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1998

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Articles 1 - 21 of 21

Full-Text Articles in Atomic, Molecular and Optical Physics

Photofragmentation Of Third-Row Hydrides Following Photoexcitation At Deep-Core Levels, D. L. Hansen, M. E. Arrasate, J. Cotter, G. R. Fisher, Oliver Hemmers, K. T. Leung, Jon C. Levin, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield, Dennis W. Lindle Nov 1998

Photofragmentation Of Third-Row Hydrides Following Photoexcitation At Deep-Core Levels, D. L. Hansen, M. E. Arrasate, J. Cotter, G. R. Fisher, Oliver Hemmers, K. T. Leung, Jon C. Levin, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield, Dennis W. Lindle

X-Ray Atomic and Molecular Science Program

The relaxation dynamics of HCl, DCl, H2S, and D2S following photoexcitation in the vicinities of the Cl and S K-shell thresholds (~2.8 keV for Cl, ~2.5 keV for S) were studied by means of ion time-of-flight mass spectroscopy. In all cases, the onset of pre-edge core-shell photoionization precedes the formation on resonance of a significant amount of neutral hydrogen as well as postcollision-interaction effects above threshold. Examination of the width of the H+ peak in spectra taken with the analyzer parallel and perpendicular to the polarization vector of the incident light indicates that on resonance, …

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Photofragmentation Of Third-Row Hydrides Following Photoexcitation At Deep-Core Levels, D. Hansen, M. E. Arrasate, J. Cotter, G. R. Fisher, Oliver Hemmers, K. T. Leung, Jon C. Levin, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield, Dennis W. Lindle Nov 1998

Photofragmentation Of Third-Row Hydrides Following Photoexcitation At Deep-Core Levels, D. Hansen, M. E. Arrasate, J. Cotter, G. R. Fisher, Oliver Hemmers, K. T. Leung, Jon C. Levin, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield, Dennis W. Lindle

Environmental Studies Faculty Publications

The relaxation dynamics of HCl, DCl, H2S, and D2S following photoexcitation in the vicinities of the Cl and S K-shell thresholds (∼2.8keV for Cl, ∼2.5 keV for S) were studied by means of ion time-of-flight mass spectroscopy. In all cases, the onset of pre-edge core-shell photoionization precedes the formation on resonance of a significant amount of neutral hydrogen as well as postcollision-interaction effects above threshold. Examination of the width of the H+ peak in spectra taken with the analyzer parallel and perpendicular to the polarization vector of the incident light indicates that on resonance, the …

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High-Resolution Electron Time-Of-Flight Apparatus For The Soft-X-Ray Region, Oliver Hemmers, S. B. Whitfield, P. Glans, H. Wang, Dennis W. Lindle, R. Wehlitz, I. A. Sellin Nov 1998

High-Resolution Electron Time-Of-Flight Apparatus For The Soft-X-Ray Region, Oliver Hemmers, S. B. Whitfield, P. Glans, H. Wang, Dennis W. Lindle, R. Wehlitz, I. A. Sellin

Environmental Studies Faculty Publications

A gas-phase time-of-flight (TOF) apparatus, capable of supporting as many as six electron-TOF analyzers viewing the same interaction region, has been developed to measure energy- and angle-resolved electrons with kinetic energies up to 5 keV. Each analyzer includes a newly designed lens system that can retard electrons to about 2% of their initial kinetic energy without significant loss of transmission; the analyzers can thus achieve a resolving power (E/ΔE) greater than 104 over a wide kinetic-energy range. Such high resolving power is comparable to the photon energy resolution of state-of-the-art synchrotron–radiation beamlines in the soft …

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Parity Nonconservation In Neutron Capture On 113cd, S J. Seestrom, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, C R. Gould, D G. Haase, M Iinuma, J N. Knudsen, P E. Koehler, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, Y P. Popov, H Postma, N R. Roberson, E I. Sharapov, H M. Shimizu, D A. Smith, Sharon L. Stephenson, Y-F Yen, V W. Yuan Nov 1998

Parity Nonconservation In Neutron Capture On 113cd, S J. Seestrom, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, C R. Gould, D G. Haase, M Iinuma, J N. Knudsen, P E. Koehler, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, Y P. Popov, H Postma, N R. Roberson, E I. Sharapov, H M. Shimizu, D A. Smith, Sharon L. Stephenson, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

Parity nonconservation was studied for 23 p-wave resonances in 113Cd up to En=500eV at the LANSCE pulsed neutron source using a longitudinally polarized neutron beam and the time-of-flight method. The helicity dependence of the total neutron capture cross section was measured with an enriched 113Cd target and with a target of natural cadmium. Parity violating effects were observed for several resonances in 113Cd and 111Cd. A root-mean-square value of the parity nonconserving matrix element MJ=1=2.9-0.9+1.3meV was obtained for the spin J=1 levels in the compound nucleus 114Cd. This …

