Physics Commons^™

Neutron-Diffraction And Mössbauer Effect Study Of The Preferential Silicon Site Occupation And Magnetic Structure Of Nd₂Fe₁₄₋ₓsiₓb, Gaya Kanishka Marasinghe, Oran Allan Pringle, Gary J. Long, William Joseph James, Dianne J. Xiao, J. L. Li, William B. Yelon, Fernande Grandjean

Physics Faculty Research & Creative Works

A neutron-diffraction study of Nd₂Fe_14-xSi_xB has shown that silicon preferentially occupies the 4c site in the transition-metal sublattice in Nd₂Fe₁₄B. Silicon also exhibits a moderate preference for the 8j₁ site, is almost excluded from the 16k₂ site, and avoids the 16k₁, 8j₂, and 4e sites. The silicon site occupancy is correlated with a preference for a silicon atom to have rare-earth atoms in its coordination environment. The Mössbauer spectra of Nd₂Fe_14-xSi_xB have been fit with a model which …

Spatially Resolved Transitions To Autoionizing States, J. Greg Story, D. I. Duncan, Thomas F. Gallagher

Physics Faculty Research & Creative Works

We have observed transitions to autoionizing states in Mg using two short optical pulses. Mg atoms are initially prepared in a high lying Rydberg wave packet with the first ps laser. A second ps laser is then used to excite the inner electron, producing an autoionizing state. The dependence of the transition probability on the delay between the two lasers shows that when the second laser is tuned away from the ionic resonance, the inner electron can make a transition only when the Rydberg wave packet is near the core.

Differential Cross Sections For Single And Double Ionization Of Helium By Protons And Antiprotons, L. Meng, Ronald E. Olson, R. Dömer, J. Ullrich, H. Schmidt-Bocking

Physics Faculty Research & Creative Works

Theoretical and experimental cross sections are presented for single and double ionization of He differential in the projectile scattering angle and the transverse energy of the outgoing recoil ion. A dynamical four-body classical trajectory Monte Carlo method that includes radial electron correlation is utilized to calculate total and differential cross sections for 300 and 500 keV protons and antiprotons in impact collisions with He. The azimuthal emission characteristics of electrons, recoil ion and projectile relative to each other are analyzed to provide detailed information on the dynamical differences between single and double ionization and between proton and antiproton impact. © …

Energy-Projected Effective-Medium Theory Of Long-Range Hopping On Energetically Disordered Lattices, Paul Ernest Parris, B. D. Bookout

Physics Faculty Research & Creative Works

We introduce energy-projected equations of motion to treat the diffusive transport of charge carriers that undergo long-range (i.e., greater than nearest-neighbor) hopping among the sites of an energetically disordered lattice. This approach leads naturally to an energy-projected effective-medium theory for treating such systems. Exact expressions for the diffusion constant associated with the energy-projected effective medium theory are obtained. Using the formalism in conjunction with what is normally a rather poor approximation, i.e., the virtual-crystal approximation, we are able to obtain the exact diffusion constant for the long-range symmetric-random-well problem. Effective-medium calculations and numerical simulations are presented for nearest-neighbor and long-range …

Quantal And Classical Correspondence Of Double Scattering, Jianyi Wang, Ronald E. Olson, Karoly Tokési

Physics Faculty Research & Creative Works

Electron emission from atom-atom collisions is analyzed within the framework, of both quantal and classical dynamics. We examine the effect of explicit electron-electron (e-e) interactions on the ejected electron spectra in hard collisions involving simultaneous excitation and ionization in the collision of two structured atoms. A double scattering sequence represented by a second order Bom approximation has been shown to give a dominant contribution over the single scattering to projectile ionization. A classical simulation confirms the double scattering process is analogous to the Thomas two-step capture mechanism. We find good agreement between quantal and classical calculations, showing the convergence of …

Transition From Quantum To Quasi-Classical Behaviour Of The Binary Encounter Peak In Collisions Of 0.6 To 3.6 Mev Amu“¹ I23+ And Xe21+ With He And Ar, J. L. Shinpaughfg, W. Wolff, H. E. Wolff, U. Ramm, O. Jagutzki, H. Schmidt-Böcking, J. Wangt, Ronald E. Olson

