Condensed Matter Physics Commons^™

Field-Like- And Self-Spin-Orbit Torques In Magnetic Multilayer Films, Kyle Jeffrey Peterson

Electronic Theses and Dissertations

Spin-orbit torques (SOTs) have been realized as an energy efficient mechanism to manipulate and drive magnetization dynamics in magnetic multilayer films. Their damping-like and field-like components provide distinct pathways for controlling the magnetization, enabling switching, sustaining magneto-oscillations, and driving domain-wall motion with potential applications in nonvolatile memory, spin-based logic, and microwave signal generation. However, the accurate quantification and interpretation of these torques remains complicated by experimental sensitivity, the co-symmetry of the Oersted field and the effective field due to the field-like torque, and assumptions regarding the material layers from which the torques originate. The body of work set forth in …

Emergent Spin Fluctuation And Structural Metastability In Self-Intercalated Cr1+Xte2 Compounds, Clayton Conner, Ali Sarikhani, Theo Volz, Mathew Pollard, Mitchel Vaninger, Xiaoqing He, Steven Kelley, Jacob Cook, Avinash Sah, John Clark, Hunter Lucker, Cheng Zhang, Paul Miceli, Yew San Hor

Physics Faculty Research & Creative Works

Intercalated van der Waals (vdW) magnetic materials host unique magnetic properties due to the interplay of competing interlayer and intralayer exchange couplings, which depend on the intercalant concentration within the van der Waals gaps. Magnetic vdW compound chromium telluride, (Formula presented.), has demonstrated rich magnetic phases at various Cr concentrations, such as the coexistence of ferromagnetic and antiferromagnetic phases in (Formula presented.) (equivalently, (Formula presented.)). The compound is created by intercalating 0.25 Cr atom per unit cell within the van der Waals gaps of (Formula presented.). In this work, we report a notably increased Curie Temperature and an emergent in-plane …

First-Principles Investigation Of Quasi-One-Dimensional Van Der Waals Magnets For Advancing Low-Dimensional Spintronics, Alyssa Horne

Dissertations, Master's Theses and Master's Reports

Van der Waals (vdW) magnets have been of great interest for advancing low- dimensional spintronics. A notable example is the quasi-one-dimensional (Q1D) vdW CrSbSe₃, as it is composed of individual one-dimensional units that are held together by the vdW forces. Finding other Q1D vdW magnets that exhibit non-metallic behavior together with long range ferromagnetic ordering is critical in developing next generation spintronics. Here in, using first-principles density functional theory (DFT), we investigate the compositional effects on electronic and magnetic behavior of Cr_1–xMn_xSbSe₃ (x = 0, 0.5, 1). When 50% of Cr is replaced …

Self Spin-Orbit Torques, Ryan Greening

Electronic Theses and Dissertations

Spin–Orbit torques (SOTs) provide an energy-efficient pathway to control magnetization in nanoscale heterostructures. Recently, spin-orbit coupling within ferromagnets has been shown to generate self spin-orbit torques (SSOTs) on the magnetization itself. Previous work on self spin-orbit torques relies on thick ferromagnets with complicated film structures with chemical disorder or compositional gradients to generate inversion symmetry breaking. This dissertation advances experimental methodology and presents data on the quantification of self spin-orbit torques in magnetic thin films due to the spin-orbit coupling of standard 3d ferromagnets.

First, I develop an oblique-incidence magneto-optical Kerr effect (MOKE) technique that exploits a mirror-assisted double reflection …

Charge And Spin Transport In Nanowires With Spin-Orbit Coupling, Ryan Perrin

All Dissertations

Nanowires exhibiting Fermi-level pinning have strong radial electron confinement and thus can be modeled as a two-dimensional electron gas wrapped around the core. In III-V semiconductor structures, two forms of spin-orbit coupling are generated by breaking inversion symmetries in the crystal (Dresselhaus) and the overall structure of the nanowires (Rashba). The first goal of this thesis is to understand the single-particle energy spectrum in nanowires with variable cross sections and the quantum oscillations that can be driven in them by the application of a magnetic field parallel to the axis of the wire. To this end, the eigenfunctions and eigenvalues …

Ge/Sige Quantum Wells: Material For The Post-Moore Era, Troy Alexander Hutchins-Delgado

