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Ionization

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Articles 91 - 101 of 101

Full-Text Articles in Physics

Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson Oct 1998

Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson

Chemistry and Biochemistry Faculty Research

The production and subsequent autoionization of the Ar+ (1D2)6d1 satellite state that is formed either by shake-up or recapture during the Auger decay of a 2p vacancy in Ar has been studied by photoelectron spectroscopy in the energy region from 243 to 256 eV. The creation of near zero energy electrons below and immediately above the Ar 2p ionization threshold is discussed. Some ambiguous points in previous studies are clarified.

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Double Photoionization Of Helium, James A.R. Samson, Wayne C. Stolte, Z. X. He, Y. Lu, J. N. Cutler, R. J. Bartlett Mar 1998

Double Photoionization Of Helium, James A.R. Samson, Wayne C. Stolte, Z. X. He, Y. Lu, J. N. Cutler, R. J. Bartlett

Chemistry and Biochemistry Faculty Research

The cross sections for double photoionization of helium and the ratios of double to single ionization have been measured from the double-ionization threshold to 820 eV. The results are in very good agreement with several recent calculations.

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Time-Resolved Studies Of Ultracold Ionizing Collisions, Scott D. Bergeson, C. Orzel, S. Kulin, S. L. Rolston Jan 1998

Time-Resolved Studies Of Ultracold Ionizing Collisions, Scott D. Bergeson, C. Orzel, S. Kulin, S. L. Rolston

Faculty Publications

Using 40 ns laser pulses, we probe the real-time dynamics of ultracold ionizing collisions in metastable xenon. We time resolve both shielding and enhancement effects, and observe the production of Xe2^+ molecular ions through associative ionization. We estimate the rate of molecule formation in excited-state collisions, and directly measure the role of both flux enhancement and excited state survival in the collisional enhancement process. Conceptually simple theoretical models are used to predict the dynamics of the collisional shielding.

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Cross Sections For The Production Of He+ (Np) 2p0 States By 50 To 150 Kev Proton Impact On Helium, Wayne C. Stolte, R. Bruch Sep 1996

Cross Sections For The Production Of He+ (Np) 2p0 States By 50 To 150 Kev Proton Impact On Helium, Wayne C. Stolte, R. Bruch

Chemistry and Biochemistry Faculty Research

Cross sections have been measured for the production of He+ (np) 2Po states, n=2,3,4, by proton impact on helium over a projectile velocity range of 1.42–2.45 a.u. (50 ≤E≤150 keV). Cross sections were determined by measuring the extreme ultraviolet photons emitted from excited He1 ions. The data indicate a lower energy than expected for the maximum cross section. A comparison of the present results in terms of projectile energy dependance with the cross sections for excitation to He (1snp) 1Po, ionization, and total electron capture suggests the primary mechanism …

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Grains In Ionized Nebulae: Spectral Line Diagnostics, J. B. Kingdon, Gary J. Ferland, W. A. Feibelman Feb 1995

Grains In Ionized Nebulae: Spectral Line Diagnostics, J. B. Kingdon, Gary J. Ferland, W. A. Feibelman

Physics and Astronomy Faculty Publications

The depletion of condensable elements onto grains in gaseous nebulae can provide evidence that dust is well mixed with the ionized gas. Al and CA are two of the most depleted elements in the general interstellar medium, and it is therefore important to measure their abundances within the ionized region of nebulae. We compute a large grid of photoionization models and identify sets of line ratios which are relatively insensitive to stellar and nebular parameters, and are thus excellent diagnostics for determining relative abundances. Based on the absence of the [Ca II] λλ7291, 7324 doublet and the detection of …

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Landau-Zener Treatment Of Intensity-Tuned Multiphoton Resonances Of Potassium, J. Greg Story, D. I. Duncan, Thomas F. Gallagher Aug 1994

Landau-Zener Treatment Of Intensity-Tuned Multiphoton Resonances Of Potassium, J. Greg Story, D. I. Duncan, Thomas F. Gallagher

Physics Faculty Research & Creative Works

When exposed to intense light of ~580 nm, the ground state of K shifts up in energy, passing through two photon resonances with Rydberg states, and finally crossing the two-photon ionization limit. We have used laser pulses of varying duration to study the nature of the population transfer from the ground state to the excited state due to the intensity-tuned resonances encountered during the rising edge of the pulse. A dynamic Floquet approach in which the resonances are treated as avoided crossings of the Floquet energy levels is used to model the population transfer and gives excellent agreement with the …

