Atomic, Molecular and Optical Physics Commons^™

Non-Gaussian Phenomena In Light Scattering And Applications, Shubham Atul Dawda

Graduate Studies Theses and Dissertations 2026

Physical reality is rarely deterministic; which, when probed by electromagnetic fields that also fluctuate, leads to observables that are most efficiently modelled as statistical processes. At equilibrium, this is usually achieved by invoking the Gaussian statistics of underlying physical processes, however, in practice, one often encounters out-of-equilibrium conditions where Gaussian descriptions may not suffice. Such situations are plentiful in nature– from biology to astronomy. This dissertation addresses several non-Gaussian phenomena associated with light scattering, and includes specific models’ derivations, experimental techniques developments, and demonstrations of potential applications. The systematic presentation will consider circumstances that infringe upon specific assumptions of the …

Investigation Of Laser Based Flow Diagnostics With Metastable Argon, Sterling S. Gordon

Physics Theses & Dissertations

The overarching motivation of this work is the development of seedless, non-intrusive, laser-based diagnostics for supersonic airflow in wind tunnels. To advance this goal, this dissertation fo-cuses on three-photon excitation in a research-grade argon beam within a tabletop vacuum system, which offers a controlled environment for testing and refining the approach. The chosen excitation scheme drives argon atoms to the 3d[5/2]₃ state using a pulsed Ti:Sapphire laser system, enabling time-of-flight (ToF) measurements on atoms that subsequently undergo a multi-step decay to the metastable 4s[3/2]₂ state. Although full realization of this excitation scheme was hindered by technical …

Interactions And Applications Of Optical Angular Momentum In Magneto-Optical Material, Seth R. Nelson

Dissertations, Master's Theses and Master's Reports

This dissertation explores the interactions and applications of optical angular momentum within magneto-optical materials. Beginning with a theoretical and experimental analysis of multiple reflection and refraction phenomena within magneto-optical material. We derive and verify the dependence of refractive indices on optical spin angular momentum and magneto-optical magnetization, resulting in nonreciprocal elliptical and linear polarization beam splitting effects and wavevector discretization. We fabricate a magnetless slab waveguide isolator with minimal optical loss. Extending our study to optical orbital angular momentum, we introduce a perturbation to the electronic transition model in bismuth-substituted iron garnets. We demonstrate that this perturbation leads to nonreciprocal …

Super-Resolution Magnetic Microscopy And Earth’S Field Magnetometry With Color Centers In Diamond, Nazanin Mosavian

Optical Science and Engineering ETDs

In recent years, the negatively charged nitrogen- vacancy (NV) center has emerged as a promising solid-state color center capable of measuring magnetic fields with high sensi- tivity and spatial resolution under ambient conditions. In this thesis I will discuss how we perform super resolution magnetic microscopy and acquire magnetic field images of nanoparticle samples at 100 nm resolution. I will explain how 3D flux concentrators increase magnetic field amplitude and allows us to measure vector component magnetic fields as low as 50 µT with a diamond magnetometer, without the use of an additional bias magnetic field. I also describe how …

Pt-Symmetry And Eigenmodes, Tamara Gratcheva

University Honors Theses

Spectra of systems with balanced gain and loss, described by Hamiltonians with parity and time-reversal (PT) symmetry is a rich area of research. This work studies by means of numerical techniques, how eigenvalues and eigenfunctions of a Schrodinger operator change as a gain-loss parameter changes. Two cases on a disk with zero boundary conditions are considered. In the first case, within the enclosing disk, we place a parity (P) symmetric configuration of three smaller disks containing gain and loss media, which does not have PT-symmetry. In the second case, we study a PT-symmetric configuration …

Nonlinear Rogue Wave Generation For All-Optical Switching In Optical Fibers And Photonic Integrated Circuits, Samuel Alexander Bechtold

Honors Program Theses and Projects

For my thesis we discuss the history of optics, electronics and photonicsproviding a framework from which I investigate the viability of engineering a Photonic Integrated Circuit (PIC) that takes advantage of the nonlinear optical process known as Rogue Wave Generation (RWG) for an all-optical switching mechanism that is capable of switching speeds in the Peta-Hertz (PHz) frequency regime. This topic is introduced through a discussion of how technological advances such as the transistor, laser and optical fiber made modern computing and telecommunications possible. This is followed by a theoretical explanation of the nonlinear optical phenomena known as supercontinuum generation (SCG) …

