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Full-Text Articles in Other Physics

Structure And Magnetism Of New Rare- Earth-Free Intermetallic Compounds: Fe3+Xco3−Xti2 (0 ≤ X ≤ 3), Balamurugan Balamurugan, Bhaskar Das, Manh Cuong Ngyuen, Xiaoshan Xu, Jie Zhang, Xiaozhe Zhang, Yaohua Liu, Ashfia Huq, Shah R. Valloppilly, Yunlong Jin, Cai-Zhuang Wang, Kai-Ming Ho, David J. Sellmyer Jan 2016

Structure And Magnetism Of New Rare- Earth-Free Intermetallic Compounds: Fe3+Xco3−Xti2 (0 ≤ X ≤ 3), Balamurugan Balamurugan, Bhaskar Das, Manh Cuong Ngyuen, Xiaoshan Xu, Jie Zhang, Xiaozhe Zhang, Yaohua Liu, Ashfia Huq, Shah R. Valloppilly, Yunlong Jin, Cai-Zhuang Wang, Kai-Ming Ho, David J. Sellmyer

Nebraska Center for Materials and Nanoscience: Faculty Publications

We report the fabrication of a set of new rare-earth-free magnetic compounds, which form the Fe3Co3Ti2-type hexagonal structure with P-6m2 symmetry. Neutron powder diffraction shows a significant Fe/Co anti-site mixing in the Fe3Co3Ti2 structure, which has a strong effect on the magnetocrystalline anisotropy as revealed by first-principle calculations. Increasing substitution of Fe atoms for Co in the Fe3Co3Ti2 lattice leads to the formation of Fe4Co2Ti2 , Fe5CoTi, and Fe6Ti2 with significantly improved …


Reconfigurable Large-Area Magnetic Vortex Circulation Patterns, Robert Streubel, Florian Kronast, Ulrich K. Rößler, Oliver G. Schmidt, Denys Makarov Sep 2015

Reconfigurable Large-Area Magnetic Vortex Circulation Patterns, Robert Streubel, Florian Kronast, Ulrich K. Rößler, Oliver G. Schmidt, Denys Makarov

Robert Streubel Papers

Magnetic vortices in nanodots own a switchable circulation sense. These nontrivial magnetization configurations can be arranged into extended and interacting patterns. We have experimentally created large arrays of magnetically reconfigurable vortex patterns in nonplanar honeycomb lattices using particle lithography. Optimizing height asymmetry of the vertices and applying an in-plane magnetic field provide means to switch between homocircular and staggered vortex patterns with a potentially high impact on magnonics and spintronics relying on chiral noncollinear spin textures. To this end, exchange coupling of extended vortex lattices with an out-of-plane magnetized layer allows one to realize artificial skyrmionic core textures with controllable …


Magnetization Dynamics Of Imprinted Non-Collinear Spin Textures, Robert Streubel, Peter Fischer, Martin Kopte, Oliver G. Schmidt, Denys Makarov Sep 2015

Magnetization Dynamics Of Imprinted Non-Collinear Spin Textures, Robert Streubel, Peter Fischer, Martin Kopte, Oliver G. Schmidt, Denys Makarov

Robert Streubel Papers

We study the magnetization dynamics of non-collinear spin textures realized via imprint of the magnetic vortex state in soft permalloy into magnetically hard out-of-plane magnetized Co/Pd nanopatterned heterostructures. Tuning the interlayer exchange coupling between soft- and hard-magnetic subsystems provides means to tailor the magnetic state in the Co/Pd stack from being vortex- to donut-like with different core sizes. While the imprinted vortex spin texture leads to the dynamics similar to the one observed for vortices in permalloy disks, the donut-like state causes the appearance of two gyrofrequencies characteristic of the early and later stages of the magnetization dynamics. The dynamics …


Retrieving Spin Textures On Curved Magnetic Thin Films With Full-Field Soft X-Ray Microscopies, Robert Streubel, Florian Kronast, Peter Fischer, Dula Parkinson, Oliver G. Schmidt, Denys Makarov Jul 2015

