Physics Commons^™

Electronic Scattering From Co/Cu Interfaces: In-Situ Measurement And Comparison With Theory, W. E. Bailey, Shan X. Wang, Evgeny Y. Tsymbal

Evgeny Tsymbal Publications

The full thickness-dependent electrical conductivity of polycrystalline NiO/Co/Cu/Co spin-valve structures was measured in situ during ion-beam deposition and compared with calculations based on realistic band structure. We have found striking features in the experimental conductivity which are unexpected from widely used semiclassical free-electron models. Addition of ∼ 1 ML Co to a NiO/Co/Cu surface causes the net film conductance to decrease; the reverse case of Cu on NiO/Co shows a strong positive curvature of the thicknessdependent conductance, indicating a reduction of the conductivity in Cu near the interface with Co. Quantitative agreement is found between the experimental thickness-dependent film conductance …

Quantum-Well Resistivity For Perpendicular Transport In Magnetic Layered Systems, Evgeny Y. Tsymbal, David G. Pettifor

Evgeny Tsymbal Publications

We show that quantum-well states enhance the current-perpendicular-to-planes resistivity of a metal film compared to the resistivity in the bulk at film thicknesses comparable with the mean free path due to the reduced number of conducting channels within the potential-well structure. This makes the mean free path an important parameter, which must be taken into account for the accurate treatment of results on currentperpendicular- to-plane giant magnetoresistance, rather than ignored by applying the two-current series-resistor model.

Inception Of Snapover And Gas Induced Glow Discharges, J. T. Galofaro, B V. Vayner, D C. Ferguson, C D. Thomson, Jr Dennison, R E. Davies

Conference Proceedings

Ground based experiments of the snapover phenomenon were conducted in the large vertical simulation chamber at the Glenn Research Center (GRC) Plasma Interaction Facility (PIF). Two Penning sources provided both argon and xenon plasmas for the experiments. The sources were used to simulate a variety of ionospheric densities pertaining to a spacecraft in a Low Earth Orbital (LEO) environment^1–4. Secondary electron emission is believed responsible for dielectric surface charging, and all subsequent snapover phenomena observed^2,5. Voltage sweeps of conductor potentials versus collected current were recorded in order to examine the specific charging history of each sample. …

Inception Of Snapover And Gas Induced Glow Discharges, J. T. Galofaro, B V. Vayner, W A. Degroot, D C. Ferguson, C D. Thomson, Jr Dennison, R E. Davies

Conference Proceedings

Ground based experiments of the snapover phenomenon were conducted in the large vertical simulation chamber at the Glenn Research Center (GRC) Plasma Interaction Facility (PIF). Two Penning sources provided both argon and xenon plasmas for the experiments. The sources were used to simulate a variety of ionospheric densities pertaining to a spacecraft in a Low Earth Orbital (LEO) environment^1-4. Secondary electron emission is believed responsible for dielectric surface charging, and all subsequent snapover phenomena observed^2,5. Voltage sweeps of conductor potentials versus collected current were recorded in order to examine the specific charging history of each sample. …

Evolution Of Secondary Electron Emission Characteristics Of Spacecraft Surfaces: Importance To Spacecraft Charging, R. E. Davies, Jr Dennison

Journal Articles

Secondary electron emission (SEE) plays a key role in spacecraft charging [Garrett, 1981; Frooninckx and Sojka, 1992] . As a result, spacecraft charging codes require knowledge of the SEE characteristics of various materials in order to predict vehicle potentials in various orbital environments [Katz, et. al., 1986]. Because SEE is a surface phenomenon, occurring in the first few atomic layers of a material, the SEE characteristics of a given surface are extremely sensitive to changes in surface condition—e.g., the addition or removal of surface contaminants, or changes in surface morphology. That spacecraft surfaces …

Digital Holography And Application In Laser Metrology, Thian Khok Yong

Student Works (2000-2009)

A digital holography system has been developed in this study. The object is recorded and the hologram is stored electronically with a charged-couple-device (CCD) camera without any focusing optics. The reconstruction of the digitally sampled hologram is done numerically with a computer. The algorithm and software for numerical reconstruction, which consists in a numerical realization of the Fresnel-Kirchhoff diffraction integral, are designed and implemented with two­dimensional and three-dimensional simple objects. The characteristics of the system have been studied. For the CCD camera (768x494 pixels) been used with spatial resolution of about I 00 lines/mm, the angle between reference and object …