Development Of A High-Resolution Mid-Infrared Spectroscopy Apparatus For The Study Of Methane And Other Astrochemical Molecules., S M Shah Riyadh

Electronic Theses and Dissertations

This research documents steps towards building a novel spectroscopic technique, namely, cavity-enhanced double-resonance (CEDR) spectroscopy, for investigating methane (CH₄) and other molecules with significance in astrochemistry. These efforts focus on tackling the complexities of their ro-vibrational energy levels and the inefficiencies in analyzing vibrational spectra, particularly for molecules with high symmetry and strong intramolecular interactions. In the CEDR spectroscopy, the first photon, generated by a continuous-wave optical parametric oscillator (CW-OPO) locked to a Doppler-free saturation absorption line, excites the molecule from its ground level to a selected excited ro-vibrational (rotational-vibrational) level, e.g., that of the asymmetric CH-stretch mode. …

Advancements In Time Resolved Spectroscopy And Nonlinear Microscopy, Bryan Semon

Theses and Dissertations

Non-linear optical processes such as coherent anti-Stokes Raman scattering and sum frequency generation offer a view into the chemical and biological interactions of molecules that is distinctly different from linear techniques like near infra-red and fluorescence. This insight comes at a cost: non-linear techniques are more sensitive to external perturbations of the system, increasing the noise and decreasing the repeatability of the data. We work here on both aspects of these non-linear techniques, taking advantage of their power to offer new imaging techniques as well as working to quantify and reduce the non-resonant noise inherent to the system. In pursuit …

Quantitative, Photocurrent Multidimensional Coherent Spectroscopy, Adam Halaoui

Electronic Theses and Dissertations

Multidimensional coherent spectroscopy (MDCS) is a quickly growing field that has a lot of advantages over more conventional forms of spectroscopy. These advantages all come from the fact that MDCS allows us to get time resolved correlated emission and absorption spectra using very precisely chosen interactions between the density matrix and the excitation laser. MDCS spectra gives the researcher a lot of information that can be extracted purely through qualitative analysis. This is possible because state couplings are entirely separated on the spectra, and once we know how to read the data, we can see how carriers transport in the …

Developing A Data Acquisition System For Use In Cold Neutral Atom Traps, Jonathan E. Fuzaro Alencar

Physics

The rising interest in quantum computing has led to new quantum systems being developed and researched. Among these are trapped neutral atoms which have several desirable features and may be configured and operated on using lasers in an optical lattice. This work describes the development of a new data acquisition system for use in tuning lasers near the precise hyperfine transition frequencies of Rb 87 atoms, a crucial step in the functionality of a neutral atom trap. This improves on previous implementations that were deprecated and limited in laser frequency sweep range. Integration into the experiment was accomplished using an …

An Overview Of Lasers And Their Applications, Luis Cristian Giovanni Guerrero

Physics

This paper is an overview of lasers and their applications. The fundamentals of laser operation are covered as well as the various applications of advanced laser systems. The primary focus is to highlight some of the technological advancements made possible by lasers in the last half-century.

The Design Of A Continuous Wave Molecular Nitrogen Stimulated Raman Laser In The Visible Spectrum, Timothy J. Bate

Theses and Dissertations

Hollow-core photonic crystal fibers (HCPCFs) shows promise as a hybrid laser with higher nonlinear process limits and small beam size over long gain lengths. This work focuses on the design of a CW molecular nitrogen (N₂) stimulated Raman laser. N₂ offers Raman gains scaling up to 900 amg, scaling higher than H₂. The cavity experiment showed the need to include Rayleigh scattering in the high pressure required for N₂ Raman lasing. Even at relatively low pressure ssuch as 1,500 psi, high conversion percentages should be found if the fiber length is chosen based on …

Structuring Light For Investigating Optical Vortices, Andrew Voitiv, Mark Siemens

