Physics Commons^™

Micromagnetic Simulations Of Field-Driven Antiferromagnetically Coupled Skyrmions, Aidan D. Kirk

Physics and Astronomy Honors Papers

Competing magnetic interactions can stabilize smooth magnetization textures and can be characterized by a topological winding number. A specific spin configuration/texture, spatially localized within a two-dimensional plane, is commonly known as a skyrmion. On the classical level, the significance of skyrmions for condensed matter physics and their potential for applications, ranging from spintronic devices to qubits, has been intensely investigated in recent years. This thesis focuses on antiferromagnetically (AF) coupled Neel-type magnetic skyrmions, which are comprised of two skyrmions with opposite topological charges, yielding a net topological charge of 0. This configuration results in the cancellation of their respective Magnus …

Designing Enhanced Nonlinearity In Plasmonic Devices With Epsilon-Near-Zero Films, Kevin Tran Le

Electrical Engineering and Computer Science (MS) Theses

The growing demand for energy-efficient optical information processing motivates compact nonlinear photonic devices that can operate at low power. Silicon photonics is a mature platform for linear optical functions, but nonlinear operation remains challenging because of its weak Kerr response, two-photon absorption at telecommunication wavelengths, and limited compatibility with deeply subwavelength plasmonic confinement. This thesis computationally investigates epsilon-near-zero thin films integrated into plasmonic waveguide architectures as a route toward stronger light–matter interaction in compact nonlinear devices.

Two waveguide geometries are examined: a hybrid metal-insulator-metal plasmonic slab waveguide incorporating an ultrathin indium tin oxide epsilon-near-zero layer (5–50 nm), and a dielectric-loaded …

Beta Particles Impact On The Optical Properties Of Tio₂ Thin Films, Farah S. Dakhil, Hassan M.Jaber Al-Ta’Ii

Al-Bahir

TiO₂ is a semiconductor with a wide band gap and is utilized in various applications, including photovoltaics, solar cells, and photocatalysis. In this work, TiO₂ thin films were fabricated using the doctor blade technique and deposited onto glass substrates. The purpose of the study was to investigate how beta irradiation affected the optical properties of the TiO₂ films. The produced samples' absorbance and photon energy were the main subjects of the measurements. While the samples exposed to beta rays for 30, 60, and 90 minutes had direct band gaps of 3.87 eV, 3.75 eV, and 3.66 eV, …

Effect Of Niobium Dopant On Zno Thin Films Prepared Via The Sol–Gel Spin Coating Method, Kevin Alvin Eswar, Nur Fairuz Rostan, Maryam Mohamad, Rabiatuladawiyah Md Akhir, Rosfayanti Rasmidi, Muliyadi Guliling, Najwa Ezira Azhar, Irmaizatussyehdany Buniyamin, Mohd Firdaus Malek, Mohamad Rusop Mahmood, Husairi Fadzilah Suhaimi, Saifollah Abdullah

Makara Journal of Science

Thin films of zinc oxide (ZnO) and niobium (Nb)-doped ZnO were deposited on a glass substrate using the sol–gel spin coating method. Diethanolamine, isopropyl alcohol, and zinc acetate served as the stabilizers, solvent, and starting ma-terial, respectively. Niobium pentachloride was employed as the dopant source. Energy-dispersive X-ray analysis con-firmed Nb incorporation. Field emission scanning electron microscopy (FESEM), X-ray diffraction (XRD), and ultravio-let–visible spectroscopy (UV–Vis) analyses characterized the morphology, structure, and optics of the films, respective-ly. Both films, comprising nanoparticles, were visible in FESEM. Nb doping reduced the particle size from 44.2 nm to 35.8 nm. The XRD peaks at 31.23°, …

Cryogenic Hybrid Magnonic Circuits Based On Spalled Yig Thin Films, Jing Xu, Connor Horn, Yu Jiang, Amin Pishehvar, Xinhao Li, Daniel Rosenmann, Xu Han, Miguel Levy, Supratik Guha, Xufeng Zhang