Retrieving Spin Textures On Curved Magnetic Thin Films With Full-Field Soft X-Ray Microscopies, Robert Streubel, Florian Kronast, Peter Fischer, Dula Parkinson, Oliver G. Schmidt, Denys Makarov

Robert Streubel Papers

X-ray tomography is a well-established technique to characterize 3D structures in material sciences and biology; its magnetic analogue - magnetic X-ray tomography - is yet to be developed. Here we demonstrate the visualization and reconstruction of magnetic domain structures in a 3D curved magnetic thin films with tubular shape by means of full-field soft X-ray microscopies. The 3D arrangement of the magnetization is retrieved from a set of 2D projections by analysing the evolution of the magnetic contrast with varying projection angle. Using reconstruction algorithms to analyse the angular evolution of 2D projections provides quantitative information about domain patterns and …


Chirally-Sensitive Electron-Molecule Interactions, J. M. Dreiling, Timothy J. Gay Jan 2015

Chirally-Sensitive Electron-Molecule Interactions, J. M. Dreiling, Timothy J. Gay

Timothy J. Gay Publications

All molecular forms of life have chemically-specific handedness. However, the origin of these asymmetries is not understood. A possible explanation was suggested by Vester and Ulbricht immediately following the discovery of parity violation in 1957: chiral beta radiation in cosmic rays may have preferentially destroyed one enantiomeric form of various biological precursors. In the experiments reported here, we observed chiral specificity in two electronmolecule interactions: quasi-elastic scattering and dissociative electron attachment. Using lowenergy longitudinally spin-polarized (chiral) electrons as substitutes for beta rays, we found that chiral bromocamphor molecules exhibited both a transmission and dissociative electron attachment rate that depended on …


Magnetic Force Microscopy Study Of Zr2co11-Based Nanocrystalline Materials: Effect Of Mo Addition, Lanping Yue, Yunlong Jin, Wenyong Zhang, David J. Sellmyer Jan 2015

Magnetic Force Microscopy Study Of Zr2co11-Based Nanocrystalline Materials: Effect Of Mo Addition, Lanping Yue, Yunlong Jin, Wenyong Zhang, David J. Sellmyer

Nebraska Center for Materials and Nanoscience: Faculty Publications

The addition of Molybdenum was used to modify the nanostructure and enhance coercivity of rare-earth-free Zr2Co11-based nanocrystalline permanent magnets. The effect of Mo addition on magnetic domain structures of melt spun nanocrystalline Zr16Co84−xMox (𝑥 = 0, 0.5, 1, 1.5, and 2.0) ribbons has been investigated. It was found that magnetic properties and local domain structures are strongly influenced by Mo doping. The coercivity of the samples increases with the increase in Mo content (𝑥 ≤ 1.5). The maximum energy product (𝐵𝐻)max increases with increasing 𝑥 from 0.5 MGOe for 𝑥 …


Magnetic Chiral Spin Textures By Imprinting, Robert Streubel, F. Kronast, U. Rössler, O. G. Schmidt, P. Fischer, D. Makarov Jan 2015

Magnetic Chiral Spin Textures By Imprinting, Robert Streubel, F. Kronast, U. Rössler, O. G. Schmidt, P. Fischer, D. Makarov

Robert Streubel Papers

The unique properties of non-trivial topological states, e.g. magnetic skyrmions [1] may path the way towards novel spintronic devices [2]. However, these spin textures have only been observed in special classes of materials possessing non-centrosymmetric crystal structure [1,3-6] and at low temperatures, which limits their application potential. We offer an alternate route to design synthetic magnetic heterostructures that resemble swirls, vortices or skyrmions with distinct topological charge densities at room temperature. By vertically stacking two magnetic nanopatterns with in-and out-of-plane magnetization and tailoring the interlayer exchange coupling, non-collinear spin textures with tunable topological charge can be imprinted (Fig. 1a).