DU Undergraduate Research Journal Archive

Vortices are well known in our world: tornadoes, hurricanes, and quickly stirred iced tea all demonstrate the vortex phenomenon. In addition to these classical fluids, vortices exist in laser light. While classical fluid vortex dynamics is one of the oldest studied physics problems, the study of optical vortices is only a few decades old. Paralleling the community’s curiosity of quantized vortices in quantum fluids, such as super fluid helium and Bose-Einstein condensate, there is immense interest in the study of optical vortices. In this article, we cover the basic theory of structuring light to generate optical vortices and then discuss …

Excitable Interplay Between Lasing Quantum Dot States, Michael Dillane, I. Dubinkin, N. Fedorov, T. Erneux, David Goulding, B. Kelleher, E.A. Viktorov

Cappa Publications

The optically injected semiconductor laser system has proven to be an excellent source of experimental nonlinear dynamics, particularly regarding the generation of excitable pulses. Typically for low-injection strengths, these pulses are the result of a small above-threshold perturbation of a stable steady state, the underlying physics is well described by the Adler phase equation, and each laser intensity pulse is accompanied by a 2π phase rotation. In this article, we show how, with a dual-state quantum dot laser, a variation of type I excitability is possible that cannot be described by the Adler model. The laser is operated so that …

Monolayer Doping Of Silicon-Germanium Alloys: A Balancing Act Between Phosphorus Incorporation And Strain Relaxation, Noel Kennedy, Ray Duffy, Gioele Mirabelli, Luke Eaton, Nikolay Petkov, Justin D. Holmes, Chris Hatem, Lee Walsh, Brenda Long

Cappa Publications

This paper presents the application of monolayer doping (MLD) to silicon-germanium (SiGe). This study was carried out for phosphorus dopants on wafers of epitaxially grown thin films of strained SiGe on silicon with varying concentrations of Ge (18%, 30%, and 60%). The challenge presented here is achieving dopant incorporation while minimizing strain relaxation. The impact of high temperature annealing on the formation of defects due to strain relaxation of these layers was qualitatively monitored by cross-sectional transmission electron microscopy and atomic force microscopy prior to choosing an anneal temperature for the MLD drive-in. Though the bulk SiGe wafers provided are …

Slow Light With Interleaved P-N Junction To Enhance Performance Of Integrated Mach-Zehnder Silicon Modulators, Marco Passoni, Dario Gerace, Liam O'Faolain, Lucio Claudio Andreani

Cappa Publications

Slow light is a very important concept in nanophotonics, especially in the context of photonic crystals. In this work, we apply our previous design of band-edge slow light in silicon waveguide gratings [M. Passoni et al, Opt. Express 26, 8470 (2018)] to Mach-Zehnder modulators based on the plasma dispersion effect. The key idea is to employ an interleaved p-n junction with the same periodicity as the grating, in order to achieve optimal matching between the electromagnetic field profile and the depletion regions of the p-n junction. The resulting modulation efficiency is strongly improved as compared to common modulators based on …

Single Metalens For Generating Polarization And Phase Singularities Leading To A Reverse Flow Of Energy, Victor V. Kotlyar, Anton G. Nalimov, Sergey S. Stafeev, Liam O'Faolain

Cappa Publications

Using Jones matrices and vectors, we show that a metasurface-based optical element composed of a set of subwavelength diffraction gratings, whose anisotropic transmittance is described by a matrix of polarization rotation by angle m, where is the polar angle, generate an mth order azimuthally or radially polarized beam, when illuminated by linearly polarized light, or an optical vortex with topological charge m, when illuminated by circularly polarized light. Such a converter performs a spin–orbit transformation, acting similarly to a liquid-crystal half-wave plate. Using the FDTD-aided numerical simulation, we show that uniform linearly or circularly polarized light passing through the …

Subwavelength Grating-Based Spiral Metalens For Tight Focusing Of Laser Light, Victor V. Kotlyar, Sergey S. Stafeev, Anton G. Nalimov, Liam O'Faolain

Cappa Publications

In this paper, we investigate a 16-sector spiral metalens fabricated on a thin film (130 nm) of amorphous silicon, consisting of a set of subwavelength binary diffractive gratings and with a numerical aperture that is close to unity. The metalens converts linearly polarized incident light into an azimuthally polarized optical vortex and focuses it at a distance approximately equal to the wavelength of the incident light, k ¼ 633 nm. Using a scanning near-field optical microscope, it is shown experimentally that the metalens forms an elliptical focal spot with diameters smaller than the diffraction limit: FWHMx ¼ 0.32k (60.03k) and …