Optical Science and Engineering ETDs

This dissertation demonstrates high-quality germanium quantum wells on a 200 mm silicon wafer platform, enabling novel device possibilities. Partnering with a commercial silicon-germanium epitaxy supplier, we obtained shallow, undoped germanium quantum wells with high-crystalline quality, confirmed through x-ray diffraction, secondary ion mass spectroscopy, high-resolution scanning transmission electron microscopy, and energy dispersive x-ray spectroscopy. Hall bar devices fabricated on single quantum wells revealed that surface preparation can tune transport properties while maintaining peak mobilities around 10⁵ cm²V⁻¹s⁻¹. Manganese-germanide spintronic contacts were integrated via solid-state reaction, with contact quality assessed through Schottky diodes, transfer length …

Spin And Charge Transport In Metallic Ferrimagnets And Disordered Magnetic Oxides, Leopoldo A. Hernandez

Electronic Theses and Dissertations

Recent efforts have been exploring the use of thin film synthetic ferrimagnets and disordered magnetic oxides for applications in spintronic devices. Due to the antiferromagnetic exchange interaction, ferrimagnetic materials offer the ultrafast dynamics of the antiferromagnetic exchange, with a net magnetization that can be influenced externally. With two, or more, competing ferromagnet sublattices, interesting properties arise that depend on the final magnetic landscape after growth of the material and it’s inherent magnetic anisotropy energies. Properties such as magnetic compensation temperatures, and perpendicular magnetic anisotropy are attractive for applications in spintronic memory and logic devices, some already being implemented in MRAM …

Magnetic Properties Of Zgnrs With Nitrogen And Fluorine Adsorbates, A Computational Study, Justin Petit

Electronic Theses and Dissertations

Imposing dimensional restrictions on graphene sheets and adding impurities can give rise to carbon nanostructures with magnetic properties. In this work, zigzag graphene nanoribbons, zGNRs, with nitrogen and fluorine adatoms are investigated for magnetic properties of interest for spin devices. Geometry optimizations were done determining which position along a zGNR electrode that N and F would favorably attach to. Edge positions were determined as the most stable attachment site. M-cell zGNR electrodes (M = 1-3) edge-functionalized by N and F adatoms were investigated with respect to their band structures and spin densities in antiferromagnetic and ferromagnetic, AFM and FM, configurations. …

The Interplay Of Spin, Charge, And Heat: From Metal/Insulator Heterostructures To Perovskite Bilayers, Sam M. Bleser

Electronic Theses and Dissertations

In this dissertation begin with an investigation of non-local spin transport in an amorphous germanium (a-Ge) sample via the inverse spin Hall effect (ISHE). In that study we show that commonly used techniques such as differential conductance and delta mode of a paired Keithley 6221/2182a for non-local resistance measurements can lead to false indicators of spin transport. Next, we turn out attention to a thickness dependent study in thermally-evaporated chromium (Cr) thin films on a bulk polycrystalline yttrium-iron-garnet (YIG) substrate. This project analyzed the spin transport in the Cr films versus thickness via the longitudinal spin Seebeck effect (LSSE). This …

Thermal, Electrical, And Spin Transport: Encompassing Low-Damping Ferromagnets And Antiferromagnetic/Ferromagnetic Heterostructures, Matthew Ryan Natale

Electronic Theses and Dissertations

Continuing technological advancements bring forth escalating challenges in global energy consumption and subsequent power dissipation, posing significant economic and environmental concerns. In response to these difficulties, the fields of thermoelectrics, spintronics, and spincaloritronics emerge as contemporary solutions, each presenting unique advantages. Thermoelectric devices, based on the Seebeck effect, other a passive, carbon-free energy generating solution from waste heat. Although current thermoelectric technology encounters hurdles in achieving optimal efficiencies without intricate designs or complex materials engineering, recently research into low-damping metallic ferromagnetic thin films have provided a new method to enhance spin wave lifetimes, thus contributing to thermoelectric voltage improvements. As …

Towards Highly Sensitive Capacitance Measurements Of A Quantum Anomalous Hall Phase In Van Der Waal Heterostructures, Kayla Cerminara

UNLV Theses, Dissertations, Professional Papers, and Capstones

One of the pioneering achievements in condensed matter physics of the 20th century is the observation of the quantum Hall e↵ect (QHE) in which the Hall resistance in a two-dimensional (2D) sample takes on quantized values in the presence of a strong perpendicular magnetic field. The precise quantization of the hall resistance to one part in a billion has provided a practical, worldwide resistance standard. A long-standing goal has been to realize a similar state of matter but without the need of a strong quantizing magnetic field. The quantum anomalous Hall e↵ect (QAHE) is such a state that is predicted …