Manipulating Topological States By Imprinting Non-Collinear Spin Textures, Robert Streubel, Luyang Han, Mi Young Im, Florian Kronast, Ulrich K. Rößler, Florin Radu, Radu Abrudan, Gungun Lin, Oliver G. Schmidt, Peter Fischer, Denys Makarov Jan 2015

Manipulating Topological States By Imprinting Non-Collinear Spin Textures, Robert Streubel, Luyang Han, Mi Young Im, Florian Kronast, Ulrich K. Rößler, Florin Radu, Radu Abrudan, Gungun Lin, Oliver G. Schmidt, Peter Fischer, Denys Makarov

Robert Streubel Papers

Topological magnetic states, such as chiral skyrmions, are of great scientific interest and show huge potential for novel spintronics applications, provided their topological charges can be fully controlled. So far skyrmionic textures have been observed in noncentrosymmetric crystalline materials with low symmetry and at low temperatures. We propose theoretically and demonstrate experimentally the design of spin textures with topological charge densities that can be tailored at ambient temperatures. Tuning the interlayer coupling in vertically stacked nanopatterned magnetic heterostructures, such as a model system of a Co/Pd multilayer coupled to Permalloy, the in-plane non-collinear spin texture of one layer can be …


Magnetic Soft X-Ray Tomography Of Magnetic Swiss Roll Architectures, Robert Streubel, F. Kronast, P. Fischer, O. G. Schmidt, D. Makarov Jan 2015

Magnetic Soft X-Ray Tomography Of Magnetic Swiss Roll Architectures, Robert Streubel, F. Kronast, P. Fischer, O. G. Schmidt, D. Makarov

Robert Streubel Papers

A further increase in performance of state-of-the-art spin-electronics can be achieved by either miniaturizing its functional components or harnessing the third dimension. The first route, however, faces physical limitations as properties of nanostructures and their response to external stimuli can drastically change in reduced dimensions. An alternative way is to go from planar 2D structures to 3D architectures [1]. Such 3D functional elements can be obtained for example by rolling up initially planar strained thin films into Swiss roll like objects with multiple windings (Fig. 1a). A major advantage of this technology platform is the possibility to fabricate compact multifunctional …


Electrostatic Charge On Flying Hummingbirds And Its Potential Role In Pollination, Marc Badger, Victor Manuel Ortega-Jimenez, Lisa Von Ribenau, Ashley Smiley, Robert Dudley, Alexei Gruverman , Editor Jan 2015

Electrostatic Charge On Flying Hummingbirds And Its Potential Role In Pollination, Marc Badger, Victor Manuel Ortega-Jimenez, Lisa Von Ribenau, Ashley Smiley, Robert Dudley, Alexei Gruverman , Editor

Alexei Gruverman Publications

Electrostatic phenomena are known to enhance both wind- and insect-mediated pollination, but have not yet been described for nectar-feeding vertebrates. Here we demonstrate that wild Anna's Hummingbirds (Calypte anna) can carry positive charges up to 800 pC while in flight (mean ± s.d.: 66 ± 129 pC). Triboelectric charging obtained by rubbing an isolated hummingbird wing against various plant structures generated charges up to 700 pC. A metal hummingbird model charged to 400 pC induced bending of floral stamens in four plants (Nicotiana, Hemerocallis, Penstemon, and Aloe spp.), and also attracted falling Lycopodium spores at distances of < 2 mm. Electrostatic forces may therefore influence pollen transfer onto nectar-feeding birds.


Chirally Sensitive Electron-Induced Molecular Breakup And The Vester-Ulbricht Hypothesis, J. M. Dreiling, Timothy J. Gay Jan 2014

Chirally Sensitive Electron-Induced Molecular Breakup And The Vester-Ulbricht Hypothesis, J. M. Dreiling, Timothy J. Gay

Timothy J. Gay Publications

We have studied dissociative electron attachment in sub-eV collisions between longitudinally polarized electrons and chiral bromocamphor molecules. For a given target enantiomer, the dissociative Br anion production depends on the helicity of the incident electrons, with an asymmetry that depends on the electron energy and is of order 3 × 10−4. The existence of chiral sensitivity in a well-defined molecular breakup reaction demonstrates the viability of the Vester-Ulbrict hypothesis, namely, that the longitudinal polarization of cosmic beta radiation was responsible for the origins of biological homochirality.


