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Articles 31 - 60 of 426
Full-Text Articles in Physics
How Do We Observe Relational Observables?, Emily Adlam
How Do We Observe Relational Observables?, Emily Adlam
Mathematics, Physics, and Computer Science Faculty Articles and Research
In theories with a diffeomorphism symmetry, such as general relativity and canonical quantum gravity, it is often proposed that the empirical content is encoded in relational observables. But how do relational observables actually make contact with experience? I argue that this question can only be answered by providing a schematization of the observer which is appropriate for the context of a diffeomorphism-invariant theory. I suggest that this may require us to move away from a ‘passive awareness’ conception of consciousness towards a more agential conception, because there is a clear sense in which an embodied agent must experience herself as …
Artificially Intelligent Maxwell's Demon For Optimal Control Of Open Quantum Systems, Paolo A. Erdman, Robert Czupryniak, Bibek Bhandari, Andrew N. Jordan, Frank Noé, Jens Eisert, Giacomo Guarnieri
Artificially Intelligent Maxwell's Demon For Optimal Control Of Open Quantum Systems, Paolo A. Erdman, Robert Czupryniak, Bibek Bhandari, Andrew N. Jordan, Frank Noé, Jens Eisert, Giacomo Guarnieri
Mathematics, Physics, and Computer Science Faculty Articles and Research
Feedback control of open quantum systems is of fundamental importance for practical applications in various contexts, ranging from quantum computation to quantum error correction and quantum metrology. Its use in the context of thermodynamics further enables the study of the interplay between information and energy. However, deriving optimal feedback control strategies is highly challenging, as it involves the optimal control of open quantum systems, the stochastic nature of quantum measurement, and the inclusion of policies that maximize a long-term time- and trajectory-averaged goal. In this work, we employ a reinforcement learning approach to automate and capture the role of a …
Measurement Time Of Weak Measurements On Large Entangled Systems, Truong-Son P. Văn, Andrew N. Jordan, David W. Snoke
Measurement Time Of Weak Measurements On Large Entangled Systems, Truong-Son P. Văn, Andrew N. Jordan, David W. Snoke
Mathematics, Physics, and Computer Science Faculty Articles and Research
It is well established that starting only with strong, projective quantum measurements, experiments can be designed to allow weak measurements, which lead to a random walk between the possible final measurement outcomes. However, one can ask the reverse question: starting with only weak measurements, can all the results of standard strong measurements be recovered? Prior work has shown that some results can be, such as the Born rule for the probability of measurement outcomes as a function of wave intensity. In this paper, we show that another crucial result can be reproduced by purely weak measurements, namely, the collapse of …
Infrared Cooling In An Anharmonic Cascade Framework: 2-Cyanoindene, The Smallest Cyano-Pah Identified In Tmc-1, Mark H. Stockett, Vincent J. Esposito, Eleanor K. Ashworth, Ugo Jacovella, James N. Bull
Infrared Cooling In An Anharmonic Cascade Framework: 2-Cyanoindene, The Smallest Cyano-Pah Identified In Tmc-1, Mark H. Stockett, Vincent J. Esposito, Eleanor K. Ashworth, Ugo Jacovella, James N. Bull
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Infrared (IR) cooling of polycyclic aromatic hydrocarbon (PAH) molecules is a major radiative stabilization mechanism of PAHs present in space and is the origin of the aromatic infrared bands (AIBs). Here, we report an anharmonic cascade model in a master equation framework to model IR emission rates and emission spectra of energized PAHs as a function of internal energy. The underlying (simple harmonic cascade) framework for fundamental vibrations has been developed through the modeling of cooling rates of PAH cations and other carboneaous ions measured in electrostatic ion storage ring experiments performed under “molecular cloud in a box” conditions. The …
A Sensitivity Analysis Of The Modeling Of Polycyclic Aromatic Hydrocarbon Emission In Galaxies, A. Maragkoudakis, C. Boersma, P. Temi, J. D. Bregman, L. J. Allamandola, Vincent J. Esposito, A. Ricca, E. Peeters
A Sensitivity Analysis Of The Modeling Of Polycyclic Aromatic Hydrocarbon Emission In Galaxies, A. Maragkoudakis, C. Boersma, P. Temi, J. D. Bregman, L. J. Allamandola, Vincent J. Esposito, A. Ricca, E. Peeters
