least Tm + 134 ± 40 K when heated by a 100-ps laser pulse. Both the Ge(100) and Ge(110) surfaces are observed to melt near the bulk melting temperature when heated with 100-ps laser pulses. Because of the low-diffraction intensity-to-background ratio at high temperatures and because of the temperature …

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Mössbauer Effect Determination Of Relative Recoilless Fractions For Iron Oxides, Sei J. Oh, Desmond C. Cook Jan 1999

Mössbauer Effect Determination Of Relative Recoilless Fractions For Iron Oxides, Sei J. Oh, Desmond C. Cook

Physics Faculty Publications

The relative recoilless fraction (F-value) of each of six iron oxides, defined as the ratio of the recoil-free fractions of two different materials, was experimentally determined relative to hematite at 300 K and 77 K by Mössbauer spectroscopy. Using the relative recoil-free fractions compared to that of hematite, the relative recoilless fractions between all pairs of the seven iron oxides were determined. The F-values can allow conversion of Mössbauer subspectral areas to the relative atomic, molecular, or weight fractions of each iron oxide present in a mixed oxide phase sample.

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Time-Resolved Reflection High-Energy Electron Diffraction Study Of The Ge(111)-C(2×8)-(1×1) Phase Transition, Xinglin Zeng, Bo Lin, Ibrahim El-Kholy, Hani E. Elsayed-Ali Jan 1999

Time-Resolved Reflection High-Energy Electron Diffraction Study Of The Ge(111)-C(2×8)-(1×1) Phase Transition, Xinglin Zeng, Bo Lin, Ibrahim El-Kholy, Hani E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The dynamics of the Ge(111)-c(2×8)-(1×1) phase transition is investigated by 100-ps time-resolved reflection high-energy electron diffraction. A laser pulse heats the surface while a synchronized electron pulse is used to obtain the surface diffraction pattern. Slow heating shows that the adatoms in Ge(111)-c(2×8) start to disorder at ∼510 K and are converted to a disordered adatom arrangement at 573 K. For heating with 100-ps laser pulses, the Ge(111)-c(2×8) reconstructed adatom arrangement starts to disorder at 584±16K, well above the onset temperature of ∼510 K for the disordering of Ge(111)-c(2×8) observed for slow …

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Two-Dimensional Ferroelectric Films, Alexander V. Bune, Vladimir M. Fridkin, Stephen Ducharme, Lev M. Blinov, Serguei P. Palto, Alexander V. Sorokin, S. G. Yudin, A. Zlatkin Feb 1998

Two-Dimensional Ferroelectric Films, Alexander V. Bune, Vladimir M. Fridkin, Stephen Ducharme, Lev M. Blinov, Serguei P. Palto, Alexander V. Sorokin, S. G. Yudin, A. Zlatkin

Stephen Ducharme Publications

Ultrathin crystalline films offer the possibility of exploring phase transitions in the crossover region between two and three dimensions. Second- order ferromagnetic phase transitions have been observed in monolayer magnetic films [1,2], where surface anisotropy energy stabilizes the two-dimensional ferromagnetic state at finite temperature [3]. Similarly, a number of magnetic materials have magnetic surface layers that show a second-order ferromagnetic–paramagnetic phase transition with an increased Curie temperature [4]. Ferroelectricity is in many ways analogous to ferromagnetism, and bulk-like ferroelectricity and finite-size modifications of it have been seen in nanocrystals as small as 250 Å in diameter [5], in perovskite films …

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Surface Morphology Of Laser-Superheated Pb(111) And Pb(100), Z. H. Zhang, Bo Lin, X. L. Zeng, H. E. Elsayed-Ali Jan 1998

Surface Morphology Of Laser-Superheated Pb(111) And Pb(100), Z. H. Zhang, Bo Lin, X. L. Zeng, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The surface step density on the vicinal Pb(111) and the surface vacancy density on Pb(100) after laser superheating and melting are investigated using reflection high-energy electron diffraction. With ∼100-ps laser pulses, Pb(111) surface superheating does not significantly change the density of the steps and step-edge roughness. However, after laser surface melting, the average terrace width and the string length at the step edge become as large as those at room temperature. The average terrace width at 573 K changes from 38±15 to 64±19 Å after laser surface melting, while the average string length at the step edge changes from 90±14 …