Spin Density Waves In Periodically Strained Graphene Nanoribbons, Nabil M. Al-Aqtash, Renat F. Sabirianov Jan 2014

Spin Density Waves In Periodically Strained Graphene Nanoribbons, Nabil M. Al-Aqtash, Renat F. Sabirianov

Nebraska Center for Materials and Nanoscience: Faculty Publications

Zigzag graphene nanoribbons (ZGNRs) are antiferromagnetic in the ground state with zero net magnetization due to the compensation of contributions from opposite edges. Uniform deformations (both shear and axial) do not produce magnetization due to symmetry restrictions. However, we report the results of first-principles calculations that predict the induction of spin density waves (SDWs) in ZGNRs under non-uniform periodic strain. Using the density functional theory (DFT) method, we show that a sinusoidal magnetization variation along the axis of the ribbon occurs under a sinusoidal transversal shear strain. SDWs appear due to the presence of a strain gradient that induced asymmetry …


The Spin State Of A Molecular Adsorbate Driven By The Ferroelectric Substrate Polarization†, Xin Zhang, Tatiana Palamarciuc, Jean-François Létard, Patrick Rosa, Eduardo Vega Lozada, Fernand Torres, Luis G. Rosa, Bernard Doudin, Peter A. Dowben Jan 2014

The Spin State Of A Molecular Adsorbate Driven By The Ferroelectric Substrate Polarization†, Xin Zhang, Tatiana Palamarciuc, Jean-François Létard, Patrick Rosa, Eduardo Vega Lozada, Fernand Torres, Luis G. Rosa, Bernard Doudin, Peter A. Dowben

Peter Dowben Publications

The spin state of [Fe(H2B(pz)2)2(bipy)] thin films is mediated by changes in the electric field at the interface of organic ferroelectric polyvinylidene fluoride with trifluoroethylene (PVDF–TrFE). Signatures of the molecular crossover transition are evident in changes in the unoccupied states and the related shift from diamagnetic to paramagnetic characteristics. This may point the way to the molecular magneto-electric effect on devices.


Positive Exchange Bias In Epitaxial Permalloy/Mgo Integrated With Si (100), S. S. Rao, J. T. Prater, Fan Wu, S. Nori, D. Kumar, Lanping Yue, Sy_Hwang Liou, Jagdish Narayan Jan 2014

Positive Exchange Bias In Epitaxial Permalloy/Mgo Integrated With Si (100), S. S. Rao, J. T. Prater, Fan Wu, S. Nori, D. Kumar, Lanping Yue, Sy_Hwang Liou, Jagdish Narayan

Sy-Hwang Liou Publications

In magnetic random access memory (MRAM) devices, soft magnetic thin film elements such as permalloy (Py) are used as unit cells of information. The epitaxial integration of these elements with the technologically important substrate Si (100) and a thorough understanding of their magnetic properties are critical for CMOS-based magnetic devices. We report on the epitaxial growth of Ni82.5Fe17.5 (permalloy, Py) on Si (100) using a TiN/MgO buffer layer. Initial stages of growth are characterized by the formation of discrete islands that gradually merge into a continuous film as deposition times are extended. Interestingly, we find that the …


Use Of Zwitterionic Molecules For Forming A Hole Or Electron Transport Layer, Bernard Doudin, Pierre Braunstein, Lucie Routaboul, Guillaume Dalmas, Zhengzheng Zhang, Peter Dowben Aug 2013

Use Of Zwitterionic Molecules For Forming A Hole Or Electron Transport Layer, Bernard Doudin, Pierre Braunstein, Lucie Routaboul, Guillaume Dalmas, Zhengzheng Zhang, Peter Dowben

Peter Dowben Publications

The invention relates to the use of zwitterionic molecules for forming a hole or electron transport layer. The preferred zwitterionic molecules of the invention are derivatives of p-benzoquinonemonoimines. The invention is useful in the field of electronic devices in particular.