Michigan Tech Publications

Yttrium iron garnet (YIG) magnonics has garnered significant research interest because of the unique properties of magnons (quasiparticles of collective spin excitation) for signal processing. In particular, hybrid systems based on YIG magnonics show great promise for quantum information science due to their broad frequency tunability and strong compatibility with other platforms. However, their broad applications have been severely constrained by substantial microwave loss in the gadolinium gallium garnet (GGG) substrate at cryogenic temperatures. In this study, we demonstrate that YIG thin films can be spalled from YIG/GGG samples. Our approach is validated by measuring hybrid devices comprising superconducting resonators …

The Use Of Two-Dimensional Detectors For Snapshot And High Accuracy Imaging Ellipsometry, Jeremy A. Vanderslice

Dissertations and Doctoral Documents, University of Nebraska-Lincoln, 2023–

Ellipsometry is a powerful and sensitive optical technique used to characterize thin film thickness and optical properties by measuring changes in the polarization state of light upon reflection or transmission. This dissertation investigates novel ellipsometry configurations that use two-dimensional detectors to enhance measurement speed, spatial resolution, or accuracy of ellipsometry measurements. The study involves the development of three different ellipsometry configurations, encompassing mechanical prototypes, mathematical models, and test measurements to evaluate each system.

Advisor: Jeffrey Shield

Modeling Permittivity Measurements Of Thin Film Materials Versus Film Thickness, Jr Dennison, Cameron Eggleston

Journal Articles

Measured permittivity of thin film polymeric samples were substantially less for thin samples, asymptotically approaching bulk values above ~500 μm. For ~25 μm samples the observed permittivities were as much as 50% less than for bulk measurements. This behavior has been studied for four common homogeneous polymeric materials for sample thickness in the range of ~10 μm to > 1000 μm. To quantify these observations, an empirical single-parameter model was developed to correct measured permittivity of thin samples based on an effective stray capacitance in series with the samples to compensate for effects attributed to instrumentation.

Effect Of Fabrication Parameters On The Ferroelectricity Of Hafnium Zirconium Oxide Films: A Statistical Study, Guillermo A. Salcedo, Ahmad E. Islam, Elizabeth Reichley, Michael Dietz, Christine M. Schubert Kabban, Kevin D. Leedy, Tyson C. Back, Weison Wang, Andrew Green, Timothy S. Wolfe, James M. Sattler

Faculty Publications

Ferroelectricity in hafnium zirconium oxide (Hf_1−xZr_xO₂) and the factors that impact it have been a popular research topic since its discovery in 2011. Although the general trends are known, the interactions between fabrication parameters and their effect on the ferroelectricity of Hf_1−xZr_xO₂ require further investigation. In this paper, we present a statistical study and a model that relates Zr concentration (x), film thickness (t_f), and annealing temperature (T_a) with the remanent polarization (P_r) in tungsten (W)-capped Hf_1−xZr_xO₂. …

Measurements Of Magnetic Field Penetration Of Materials For Superconducting Radiofrequency Cavities, Iresha Harshani Senevirathne

Physics Theses & Dissertations

Superconducting Radio Frequency (SRF) cavities used in particle accelerators are typically formed from or coated with superconducting materials. Currently high purity niobium is the material of choice for SRF cavities which have been optimized to operate near their theoretical field limits. This brings about the need for significant R&D efforts to develop next generation superconducting materials which could outperform Nb and keep up with the demands of new accelerator facilities. To achieve high quality factors and accelerating gradients, the cavity material should be able to remain in the superconducting Meissner state under high RF magnetic field without penetration of quantized …

The Influence Of The Substrate On The Functionality Of Spin Crossover Molecular Materials, Saeed Yazdani, Jared Phillips, Thilini K. Ekanayaka, Ruihua Cheng, Peter A. Dowben

Department of Physics and Astronomy: Faculty Publications

Spin crossover complexes are a route toward designing molecular devices with a facile readout due to the change in conductance that accompanies the change in spin state. Because substrate effects are important for any molecular device, there are increased efforts to characterize the influence of the substrate on the spin state transition. Several classes of spin crossover molecules deposited on different types of surface, including metallic and non-metallic substrates, are comprehensively reviewed here. While some non-metallic substrates like graphite seem to be promising from experimental measurements, theoretical and experimental studies indicate that 2D semiconductor surfaces will have minimum interaction with …