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Temperature Dependence Of Step Density On Vicinal Pb(111), Z. H. Zhang, H. E. Elsayed-Ali Jan 1998

Temperature Dependence Of Step Density On Vicinal Pb(111), Z. H. Zhang, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The temperature dependence of step density on the vicinal Pb(111) surface is investigated using reflection high-energy electron diffraction. When the temperature is increased from 323 to 590 K. the average terrace width and the average string length at the step edge decrease from 85±25 to 37±16 Å and from 220±33 to 25±8 Å, respectively. Thermal step collapse on the Pb(111) surface near its bulk melting temperature is not observed. Above 530±7 K, the change in the string length at the step edge with temperature becomes small, and the intensity of the (00) beam is significantly decreased. We conclude that partial …

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Femtosecond Photoemission Study Of Ultrafast Electron Dynamics In Single-Crystal Au(111) Films, J. Cao, Y. Gao, H. E. Elsayed-Ali, R. J. D. Miller, D. A. Mantell Jan 1998

Femtosecond Photoemission Study Of Ultrafast Electron Dynamics In Single-Crystal Au(111) Films, J. Cao, Y. Gao, H. E. Elsayed-Ali, R. J. D. Miller, D. A. Mantell

Electrical & Computer Engineering Faculty Publications

The energy-dependent relaxation of photoexcited electrons has been measured by time-resolved two-photon photoemission spectroscopy on single-crystal Au(111) films with thickness ranging from 150 to 3000 Å. It is found that the energy-dependent relaxation does not show any significant thickness dependence, which indicates that electron transport is a much slower dynamical process in the near-surface region than expected from bulk properties. Furthermore, lifetimes of the photoexcited electrons can be fitted well by the Fermi-liquid theory with a scaling factor plus an effective upper lifetime. This observation enables separation of electron-electron scattering, and to a lesser extent electron-phonon scattering, processes from electron-transport …

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Femtosecond Photoemission Study Of Ultrafast Electron Dynamics On Cu(100), J. Cao, Y. Gao, R. J. D. Miller, Hani E. Elsayed-Ali, D. A. Mantell Jan 1997

Femtosecond Photoemission Study Of Ultrafast Electron Dynamics On Cu(100), J. Cao, Y. Gao, R. J. D. Miller, Hani E. Elsayed-Ali, D. A. Mantell

Electrical & Computer Engineering Faculty Publications

The energy dependence of the relaxation of photoexcited electrons in copper was measured using femtosecond time-resolved photoemission spectroscopy to within 0.3 eV above the Fermi level. By performing lifetime measurements under different surface conditions, several surface dynamical processes were investigated. In particular, an anomalous long lifetime feature, which cannot be explained with Fermi-liquid theory, was observed in the lifetime-energy curve. This feature was found originating from the photoexcitation of the strongly localized Cu 3d electrons. ©1997 American Physical Society

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Reflection High-Energy Electron-Diffraction Study Of Melting And Solidification Of Pb On Graphite, Z. H. Zhang, P. Kulatunga, H. E. Elsayed-Ali Jan 1997

Reflection High-Energy Electron-Diffraction Study Of Melting And Solidification Of Pb On Graphite, Z. H. Zhang, P. Kulatunga, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The melting and solidification of Pb thin films on pyrolytic graphite are investigated in situ by reflection high-energy electron diffraction. Thin films with thicknesses of 4-150 monolayers are investigated. The surface morphology of the thin films were studied by scanning electron microscopy. Superheating of the Pb thin films by 4±2 to 12±2 K is observed from diffraction intensity measurements. Upon cooling the substrate, the Pb on graphite is seen to supercool by ∼69±4 K.

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