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
We have conducted a sensitivity analysis on the mid-infrared spectral decomposition of galaxies and the modeling of the polycyclic aromatic hydrocarbon (PAH) emission spectrum with the NASA Ames PAH Infrared Spectroscopic Database (PAHdb) to assess the variance on the average galaxy PAH population properties under a grid of different modeling parameters. We find that the short-low and short-low+long-low Spitzer-IRS decomposition with PAHFIT provides consistent modeling and recovery of the 5–15 μm PAH emission spectrum. For PAHdb modeling, application of a redshift to the calculated spectra to account for anharmonic effects introduces a 15%–20% variance on the derived parameters, while its …
Photolysis And Sublimation Chemistry Of Ammonium Cyanide With Relevance To Cometary Environments, O. H. Wilkins, K. M. Yocum, Vincent J. Esposito, E. Harel, S. N. Milam, P. A. Gerakines
Photolysis And Sublimation Chemistry Of Ammonium Cyanide With Relevance To Cometary Environments, O. H. Wilkins, K. M. Yocum, Vincent J. Esposito, E. Harel, S. N. Milam, P. A. Gerakines
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Bulk nitrogen is depleted in solar system objects, including the terrestrial planets, chondritic meteorites, and comets. Recently, it was suggested that cometary nitrogen may be locked up in ammonium salts—ionic solids comprising ammonia (NH3) and an acid such as hydrogen cyanide (HCN)—based on Rosetta/ROSINA data from comet 67P/Churyumov–Gerasimanko. Among the proposed salts to have been found in 67P were ammonium cyanide (NH4CN) and ammonium cyanate (NH4OCN), which were inferred from identifying HCN, cyanamide (NH2CN), and isocyanic acid (HNCO) in the mass spectrometry data collected in the coma of 67P. However, the relationship …
A New Form Of Soft Supersymmetry Breaking?, Scott Chapman
A New Form Of Soft Supersymmetry Breaking?, Scott Chapman
Mathematics, Physics, and Computer Science Faculty Articles and Research
Starting with a supersymmetric U(N) × U(N) gauge theory built in N = 1 superspace, a nonsupersymmetric theory is obtained by “twisting” the gauginos into a different representation of the group than the gauge bosons. Despite the fact that this twisting breaks supersymmetry, it is still possible to construct an action that is holomorphic and invariant to local “twisted” gauge transformations in superspace. It is conjectured that these two properties may allow the theory to be free of quadratic divergences to all orders, despite a lack of supersymmetry. An explicit calculation shows that the theory is free of quadratic divergences …
Reconstructing Superoscillations Buried Deeply In Noise, Derek D. White, Shunxing Zhang, Barbara Šoda, Achim Kempf, Daniele C. Struppa, Andrew N. Jordan, John C. Howell
Reconstructing Superoscillations Buried Deeply In Noise, Derek D. White, Shunxing Zhang, Barbara Šoda, Achim Kempf, Daniele C. Struppa, Andrew N. Jordan, John C. Howell
Mathematics, Physics, and Computer Science Faculty Articles and Research
We utilize a method using frequency combs to construct waves that feature superoscillations—local regions of the wave that exhibit a change in phase that the bandlimits of the wave should not otherwise allow. This method has been shown to create superoscillating regions that mimic any analytic function—even ones well outside the bandlimits—to an arbitrary degree of accuracy. We experimentally demonstrate that these waves are extremely robust against noise, allowing for accurate reconstruction of a superoscillating target function thoroughly buried in noise. We additionally show that such a construction can be easily used to range-resolve a signal well below the commonly …
Vibrational And Electronic Spectroscopy Of 2-Cyanoindene Cations, Thomas E. Douglas-Walker, Eleanor K. Ashworth, Mark H. Stockett, Francis C. Daly, Isabelle Chambrier, Vincent J. Esposito, Marius Gerlach, Angel Zheng, Julianna Palotás, Andrew N. Cammidge, Ewen K. Campbell, Sandra BrüNken, James N. Bull
Vibrational And Electronic Spectroscopy Of 2-Cyanoindene Cations, Thomas E. Douglas-Walker, Eleanor K. Ashworth, Mark H. Stockett, Francis C. Daly, Isabelle Chambrier, Vincent J. Esposito, Marius Gerlach, Angel Zheng, Julianna Palotás, Andrew N. Cammidge, Ewen K. Campbell, Sandra BrüNken, James N. Bull
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
