Physics Commons^™

Theoretical Study Of Localized Surface Plasmons Of Metal Nanoparticles, Clusters And Embedded Metal Nanoparticles In Matrices, Masoud Shabani Nezhad Navrood

Dissertations

Localized surface plasmons resonances (LSPRs) in metallic nanoparticles (NPs) arise from the interactions between incident light and conduction electrons and have attracted enormous research interest in recent years both for their fundamental nature as well as applications in interdisciplinary areas of sciences such as biological imaging, plasmonic photo-thermal therapy, photovoltaics, and plasmonic sensors. LSPRs are strongly localized and depend on the shape, size, the composition of the NPs, the polarization direction of the incident light, refractive index (RI) of the surrounding medium as well as on the chemical environment that surrounded NPs. Although significant research has progressed both theoretically and …

High Resolution Solar Observations From First Principles To Applications, Angelo P. Verdoni

Dissertations

The expression "high-resolution observations" in Solar Physics refers to the spatial, temporal and spectral domains in their entirety. High-resolution observations of solar fine structure are a necessity to answer many of the intriguing questions related to solar activity. However, a researcher building instruments for high-resolution observations has to cope with the fact that these three domains often have diametrically opposed boundary conditions. Many factors have to be considered in the design of a successful instrument. Modern post-focus instruments are more closely linked with the solar telescopes that they serve than in past. In principle, the quest for high-resolution observations already …

Carbon Nanotube Electronic Structures As Anti-Corrosion Coatings, Sreeya Sreevatsa

Dissertations

A new concept of corrosion prevention is considered in this study. Diode-like and transistor-like structures have been fabricated and analyzed in the study of ionic flow through the resulting potential barriers. The structures were made of functionalized carbon nanotubes. Carbon nanotubes are known for many remarkable properties among which is being chemically inert. Taking advantage of this property, a study of corrosion of steel was undertaken.

In the first case study, successive layers of functionalized carbon nanotubes were deposited to form p-n junctions on steel substrates. It was demonstrated that the corrosion was indeed impeded by the potential barrier formed …

Probing The Complex Magnetic, Electronic And Structural Properties In Correlated Manganese Oxides, Peng Gao

Dissertations

Rare-earth Manganese Oxides (RMnO₃) exhibit two distinct structural phases: the orthorhombic structure and the hexagonal structure. The doped orthorhombic phase exhibits a metal to insulator transition, charge ordering and a strong response of electron transport properties to magnetic fields (colossal magneto-resistance). At low temperatures, this system may also exhibit a finite polarization which couples to external magnetic fields. The hexagonal phase is known to have a large spontaneous polarization at high temperatures which couples to the low temperature magnetic order. These materials are important from the basic point of view of understanding strong electronic correlations and …

Photoionization Of Rare Gas Clusters, Huaizhen Zhang

Dissertations

This thesis concentrates on the study of photoionization of van der Waals clusters with different cluster sizes. The goal of the experimental investigation is to understand the electronic structure of van der Waals clusters and the electronic dynamics. These studies are fundamental to understand the interaction between UV-X rays and clusters. The experiments were performed at the Advanced Light Source at Lawrence Berkeley National Laboratory. The experimental method employs angle-resolved time-of-flight photoelectron spectrometry, one of the most powerful methods for probing the electronic structure of atoms, molecules, clusters and solids.

The van der Waals cluster photoionization studies are focused on …

Entanglement Perturbation Theory For Antiferromagnetic Spin Chains, Lihua Wang

Dissertations

In this dissertation, we use the recently developed Entanglement Perturbation Theory (EPT) to solve antiferromagnetic spin chain problems, for both spin 1/2 and spin 1. We firs use EPT-g (EPT algorithm for ground state) to get the ground state properties. We calculated precisely energies, magnetization and spin-spin correlations. The precision of the long range spin-spin correlation functions for spin 1/2 chains is unprecedented. Due to its special structure, we also use EPT-g to calculate the firs excited state properties for spin 1 chains. Hence we plotted the phase diagram for spin 1 xxz chains. Also a generalization of EPT (EPT-e) …