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Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson Oct 1998

Auger Resonance Decay Process In Ar 2p Shell Excitation And Ionization, Y. Lu, Wayne C. Stolte, J.A. R. Samson

Chemistry and Biochemistry Faculty Research

The production and subsequent autoionization of the Ar+ (1D2)6d1 satellite state that is formed either by shake-up or recapture during the Auger decay of a 2p vacancy in Ar has been studied by photoelectron spectroscopy in the energy region from 243 to 256 eV. The creation of near zero energy electrons below and immediately above the Ar 2p ionization threshold is discussed. Some ambiguous points in previous studies are clarified.

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Measured Stark Widths And Shifts Of Several Niii Sectral Lines: Temperature Dependence, Stevan Djenize, Vladimir Milosavljevic Aug 1998

Measured Stark Widths And Shifts Of Several Niii Sectral Lines: Temperature Dependence, Stevan Djenize, Vladimir Milosavljevic

Articles

Stark parameters (width and shift) of four doubly ionized nitrogen spectral lines, that belong to 3s-3p and 3p-3d transitions (lower multiplets), have been measured in a linear pulsed, low pressure, arc discharge in the nitrogen-oxygen and helium-nitrogen-oxygen plasmas in a (30 000 - 54 000) K electron temperature and a (0.75 1023 - 2.8 1023) electron density ranges. The measured values have been compared to the existing experimental and calculated data.

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Parity Nonconservation In Neutron Resonances In 232th,, Sharon L. Stephenson, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Y-F Yen, V W. Yuan Aug 1998

Parity Nonconservation In Neutron Resonances In 232th,, Sharon L. Stephenson, J D. Bowman, Bret E. Crawford, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

Parity nonconservation (PNC) was measured for 24 p-wave resonances from 8 to 300 eV in 232Th by measuring the helicity dependence of the total neutron cross section for epithermal neutrons with an improved experimental system. Ten resonances show statistically significant parity violation. For these ten resonances the analyzing powers are all positive, thus confirming the previously observed sign correlation. The data are fit to the sum of two terms, a constant asymmetry and a fluctuating asymmetry. With this ansatz the root-mean-square PNC matrix element M=1.12 meV, which corresponds to a weak spreading widthΓw=4.7×10-7 eV. For the …

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Parity Nonconservation In Neutron Resonances In 238u, Bret E. Crawford, J D. Bowman, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, Y-F Yen, V W. Yuan Aug 1998

Parity Nonconservation In Neutron Resonances In 238u, Bret E. Crawford, J D. Bowman, P P J. Delheij, C M. Frankle, M Iinuma, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

Parity nonconservation (PNC) was studied for 24 p-wave neutron resonances in 238U from 10 to 300 eV by measuring the helicity dependence of the total neutron cross section with an improved experimental apparatus. Six resonances show statistically significant (greater than 2.9σ) parity violation. An analysis treating the PNC matrix elements as random variables yields a root-mean-square PNC matrix element M=0.67-0.16+0.24 meV. The corresponding weak spreading width Γw=(1.35-0.64+0.97)×10-7 eV.

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Neutron Resonance Spectroscopy Of 106pd, And 108pd From 20–2000 Ev, Bret E. Crawford, J D. Bowman, P P J. Delheij, T Haseyama, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, V W. Yuan Aug 1998

Neutron Resonance Spectroscopy Of 106pd, And 108pd From 20–2000 Ev, Bret E. Crawford, J D. Bowman, P P J. Delheij, T Haseyama, J N. Knudsen, L Y. Lowie, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, V W. Yuan

Physics and Astronomy Faculty Publications

Parity nonconserving asymmetries have been measured in p-wave resonances of 106Pd and 108Pd. The data analysis requires knowledge of the neutron resonance parameters. Transmission and capture γ-ray yields were measured for En=20–2000 eV with the time-of-flight method at the Los Alamos Neutron Science Center (LANSCE). A total of 28 resonances in 106Pd and 32 resonances in 108Pd were studied. The resonance parameters for 106Pd are new for all except one resonance. In 108Pd six new resonances were observed and the precision improved for many of the resonance parameters. A Bayesian analysis was …

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Low Saturation Intensities In Two-Photon Ultracold Collisions, C. I. Sukenik, D. Hoffman, S. Bali, T. Walker Jul 1998

Low Saturation Intensities In Two-Photon Ultracold Collisions, C. I. Sukenik, D. Hoffman, S. Bali, T. Walker

Physics Faculty Publications

We have observed violet photon emission resulting from energy-pooling collisions between ultracold Rb atoms illuminated by two colors of near-resonant infrared laser light. We have used this emission as a probe of doubly excited state ultracold collision dynamics. We have observed the lowest saturation intensity for light-induced ultracold collisions seen to date which we identify as due to depletion of incoming ground state flux. We have also varied the detuning of the lasers which allows us to clearly identify the effect of spontaneous emission and optical shielding.