Novel As-S-Se Compositions Of Solution-Processed Chalcogenide Thin Films For Infrared Optics, Annabella Orsini

Physics and Astronomy Honors Papers

Chalcogenide glasses (ChGs) have a wide range of interdisciplinary applications. In industry, ChGs are used to vastly improve infrared sight abilities. There are, however, improvements that can be made to the films’ stability, cost, and flexibility. Our project seeks to produce thin films that have these improvements, with capabilities comparable or better than what is widely used in the field. Thin films created through solution-based processes have proven to be much more flexible in comparison to bulk glass versions. Other elements in Group 16, such as Sulfur and Selenium have shown across literature to be a cost-effective alternative to Tellurium …

Design And Fabrication Of A Low-Cost Dip Coating System For Depositing Homogeneous And Transparent Zno Thin Films, Asaad S. Yasir, Basheer M. Hussein, Ammar S. Hameed, Noor J. Ridha, Firas K. Mohamad Alosfur, Khawla J. Tahir, Rajaa A. Madlol

Al-Bahir

ZnO has a resistivity of up to 104 Ω cm-1 in most cases. Nevertheless, by increasing the layer thickness, the resistivity decreases as well, resulting in greater current transport. The dip coating system was developed to prepare the ultra-thin film, it relied on a controller, stepper motor and some low-cost recycled materials. Thin films of ZnO were successfully deposited on indium tin oxide substrates. The effects of the dipping cycles were investigated. Dipping processes were applied several times (1, 2, and 3) for the same concentrations (0.1) M to obtain homogeneous thin films. X-ray diffraction showed that the structure of …

Direct Current Magnetic Hall Probe Technique For Measurement Of Field Penetration In Thin Film Superconductors For Superconducting Radio Frequency Resonators, Iresha Harshani Senevirathne, Alex Gurevich, Jean Delayen

Physics Faculty Publications

Superconducting Radio Frequency (SRF) cavities used in particle accelerators are typically formed from or coated with superconducting materials. Currently, high purity niobium is the material of choice for SRF cavities that have been optimized to operate near their theoretical field limits. This brings about the need for significant R & D efforts to develop next generation superconducting materials that could outperform Nb and keep up with the demands of new accelerator facilities. To achieve high quality factors and accelerating gradients, the cavity material should be able to remain in the superconducting Meissner state under a high RF magnetic field without …

Some Optical Properties Of (Znte) Thin Films Prepared By Thermal Evaporation Technique On A Glass Substrate, Abdulla Saeed Ba-Sabiah, Mohamed Ali Seyam

Hadhramout University Journal of Natural & Applied Sciences

Thin films of Zinc telluride (ZnTe)were deposited by thermal evaporation technique on a glass substrate. The optical obtained data were analyzed using a numerical analysis program which showed that the transition mechanism involved indirectly allows transition since the best line dependence is obtained from a plot of 0.5 ( )  h versus photon energy ( ) h . The bandgap decreased from 1.15 to 0.96 eV as the substrate temperature varied from 410 to 510 K. Such behaviour is attributed to unsaturated defects, which are confirmed by XRD examinations. PACS:78.20.Ci, 71.30.+h, 72.90. +y

The Magnetic Field Penetration Measurement Of Thin Film And Multilayered Superconductors For Srf Cavities, Iresha Harshani Senevirathne, Jean Delayen

College of Sciences Posters

Radio Frequency (RF) Cavities are used in particle accelerators and they are typically formed from or coated with superconducting materials. High purity niobium is the material of choice for SRF cavities and niobium cavities operate at their theoretical field limits. SRF researchers have begun a significant R&D effort to develop alternative materials to continue to keep up with the demands of new accelerator facilities. To achieve high performance with high accelerating gradient, cavity material should have an ability to persist in superconducting state under high magnetic field without magnetic flux penetration through the cavity wall. Therefore, the magnetic field at …