Study Of The Growth And Switching Kinetics On Ferroelectric Nanocrystals Of Copolymer Vinylidene Fluoride And Trifluoroethylene On An Atomic Force Microscope, R. V. Gaynutdinov, O. A. Lysova, A. L. Tolstikhina, V. M. Fridkin, S. G. Yudin, Stephen Ducharme Mar 2013

Study Of The Growth And Switching Kinetics On Ferroelectric Nanocrystals Of Copolymer Vinylidene Fluoride And Trifluoroethylene On An Atomic Force Microscope, R. V. Gaynutdinov, O. A. Lysova, A. L. Tolstikhina, V. M. Fridkin, S. G. Yudin, Stephen Ducharme

Stephen Ducharme Publications

The growth of nanocrystals obtained from Langmuir-Blodgett films of ferroelectric copolymer consisting of 70% vinylidene fluoride and 30% trifluoroethylene has been investigated by atomic force microscopy (AFM). The radius and concentration of nanocrystals are found to depend on the annealing time of the film. A model for nanocrystal growth is proposed which yields adequate time dependences for nanocrystal size parameters. The switching kinetics of individual ferroelectric nanocrystals with an average diameter of 100–200 nm and a height of 15–20 nm has been investigated in the piezoelectric response mode. It is shown that the switching of nanocrystals has an activation character.


Strain-Mediated Elastic Coupling In Magnetoelectric Nickel/Barium-Titanate Heterostructures, Robert Streubel, Denny Köhler, Rudolf Schäfer, Lukas M. Eng Feb 2013

Strain-Mediated Elastic Coupling In Magnetoelectric Nickel/Barium-Titanate Heterostructures, Robert Streubel, Denny Köhler, Rudolf Schäfer, Lukas M. Eng

Robert Streubel Papers

Multiferroic nanomaterials bear the potential for assembling a manifold of novel and smart devices. For room temperature (RT) applications, however, only the BiFeO3 single-phase perovskites are potential candidates to date. Nevertheless, vertical heterostructures separating magnetic and ferroelectric functionality into different layers are now widely proposed to circumvent this lack in materials' availability. We show here that the second approach is very profitable as illustrated by the strain-mediated coupling between such two layers, i.e., a ferroelectric barium titanate single-crystal (BTO) and a magnetostrictive nickel (Ni) thin film. Applying an electric field across the BTO substrate forces the magnetic easy axis in …


Adherent Cells Avoid Polarization Gradients On Periodically Poled Litao3 Ferroelectrics, Christof Christophis, Elisabetta Ada Cavalcanti-Adam, Maximilian Hanke, Kenji Kitamura, Alexei Gruverman, Michael Grunze, Peter A. Dowben, Axel Rosenhahn Jan 2013

Adherent Cells Avoid Polarization Gradients On Periodically Poled Litao3 Ferroelectrics, Christof Christophis, Elisabetta Ada Cavalcanti-Adam, Maximilian Hanke, Kenji Kitamura, Alexei Gruverman, Michael Grunze, Peter A. Dowben, Axel Rosenhahn

Peter Dowben Publications

The response of fibroblast cells to periodically poled LiTaO3 ferroelectric crystals has been studied. While fibroblast cells do not show morphological differences on the two polarization directions, they show a tendency to avoid the field gradients that occur between polarization domains of the ferroelectric. The response to the field gradients is fully established after one hour, a time at which fibroblasts form their first focal contacts. If suspension cells, with a lower tendency to establish strong surface contacts are used, no influence of the field gradients is observed.


Search For Spin-Polarized Photoemission From Gaas Using Light With Orbital Angular Momentum, Nathan B. Clayburn, J. L. Mccarter, J. M. Dreiling, M. Poelker, D. M. Ryan, Timothy J. Gay Jan 2013

Search For Spin-Polarized Photoemission From Gaas Using Light With Orbital Angular Momentum, Nathan B. Clayburn, J. L. Mccarter, J. M. Dreiling, M. Poelker, D. M. Ryan, Timothy J. Gay

Timothy J. Gay Publications

Laser light with photon energy near the band gap of GaAs and in Laguerre-Gaussian modes with different amounts of orbital angular momentum was used to produce photoemission from unstrained GaAs. The degree of electron spin polarization was measured using a micro-Mott polarimeter and found to be consistent with zero with an upper limit of ∼3% for light with up to ±5h of orbital angular momentum. In contrast, the degree of spin polarization of 32.3 ± 1.4% using circularly polarized laser light at the as the same wavelength, which is typical for bulk GaAs photocathodes.