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Electron Emission Following The Interaction Of Slow Highly Charged Ions With Solids, Joseph W. Mcdonald Jun 1998

Electron Emission Following The Interaction Of Slow Highly Charged Ions With Solids, Joseph W. Mcdonald

Dissertations

The interaction of highly-charged ions with surfaces involves many excitation processes of the surface atoms and the bulk material. One such process, the emission of electrons from surfaces due to the potential energy of the incident ions has been studied. The experimental results presented here confirm that the majority of electrons emitted as a result of highly-charged ions interacting with a solid surface have energies of about 20 eV. Auger processes contribute a smaller fraction of the total emitted electrons with increasing Z o f the projectile. This contribution to the total electron emission yield is found to be less …

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Quantum-Statistical Properties Of Two Coupled Modes Of Electromagnetic Field, Serguei Y. Kalmykov, Mikhail E. Veisman Apr 1998

Quantum-Statistical Properties Of Two Coupled Modes Of Electromagnetic Field, Serguei Y. Kalmykov, Mikhail E. Veisman

Serge Youri Kalmykov

Squeezing the quantum fluctuations of the two-mode light due to the nonstationary coupling between the quadrature components q_1 and q_2 is examined. The delta-function and step-function mode couplings are considered. The conditions of weak and strong step-function coupling are distinguished, the latter being the condition of the instability for the classical counterpart of the quantum system under study. Under the conditions of weak coupling the quadrature squeezing is established in both a two-mode electromagnetic noise in thermal equilibrium (the thermal state) and a two- mode correlated coherent state (CCS). Squeezing in the thermal state is suppressed at a high temperature. …

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Neutral Dissociation Of Hydrogen Following Photoexcitation Of Hcl At The Chlorine K Edge, D. L. Hansen, J. Cotter, G. R. Fisher, K. T. Leung, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield Apr 1998

Neutral Dissociation Of Hydrogen Following Photoexcitation Of Hcl At The Chlorine K Edge, D. L. Hansen, J. Cotter, G. R. Fisher, K. T. Leung, R. Martin, Paul Neill, Rupert C. Perera, I. A. Sellin, Marc Simon, Y. Uehara, B. Vanderford, S. B. Whitfield

Chemistry and Biochemistry Faculty Research

Time-of-flight mass spectroscopy was used to study the relaxation dynamics of HCl following photoexcitation in the vicinity of the Cl K edge (~2.8 keV) using monochromatic synchrotron radiation. At the lowest resonant excitation to the 6ơ* antibonding orbital, almost half of the excited molecules decay by emission of a neutral H atom, mostly in coincidence with a highly charged Cln1 ion. The present work demonstrates that neutral-atom emission can be a significant decay channel for excited states with very short lifetimes (1 fs). [S1050-2947(98)03604-X]

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The Effects Of Fabry-Perot Fringing On The Sensitivity Of A Wavelength Modulation Experiment, Patrick C. Shea Apr 1998

The Effects Of Fabry-Perot Fringing On The Sensitivity Of A Wavelength Modulation Experiment, Patrick C. Shea

Electrical & Computer Engineering Theses & Dissertations

Parasitic Fabry-Perot etaloning plagues many experiments which use wavelength modulation spectroscopy. This fringing, which is an artifact that almost always appears in such experiments, arises from multiple reflections in the optical elements in the experimental apparatus. The etaloning plays a detrimental role and limits the ultimate sensitivity of wavelength modulation spectroscopy experiments. The research described in this thesis investigates this phenomenon. Experimental results are presented which show that when the Q-factor of the parasitic etalon is smaller that that of the absorption line being measured, significant improvement in the Signal to Fringe Noise Ratio can be obtained through the use …

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Double Photoionization Of Helium, James A.R. Samson, Wayne C. Stolte, Z. X. He, Y. Lu, J. N. Cutler, R. J. Bartlett Mar 1998

Double Photoionization Of Helium, James A.R. Samson, Wayne C. Stolte, Z. X. He, Y. Lu, J. N. Cutler, R. J. Bartlett

Chemistry and Biochemistry Faculty Research

The cross sections for double photoionization of helium and the ratios of double to single ionization have been measured from the double-ionization threshold to 820 eV. The results are in very good agreement with several recent calculations.