Magnetic Properties Of Lsmo/Sto Thin Films: Magnetocaloric, Spin Dynamics And Magnetic Viscosity Investigations, Navid Mottaghi

Graduate Theses, Dissertations, and Problem Reports (ETD)

While other films are discussed, this dissertation will focus on detailed studies of the dc and ac bulk magnetometry in a characteristic 7.6 nm thin film of La_0.7Sr_0.3MnO₃ grown on SrTiO₃ (001). The dc bulk magnetometry measurements show that the sample is magnetically inhomogeneous. Temperature variation of magnetization (M vs. T) was measured in zero-field-cooled and field-cooled protocols to determine the blocking temperature T_B in different applied magnetic fields. The field variation of T_B is interpreted as the presence of embedded spin clusters of 1.4 nm. Moreover, the M vs. …

2 × 2 Anisotropic Transfer Matrix Approach For Optical Propagation In Uniaxial Transmission Filter Structures, Hammid Al-Ghezi, Rudra Gnawali, Partha P. Banerjee, Lirong Sun, Jonathan E. Slagle, Dean Evans

Student Publications

Multi-layered metamaterial structures show promise in a wide variety of optical applications such as superlenses, electromagnetic cloaking, tunable filters, sensors, and spatial light modulators. Optical transmission analysis of multilayer metallo-dielectric stacks with overall thickness less than the wavelength of light can be modeled using effective medium theory and the Berreman matrix method. For multilayer anisotropic stacks of arbitrary thickness, a rigorous 4 × 4 transfer matrix embodiment is typically used. In this work, a 2 × 2 anisotropic transfer matrix method is developed to analyze optical propagation through multilayer uniaxial stacks of arbitrary thicknesses. Optical transmission of a multilayer silver–zinc …

Artificial Neural Network Discovery Of A Switchable Metasurface Reflector, J. R. Thompson, J. A. Burrow, P. J. Shah, Jonathan E. Slagle, E. S. Harper, A. Van Rynbach, I. Agha, M. S. Mills

Student Publications

Optical materials engineered to dynamically and selectively manipulate electromagnetic waves are essential to the future of modern optical systems. In this paper, we simulate various metasurface configurations consisting of periodic 1D bars or 2D pillars made of the ternary phase change material Ge2Sb2Te5 (GST). Dynamic switching behavior in reflectance is exploited due to a drastic refractive index change between the crystalline and amorphous states of GST. Selectivity in the reflection and transmission spectra is manipulated by tailoring the geometrical parameters of the metasurface. Due to the immense number of possible metasurface configurations, we train deep neural networks capable of exploring …

Heterostructure Of 2d Materials: Hfs2/Hfo2/Si, Christopher J. Robledo

Graduate Theses/Dissertations

Heterostructures have been utilized in electronic devices for over 50 years with the proposal for the first heterostructure transistor in 1957. With the scaling of devices, it is necessary to create new heterostructures that will comply with Moore’s Law, as well as make devices faster and consume less power. Novel 2D materials, such as hafnium disulfide, have shown promise as an active channel layer, while hafnium dioxide is already proven to be a replacement of silicon dioxide for the gate insulating layer. However, fabrication techniques for wide-scale integration of these heterostructures have not yet been achieved. Also, the dielectric properties …

High-Temperature Optical Properties Of Indium Tin Oxide Thin-Films, Jiwoong Kim, Sujan Shrestha, Maryam Souri, John G. Connell, Sungkyun Park, Ambrose Seo

Physics and Astronomy Faculty Publications

Indium tin oxide (ITO) is one of the most widely used transparent conductors in optoelectronic device applications. We investigated the optical properties of ITO thin films at high temperatures up to 800 °C using spectroscopic ellipsometry. As temperature increases, amorphous ITO thin films undergo a phase transition at ~ 200 °C and develop polycrystalline phases with increased optical gap energies. The optical gap energies of both polycrystalline and epitaxial ITO thin films decrease with increasing temperature due to electron-phonon interactions. Depending on the background oxygen partial pressure, however, we observed that the optical gap energies exhibit reversible changes, implying that …

Fabrication Of Magnetocaloric La(Fe,Si)13 Thick Films, N H. Dung, N B. Doan, P De Rango, L Ranno, Karl G. Sandeman, N M. Dempsey