Changing Molecular Band Offsets In Polymer Blends Of (P3ht/P(Vdf–Trfe)) Poly(3-Hexylthiophene) And Poly(Vinylidene Fluoride With Trifluoroethylene) Due To Ferroelectric Poling, Freddy Wong, Godohaldo Perez, Manuel Bonilla, Juan A. Colon-Santana, Xin Zhang, Pankaj Sharma, Alexei Gruverman, Peter A. Dowben, Luis G. Rosa Jan 2013

Changing Molecular Band Offsets In Polymer Blends Of (P3ht/P(Vdf–Trfe)) Poly(3-Hexylthiophene) And Poly(Vinylidene Fluoride With Trifluoroethylene) Due To Ferroelectric Poling, Freddy Wong, Godohaldo Perez, Manuel Bonilla, Juan A. Colon-Santana, Xin Zhang, Pankaj Sharma, Alexei Gruverman, Peter A. Dowben, Luis G. Rosa

Peter Dowben Publications

Photoelectron emission and inverse photoemission spectroscopy studies of polymer blends of poly(vinylidene fluoride (70%) – trifluoroethylene (30%)) P(VDF–TrFE 70 : 30) and regio-regular poly(3- hexylthiophene) (P3HT) provide evidence of changes in the molecular band offsets as a result of changes in the ferroelectric polarization in P(VDF–TrFE). Investigation of the blends with higher concentrations of the semiconducting P3HT component revealed that the organic semiconductor component of the blend dominates the electronic structure in the vicinity of the chemical potential. Specifically, the states of P3HT at the conduction band minimum and valence band maximum fall within the HOMO–LUMO gap of the dielectric …


Induced Magneto-Electric Coupling In Ferroelectric/Ferromagnetic Heterostructures, Jeffery Carvell, Ruihua Cheng, Peter A. Dowben, Q Yang Jan 2013

Induced Magneto-Electric Coupling In Ferroelectric/Ferromagnetic Heterostructures, Jeffery Carvell, Ruihua Cheng, Peter A. Dowben, Q Yang

Peter Dowben Publications

Using an external magnetic field, we have demonstrated room temperature control of the electric polarization of a ferroelectric polymer, polyvinylidene fluoride (PVDF), in an artificial multiferroic structure. For ferroelectric PVDF polymer thin films in an iron-PVDF-iron heterostructure, both the ferroelectric coercivity and polarization display a hysteresis dependence on the external magnetic field. We also find that the thickness of the PVDF layer has an effect on the magnetoelectric coupling in our samples. We observe a giant magnetoelectric coupling with values as large as 3700 V/cm Oe to 41700 V/cm Oe.


Magnetoelectric Coupling At The Euo/Batio3 Interface, Shi Cao, P Liu, Jinke Tang, Haidong Lu, C W. Bark, Sangjin Ryu, Chang-Beom Eom, Alexei Gruverman, Peter A. Dowben Jan 2013

Magnetoelectric Coupling At The Euo/Batio3 Interface, Shi Cao, P Liu, Jinke Tang, Haidong Lu, C W. Bark, Sangjin Ryu, Chang-Beom Eom, Alexei Gruverman, Peter A. Dowben

Peter Dowben Publications

Magnetization modulation by ferroelectric polarization switching is reported for the ferromagnetic-ferroelectric EuO/BaTiO3heterostructure. The value of the magnetization critical exponent β is consistent with the expected Heisenberg-like ferromagnetism of EuO and reported Curie temperature. The critical exponent is seen to decrease with increased magnetic coupling. The results are discussed in the context of data obtained earlier for epitaxial La0.67Sr0.33MnO3/BaTiO3 heterostructures, where magnetization increases and critical exponent b also declines with ferroelectric polarization pointing away from ferromagnetic layer. The observed similarity between two systems illustrates an importance of charge doping in magnetoelectric coupling, …


Adsorption Of Tcnqh-Functionalized Quinonoid Zwitterions On Gold And Graphene: Evidence For Dominant Intermolecular Interactions+, Lingmei Kong, Lucie Routaboul, Pierre Braunstein, Hong-Gi Park, Jaewu Choi, John P. Colon Cordova, E Vega, Luis G. Rosa, Bernard Doudin, Peter A. Dowben Jan 2013

