Atomic, Molecular and Optical Physics Commons^™

Topics In Three-Dimensional Imaging, Source Localization And Super-Resolution, Zhixian Yu

Physics & Astronomy ETDs

The realization that twisted light beams with helical phasefronts could carry orbital angular momentum (OAM) that is in excess of the photon's spin angular momentum (SAM) has spawned various important applications. One example is the design of novel imaging systems that achieve three-dimensional (3D) imaging in a single snapshot via the rotation of point spread function (PSF).

Based on a scalar-field analysis, a particular simple version of rotating PSF imagery, which was proposed by my advisor Dr. Prasad, furnishes a practical approach to perform 3D source localization using a spiral phase mask that generates a combination of Bessel vortex beams. …

Analytic Description Of High-Order Harmonic Generation In The Adiabatic Limit With Application To An Initial S State In An Intense Bicircular Laser Pulse, M. V. Frolov, N. L. Manakov, A. A. Minina, A. A. Silaev, N. V. Vvedenskii, M. Yu. Ivanov, Anthony F. Starace

Anthony F. Starace Publications

An analytic description of high-order harmonic generation (HHG) is proposed in the adiabatic (low-frequency) limit for an initial s state and a laser field having an arbitrary wave form. The approach is based on the two-state time-dependent effective range theory and is extended to the case of neutral atoms and positively charged ions by introducing ad hoc the Coulomb corrections for HHG. The resulting closed analytical form for the HHG amplitude is discussed in terms of real classical trajectories. The accuracy of the results of our analytic model is demonstrated by comparison with numerical solutions of the time-dependent Schrödinger equation …

Scope Of Self-Interacting Thermal Wimps In A Minimal U(1) D Extension And Its Future Prospects, Rahool Kumar Barman, Biplob Bhattacherjee, Arindam Chatterjee, Arghya Choudhury, Aritra Gupta

Journal Articles

In this work we have considered a minimal extension of Standard Model by a local U(1) gauge group in order to accommodate a stable (fermionic) Dark Matter (DM) candidate. We have focussed on parameter regions where DM possesses adequate self-interaction, owing to the presence of a light scalar mediator (the dark Higgs), alleviating some of the tensions in the small-scale structures. We have studied the scenario in the light of a variety of data, mostly from dark matter direct searches, collider searches and flavor physics experiments, with an attempt to constrain the interactions of the standard model (SM) particles with …

Free Electron Sources And Diffraction In Time, Eric R. Jones

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The quantum revolution of the last century advanced synergistically with technology, for example, with control of the temporal and spatial coherence, and the polarization state of light. Indeed, experimental confirmation of the quirks of quantum theory, as originally highlighted by Einstein, Podolsky, and Rosen, through Bohm, and then Bell, have been performed with photons, i.e., electromagnetic wave packets prepared in the same quantum states. Experimental tests of quantum mechanics with matter wave packets have been limited due to challenges in preparing all of the packets with similar quantum states. While great strides have been made for trapped atoms and Bose-Einstein …

A Theoretical Investigation Of Small Organic Molecules On Transition Metal Surfaces, Walter Malone

Electronic Theses and Dissertations

With the ever growing number of proposed desnity functional theory (DFT) functionals it becomes necessary to thoroughly screen any new method to determine its merit. Especially relevant methods include a proper description of the van der Waals (vdW) interaction, which can prove vital to a correct description of a myriad of systems of technological importance. The first part of this dissertation explores the utility of several vdW-inclusive DFT functionals including optB86b-vdW, optB88-vdW, optPBE-vdW, revPBE-vdW, rPW86-vdW2, and SCAN+rVV10 by applying them to model systems of small organic molecules, pyridine and thiophene, on transition metal surfaces. Overall, we find the optB88-vdW functional …

Large-Scale Atomistic Simulations Of Complex And Functional Properties Of Ferroic Materials, Raymond Thomas Walter

Graduate Theses and Dissertations

Ferroelectric (FE) nanostructures have attracted considerable attention as our abilities improve to synthesize them and to predict their properties by theoretical means. Depolarizing field effects at interfaces of FE heterostructures are particularly notable for causing topological defects such as FE vortices and negative dielectric responses in superlattices. In this thesis, I employ two large-scale atomistic techniques, the first-principles-based effective Hamiltonian (HEff) method and the linear-scaling three-dimensional fragment (LS3DF) method. I use these methods to explore optical rotation in FE vortices, electro-optic effects in FE vortices and skyrmions, and voltage amplification via negative capacitance in ferroelectric-paraelectric superlattices. We employ HEff in …

Chemistry And Dissipation At Mineral Surfaces In The Space Environment, William Tucker