Physics Faculty Research & Creative Works

Double differentia] cross sections are reported for the production of binary encounter electrons in collisions of 0.6 MeV amu^-1 I²³⁺ and 1.4, 2.4, and 3.6 MeV amu^-1 Xe²¹⁺ projectiles incident on He and Ar targets. Electron energy spectra were measured between 0: and 45: in the case of the two lower projectile energies, and between 17.5° and 60- for the two higher projectile energies. The data are compared with quantum mechanical impulse approximation and classical trajectory Monte Carlo calculations. While the quantum model calculation predicts a rapid disappearance of diffraction effects in the binary encounter peak …

Dependence Of Binary Encounter Electron Production On The Charge State Of The Recoil Ion, Jee-Ching Wang, Ronald E. Olson, H. Wolf, J. Shinpaugh, W. Wolff, H. Schmidt Böcking

Chemical and Biochemical Engineering Faculty Research & Creative Works

We study the dependence of the production of binary encounter electrons on the charge state of recoil ions for 2.4 MeV u^-l Xe²¹⁺ on He and Ar. Doubly differential cross sections of electron emission are calculated with the ncrMC method. We find that the contributions to the binary electron cross section from various recoil ion charge states reach a maximum near Ar⁵⁺ for the Ar target. In the case of the He target; double ionization dominates over single ionization for alt ejected electron energies above 100 eV. However, an unexpected local drop of double ionization in the …

Temperature And Supersaturation Dependent Nucleation Rates Of Heterogeneous Water By Molecular Cluster Model Calculation, Chen K. Lutrus, Donald E. Hagen, Sung-Ho Suck Salk

Physics Faculty Research & Creative Works

A statistical mechanical method to evaluate the energy of formation of water clusters attached to a foreign particle surface is described, with the binding energy being evaluated on a molecular level, using semiempirical modified neglect of diatomic overlap (MNDO) theory. The model is applied to water nucleation on a silicon oxide surface. The binding energy contribution, which represents the energy of formation at T=0 K, is found to slightly (but not negligibly in the thermal sense) increase with the number of hydrogen bonds between the water cluster and the condensation nucleus whose surface is made of silicon oxide. An analytic …

Connection Between Superelastic And Inelastic Electron-Atom Collisions Involving Polarized Collision Partners, Klaus Bartschat, Don H. Madison

Physics Faculty Research & Creative Works

It is shown how the results of a recent experiment by Jiang, Zuo, Vuković, and Bederson [Phys. Rev. Lett. 68, 915 (1992)], who investigated low-energy electron scattering from laser-excited polarized sodium atoms in the initial (3p) ²P°_3/2 (F=3, M_F=3) state, can be related to the inelastic 3S→3P transition involving initially unpolarized electron and atom beams. Hence, this method can provide an independent check of the traditional electron-scattering experiment with unpolarized beams.

A Neutron Diffraction And Mössbauer Effect Study Of The Magnetic Properties Of Pr₂Fe₁₇ And Pr₂Fe₁₇N₂.₆, Gary J. Long, Oran Allan Pringle, Fernande Grandjean, William B. Yelon, K. H. Buschow

Chemistry Faculty Research & Creative Works

The neutron diffraction powder patterns of Pr₂Fe₁₇ and Pr₂Fe₁₇N_2.6 have been measured at 295 K and refined within the Th₂Zn₁₇ structure type to give the structural changes which occur upon nitrogenation; changes which include a 6.4% expansion of the unit cell volume. The Mössbauer spectra of Pr ₂Fe₁₇ and Pr₂Fe₁₇N_2.6 have been measured between 85 and 295 K and analyzed with a model which is based on the Wigner-Seitz cell environment of each iron site, the basal orientation of the magnetization, and …

Three-Body Distorted-Wave Born Approximation For Electron-Atom Ionization, Stephenie J. Jones, Don H. Madison, Achim Franz, P. L. Altick

Physics Faculty Research & Creative Works

We report a theoretical calculation for electron-impact ionization of atoms that includes short-range electron-atom effects for wave functions that satisfy the exact asymptotic boundary conditions. Results of this theory, which we label as the three-body distorted-wave Born approximation, are compared with experiment and other theories for ionization of hydrogen and helium for incident-electron energies from 4 to 18 times the ionization energy.