Adsorption Of Tcnqh-Functionalized Quinonoid Zwitterions On Gold And Graphene: Evidence For Dominant Intermolecular Interactions+, Lingmei Kong, Lucie Routaboul, Pierre Braunstein, Hong-Gi Park, Jaewu Choi, John P. Colon Cordova, E Vega, Luis G. Rosa, Bernard Doudin, Peter A. Dowben

Peter Dowben Publications

We experimentally investigate the electronic structure of the strongly dipolar, quinonoid-type molecule obtained by TCNQH-functionalization (TCNQH = (NC)2CC6H4CH(CN)2) of (6Z)-4-(butylamino)-6-(butyliminio)- 3-oxocyclohexa-1,4-dien-1-olate C6H2(...NHR)2(...O)2 (where R = n-C4H9) to be very similar after deposition from solution on either graphene or gold substrates. These zwitterion adsorbate thin films form structures that are distinct from those formed by related quinonoid molecules previously studied. We argue that adsorbate–adsorbate interactions dominate and lead to a Stranski–Krastanov ‘island growth’ mechanism.


Threshold Alignment Reversal And Circularly Polarized Fluorescence In Rotationally Resolved H2, Jack W. Maseberg, Klaus Bartschat, Timothy J. Gay Jan 2013

Threshold Alignment Reversal And Circularly Polarized Fluorescence In Rotationally Resolved H2, Jack W. Maseberg, Klaus Bartschat, Timothy J. Gay

Timothy J. Gay Publications

Using H2 and D2 targets, we have measured the polarization of Fulcher-band fluorescence resulting from spin-polarized electron-impact excitation of vibrationally and rotationally resolved d 3Πu→ a 3 ∑g+ transitions for incident electron energies from 14.3 to 28.5 eV. Near threshold, the linear polarization P1 descends from positive values through zero to negative values, indicating a dynamic production of MN = 0 states. The circular polarization P3 is measured to be nonzero, indicating the orientation of rotationally resolved molecular states. For Q-branch transitions, P3 is consistent with theory based …


Compact Inline Optical Electron Polarimeter, Munir Pirbhai, D. M. Ryan, G. Richards, Timothy J. Gay Jan 2013

Compact Inline Optical Electron Polarimeter, Munir Pirbhai, D. M. Ryan, G. Richards, Timothy J. Gay

Timothy J. Gay Publications

A compact optical electron polarimeter using a helium target is described. It offers a maximum fluorescence detection efficiency of ∼20 Hz/nA, which is an order of magnitude higher than that of earlier designs. With an argon target, this device is expected to have a polarimetric figure-of-merit of 270 Hz/nA. By relying on a magnetic field to guide a longitudinally spin-polarized electron beam, the present instrument employs fewer electrodes. It also uses a commercially available integrated photon counting module. These features allow it to occupy a smaller volume and make it easier to operate.


Optically Pumped Spin-Exchange Polarized-Electron Source, Munir Pirbhai, J. Knepper, E. T. Litaker, D. Tupa, Timothy J. Gay Jan 2013

Optically Pumped Spin-Exchange Polarized-Electron Source, Munir Pirbhai, J. Knepper, E. T. Litaker, D. Tupa, Timothy J. Gay

Timothy J. Gay Publications

We describe the operation of a prototype polarized-electron source. Rubidium vapor, contained in a cell, is optically pumped in the presence of a buffer gas. Unpolarized electrons from a tungsten filament are injected into the cell and extracted after undergoing spin exchange with the Rb atoms. We compare the performance of the source when different buffer gases are used. We measure a decrease in electron polarization as their injection energy increases, but find an unexpected regime at higher injection energies yielding increased electron polarization accompanied by a 40-fold increase in current, suggesting the production of slow secondary electrons in the …


Two Novel Approaches For Electron Beam Polarization From Unstrained Gaas, James L. Mccarter, Nathan B. Clayburn, J. M. Dreiling, Timothy J. Gay, Dominic M. Ryan, John Hansknecht, Matt Poelker, Andrei Afanasev, Ara Kechiantz Jan 2013