2-Cyanoindene is one of the few specific aromatic or polycyclic aromatic hydrocarbon (PAH) molecules positively identified in Taurus molecular cloud-1 (TMC-1), a cold, dense molecular cloud that is considered the nearest star-forming region to Earth. We report cryogenic mid-infrared (550–3200 cm–1) and visible (16,500–20,000 cm–1, over the D2 ← D0 electronic transition) spectra of 2-cyanoindene radical cations (2CNI+), measured using messenger tagging (He and Ne) photodissociation spectroscopy. The infrared spectra reveal the prominence of anharmonic couplings, particularly over the fingerprint region. There is a strong CN-stretching mode at 2177 ± 1 cm–1 (4.593 …
Exploring The Accuracy Of Interferometric Quantum Measurements Under Conservation Laws, Nicolò Piccione, Maria Maffei, Andrew N. Jordan, Kater W. Murch, Alexia Auffèves
Exploring The Accuracy Of Interferometric Quantum Measurements Under Conservation Laws, Nicolò Piccione, Maria Maffei, Andrew N. Jordan, Kater W. Murch, Alexia Auffèves
Mathematics, Physics, and Computer Science Faculty Articles and Research
A (target) quantum system is often measured through observations performed on a second (meter) system to which the target is coupled. In the presence of global conservation laws holding on the joint meter-target system, the Wigner-Araki-Yanase theorem and its generalizations predict a lower bound on the measurement’s error (Ozawa’s bound). While practically negligible for macroscopic meters, it becomes relevant for microscopic ones. Here, we propose a simple interferometric setup, arguably within reach of present technology, in which a flying particle (a microscopic quantum meter) is used to measure a qubit by interacting with it in one arm of the interferometer. …
Moderate Physical Perspectivalism, Emily Adlam
Moderate Physical Perspectivalism, Emily Adlam
Philosophy Faculty Articles and Research
Recent developments in the foundations of physics have given rise to a class of views suggesting that physically meaningful descriptions must always be relativized to a physical perspective. In this article, I distinguish between strong physical perspectivalism, which maintains that all facts must be relativized to a perspective, and moderate physical perspectivalism, which maintains that all empirically meaningful descriptions must be relativized to a perspective. I argue that scientific evidence and philosophical considerations support moderate physical perspectivalism over strong physical perspectivalism. In particular, motivations connected to epistemic humility and the social nature of science are more compatible with the moderate …
Separating A Particle's Mass From Its Momentum, Mordecai Waegell, Jeff Tollaksen, Yakir Aharonov
Separating A Particle's Mass From Its Momentum, Mordecai Waegell, Jeff Tollaksen, Yakir Aharonov
Mathematics, Physics, and Computer Science Faculty Articles and Research
The Quantum Cheshire Cat experiment showed that when weak measurements are performed on pre- and post-selected system, the counterintuitive result has been obtained that a neutron is measured to be in one place without its spin, and its spin is measured to be in another place without the neutron. A generalization of this effect is presented with a massive particle whose mass is measured to be in one place with no momentum, while the momentum is measured to be in another place without the mass. The new result applies to any massive particle, independent of its spin or charge. A …
High-Coherence Kerr-Cat Qubit In 2d Architecture, Ahmed Hajr, Bingcheng Qing, Ke Wang, Gerwin Koolstra, Zahra Pedramrazi, Ziqi Kang, Larry Chen, Long B. Nguyen, Christian Jünger, Noah Goss, Irwin Huang, Bibek Bhandari, Nicholas E. Frattini, Shruti Puri, Justin Dressel, Andrew N. Jordan, David I. Santiago, Irfan Siddiqi
High-Coherence Kerr-Cat Qubit In 2d Architecture, Ahmed Hajr, Bingcheng Qing, Ke Wang, Gerwin Koolstra, Zahra Pedramrazi, Ziqi Kang, Larry Chen, Long B. Nguyen, Christian Jünger, Noah Goss, Irwin Huang, Bibek Bhandari, Nicholas E. Frattini, Shruti Puri, Justin Dressel, Andrew N. Jordan, David I. Santiago, Irfan Siddiqi
Mathematics, Physics, and Computer Science Faculty Articles and Research
The Kerr-cat qubit is a bosonic qubit in which multiphoton Schrödinger cat states are stabilized by applying a two-photon drive to an oscillator with a Kerr nonlinearity. The suppressed bit-flip rate with increasing cat size makes this qubit a promising candidate to implement quantum error correction codes tailored for noise-biased qubits. However, achieving strong light-matter interactions necessary for stabilizing and controlling this qubit has traditionally required strong microwave drives that heat the qubit and degrade its performance. In contrast, increasing the coupling to the drive port removes the need for strong drives at the expense of large Purcell decay. By …