Spin-Dependent Electronic Transport In Noncollinear Antiferromagnetic Antiperovskites, Gautam Gurung

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Spin-dependent properties are the heart of spintronic devices. Spintronics exploits electron’s spin, in addition to charge, to process and store the information. Recently, antiferromagnetic (AFM) spintronics has emerged as a subfield of spintronics, where an AFM order parameter (the Néel vector) is exploited to control spin-dependent transport properties. Due to being robust against magnetic perturbations, producing no stray fields, and exhibiting ultrafast dynamics, antiferromagnets can serve as promising functional materials for spintronic applications.

Among antiferromagnets, high Néel temperature noncollinear antiperovskites ANMn₃ (A = Ga, Ni, Sn, and Pt) are interesting due to their magnetic group symmetry supporting non-trivial spin-dependent …

Developing Dynamical Probes Of Quantum Spin Liquids Inspired By Techniques From Spintronics, Joshua Aftergood

Dissertations, Theses, and Capstone Projects

We theoretically study low dimensional insulating spin systems using spin fluctuations as a probe of the spin dynamics. In some systems, low dimensionality in conjunction with other quantum fluctuation enhancing effects impedes spontaneous generation of long range magnetic ordering down to zero absolute temperature. In particular, we focus on exotic spin systems hosting mobile, fractionalized spin excitations above their ground state, and ultimately show that techniques already commonplace in spintronics can be utilized in the context of quantum magnetism to develop probes of exotic ground states.

We initially consider quantum spin chains (QSCs), and examine a system of two exchange-coupled …

Manipulation Of Spin Crossover Phenomenon In An Fe(Ii) Molecular Complex And Application To Molecular Spintronics, Guanhua Hao

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

Molecules with a large local magnetic moment have attracted considerable attention for application in spintronic devices. One candidate of a suitable device goes to the spin crossover molecule, where these 3d transition metal compounds are able to exhibit a robust spin state transition between distinct states. By proper design, the spintronic devices fabricated via spin crossover molecular thin films could achieve novel functionality while retaining flexibility and other traits based on its “organic” nature.

Controlling the spin state transition is a key factor of these possibilities. This thesis work investigates the manipulation of the spin state transition in [Fe{H …

Ligand Effects On Electronic, Magnetic, And Catalytic Properties Of Clusters And Cluster Assemblies, Dinesh Bista 9288522

Theses and Dissertations

Ligands commonly protect metallic clusters against reacting with outside reactants. However, ligands can also be used to control the redox properties enabling the formation of super donors/acceptors that can donate/accept multiple electrons. This thesis focuses on how the ligands can be used to control the electronic and magnetic features of clusters and ligand stabilized cluster-based assemblies, leading to nano pn junctions with directed transport, the possibility of light-harvesting, and catalysts for cross-coupling reactions. The thesis addresses three distinct classes of clusters and their applications. The first class of cluster “metal chalcogen clusters” is the central idea of the thesis focused …

Band Structure Topology And Spin Transport In Magnon Systems, Bo Li

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

As the spin excitation quanta in magnetic materials, the magnon is at the heart of the spintronics research because it plays a key role in magnetic dynamics, energy and spin transport, and even determining the ground state of magnetic systems. In this thesis, we will study the band-structure topology and transport properties of magnons in both collinear and noncollinear magnets. Inspired by the great success of topological insulators, exploring magnon topology can unveil the topological nature of bosonic particles and widen the zoo of topological materials. We propose a three-dimensional magnon topological insulator model protected by sublattice chiral symmetries, which …

Electron-Induced Massive Dynamics Of Magnetic Domain Walls, Hilary M. Hurst, Victor Galitski, Tero T. Heikkilä

Faculty Research, Scholarly, and Creative Activity

We study the dynamics of domain walls (DWs) in a metallic, ferromagnetic nanowire. We develop a Keldysh collective coordinate technique to describe the effect of conduction electrons on rigid magnetic structures. The effective Lagrangian and Langevin equations of motion for a DW are derived. The DW dynamics is described by two collective degrees of freedom: position and tilt-angle. The coupled Langevin equations therefore involve two correlated noise sources, leading to a generalized fluctuation-dissipation theorem (FDT). The DW response kernel due to electrons contains two parts: one related to dissipation via FDT, and another `inertial' part. We prove that the latter …