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Nebular Properties And The Ionizing Radiation Field In The Galactic Center, Joseph C. Shields, Gary J. Ferland Apr 1994

Nebular Properties And The Ionizing Radiation Field In The Galactic Center, Joseph C. Shields, Gary J. Ferland

Physics and Astronomy Faculty Publications

Nebulosity in the central parsec of the Milky Way exhibits a low-ionization spectrum that has led previous analyses of this region to conclude that this material is photoionized by a relatively soft continuum. We have reanalyzed the infrared emission-line spectrum of te Galactic center in order to consider whether the data could actually be explained with photoionization by a relatively hard, yet dilute continuum, and additionally to constrain the properties of the reaiating plasma. We conclude that the composite infrared spectrum does not place strong restrictions on the nature of the ionizing continuum and that much of the ionized gas …

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Molecular-Orbital Studies Via Satellite-Free X-Ray Fluorescence: Cl-K Absorption And K–Valence-Level Emission Spectra Of Chlorofluoromethanes, Rupert C. Perera, P. L. Cowan, Dennis W. Lindle, R. E. Lavilla, T. Jach, R. D. Deslattes Apr 1991

Molecular-Orbital Studies Via Satellite-Free X-Ray Fluorescence: Cl-K Absorption And K–Valence-Level Emission Spectra Of Chlorofluoromethanes, Rupert C. Perera, P. L. Cowan, Dennis W. Lindle, R. E. Lavilla, T. Jach, R. D. Deslattes

Chemistry and Biochemistry Faculty Research

X-ray absorption and emission measurements in the vicinity of the chlorine K edge of the three chlorofluoromethanes have been made using monochromatic synchrotron radiation as the source of excitation. By selectively tuning the incident radiation to just above the Cl 1s single-electron ionization threshold for each molecule, less complex x-ray-emission spectra are obtained. This reduction in complexity is attributed to the elimination of multielectron transitions in the Cl K shell, which commonly produce satellite features in x-ray emission. The resulting "satellite-free" x-ray-emission spectra exhibit peaks due only to electrons in valence molecular orbitals filling a single Cl 1s vacancy. These …

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Argon-Photoion–Auger-Electron Coincidence Measurements Following K-Shell Excitation By Synchrotron Radiation, Jon C. Levin, C. Biedermann, N. Keller, L. Liljeby, C.-S. O, R. T. Short, Ivan A. Sellin, Dennis W. Lindle Aug 1990

Argon-Photoion–Auger-Electron Coincidence Measurements Following K-Shell Excitation By Synchrotron Radiation, Jon C. Levin, C. Biedermann, N. Keller, L. Liljeby, C.-S. O, R. T. Short, Ivan A. Sellin, Dennis W. Lindle

Chemistry and Biochemistry Faculty Research

Argon photoion spectra have been obtained for the first time in coincidence with K-LL and K-LM Auger electrons, as a function of photon energy. The simplified charge distributions which result exhibit a much more pronounced photon-energy dependence than do the more complicated noncoincident spectra. In the near-K-threshold region, Rydberg shakeoff of np levels, populated by resonant excitation of K electrons, occurs with significant probability, as do double-Auger processes and recapture of the K photoelectron through postcollision interaction.

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Ionization Of Heavy Atoms By Polarized Relativistic Protons, P.T. Leung, M. L. Rustgi Oct 1983

Ionization Of Heavy Atoms By Polarized Relativistic Protons, P.T. Leung, M. L. Rustgi

Physics Faculty Publications and Presentations

The effect due to the polarization of the incident high-energy (~GeV) proton beam on the ionization cross section of heavy atoms is investigated. In particular, with the use of Darwin wave functions for the atomic electron, the effect for hydrogenlike atoms is worked out. A numerical illustration shows that the polarization effect is completely insignificant. The authors also conclude that the K-shell ionization process is completely insensitive to the polarization of the incident beam.

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Ionization Enhanced Diffusion, David Peak, J W. Corbett, J Bourgoin Jan 1976

Ionization Enhanced Diffusion, David Peak, J W. Corbett, J Bourgoin

All Physics Faculty Publications

The general three‐dimensional diffusion equations, along with the corresponding tensor diffusivities, are established for the normal ionization‐enhanced diffusion mechanism (which is equivalent to a general two‐channel diffusion mechanism) and for the Bourgoin mechanism, the latter being explicitly developed for the diamond lattice.

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