Battle Of The Ch Motions: Aliphatic Vs Aromatic Contributions To Astronomical Pah Emission And Exploration Of The Aliphatic, Aromatic, And Ethynyl Ch Stretches, Vincent J. Esposito, Salma Bejaoui, Brant E. Billinghurst, Christiaan Boersma, Ryan C. Fortenberry, Farid Salama
Battle Of The Ch Motions: Aliphatic Vs Aromatic Contributions To Astronomical Pah Emission And Exploration Of The Aliphatic, Aromatic, And Ethynyl Ch Stretches, Vincent J. Esposito, Salma Bejaoui, Brant E. Billinghurst, Christiaan Boersma, Ryan C. Fortenberry, Farid Salama
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Strong anharmonic coupling between vibrational states in polycyclic aromatic hydrocarbons (PAH) produces highly mixed vibrational transitions that challenge the current understanding of the nature of the astronomical mid-infrared PAH emission bands. Traditionally, PAH emission bands have been characterized as either aromatic or aliphatic, and this assignment is used to determine the fraction of aliphatic carbon in astronomical sources. In reality, each of the transitions previously utilized for such an attribution is highly mixed with contributions from both aliphatic and aromatic CH motions as well as non-CH motions such as CC stretches. High-resolution gas-phase IR absorption measurements of the spectra of …
Long-Distance Photon-Mediated And Short-Distance Entangling Gates In Three-Qubit Quantum Dot Spin Systems, Nooshin M. Estakhri, Ada Warren, Sophia E. Economou, Edwin Barnes
Long-Distance Photon-Mediated And Short-Distance Entangling Gates In Three-Qubit Quantum Dot Spin Systems, Nooshin M. Estakhri, Ada Warren, Sophia E. Economou, Edwin Barnes
Engineering Faculty Articles and Research
Superconducting resonator couplers will likely become an essential component in modular semiconductor quantum dot (QD) spin qubit processors, as they help alleviate crosstalk and wiring issues as the number of qubits increases. Here, we focus on a three-qubit system composed of two modules: a two-electron triple QD resonator coupled to a single-electron double QD. Using a combination of analytical techniques and numerical results, we derive an effective Hamiltonian that describes the three-qubit logical subspace and show that it accurately captures the dynamics of the system. We examine the performance of short-range and long-range entangling gates, revealing the effect of a …
Optimal Radar Ranging Pulse To Resolve Two Reflectors, Andrew N. Jordan, John C. Howell, Achim Kempf, Shunxing Zhang, Derek White
Optimal Radar Ranging Pulse To Resolve Two Reflectors, Andrew N. Jordan, John C. Howell, Achim Kempf, Shunxing Zhang, Derek White
Mathematics, Physics, and Computer Science Faculty Articles and Research
Previous work established fundamental bounds on subwavelength resolution for the radar range resolution problem, called superradar [Phys. Rev. Appl. 20, 064046 (2023)]. In this work, we identify the optimal waveforms for distinguishing the range resolution between two reflectors of identical strength, leveraging results in quantum metrology. We discuss both the unnormalized optimal waveform as well as the best square-integrable pulse and their variants. Using orthogonal function theory, we give an explicit algorithm to optimize the wave pulse in finite time to have the best performance. We also explore range resolution estimation with unnormalized waveforms with multiparameter methods to …
Angular Momentum Flow Without Anything Carrying It, Yakir Aharonov, Daniel Collins, Sandu Popescu
Angular Momentum Flow Without Anything Carrying It, Yakir Aharonov, Daniel Collins, Sandu Popescu
Mathematics, Physics, and Computer Science Faculty Articles and Research
Transfer of conserved quantities between two remote regions is generally assumed to be a rather trivial process: a flux of particles carrying the conserved quantities propagates from one region to another. However, we demonstrate a flow of angular momentum from one region to another across a region of space in which there is a vanishingly small probability of any particles (or fields) being present. This shows that the usual view of how conservation laws work needs to be revisited.