Long-Range Random Walks On Energetically Disordered Lattices, B. D. Bookout, Paul Ernest Parris

Physics Faculty Research & Creative Works

Although the master equation describing long-range random walks on an energetically disordered lattice is governed by a nonsymmetric transition matrix W, it may be mapped through a similarity transform onto an imaginary-time Schrödinger equation governed by a Hermitian (Hamiltonian) operator H₀ having a nondegenerate ground state. Under this mapping the diffusion constant D can be expressed in terms of the exact ground state energy of operators that are infinitesimally perturbed from H₀.

Temporal Effects In Multiphoton Ionization Of Lithium, J. Greg Story, Thomas F. Gallagher

Physics Faculty Research & Creative Works

The temporal effects of multiphoton ionization are investigated using a two-color method which determines both the time and intensity at which the process occurs. We show that the total ionization efficiency depends strongly on the time at which an atom makes a transition to an excited state during an intense laser pulse. This result clearly shows that the ac-Stark-shifted bound-state resonances not only enhance the cross section for photoionization, but that the excited bound states provide temporary storage states for the atomic population during the photoionization process.

A Neutron Diffraction And Mössbauer Effect Study Of The Magnetic Structure Of Y₂(Fe₁₋ₓmnₓ)₁₄B, Gaya Kanishka Marasinghe, Oran Allan Pringle, Gary J. Long, William Joseph James, William B. Yelon, Fernande Grandjean

Physics Faculty Research & Creative Works

The magnetic structures of a series of Y₂(Fe _1-xMn_x)₁₄B samples, with x equal to 0.03, 0.10, 0.25, and 0.37, have been studied by powder neutron diffraction and Mössbauer spectroscopy. Y₂(Fe_0.97Mn _0.03)₁₄B and Y₂(Fe_0.9Mn _0.1)₁₄B are ferromagnetic at both 295 and 85 K, Y ₂(Fe_0.63Mn_0.37)₁₄B is paramagnetic at both 295 and 85 K, whereas Y₂(Fe_0.75Mn _0.25)₁₄B is paramagnetic at 295 K and is partially ordered at …

120kev Ar8+-Li Collisions Studied By Near Uv And Visible Photon Spectroscopy, E. Jacquet, P. Boduch, M. Chantepie, M. Druetta, D. Hennecart, X. Husson, D. Lecler, Ronald E. Olson, J. Pascale, N. Stolterfoht, M. Wilson

Physics Faculty Research & Creative Works

A spectroscopic analysis of light emitted in the 200-600 nm wavelength range by Ar⁷⁺, Ar⁶⁺ and Ar⁵⁺ ions after charge exchange in 120keV Ar⁸⁺-Li collisions is performed. Transitions with Δn = 1 and Δn = 2 for n = 8, 9, 10 and 11 states of Ar8 following single electron capture are identified and the production cross sections for n = 8 and n = 9 are deduced from emission cross sections and compared with those calculated by the three-body classical trajectory Monte-Carlo method. Lines due to double capture process were observed and identified …

Resonant Inhibition Of Multiphoton Ionization, J. Greg Story, D. I. Duncan, Thomas F. Gallagher

Physics Faculty Research & Creative Works

When exposed to intense light of ~580 nm, the ground state of K shifts up in energy, passing through two-photon resonances with Rydberg states and finally crossing the two-photon ionization limit. Using laser pulses of 0.5 to 13 ps duration, we have shown experimentally that ionization occurs for short pulses, but for long pulses the population is diverted into the Rydberg states where some population survives the peak intensity of the pulse, in excellent agreement with a dynamic Floquet model.