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Optical Physics Of Microcavity Surface Emitting Lasers, Michael J. Noble Mar 1998

Optical Physics Of Microcavity Surface Emitting Lasers, Michael J. Noble

Theses and Dissertations

This dissertation consists of an in-depth theoretical analysis of the optical impact of transverse index confinement on the lasing modes of microcavity surface emitting lasers. Two different variational techniques were employed to calculate the relevant optical laser parameters: (1) modal resonance, field profile, (2) confinement factor, and (3) threshold gain. Through a semianalytic field analysis, two new confinement related effects were discovered: (1) a polarization dependent change in mirror reflectance with aperture radius, and (2) a mode dependent blueshift. Through a numerical field analysis, the physical mechanisms governing diffraction were ascertained. These are: (1) the transverse confinement of the optical …

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Electron Attachment Energies Of The Dna Bases, Kayvan Aflatooni, Gordon A. Gallup, Paul Burrow Jan 1998

Electron Attachment Energies Of The Dna Bases, Kayvan Aflatooni, Gordon A. Gallup, Paul Burrow

Paul Burrow Publications

Injection of electrons into the empty π* molecular orbitals of uracil and the DNA bases creates short-lived anion states whose energies have been determined by electron scattering. A common range of attachment energies into the lowest orbitals is observed in all the bases. Evidence for nuclear motion during the lifetimes of the anions is found in all the compounds except adenine. These properties of the bases as bridge sites along the π-stack of DNA, namely, the effective degeneracy of the anion energies and the strong excitation of vibration, are key parameters for theories of electron-transfer rate, some of …

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Emission Of Excimer Radiation From Direct Current, High-Pressure Hollow Cathode Discharge, Ahmed El-Habachi, Karl H. Schoenbach Jan 1998

Emission Of Excimer Radiation From Direct Current, High-Pressure Hollow Cathode Discharge, Ahmed El-Habachi, Karl H. Schoenbach

Bioelectrics Publications

A novel, nonequilibrium, high-pressure, direct current discharge, the microhollow cathode discharge, has been found to be an intense source of xenon and argon excimer radiation peaking at wavelengths of 170 and 130 nm, respectively. In argon discharges with a 100 μm diam hollow cathode, the intensity of the excimer radiation increased by a factor of 5 over the pressure range from 100 to 800 mbar. In xenon discharges, the intensity at 170 nm increased by two orders of magnitude when the pressure was raised from 250 mbar to 1 bar. Sustaining voltages were 200 V for argon and 400 V …

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Speed Cut-Off Point For Antiforce Waves, Mostafa Hemmati, Mathues Shane Doss, Eric L. George Jan 1998

Speed Cut-Off Point For Antiforce Waves, Mostafa Hemmati, Mathues Shane Doss, Eric L. George

Journal of the Arkansas Academy of Science

A one-dimensional, three-component, fluid model has been employed to investigate the existence of a speed cut-off point for antiforce breakdown waves. The term antiforce wave is used to identify breakdown waves for which the electric field force on electrons is in the opposite direction of wave propagation. The electron fluid-dynamical equations for antiforce waves are different from those of proforce waves. This presentation will address the difference in the set of equations for proforce and antiforce waves and the method of integration of the set of equations through the dynamical transition region for antiforce waves. Also, for antiforce waves, the …

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Superfluorescence From Optically Trapped Calcium Atoms, Xianming Han Jan 1998

Superfluorescence From Optically Trapped Calcium Atoms, Xianming Han

Scholarship and Professional Work - LAS

We have studied superfluorescence (SF) under highly unfavorable conditions of rapid collisional and radiative distribution in a Doppler-broadened medium. Nanosecond SF pulses at 5.5 μm were generated on the Ca 4s4p1P1–3d4s1D2 transition from a column of calcium vapor buffered with Ar by optically pumping the 4s21S0–4s4p1P1 transition. The Rabi frequency associated with the intense pump pulse prevents the occurrence of SF while the pump laser is on. As a result, the predicted scaling laws that describe the properties of SF in a transversely excited system, such as peak heights, pulse widths, and delay times, are shown to apply in our …

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Photolithographic Patterning Of Vacuum-Deposited Organic Light Emitting Devices, Peifang Tian, P. Burrows, B. Bulovic, S. Forrest Dec 1997

Photolithographic Patterning Of Vacuum-Deposited Organic Light Emitting Devices, Peifang Tian, P. Burrows, B. Bulovic, S. Forrest

Peifang Tian

No abstract provided.

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