Rotation Of Two-Petal Laser Beams In The Near Field Of A Spiral Microaxicon, S. S. Stafeev, Liam O'Faolain, M. V. Kotlyar

Cappa Publications

Using a spiral microaxicon with the topological charge 2 and NA = 0.6 operating at a 532-nm wavelength and fabricated by electron-beam lithography, we experimentally demonstrate the rotation of a two-petal laser beam in the near field (several micrometers away from the axicon surface). The estimated rotation rate is 55 °/mm and linearly dependent on the on-axis distance, with the theoretical rotation rate being 53 °/mm. The experimentally measured rotation rate is found to be linear and coincident with the simulation results only on the on-axis segment from 1.5 to 3 mm. The experimentally measured rotation rate is 66 °/mm …

Assembling And Characterizing The Efficiency Of An Injection Locked Laser System For Cold Neutral Atom Optical Traps, Alexandra Papa Crawford

Physics

Creating a quantum computer requires a system of particles that can be well-controlled to achieve quantum operations. We need a large array of these particles – called qubits – with long coherence times, which can be initialized, operated on by single and two qubit gates, and read out. For neutral atoms, the qubit states are stable ground states that interact minimally with the environment, leading to long coherence times. Experimentally, the qubits are manipulated using carefully timed laser beam pulses with controlled frequency and intensity, but the outstanding issue for optically trapping cold atoms is finding a light pattern that …

Precision Spectroscopy Of Beryllium, Advik D. Vira

Theses, Dissertations, and Projects

We report on the calibration and absolute frequency results for the 2s2p1P1 state in neutral atomic beryllium-9. We start off with a discussion of the method used to calibrate the laser, which includes a detailed explanation of the basic physics involved, and then discuss the results for the lowest singlet state in neutral beryllium-9. We discuss a way to predict the spectra using optical Bloch equations and then present and analyze the experimental results. We found the absolute frequency for the 1P1 state to be 42565.4487(30) cm-1, which is in agreement with the current best theoretical estimateof42565.441(11)cm-1 [49]. Amoresophisticatedanalyticaltechniqueisproposed; however, …

Tunable Optical Buffer Through An Analogue To Electro-Magnetically Induced Transparency In Coupled Photonic Crystal Cavities, Changyu Hu, Sebastian A. Schulz, Alexandros A. Liles, Liam O'Faolain

Cappa Publications

Tunable on-chip optical delay has long been a key target for the research community, as it is the enabling technology behind delay lines, signal re-timing and other applications vital to optical signal processing. To date the field has been limited by high optical losses associated with slow light or delay structures. Here, we present a novel tunable delay line, based on a coupled cavity system exhibiting an Electromagnetically Induced Transparency-like transmission spectrum, with record low loss, around 15dB/ns. By tuning a single cavity the delay of the complete structure can be tuned over 120ps, with the maximum delay approaching 300ps.

Analysis Of The Red And Green Optical Absorption Spectrum Of Gas Phase Ammonia, Nikolai F. Zobov, Phillip A. Coles, Roman I. Ovsyannikov, Aleksandra A. Kyuberis, Robert J. Hargreaves, Peter F. Bernath, Jonathan Tennyson, Sergei N. Yurchenko, Oleg L. Polyansky

Chemistry & Biochemistry Faculty Publications

Room temperature NH₃ absorption spectra recorded at the Kitt Peak National Solar Observatory in 1980 are analyzed. The spectra cover two regions in the visible: 15,200 - 15,700 cm^-1 and 17,950 - 18,250 cm^-1. These high overtone rotation-vibration spectra are analyzed using both combination differences and variational line lists. Two variational line lists were computed using the TROVE nuclear motion program: one is based on an ab initio potential energy surface (PES) while the other used a semi-empirical PES. Ab initio dipole moment surfaces are used in both cases. 95 energy levels with J = 1 …

Studies In Mesoscopics And Quantum Microscopies, Zhenghao Ding, Gabriel C. Spalding