Experimental Realization Of Supergrowing Fields, Sethuraj K. R., Tathagata Karmakar, S. A. Wadood, Andrew N. Jordan, A. Nick Vamivakas
Experimental Realization Of Supergrowing Fields, Sethuraj K. R., Tathagata Karmakar, S. A. Wadood, Andrew N. Jordan, A. Nick Vamivakas
Mathematics, Physics, and Computer Science Faculty Articles and Research
Supergrowth refers to the local amplitude growth rate of a signal being faster than its fastest Fourier mode. In contrast, superoscillation pertains to the variation of the phase. Compared to the latter, supergrowth can have exponentially higher intensities and promises improvement over superoscillation-based superresolution imaging. Here, we demonstrate the experimental synthesis of controlled supergrowing fields with a maximum growth rate of ∼19.07 times the system bandlimit. Our work is an essential step toward realizing supergrowth-based far-field superresolution imaging.
On The Formation And Detectability Of H2Cncn And Its Progenitors, Ryan C. Fortenberry, Vincent J. Esposito
On The Formation And Detectability Of H2Cncn And Its Progenitors, Ryan C. Fortenberry, Vincent J. Esposito
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
New highly exothermic formation pathways incorporating both thermodynamic and kinetic control for the newly astronomically detected H2CNCN molecule are paired with extremely accurate quantum chemical rovibrational spectroscopic computations. The reactions between astronomically known CH2CN/CH2CCH + HNCN follow effectively identical pathways and proceed through stable intermediates and over deeply submerged transition states to form H2CNCN and HCN/HCCH coproducts. Similarly, the reaction between CHM2CN and NCN− can also form H2CNCN, although this pathway first requires the initial formation of NCN−, which is currently undetected in space, via …
Quantum Field Theory And The Limits Of Reductionism, Emily Adlam
Quantum Field Theory And The Limits Of Reductionism, Emily Adlam
Mathematics, Physics, and Computer Science Faculty Articles and Research
I suggest that the current situation in quantum field theory (QFT) provides some reason to question the universal validity of ontological reductionism. I argue that the renormalization group flow is reversible except at fixed points, which makes the relation between large and small distance scales quite symmetric in QFT, opening up at least the technical possibility of a non-reductionist approach to QFT. I suggest that some conceptual problems encountered within QFT may potentially be mitigated by moving to an alternative picture in which it is no longer the case that the large supervenes on the small. Finally, I explore some …
Experimental Determination Of The Unusual Ch Stretch Frequency Of Protonated Fullerenes, Laura Finazzi, Vincent J. Esposito, Julianna Palotás, Jonathan Martens, Els Peeters, Jan Cami, Giel Berden, Jos Oomens
Experimental Determination Of The Unusual Ch Stretch Frequency Of Protonated Fullerenes, Laura Finazzi, Vincent J. Esposito, Julianna Palotás, Jonathan Martens, Els Peeters, Jan Cami, Giel Berden, Jos Oomens
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
We report experimental values for the CH stretch frequencies of the protonated fullerenes C60H+ and C70H+. Anharmonic frequency calculations at the B3LYP/6-31G level of theory, which are independent of empirical scaling factors, reproduce the experimental values to within approximately 5 cm−1. Scaling theoretical harmonic frequencies by applying factors derived for polycyclic aromatic hydrocarbons deviate significantly from the experimentally measured frequency. We attribute this deviation to the unusual hydrocarbon structure that affects the degree of anharmonicity of the CH stretch. This result allows us to propose an original, specific scaling factor of …
Madelung Mechanics And Superoscillations, Mordecai Waegell
Madelung Mechanics And Superoscillations, Mordecai Waegell
Mathematics, Physics, and Computer Science Faculty Articles and Research
In single-particle Madelung mechanics, the single-particle quantum state Ψ(⃗x, t) = R(⃗x, t)eiS(⃗x,t)/h is interpreted as comprising an entire conserved fluid of classical point particles, with local density R(⃗x, t)2 and local momentum ⃗∇S(⃗x, t) (where R and S are real). The Schrödinger equation gives rise to the continuity equation for the fluid, and the Hamilton–Jacobi equation for particles of the fluid, which includes an additional density-dependent quantum potential energy term Q(⃗x, t) = − ¯h2 2m ⃗∇R(⃗x,t) R(⃗x,t) , which is all that makes the fluid behavior nonclassical. In particular, the quantum potential can become negative and create a …
Three-Wave Mixing Experiments In Indium–Tin–Oxide Thin-Films With No Phase Matching, Kyle Wynne, Marjan Bazian, Mark C. Harrison
Three-Wave Mixing Experiments In Indium–Tin–Oxide Thin-Films With No Phase Matching, Kyle Wynne, Marjan Bazian, Mark C. Harrison
Engineering Faculty Articles and Research
One challenge of using nonlinear optical phenomena for practical applications is the need to perform phase-matching. Recently, epsilon-near-zero materials have been shown to demonstrate strong optical nonlinearities, in addition to their other unique properties. As suggested by their name, the permittivity of the material is close to zero for a certain wavelength range. We demonstrate that this small permittivity allows for efficient three-wave mixing interactions to take place in indium–tin–oxide thin films without the need for phase matching the pump and signal beams. The efficiency of the second-order nonlinear interactions is characterized, and cascaded three-wave mixing is demonstrated.