Charge Dynamics In The Half-Metallic Ferromagnet Cro2, E. J. Singley, Christopher P. Weber, D. N. Basov, A. Barry, J. M. D. Coey

Physics

Infrared spectroscopy is used to investigate the electronic structure and charge carrier relaxation in crystalline films of CrO₂ which is the simplest of all half-metallic ferromagnets. Chromium dioxide is a bad metal at room temperature but it has a remarkably low residual resistivity (<5 >μΩ cm) despite the small spectral weight associated with free carrier absorption. The infrared measurements show that low residual resistivity is due to the collapse of the scattering rate at ω<2000 >cm^-1. The blocking of the relaxation channels at low v and T can be attributed to the unique electronic structure of a …

Time-Resolved Reflection High-Energy Electron Diffraction Study Of The Ge(111)-C(2×8)-(1×1) Phase Transition, Xinglin Zeng, Bo Lin, Ibrahim El-Kholy, Hani E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The dynamics of the Ge(111)-c(2×8)-(1×1) phase transition is investigated by 100-ps time-resolved reflection high-energy electron diffraction. A laser pulse heats the surface while a synchronized electron pulse is used to obtain the surface diffraction pattern. Slow heating shows that the adatoms in Ge(111)-c(2×8) start to disorder at ∼510 K and are converted to a disordered adatom arrangement at 573 K. For heating with 100-ps laser pulses, the Ge(111)-c(2×8) reconstructed adatom arrangement starts to disorder at 584±16K, well above the onset temperature of ∼510 K for the disordering of Ge(111)-c(2×8) observed for slow …

Mössbauer Effect Determination Of Relative Recoilless Fractions For Iron Oxides, Sei J. Oh, Desmond C. Cook

Physics Faculty Publications

The relative recoilless fraction (F-value) of each of six iron oxides, defined as the ratio of the recoil-free fractions of two different materials, was experimentally determined relative to hematite at 300 K and 77 K by Mössbauer spectroscopy. Using the relative recoil-free fractions compared to that of hematite, the relative recoilless fractions between all pairs of the seven iron oxides were determined. The F-values can allow conversion of Mössbauer subspectral areas to the relative atomic, molecular, or weight fractions of each iron oxide present in a mixed oxide phase sample.

Saturation In “Nonmagnetic” Stainless Steel, Christopher P. Weber, J. Fajans

Physics

Scientific equipment often uses “nonmagnetic” stainless steel, relying on the steel’s nonmagnetic behavior to leave external magnetic fields unaltered. However, stainless steel’s permeability can rise significantly when it is welded or machined, possibly perturbing an external field. Such perturbations will diminish well above the stainless steel’s saturation point. The authors measured the permeability of both welded and machined 304 stainless steel as a function of an external magnetic field, and found that both saturate at fields of approximately 0.25 T.

Low Energy Electron Gun Power Control Unit, Chad Fish, Jr Dennison

Senior Theses and Projects

Near-Earth orbiting spacecraft are subject to a variety of physical environmental elements. Of these, natural space plasma and solar radiation produce spacecraft charging. Spacecraft charging consists of surface (external) and deep (internal) dielectric charging.

Natural space plasma is composed of electrons and positively charged atoms called ions. The plasma is generated by energy from solar radiation and high energy particles emitted by geomagnetic storms. The electrons produce a negative current and the ions produce a positive current. Positive photoelectron currents produced by solar radiation of spacecraft surfaces also add to the electrical fluxesⁱ.

As spacecraft move through the …

Two-Dimensional Ferroelectric Films, Alexander V. Bune, Vladimir M. Fridkin, Stephen Ducharme, Lev M. Blinov, Serguei P. Palto, Alexander V. Sorokin, S. G. Yudin, A. Zlatkin

Stephen Ducharme Publications

Ultrathin crystalline films offer the possibility of exploring phase transitions in the crossover region between two and three dimensions. Second- order ferromagnetic phase transitions have been observed in monolayer magnetic films [1,2], where surface anisotropy energy stabilizes the two-dimensional ferromagnetic state at finite temperature [3]. Similarly, a number of magnetic materials have magnetic surface layers that show a second-order ferromagnetic–paramagnetic phase transition with an increased Curie temperature [4]. Ferroelectricity is in many ways analogous to ferromagnetism, and bulk-like ferroelectricity and finite-size modifications of it have been seen in nanocrystals as small as 250 Å in diameter [5], in perovskite films …

