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West Virginia University

Terahertz Time-Resolved Spectroscopy

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Full-Text Articles in Physics

Hot-Carrier Dynamics And Transport Mechanisms In Inas/Alassb Multiple Quantum Wells, Herath Pathiranage Janaka Chathuranga Piyathilaka Jan 2022

Hot-Carrier Dynamics And Transport Mechanisms In Inas/Alassb Multiple Quantum Wells, Herath Pathiranage Janaka Chathuranga Piyathilaka

Graduate Theses, Dissertations, and Problem Reports

Semiconductor photovoltaics convert light into electricity through the extraction of photo-excited charge carriers. Among the most important parameters for a photovoltaic cell are good optical absorption in the desired region of the electromagnetic spectrum, and sufficient excited-state lifetimes and mobilities of the photocarriers to allow for charge separation and extraction before recombination. For solar cell applications there are significant challenges to overcome to improve the efficiency of the light-to-electricity conversion. The cells are most commonly made of silicon, which has a nearly perfect bandgap for absorbing the most solar radiation, an indirect bandgap to give a long photocarrier lifetime and …


Equilibrium And Non-Equilibrium Ultrafast Carrier Transport And Dynamics In Chalcopyrite Semiconductors, Rishmali Thanuja Sooriyagoda Jan 2021

Equilibrium And Non-Equilibrium Ultrafast Carrier Transport And Dynamics In Chalcopyrite Semiconductors, Rishmali Thanuja Sooriyagoda

Graduate Theses, Dissertations, and Problem Reports

Chalcopyrite crystals in the II-IV-V2 family have received significant interest due to their high nonlinearity, composition-tunable bandgaps, wide transparency windows, and high damage threshold. These semiconductors have been explored for electromagnetic (EM) screening, spintronic and photovoltaic applications, making them good optical and optoelectronic materials. This thesis uses terahertz spectroscopy to understand optical, electronic, and vibrational dynamical processes in CdGeP2, ZnGeP2 and CdSiP2 chalcopyrite semiconductors.

We have employed Terahertz time-domain spectroscopy to investigate temperature-dependent ground-state properties of bulk chalcopyrite crystals that can be related to electronic transport and electron-lattice interactions. The complex spectra provide refraction and …