Electric Field Control Of Fixed Magnetic Skyrmions For Energy Efficient Nanomagnetic Memory, Dhritiman Bhattacharya

Theses and Dissertations

To meet the ever-growing demand of faster and smaller computers, increasing number of transistors are needed in the same chip area. Unfortunately, Silicon based transistors have almost reached their miniaturization limits mainly due to excessive heat generation. Nanomagnetic devices are one of the most promising alternatives of CMOS. In nanomagnetic devices, electron spin, instead of charge, is the information carrier. Hence, these devices are non-volatile: information can be stored in these devices without needing any external power which could enable computing architectures beyond traditional von-Neumann computing. Additionally, these devices are also expected to be more energy efficient than CMOS devices …

Theoretical Investigations Of The Electronic, Magnetic, And Thermoelectric Properties Of Transition-Metal Based Compounds, Haleoot Edaan Raad

Graduate Theses and Dissertations

The electronic, magnetic, and thermoelectric properties of transition-metal based compounds were investigated by using the density functional theory and Boltzmann transport formalism. It was found that the Co-based Heusler compounds and InSe monochalcogenide are among the materials that may be used for future thermoelectric devices. Furthermore, the investigation showed that the quaternary Heusler compounds, such as, CoFeYGe, where Y is Ti or Cr, are half-metallic ferromagnetic materials with full electron spin polarization. The lattice thermal conductivity (κL) was found to decrease for these alloys as the temperature increases. The present investigation indicated that the phonon optical modes have a major …

Space-Charge Limited Conduction In Epitaxial Chromia Films Grown On Elemental And Oxide-Based Metallic Substrates, C.-P. Kwan, Mike Street, Ather Mahmood, Will Echtenkamp, M. Randle, K. He, J. Nathawat, N. Arabchigavkani, B. Barut, S. Yin, R. Dixit, Uttam Singisetti, Christian Binek, J. P. Bird

Christian Binek Publications

We study temperature dependent (200 – 400 K) dielectric current leakage in high-quality, epitaxial chromia films, synthesized on various conductive substrates (Pd, Pt and V2O3). We find that trap-assisted space-charge limited conduction is the dominant source of electrical leakage in the films, and that the density and distribution of charge traps within them is strongly dependent upon the choice of the underlying substrate. Pd-based chromia is found to exhibit leakage consistent with the presence of deep, discrete traps, a characteristic that is related to the known properties of twinning defects in the material. The Pt- and V2O3-based films, in contrast, …

Dirac Nodal Line Metal For Topological Antiferromagnetic Spintronics, Ding-Fu Shao, Gautam Gurung, Shu-Hui Zhang, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

Topological antiferromagnetic (AFM) spintronics is an emerging field of research, which exploits the N´eel vector to control the topological electronic states and the associated spin-dependent transport properties. A recently discovered N´eel spin-orbit torque has been proposed to electrically manipulate Dirac band crossings in antiferromagnets; however, a reliable AFM material to realize these properties in practice is missing. In this Letter, we predict that room-temperature AFM metal MnPd₂ allows the electrical control of the Dirac nodal line by the N´eel spin-orbit torque. Based on first-principles density functional theory calculations, we show that reorientation of the N´eel vector leads to switching …

Straintronic Nanomagnetic Devices For Non-Boolean Computing, Md Ahsanul Abeed

Theses and Dissertations

Nanomagnetic devices have been projected as an alternative to transistor-based switching devices due to their non-volatility and potentially superior energy-efficiency. The energy efficiency is enhanced by the use of straintronics which involves the application of a voltage to a piezoelectric layer to generate a strain which is ultimately transferred to an elastically coupled magnetostrictive nanomaget, causing magnetization rotation. The low energy dissipation and non-volatility characteristics make straintronic nanomagnets very attractive for both Boolean and non-Boolean computing applications. There was relatively little research on straintronic switching in devices built with real nanomagnets that invariably have defects and imperfections, or their adaptation …

Persistent Spin Texture Enforced By Symmetry, Lingling Tao, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

Persistent spin texture (PST) is the property of some materials to maintain a uniform spin configuration in the momentum space. This property has been predicted to support an extraordinarily long spin lifetime of carriers promising for spintronics applications. Here, we predict that there exists a class of noncentrosymmetric bulk materials, where the PST is enforced by the nonsymmorphic space group symmetry of the crystal. Around certain high symmetry points in the Brillouin zone, the sublattice degrees of freedom impose a constraint on the effective spin–orbit field, which orientation remains independent of the momentum and thus maintains the PST. We illustrate …