Monte Carlo Simulations Of Water-Ice Layers On A Model Silver Iodide Substrate: A Comparison With Bulk Ice Systems, James H. Taylor, Barbara N. Hale

Physics Faculty Research & Creative Works

Two water layers adsorbed on a model silver iodide basal face are simulated at nine temperatures from 150 to 425 K using Monte Carlo methods. The periodic unit cell of 96 internally rigid water molecules (interacting via the revised central-force potentials) couples to the rigid-substrate atoms via effective pair potentials with Lennard-Jones short-range and Coulomb long-range terms. The distribution of molecules perpendicular to the substrate exhibits layering, and individual layer structure factors, dipole moments, and "pseudodiffusion" coefficients are calculated. A complex temperature dependence with the two layers taking on different solidlike, quasiliquid, or liquid properties at the same T is …

Residual-Ion Orientation After Autoionization, G. T. Xu, Xiao Wang, J. Greg Story, William E. Cooke

Physics Faculty Research & Creative Works

We have measured the relative population in the two m_j states of barium 6p_1/2 ions produced by the autoionization of (6p_3/2nd)_J=MJ=3 states by detecting the helicity of the emitted fluorescence. These populations can be related to the relative branching ratio into the 6p_1/2εd_5/2 and 6p_1/2εg_7/2 continuum channels. Rydberg states with n=16-23 have similar branching ratios, producing approximately six times as much 6p_1/2εd_5/2 population as 6p_1/2εg_7/2 population.

Evolution Of Atomic Motion In An Intense Standing Wave, Jian Chen, J. Greg Story, Randall G. Hulet

Physics Faculty Research & Creative Works

We have investigated the effect of the dipole force and its fluctuation on the motion of Li atoms in an intense, one-dimensional, near-resonant standing light wave. The duration of the interaction of the atoms with the standing wave was varied from several tens of spontaneous-emission lifetimes to several hundreds. For a standing-wave frequency blue detuned from resonance, diffusive heating can dominate the time-averaged dissipative dipole force so that there is no steady-state momentum distribution. However, for sufficiently large blue detunings, the rate of diffusion is so slow that the resulting distribution approaches a quasisteady state. For red detunings, the diffusion …

Performance Analysis For The Ccn Collection Apparatus, Deborah K. Bircher

Opportunities for Undergraduate Research Experience Program (OURE)

This paper concerns the performance testing of a system to collect and chemically analyze cloud condensation nuclei (CCN). These are the atmospheric particles which nucleate cloud drops.

The air is humidified by passage through the "haze chamber", consisting of parallel vertical plates that are covered with cotton cloth and are kept wet by water supplied at the top edge. The plates are adiabatic , and should equilibrate in temperature at the wet bulb temperature of the incoming air. Measurements of the plate temperature with eighty thermocouples indicate behavior consistent with theory.

Another part of the system is called the CFD …

Motorized Throttle Plate, John D. Crawford

Opportunities for Undergraduate Research Experience Program (OURE)

The objective of this project was to develop a throttle plate mechanism that can be used to simulate transient engine operation. This throttle plate was designed so as to regulate the quantity of air flow entering a Port Fuel Injected (PFI) spark ignition engine prior to the combustion of the fuel-air mixture. The throttle plate is linked to a data acquisition system in order to study the port fuel injection characteristics of the fuel-air mixture. This data acquisition system links the throttle plate angular position information to data obtained using a nonintrusive laser based diagnostic technique, therefore enabling the study …

Active Buckling Control Of Composite Plates, Bradley Wayne Gentelin

Opportunities for Undergraduate Research Experience Program (OURE)

The objective of the research project is to investigate the feasibility of using the rapidly growing technology of smart materials in actively controlling the buckling of laminated composite plates. Advanced composite structures are susceptible to structural instabilities under compression loadings, and the proper control of such instabilities is essential to the effective performance of the structures. The focus of the research activity is to perform an experimental study of using embedded piezoelectric materials for enhancing the critical buckling loads of laminated composite plates. The forces induced by the piezoelectric actuators under the applied voltage fields will be used to counterbalance …

Two Methods For Attenuation Of Vibration In Structures, Kevin Mark Mcclendon

Opportunities for Undergraduate Research Experience Program (OURE)

The purpose of this report is to discuss methods of suppressing vibration in space trusses. The discussion is centered on the approach, structural attributes, and effectiveness of each method. One approach uses structural active members which are actuated to produce “anti-vibration” to cancel vibrations in the truss. The other method is to implement passive and active damping devices at the base of the space truss, where it will absorb vibrations by fluctuating the stiffness of the structures foundation.