Electronic Theses and Dissertations

The composition and morphology of mineral surfaces is known to play an important role in various phenomena relevant to planetary science. For example, the synthesis and processing of complex organics likely occurs at mineral surfaces strongly affected by the space environment. Furthermore, the dissipative and adhesive properties of dust grains may depend strongly on the chemical state of the surface including the presence of dangling bonds, adsorbates, and radicals. In this dissertation, experimental results are first presented which demonstrate that mineral grains subjected to high temperatures in a reducing environment lead to iron nanoparticles which are strongly catalytic for the …

The Population Densities Of Argon Metastable Levels, Nada Khogeer, Chelsy Gonzalez, Milka Nikolic

Physics and Astronomy

In this experiment, we used the optical emission spectroscopy (OES) method to obtain the main properties of low temperature Argon plasma. The experiment was sustained in powers and pressures that ranges from 30-100 W and 15-100 mTorr. We used numerical methods for the Argon kinetic model to calculate metastable levels and resonant states for the first excited states in low temperature Argon plasma. By finding the ratio of two spectral lines and finding another ratio from a different upper energy level that goes down to the same two lower energy levels, we can construct a system of two nonlinear equations. …

Origin Of Enhanced Anisotropy In Fept-C Granular Films Revealed By Xmcd, Robert Streubel, Alpha T. N'Diaye, Kumar Srinivasan, Antony Ajan, Peter Fischer

Robert Streubel Papers

We study the effect of carbon segregants on the spin and orbital moments of L10 FePt granular media using x-ray magnetic circular dichroism (XMCD) spectroscopy and report an effective decoupling of the structural film properties from the magnetic parameters of the grains. The carbon concentration reduces the grain size from (200 ± 160) nm2 down to (50 ± 20) nm2 for 40 mol. %C and improves sphericity and the order of grains, while preserving the crystalline order, spin and orbital moments, and perpendicular magnetocrystalline anisotropy. We identify the primary cause of enhanced saturation and coercive fields as the reduced demagnetization …

High Resolution Near-Infrared/Visible Intracavity Laser Spectroscopy Of Small Molecules, Jack Harms

Dissertations

Intracavity laser spectroscopy has been used to study the electronic structure of several small molecules. The molecules studied as part of this dissertation include germanium hydride (GeH), copper oxide (CuO), nickel chloride (NiCl), platinum fluoride (PtF), platinum chloride (PtCl), and copper hydroxide (CuOH). This work encompasses five peer-reviewed publications and two submitted manuscripts.

Single Metalens For Generating Polarization And Phase Singularities Leading To A Reverse Flow Of Energy, Victor V. Kotlyar, Anton G. Nalimov, Sergey S. Stafeev, Liam O'Faolain

Cappa Publications

Using Jones matrices and vectors, we show that a metasurface-based optical element composed of a set of subwavelength diffraction gratings, whose anisotropic transmittance is described by a matrix of polarization rotation by angle m, where is the polar angle, generate an mth order azimuthally or radially polarized beam, when illuminated by linearly polarized light, or an optical vortex with topological charge m, when illuminated by circularly polarized light. Such a converter performs a spin–orbit transformation, acting similarly to a liquid-crystal half-wave plate. Using the FDTD-aided numerical simulation, we show that uniform linearly or circularly polarized light passing through the …

Roadmap On Superoscillations, Michael Berry, Nicolay Zheludev, Yakir Aharonov, Fabrizio Colombo, Irene Sabadini, Daniele C. Struppa, Jeff Tollaksen, Edward T. F. Rogers, Fei Qin, Minghui Hong, Xiangang Luo, Roei Remez, Ady Arie, Jörg B. Götte, Mark R. Dennis, Alex M. H. Wong, George V. Eleftheriades, Yaniv Eliezer, Alon Bahabad, Gang Chen, Zhongquan Wen, Gaofeng Liang, Chenglong Hao, C-W Qiu, Achim Kempf, Eytan Katzav, Moshe Schwartz

Mathematics, Physics, and Computer Science Faculty Articles and Research

Superoscillations are band-limited functions with the counterintuitive property that they can vary arbitrarily faster than their fastest Fourier component, over arbitrarily long intervals. Modern studies originated in quantum theory, but there were anticipations in radar and optics. The mathematical understanding—still being explored—recognises that functions are extremely small where they superoscillate; this has implications for information theory. Applications to optical vortices, sub-wavelength microscopy and related areas of nanoscience are now moving from the theoretical and the demonstrative to the practical. This Roadmap surveys all these areas, providing background, current research, and anticipating future developments.