Publications and Research

La(Fe,Si)₁₃–based compounds are considered to be very promising magnetocaloric materials for magnetic refrigeration applications. Many studies have focused on this material family but only in bulk form. In this paper we report on the fabrication of thick films of La(Fe,Si)₁₃, both with and without post-hydriding. These films exhibit magnetic and structural properties comparable to bulk materials. We also observe that the ferromagnetic phase transition has a negative thermal hysteresis, a phenomenon not previously found in this material but which may have its origins in the availability of a strain energy reservoir, as in the cases of …

Fabrication Of Nanoscale Columnar Diodes By Glancing Angle Deposition, Jacob D. Weightman

Macalester Journal of Physics and Astronomy

Glancing angle deposition (GLAD) is a process in which thin films are deposited onto a substrate with obliquely incident vapor together with precisely controlled azimuthal substrate rotation. Ballistic shadowing effects due to the oblique incidence produce nanoscale structures, and a variety of feature shapes, including tilted columns, helices, and vertical columns can be achieved by varying the azimuthal rotation during the deposition process. Due to this control of morphology and the compatibility of the process with a wide variety of materials, GLAD films have found applications in a variety of fields including sensing, photonics, photovoltaics, and catalysis, where they are …

Investigation Of Mnxni1-Xo Thin Films Using Pulsed Laser Deposition, Md Ashif Anwar

Graduate Theses/Dissertations

The exchange bias (EB) effect, especially in nanomaterials, is highly promising for use in antiferromagnet-based spintronics applications. NiO is a well known antiferromagnetic material with a high Néel temperature (525K) and can exhibit ferromagnetism/ ferrimagnetism by adding other magnetic transition elements. Our previous work has shown that the antiferromagnetic characteristics of conventional NiO insulating nanostructured material can be altered to have substantial ferrimagnetic characteristics by doping NiO with Mn or Co. Pulsed laser deposition (PLD) was used to grow heterostructures comprised of a nanostructured thin NiO film deposited on the surface of a MgO (100) and Al₂O_{3 …}

Vanadyl Tetrabutyltetrakis(Dimethylamino) Phthalocyanine Based Thin Films For Organic Sensor And Transistor Applications, Nur Adilah Roslan

Student Works (2020-2029)

Organic electronic devices have been successively making progress into the commercial market to substitute conventional inorganic electronic devices. The endeavor to improve the performance displayed by organic semiconductor materials has urged a substantial number of researchers set to seek new materials. Metal phthalocyanines (MPcs), in particular, have garnered much attention due to their enticing benefits viz., cost efficiency, eco-friendly organic material, as well as thermal and chemical stability. Primarily, this study investigated the physical, morphological, optical, and electrical properties of vanadyl 3,10,17,24-tetra-tert-butyl-1,8,15,22-tetrakis(dimethylamino)-29H,31H-phthalocyanine or synonymously known as vanadyl tetrabutyltetrakis (dimethylamino) phthalocyanine (VTP). Subsequently, this study looked into the potential applications of …

Gamma-Ray Radiation Effects In Graphene-Based Transistors With H-Bn Nanometer Film Substrates, E. J. Cazalas, Michael R. Hogsed, S. R. Vangala, Michael R. Snure, John W. Mcclory

Faculty Publications

Radiation effects on graphene field effect transistors (GFETs) with hexagonal boron nitride (h-BN) thin film substrates are investigated using 60Co gamma-ray radiation. This study examines the radiation response using many samples with varying h-BN film thicknesses (1.6 and 20 nm thickness) and graphene channel lengths (5 and 10 μm). These samples were exposed to a total ionizing dose of approximately 1 Mrad(Si). I-V measurements were taken at fixed time intervals between irradiations and postirradiation. Dirac point voltage and current are extracted from the I-V measurements, as well as mobility, Dirac voltage hysteresis, and the total number of GFETs that remain …

Erratum: "Imaging The Three‐Dimensional Orientation And Rotational Mobility Of Fluorescent Emitters Using The Tri‐Spot Point Spread Function", Oumeng Zhang, Jin Lu, Tianben Ding, Matthew D. Lew

Electrical & Systems Engineering Publications and Presentations

In the original paper, a calibration error exists in the image-formation model used to analyze experimental images taken by our microscope, causing a bias in the orientation measurements in Figs. 2 and 3. The updated measurements are shown in Fig. E1. We have also updated the supplementary material for the original article to discuss the revised PSF model and estimation algorithms (supplementary material 2) and show the revised model and measurements (Figs. S1, S3, S7, S8, and S10–S13).