African-American College Student Attitudes Toward Physics And Their Effect On Achievement, Carl Timothy Drake

Dissertations

The purpose of this study was to investigate factors affecting the attitudes that African-American college students have towards introductory college physics. The population targeted for this study consisted of African-American males and females enrolled in introductory college physics classes at an urban public historical black college or university (HBCU) located in the southeastern United States. Nine of the Fennema- Sherman Mathematics Attitude Scales, modified for physics, were used to analyze the attitudes of the 135 participants enrolled in an introductory college physics class. The nine scales used to measure the students' attitudes were Attitude Toward Success in Physics Scale (AS), …

Transmission And Guiding Of Fast Electrons Through Insulating Nanocapillaries And Comparison With Ion Guiding, Susanta Das

Dissertations

Transmission and guiding of fast electrons (500 and 1000 eV) through an insulating polyethylene terephthalate nanocapillary foil has been investigated and compared with results for slow highly charged ions. As for slow ions, guiding is attributed to charge-up of the inner walls near the capillary entrance, which, after a characteristic time, electrostatically deflects the traversing ions causing them to be guided through the sample along the capillary axis. The measurements were performed at WMU. Electron guiding is found to decrease faster with both energy and foil tilt angle than for ions. Ions lose negligible energy during the course of guiding, …

Terahertz Response Of Microfluidic-Jetted Fabricated 3d Flexible Metamaterials, Yew Li Hor

Dissertations

Conventional materials exhibit some restrictions on their electromagnetic properties. Especially in terahertz region, for example, materials that exhibit magnetic response are far less common in nature than materials that exhibit electric response. However, materials can be designed, namely artificial man-made metamaterials that exhibit electromagnetic properties that are not found in natural materials by adjusting, for example, the dielectric, magnetic or structural parameters of the constituent elements.

This dissertation demonstrates the use of new fabrication techniques to construct metamaterials in THz range via a material deposition system. The metamaterials are fabricated by stacking alternative layers with conventional designs such as single …

Synchrotron Radiation-Based Characterization Of Gan- Based Mqw Structures And Strongly Correlated Materials, Sean M. O'Malley

Dissertations

The following dissertation applies synchrotron radiation-based characterization techniques to the fields of gallium nitrides, multiferroic manganites, and self-assembled nano-domain oxide films. These material systems were chosen due to their unusual properties and potential device applications, which have made them very attractive to the scientific community.

Synchrotron-based High Resolution X-ray Diffraction (HRXRD) was used to characterize the structural properties of GaN-based multiple quantum well (MQW) structures grown on trapezoidal shaped GaN ridges. Results where interpreted within the framework of vapor-phase diffusion and surface-migration effects during the metalorganic vapor phase epitaxial growth. The relatively short diffusion length of group- III precursors and …

Characterization And Synthesis Of Nanoscale Materials, Jinfeng Wang

Dissertations

This dissertation focuses on the systematic study of techniques for characterization and synthesis of nanoscale materials. We have achieved several goals. Firstly, high number density uniform zinc oxide nanostructure growth has been achieved using thermal evaporation, through control of experimental parameters that include source material temperature, substrate temperature, substrate material, gas flow rate, and choice of catalyst. Aligned zinc oxide nanowires, randomly oriented zinc oxide nanowires, zinc oxide container-shaped structures, and zinc oxide nanobelts have been synthesized with high yield. Secondly, using a one parameter family of lattice fringe geometry curves, we show how to examine the epitaxial relationship between …

Calculations Of K-Shell Fluorescence Yields And Photoabsorption Cross Sections For Carbon Ions At The K-Edge, Muhammet Fatih Hasoglu

Dissertations

The advent of new space missions providing high-precision observations has engendered the need for reliable and precise K-shell atomic data in order to interpret these X-ray spectra. In response to this need, we focused on the calculation of K-shell fluorescence yields for 2 nd -row ions. A secondary project was undertaken in order to treat theoretically the K-shell X-ray absorption processes in carbon ions. These calculated fluorescence yields of 2nd -row ions and theX-ray photoabsorption cross sections of carbon are astrophysically important in determining (1) charge-changing probabilities, such as Auger vs. radiative decay, and (2) chemical abundances of the interstellar …

Flexible Electronics : Materials And Sensor Fabrication, Katherine J. Duncan

Dissertations

This dissertation demonstrates how to fabricate piezoelectric/pyroelectric thin films by using different printing techniques. These techniques could replace vacuum techniques for manufacturing piezoelectric/pyroelectric sensors. Ink-jet, screen and stencil printing techniques were developed to print these devices.

