Atomic, Molecular and Optical Physics Commons^™

Resolution Of Overlapping Spectra By Wavelength Modulation Spectroscopy, Audra Michiele Bullock

Electrical & Computer Engineering Theses & Dissertations

Wavelength modulation absorption spectroscopy is a highly sensitive, non-intrusive technique for probing gaseous species, which employs the well-known principles of modulation spectroscopy in a novel way. With this technique, parameters such as velocity, density, and temperature can be measured with a high degree of precision. The research presented here shows that wavelength modulation is a convenient means of increasing the sensitivity of an absorption spectroscopy measurement because it allows for harmonic detection. The focus of the dissertation is resolution of overlapping spectra by harmonic detection and the advantages gained by performing detection at the higher harmonics, e.g., sixth and eighth. …

New Search For Parity Violation In Nonresonant Neutron Scattering On Thorium, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

The parity-violating longitudinal asymmetry of the neutron scattering cross section has been measured for thorium in the off-resonance energy intervals from 30 to 300 eV. The observed result of (0.5±1.6)×10^-6 is compared with theoretical predictions.

Electric-Octupole And Pure-Electric-Quadrupole Effects In Soft X-Ray Photoemission, Andrei Derevianko, Oliver Hemmers, S. Oblad, P. Glans, H. Wang, S. B. Whitfield, R. Wehlitz, I. A. Sellin, W. R. Johnson, Dennis W. Lindle

Environmental Studies Faculty Publications

Second-order [O(k²), k = ω/c] nondipole effects in soft-x-ray photoemission are demonstrated via an experimental and a theoretical study of angular distributions of neon valence photoelectrons in the 100–1200 eV photon-energy range. A newly derived theoretical expression for nondipolar angular distributions characterizes the second-order effects using four new parameters with primary contributions from pure-quadrupole and octupole-dipole interference terms. Independent-particle calculations of these parameters account for a significant portion of the existing discrepancy between experiment and theory for Ne 2p first-order nondipole parameters.

Parity Violation In Neutron Resonances In 115in, Sharon L. Stephenson, J D. Bowman, J Corvi, Bret E. Crawford, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, H M. Shimizu, Y-F Yen, V W. Yuan, L Zanini

Physics and Astronomy Faculty Publications

Parity nonconservation (PNC) was studied in p-wave resonances in indium by measuring the helicity dependence of the neutron total cross section in the neutron energy range 6.0–316 eV with the time-of-flight method at LANSCE. A total of 36 p-wave neutron resonances were studied in ¹¹⁵In, and statistically significant asymmetries were observed for nine cases. An analysis treating the PNC matrix elements as random variables yields a weak matrix element of M=(0.67_-0.12^+0.16) meV and a weak spreading width of Γ_w=(1.30_-0.43^+0.76)×10^-7 eV.

Classical Versus Quantum Dynamics For A Driven Relativistic Oscillator, Rainer Grobe, Qichang Su, P J. Peverly, R E. Wagner

Faculty publications – Physics

We compare the time evolution of the quantum-mechanical spatial probability density obtained by solving the time-dependent Dirac equation with its classical counterpart obtained from the relativistic Liouville equation for the phase-space density in a regime in which the dynamics is essentially relativistic. For a resonantly driven one-dimensional harmonic oscillator, the simplest nontrivial model system to perform this comparison, we find that, despite the nonlinearity induced by relativity, the classical ensemble description matches the quantum evolution remarkably well.

Tunable Mid-Ir Optical Parametric Oscillator Using Periodically Poled Rubidum Titanyl Arsenate, Frank J. Glavic

Theses and Dissertations

Tunable sources of coherent radiation are needed for a variety of military and commercial applications, including infrared countermeasures and atmospheric remote sensing. This research investigates a tunable mid-infrared coherent source using periodically-poled rubidium titanyl arsenate (PPRTA) as a quasi-phase matched (QPM) optical parametric oscillator (OPO). The advantages of PPRTA over periodically poled lithium niobate (PPLN) are presented. Quasi-phase matching and periodic poling theory are discussed, along with some important historical results and current developments. Experimental setups for determining threshold, conversion efficiency, pump depletion, and beam quality are presented along with experimental results. The research effort is focused on characterizing PPRTA …

Optical Investigation Of Molecular Beam Epitaxy AlXGa1-XN To Determine Material Quality, Judith L. Mcfall