Voltage Controlled Magnetism In Cr2o3 Based All-Thin-Film Systems, Junlei Wang, Will Echtenkamp, Ather Mahmood, Christian Binek

Christian Binek Publications

Voltage-control of exchange biases through active selection of distinct domain states of the magnetoelectric and antiferromagnetic pinning layer is demonstrated for Cr2O3/CoPd heterostructures. Progress and obstacles towards an isothermal switching of exchange bias are discussed. An alternative approach avoiding exchange bias for voltage-controlled memory exploits boundary magnetization at the surface of Cr2O3 as voltage-controlled state variable. We demonstrate readout and switching of boundary magnetization in ultra-thin Cr2O3/Pt Hall bar devices where reversal of boundary magnetization is achieved via magnetoelectric annealing with simultaneously applied ±0.5 V and 400 mT electric and magnetic fields.

Space-Charge Limited Conduction In Epitaxial Chromia Films Grown On Elemental And Oxide-Based Metallic Substrates, C.-P. Kwan, Mike Street, Ather Mahmood, Will Echtenkamp, M. Randle, K. He, J. Nathawat, N. Arabchigavkani, B. Barut, S. Yin, R. Dixit, Uttam Singisetti, Christian Binek, J. P. Bird

Christian Binek Publications

We study temperature dependent (200 – 400 K) dielectric current leakage in high-quality, epitaxial chromia films, synthesized on various conductive substrates (Pd, Pt and V2O3). We find that trap-assisted space-charge limited conduction is the dominant source of electrical leakage in the films, and that the density and distribution of charge traps within them is strongly dependent upon the choice of the underlying substrate. Pd-based chromia is found to exhibit leakage consistent with the presence of deep, discrete traps, a characteristic that is related to the known properties of twinning defects in the material. The Pt- and V2O3-based films, in contrast, …

Studying The Interface Between Croconic Acid Thin Films And Substrates Using A Slow Positron Beam, Dean Peterson, Jiandang Liu, Jonas Etzweiler, Gabriel Sontoyo, Sara J. Callori, Kimberley R. Cousins, Timothy Usher, Renwu Zhang

Physics Faculty Publications

Croconic acid (CA) is the first organic ferroelectric with a spontaneous polarity in bulk samples comparable to its inorganic counterparts. As a natural extension of study, ultrathin CA films (∼nm scale) were investigated to reveal ferroelectric effects in films on different substrates for their fundamental and industrial significance. However, the void defect at the interface between the film and substrate is presumed to interfere with surface effects. In this work, a non-invasive technique, a slow positron beam, coupled with Doppler broadening energy spectroscopy (DBES), is applied to study the void defects within the interfacial layer between CA films and Si …

Imaging The Three-Dimensional Orientation And Rotational Mobility Of Fluorescent Emitters Using The Tri-Spot Point Spread Function, Oumeng Zhang, Jin Lu, Tianben Ding, Matthew D. Lew

Electrical & Systems Engineering Publications and Presentations

Fluorescence photons emitted by single molecules contain rich information regarding their rotational motions, but adapting single-molecule localization microscopy (SMLM) to measure their orientations and rotational mobilities with high precision remains a challenge. Inspired by dipole radiation patterns, we design and implement a Tri-spot point spread function (PSF) that simultaneously measures the three-dimensional orientation and the rotational mobility of dipole-like emitters across a large field of view. We show that the orientation measurements done using the Tri-spot PSF are sufficiently accurate to correct the anisotropy-based localization bias, from 30 nm to 7 nm, in SMLM. We further characterize the emission anisotropy …