Suppression Of Switchable Polarization In Kdp By Ionizing Radiation, Timothy D. Usher

Physics Faculty Publications

Switching curves were obtained from KH₂PO₄ single crystals exposed to x-ray radiation for various time intervals, up to 8 h. The applied electric field was varied between 370 and 740 V/cm, as well. The temperature was held constant at 99 K. The switching curves were fit to a three-parameter nucleation and growth model based on the original works by Johnson and Mehl, and independently by Avrami. The two dynamic parameters, characteristic time t_c, and effective domain wall dimensionality n, produced values consistent with unirradiated studies, however, they did not show any clear dependancy on …

Physisorbed Co On Ionic Crystals: An Extended Beg Spin-Lattice Model Of Adsorbed Dipolar Molecules, T. E. Burns, Jr Dennison

Journal Articles

The 2D dielectric phases and phase transitions of adsorbed dipolar molecules are studied using a dilute spin-one Ising model. The spin-one formulation assigns a spin S_i = ±1 to a (up/down) dipole occupying a lattice site i adsorbed perpendicular to the substrate surface and Si = 0 to unoccupied sites. We relate the mean field expression for the spin-model interaction energy to a more detailed microscopic model involving dipolar, quadrupolar and dispersive interactions beyond nearest neighbor. Analytic solutions in the mean field approximation are discussed for dipole-orientation order-disorder transitions and ferroelectric-to-antiferroelectric transitions as a function of temperature and …

Surface Morphology Of Laser-Superheated Pb(111) And Pb(100), Z. H. Zhang, Bo Lin, X. L. Zeng, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The surface step density on the vicinal Pb(111) and the surface vacancy density on Pb(100) after laser superheating and melting are investigated using reflection high-energy electron diffraction. With ∼100-ps laser pulses, Pb(111) surface superheating does not significantly change the density of the steps and step-edge roughness. However, after laser surface melting, the average terrace width and the string length at the step edge become as large as those at room temperature. The average terrace width at 573 K changes from 38±15 to 64±19 Å after laser surface melting, while the average string length at the step edge changes from 90±14 …

Temperature Dependence Of Step Density On Vicinal Pb(111), Z. H. Zhang, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The temperature dependence of step density on the vicinal Pb(111) surface is investigated using reflection high-energy electron diffraction. When the temperature is increased from 323 to 590 K. the average terrace width and the average string length at the step edge decrease from 85±25 to 37±16 Å and from 220±33 to 25±8 Å, respectively. Thermal step collapse on the Pb(111) surface near its bulk melting temperature is not observed. Above 530±7 K, the change in the string length at the step edge with temperature becomes small, and the intensity of the (00) beam is significantly decreased. We conclude that partial …

Femtosecond Photoemission Study Of Ultrafast Electron Dynamics In Single-Crystal Au(111) Films, J. Cao, Y. Gao, H. E. Elsayed-Ali, R. J. D. Miller, D. A. Mantell

Electrical & Computer Engineering Faculty Publications

The energy-dependent relaxation of photoexcited electrons has been measured by time-resolved two-photon photoemission spectroscopy on single-crystal Au(111) films with thickness ranging from 150 to 3000 Å. It is found that the energy-dependent relaxation does not show any significant thickness dependence, which indicates that electron transport is a much slower dynamical process in the near-surface region than expected from bulk properties. Furthermore, lifetimes of the photoexcited electrons can be fitted well by the Fermi-liquid theory with a scaling factor plus an effective upper lifetime. This observation enables separation of electron-electron scattering, and to a lesser extent electron-phonon scattering, processes from electron-transport …

Photoluminescence Properties Of Silicon Quantum-Well Layers, Peter N. Saeta, A. C. Gallagher

All HMC Faculty Publications and Research

Nanometer-scale crystal silicon films surrounded by SiO₂ were prepared by oxidizing silicon-on-insulator substrates prepared from SIMOX (separation by implantation of oxygen) and crystallized hydrogenated amorphous silicon films. Average silicon layer thickness was determined from reflection spectra. When sufficiently thin (<2 >nm), all layers emitted red photoluminescence under blue and UV cw excitation, with a spectrum that did not depend on the mean layer thickness. The spectrum was roughly Gaussian with a peak energy of 1.65 eV, which is lower than for most porous silicon spectra. The time scale for the luminescence decay was ~35 μs at room temperature and …

Reflection High-Energy Electron-Diffraction Study Of Melting And Solidification Of Pb On Graphite, Z. H. Zhang, P. Kulatunga, H. E. Elsayed-Ali

Electrical & Computer Engineering Faculty Publications

The melting and solidification of Pb thin films on pyrolytic graphite are investigated in situ by reflection high-energy electron diffraction. Thin films with thicknesses of 4-150 monolayers are investigated. The surface morphology of the thin films were studied by scanning electron microscopy. Superheating of the Pb thin films by 4±2 to 12±2 K is observed from diffraction intensity measurements. Upon cooling the substrate, the Pb on graphite is seen to supercool by ∼69±4 K.