Two Novel Approaches For Electron Beam Polarization From Unstrained Gaas, James L. Mccarter, Nathan B. Clayburn, J. M. Dreiling, Timothy J. Gay, Dominic M. Ryan, John Hansknecht, Matt Poelker, Andrei Afanasev, Ara Kechiantz

Timothy J. Gay Publications

Two novel approaches to producing highly-polarized electron beams from unstrained GaAs were tested using a micro-Mott polarimeter. Based on a suggestion by Nakanishi [1]], twophoton photoemission with 1560 nm light was used with photocathodes of varying thickness: 625m, 0.32m, and 0.18m. For each of these photocathodes, the degree of spin polarization of the photoemitted beam was less than 50%. Polarization via two-photon absorption was highest from the thinnest photocathode sample and close to that obtained from one-photon absorption (using 778 nm light), with values 40.3±1.0% and 42.6±1.0%, respectively. The second attempt to produce highly-polarized electrons used one-photon emission with 778 …


Equilibrium Magnetic States In Individual Hemispherical Permalloy Caps, Robert Streubel, Volodymyr P. Kravchuk, Denis D. Sheka, Denys Makarov, Florian Kronast, Oliver G. Schmidt, Yuri Gaididei Sep 2012

Equilibrium Magnetic States In Individual Hemispherical Permalloy Caps, Robert Streubel, Volodymyr P. Kravchuk, Denis D. Sheka, Denys Makarov, Florian Kronast, Oliver G. Schmidt, Yuri Gaididei

Robert Streubel Papers

The magnetization distributions in individual soft magnetic permalloy caps on non-magnetic spherical particles with sizes ranging from 50 to 800nm are investigated. We experimentally visualize the magnetic structures at the resolution limit of the x-ray magnetic circular dichroism photoelectron emission microscopy (XMCD-PEEM). By analyzing the so-called tail contrast in XMCD-PEEM, the spatial resolution is significantly enhanced, which allowed us to explore magnetic vortices and their displacement on curved surfaces. Furthermore, cap nanostructures are modeled as extruded hemispheres to determine theoretically the phase diagram of equilibrium magnetic states. The calculated phase diagram agrees well with the experimental observations. © 2012 American …


Magnetic Vortices On Closely Packed Spherically Curved Surfaces, Robert Streubel, Denys Makarov, Florian Kronast, Volodymyr Kravchuk, Manfred Albrecht, Oliver G. Schmidt May 2012

Magnetic Vortices On Closely Packed Spherically Curved Surfaces, Robert Streubel, Denys Makarov, Florian Kronast, Volodymyr Kravchuk, Manfred Albrecht, Oliver G. Schmidt

Robert Streubel Papers

We investigate the change of magnetic vortex states driven by curvature. The equilibrium state and magnetization reversal of soft magnetic permalloy (Py, Ni 80Fe 20) caps on self-assembled spherical particles with diameters of 100, 330, and 800 nm are investigated, revealing the vortex ground state for individual caps and closely packed cap arrays. The magnetic coupling between vortices is substantially reduced due to the shape of the cap as apparent in a much weaker dependence of the magnetization reversal process on the separation distance. Interestingly, the remaining coupling is still sufficiently large to introduce chirality frustrated vortex states …


Out-Of-Surface Vortices In Spherical Shells, Volodymyr P. Kravchuk, Denis D. Sheka, Robert Streubel, Denys Makarov, Oliver G. Schmidt, Yuri Gaididei Apr 2012

Out-Of-Surface Vortices In Spherical Shells, Volodymyr P. Kravchuk, Denis D. Sheka, Robert Streubel, Denys Makarov, Oliver G. Schmidt, Yuri Gaididei

Robert Streubel Papers

The interplay of topological defects with curvature is studied for out-of-surface magnetic vortices in thin spherical nanoshells. In the case of an easy-surface Heisenberg magnet it is shown that the curvature of the underlying surface leads to a coupling between the localized out-of-surface component of the vortex with its delocalized in-surface structure, i.e., polarity-chirality coupling. © 2012 American Physical Society.