Application Of Sunlight Mapping In Solar Car Design, Jeffrey Shapiro, Rob Ziegler, Matt Spaethe, Rick Jenkins

Opportunities for Undergraduate Research Experience Program (OURE)

The design of a solar car is a combination of trade-offs between the mechanical, aerodynamic, and photovoltaic systems. The mechanical and aerodynamic systems can be computationally modeled very well using commercial software. Clouds prevent the photovoltaic system from being modeled as well. This research explores a new way to accurately simulate almost every array configuration imaginable. Using this method, quantitative simulations are produced.

Astronomical Ccd Imaging At Umr: An Interim Report, David A. Thilker, Jon R. Fox

Opportunities for Undergraduate Research Experience Program (OURE)

Progress towards the modernization and update of the UMR observatory through the implementation of astronomical CCD technology is detailed. Preliminary image data is presented, specifically: globular cluster M13 and the lunar surface. An evaluation of the Santa Barbara Instrument Group’s (SBIG) ST-6 CCD camera is presented; bias frames, dark frames, and flat-fields are all examined. A custom optical assembly for instrument focusing and housing BVRI photometry and RGB colorimetry filters is described. The ST60PS data acquisition program, provided by SBIG, is reviewed. Additional work towards the development of a custom image processing utility program is mentioned. Finally, optical telescope collimation …

Catalysis Of Charcoal Emissions, James M. Horak

Opportunities for Undergraduate Research Experience Program (OURE)

This paper is about the development of a system to reduce the emissions of charcoal kilns with the catalyst from automotive catalytic converters. This device, called the charcoal kiln emissions oxidizer (CKEO), was designed and fabricated to meet the goal of a cost effective means to reduce the carbon monoxide and hydrocarbon emissions from charcoal kilns. Testing of the CKEO was never carried out as a test site could not be secured by this writing. The need for the CKEO, the theory behind it, and a procedure to test it are presented.

Damage Assessment Of Composite Structures With Embedded Optical Fibers, Peter E. Hackett

Opportunities for Undergraduate Research Experience Program (OURE)

One of the important features of smart composite structures is their capability to observe their own performance for proper functioning and self-diagnostic purposes. The low velocity impact damage of composite structures (matrix cracking, fiber breakage, delamination, etc.) is often difficult to detect visually and can significantly reduce the strength of the structure. The objective of this research is to develop a technique for fabricating composite laminates that will facilitate the embedment of optical fibers. Composite test specimens will be fabricated in the composite material laboratory. The fabrication of composite laminates with a health monitoring and damage assessment system capable of …

Trapping-To-Percolation Transition In The Hopping Diffusion Of Substitutionally Disordered Solids With A Binary Energy Distribution, Paul Ernest Parris, B. D. Bookout

Physics Faculty Research & Creative Works

We consider charge carriers that undergo nearest-neighbor hopping among the sites of a binary random lattice, each site of which is associated with one of two possible energies E₁ or E₂. A general and recently observed feature of this problem not predicted by previous treatments of disordered hopping models is a crossover between trap-limited conduction and percolation. We introduce new energy-projected equations of motion whose solutions reveal the deep conductivity minimum associated with this phenomenon, and compare the results predicted to numerical simulations.

A Pulsed Power Design For The Linear Inductive Accelerator Modules For The Laboratory Microfusion Fa, Ronald E. Olson, D. L. Smith, M. G. Mazarakis, L. F. Bennett, T. R. Lockner

Physics Faculty Research & Creative Works

No abstract provided.

Defect Structure Of Y1-Ycaymno3 And La1-Ycaymno3. Ii. Oxidation-Reduction Behavior, J. W. Stevenson, M. M. Nasrallah, Harlan U. Anderson, Don M. Sparlin

Materials Science and Engineering Faculty Research & Creative Works

Electrical conductivity, Seebeck coefficient, and thermogravimetric behavior of compositions in the systems Y_1-yCa_yMnO₃ and Y_1-yCa_yMnO₃ were studied as functions of temperature and ambient oxygen activity in order to determine the mechanism of electrical transport and defect structure. Compositions in Y_1-yCa_yMnO₃ exhibited very slight oxygen activity-dependent behavior as the ambient oxygen activity was reduced. A defect model which includes the thermally excited disproportionation of Mn³⁺ into Mn²⁺ and Mn⁴⁺ pairs was applied to the oxygen-activity-dependent data for La_0.80Ca_0.20MnO_{3 …}