Femtosecond Photoemission Study Of Ultrafast Electron Dynamics On Cu(100), J. Cao, Y. Gao, R. J. D. Miller, Hani E. Elsayed-Ali, D. A. Mantell

Electrical & Computer Engineering Faculty Publications

The energy dependence of the relaxation of photoexcited electrons in copper was measured using femtosecond time-resolved photoemission spectroscopy to within 0.3 eV above the Fermi level. By performing lifetime measurements under different surface conditions, several surface dynamical processes were investigated. In particular, an anomalous long lifetime feature, which cannot be explained with Fermi-liquid theory, was observed in the lifetime-energy curve. This feature was found originating from the photoexcitation of the strongly localized Cu 3d electrons. ©1997 American Physical Society

Voltage Responses To Optical Pulses Of Unbiased Normal And Superconducting Samples, D. Van Vechten, K. S. Wood, G. G. Fritz, J. S. Horitz, G. M. Daly, J. B. Thrasher, D. M. Photiadis, J. Ding, J. F. Pinto, M. G. Blamire, G. Burnell, A. L. Gyulamiryan, V. H. Vartanyan, R. B. Akopyan, Armen Gulian

Mathematics, Physics, and Computer Science Faculty Articles and Research

The direct transformation of the energy of an incident high-energy photon into a measurable potential difference within an absorbing metal is investigated. Experimental evidence is presented that the effect arises from the inherent energy dependence of the electronic density of states, rather than from a simple temperature excursion. The similarities between the results on Al and YBa₂Cu₃O₇ samples indicate that the effect is universal in nature. We assert it may be used as the basis of a fast, energy resolving, individual photon detector for the ultraviolet radiation and x-rays.

Raman Spectroscopy Of Carbon Materials, Jr Dennison, Mark Holtz, Greg Swain

Journal Articles

Use of carbon materials is no longer limited to diamond jewelry or graphite pencils and lubricants. The last decade has witnessed an explosion of technological applications driven by the development of fabrication methods and the discovery of several new classes of pure carbon. Structural diversity exhibited by the carbon atoms, from local chemical order to long-range crystalline order, is key to understanding their physical and chemical properties and in future materials development. This article summarizes the use of Raman spectroscopy as a principal tool to investigate the vibrational dynamics of carbon materials and to provide indirect structural characterization of their …

Application Of (E,2e) Spectroscopy To The Electronic Structure Of Valence Electrons In Crystalline And Amorphous Solids, Jr Dennison, A. L. Ritter

Journal Articles

This review presents theoretical and experimental aspects of (e,2e) spectroscopy specific to the study of crystalline and amorphous solids. The cross section for (e,2e) scattering is proportional to the spectral momentum density of the ejected electron under certain approximations. The theoretical framework for interpreting (e,2e) measurements is summarized here and general properties of the spectral momentum density of solids are discussed. Different designs of the (e,2e) spectrometer are described and sample preparation techniques are briefly reviewed. A summary of recent (e,2e) experiments on the electronic structure of valence electrons in graphite, ion sputtered and evaporated amorphous carbon, and aluminum-aluminum oxide …

Mechanical Alloying Of Nitrogen Into Iron Powders, J. Rawers, D. Govier, D. C. Cook

Physics Faculty Publications

Mechanical alloying of nitrogen into bcc-fe powder is a very effective and efficient means of obtaining very high concentration of nitrogen in micron-size iron particles. Mechanical alloying increases the concentration of nitrogen in the iron powder far in excess of the bcc-Fe lattice low nitrogen solubility, however most of the infused nitrogen resides on the nano-size grain boundaries and in nano-size bct-fe that forms during mechanical alloying.