Subwavelength Grating-Based Spiral Metalens For Tight Focusing Of Laser Light, Victor V. Kotlyar, Sergey S. Stafeev, Anton G. Nalimov, Liam O'Faolain

Cappa Publications

In this paper, we investigate a 16-sector spiral metalens fabricated on a thin film (130 nm) of amorphous silicon, consisting of a set of subwavelength binary diffractive gratings and with a numerical aperture that is close to unity. The metalens converts linearly polarized incident light into an azimuthally polarized optical vortex and focuses it at a distance approximately equal to the wavelength of the incident light, k ¼ 633 nm. Using a scanning near-field optical microscope, it is shown experimentally that the metalens forms an elliptical focal spot with diameters smaller than the diffraction limit: FWHMx ¼ 0.32k (60.03k) and …

Testing Quantum Coherence In Stochastic Electrodynamics With Squeezed Schrödinger Cat States, Wayne Cheng-Wei Huang, Herman Batelaan

Department of Physics and Astronomy: Faculty Publications

The interference pattern in electron double-slit diffraction is a hallmark of quantum mechanics. A long-standing question for stochastic electrodynamics (SED) is whether or not it is capable of reproducing such effects, as interference is a manifestation of quantum coherence. In this study, we used excited harmonic oscillators to directly test this quantum feature in SED. We used two counter-propagating dichromatic laser pulses to promote a ground-state harmonic oscillator to a squeezed Schrödinger cat state. Upon recombination of the two well-separated wavepackets, an interference pattern emerges in the quantum probability distribution but is absent in the SED probability distribution. We thus …

Novel Data Analysis Methods In Multi-Channel And Multi-State Binding Experiments, Joseph Tibbs, Elizabeth Boehm, Wayne Bowie, Todd Washington, Maria Spies, Ali Tabei

Research in the Capitol

Single-Molecule studies use advanced microscopy techniques to view biomolecules, such as proteins and DNA, individually. On a slide, fluorescently-labeled molecules are immobilized and imaged using lasers, and the patterns of fluorescence can give important information about the interactions of multiple molecules. To extract this information, advanced, customizable data analysis tools must be created. The first goal is to create a method to robustly normalize (correct for brightness) single-channel fluorescence data. The second goal is to extend pattern recognition of binding order to multi-state and multi-channel binding patterns. The KERA 3.0 suite links creative pattern-recognition and normalization techniques with the abilities …

Perturbative Generalization Of Nonparaxial Ultrashort Tightly-Focused Elegant Laguerre–Gaussian Beams, Andrew M. Vikartofsky

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

An analytical method for calculating the electromagnetic fields of a nonparaxial elegant Laguerre-Gaussian (eLG) vortex beam is presented for arbitrary pulse duration, spot size, and LG mode. This perturbative approach provides a numerically tractable model for the calculation of arbitrarily high radial and azimuthal LG modes in the nonparaxial regime, without requiring integral representations of the fields. A key feature of this perturbative model is its use of a Poisson-like frequency spectrum, which allows for the proper description of pulses of arbitrarily short duration. The time-domain representation of this model is presented as a non-recursive closed-form expression to any order …

Optical Excitation Of Metastable Krypton And Photoassociative Spectroscopy Of Ultracold Rbar, Grady R. White

Physics Theses & Dissertations

In this presentation, we discuss results from two separate bodies of work. In the first, we investigate all-optical excitation methods to produce metastable-state krypton. The high energies required to excite rare gases out of their ground state present a unique challenge in the context of laser experiments. Laser physics work with rare gases often relies on excitation within an RF discharge. All-optical excitation is a promising replacement for RF discharges, avoids problems caused by ion production and may eventually allow for higher efficiencies. We examine three separate methods of all-optical metastable-state production: using an ArF excimer laser, using the third …

Investigating The Talbot Effect In Arrays Of Optical Dipole Traps For Neutral Atom Quantum Computing, Sergio Aguayo

Physics

Quantum computers are devices that are able to perform calculations not achievable for classical computers. Although there are many methods for creating a quantum computer, using neutral atoms offers the advantage of being stable when compared to other methods. The purpose of this investigation is to explore possible optical dipole trap configurations that would be useful for implementing a quantum computer with neutral atoms. Specifically, we computationally investigate arrays of pinholes, the diffraction pattern generated by them, and the onset of the Talbot effect in these traps. We manipulate the radius of the pinholes, the number of pinholes in the …

Magnetization Reversal And Local Switching Fields Of Ferromagnetic Co/Pd Microtubes With Radial Magnetization, Norbert Puwenberg, Christopher F. Reiche, Robert Streubel, Mishal Khan, Dipankar Mukherjee, Ivan V. Soldatov, Michael Melzer, Oliver G. Schmidt, Bernd Büchner, Thomas Mühl