Honors Projects

This thesis begins with a foundational section on quantum optics. The single-photon detectors used in the first chapter were obtained through the Advanced Laboratory Physics Association (ALPhA), which brokered reduced cost for educational use, and the aim of the single-photon work presented in Chapter 1 is to develop modules for use in Illinois Wesleyan's instructional labs beyond the first year of university. Along with the American Association of Physics Teachers, ALPhA encourages capstone-level work, such as Chapter 1 of this honors thesis, which is explicitly designed to play the role of passing on, to a next generation of physics majors, …

Using An Atomic Molecular Optics Laboratory For Undergraduate Research And Mentoring Of Physics Students In Georgia, Matthew P. Dallas

Georgia College Student Research Events

Using an Atomic Molecular Optics Laboratory for Undergraduate Research and Mentoring of Physics Students in Georgia

An Atomic and Molecular Optical (AMO) Physics research lab is an excellent tool to train and mentor undergraduate students in advanced laboratory techniques. Students gain valuable basic experience in experimental designs, data acquisition techniques, working with high precision optical equipment, building electronics, and working in the machine shop. The current project is building and testing an enclosure for the diode laser to reduce sound and vibrational interference. In addition, we are developing and evaluating a new, more compact laser cavity which is 3d printed. …

Experimental Realization Of Slowly Rotating Modes Of Light, Fangzhao A. An

HMC Senior Theses

Beams of light can carry spin and orbital angular momentum. Spin angular momentum describes how the direction of the electric field rotates about the propagation axis, while orbital angular momentum describes the rotation of the field amplitude pattern. These concepts are well understood for monochromatic beams, but previous theoretical studies have constructed polychromatic superpositions where the connection between angular momentum and rotation of the electric field becomes much less clear. These states are superpositions of two states of light carrying opposite signs of angular momentum and slightly detuned frequencies. They rotate at the typically small detuning frequency and thus we …

Forcing Mutual Coherence In Diode Laser Stacks, Jonathan R. Wurtz

Honors Theses and Capstones

This paper will discuss both theoretical and experimental attempts to improve the spatial beam quality of diode laser stacks using an external optical system. An overview and derivation of the mathematics of both the optical system and diode lasers will be discussed. The experimental setup will be presented, as well as the fundamental theoretical and experimental results that suggest the external optical system used for this thesis fails to improve the beam quality of a diode laser stack.

Computational Renormalization Scheme For Quantum Field Theories, Rainer Grobe, Qichang Su, R E. Wagner

Faculty publications – Physics

We propose an alternative technique for numerically renormalizing quantum field theories based on their Hamiltonian formulation. This method is nonperturbative in nature and, therefore, exact to all orders. It does not require any correlation functions or Feynman diagrams. We illustrate this method for a model Yukawa-like theory describing the interaction of electrons and positrons with model photons in one spatial dimension. We show that, after mass renormalization of the fermionic and bosonic single-particle states, all other states in the Fock space have finite energies, which are independent of the momentum cutoff.

Enhancement Of Electron-Positron Pair Creation Due To Transient Excitation Of Field-Induced Bound States, M Jiang, Q Z. Lv, Z M. Sheng, Rainer Grobe, Qichang Su

Faculty publications – Physics

We study the creation of electron-positron pairs induced by two spatially separated electric fields that vary periodically in time. The results are based on large-scale computer simulations of the time-dependent Dirac equation in reduced spatial dimensions. When the separation of the fields is very large, the pair creation is caused by multiphoton transitions and mainly determined by the frequency of the fields. However, for small spatial separations a coherence effect can be observed that can enhance or reduce the particle yield compared to the case of two infinitely separated fields. If the travel time for a created electron or positron …

Pair Creation For Bosons In Electric And Magnetic Fields, Q Z. Lv, A C. Su, M Jiang, Rainer Grobe, Qichang Su

Faculty publications – Physics

By solving the quantum field theoretical version of the Klein-Gordon equation numerically, we study the creation process for charged boson-antiboson pairs in static electric and magnetic fields. The fields are perpendicular to each other and spatially localized along the same direction, which permits us to study the crucial impact of the magnetic field's spatial extension on dynamics. If its width is comparable to that of the electric field, we find a magnetically induced Lorentz suppression of the pair-creation process. When the width is increased such that the created bosons can revisit the interaction region, we find a region of exponential …