Theses and Dissertations

The purpose of this research was to determine the quality of AIGaN samples with various mole fractions of aluminum doped with silicon. The samples utilized for this study were composed of an AIN buffer layer sandwiched between the sapphire substrate and AIGaN epilayer grown by molecular beam epitaxy (MBE). Cathodoluminescence (CL) and photoluminescence (PL) were employed to determine the mole fraction of aluminum in each sample. These techniques also gave insight into the material's nonuniformity, defects, and impurities. CL was run at 4 different beam energies (2,5,10, & 15 keV) with four different currents (1,10,50, & 90 µA) for the …

Collection Of Detonation Signatures And Characterization Of Spectral Features, Jay A. Orson

Theses and Dissertations

The remote observations of the temporal and spectral characteristics of the infrared (IR) emissions from exploding ordnance have been correlated with explosion conditions. A Bomem MR-154 Fourier Transform Interferometer with two detectors, InSb and HgCdTe, and a 75 mrad telescope was used to record spectra in the 1.3 - 20 µm range. Data was collected at spectral resolutions of 16 cm^-1 and 4 cm^-1 and temporal resolutions of 0.045 s and 0.123 s respectively. Two field tests were conducted: (1) a set of dynamic drop explosions and (2) a series of static detonations. In most events, the temporal …

Atmospheric Temperature Profiles By Ground-Based Infrared Spectrometer Measurements, Jon M. Saul

Theses and Dissertations

A method to recover atmospheric temperature profiles using a ground-based Fourier Transform Infrared spectrometer was investigated. The method used a difference form of the radiative transfer equation, a Bomem MR series Fourier Transform Infrared Spectrometer to collect atmospheric radiance values, and the Phillips Laboratory Expert- assisted User Software (PLEXUS) atmospheric radiance model, to recover an atmospheric temperature profile. The method researched uses radiance values from both the spectrometer measurements and the atmospheric model, along with kernel functions calculated by the atmospheric model as input to a difference form of the radiation transfer equation. From this the change in brightness temperatures …

Pion-Induced Transport Of Π Mesons In Nuclei, S. G. Mashnik, R. J. Peterson, A. J. Sierk, Michael R. Braunstein

All Faculty Scholarship for the College of the Sciences

A large body of data for pion-induced neutral pion continuum spectra spanning outgoing energies near 180 MeV shows no dip there that might be ascribed to internal strong absorption processes involving the formation of Δ’s. This is the same observation previously made for the charged pion continuum spectra. Calculations in an intranuclear cascade model or a cascade exciton model with free-space parameters predict such a dip for both neutral and charged pions. We explore several medium modifications to the interactions of pions with internal nucleons that are able to reproduce the data for nuclei from ⁷Li through Bi.

Lifetime Effects On The Dissociation Of Core-Excited N2 And Co Molecules, N. Saito, A. Hempelmann, F. Heiserq, Oliver Hemmers, K. Wieliczek, J. Viefhaus, U. Becker

Environmental Studies Faculty Publications

Vibrational-resolved ion and ion-pair yield spectra of N₂ and CO taken at their 1s⃗π^* resonance excitations reveal decay-channel-dependent core hole lifetimes. The linewidths of the yield spectra tend to be shortened when the number of electrons ejected in the deexcitation process increases, finally becoming narrower than the total ion yield or absorption natural lifetime width of the core-excited states of N₂ and CO, respectively. In contrast to this, the linewidths of the yield spectra for the singly charged molecular ions, N₂⁺ and CO⁺, are shown to be broader than their corresponding natural linewidths. …

Parity Violation In 232th Neutron Resonances Above 250 Ev, E I. Sharapov, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, J E. Lynch, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, Sharon L. Stephenson, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

The analysis of parity nonconservation (PNC) measurements performed on ²³²Th by the TRIPLE Collaboration has been extended to include the neutron energy range of 250 to 1900 eV. Below 250 eV all ten statistically significant parity violations have the same sign. However, at higher energies PNC effects of both signs were observed in the transmission of longitudinally polarized neutrons through a thick thorium target. Although the limited experimental energy resolution precluded analysis in terms of the longitudinal asymmetry, parity violations were observed and the cross section differences for positive and negative neutron helicities were obtained. For comparison, a similar …