This work outlines attempts to develop a solution processable conductive ink for ink-jet printing. It then details the printing of commercial conductive ink on flexible substrates employing the three printing methods. Raman spectroscopy and Fourier transform infrared spectroscopy, are both used to investigate the structure of the P(VDF-TrFE) films. Optical microscopy is used to investigate the thickness and uniformity of the deposited films. The …

Synthesis And Characterization Of Plasma Enhanced Chemically Vapor Deposited Tantalum Films, Weizhong Chen

Dissertations

A low temperature inorganic plasma-enhanced chemical vapor deposition (PECVD) process has been developed for the growth of Ta using tantalum pentachloride (TaC15) as the preferred precursor and hydrogen as the reactant gas. Ta coatings were deposited at substrate temperature of 370-400 °C, reactor working pressures of 0.7-2 Ton, hydrogen carrier flow rate of 10-20 sccm, hydrogen reactant flow rates of 500 sccm, and plasma power ranging from 60 to 100W. Ta coatings were characterized with respect to their chemical, structural, and morphological properties by Auger electron spectroscopy (AES), x-ray diffraction (XRD), atomic force microscopy (AFM), x-ray photoelectron spectroscopy (XPS), scanning …

Automatic Prediction Of Solar Flares And Super Geomagnetic Storms, Hui Song

Dissertations

Space weather is the response of our space environment to the constantly changing Sun. As the new technology advances, mankind has become more and more dependent on space system, satellite-based services. A geomagnetic storm, a disturbance in Earth's magnetosphere, may produce many harmful effects on Earth. Solar flares and Coronal Mass Ejections (CMEs) are believed to be the major causes of geomagnetic storms. Thus, establishing a real time forecasting method for them is very important in space weather study.

The topics covered in this dissertation are: the relationship between magnetic gradient and magnetic shear of solar active regions; the relationship …

Electron Beam Characterization Of Carbon Nanostructures, Eric Samuel Mandell

Dissertations

Atom-thick carbon nanostructures represent a class of novel materials that are of interest to those studying carbon's role in fossil fuel, hydrogen storage, scaled-down electronics, and other nanotechnology. Electron microscope images of "edge-on" graphene sheets show linear image features due to the projected potential of the sheets. Here, intensity profiles along these linear features can measure the curvature of the sheet, as well as the shape of the sheet (i.e. hexagonal, triangular). Also, electron diffraction powder profiles calculated for triangular graphene sheet shapes show a broadening of the low-frequency edge of diffraction rings, in comparison to those calculated for hexagonal …

Structure And Excitations In Metal Ammonia Compounds, Xue Wang

Dissertations

This work has two parts. In the first part, inelastic x-ray scattering was used to measure the plasmon excitations in liquid lithium ammonia systems. The measurements were carried out for different metal concentrations, 8 mole per metal (MPM), 10 MPM, 11 MPM, 16 MPM and 20 MPM of temperature 200K. The data were analyzed to determine the plasmon energy and the linewidth as a function of momentum for each metal concentration. Deviations from the random phase approximation (RPA) in the jellium model increase as the concentration is lowered.