Robert Streubel Papers

Three-dimensional nanomagnetism is a rapidly growing field of research covering both noncollinear spin textures and curved magnetic geometries including microtubular structures. We spatially resolve the field-induced magnetization reversal of free-standing ferromagnetic microtubes utilizing multifrequency magnetic force microscopy (MFM). The microtubes are composed of Co/Pd multilayer films with perpendicular magnetic anisotropy that translates to an anisotropy with radial easy axis upon rolling-up. Simultaneously mapping the topography and the perpendicular magnetostatic force derivative, the relation between surface angle and local magnetization configuration is evaluated for a large number of locations with slopes exceeding 45 degrees. The angle-dependence of the switching field is …

Compact Optical Frequency Standards For Future Applications Beyond The Laboratory, Kyle Martin

Physics & Astronomy ETDs

Atomic clocks provide one of the fundamental building blocks upon which modern telecommunications systems are constructed. Since the invention of the frequency comb in the early 2000s, laboratory frequency standards have quickly outpaced their compact counterparts. Compact clocks, however, have continued to leverage microwave transitions not yet exploring the advantages of an optical atomic clock. With the recent development of robust frequency combs compact optical clocks can now be realized. In this dissertation two atomic species are investigated for a compact atomic frequency standards. Both of these clocks are in different development stages but offer unique advantages. The optical rubidium …

Development Of A Model For 11C Production Via The 14N(P,Α) Reaction Using A Ge Pettrace Cyclotron, Amy C. Hall

Theses and Dissertations

The GE PETtrace 800 Series cyclotron at the Missouri University Research Reactor (MURR) facility is used extensively for medical and research radioisotope production. However, no model exists of its radioisotope production performance, and the energy, full intensity, and spatial profile of the cyclotron proton beam has never been measured. To improve production planning for research and medical isotopes, a MCNP6 model of the isotope production process was developed to maximize efficiency in target design and better understand irradiation conditions. Since the cyclotron beam energy and profile has a significant impact on the types of reactions that take place and the …

Sheet Velocity Measurements Using Laser Absorption Spectroscopy In A Xenon Hall Effect Thruster Plume, Avery W. Leonard

Theses and Dissertations

A new laser absorption spectroscopy (LAS) velocimetry system, designed to obtain 2D planar velocity fields for ionized Xenon in the plume of a Hall effect thruster by probing the transition of Xe II at 834.72 nm, was implemented at the Air Force Institute of Technology (AFIT) Space Propulsion Analysis and System Simulator (SPASS) Lab vacuum chamber. A single horizontal laser sheet was used to probe singly-ionized Xenon in the plume of a Busek BHT-600 Hall thruster and obtain a histogram of estimated axial velocity, to validate the system. Similar velocities to those obtained by an earlier intrusive characterization of the …

Characterization And Anomalous Diffusion Analysis Of A 100w Low Power Annular Hall Effect Thruster, Megan N. Maikell

Theses and Dissertations

A Busek 100W low-power annular Hall effect thruster was characterized to determine the thruster’s best operating parameter range and to study plasma oscillations within the thruster. These experiments were conducted using xenon gas in the Space Propulsion Analysis and System Simulator chamber at the Air Force Institute of Technology on Wright-Patterson Air Force Base. The thruster’s performance characteristics were evaluated at nominal discharge voltages and constant total mass flow rate, solenoid current, and keeper current to determine the operating conditions optimizing divergence angle, beam efficiency, and discharge loss. This was accomplished using a Faraday probe to determine the plume’s current …

Violation Of Centrosymmetry In Time-Resolved Coherent X-Ray Diffraction From Rovibrational States Of Diatomic Molecules, Hua-Chieh Shao, Anthony F. Starace

Anthony F. Starace Publications

Owing to increasing applications of time-resolved coherent x-ray scattering for the investigation of molecular reaction dynamics, we develop a theoretical model for time-dependent x-ray diffraction from molecular and/or electronic motion in molecules. Our model shows that the violation of centrosymmetry (VOC) is a general phenomenon in time-resolved diffraction patterns. We employ our theoretical model to illustrate the VOC in time-resolved coherent x-ray diffraction from two oriented diatomic molecules undergoing rovibrational motion: lithium hydride (LiD) and hydrogen (HD). Our simulations show asymmetric x-ray diffraction images that reflect the directions of the molecular motions.