Beyond The Dipole Approximation: Angular-Distribution Effects In The 1s Photoemission From Small Molecules, Dennis W. Lindle, Oliver Hemmers, H. Wang, P. Focke, I. A. Sellin, J. D. Mills, J. A. Sheehy, P. W. Langhoff

Environmental Studies Faculty Publications

Over the past two decades, the dipole approximation has facilitated a basic understanding of the photoionization process in atoms and molecules. Recent experiments on the 1s inner shells of small molecules at relatively low photon energies (⩽ 1000 eV) show strong nondipole effects. They are significant and measurable at energies close to threshold, in conflict with a common assumption that the dipole approximation is valid for photon energies below 1 keV.

Production Of A Signal By Irradiated Cells Which Leads To A Response In Unirradiated Cells Characteristic Of Initiation Of Apoptosis, Fiona Lyng, C. Seymour, C. Mothersill

Articles

This study investigated the ability of medium from irradiated cells to induce early events in the apoptotic cascade, such as mobilization of intracellular calcium, loss of mitochondrial membrane potential and increase in reactive oxygen species, in cells which were never exposed to radiation. Medium from irradiated human keratinocytes was harvested and transferred to unirradiated keratinocytes. Endpoints characteristic of the initiation of apoptosis were monitored for a period of 24 h following medium transfer. Clonogenic survival was also measured. Rapid calcium fluxes (within 30 s), loss of mitochondrial membrane potential, increases in reactive oxygen species (from 6 h after medium transfer), …

Experimental Investigation Of Long-Lived "Zeke" Rydberg States In Ultracold Argon, Gambhir Ranjit

Physics Theses & Dissertations

There is considerable interest in the dynamics of ultracold plasmas and ultracold Rydberg gases. Ultracold plasmas are typically formed by photo-excitation of ultracold atoms to an energy region near (both above and below) an ionization threshold. Excitation to bound, highly-excited Rydberg states can lead to formation of a plasma via several processes, including collisions between Rydberg atoms. Three-body recombination in an ultracold plasma can also result in the production of ultracold Rydberg atoms. Understanding the dynamics of ultracold Rydberg gases is therefore important for understanding the dynamics of ultracold plasmas. In this dissertation, we have investigated the formation and survival …

Applications Of The Atomic Force Microscope Within The Fields Of Haematology And Cytogenetics, Margaret O'Reilly-Crowley

Theses

Atomic force microscopy [AFM] has become a rapidly developing interdisciplinary field of research in recent years. The technique, including instrumentation and specimen preparation methods, is now more sophisticated and its application has increased dramatically. The key advantage of AFM is in providing three-dimensional images of samples imaged. Both size and shape of samples imaged can be obtained allowing their subsequent quantification. Red blood cells [RBCs] and chromosomes were imaged in this work. A brief overview of the current status of biomedical AFM, has been presented in the review.

Measurement of mean cell volume [MCV] of immobilised red blood cells with …

The Absorption Spectrum Of The Hydrogen Atom In Crossed Electric And Magnetic Fields, Dongmei Wang

Dissertations, Theses, and Masters Projects

This dissertation reports the theoretical interpretation of the measured absorption spectrum of hydrogen atoms in crossed electric and magnetic fields. Closed-orbit theory is modified from two-dimensions to three-dimensions to interpret the large scale structure in the absorption spectrum. A new computational method---a Chirped-Fourier-Transform---is developed to extract the closed orbits from an energy spectrum. A quantitative model is provided to calculate the continuum absorption. We prove that the observed continuum absorption is proportional to the flux of electrons along trajectories which escape within a short time. Einstein-Brillouin-Keller (EBK) quantization theory is applied to obtain an approximate energy spectrum. Our results prove …

Redistribution Of Rydberg States By Terahertz Radiation, Jonathan David Curley

Dissertations, Theses, and Masters Projects

We present the technique and results of our study of the redistribution of Rydberg states in barium by a half cycle pulse (HCP). A survey of previous research concerning the interaction of half cycle pulses with Rydberg atoms reveals a lack of experimental data in the area of state redistribution. This is primarily due to an inability to identify the redistributed states accurately using the currently available tool: selective field ionization (SFI). We present the limitations of SFI as a state identification tool. We then present a survey of isolated core excitation as a state identification tool, along with its …