In the second part of this work, elastic x-ray scattering was used …

Quantum Properties Of Light Emitted By Dipole Nano-Laser, Talal Ghannam

Dissertations

Recent technological advances allow entire optical systems to be lithographically implanted on small silicon chips. These systems include tiny semiconductor lasers that function as light sources for digital optical signals. Future advances will rely on even smaller components. At the theoretical limit of this process, the smallest lasers will have an active medium consisting of a single atom (natural or artificial). Several suggestions for how this can be accomplished have already been published, such as nano-lasers based on photonic crystals and nano wires. In particular, the "dipole nanolaser" consists of a single quantum dot functioning as the active medium. It …

Design And Application Of Near Infrared Tunable Filter For Atst And Nst, Jun Ma

Dissertations

This thesis includes the following sections: a general design of the Near Infrared Tunable Filter (NIRTF) of Advanced Technology Solar Telescope (ATST) project and the Near Infrared Imaging Magnetograph (IRIM) of the New Solar Telescope (NST), the design of achromatic waveplates, the narrowband continuum observation of a Sunspot at 1.56 µm using IRIM instruments, and the coronal hole observation using the Digital Vector Magnetograph (VMG) at Big Bear Solar Observatory (BBSO).

A near infrared tunable filter system is designed with detailed optical parameters for each component in the system. Among these components, the achromatic waveplates, which used to be an …

Design, Fabrication And Testing Of A Fiber Optic Stress/Strain Sensor For Soft Stretchable Materials Using Polarization Imaging Technique, Jianjun Zheng

Dissertations

The polarization imaging technique has been used to obtain high quality surface images of turbid media. This technique can be slightly modified and used for noninvasive sensing of strain and stress in soft stretchable materials, such as latex and human tissues. Previously this sensing method was developed with free space bulk optics. In this study, a fiber optic based system is developed to investigate the potential application of this technology on the strain/stress as well as surface roughness measurements of stretchable materials. In this system, polarizers are simply attached to the fiber ends to form a polarizing three-fiber probe. Furthermore, …

Wireless Passive Surface Acoustic Wave (Saw) Sensing System, Sridevi Krishnamurthy

Dissertations

Due to their small size and ruggedness, Surface Acoustic Wave (SAW) devices have been widely used as part of wireless sensing or identification system especially in inaccessible and inhospitable environments. In addition, SAW devices find widespread applications as filters in communication systems and also as physical, chemical and bio-sensors and ID tags. The passive wireless SAW sensing system mainly consists of a passive SAW sensor and an interrogation unit which sends a burst signal to the SAW sensor and processes the sensor response. Theobjectives of this work were designing, prototyping and fabricating the interrogation unit on a PCB and also …

Inelastic X-Ray Scattering Studies On Organic Semiconductors And Organic Superconductors, Chaminda Nalaka Kodituwakku

Dissertations

We have measured electronic excitations and excitons in CuPc polycrystalline and single crystal samples. Measurements on the polycrystalline sample were done with 300 meV resolution and measurements on the single crystal were done using 120 meV resolution. Time dependant density functional theory (TD-DFT) calculations were done on the CuPc molecule to understand the electronic excitations in this system.

Long Exposure Point Spread Function Estimation From Solar Adaptive Optics Loop Data, Jose Marino

Dissertations

Adaptive optics (AG) systems provide partial correction to wavefront distortions introduced by the Earth's atmosphere. They have become an essential tool to obtain diffraction-limited observations from ground-based telescopes. However, the AG correction is only partial and post-processing with a good estimate of the point spread function (PSF) is required.

PSF estimates are impossible to measure directly during solar observations due to the lack of point sources in the field-of-view. Moreover, the highly variable day-time seeing conditions require the estimated PSF to be simultaneous with the captured image. A method is presented to estimate the long-exposure PSF of AG-corrected solar observations …

Construction Of Fasr Subsystem Testbed And Application For Solar Burst Trajectories And Rfi Study, Zhiwei Liu

Dissertations

The construction of the Frequency Agile Solar Radiotelescope (FASR) Subsystem Testbed (FST) and observational results are described. Three antennas of Owens Valley Solar Array (OVSA) have been upgraded with newly designed, state of art technology. The 1-9 GHz RF signal from the antenna feed is transmitted via broadband (45 MHz-9.5 GHz) optical fiber links to the control room. The RF is then downconverted to a 500 MHz, single-sideband signal that can be tuned across the 1-9 GHz RF band. The data are sampled with an 8-bit, 1 GHz sampling-rate digitizer, and further saved to a computer hard disk. The full-resolution …

High Resolution Studies Of Complex Solar Active Regions, Na Deng

Dissertations

Flares and Coronal Mass Ejections (CMEs) are energetic events, which can even impact the near-Earth environment and are the principal source of space weather. Most of them originate in solar active regions. The most violent events are produced in sunspots with a complex magnetic field topology. Studying their morphology and dynamics is helpful in understanding the energy accumulation and release mechanisms for flares and CMEs, which are intriguing problems in solar physics.

