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Full-Text Articles in Condensed Matter Physics
Simultaneous Metal-Insulator And Antiferromagnetic Transitions In Orthorhombic Perovskite Iridate Sr0.94Ir0.78O2.68 Single Crystals, Hao Zheng, Jsaminka Terzic, Feng Ye, X. G. Wan, D. Wang, Jinchen Wang, Xiaoping Wang, P. Schlottmann, Shujuan Yuan, Gang Cao
Simultaneous Metal-Insulator And Antiferromagnetic Transitions In Orthorhombic Perovskite Iridate Sr0.94Ir0.78O2.68 Single Crystals, Hao Zheng, Jsaminka Terzic, Feng Ye, X. G. Wan, D. Wang, Jinchen Wang, Xiaoping Wang, P. Schlottmann, Shujuan Yuan, Gang Cao
Center for Advanced Materials Faculty Publications
The orthorhombic perovskite SrIrO3 is a semimetal, an intriguing exception in iridates where the strong spin-orbit interaction coupled with electron correlations tends to impose an insulating state. We report results of our investigation of bulk single-crystal Sr0.94Ir0.78O2.68 or Ir-deficient, orthorhombic perovskite SrIrO3. It retains the same crystal structure as stoichiometric SrIrO3 but exhibits a sharp, simultaneous antiferromagnetic (AFM) and metal-insulator (MI) transition occurring in the basal-plane resistivity at 185 K. Above it, the basal-plane resistivity features an extended regime of almost linear temperature dependence up to 800 K but the strong …
Ground-State Tuning Of Metal-Insulator Transition By Compositional Variations In Bair1−XRuXO3 (0 ≤ X ≤ 1), Shujuan Yuan, Kamal H. Butrouna, Jsaminka Terzic, Hao Zheng, Saicharan Aswartham, Lance E. Delong, Feng Ye, P. Schlottmann, Gang Cao
Ground-State Tuning Of Metal-Insulator Transition By Compositional Variations In Bair1−XRuXO3 (0 ≤ X ≤ 1), Shujuan Yuan, Kamal H. Butrouna, Jsaminka Terzic, Hao Zheng, Saicharan Aswartham, Lance E. Delong, Feng Ye, P. Schlottmann, Gang Cao
Physics and Astronomy Faculty Publications
Hexagonal BaIrO3 is a magnetic insulator driven by the spin-orbit interaction (SOI), whereas BaRuO3 is an enhanced paramagnetic metal. Our investigation of structural, magnetic, transport, and thermal properties reveals that substitution of Ru4+ (4d4) ions for Ir4+ (5d5) ions in BaIrO3 reduces the magnitudes of the SOI and a monoclinic structural distortion and rebalances the competition between the SOI and the lattice degrees of freedom to render an evolution from a magnetic insulting state to a robust metallic state. The central findings of this paper are as follows: (1) light …