Measurement Of Nuclear Quadrupole Interactions Using Mössbauer Spectroscopy, Desmond C. Cook

Physics Faculty Publications

Mössbauer spectroscopy is a useful probe for investigating nuclear quadrupole interactions. It enables the magnitude, sign and asymmetry of the electric quadrupole coupling constant to be determined. It is especially important for its ability to measure these parameters for excited nuclear states. The Mössbauer effect is used to measure excited state quadrupole moments in materials whose electric field gradient (EFG) is known. More commonly however, it is used to determine the EFG from which atomic bonding and electronic structure are determined. The technique also allows temperature dependent orientation of sublattice magnetization to be measured using the direction of the electric …

Nuclear Forward-Scattering Of Synchrotron Radiation From Krypton: First Observation And Application To The Study Of Lattice Dynamics In Near-Monolayer Krypton-On-Graphite, David Eric Johnson

Physics Theses & Dissertations

Since 1985 nuclear-resonant scattering, and in particular nuclear forward-scattering, of synchrotron radiation has been observed in a select few Mossbauer isotopes including: ⁵⁷Fe, ¹¹⁹Sn, ¹⁶⁹Tm. For the first time, nuclear forward-scattering from the 9.4 keV Mossbauer level in ⁸³Kr has been observed. A large resonance effect, comparable to that in ⁵⁷Fe, has been observed in a variety of systems containing Kr including bulk crystals and physisorbed Kr-on-exfoliated graphite. Previous nuclear-resonant scattering experiments using synchrotron radiation have consisted of demonstration experiments. Nuclear forward-scattering from Kr has been applied to study the lattice dynamics of near-monolayer Kr-on-graphite …

Visible Luminescence From Single Crystal‐Silicon Quantum Wells, Peter N. Saeta, A. C. Gallagher

All HMC Faculty Publications and Research

Single crystal‐silicon quantum wells with SiO₂ barriers have been grown from SIMOX silicon‐on‐insulator substrates. Photoluminescence in the red and near‐infrared is observed for average well width <8 >nm, with peak signal for 2‐nm average width. The luminescence spectrum is independent of well width for SiO₂ barriers, but shifts 0.3 eV to higher energy upon removal of the upper oxide layer with HF. Both results suggest the importance of radiation from surface states.

Characterization Of Piezoceramic Crosses With Large Range Scanning Capability And Applications For Low Temperature Scanning Tunneling Microscopy, J. A. Helfrich, Shireen Adenwalla, J. B. Ketterson, G. A. Zhitomirsky

Shireen Adenwalla Papers

We have developed a large amplitude piezoceramic scanner which should have numerous applications. Scanning tunneling microscopy (STM) and other scanning probe microscopies predominantly use piezoceramics for the scanning elements. Similarly adaptive optics, high resolution lithography, and micromanipulators are other examples of research which regularly utilize piezoceramic scanners. We present a new geometry for a piezoceramic scanner which allows for both high resolution (~nanometers) and large amplitude (~400 µm) displacements. The cross-shaped geometry makes it possible to produce extremely long pieces with very high tolerances. We have shown its effectiveness by using it as the major component of a low temperature …

Scanning-Tunneling-Microscopy Study Of Pb On Si(111), D. Tang, H. E. Elsayed-Ali, J. Wendelken, J. Xu

Electrical & Computer Engineering Faculty Publications

Scanning-tunneling microscopy has been used to study temperature and coverage dependence of the structure of lead on the Si(111)-7×7 surface. For low Pb coverage, the Pb atoms favored the faulted sites. The ratio between the number of Pb atoms on faulted to unfaulted sites increased after sample annealing. An energy difference of 0.05 eV associated with a Pb atom on these two sites is estimated. The mobility of Pb atoms on Si(111) was observed at a temperature as low as 260°C for a coverage of 0.1 and 1 ML. © 1995 The American Physical Society.

Compensation And Characterization Of Gallium Arsenide, Randy A. Roush

Electrical & Computer Engineering Theses & Dissertations

The properties of transition metals in gallium arsenide have been previously investigated extensively with respect to activation energies, but little effort has been made to correlate processing parameters with electronic characteristics. Diffusion of copper in gallium arsenide is of technological importance due to the development of GaAs:Cu bistable photoconductive devices. Several techniques are demonstrated in this work to develop and characterize compensated gallium arsenide wafers. The material is created by the thermal diffusion of copper into silicon-doped GaAs. Transition metals generally form deep and shallow acceptors in GaAs, and therefore compensation is possible by material processing such that the shallow …