Superphenomena For Arbitrary Quantum Observables, Andrew N. Jordan, Yakir Aharonov, Daniele C. Struppa, Fabrizio Colombo, Irene Sabadini, Tomer Shushi, Jeff Tollaksen, John C. Howell, A. Nick Vamivakas
Superphenomena For Arbitrary Quantum Observables, Andrew N. Jordan, Yakir Aharonov, Daniele C. Struppa, Fabrizio Colombo, Irene Sabadini, Tomer Shushi, Jeff Tollaksen, John C. Howell, A. Nick Vamivakas
Mathematics, Physics, and Computer Science Faculty Articles and Research
Superoscillations occur when a globally band-limited function locally oscillates faster than its highest Fourier component. We generalize this effect to arbitrary quantum-mechanical operators as a weak value, where the preselected state is a superposition of eigenstates of the operator with eigenvalues bounded to a range, and the postselection state is a local position. Superbehavior of this operator occurs whenever the operator's weak value exceeds its eigenvalue bound. We give illustrative examples of this effect for total angular momentum and energy. In the latter case, we demonstrate a sequence of harmonic oscillator potentials where a finite-energy state converges everywhere on the …
Generation Of Kochen-Specker Contextual Sets In Higher Dimensions By Dimensional Upscaling Whose Complexity Does Not Scale With Dimension And Their Applications, Mladen Pavičić, Mordecai Waegell
Generation Of Kochen-Specker Contextual Sets In Higher Dimensions By Dimensional Upscaling Whose Complexity Does Not Scale With Dimension And Their Applications, Mladen Pavičić, Mordecai Waegell
Mathematics, Physics, and Computer Science Faculty Articles and Research
Recently, handling of contextual sets, in particular Kochen-Specker (KS) sets, in higher dimensions has been given an increasing attention, both theoretically and experimentally. However, methods of their generation are diverse, not generally applicable in every dimension, and of exponential complexity. Therefore, we design a dimensional upscaling method, whose complexity does not scale with dimension. As a proof of principle we generate manageable-sized KS master sets in up to 27 dimensional spaces and show that well over 32 dimensions can be reached. From these master sets we obtain an ample number of smaller KS sets. We discuss three kinds of applications …
How Are Entanglement Entropies Related To Entropy Bounds?, Emily Adlam
How Are Entanglement Entropies Related To Entropy Bounds?, Emily Adlam
Philosophy Faculty Articles and Research
In this paper we seek to understand what current knowledge of entanglement entropies suggests about the appropriate way to interpret the covariant entropy bound. We first begin by arguing that just as in the classical case, a universal bound on the von Neumann entropy could have either an epistemic or ontological origin. We then consider several possible ways of explaining the bound as a consequence of features of the entanglement entropy. We discuss consider area laws in condensed matter and quantum field theory, arguing that they suggest an epistemic reading of the bound. We also discuss the ‘spacetime from entanglement’ …
Fundamental Mechanisms Of Energy Exchanges In Autonomous Measurements Based On Dispersive Qubit-Light Interaction, Nicolò Piccione, Maria Maffei, Xiayu Linpeng, Andrew N. Jordan, Kater W. Murch, Alexia Auffèves
Fundamental Mechanisms Of Energy Exchanges In Autonomous Measurements Based On Dispersive Qubit-Light Interaction, Nicolò Piccione, Maria Maffei, Xiayu Linpeng, Andrew N. Jordan, Kater W. Murch, Alexia Auffèves
Mathematics, Physics, and Computer Science Faculty Articles and Research