The study of complex active regions is based on high-resolution observations from space missions and new instruments at the Big Bear Solar Observatory (BBSO). Adaptive optics (AG) in …

Small And Large-Scale Magnetic Fields Involved With Solar Flares, Chang Liu

Dissertations

Solar flares are generally identified as an important source of disturbances that affect space weather, while many aspects of the basic flare process are still not well understood. The purpose of the present work has been to investigate the small and large-scale magnetic structures and their evolution associated with flares in the context of magnetic reconnection, based on which the goal of this dissertation is to further the understanding of the various properties of flares and related phenomena, including their origin, precursors, and evolution of morphology in solar atmosphere.

The research presented in this dissertation relied upon multiwavelength observations of …

Feasibility Of Superconductivity In Semiconductor Superlatices, Kenneth P. Walsh

Dissertations

The objective of this thesis is to explore superconductivity in semiconductor superlattices of alternating hole and electron layers. The feasibility of superconductivity in semiconductor superlattices is based on a model formulated by Harshrnan and Mills. In this model, a semiconductor superlattice forms the layered electron and hole reservoirs of high transition temperature (high-Tc) superconductors.

A GaAs-A1xGa1-xAs semiconductor structure is proposed which is predicted to superconduct at Tc = 2.0 K and may be analogous to the layered electronic structure of high-Tc superconductors. Formation of an alternating sequence of electron- and hole-populated quantum wells (an electron-hole superlattice) in a modulation-doped GaAs- …

Study Of Propagation And Detection Methods Of Terahertz Radiation For Spectroscopy And Imaging, Aparajita Bandyopadhyay

Dissertations

The applications of terahertz (THz, 1 THz is 1012 cycles per second or 300 pm in wavelength) radiation are rapidly expanding. In particular, THz imaging is emerging as a powerful technique to spatially map a wide variety of objects with spectral features which are present for many materials in THz region. Objects buried within dielectric structures can also be imaged due to the transparency of most dielectrics in this regime. Unfortunately, the image quality in such applications is inherently influenced by the scattering introduced by the sample inhomogeneities and by the presence of barriers that reduces both the transmitted power …

Novel Characterization Of Materials Using Thz Spectroscopic Techniques, Amartya Sengupta

Dissertations

Significant scientific and technical challenges within the terahertz (THz) frequency regime have recently motivated an array of new research activities. This involves numerous applications of this region of the electromagnetic spectrum between approximately 100 GHz (3mm) and 3 THz (100 µm) for both spectroscopy and imaging purposes. THz time domain spectroscopy is unique in that the time domain waveforms are measured and the complex optical constants are deduced directly without resorting to the Kramers-Kronig Analysis.

In this work, THz spectroscopy has been used to characterize different types of materials. Materials investigated consisted of semiconductors, gate dielectric materials, high energetic materials …

Photoexcitation And Photoionization Of The Argon Atom And The Hydrogen Bromide Molecule, Ximao Feng

Dissertations

Interaction between synchrotron radiation with inner-shell electrons is a fundamental method to study the structure and dynamics of atoms and molecules. This thesis, under the guidance of Dr. Nora Berrah, concentrates on the study of the interaction between soft x-ray photons with Ar atoms and HBr moleculeswith time-of-flight (TOF) electron spectrometers and two-dimensional photoelectron spectroscopy (2DPES). Both of the experiments were performed on theAtomic, Molecular and Optical Physics undulator beamline at the Advanced Light Source at Lawrence Berkeley National Laboratory.

The argon study focused on photoelectron recapture when the 2p electrons are ionized just above the thresholds of the two …