Nv Center Detection Of Electric Fields And Low-Intensity Light, Nicholas Harmon, Michael Flatte

Faculty Works

Nitrogen vacancy (NV) center spins in diamond are attractive candidates for quantum information processing and sensitive, nanoscale magnetometers due to their long spin coherence times under ambient conditions [1]. The ground state of the NV spin is also sensitive to electric fields [2]. We present a theory of quantum detection using positive operator valued measurements (POVMs) wherein the presence of an electric field is determined by spin-dependent fluorescence of an NV center. The predicted sensitivity to small electric fields can also be used for photon detection. Photons incident upon a chromophore near the diamond interface may induce a charge polarization …

Novel Half-Metallic And Spin-Gapless Heusler Compounds, Yunlong Jin

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

This thesis is devoted to experimental studies of Heusler compounds CoFeCrAl, CoFeCrX (X = Si, Ge) and Mn₂PtSn. These Heusler alloys present an interesting class of ferromagnetic materials for spintronic applications since they are predicted to be spin gapless semiconductors and have half-metallic properties with 100 % spin polarization at the Fermi level. In this thesis, the structural, magnetic, spin-polarization and electron- transport properties of the fabricated alloys were studied. CoFeCrAl thin films deposited on MgO exhibit nearly perfect epitaxy and a high degree of L2₁ Heusler order. All considered types of chemical disorder destroy the spin-gapless …

Materials For Giant Spin Hall Effect Devices, Avyaya Jayanthinarasimham

Legacy Theses & Dissertations (2009 - 2024)

Studies presented in this thesis are an effort to control the growth of β W and explore

Temperature Dependence Of Dynamical Spin Injection In A Superconducting Niobium Thin Film, Tyler S. Townsend

Honors Undergraduate Theses

Spintronics is a research field that focuses on the manipulation of the quantum mechanical spin of charge carriers in solid state materials for future technological applications. Creating large spin currents with large relaxation times is sought after in the field of spintronics which may be aided by combining spintronics with superconductivity. This thesis provides a phenomological study of the effective change in ferromagnetic resonance linewidth, by dynamical spin injection into a permalloy-copper-niobium tri-layer in the superconducting state. The ferromagetic resonance linewidth was measured from 2-14 K. It was observed that there was a change in the behavior of the resonance …

Thermal Effects On Spin Currents In Non-Local Metallic Spin Valves, Alex Hojem

Electronic Theses and Dissertations

The study of non-local spin valves (NLSVs) has recently proven to be a fertile area for both applied and fundamental research in nanomagnetism due to the unique ability to separate charge currents and spin currents. NLSVs may also prove essential for a new class of high-density hard disk read heads due to their favorable scalability. Recent studies have shown thermal effects created by high current densities play a significant role in the response of NLSVs. These thermal effects also provide the opportunity to create a pure spin current from thermal gradients via a mechanism call the spin dependent Seebeck effect …

Understanding Electronic Structure And Transport Properties In Nanoscale Junctions, Kamal B. Dhungana

Dissertations, Master's Theses and Master's Reports - Open

Understanding the electronic structure and the transport properties of nanoscale materials are pivotal for designing future nano-scale electronic devices. Nanoscale materials could be individual or groups of molecules, nanotubes, semiconducting quantum dots, and biomolecules. Among these several alternatives, organic molecules are very promising and the field of molecular electronics has progressed significantly over the past few decades. Despite these progresses, it has not yet been possible to achieve atomic level control at the metal-molecule interface during a conductance measurement, which hinders the progress in this field. The lack of atomic level information of the interface also makes it much harder …

Interface States In Cofe2O4 Spin-Filter Tunnel Junctions, Pavel V. Lukashev, John D. Burton, Alexander Smogunov, Julian P. Velev, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

Spin-filter tunneling is a promising way to generate highly spin-polarized current, a key component for spintronics applications. In this paper we explore the tunneling conductance across the spin-filter material CoFe₂O₄ interfaced with Au electrodes, a geometry which provides nearly perfect lattice matching at the CoFe₂O₄/Au(001) interface. Using density functional theory calculations we demonstrate that interface states play a decisive role in controlling the transport spin polarization in this tunnel junction. For a realistic CoFe₂O₄ barrier thickness, we predict a tunneling spin polarization of about −60%. We show that this value …