Measuring an observable which does not commute with the Hamiltonian of a quantum system usually modifies the mean energy of this system. In an autonomous measurement scheme, coupling the system to a quantum meter, the system's energy change must be compensated by the meter's energy change. Here, we theoretically study such an autonomous meter-system dynamics: a qubit interacting dispersively with a light pulse propagating in a one-dimensional waveguide. The phase of the light pulse is shifted, conditioned to the qubit's state along the 𝑧 direction, while the orientation of the qubit Hamiltonian is arbitrary. As the interaction is dispersive, photon …
Assigning The Ch Stretch Overtone Spectrum Of Benzene And Naphthalene With Extension To Anthracene And Tetracene Using 2- And 3-Quanta Anharmonic Quantum Chemical Computations, Vincent J. Esposito, Ryan C. Fortenberry, Christiaan Boersma, Louis J. Allamandola
Assigning The Ch Stretch Overtone Spectrum Of Benzene And Naphthalene With Extension To Anthracene And Tetracene Using 2- And 3-Quanta Anharmonic Quantum Chemical Computations, Vincent J. Esposito, Ryan C. Fortenberry, Christiaan Boersma, Louis J. Allamandola
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
The CH stretch overtone region (5750–6300 cm−1) of benzene and naphthalene is assigned herein using anharmonic quantum chemical computations, and the trend of how this extends to larger polycyclic aromatic hydrocarbons (PAHs) is established. The assignment of all experimental bands to specific vibrational states is performed for the first time. Resonance polyads and the inclusion of 3-quanta vibrational states are both needed to compute accurate vibrational frequencies with the proper density-of-states to match the experimental band shape. Hundreds of 3-quanta states produce the observed band structure in naphthalene, anthracene, and tetracene, and this number is expected to increase …
Quantum Measurement: Theory And Practice, Andrew N. Jordan, Irfan A. Siddiqi
Quantum Measurement: Theory And Practice, Andrew N. Jordan, Irfan A. Siddiqi
Mathematics, Physics, and Computer Science Faculty Books and Book Chapters
This book adopts a novel, physics-first approach to quantum measurement, using physical experiments as the basis to describe the underlying mathematical formalism. Topics covered include weak measurements, quantum measurement reversal, quantum trajectories and the stochastic path integral formalism. The theory of quantum measurement is also covered in detail, including discussion of how it can be tested and demonstrated in a laboratory: how to build quantum-limited amplifiers, fundamental noise limits imposed on measurement by quantum mechanics, and the design of superconducting circuits. This text is an excellent introduction for students with a basic understanding of quantum mechanics wanting to learn more …
Cn Stretches Around 4.4 Microns Dominate The Ir Absorption Spectra Of Cyanopolycyclic Aromatic Hydrocarbons, Vincent J. Esposito, Ryan C. Fortenberry, Christiaan Boersma, Alexandros Maragkoudakis, Louis J. Allamandola
Cn Stretches Around 4.4 Microns Dominate The Ir Absorption Spectra Of Cyanopolycyclic Aromatic Hydrocarbons, Vincent J. Esposito, Ryan C. Fortenberry, Christiaan Boersma, Alexandros Maragkoudakis, Louis J. Allamandola
Biology, Chemistry, and Environmental Sciences Faculty Articles and Research
Anharmonic quantum chemical computations reveal a strong, narrow (width = 0.075 μm) band in the 4.3–4.5 μm region of the absorption spectra of the cyano-substituted polycyclic aromatic hydrocarbons (CN-PAHs) cyanonaphthalene, cyanoanthracene, c yanophenanthrene, and c yanopyrene. This narro w windo w with intense IR lines implies that CN-PAHs of various shapes and sizes offer little variation in both wavelength and intensity in this region. Subsequently, this band can be used as a tracer for CN-PAHs. The distinct features making up the band are assigned to mixed vibrational states consisting of the CN stretch fundamental and various combination bands, including in-plane …