Optimization Of Quantum Optical Metrology Systems, Nicholas Michael Studer

LSU Doctoral Dissertations

It can be said that all of humanity's efforts can be understood as a problem of optimization. We each have a natural sense of what is ``good'' or ``bad'' and thus our actions tend towards maximizing -- or optimizing -- some notion of good and minimizing those things we perceive as bad or undesirable.

Within the sciences, the greatest form of good is knowledge. It is this pursuit of knowledge that leads to not only life-saving innovations and technology, but also to furthering our understanding of our natural world and driving our philosophical pursuits.

The principle method of obtaining knowledge …

Measurement Of Solar Spectral Irradiance And Surface Ozone At Carrollton, Georgia, Usa, During The Great American Eclipse On 21 August 2017, Kirthi Tennakone, L Ajith Desilva, Charles A. Zander*, Shea Rose, Austin B. Kerlin

Georgia Journal of Science

Measurements conducted at the University of West Georgia, Carrollton, Georgia, during the time of the solar eclipse of 21^st August 2017 demonstrated that the integrated spectral irradiance in defined wavelength ranges in the ultraviolet and visible calculated as a fraction of the total irradiance reached a minimum at maximum obscuration of the Sun, whereas in an infrared range it was maximum. The method of analysis adopted supports the view that the changes in spectral irradiance during highly obscured partial phases is a consequence of limb darkening. In a surface ozone measurement, a minimum in ozone concentration occurred 30 +_ …

Phase Estimation In Linear And Nonlinear Interferometers, Sushovit Adhikari

LSU Doctoral Dissertations

Phase estimation has a wide range of applications. Over the years, several strategies have been studied to improve precision in phase estimation. These strategies include using exotic quantum states to quantum detection schemes. This dissertation summarizes my effort in improving the precision of phase estimation with a linear and nonlinear interferometer.

Chapter 1 introduces quantum optics and quantum metrology. I introduce all relevant quantum states of light used. We also look into tools and terminologies of quantum metrology such as Fisher information, shot-noise limit, Heisenberg limit, etc., along with examples of phase estimation with a Mach-Zehnder interferometer.

In Chapter 2, …

X-Ray Ptychography On Low-Dimensional Hard-Condensed Matter Materials, Xiaowen Shi, Nicolas Burdet, Bo Chen, Gang Xiong, Robert Streubel, Ross Harder, Ian K. Robinson

Robert Streubel Papers

Tailoring structural, chemical, and electronic (dis-)order in heterogeneous media is one of the transformative opportunities to enable new functionalities and sciences in energy and quantum materials. This endeavor requires elemental, chemical, and magnetic sensitivities at the nano/atomic scale in two- and three-dimensional space. Soft X-ray radiation and hard X-ray radiation provided by synchrotron facilities have emerged as standard characterization probes owing to their inherent element-specificity and high intensity. One of the most promising methods in view of sensitivity and spatial resolution is coherent diffraction imaging, namely, X-ray ptychography, which is envisioned to take on the dominance of electron imaging techniques …

Exploring Laser Induced Breakdown Spectroscopy (Libs) For Post-Detonation Nuclear Forensics Debris Analysis, Justin Knoll, Chad Schools, David Fobar

Purdue Workshop on Nonproliferation: Technology and Approaches

In the unlikely but catastrophic event of a nuclear terrorist attack our government leadership will need reliable information to rapidly inform critical decisions. This research explores the use of Laser Induced Breakdown Spectroscopy (LIBS) as a potential analysis tool in the National Technical Nuclear Forensics process. The current state of post detonation nuclear forensics requires ground and air samples be collected and shipped to state-of-the-art laboratories for radiochemical analysis. The samples undergo many measurements and useable data is produced as these measurements are completed. This data flows back into the process to guide additional measurements and inform the process of …

Kondo Signatures Of A Quantum Magnetic Impurity In Topological Superconductors, Rui Wang, Wei-Yi Su, Jian-Xin Zhu, Chin-Sen Ting, Hai Li, Changfeng Chen, Baigeng Wang, Xiaoqun Wang

Physics & Astronomy Faculty Research

We study the Kondo physics of a quantum magnetic impurity in two-dimensional topological superconductors (TSCs), either intrinsic or induced on the surface of a bulk topological insulator, using a numerical renormalization group technique. We show that, despite sharing the p+ip pairing symmetry, intrinsic and extrinsic TSCs host different physical processes that produce distinct Kondo signatures. Extrinsic TSCs harbor an unusual screening mechanism involving both electron and orbital degrees of freedom that produces rich and prominent Kondo phenomena, especially an intriguing pseudospin Kondo singlet state in the superconducting gap and a spatially anisotropic spin correlation. In sharp contrast, intrinsic TSCs support …